FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Kim, J Yoo, G Lee, H Lim, J Kim, K Kim, CW Park, MS Yang, JW AF Kim, Jungmin Yoo, Gursong Lee, Hansol Lim, Juntaek Kim, Kyochan Kim, Chul Woong Park, Min S. Yang, Ji-Won TI Methods of downstream processing for the production of biodiesel from microalgae SO BIOTECHNOLOGY ADVANCES LA English DT Review DE Biodiesel; Downstream process; Extraction; Harvest; Microalgae; Transesterification ID ALGA BOTRYOCOCCUS-BRAUNII; SYNECHOCYSTIS PCC 6803; CHLORELLA-VULGARIS; LIPID EXTRACTION; CELL-DISRUPTION; VEGETABLE-OILS; SUPERCRITICAL METHANOL; ULTRASONIC CAVITATION; MAGNETIC SEPARATION; ASSISTED EXTRACTION AB Despite receiving increasing attention during the last few decades, the production of microalgal biofuels is not yet sufficiently cost-effective to compete with that of petroleum-based conventional fuels. Among the steps required for the production of microalgal biofuels, the harvest of the microalgal biomass and the extraction of lipids from microalgae are two of the most expensive. In this review article, we surveyed a substantial amount of previous work in microalgal harvesting and lipid extraction to highlight recent progress in these areas. We also discuss new developments in the biodiesel conversion technology due to the importance of the connectivity of this step with the lipid extraction process. Furthermore, we propose possible future directions for technological or process improvements that will directly affect the final production costs of microalgal biomass-based biofuels. (C) 2013 Elsevier Inc. All rights reserved. C1 [Kim, Jungmin; Yoo, Gursong; Lee, Hansol; Lim, Juntaek; Kim, Kyochan; Kim, Chul Woong; Park, Min S.; Yang, Ji-Won] Korea Adv Inst Sci & Technol, Dept Chem & Biomol Engn, Taejon 305701, South Korea. [Lim, Juntaek; Park, Min S.; Yang, Ji-Won] Korea Adv Inst Sci & Technol, Adv Biomass R&D Ctr, Taejon 305701, South Korea. [Park, Min S.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. RP Park, MS (reprint author), Korea Adv Inst Sci & Technol, Adv Biomass R&D Ctr, 291 Daehak Ro, Taejon 305701, South Korea. EM minsungpark0@kaist.ac.kr; jwyang@kaist.ac.kr RI Yang, Ji-Won/C-1933-2011; OI Kim, Jungmin/0000-0002-8580-8134 FU Advanced Biomass R&D Center (ABC) of Global Frontier Project; Ministry of Education, Science and Technology [ABC-2011-K000908]; National Energy Technology Innovation of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant; Korea government Ministry of Knowledge Economy [2012 T100201665]; Brain Pool Program; Korean Federation of Science and Technology Societies Grant by Korea Government (MEST, Basic Research Promotion Fund) FX This work was supported by the Advanced Biomass R&D Center (ABC) of Global Frontier Project funded by the Ministry of Education, Science and Technology (ABC-2011-K000908). This work was also supported by the National Energy Technology Innovation of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by the Korea government Ministry of Knowledge Economy (No. 2012 T100201665). MSP was supported by the Brain Pool Program funded by the Korean Federation of Science and Technology Societies Grant by Korea Government (MEST, Basic Research Promotion Fund). NR 116 TC 106 Z9 108 U1 12 U2 371 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0734-9750 J9 BIOTECHNOL ADV JI Biotechnol. Adv. PD NOV 1 PY 2013 VL 31 IS 6 SI SI BP 862 EP 876 DI 10.1016/j.biotechadv.2013.04.006 PG 15 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA 217IH UT WOS:000324352700012 PM 23632376 ER PT J AU Hansen, N Merchant, SS Harper, MR Green, WH AF Hansen, Nils Merchant, Shamel S. Harper, Michael R. Green, William H. TI The predictive capability of an automatically generated combustion chemistry mechanism: Chemical structures of premixed iso-butanol flames SO COMBUSTION AND FLAME LA English DT Article DE iso-Butanol; Chemical mechanism; Mass spectrometry; Premixed flame ID PHOTOIONIZATION MASS-SPECTROMETRY; JET-STIRRED REACTOR; MASTER EQUATION METHODS; LOW-PRESSURE FLAMES; N-BUTANOL; SHOCK-TUBE; CROSS-SECTIONS; GAS-PHASE; OXIDATION; KINETICS AB The chemical compositions of four low-pressure premixed flames of iso-butanol are investigated with an emphasis on assessing the predictive capabilities of an automatically generated combustion chemistry model. This kinetic model had been extensively tested against earlier experimental data [S.S. Merchant, E.F. Zanoelo, R.L. Speth, M.R. Harper, K.M. Van Geem, W.H. Green, Combust. Flame (2013), http://dx.doLorg/10.1016/j.combustflame.2013.04.023.] and also shows impressive capabilities for predicting the new flame data presented here. The new set of data consists of isomer-resolved mole fraction profiles for more than 40 species in each of the four flames and provides a comprehensive benchmark for testing of any combustion chemistry model for iso-butanol. Isomer-specificity is achieved by analyzing flames, which are burner-stabilized at equivalence ratios of phi = 1.0-1.5 and at pressures between 15 and 30 Torr, with molecular-beam mass spectrometry and single-photon ionization by tunable vacuum-ultraviolet synchrotron radiation. Predictions of the C2H4O, C3H6O, and C4H8O enol-aldehyde-ketone isomers are improved compared to the earlier work by Hansen et al. [N. Hansen, M. R. Harper, W. H. Green, Phys. Chem. Chem. Phys. 13 (2011) 20262-20274] on similar n-butanol flames. A reaction path analysis identifies prominent fuel-consumption and oxidation sequences. Almost all of the species mole fraction data reported here are predicted within the measurement uncertainties of a factor of two to three. Some significant differences with previous published models are highlighted. (C) 2013 The Combustion Institute. Published by Elsevier Inc. All rights reserved. C1 [Hansen, Nils] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Merchant, Shamel S.; Harper, Michael R.; Green, William H.] MIT, Dept Chem Engn, Cambridge, MA 02139 USA. RP Hansen, N (reprint author), Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. EM nhansen@sandia.gov; whgreen@mit.edu RI Green, William/C-9684-2012; Hansen, Nils/G-3572-2012 OI Green, William/0000-0003-2603-9694; FU U.S. Department of Energy, Office of Basic Energy Sciences under the Energy Frontier Research Center for Combustion Science [DE-SC0001198]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Nuclear Security Administration [DE-AC04-94-AL85000] FX The work is supported by the U.S. Department of Energy, Office of Basic Energy Sciences under the Energy Frontier Research Center for Combustion Science (Grant No. DE-SC0001198). The authors thank P. Osswald, K. Kohse-Hoinghaus, and F. Qi for sharing their temperature and speciation data. SSM thanks Dr. Judit Zador and Dr. J. A. Miller for sharing their recent calculations on the propene + OH potential energy surface. The measurements are performed within the "Flame Team" collaboration at the Advanced Light Source (ALS), Lawrence Berkeley National Laboratory, Berkeley, USA, and we thank the students and postdocs for the help with the data acquisition. The experiments have profited from the expert technical assistance of Paul Fugazzi. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration under Contract DE-AC04-94-AL85000. NR 65 TC 21 Z9 21 U1 5 U2 67 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0010-2180 J9 COMBUST FLAME JI Combust. Flame PD NOV PY 2013 VL 160 IS 11 BP 2343 EP 2351 DI 10.1016/j.combustflame.2013.05.013 PG 9 WC Thermodynamics; Energy & Fuels; Engineering, Multidisciplinary; Engineering, Chemical; Engineering, Mechanical SC Thermodynamics; Energy & Fuels; Engineering GA 212TT UT WOS:000324006400005 ER PT J AU Chatakonda, O Hawkes, ER Aspden, AJ Kerstein, AR Kolla, H Chen, JH AF Chatakonda, Obulesu Hawkes, Evatt R. Aspden, Andrew J. Kerstein, Alan R. Kolla, Hemanth Chen, Jacqueline H. TI On the fractal characteristics of low Damkohler number flames SO COMBUSTION AND FLAME LA English DT Article DE Turbulent premixed combustion; Fractal; Fractal dimension; Inner cut-off; Direct numerical simulation; Large-eddy simulation ID PREMIXED TURBULENT COMBUSTION; LARGE-EDDY SIMULATION; DIRECT NUMERICAL SIMULATIONS; PLANE JET FLAMES; SURFACE-DENSITY; IA SUPERNOVAE; DYNAMIC FORMULATION; BURNING VELOCITY; WRINKLING MODEL; HEATED COFLOW AB Knowledge of the fractal properties of premixed flame surfaces can potentially be used to help develop turbulent combustion models. Here, direct numerical simulations of low Damkohler number flames are used to analyse the fractal nature of the flames. Two sets of data are considered: (i) thermochemical hydrogen-air turbulent premixed plane-jet flames with detailed chemistry and (ii) thermonuclear flames in type la supernovae. A three-dimensional box counting method is used to investigate fractal dimension of the flame surface, characterising the self similarity of flame fronts. In the premixed flames, the fractal dimension is found to vary in time between 2.1 and 2.7. The supernovae flames in distributed combustion regimes yield fractal dimension about 2.7. The results for the maximum fractal dimensions are higher than previously reported. They are explained theoretically by a Reynolds number similarity argument which posits that the high Reynolds number, low Damkohler number limiting value of the fractal dimension is 8/3. Also tested is Mandelbrot's fractal additive law which relates the fractal dimension determined in two dimensions, which is typical of experimental measurements, to that in three dimensions. The comparison of the fractal dimension in both two-dimensional and three-dimensional spaces supports the additive law, even though the flames considered do not formally satisfy isotropy. Finally, the inner-cut off is extracted from the hydrogen flames and found to be consistent in order of magnitude with Kolmogorov scaling. (C) 2013 The Combustion Institute. All rights reserved. C1 [Chatakonda, Obulesu; Hawkes, Evatt R.] Univ New S Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia. [Hawkes, Evatt R.] Univ New S Wales, Sch Mech & Mfg Engn, Sydney, NSW 2052, Australia. [Aspden, Andrew J.] Univ Portsmouth, Sch Engn, Portsmouth PO1 3DJ, Hants, England. [Kerstein, Alan R.; Kolla, Hemanth; Chen, Jacqueline H.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. RP Hawkes, ER (reprint author), Univ New S Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia. EM evatt.hawkes@unsw.edu.au RI Kolla, Hemanth/L-2142-2013; Aspden, Andy/A-7391-2017; Hawkes, Evatt/C-5307-2012 OI Kolla, Hemanth/0000-0003-4969-5870; Aspden, Andy/0000-0002-2970-4824; Hawkes, Evatt/0000-0003-0539-7951 FU Australian Research Council [FT100100536]; Office of Science of the U.S. Department of Energy [DEAC05-00OR22725] FX This work was supported by the Australian Research Council under Grant No. FT100100536. The research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DEAC05-00OR22725, and the resources of the National Computational Infrastructure, Australia through the National Merit Allocation Scheme and the Intersect, Australia partner share. NR 73 TC 20 Z9 21 U1 0 U2 36 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0010-2180 J9 COMBUST FLAME JI Combust. Flame PD NOV PY 2013 VL 160 IS 11 BP 2422 EP 2433 DI 10.1016/j.combustflame.2013.05.007 PG 12 WC Thermodynamics; Energy & Fuels; Engineering, Multidisciplinary; Engineering, Chemical; Engineering, Mechanical SC Thermodynamics; Energy & Fuels; Engineering GA 212TT UT WOS:000324006400012 ER PT J AU Coriton, B Frank, JH Gomez, A AF Coriton, Bruno Frank, Jonathan H. Gomez, Alessandro TI Effects of strain rate, turbulence, reactant stoichiometry and heat losses on the interaction of turbulent premixed flames with stoichiometric counterflowing combustion products SO COMBUSTION AND FLAME LA English DT Article DE Turbulent premixed flames; Extinction; Ignition; Counterflow; Strain rate; Heat loss ID OPPOSED-JET FLAMES; LARGE-EDDY SIMULATION; BURNING RATE; FLOW-FIELD; AIR FLAMES; EXTINCTION; VELOCITY; CHEMISTRY; STREAMS; CURVATURE AB Intense strain, turbulence, heat transfer, and mixing with combustion products can affect premixed flames in practical combustion devices. These effects are systematically studied in turbulent premixed CH4/N-2/O-2 flames using a reactant versus product counterflow system and independently varying bulk strain rate, turbulent Reynolds number, equivalence ratio of the reactant mixture, and temperature of the stoichiometric counterflowing combustion products. The flow field and the turbulent flames are investigated using particle image velocimetry (PIV) measurements and laser-induced fluorescence (LIF) imaging of OH. The OH-LIF images are used to identify the interface between the counterflowing streams, referred to here as the gas mixing layer interface (GMLI). The flame response for different flow conditions is compared in terms of the probability of localized extinction along the GMLI, the turbulent flame brush thickness, and flame position relative to the GMLI, by using an OH-LIF-based progress variable. The probability of localized extinction at the GMLI increases as the separation between the turbulent flame brush and the GMLI decreases. Flame fronts in the vicinity of the GMLI are more likely to extinguish as a result of heat losses, dilution of the reaction zone by the product stream, and large local strain rates. A higher probability of localized extinction at the GMLI is induced by either a larger bulk strain rate or a slower flame speed. As the turbulent Reynolds number increases, the corresponding increase in turbulent flame brush thickness enhances the interactions of the flame fronts with the GMLI. Heat losses are substantially less significant for cases in which the turbulent flame brush is sufficiently separated from the GMLI. For flames in close proximity to the GMLI, the effects of the product stream on the flame front differ for lean and rich reactant mixtures. These disparities are attributed in part to differences in the ignitibility of the reactant mixtures by the hot product stream. (C) 2013 The Combustion Institute. Published by Elsevier Inc. All rights reserved. C1 [Coriton, Bruno; Frank, Jonathan H.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Gomez, Alessandro] Yale Univ, Dept Mech Engn & Mat Sci, Yale Ctr Combust Studies, New Haven, CT 06520 USA. RP Gomez, A (reprint author), Yale Univ, Dept Mech Engn & Mat Sci, Yale Ctr Combust Studies, New Haven, CT 06520 USA. EM alessandro.gomez@yale.edu FU American Chemical Society (ACS) [46991-AC9]; NSF [1060762.1.D1692.652001]; US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; US Department of Energy [DE-AC04-94-AL85000] FX The authors gratefully acknowledge the support of the American Chemical Society (ACS) through Grant PRF#46991-AC9 and of NSF (Grant #1060762.1.D1692.652001, Drs. Arvind Atreya and Ruey-Hung Chen, Program Directors) and the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the US Department of Energy under Contract DE-AC04-94-AL85000. NR 55 TC 15 Z9 16 U1 4 U2 49 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0010-2180 J9 COMBUST FLAME JI Combust. Flame PD NOV PY 2013 VL 160 IS 11 BP 2442 EP 2456 DI 10.1016/j.combustflame.2013.05.009 PG 15 WC Thermodynamics; Energy & Fuels; Engineering, Multidisciplinary; Engineering, Chemical; Engineering, Mechanical SC Thermodynamics; Energy & Fuels; Engineering GA 212TT UT WOS:000324006400014 ER PT J AU Cooper, MA Oliver, MS AF Cooper, Marcia A. Oliver, Michael S. TI The burning regimes and conductive burn rates of titanium subhydride potassium perchlorate (TiH1.65/KClO4) in hybrid closed bomb-strand burner experiments SO COMBUSTION AND FLAME LA English DT Article DE Pyrotechnic; Strand burner; Closed bomb; Conductive burning; Conductive-to-convective transition AB A hybrid closed bomb-strand burner is used to measure the burning behavior of the titanium subhydride potassium perchlorate pyrotechnic with an equivalent hydrogen concentration of 1.65. This experimental facility allows for simultaneous measurement of the closed bomb pressure rise and pyrotechnic burn rate as detected by electrical break wires over a range of pressures. Strands were formed by pressing the pyrotechnic powders to bulk solid volume fractions between 0.58 and 0.88 theoretical maximum density. The burn rate dependence on average pressed powder density and initial vessel pressure are measured. Data from the strands with a 0.68 theoretical maximum density are compared to available literature. At all initial strand densities, the burn is observed to transition from a steady conductive burn to an unsteady convective burn within the strand. The conductive burning regime is analyzed following traditional closed bomb methods used with propellants and incorporating a relevant instantaneous burning surface area for the pyrotechnic powder bed. The transition to convective burning is analyzed and a relationship between the initial material characteristics of the pyrotechnic powder bed and the critical pressure at transition is developed. (c) 2013 The Combustion Institute. All rights reserved. C1 [Cooper, Marcia A.; Oliver, Michael S.] Sandia Natl Labs, Explos Technol Grp, Albuquerque, NM 87185 USA. EM macoope@sandia.gov FU Stockpile Weapons Research Program at Sandia National Laboratories; United States Department of Energys National Nuclear Security Administration [DE-AC04-94AL85000] FX This work has been funded by the Stockpile Weapons Research Program at Sandia National Laboratories. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed-Martin Company, for the United States Department of Energys National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 37 TC 2 Z9 2 U1 0 U2 12 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0010-2180 J9 COMBUST FLAME JI Combust. Flame PD NOV PY 2013 VL 160 IS 11 BP 2619 EP 2630 DI 10.1016/j.combustflame.2013.05.015 PG 12 WC Thermodynamics; Energy & Fuels; Engineering, Multidisciplinary; Engineering, Chemical; Engineering, Mechanical SC Thermodynamics; Energy & Fuels; Engineering GA 212TT UT WOS:000324006400029 ER PT J AU Su, D Gaffrey, MJ Guo, J Clauss, TRW Thrall, BD Smith, RD Qian, WJ AF Su, Dian Gaffrey, Matthew J. Guo, Jia Clauss, Therese R. W. Thrall, Brian D. Smith, Richard D. Qian, Wei-Jun TI A General Proteomics Approach for Site-Specific Quantification of Cysteine Redox Modifications and Its Application for Profiling S-Glutathionylation in Macrophages SO FREE RADICAL BIOLOGY AND MEDICINE LA English DT Meeting Abstract C1 [Su, Dian; Gaffrey, Matthew J.; Guo, Jia; Clauss, Therese R. W.; Thrall, Brian D.; Smith, Richard D.; Qian, Wei-Jun] Pacific NW Natl Lab, Richland, WA 99352 USA. RI Smith, Richard/J-3664-2012 OI Smith, Richard/0000-0002-2381-2349 NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0891-5849 EI 1873-4596 J9 FREE RADICAL BIO MED JI Free Radic. Biol. Med. PD NOV 1 PY 2013 VL 65 SU 2 MA 356 BP S152 EP S153 DI 10.1016/j.freeradbiomed.2013.10.782 PG 2 WC Biochemistry & Molecular Biology; Endocrinology & Metabolism SC Biochemistry & Molecular Biology; Endocrinology & Metabolism GA V40JU UT WOS:000209475700374 ER PT J AU Moyer, JA Kumah, DP Vaz, CAF Arena, DA Henrich, VE AF Moyer, J. A. Kumah, D. P. Vaz, C. A. F. Arena, D. A. Henrich, V. E. TI Role of epitaxial strain on the magnetic structure of Fe-doped CoFe2O4 SO JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS LA English DT Article DE Iron-doped cobalt ferrite; Magnetic structure; Molecular beam epitaxy; Epitaxial strain ID TRANSITION-METAL COMPOUNDS; FERRITE THIN-FILMS; RAY CIRCULAR-DICHROISM; 2P ABSORPTION-SPECTRA; COBALT FERRITE; ANISOTROPY; ORIGIN; FE3O4; NANOSTRUCTURES; BEHAVIOR AB The magnetic structure of Fe-doped CoFe2O4 (Co1-xFe2+xO4) grown on MgO (0 0 1) and SrTiO3 (0 0 1) substrates is studied with superconducting quantum interference device magnetometry and soft x-ray magnetic spectroscopies. X-ray and electron diffraction show that the choice of substrate has large effects on the strain, crystal structure and surface morphology of Co1-xFe2+xO4 thin films. Samples grown on MgO have small, coherent strains and surfaces that are nearly atomically flat, whereas films grown on SrTiO3 have large tensile strains and surfaces terminated with islands, which indicate the presence of a large density of misfit dislocations. These differences in structural properties correlate with the large differences seen in the magnetic structure; samples grown on SrTiO3 have larger magnetic moments and increased anisotropies compared to those grown on MgO. Most strikingly, the large magnetic spin and orbital moments found in the films grown on SrTiO3 suggest a suppression of anti-phase boundary formation, which we attribute to the large compressive lattice mismatch and the formation of misfit dislocations during the film growth in order to relieve the epitaxial strain. This results in the films grown on SrTiO3 having magnetic properties that are more similar to bulk Co1-xFe2+xO4 than those grown on MgO, demonstrating that epitaxial strain can result in large changes in the magnetic structure of Co1-xFe2+xO4. (C) 2013 Elsevier B.V. All rights reserved. C1 [Moyer, J. A.; Kumah, D. P.; Henrich, V. E.] Yale Univ, Dept Appl Phys, New Haven, CT 06511 USA. [Moyer, J. A.; Kumah, D. P.; Henrich, V. E.] Yale Univ, Ctr Res Interface Struct & Phenomena, New Haven, CT 06511 USA. [Vaz, C. A. F.] Paul Scherrer Inst, SwissFEL, CH-5232 Villigen, Switzerland. [Arena, D. A.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. RP Moyer, JA (reprint author), Univ Illinois, Dept Phys, Urbana, IL 61801 USA. EM moyerja@illinois.edu RI Vaz, Carlos/A-7240-2012; Kumah, Divine/A-7031-2011 OI Vaz, Carlos/0000-0002-6209-8918; Kumah, Divine/0000-0003-0715-1285 FU NSF through MRSEC [DMR 1119826 (CRISP)]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX The authors acknowledge primary financial support by the NSF through MRSEC DMR 1119826 (CRISP). Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 44 TC 5 Z9 5 U1 3 U2 80 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-8853 J9 J MAGN MAGN MATER JI J. Magn. Magn. Mater. PD NOV PY 2013 VL 345 BP 180 EP 189 DI 10.1016/j.jmmm.2013.06.031 PG 10 WC Materials Science, Multidisciplinary; Physics, Condensed Matter SC Materials Science; Physics GA 213HB UT WOS:000324045300032 ER PT J AU Bell, CW Fricks, BE Rocca, JD Steinweg, JM McMahon, SK Wallenstein, MD AF Bell, Colin W. Fricks, Barbara E. Rocca, Jennifer D. Steinweg, Jessica M. McMahon, Shawna K. Wallenstein, Matthew D. TI High-throughput Fluorometric Measurement of Potential Soil Extracellular Enzyme Activities SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS LA English DT Article DE Environmental Sciences; Issue 81; Ecological and Environmental Phenomena; Environment; Biochemistry; Environmental Microbiology; Soil Microbiology; Ecology; Eukaryota; Archaea; Bacteria; Soil extracellular enzyme activities (EEAs); fluorometric enzyme assays; substrate degradation; 4-methylumbelliferone (MUB); 7-amino-4-methylcoumarin (MUC); enzyme temperature kinetics; soil AB Microbes in soils and other environments produce extracellular enzymes to depolymerize and hydrolyze organic macromolecules so that they can be assimilated for energy and nutrients. Measuring soil microbial enzyme activity is crucial in understanding soil ecosystem functional dynamics. The general concept of the fluorescence enzyme assay is that synthetic C-, N-, or P-rich substrates bound with a fluorescent dye are added to soil samples. When intact, the labeled substrates do not fluoresce. Enzyme activity is measured as the increase in fluorescence as the fluorescent dyes are cleaved from their substrates, which allows them to fluoresce. Enzyme measurements can be expressed in units of molarity or activity. To perform this assay, soil slurries are prepared by combining soil with a pH buffer. The pH buffer (typically a 50 mM sodium acetate or 50 mM Tris buffer), is chosen for the buffer's particular acid dissociation constant (pKa) to best match the soil sample pH. The soil slurries are inoculated with a nonlimiting amount of fluorescently labeled (i.e. C-, N-, or P-rich) substrate. Using soil slurries in the assay serves to minimize limitations on enzyme and substrate diffusion. Therefore, this assay controls for differences in substrate limitation, diffusion rates, and soil pH conditions; thus detecting potential enzyme activity rates as a function of the difference in enzyme concentrations (per sample). Fluorescence enzyme assays are typically more sensitive than spectrophotometric (i.e. colorimetric) assays, but can suffer from interference caused by impurities and the instability of many fluorescent compounds when exposed to light; so caution is required when handling fluorescent substrates. Likewise, this method only assesses potential enzyme activities under laboratory conditions when substrates are not limiting. Caution should be used when interpreting the data representing cross-site comparisons with differing temperatures or soil types, as in situ soil type and temperature can influence enzyme kinetics. C1 [Bell, Colin W.; Fricks, Barbara E.; Rocca, Jennifer D.; Wallenstein, Matthew D.] Colorado State Univ, Nat Resource Ecol Lab, Ft Collins, CO 80523 USA. [Steinweg, Jessica M.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [McMahon, Shawna K.] Univ Colorado, Dept Bioengn, Boulder, CO 80309 USA. RP Wallenstein, MD (reprint author), Colorado State Univ, Nat Resource Ecol Lab, Ft Collins, CO 80523 USA. EM matthew.wallenstein@colostate.edu RI Wallenstein, Matthew/C-6441-2008 OI Wallenstein, Matthew/0000-0002-6219-1442 FU Enzymes in the Environment Research Coordination Network Research - US National Science Foundation [1021559]; US National Science Foundation [1021559]; US Department of Energy's Office of Science (Biological and Environmental Research) FX This publication was funded by the Enzymes in the Environment Research Coordination Network Research supported by the US National Science Foundation (DEB# 1021559). This research was supported by the US National Science Foundation (DEB# 1021559), and the US Department of Energy's Office of Science (Biological and Environmental Research). Any opinions, findings, and conclusions or recommendations expressed in this material are those of the authors and do not necessarily reflect the views of the US NSF. NR 50 TC 14 Z9 14 U1 10 U2 46 PU JOURNAL OF VISUALIZED EXPERIMENTS PI CAMBRIDGE PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA SN 1940-087X J9 JOVE-J VIS EXP JI J. Vis. Exp. PD NOV PY 2013 IS 81 AR UNSP e50961 DI 10.3791/50961 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA V36RQ UT WOS:000209228900060 PM 24299913 ER PT J AU Doeff, MM Chen, GY Cabana, J Richardson, TJ Mehta, A Shirpour, M Duncan, H Kim, C Kam, KC Conry, T AF Doeff, Marca M. Chen, Guoying Cabana, Jordi Richardson, Thomas J. Mehta, Apurva Shirpour, Mona Duncan, Hugues Kim, Chunjoong Kam, Kinson C. Conry, Thomas TI Characterization of Electrode Materials for Lithium Ion and Sodium Ion Batteries Using Synchrotron Radiation Techniques SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS LA English DT Article DE Physics; Issue 81; X-Ray Absorption Spectroscopy; X-Ray Diffraction; inorganic chemistry; electric batteries (applications); energy storage; Electrode materials; Li-ion battery; Na-ion battery; X-ray Absorption Spectroscopy (XAS); in situ X-ray diffraction (XRD) AB Intercalation compounds such as transition metal oxides or phosphates are the most commonly used electrode materials in Li-ion and Na-ion batteries. During insertion or removal of alkali metal ions, the redox states of transition metals in the compounds change and structural transformations such as phase transitions and/or lattice parameter increases or decreases occur. These behaviors in turn determine important characteristics of the batteries such as the potential profiles, rate capabilities, and cycle lives. The extremely bright and tunable x-rays produced by synchrotron radiation allow rapid acquisition of high-resolution data that provide information about these processes. Transformations in the bulk materials, such as phase transitions, can be directly observed using X-ray diffraction (XRD), while X-ray absorption spectroscopy (XAS) gives information about the local electronic and geometric structures (e.g. changes in redox states and bond lengths). In situ experiments carried out on operating cells are particularly useful because they allow direct correlation between the electrochemical and structural properties of the materials. These experiments are time-consuming and can be challenging to design due to the reactivity and air-sensitivity of the alkali metal anodes used in the half-cell configurations, and/or the possibility of signal interference from other cell components and hardware. For these reasons, it is appropriate to carry out ex situ experiments (e.g. on electrodes harvested from partially charged or cycled cells) in some cases. Here, we present detailed protocols for the preparation of both ex situ and in situ samples for experiments involving synchrotron radiation and demonstrate how these experiments are done. C1 [Doeff, Marca M.; Chen, Guoying; Cabana, Jordi; Richardson, Thomas J.; Shirpour, Mona; Duncan, Hugues; Kim, Chunjoong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Cabana, Jordi] Univ Illinois, Dept Chem, Chicago, IL 60680 USA. [Mehta, Apurva] Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA USA. [Kam, Kinson C.] Haldor Topsoe Res Labs, Ravnholm, Denmark. [Conry, Thomas] PolyPlus Battery Co, Berkeley, CA USA. RP Doeff, MM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM mmdoeff@lbl.gov RI Cabana, Jordi/G-6548-2012 OI Cabana, Jordi/0000-0002-2353-5986 FU Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy [DE-AC02-05CH11231]; DOE Office of Biological and Environmental Research; National Institutes of Health, National Center for Research Resources, Biomedical Technology Program [P41RR001209] FX This work is supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a Directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. The SSRL Structural Molecular Biology Program is supported by the DOE Office of Biological and Environmental Research, and by the National Institutes of Health, National Center for Research Resources, Biomedical Technology Program (P41RR001209). NR 22 TC 2 Z9 2 U1 8 U2 31 PU JOURNAL OF VISUALIZED EXPERIMENTS PI CAMBRIDGE PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA SN 1940-087X J9 JOVE-J VIS EXP JI J. Vis. Exp. PD NOV PY 2013 IS 81 AR UNSP e50594 DI 10.3791/50594 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA V36RQ UT WOS:000209228900011 PM 24300777 ER PT J AU Gutschow, C Marshall, Z AF Guetschow, Christian Marshall, Zachary TI Setting Limits on Supersymmetry Using Simplified Models SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS LA English DT Article DE Physics; Issue 81; high energy physics; particle physics; Supersymmetry; LHC; ATLAS; CMS; New Physics Limits; Simplified Models AB Experimental limits on supersymmetry and similar theories are difficult to set because of the enormous available parameter space and difficult to generalize because of the complexity of single points. Therefore, more phenomenological, simplified models are becoming popular for setting experimental limits, as they have clearer physical interpretations. The use of these simplified model limits to set a real limit on a concrete theory has not, however, been demonstrated. This paper recasts simplified model limits into limits on a specific and complete supersymmetry model, minimal supergravity. Limits obtained under various physical assumptions are comparable to those produced by directed searches. A prescription is provided for calculating conservative and aggressive limits on additional theories. Using acceptance and efficiency tables along with the expected and observed numbers of events in various signal regions, LHC experimental results can be recast in this manner into almost any theoretical framework, including nonsupersymmetric theories with supersymmetry-like signatures. C1 [Guetschow, Christian] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Marshall, Zachary] CERN, CH-1211 Geneva 23, Switzerland. [Marshall, Zachary] Lawrence Berkeley Natl Lab, Phys Div, Berkeley, CA USA. RP Marshall, Z (reprint author), CERN, CH-1211 Geneva 23, Switzerland. EM zach.marshall@cern.ch NR 47 TC 0 Z9 0 U1 0 U2 0 PU JOURNAL OF VISUALIZED EXPERIMENTS PI CAMBRIDGE PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA SN 1940-087X J9 JOVE-J VIS EXP JI J. Vis. Exp. PD NOV PY 2013 IS 81 AR UNSP e50419 DI 10.3791/50419 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA V36RQ UT WOS:000209228900003 PM 24300306 ER PT J AU Krishna, KS Biswas, S Navin, CV Yamane, DG Miller, JT Kumar, CSSR AF Krishna, Katla Sai Biswas, Sanchita Navin, Chelliah V. Yamane, Dawit G. Miller, Jeffrey T. Kumar, Challa S. S. R. TI Millifluidics for Chemical Synthesis and Time-resolved Mechanistic Studies SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS LA English DT Article DE Bioengineering; Issue 81; Millifluidics; Millifluidic Device; Time-resolved Kinetics; Synthesis; Catalysis; Nanomaterials; Lab-on-a-Chip AB Procedures utilizing millifluidic devices for chemical synthesis and time-resolved mechanistic studies are described by taking three examples. In the first, synthesis of ultra-small copper nanoclusters is described. The second example provides their utility for investigating time resolved kinetics of chemical reactions by analyzing gold nanoparticle formation using in situ X-ray absorption spectroscopy. The final example demonstrates continuous flow catalysis of reactions inside millifluidic channel coated with nanostructured catalyst. C1 [Krishna, Katla Sai; Biswas, Sanchita; Navin, Chelliah V.; Yamane, Dawit G.; Kumar, Challa S. S. R.] Louisiana State Univ, CAMD, Baton Rouge, LA 70803 USA. [Krishna, Katla Sai; Biswas, Sanchita; Navin, Chelliah V.; Kumar, Challa S. S. R.] Louisiana State Univ, Ctr Atom Level Catalyst Design, Cain Dept Chem Engn, Baton Rouge, LA 70803 USA. [Navin, Chelliah V.] Louisiana State Univ, Dept Biol & Agr Engn, Baton Rouge, LA 70803 USA. [Miller, Jeffrey T.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Kumar, CSSR (reprint author), Louisiana State Univ, CAMD, Baton Rouge, LA 70803 USA. EM ckumar1@lsu.edu FU Center for Atomic Level Catalyst Design, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001058]; Board of Regents [LEQSF (2009-14)-EFRC-MATCH, LEDSF-EPS(2012)-OPT-IN-15]; Department of Energy; MRCAT member institutions; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX This research work is supported as part of the Center for Atomic Level Catalyst Design, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001058 and also supported by Board of Regents under grants award number LEQSF (2009-14)-EFRC-MATCH and LEDSF-EPS(2012)-OPT-IN-15. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. The use of the Advanced Photon Source at ANL is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Financial support for JTM was provided as part of the Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. NR 24 TC 1 Z9 1 U1 1 U2 12 PU JOURNAL OF VISUALIZED EXPERIMENTS PI CAMBRIDGE PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA SN 1940-087X J9 JOVE-J VIS EXP JI J. Vis. Exp. PD NOV PY 2013 IS 81 AR UNSP e50711 DI 10.3791/50711 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA V36RQ UT WOS:000209228900022 ER PT J AU Jeen, H Choi, WS Biegalski, MD Folkman, CM Tung, IC Fong, DD Freeland, JW Shin, D Ohta, H Chisholm, MF Lee, HN AF Jeen, Hyoungjeen Choi, Woo Seok Biegalski, Michael D. Folkman, Chad M. Tung, I-Cheng Fong, Dillon D. Freeland, John W. Shin, Dongwon Ohta, Hiromichi Chisholm, Matthew F. Lee, Ho Nyung TI Reversible redox reactions in an epitaxially stabilized SrCoOx oxygen sponge SO NATURE MATERIALS LA English DT Article ID FUEL-CELLS; MAGNETIC-PROPERTIES; OXIDE; SRCOO3-DELTA; SPECTROSCOPY; TEMPERATURE; PERFORMANCE; REDUCTION; DIFFUSION; TRANSPORT AB Fast, reversible redox reactions in solids at low temperatures without thermomechanical degradation are a promising strategy for enhancing the overall performance and lifetime of many energy materials and devices. However, the robust nature of the cation's oxidation state and the high thermodynamic barrier have hindered the realization of fast catalysis and bulk diffusion at low temperatures. Here, we report a significant lowering of the redox temperature by epitaxial stabilization of strontium cobaltites (SrCoOx) grown directly as one of two distinct crystalline phases, either the perovskite SrCoO3-delta or the brownmillerite SrCoO2.5. Importantly, these two phases can be reversibly switched at a remarkably reduced temperature (200-300 degrees C) in a considerably short time (<1 min) without destroying the parent framework. The fast, low-temperature redox activity in SrCoO3-delta is attributed to a small Gibbs free-energy difference between two topotatic phases. Our findings thus provide useful information for developing highly sensitive electrochemical sensors and low-temperature cathode materials. C1 [Jeen, Hyoungjeen; Choi, Woo Seok; Shin, Dongwon; Chisholm, Matthew F.; Lee, Ho Nyung] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Biegalski, Michael D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Folkman, Chad M.; Fong, Dillon D.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Tung, I-Cheng; Freeland, John W.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Tung, I-Cheng] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Ohta, Hiromichi] Hokkaido Univ, Res Inst Elect Sci, Sapporo, Hokkaido 0010020, Japan. RP Lee, HN (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM hnlee@ornl.gov RI Choi, Woo Seok/G-8783-2014; Shin, Dongwon/C-6519-2008; Ohta, Hiromichi/H-4468-2012; Lee, Ho Nyung/K-2820-2012 OI Shin, Dongwon/0000-0002-5797-3423; Ohta, Hiromichi/0000-0001-7013-0343; Lee, Ho Nyung/0000-0002-2180-3975 FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; US Department of Energy, Office of Science [DE-AC02-06CH11357]; MEXT [25246023] FX The work was supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. The in situ XRD measurement was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. Use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. H.O. was supported by MEXT (25246023). NR 36 TC 68 Z9 68 U1 15 U2 113 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD NOV PY 2013 VL 12 IS 11 BP 1057 EP 1063 DI 10.1038/NMAT3736 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA 240LZ UT WOS:000326099300023 PM 23975056 ER PT J AU Thomas, JL AF Thomas, Jennifer L. TI Helpful or Harmful? Potential Effects of Exercise on Select Inflammatory Conditions SO PHYSICIAN AND SPORTSMEDICINE LA English DT Article DE inflammation; exercise; rheumatic diseases; cytokines; physical activity ID NECROSIS-FACTOR-ALPHA; NF-KAPPA-B; HUMAN SKELETAL-MUSCLE; UBIQUITIN-PROTEASOME PATHWAY; SYSTEMIC-LUPUS-ERYTHEMATOSUS; ANKYLOSING-SPONDYLITIS; INSULIN-RESISTANCE; RHEUMATOID-ARTHRITIS; ECCENTRIC EXERCISE; AEROBIC EXERCISE AB Inflammation has been characterized as a double-edged sword, requiring a balance between health as maintained by regular exercise and activities that would exacerbate inflammatory diseases. The influence of exercise on inflammation is complex and has been widely studied in both healthy patient populations as well as populations of patients with many inflammatory and/or autoimmune rheumatic diseases. Inflammatory markers can be affected by the type of exercise and muscle contraction, as well as the intensity, duration, and consistency of the exercise sessions. Because of these potentially important effects, many members of the general public, as well as some clinicians, believe that exercise could exacerbate symptoms and accelerate the progression of such conditions. The effects of different types of exercise have been studied among patients with inflammatory conditions such as ankylosing spondylitis, systemic lupus erythematosus, rheumatoid arthritis, osteoarthritis, fibromyalgia, and idiopathic inflammatory myopathies, as well as congestive heart failure, type 2 diabetes mellitus, and metabolic syndrome, which are considered lowgrade systemic inflammatory diseases. This review will help exercise professionals and clinicians understand the effects of exercise on inflammatory markers, as well as offer effective treatment options and recommendations for patients exercising with rheumatic or inflammatory conditions. C1 [Thomas, Jennifer L.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Thomas, Jennifer L.] Univ New Mexico, Dept Hlth Exercise & Sports Sci, Albuquerque, NM 87131 USA. RP Thomas, JL (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. NR 53 TC 6 Z9 6 U1 2 U2 15 PU JTE MULTIMEDIA PI WEST CONSHOHOCKEN PA 18 ELIZABETH ST, STE 110, WEST CONSHOHOCKEN, PA 19428 USA SN 0091-3847 J9 PHYSICIAN SPORTSMED JI Physician Sportsmed. PD NOV PY 2013 VL 41 IS 4 BP 93 EP 100 DI 10.3810/psm.2013.11.2040 PG 8 WC Primary Health Care; Orthopedics; Sport Sciences SC General & Internal Medicine; Orthopedics; Sport Sciences GA AR2FB UT WOS:000343397900010 PM 24231601 ER PT J AU Cornillon, PA Hengartner, N Jegou, N Matzner-Lober, E AF Cornillon, P-A Hengartner, N. Jegou, N. Matzner-Lober, E. TI Iterative bias reduction: a comparative study SO STATISTICS AND COMPUTING LA English DT Article DE Multivariate smoothing; Thin-plate splines; Duchon splines; Kernel regression; Iterative bias reduction ID GENERALIZED CROSS-VALIDATION; ADDITIVE LOGISTIC-REGRESSION; STATISTICAL VIEW; MODELS AB Multivariate nonparametric smoothers, such as kernel based smoothers and thin plate splines smoothers, are adversely impacted by the sparseness of data in high dimension, also known as the curse of dimensionality. Adaptive smoothers, that can exploit the underlying smoothness of the regression function, may partially mitigate this effect. This paper presents a comparative simulation study of a novel adaptive smoother (IBR) with competing multivariate smoothers available as package or function within the R language and environment for statistical computing. Comparison between the methods are made on simulated datasets of moderate size, from 50 to 200 observations, with two, five or 10 potential explanatory variables, and on a real dataset. The results show that the good asymptotic properties of IBR are complemented by a very good behavior on moderate sized datasets, results which are similar to those obtained with Duchon low rank splines. C1 [Cornillon, P-A] Univ Rennes 2, IRMAR, F-35043 Rennes, France. [Jegou, N.; Matzner-Lober, E.] Univ Rennes 2, F-35043 Rennes, France. [Hengartner, N.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Matzner-Lober, E (reprint author), Univ Rennes 2, F-35043 Rennes, France. EM pac@uhb.fr; nickh@lanl.gov; nicolas.jegou@uhb.fr; eml@uhb.fr NR 32 TC 2 Z9 2 U1 1 U2 7 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0960-3174 J9 STAT COMPUT JI Stat. Comput. PD NOV PY 2013 VL 23 IS 6 BP 777 EP 791 DI 10.1007/s11222-012-9346-4 PG 15 WC Computer Science, Theory & Methods; Statistics & Probability SC Computer Science; Mathematics GA 214MS UT WOS:000324138300008 ER PT J AU Du, MH Biswas, K AF Du, Mao-Hua Biswas, Koushik TI Electronic structure engineering of elpasolites: Case of Cs2AgYCl6 SO JOURNAL OF LUMINESCENCE LA English DT Article DE Cs2AgYCl6; Elpasolite; Scintillator; Radiation detection ID DOPED HALIDE SCINTILLATORS; AUGMENTED-WAVE METHOD; ANOMALOUS EMISSION; CRYSTALS; GAMMA; CS2LIYCL6-CE3+; SPECTROSCOPY; EFFICIENT; GROWTH; RAY AB Electronic structure engineering of elpasolite-based scintillators is explored for improving light yield and scintillation response. First-principles calculations of electronic structure, polarons, and Ce activator in CS2AgYCl6 show that the electronegativity of constituent elements of a quaternary elpasolite compound can be manipulated to reduce the band gap and carrier self-trapping energy, which should lead to higher light yield and faster scintillation decay. (C) 2013 Elsevier B.V. All rights reserved. C1 [Du, Mao-Hua] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Du, Mao-Hua] Oak Ridge Natl Lab, Ctr Radiat Detect Mat & Syst, Oak Ridge, TN 37831 USA. [Biswas, Koushik] Arkansas State Univ, Dept Chem & Phys, State Univ, AR 72467 USA. RP Du, MH (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM mhdu@ornl.gov RI Du, Mao-Hua/B-2108-2010 OI Du, Mao-Hua/0000-0001-8796-167X FU U.S. Department of Energy's Office of Nonproliferation and Verification Research and Development [NA-22] FX We are grateful for helpful discussions with Zane W. Bell, David J. Singh and Lynn A. Boatner. This work was supported by the U.S. Department of Energy's Office of Nonproliferation and Verification Research and Development (NA-22). NR 32 TC 6 Z9 6 U1 2 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-2313 J9 J LUMIN JI J. Lumines. PD NOV PY 2013 VL 143 BP 710 EP 714 DI 10.1016/j.jlumin.2013.05.033 PG 5 WC Optics SC Optics GA 211MN UT WOS:000323912400116 ER PT J AU Chou, CP AF Chou, Chung-Pin TI Low-lying quasiparticle excitations in strongly correlated superconductors: An ansatz from BCS quasiparticle excitations? SO JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS LA English DT Article DE Superconductors; Variational Monte Carlo; Strong correlation; Quasiparticle excitations ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; ANGLE-RESOLVED PHOTOEMISSION; MEAN-FIELD THEORY; FERMION SYSTEMS; MONTE-CARLO; SIMULATION AB The question about the existence of Bogoliubov's quasiparticles in the BCS wave functions underneath Gutzwiller's projection is of importance to strongly correlated systems. We develop a method to examine the two-particle excitations of Gutzwiller-projected BCS wave functions by using the variational Monte Carlo approach. We find that the exact Gutzwiller-projected quasiparticle (GQP) dispersions are quantitatively reproduced by the Gutzwiller-projected Bogoliubov quasiparticles (GBQP) except the regions where d-wave Cooper pairing is strong. We believe GBQP provides a reasonable description to the low-energy excitations in strongly correlated superconducting systems because GBQP becomes more stable than GQP near the antinodes. Our framework offers a route to understand the intimate connection between Gutzwiller's projection and d-wave Cooper pairing. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Chou, Chung-Pin] Beijing Computat Sci Res Ctr, Beijing 100084, Peoples R China. [Chou, Chung-Pin] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Chou, CP (reprint author), Beijing Computat Sci Res Ctr, Beijing 100084, Peoples R China. EM cpc63078@gmail.com FU Brookhaven Science Associates, LLC [DE-AC02-98CH10886]; U.S. Department of Energy; National Science Council in Taiwan [NSC 101-2917-I-564-010] FX The author thanks T.-K. Lee and W. Ku for useful discussions. We also acknowledge W. Yin for helpful proofreading on the manuscript. This work is supported by Brookhaven Science Associates, LLC under Contract no. DE-AC02-98CH10886 with the U.S. Department of Energy and the Postdoctoral Research Abroad Program sponsored by National Science Council in Taiwan with Grant no. NSC 101-2917-I-564-010. NR 36 TC 1 Z9 1 U1 0 U2 14 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-3697 J9 J PHYS CHEM SOLIDS JI J. Phys. Chem. Solids PD NOV PY 2013 VL 74 IS 11 BP 1589 EP 1593 DI 10.1016/j.jpcs.2013.05.027 PG 5 WC Chemistry, Multidisciplinary; Physics, Condensed Matter SC Chemistry; Physics GA 207HR UT WOS:000323590000012 ER PT J AU Lee, KJ Smith, K Pesaran, A Kim, GH AF Lee, Kyu-Jin Smith, Kandler Pesaran, Ahmad Kim, Gi-Heon TI Three dimensional thermal-, electrical-, and electrochemical-coupled model for cylindrical wound large format lithium-ion batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium-ion battery; Wound cylindrical cell; Multiscale model; Orthotropic continuum; Wound potential-pair continuum model ID POSITIVE ELECTRODES; DESIGN; CELL AB A numerical model for cylindrical wound lithium-ion cells, which resolves thermal, electrical and electrochemical coupled physics, is presented in this paper. Using the Multi-Scale Multi-Domain (MSMD) model framework, the wound potential-pair continuum (WPPC) model is developed as a cell domain submodel to solve heat and electron transfer across the length scale of cell dimension. By defining the cell composite as a wound continuum, the WPPC model can evaluate layer-to-layer differences in electrical potential along current collectors, and electric current in the winding direction to investigate the effects of thermal and electrical configurations of a cell design, such as number and location of tabs, on performance and life of a cylindrical cell. In this study, 20-Ah large-format cylindrical cell simulations are conducted using the WPPC model with the number of electrical tabs as a control parameter to investigate how macroscopic design for electrical current transport affects microscopic electrochemical processes and apparent electrical and thermal output. (C) 2013 Elsevier B.V. All rights reserved. C1 [Lee, Kyu-Jin; Smith, Kandler; Pesaran, Ahmad; Kim, Gi-Heon] Natl Renewable Energy Lab, Golden, CO USA. [Lee, Kyu-Jin] Myongji Univ, Dept Mech Engn, Yongin, Gyeonggi Do, South Korea. RP Kim, GH (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO USA. EM gi-heon.kim@nrel.gov RI Khan, Mohammad Rezwan/E-1422-2011 OI Khan, Mohammad Rezwan/0000-0002-1532-0598 FU U.S. Department of Energy Office of Vehicle Technologies' Energy Storage Program; U.S. DOE's Computer Aided Engineering for Electric Drive Batteries (CAEBat) FX The authors acknowledge David Howell, Brian Cunningham, and the U.S. Department of Energy Office of Vehicle Technologies' Energy Storage Program for their funding and support. The present work was supported by the U.S. DOE's Computer Aided Engineering for Electric Drive Batteries (CAEBat). NR 21 TC 39 Z9 40 U1 5 U2 74 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 J9 J POWER SOURCES JI J. Power Sources PD NOV 1 PY 2013 VL 241 BP 20 EP 32 DI 10.1016/j.jpowsour.2013.03.007 PG 13 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 200TL UT WOS:000323093700004 ER PT J AU Vijayakumar, M Wang, W Nie, ZM Sprenkle, V Hu, JZ AF Vijayakumar, M. Wang, Wei Nie, Zimin Sprenkle, Vincent Hu, JianZhi TI Elucidating the higher stability of vanadium(V) cations in mixed acid based redox flow battery electrolytes SO JOURNAL OF POWER SOURCES LA English DT Article DE Cl-35 and V-51 NMR; Vanadium redox flow battery; Electrolyte stability and DFT; Ligand exchange process ID RESEARCH-AND-DEVELOPMENT; ENERGY-STORAGE; DENSITY; PROGRESS; CELL; THERMOCHEMISTRY; APPROXIMATION; ORBITALS AB The vanadium(V) cation structures in mixed acid based electrolyte solution were analyzed by density functional theory (DFT) based computational modeling and V-51 and Cl-35 nuclear magnetic resonance (NMR) spectroscopy. The vanadium(V) cation exists as di-nuclear [V2O3Cl2 center dot 6H(2)O](2+) compound at higher vanadium concentrations (>= 1.75 M). In particular, at high temperatures (>295 K) this di-nuclear compound undergoes ligand exchange process with nearby solvent chlorine molecule and forms chlorine bonded [V2O3Cl center dot 6H(2)O](2+) compound. This chlorine bonded [V2O3Cl2 center dot 6H(2)O]2+ compound might be resistant to the de-protonation reaction which is the initial step in the precipitation reaction in vanadium based electrolyte solutions. The combined theoretical and experimental approach reveals that formation of chlorine bonded [V2O3Cl2 center dot 6H(2)O](2+) compound might be central to the observed higher thermal stability of mixed acid based vanadium(V) electrolyte solutions. (C) 2013 Elsevier B.V. All rights reserved. C1 [Vijayakumar, M.; Wang, Wei; Nie, Zimin; Sprenkle, Vincent; Hu, JianZhi] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Vijayakumar, M (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM Vijay@pnnl.gov; wei.wang@pnnl.gov RI Murugesan, Vijayakumar/C-6643-2011; Wang, Wei/F-4196-2010; Hu, Jian Zhi/F-7126-2012 OI Murugesan, Vijayakumar/0000-0001-6149-1702; Wang, Wei/0000-0002-5453-4695; FU Office of Electricity Delivery & Energy Reliability; U.S. Department of Energy (DOE) [57558]; PNNL through LDRD program; DOE by Battelle [DE-AC05-76RL01830]; DOE's Office of Biological and Environmental Research (BER) FX This work was supported by the Office of Electricity Delivery & Energy Reliability (project manager: Dr. Imre Gyuk), U.S. Department of Energy (DOE) under contract #57558. We also are grateful for insightful discussions with Dr. Imre Gyuk of the DOE-OE Grid Storage Program. We also acknowledge PNNL for the funding through LDRD program. PNNL is a multi-program laboratory operated for DOE by Battelle under Contract DE-AC05-76RL01830. The NMR and DFT computation work were carried out at the Environmental and Molecular Science Laboratory (EMSL), a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research (BER). We thank Sarah D. Burton from EMSL for her help in measuring NMR. NR 27 TC 25 Z9 26 U1 1 U2 104 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD NOV 1 PY 2013 VL 241 BP 173 EP 177 DI 10.1016/j.jpowsour.2013.04.072 PG 5 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 200TL UT WOS:000323093700021 ER PT J AU Kalnaus, S Tenhaeff, WE Sakamoto, J Sabau, AS Daniel, C Dudney, NJ AF Kalnaus, Sergiy Tenhaeff, Wyatt E. Sakamoto, Jeffrey Sabau, Adrian S. Daniel, Claus Dudney, Nancy J. TI Analysis of composite electrolytes with sintered reinforcement structure for energy storage applications SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium ion battery; Composite electrolyte; Sintering; Lithium anode; Dendrites ID LITHIUM SECONDARY BATTERIES; SOLID POLYMER ELECTROLYTES; THIN-FILM LITHIUM; ELASTIC PROPERTIES; ION BATTERIES; ELECTRICAL-PROPERTIES; GLASS-CERAMICS; CONDUCTIVITY; MODULUS; LI7LA3ZR2O12 AB Effective conductivity and mechanical properties of composite polymer electrolytes, in which the reinforcement phase is a sintered packed bed of Li-ion conductive ceramics particles, were estimated using finite element analyses. The computations targeted estimation of the effect of sintering degree, i.e. size of the inter-particle connective necks, on the overall properties of the composite. Methods for microstructure generation and computational procedures were presented. The mechanical ability of the membrane to block lithium dendrites was assessed based on a stability criterion, which depends on the computed effective stiffness. It was found that the minimum size of the inter-particle connections necessary to provide mechanical stability without losing the enhancement in conductivity was 0.05 times the mean particle radius. (C) 2013 Elsevier B.V. All rights reserved. C1 [Kalnaus, Sergiy; Tenhaeff, Wyatt E.; Sabau, Adrian S.; Daniel, Claus; Dudney, Nancy J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Sakamoto, Jeffrey] Michigan State Univ, Dept Mat Sci & Engn, E Lansing, MI 48824 USA. [Daniel, Claus] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. [Daniel, Claus] Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Grad Educ, Knoxville, TN 37996 USA. RP Kalnaus, S (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM kalnauss@oml.gov RI Sabau, Adrian/B-9571-2008; Dudney, Nancy/I-6361-2016; Daniel, Claus/A-2060-2008; OI Sabau, Adrian/0000-0003-3088-6474; Dudney, Nancy/0000-0001-7729-6178; Daniel, Claus/0000-0002-0571-6054; Kalnaus, Sergiy/0000-0002-7465-3034 FU U.S. Department of Energy [DE-AC05-00OR22725]; Vehicle Technologies Program for the Office of Energy Efficiency and Renewable Energy; Laboratory Directed Research and Development Program (LDRD) of ORNL; Office of Naval Research FX This research at Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725, was sponsored by the Vehicle Technologies Program for the Office of Energy Efficiency and Renewable Energy. The seeding algorithm was developed in earlier work sponsored by the Laboratory Directed Research and Development Program (LDRD) of ORNL. Work at Michigan State University was supported by the Office of Naval Research. NR 42 TC 2 Z9 2 U1 2 U2 105 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 J9 J POWER SOURCES JI J. Power Sources PD NOV 1 PY 2013 VL 241 BP 178 EP 185 DI 10.1016/j.jpowsour.2013.04.096 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 200TL UT WOS:000323093700022 ER PT J AU Suss, ME Baumann, TF Worsley, MA Rose, KA Jaramillo, TF Stadermann, M Santiago, JG AF Suss, Matthew E. Baumann, Theodore F. Worsley, Marcus A. Rose, Klint A. Jaramillo, Thomas F. Stadermann, Michael Santiago, Juan G. TI Impedance-based study of capacitive porous carbon electrodes with hierarchical and bimodal porosity SO JOURNAL OF POWER SOURCES LA English DT Article DE Energy storage; Carbon aerogel; Supercapacitor; Capacitive deionization; Electrochemical impedance spectroscopy; Hierarchical carbon ID ELECTROCHEMICAL CAPACITORS; CONCENTRATION POLARIZATION; RATE CAPABILITY; WATER; SUPERCAPACITORS; DESALINATION; DEIONIZATION; SPECTROSCOPY; PROPAGATION; ENERGY AB Porous electrode capacitors are used extensively in systems which store energy, harvest mixing energy, or desalinate water. These electrodes can possess a hierarchical pore structure with larger macroscale pores allowing for facile ion and fluid transport, and smaller, nanometer-scale pores enabling significant ion storage. We here present a combined theoretical (linear circuit model) and experimental (electrochemical impedance spectroscopy) study of porous carbon electrode capacitors which integrate nanoscale pores into a micron-scale porous network. Our experiments are performed on a set of custom-fabricated hierarchical carbon aerogel electrodes with varying pore structure, including electrodes with sub-nanometer (sub-nm) pores. Our combined theory and experimental approach allows us to demonstrate the utility of our model, perform detailed characterizations of our electrodes, study the effects of pore structure variations on impedance, and propose hierarchical electrode design and characterization guidelines. Further, we demonstrate that our approach is promising toward the detailed study of ion storage mechanisms in sub-nm pores. (C) 2013 Elsevier B.V. All rights reserved. C1 [Suss, Matthew E.; Santiago, Juan G.] Stanford Univ, Dept Mech Engn, Stanford, CA 94305 USA. [Suss, Matthew E.; Baumann, Theodore F.; Worsley, Marcus A.; Rose, Klint A.; Stadermann, Michael] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Jaramillo, Thomas F.] Stanford Univ, Dept Chem Engn, Stanford, CA 94305 USA. RP Stadermann, M (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM stadermann2@llnl.gov; juan.santiago@stanford.edu RI Jaramillo, Thomas/C-4174-2014; Worsley, Marcus/G-2382-2014 OI Jaramillo, Thomas/0000-0001-9900-0622; Worsley, Marcus/0000-0002-8012-7727 FU National Science Foundation [0967600]; State of California's Proposition 50 funds; Natural Sciences and Engineering Research Council (NSERC) of Canada; US DOE by LLNL [DE-AC52-07NA27344] FX This work was supported by the National Science Foundation under grant no. 0967600 and State of California's Proposition 50 funds administered by the Department of Water Resources. Any opinions, findings, and conclusions or recommendations expressed in this material are those of the authors and do not necessarily reflect the views of the National Science Foundation. MES would like to thank the Lawrence Scholar program and a postgraduate scholarship from the Natural Sciences and Engineering Research Council (NSERC) of Canada. Work at LLNL was performed under the auspices of the US DOE by LLNL under Contract DE-AC52-07NA27344. We would like to thank Kendra Kuhl, Benjamin Reinecke, Zhebo Chen, and Etosha Cave for their training and technical assistance in the use of three-electrode cells and the potentiostat. NR 42 TC 21 Z9 21 U1 8 U2 185 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD NOV 1 PY 2013 VL 241 BP 266 EP 273 DI 10.1016/j.jpowsour.2013.03.178 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 200TL UT WOS:000323093700034 ER PT J AU He, QP Joy, DC Keffer, DJ AF He, Qianping Joy, David C. Keffer, David J. TI Nanoparticle adhesion in proton exchange membrane fuel cell electrodes SO JOURNAL OF POWER SOURCES LA English DT Article DE Nanoparticle adhesion; PEM fuel cell; Carbon supported platinum catalyst; Catalyst deactivation; Nafion ID MOLECULAR-DYNAMICS SIMULATION; DOPED CARBON NANOTUBES; SURFACE-AREA LOSS; PHOSPHORIC-ACID; PLATINUM NANOPARTICLES; CATALYST DEGRADATION; NAFION; DURABILITY; ELECTROCATALYSTS; WATER AB Carbon supported platinum (Pt/C) catalyst remains among the most preferable catalyst materials for Proton Exchange Membrane (PEM) fuel cells. However, platinum (Pt) particles suffer from poor durability and encounter electrochemical surface area (ESA) loss under operation with the accompany of Pt nanoparticle coarsening. Several proposed mechanisms have involved the Pt detachment from its carbonate support as an initial step for the deactivation of Pt nanoparticles. In this study, we investigated the detachment mechanism from the nano-adhesion point of view. Classic molecular dynamics simulations are performed on systems contain Pt nanoparticles of different sizes and shapes. A thin Nafion film (1 nm) at different hydration levels is also included in the system to study the environmental effect on nanoparticle adhesion. We found that the adhesion force strengthens as the Pt size goes up. Pt nanoparticles of tetrahedral shape exhibit relatively stronger connection with the carbon substrate due to its unique 'anchor-like' structure. Adhesion is enhanced with the introduction of a Nafion. The humidity level in the Nafion film has a rather complicated effect on the strength of nanoparticle adhesion. The binding energies and maximum adhesive forces are reported for all systems studied. (C) 2013 Elsevier B.V. All rights reserved. C1 [He, Qianping] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. [Joy, David C.; Keffer, David J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Joy, David C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37830 USA. RP Keffer, DJ (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM dkeffer@utk.edu RI Keffer, David/C-5133-2014 OI Keffer, David/0000-0002-6246-0286 FU Sustainable Energy and Education Research Center at the University of Tennessee; National Science Foundation [DGE-0801470]; US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; NSF [OCI 07-11134.5] FX This research was supported by the Sustainable Energy and Education Research Center at the University of Tennessee, by a grant from the National Science Foundation (DGE-0801470) and by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. This research project used resources of the National Institute for Computational Sciences (NICS) supported by NSF under agreement number: OCI 07-11134.5. NR 79 TC 11 Z9 13 U1 6 U2 100 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 J9 J POWER SOURCES JI J. Power Sources PD NOV 1 PY 2013 VL 241 BP 634 EP 646 DI 10.1016/j.jpowsour.2013.05.011 PG 13 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 200TL UT WOS:000323093700082 ER PT J AU Zerovnik, G Trkov, A Smith, DL Capote, R AF Zerovnik, Gasper Trkov, Andrej Smith, Donald L. Capote, Roberto TI Transformation of correlation coefficients between normal and lognormal distribution and implications for nuclear applications SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Multivariate normal distribution; Multivariate lognormal distribution; Correlation matrix; Evaluated nuclear data formats ID UNIFIED MONTE-CARLO AB Inherently positive parameters with large relative uncertainties (typically greater than or similar to 300) are often considered to be governed by the lognormal distribution. This assumption has the practical benefit of avoiding the possibility of sampling negative values in stochastic applications. Furthermore, it is typically assumed that the correlation coefficients for comparable multivariate normal and lognormal distributions are equivalent. However, this ideal situation is approached only in the linear approximation which happens to be applicable just for small uncertainties. This paper derives and discusses the proper transformation of correlation coefficients between both distributions for the most general case which is applicable for arbitrary uncertainties. It is seen that for lognormal distributions with large relative uncertainties strong anti-correlations (negative correlations) are mathematically forbidden. This is due to the asymmetry that is an inherent feature of these distributions. Some implications of these results for practical nuclear applications are discussed and they are illustrated with examples in this paper. Finally, modifications to the ENDF-6 format used for representing uncertainties in evaluated nuclear data libraries are suggested, as needed to deal with this issue. (C) 2013 Elsevier B.V. All rights reserved. C1 [Zerovnik, Gasper; Trkov, Andrej] Jozef Stefan Inst, SI-1000 Ljubljana, Slovenia. [Smith, Donald L.] Argonne Natl Lab, Coronado, CA 92118 USA. [Capote, Roberto] IAEA, NAPC Nucl Data Sect, A-1400 Vienna, Austria. RP Zerovnik, G (reprint author), Jozef Stefan Inst, Jamova Cesta 39, SI-1000 Ljubljana, Slovenia. EM gasper.zerovnik@ijs.si; andrej.trkov@ijs.si; donald.l.smith@anl.gov; roberto.capotenoy@iaea.org RI Capote Noy, Roberto/M-1245-2014 OI Capote Noy, Roberto/0000-0002-1799-3438 NR 11 TC 8 Z9 8 U1 0 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD NOV 1 PY 2013 VL 727 BP 33 EP 39 DI 10.1016/j.nima.2013.06.025 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 206WY UT WOS:000323557700006 ER PT J AU Best, A Couder, M Famiano, M Lemut, A Wiescher, M AF Best, Andreas Couder, Manoel Famiano, Michael Lemut, Alberto Wiescher, Michael TI Study of the beam-induced neutron flux and required shielding for DIANA SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Neutron shielding; Monte Carlo simulation; Underground laboratory ID GEANT4 AB Low energy accelerators in underground locations have emerged as a powerful tool for the measurement of critical nuclear reactions for the study of energy production and element synthesis in astrophysics. While cosmic ray induced background is substantially reduced, beam induced background on target impurities and depositions on target and collimator materials remain a matter of serious concern. The Dual Ion Accelerator for Nuclear Astrophysics (DIANA) is proposed to operate as a low-level background facility in an underground location. One of the main goals of DIANA is the study of neutron sources in stellar helium burning. For these experiments DIANA is a neutron radiation source which may affect other nearby low background level experiments. We therefore investigated the required laboratory layout to attenuate the neutron flux generated in a worst-case scenario to a level below the natural background in the underground environment. Detailed Monte Carlo calculations of the neutron propagation in the laboratory show that a neutron flux many orders of magnitude above expected values gets attenuated below the natural background rate using a 1 m thick water-shielded door as well as an emergency access/egress maze. (C) 2013 Elsevier B.V. All rights reserved. C1 [Best, Andreas; Couder, Manoel; Wiescher, Michael] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Best, Andreas; Couder, Manoel; Wiescher, Michael] Univ Notre Dame, Joint Inst Nucl Astrophys, Notre Dame, IN 46556 USA. [Best, Andreas; Lemut, Alberto] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Famiano, Michael] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA. RP Best, A (reprint author), Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. EM abest1@nd.edu RI Couder, Manoel/B-1439-2009; OI Couder, Manoel/0000-0002-0636-744X; Best, Andreas/0000-0001-8869-9757 FU National Science Foundation [PHY-0918728]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Building Technology, State, and Community Programs, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the National Science Foundation through Grant number PHY-0918728. This work was also supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract no. DE-AC02-05CH11231 and by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Building Technology, State, and Community Programs, of the U.S. Department of Energy under Contract no. DE-AC02-05CH11231. NR 28 TC 5 Z9 5 U1 0 U2 29 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD NOV 1 PY 2013 VL 727 BP 104 EP 108 DI 10.1016/j.nima.2013.06.032 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 206WY UT WOS:000323557700016 ER PT J AU Gidalevitz, T Stevens, F Argon, Y AF Gidalevitz, Tali Stevens, Fred Argon, Yair TI Orchestration of secretory protein folding by ER chaperones SO BIOCHIMICA ET BIOPHYSICA ACTA-MOLECULAR CELL RESEARCH LA English DT Review DE Endoplasmic reticulum; Chaperones; Protein folding; Secretome ID ENDOPLASMIC-RETICULUM CHAPERONES; DISULFIDE BOND FORMATION; VIRUS-G PROTEIN; MHC CLASS-I; PHOSPHATIDYLSERINE-CONTAINING MEMBRANES; NEMATODE CAENORHABDITIS-ELEGANS; HUMAN CHORIONIC-GONADOTROPIN; NUCLEOTIDE EXCHANGE FACTOR; MARINESCO-SJOGREN-SYNDROME; NEWLY SYNTHESIZED PROTEINS AB The endoplasmic reticulum is a major compartment of protein biogenesis in the cell, dedicated to production of secretory, membrane and organelle proteins. The secretome has distinct structural and post-translational characteristics, since folding in the ER occurs in an environment that is distinct in terms of its ionic composition, dynamics and requirements for quality control. The folding machinery in the ER therefore includes chaperones and folding enzymes that introduce, monitor and react to disulfide bonds, glycans, and fluctuations of luminal calcium. We describe the major chaperone networks in the lumen and discuss how they have distinct modes of operation that enable cells to accomplish highly efficient production of the secretome. This article is part of a Special Issue entitled: Functional and structural diversity of endoplasmic reticulum. (c) 2013 Elsevier B.V. All rights reserved. C1 [Gidalevitz, Tali] Drexel Univ, Dept Biol, Philadelphia, PA 19104 USA. [Stevens, Fred] Argonne Natl Lab, Argonne, IL 60439 USA. [Argon, Yair] Childrens Hosp Philadelphia, Dept Pathol & Lab Med, Div Cell Pathol, Philadelphia, PA 19104 USA. [Argon, Yair] Univ Penn, Philadelphia, PA 19104 USA. RP Argon, Y (reprint author), Childrens Hosp Philadelphia, Dept Pathol & Lab Med, Div Cell Pathol, 3615 Civ Ctr Blvd, Philadelphia, PA 19104 USA. EM yargon@mail.med.upenn.edu RI Gidalevitz, Tali/C-9217-2009 FU NIH [AG18001, GM07748] FX We thank Drs. J. Brodsky (Univ. Pitt.), E. Snapp (Albert Einstein College of Medicine), M. Molinari (Institute for Research in Biomedicine, Bellinzona, Switserland), P. Cresswell (Yale Univ.) and D. Hebert (Univ. Mass.) for helpful comments and personal communications. Work in the authors' lab was supported by NIH grants AG18001 and GM07748. NR 241 TC 37 Z9 39 U1 3 U2 60 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-4889 EI 0006-3002 J9 BBA-MOL CELL RES JI Biochim. Biophys. Acta-Mol. Cell Res. PD NOV PY 2013 VL 1833 IS 11 SI SI BP 2410 EP 2424 DI 10.1016/j.bbamcr.2013.03.007 PG 15 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA 204VS UT WOS:000323400000004 PM 23507200 ER PT J AU Givens, GH Beveridge, JR Phillips, PJ Draper, B Lui, YM Bolme, D AF Givens, G. H. Beveridge, J. R. Phillips, P. J. Draper, B. Lui, Y. M. Bolme, D. TI Introduction to face recognition and evaluation of algorithm performance SO COMPUTATIONAL STATISTICS & DATA ANALYSIS LA English DT Article DE Face recognition; Biometrics; Computer vision; Generalized linear mixed model; GLMM ID LINEAR MIXED MODELS; GRAND CHALLENGE; DISCRIMINANT-ANALYSIS; LIKELIHOOD; INFERENCE; FEATURES; IMAGES; SYSTEM AB The field of biometric face recognition blends methods from computer science, engineering and statistics, however statistical reasoning has been applied predominantly in the design of recognition algorithms. A new opportunity for the application of statistical methods is driven by growing interest in biometric performance evaluation. Methods for performance evaluation seek to identify, compare and interpret how characteristics of subjects, the environment and images are associated with the performance of recognition algorithms. Some central topics in face recognition are reviewed for background and several examples of recognition algorithms are given. One approach to the evaluation problem is then illustrated with a generalized linear mixed model analysis of the Good, Bad, and Ugly Face Challenge, a pre-eminent face recognition dataset used to test state-of-the-art still-image face recognition algorithms. Findings include that (i) between-subject variation is the dominant source of verification heterogeneity when algorithm performance is good, and (ii) many covariate effects on verification performance are 'universal' across easy, medium and hard verification tasks. Although the design and evaluation of face recognition algorithms draw upon some familiar statistical ideas in multivariate statistics, dimension reduction, classification, clustering, binary response data, generalized linear models and random effects, the field also presents some unique features and challenges. Opportunities abound for innovative statistical work in this new field. (C) 2013 Elsevier B.V. All rights reserved. C1 [Givens, G. H.] Colorado State Univ, Dept Stat, Ft Collins, CO 80523 USA. [Beveridge, J. R.; Draper, B.; Lui, Y. M.] Colorado State Univ, Dept Comp Sci, Ft Collins, CO 80523 USA. [Phillips, P. J.] NIST, Gaithersburg, MD 20899 USA. [Bolme, D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Givens, GH (reprint author), Colorado State Univ, Dept Stat, Ft Collins, CO 80523 USA. EM geof@lamar.colostate.edu FU Technical Support Working Group (TSWG) [SC-AS-3181C]; Federal Bureau of Investigation (FBI) FX This work was supported by the Technical Support Working Group (TSWG) under Task SC-AS-3181C. P. Jonathon Phillips thanks the Federal Bureau of Investigation (FBI) for their support of this work. The identification of any commercial product or trade name does not imply endorsement or recommendation by Colorado State University and the National Institute of Standards. NR 46 TC 12 Z9 13 U1 0 U2 57 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-9473 J9 COMPUT STAT DATA AN JI Comput. Stat. Data Anal. PD NOV PY 2013 VL 67 BP 236 EP 247 DI 10.1016/j.csda.2013.05.025 PG 12 WC Computer Science, Interdisciplinary Applications; Statistics & Probability SC Computer Science; Mathematics GA 203MJ UT WOS:000323297000018 ER PT J AU Wu, X Baker, I Miller, MK More, KL Cai, Z Chen, S AF Wu, X. Baker, I. Miller, M. K. More, K. L. Cai, Z. Chen, S. TI Microstructure and mechanical properties of two-phase Fe30Ni20Mn20Al30. Part I: Microstructure SO JOURNAL OF MATERIALS SCIENCE LA English DT Article ID LONG-RANGE ORDER; COMPOSITION DEPENDENCE; MODULATED STRUCTURE; YOUNG MODULUS; ALLOY; TEMPERATURE; PRECIPITATION; STRENGTH; PHASE; FE35NI15MN25AL25 AB The microstructure of Fe30Ni20Mn20Al30 in both the as-cast condition and after annealing at 823 K for various times up to 72 h was characterized using transmission electron microscopy, scanning transmission electron microscopy, synchrotron-based X-ray diffraction, and atom probe tomography. The microstructure exhibited a basketweave morphology of (Mn, Fe)-rich B2-ordered (ordered b.c.c.) and (Ni, Al)-rich L2(1)-ordered (Heusler type) phases with a lattice misfit of only 0.85 % and interfaces aligned along aOE (c) 100 >. The phase width increased from 5 nm for the as-cast alloy to 25 nm for 72 h annealed material, with no change in the elemental partitioning between the phases, with a time exponent for the coarsening kinetics of 0.19. Surprisingly, it was found that the room temperature hardness was largely independent of the phase width. C1 [Wu, X.; Baker, I.] Dartmouth Coll, Thayer Sch Engn, Hanover, NH 03755 USA. [Miller, M. K.; More, K. L.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Cai, Z.; Chen, S.] Argonne Natl Lab, Adv Photon Source, X Ray Sci Div, Argonne, IL 60439 USA. RP Baker, I (reprint author), Dartmouth Coll, Thayer Sch Engn, Hanover, NH 03755 USA. EM ian.baker@dartmouth.edu RI More, Karren/A-8097-2016 OI More, Karren/0000-0001-5223-9097 FU US Department of Energy (DOE), Office of Basic Energy Sciences [DE-FG02-07ER46392]; ORNL's ShaRE User Facility; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. DOE [DE-AC02-06CH11357] FX This research was supported by the US Department of Energy (DOE), Office of Basic Energy Sciences grant DE-FG02-07ER46392 (X. W and I. B). Research was supported ORNL's ShaRE User Facility, which is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (M. K. M. and K. L. M.). Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357 (Z. C. and S. C.). The authors gratefully acknowledge K. F. Russell for technical assistance. Prof. Paul Munroe of the University of New South Wales is thanked for the electron probe microanalyzer measurements. We would also like to thanks the reviewers for their numerous useful comments. The views and conclusions contained herein are those of the authors and should not be interpreted as necessarily representing official policies, either expressed or implied of the DOE or the U.S. Government. NR 46 TC 2 Z9 2 U1 0 U2 24 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2461 EI 1573-4803 J9 J MATER SCI JI J. Mater. Sci. PD NOV PY 2013 VL 48 IS 21 BP 7435 EP 7445 DI 10.1007/s10853-013-7558-4 PG 11 WC Materials Science, Multidisciplinary SC Materials Science GA 202VW UT WOS:000323249500010 ER PT J AU Pilania, G Sharma, V AF Pilania, G. Sharma, Vinit TI First principles investigations of structural, electronic, elastic, and dielectric properties of KMgF3 SO JOURNAL OF MATERIALS SCIENCE LA English DT Article ID GENERALIZED GRADIENT APPROXIMATION; FUNCTIONAL PERTURBATION-THEORY; AB-INITIO; PEROVSKITE OXIDES; FORCE-CONSTANTS; DOPED KMGF3; CRYSTAL; IMPURITIES; PRESSURE; FLUORIDE AB An ab initio study of structural, electronic, elastic, and dielectric properties of KMgF3 in cubic perovskite structure is presented in the framework of density functional theory. The calculations presented here employ generalized gradient approximation with projector augmented wave method. The fully relaxed structural parameters are found to be in reasonable agreement with available experimental data and with previous theoretical work. The independent elastic constants of cubic KMgF3 are derived from the derivative of total energy as a function of lattice strain in full detail. The bulk modulus and its first pressure derivative are obtained by fitting total energy versus volume data to a Murnaghan equation of state. The electronic band structure, total density of states, and projected density of states on each of the K, Mg, and F atoms are calculated and found to be in good agreement with previous theoretical results. First principles computed phonon dispersions for the cubic KMgF3 are reported for the first time. The imaginary part of frequency-dependent dielectric function is determined by summing over all possible transitions from occupied to unoccupied states and taking the appropriate transition matrix element into account. The Born effective charges computed by linear response within density functional perturbation theory are used together with the mode eigenvectors to decompose the lattice dielectric susceptibility tensor into contributions arising from individual IR-active phonon modes. Our results for the static and optical dielectric constant are in good agreement with previously reported experimental results. C1 [Pilania, G.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Sharma, Vinit] Univ Connecticut, Storrs, CT 06269 USA. RP Pilania, G (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. EM gpilania@gmail.com RI Pilania, Ghanshyam/K-4468-2013; sharma, Vinit/K-3407-2015 OI Pilania, Ghanshyam/0000-0003-4460-1572; NR 46 TC 3 Z9 3 U1 3 U2 35 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2461 EI 1573-4803 J9 J MATER SCI JI J. Mater. Sci. PD NOV PY 2013 VL 48 IS 21 BP 7635 EP 7641 DI 10.1007/s10853-013-7581-5 PG 7 WC Materials Science, Multidisciplinary SC Materials Science GA 202VW UT WOS:000323249500033 ER PT J AU Romano, PK Siegel, AR Forget, B Smith, K AF Romano, Paul K. Siegel, Andrew R. Forget, Benoit Smith, Kord TI Data decomposition of Monte Carlo particle transport simulations via tally servers SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Monte Carlo; Neutron transport; Data decomposition; Exascale; Tally server ID ALGORITHMS AB An algorithm for decomposing large tally data in Monte Carlo particle transport simulations is developed, analyzed, and implemented in a continuous-energy Monte Carlo code, OpenMC. The algorithm is based on a non-overlapping decomposition of compute nodes into tracking processors and tally servers. The former are used to simulate the movement of particles through the domain while the latter continuously receive and update tally data. A performance model for this approach is developed, suggesting that, for a range of parameters relevant to LWR analysis, the tally server algorithm should perform with minimal overhead on contemporary supercomputers. An implementation of the algorithm in OpenMC is then tested on the Intrepid and Titan supercomputers, supporting the key predictions of the model over a wide range of parameters. We thus conclude that the tally server algorithm is a successful approach to circumventing classical on-node memory constraints en route to unprecedentedly detailed Monte Carlo reactor simulations. (C) 2013 Elsevier Inc. All rights reserved. C1 [Romano, Paul K.; Forget, Benoit; Smith, Kord] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA. [Siegel, Andrew R.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Romano, PK (reprint author), MIT, Dept Nucl Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM paul.k.romano@gmail.com; siegala@mcs.anl.gov; bforget@mit.edu; kord@mit.edu OI Romano, Paul/0000-0002-1147-045X FU Naval Reactors Division of the U.S Department of Energy; Office of Advanced Scientific Computing Research, Office of Science, US Department of Energy [DE-AC02-06CH11357]; Consortium for Advanced Simulation of Light Water Reactors, an Energy Innovation Hub for Modeling and Simulation of Nuclear Reactors under US Department of Energy [DE-AC05-00OR22725] FX This research was performed under appointment of the first author to the Rickover Fellowship Program in Nuclear Engineering sponsored by Naval Reactors Division of the U.S Department of Energy. This work was also supported in part by the Office of Advanced Scientific Computing Research, Office of Science, US Department of Energy, under Contract DE-AC02-06CH11357 and by the Consortium for Advanced Simulation of Light Water Reactors, an Energy Innovation Hub for Modeling and Simulation of Nuclear Reactors under US Department of Energy Contract No. DE-AC05-00OR22725. The authors would also like to thank Forrest Brown for advice and guidance regarding data decomposition. NR 17 TC 8 Z9 9 U1 1 U2 18 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 J9 J COMPUT PHYS JI J. Comput. Phys. PD NOV 1 PY 2013 VL 252 BP 20 EP 36 DI 10.1016/j.jcp.2013.06.011 PG 17 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 194KZ UT WOS:000322633500002 ER PT J AU Scovazzi, G Huang, H Collis, SS Yin, J AF Scovazzi, G. Huang, H. Collis, S. S. Yin, J. TI A fully-coupled upwind discontinuous Galerkin method for incompressible porous media flows: High-order computations of viscous fingering instabilities in complex geometry SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Viscous fingering; Discontinuous Galerkin method; Porous media flows ID MISCIBLE DISPLACEMENT PROBLEMS; QUARTER 5-SPOT CONFIGURATION; REACTIVE TRANSPORT PROBLEMS; LINEAR-STABILITY ANALYSIS; IMMISCIBLE 2-PHASE FLOW; FINITE-ELEMENT METHODS; ELLIPTIC PROBLEMS; PERMEABILITY HETEROGENEITY; NUMERICAL-SIMULATION; DARCY FLOW AB We present a new approach to the simulation of viscous fingering instabilities in incompressible, miscible displacement flows in porous media. In the past, high resolution computational simulations of viscous fingering instabilities have always been performed using high-order finite difference or Fourier-spectral methods which do not posses the flexibility to compute very complex subsurface geometries. Our approach, instead, by means of a fully-coupled nonlinear implementation of the discontinuous Galerkin method, possesses a fundamental differentiating feature, in that it maintains high-order accuracy on fully unstructured meshes. In addition, the proposed method shows very low sensitivity to mesh orientation, in contrast with classical finite volume approximation used in porous media flow simulations. The robustness and accuracy of the method are demonstrated in a number of challenging computational problems. (C) 2013 Elsevier Inc. All rights reserved. C1 [Scovazzi, G.] Duke Univ, Dept Civil & Environm Engn, Durham, NC 27708 USA. [Huang, H.; Yin, J.] ExxonMobil Upstream Res Co, Houston, TX 77252 USA. [Collis, S. S.] Sandia Natl Labs, Numer Anal & Applicat Dept, Albuquerque, NM 87185 USA. RP Scovazzi, G (reprint author), Duke Univ, Dept Civil & Environm Engn, Room 121,Hudson Hall,POB 90287, Durham, NC 27708 USA. EM guglielmo.scovazzi@duke.edu RI Huang, Hao/A-1376-2012; OI Huang, Hao/0000-0002-5186-180X; Yin, Jichao/0000-0003-0311-9392 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 57 TC 5 Z9 5 U1 2 U2 37 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD NOV 1 PY 2013 VL 252 BP 86 EP 108 DI 10.1016/j.jcp.2013.06.012 PG 23 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 194KZ UT WOS:000322633500006 ER PT J AU Arazi, A Pendergraft, WF Ribeiro, RM Perelson, AS Hacohen, N AF Arazi, Arnon Pendergraft, William F., III Ribeiro, Ruy M. Perelson, Alan S. Hacohen, Nir TI Human systems immunology: Hypothesis-based modeling and unbiased data-driven approaches SO SEMINARS IN IMMUNOLOGY LA English DT Review DE Systems immunology; Hypothesis-based modeling; Unbiased data-driven approaches; Dynamical modeling; Viral infections; Autoimmunity ID HEPATITIS-C VIRUS; T-CELL VACCINATION; DYNAMICS IN-VIVO; GENE-EXPRESSION PROFILES; IMMUNODEFICIENCY-VIRUS; HIV-1 INFECTION; MULTIPLE-SCLEROSIS; INSULIN SENSITIVITY; IMMUNE-SYSTEM; ANTIRETROVIRAL THERAPY AB Systems immunology is an emerging paradigm that aims at a more systematic and quantitative understanding of the immune system. Two major approaches have been utilized to date in this field: unbiased data-driven modeling to comprehensively identify molecular and cellular components of a system and their interactions; and hypothesis-based quantitative modeling to understand the operating principles of a system by extracting a minimal set of variables and rules underlying them. In this review, we describe applications of the two approaches to the study of viral infections and autoimmune diseases in humans, and discuss possible ways by which these two approaches can synergize when applied to human immunology. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Pendergraft, William F., III; Hacohen, Nir] Massachusetts Gen Hosp, Ctr Immunol & Inflammatory Dis, Charlestown, MA 02129 USA. [Arazi, Arnon; Pendergraft, William F., III; Hacohen, Nir] Broad Inst MIT & Harvard, Cambridge Ctr 7, Cambridge, MA 02142 USA. [Pendergraft, William F., III; Hacohen, Nir] Harvard Univ, Sch Med, Dept Med, Boston, MA 02115 USA. [Pendergraft, William F., III] Massachusetts Gen Hosp, Dept Med, Div Nephrol, Boston, MA 02114 USA. [Ribeiro, Ruy M.; Perelson, Alan S.] Los Alamos Natl Lab, Theoret Biol & Biophys Grp, Los Alamos, NM 87545 USA. RP Perelson, AS (reprint author), Los Alamos Natl Lab, Theoret Biol & Biophys Grp, MS-K710, Los Alamos, NM 87545 USA. EM arnonar@broadinstitute.org; wpendergraft@partners.org; ruy@lanl.gov; asp@lanl.gov; nhacohen@partners.org OI Ribeiro, Ruy/0000-0002-3988-8241 FU U.S. Department of Energy [DE-AC52-06NA25396]; NIH [AI028433, OD011095, P20-RR018754, HHSN272201000055C]; New Innovator Award [OD002230, P50 HG006193, GM093080]; Foundation for Science and Technology of Portugal [PCOFUND-GA-2009-246542]; American Society of Nephrology FX Portions of this work were done under the auspices of the U.S. Department of Energy under contract DE-AC52-06NA25396 (AP) and supported by NIH grants AI028433 (AP), OD011095 (AP), P20-RR018754 (APRMR), New Innovator Award DP2 OD002230 (NH), P50 HG006193 (NH), GM093080 (NH), and NIH contract HHSN272201000055C (AP). RMR received partial funding from the Foundation for Science and Technology of Portugal (PCOFUND-GA-2009-246542). WFPIII is supported by a research fellowship from the American Society of Nephrology. NR 115 TC 9 Z9 9 U1 3 U2 9 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 1044-5323 J9 SEMIN IMMUNOL JI Semin. Immunol. PD OCT 31 PY 2013 VL 25 IS 3 BP 193 EP 200 DI 10.1016/j.smim.2012.11.003 PG 8 WC Immunology SC Immunology GA 257WS UT WOS:000327419100002 PM 23375135 ER PT J AU Polizos, G Vaia, RA Koerner, H Manias, E AF Polizos, Georgios Vaia, Richard A. Koerner, Hilmar Manias, Evangelos TI Dynamics of Amphiphilic Surfactants Confined in Montmorillonite Slits with Different Cation Exchange Capacities SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID LOW-FREQUENCY DISPERSION; POLYMER/LAYERED SILICATE NANOCOMPOSITES; POLYMER-CLAY NANOCOMPOSITES; MODIFIED LAYERED SILICATES; VITREOUS IONIC CONDUCTORS; DIELECTRIC-RELAXATION; MOLECULAR-DYNAMICS; ELECTRICAL-CONDUCTIVITY; COMPUTER-SIMULATION; COLLOIDAL PARTICLES AB Alkylammonium surfactants were nanoscopically confined between montmorillonite layers of varied negative surface charge, i.e., of varied cation exchange capacities. Dielectric relaxation spectroscopy was employed to probe the interfacial dynamics, arising from the mobility of the cations on the silicate surfaces, as a function of the confining walls' surface charge. Standard methods to dry the organo-silicates were employed; however, water was still detected physisorbed in the galleries; the dynamics of these water molecules were also detected and were found to be coupled with the dynamics of the ammoniums at high temperatures. A transition in the mobility of the cations, approximately at 75 degrees C (which is in good agreement with the conformational changes of the alkyl groups, reported in the literature), is observed, and a model is proposed on the basis of the dynamics of the confined water. Entropic contributions arising from variation in the surface charge density are also discussed in detail. The existence of water in the interlayer-in spite of drying the nanofillers in accordance to industrial practices and the interrelated surfactant/water dynamics bring forward important implications for the design and processing of polymer-based nanocomposites based on these fillers. C1 [Polizos, Georgios] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Vaia, Richard A.; Koerner, Hilmar; Manias, Evangelos] Mat & Mfg Directorate, Air Force Res Lab, Wright Patterson AFB, OH 45433 USA. [Polizos, Georgios; Manias, Evangelos] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. RP Polizos, G (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM polyzosg@ornl.gov; manias@psu.edu RI Manias, Evangelos/A-7557-2011 FU National Science Foundation [DMR-0602877]; US Air Force SFFP fellowship; U.S. Department of Energy, Office of Electricity Delivery and Energy Reliability - Power Electronics Program; U.S. Department of Energy [DE-AC05-00OR22725] FX This work was supported by the National Science Foundation (MWN grant, NSF Grant No. DMR-0602877); E.M.'s stay in AFRL was supported through an US Air Force SFFP fellowship, administered through NRC. Work was also supported by the U.S. Department of Energy, Office of Electricity Delivery and Energy Reliability - Power Electronics Program. Oak Ridge National Laboratory is operated for the U.S. Department of Energy by U.T.-Battelle under Contract No. DE-AC05-00OR22725. NR 99 TC 4 Z9 4 U1 0 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 EI 1520-5207 J9 J PHYS CHEM B JI J. Phys. Chem. B PD OCT 31 PY 2013 VL 117 IS 43 BP 13667 EP 13678 DI 10.1021/jp4067845 PG 12 WC Chemistry, Physical SC Chemistry GA 247HM UT WOS:000326608500031 PM 24083909 ER PT J AU Chen, HA Hsin, CL Huang, YT Tang, ML Dhuey, S Cabrini, S Wu, WW Leone, SR AF Chen, Hsiang-An Hsin, Cheng-Lun Huang, Yu-Ting Tang, Ming Lee Dhuey, Scott Cabrini, Stefano Wu, Wen-Wei Leone, Stephen R. TI Measurement of Interlayer Screening Length of Layered Graphene by Plasmonic Nanostructure Resonances SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SILVER NANOPARTICLES; RAMAN-SCATTERING; FILMS; SPECTROSCOPY; SUBSTRATE; DEVICES; SIO2 AB The variation in localized surface plasmon resonances of single Au nanodisks (diameter 100 nm and height 25 nm) on 0-13 graphene layers is investigated using dark-field scattering spectroscopy to obtain the graphene electric field screening length. For nanodisks (NDs) with and without underlying graphene layers on a SiO2 (300 nm)/Si substrate, the plasmon resonance red shifts from 604 to 620 nm with increasing graphene layers. The spectra of the plasmonic nanostructures obey an exponential saturation function versus increasing number of layers of graphene from 0 to 13. As a conducting film, the graphene layers screen the electric field generated by the plasmonic resonance of the Au NDs in the vicinity of the interface, and the red shifts of the resonance wavelength are explained in the framework of the electromagnetic field coupling between in-plane antiparallel image dipoles in the graphene layers and the ND dipole. A screening length of 1.2 +/- 0.2 nm, equivalent to 3-4 graphene layers, is experimentally obtained, in good agreement with the measurement by field-effect transistors and theoretical calculation in doped graphene. The resonance shift of plasmonic nanostructures on a layered graphene system provides an alternative and convenient method for screening length measurement of graphene films. C1 [Chen, Hsiang-An; Tang, Ming Lee; Leone, Stephen R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Hsin, Cheng-Lun] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Leone, Stephen R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Hsin, Cheng-Lun] Natl Cent Univ, Dept Elect Engn, Tao Yuan 32001, Taiwan. [Huang, Yu-Ting; Wu, Wen-Wei] Natl Chiao Tung Univ, Dept Mat Sci & Engn, Hsinchu 30010, Taiwan. [Dhuey, Scott; Cabrini, Stefano] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Leone, Stephen R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Leone, SR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM srl@berkeley.edu RI Foundry, Molecular/G-9968-2014 FU National Security Science and Engineering Faculty Fellowship; Air Force Office of Scientific Research [AFOSR-NSSEFF-FA9550-10-1-0195]; postdoctoral research abroad program; National Science Council, Taiwan [NSC100-2917-I-564-056, NCS 101-2218-E-008-014-MY2, NSC 100-2628-E-009-023-MY3]; Office of Science, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors acknowledge Sarah Brittman for technical assistance and Terefe G. Habteyes for valuable discussions. This work is supported by a National Security Science and Engineering Faculty Fellowship, Air Force Office of Scientific Research under Grant No. AFOSR-NSSEFF-FA9550-10-1-0195, and postdoctoral research abroad program, National Science Council, Taiwan, under Contract No. NSC100-2917-I-564-056. Supplies and equipment are provided through the Materials Science Division (MSD) and Molecular Foundry, Lawrence Berkeley National Laboratory (LBNL), through support of the Director, Office of Science, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Portions of the experimental supplies are provided by Cheng-Lun Hsin and Wen-Wei Wu under National Science Council, Taiwan, Grant No. NCS 101-2218-E-008-014-MY2 and No. NSC 100-2628-E-009-023-MY3, respectively. NR 38 TC 9 Z9 9 U1 2 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 EI 1932-7455 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 31 PY 2013 VL 117 IS 43 BP 22211 EP 22217 DI 10.1021/jp312363x PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 247HJ UT WOS:000326608200007 ER PT J AU Lawton, TJ Pushkarev, V Wei, D Lucci, FR Sholl, DS Gellman, AJ Sykes, ECH AF Lawton, T. J. Pushkarev, V. Wei, D. Lucci, F. R. Sholl, D. S. Gellman, A. J. Sykes, E. C. H. TI Long Range Chiral Imprinting of Cu(110) by Tartaric Acid SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ENANTIOSELECTIVE HETEROGENEOUS CATALYSIS; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; DIRECT STM EVIDENCE; WAVE BASIS-SET; METAL-SURFACES; ASYMMETRIC HYDROGENATION; (R,R)-TARTARIC ACID; ORGANIC-MOLECULES; FUNDAMENTAL INVESTIGATIONS AB Restructuring of metals by chiral molecules represents an important route to inducing and controlling enantioselective surface chemistry. Tartaric acid adsorption on Cu(110) has served as a useful system for understanding many aspects of chiral molecule adsorption and ordering on a metal surface, and a number of chiral and achiral unit cells have been reported. Herein, we show that given the appropriate annealing treatment, singly deprotonated tartaric acid monolayers can restructure the Cu metal itself, and that the resulting structure is both highly ordered and chiral. Molecular resolution scanning tunneling microscopy reveals that singly deprotonated tartaric acid extracts Cu atoms from the Cu(110) surface layer and incorporates them into highly ordered, chiral adatom arrays capped by a continuous molecular layer. Further evidence for surface restructuring comes from images of atom-deep trenches formed in the Cu(110) surface during the process. These trenches also run in low symmetry directions and are themselves chiral. Simulated scanning tunneling microscopy images are consistent with the appearance of the added atom rows and etched trenches. The chiral imprinting results in a long-range, highly ordered ((2)(6) (-1)(7)) unit cell covering the whole surface as confirmed by low energy electron diffraction. Details of the restructuring mechanism were further investigated via time-lapse imaging at elevated temperature. This work reveals the stages of nanoscale surface restructuring and offers an interesting method for chiral modification of an achiral metal surface. C1 [Lawton, T. J.; Lucci, F. R.; Sykes, E. C. H.] Tufts Univ, Dept Chem, Medford, MA 02155 USA. [Pushkarev, V.; Gellman, A. J.] Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA. [Wei, D.; Sholl, D. S.] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA. [Gellman, A. J.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Sykes, ECH (reprint author), 62 Talbot Ave, Medford, MA 02155 USA. EM charles.sykes@tufts.edu RI Gellman, Andrew/M-2487-2014 OI Gellman, Andrew/0000-0001-6618-7427 FU National Science Foundation [CHE-1012358, CHE-1012307, CHE-1012524] FX This work has been supported by the National Science Foundation through a collaborative grant CHE-1012358 (V.P., A.J.G.), CHE-1012307 (T.J.L., E.C.H.S.) and CHE-1012524 (D.W., D.S.S.). NR 71 TC 20 Z9 20 U1 3 U2 77 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 EI 1932-7455 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 31 PY 2013 VL 117 IS 43 BP 22290 EP 22297 DI 10.1021/jp402015r PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 247HJ UT WOS:000326608200018 ER PT J AU Rosenberg, RA Symonds, JM Kalyanaraman, V Markus, T Orlando, TM Naaman, R Medina, EA Lopez, FA Mujica, V AF Rosenberg, Richard A. Symonds, Joshua M. Kalyanaraman, Vijayalakshmi Markus, Tal Orlando, Thomas M. Naaman, Ron Medina, Ernesto A. Lopez, Floralba A. Mujica, Vladimiro TI Kinetic Energy Dependence of Spin Filtering of Electrons Transmitted through Organized Layers of DNA SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PHOTOELECTRON-SPECTROSCOPY; FILMS; TRANSMISSION; MONOLAYERS AB We present an experimental and theoretical study of the kinetic energy dependence of spin filtering of electrons by organized layers of DNA adsorbed on a gold substrate. When Au 4f(7/2,5/2) levels are ionized by circularly polarized X-rays, the emitted electrons will be spin polarized. The spin distribution depends on the particular sublevel and is opposite for right versus left circularly polarized light. If the DNA overlayer preferentially attenuates one spin over another, then there should be a circular dichroism (CD) in the X-ray photoelectron spectroscopy (XPS) spectra observed with the different polarizations. Using synchrotron radiation excitation, XPS CD measurements were made of electrons with kinetic energies in the range 30 to 760 eV. In all cases there was no evidence of any significant dichroism. These results are explained by a model in which the longitudinal polarization is strongly dependent on the k-vector, and hence the energy or the wavelength, which are simply connected to the magnitude of this vector of the incoming electrons. For a helix with a fixed number of turns, this dependence is due to a coherent process associated with multiple scattering. This model predicts that there is a window of energies where changes in the polarization should be expected. Two competing effects determine this window: The energy has to be small enough to allow for at least double scattering, but large enough so that the de Broglie wavelength probes the chiral structure. Also at very low energies the spin-orbit interaction weakens and no polarization results. C1 [Rosenberg, Richard A.; Kalyanaraman, Vijayalakshmi] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Symonds, Joshua M.; Orlando, Thomas M.] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA. [Symonds, Joshua M.; Orlando, Thomas M.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Markus, Tal; Naaman, Ron] Weizmann Inst Sci, Dept Chem Phys, IL-76100 Rehovot, Israel. [Medina, Ernesto A.] Inst Venezolano Invest Cient, Ctr Fis, Lab Fis Estadist Sist Desordenados, Caracas 1020A, Venezuela. [Lopez, Floralba A.] Univ Los Andes, Dept Quim, Quimicofis Fluidos & Fenomenos Interfaci QUIFFIS, Merida 5101, Venezuela. [Mujica, Vladimiro] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Mujica, Vladimiro] Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA. [Mujica, Vladimiro] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Rosenberg, RA (reprint author), Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Argonne, IL 60439 USA. EM rar@aps.anl.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; National Science Foundation [DMR-0537588]; NSF [NSF CHE-1124895]; U.S. Department of Energy, Office of Science [DE-FG02-02ER15337]; Nir Eliyahu FX The work performed at the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. This work is based in part upon research conducted at the Synchrotron Radiation Center, University of Wisconsin Madison, which is supported by the National Science Foundation under Award No. DMR-0537588. V.M. acknowledges the support of NSF through Award No. NSF CHE-1124895. T.M.O. and J.M.S. wish to acknowledge support from the U.S. Department of Energy, Office of Science, Contract No. DE-FG02-02ER15337. We would like to thank Nir Eliyahu for experimental support. NR 24 TC 6 Z9 6 U1 3 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 EI 1932-7455 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 31 PY 2013 VL 117 IS 43 BP 22307 EP 22313 DI 10.1021/jp402387y PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 247HJ UT WOS:000326608200020 ER PT J AU Yaffe, O Ely, T Har-Lavan, R Egger, DA Johnston, S Cohen, H Kronik, L Vilan, A Cahen, D AF Yaffe, Omer Ely, Tal Har-Lavan, Rotem Egger, David A. Johnston, Steve Cohen, Hagai Kronik, Leeor Vilan, Ayelet Cahen, David TI Effect of Molecule-Surface Reaction Mechanism on the Electronic Characteristics and Photovoltaic Performance of Molecularly Modified Si SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID HYDROGEN-TERMINATED SILICON; SELF-ASSEMBLED MONOLAYERS; ORGANIC MONOLAYERS; ALKYL MONOLAYERS; AQUEOUS-SOLUTIONS; CURRENT TRANSPORT; SI(111) SURFACE; CHEMICAL-BOND; WORK FUNCTION; RECOMBINATION AB We report on the passivation properties of molecularly modified, oxide-free Si(111) surfaces. The reaction of 1-alcohol with the H-passivated Si(111) surface can follow two possible paths, nucleophilic substitution (S-N) and radical chain reaction (RCR), depending on adsorption conditions. Moderate heating leads to the SN reaction, whereas with UV irradiation RCR dominates, with SN as a secondary path. We show that the site-sensitive SN reaction leads to better electrical passivation, as indicated by smaller surface band bending and a longer lifetime of minority carriers. However, the surface-insensitive RCR reaction leads to more dense monolayers and, therefore, to much better chemical stability, with lasting protection of the Si surface against oxidation. Thus, our study reveals an inherent dissonance between electrical and chemical passivation. Alkoxy monolayers, formed under UV irradiation, benefit, though, from both chemical and electronic passivation because under these conditions both SN and RCR occur. This is reflected in longer minority carrier lifetimes, lower reverse currents in the dark, and improved photovoltaic performance, over what is obtained if only one of the mechanisms operates. These results show how chemical kinetics and reaction paths impact electronic properties at the device level. It further suggests an approach for effective passivation of other semiconductors. C1 [Yaffe, Omer; Ely, Tal; Har-Lavan, Rotem; Kronik, Leeor; Vilan, Ayelet; Cahen, David] Weizmann Inst Sci, Dept Mat & Interfaces, IL-76100 Rehovot, Israel. [Egger, David A.] Graz Univ Technol, Inst Solid State Phys, A-8010 Graz, Austria. [Johnston, Steve] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Cohen, Hagai] Weizmann Inst Sci, Dept Chem Res Support, IL-76100 Rehovot, Israel. RP Cahen, D (reprint author), Weizmann Inst Sci, Dept Mat & Interfaces, IL-76100 Rehovot, Israel. EM leeor.kronik@weizmann.ac.il; ayelet.vilan@weizmann.ac.il; david.cahen@weizmann.ac.il RI Egger, David/M-8926-2015 FU Israel Science Foundation; Wolfson family trust; Leona M. and Harry B. Helmsley Charitable Trust; Grand Centre for Sensors and Security; Kimmel Centre for Nanoscale Science; Austrian Academy of Sciences; Austrian Science Fund (FWF) [I937-N19]; Azrieli Foundation FX We thank Ofer Sinai, Ariel Biller, Pabitra Kumar Nayak (WIS), Chaim Sukenik (Bar-Ilan), J. Schwartz (Princeton), and Yves Chabal (UT Dallas) for useful discussions and guidance. A.V., L.K, and D.C. thank the Israel Science Foundation via its centres of Excellence program, for partial support. D.C. & L.K. thank the Wolfson family trust and the Leona M. and Harry B. Helmsley Charitable Trust, and D.C. thanks the Grand Centre for Sensors and Security and the Kimmel Centre for Nanoscale Science for support. L.K. thanks the Lise Meitner Minerva Center for Computational Chemistry. D.A.E. is a recipient of a DOC-fellowship by the Austrian Academy of Sciences, and further financial support by the Austrian Science Fund (FWF): I937-N19 is gratefully acknowledged. O.Y. thanks the Azrieli Foundation for the award of an Azrieli Fellowship. D.C. holds the Rowland and Sylvia Schaefer chair in Energy research. NR 78 TC 10 Z9 10 U1 0 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 31 PY 2013 VL 117 IS 43 BP 22351 EP 22361 DI 10.1021/jp4027755 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 247HJ UT WOS:000326608200025 ER PT J AU Lockyear, JF Welz, O Savee, JD Goulay, F Trevitt, AJ Taatjes, CA Osborn, DL Leone, SR AF Lockyear, Jessica F. Welz, Oliver Savee, John D. Goulay, Fabien Trevitt, Adam J. Taatjes, Craig A. Osborn, David L. Leone, Stephen R. TI Isomer Specific Product Detection in the Reaction of CH with Acrolein SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID SET MODEL CHEMISTRY; RING-DOWN SPECTROSCOPY; RATE CONSTANTS; LOW-PRESSURE; CAVITY RING; UNSATURATED-HYDROCARBONS; COMBUSTION CHEMISTRY; CARBONYL-COMPOUNDS; RADICAL REACTIONS; BRANCHING RATIOS AB The products formed in the reaction between the methylidene radical (CH) and acrolein (CH2=CHCHO) are probed at 4 Torr and 298 K employing tunable vacuum-ultraviolet synchrotron light and multiplexed photoionization mass-spectrometry. The data suggest a principal exit channel of H loss from the adduct to yield C4H4O, accounting for (78 +/- 10)% of the products. Examination of the photoionization spectra measured upon reaction of both CH and CD with acrolein reveals that the isomeric composition of the C4H4O product is (60 +/- 12)% 1,3-butadienal and (17 +/- 10)% furan. The remaining 23% of the possible C4H4O products cannot be accurately distinguished without more reliable photoionization spectra of the possible product isomers but most likely involves oxygenated butyne species. In addition, C2H2O and C3H4 are detected, which account for (14 +/- 10)% and (8 +10, -8)% of the products, respectively. The C2H2O photoionization spectrum matches that of ketene and the C3H4 signal is composed of (24 +/- 14)% allene and (76 +/- 22)% propyne, with an upper limit of 8% placed on the cyclopropene contribution. The reactive potential energy surface is also investigated computationally, coefficients are calculated with RRKM theory. These calculations predict overall branching fractions for 1,3-butadienal and furan of 27% and 12%, respectively, in agreement with the experimental results. In contrast, the calculations predict a prominent CO + 2-methylvinyl product channel that is at most a minor channel according to the experimental results. Studies with the CD radical strongly suggest that the title reaction proceeds predominantly via cycloaddition of the radical onto the C=O bond of acrolein, with cycloaddition to the C=C bond being the second most probable reactive mechanism. C1 [Lockyear, Jessica F.; Leone, Stephen R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Welz, Oliver; Savee, John D.; Taatjes, Craig A.; Osborn, David L.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Goulay, Fabien] W Virginia Univ, Dept Chem, Morgantown, WV 26506 USA. [Trevitt, Adam J.] Univ Wollongong, Sch Chem, Wollongong, NSW 2522, Australia. [Leone, Stephen R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Leone, Stephen R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Leone, SR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM srl@berkeley.edu RI Trevitt, Adam/A-2915-2009; Welz, Oliver/C-1165-2013 OI Trevitt, Adam/0000-0003-2525-3162; Welz, Oliver/0000-0003-1978-2412 FU Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy at Lawrence Berkeley National Laboratory [DE-AC03-76SF0098]; West Virginia University; Australian Research Council [DP1094135]; International Synchrotron Access Program (ISAP); National Collaborative Research Infrastructure Strategy grant by the Federal Government of Australia; Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences, the U.S. Department of Energy; National Nuclear Security Administration [DE-AC04-94AL85000] FX The Advanced Light Source and Chemical Sciences Division (S.R.L. and J.F.L.) are supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC03-76SF0098 at Lawrence Berkeley National Laboratory. F.G. acknowledges West Virginia University for funding (start up package). A.J.T. acknowledges funding support from the Australian Research Council (DP1094135) and travel funding provided by the International Synchrotron Access Program (ISAP) managed by the Australian Synchrotron. The ISAP is funded by a National Collaborative Research Infrastructure Strategy grant provided by the Federal Government of Australia. We thank Mr. Howard Johnsen for technical support of this experiment. Sandia authors (O.W., J.D.S., D.L.O., and CAT.) and the instrumentation for this work are supported by the Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences, the U.S. Department of Energy. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration under Contract Number DE-AC04-94AL85000. NR 84 TC 7 Z9 7 U1 3 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 EI 1520-5215 J9 J PHYS CHEM A JI J. Phys. Chem. A PD OCT 31 PY 2013 VL 117 IS 43 BP 11013 EP 11026 DI 10.1021/jp407428v PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 247HL UT WOS:000326608400004 PM 24088057 ER PT J AU Lee, D Greenman, L Sarovar, M Whaley, KB AF Lee, Donghyun Greenman, Loren Sarovar, Mohan Whaley, K. Birgitta TI Ab Initio Calculation of Molecular Aggregation Effects: A Coumarin-343 Case Study SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID DENSITY-FUNCTIONAL THEORY; EXCITATION-ENERGY TRANSFER; COUPLED-CLUSTER METHODS; BASIS-SETS; ORBITAL METHODS; CONFIGURATION-INTERACTION; REACTION CENTERS; WAVE-FUNCTIONS; SYSTEMS; ACCURACY AB We present time-dependent density functional theory (TDDFT) calculations for single and dimerized Coumarin-343 molecules to investigate the quantum mechanical effects of chromophore aggregation in extended systems designed to function as a new generation of sensors and light-harvesting devices. Using the single-chromophore results, we describe the construction of effective Hamiltonians to predict the excitonic properties of aggregate systems. We compare the electronic coupling properties predicted by such effective Hamiltonians to those obtained from TDDFT calculations of dimers and to the coupling predicted by the transition density cube (TDC) method. We determine the accuracy of the dipole dipole approximation and TDC with respect to the separation distance and orientation of the dimers. In particular, we investigate the effects of including Coulomb coupling terms ignored in the typical tight-binding effective Hamiltonian. We also examine effects of orbital relaxation which cannot be captured by either of these models. C1 [Lee, Donghyun; Greenman, Loren; Whaley, K. Birgitta] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Sarovar, Mohan] Sandia Natl Labs, Livermore, CA 94550 USA. RP Whaley, KB (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM whaley@berkeley.edu FU NSF [CHE-0233882, CHE-0840505]; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; DARPA QuBE (Quantum Effects in Biological Environments) program [N66001-10-1-4068] FX We thank Matthew Francis and Dan Finley for useful discussions on virus-templated assembly for light harvesting. We thank the Molecular Graphics and Computation Facility at UC-Berkeley for computational resources, which were made possible by the NSF under contract numbers CHE-0233882 and CHE-0840505. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the United States Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. Financial support for this research was provided by the DARPA QuBE (Quantum Effects in Biological Environments) program under contract number N66001-10-1-4068 and by the NSF (grants CHE-0233882 and CHE-0840505). NR 68 TC 6 Z9 6 U1 4 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD OCT 31 PY 2013 VL 117 IS 43 BP 11072 EP 11085 DI 10.1021/jp405152h PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 247HL UT WOS:000326608400009 PM 24044623 ER PT J AU Ciappina, MF Lee, TG Pindzola, MS Colgan, J AF Ciappina, M. F. Lee, T. -G. Pindzola, M. S. Colgan, J. TI Nucleus-nucleus effects in differential cross sections for antiproton-impact ionization of H atoms SO PHYSICAL REVIEW A LA English DT Article ID HYDROGEN AB We investigate the differential cross sections for antiproton-impact ionization of H atoms within the framework of time-dependent close-coupling theory. A Fourier transform method is employed in order to extract the fully differential cross sections for a specific value of projectile momentum transfer. The method allows us to incorporate the information about the interaction between the incoming projectile and the target nucleus, the so-called nucleus-nucleus interaction, and to assess its effect on the fully differential cross sections and double differential cross sections in projectile variables. C1 [Ciappina, M. F.; Lee, T. -G.; Pindzola, M. S.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Colgan, J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Ciappina, MF (reprint author), Auburn Univ, Dept Phys, Auburn, AL 36849 USA. RI Lee, Teck Ghee/D-5037-2012; OI Lee, Teck Ghee/0000-0001-9472-3194; Ciappina, Marcelo/0000-0002-1123-6460; Colgan, James/0000-0003-1045-3858 FU US Department of Energy (DOE); US National Science Foundation (NSF); DOE ERCAP award at the National Energy Research Scientific Computing Center in Oakland, California, USA FX This work was supported in part by grants from the US Department of Energy (DOE) and the US National Science Foundation (NSF). The computational work was carried out under a DOE ERCAP award at the National Energy Research Scientific Computing Center in Oakland, California, USA. We thank Igor Bray and Ilkhom Abdurakhmanov for sending us their CCC data. NR 20 TC 2 Z9 2 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD OCT 31 PY 2013 VL 88 IS 4 AR 042714 DI 10.1103/PhysRevA.88.042714 PG 6 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 244LE UT WOS:000326389100007 ER PT J AU Guo, H He, Y Chien, CC Levin, K AF Guo, Hao He, Yan Chien, Chih-Chun Levin, K. TI Compressibility in strongly correlated superconductors and superfluids: From the BCS regime to Bose-Einstein condensates SO PHYSICAL REVIEW A LA English DT Article ID FERMI-GAS; UNIVERSAL THERMODYNAMICS; TEMPERATURE; CROSSOVER AB We present a theoretical study of the compressibility kappa in a Fermi gas with attractive contact interactions, providing predictions for the strongly attractive regime and the superfluid phase. Our work emphasizes the compressibility sum rule and gauge invariance as constraints on kappa, and we show how within a Gor'kov-based t-matrix approach, these can be satisfied in the normal phase when no approximations are made. For tractability, approximations must be introduced, and it is believed that thermodynamical approaches to kappa are more reliable than correlation-function-based schemes. Contrasting with other studies in the literature, we present thermodynamic calculations of kappa. As expected of an approximate approach, ours do not satisfy the compressibility sum rule. However, without adjusting parameters, they yield semiquantitative agreement with experiment and provide physical insight into similar results obtained via quantum Monte Carlo simulations. C1 [Guo, Hao] Southeast Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China. [He, Yan; Levin, K.] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [He, Yan; Levin, K.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Chien, Chih-Chun] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Guo, H (reprint author), Southeast Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China. FU NSF-MRSEC [0820054]; National Natural Science Foundation (NSF) of China; NSF of Jiangsu Province [11204032, SBK201241926] FX We thank M. Zwierlein and A. Rancon for their help. K.L. and Y.H. are supported by NSF-MRSEC Grant No. 0820054. H.G. is supported by the National Natural Science Foundation (NSF) of China and the NSF of Jiangsu Province (Grants No. 11204032 and No. SBK201241926). C.C.C. thanks the U.S. DOE via the LANL/LDRD Program. NR 27 TC 4 Z9 4 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD OCT 31 PY 2013 VL 88 IS 4 AR 043644 DI 10.1103/PhysRevA.88.043644 PG 5 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 244LE UT WOS:000326389100011 ER PT J AU Coh, S Tan, LZ Louie, SG Cohen, ML AF Coh, Sinisa Tan, Liang Z. Louie, Steven G. Cohen, Marvin L. TI Theory of the Raman spectrum of rotated double-layer graphene SO PHYSICAL REVIEW B LA English DT Article ID BILAYER GRAPHENE AB We study theoretically the Raman spectrum of the rotated double-layer graphene, consisting of two graphene layers rotated with respect to each other by an arbitrary angle.. We find a relatively simple dependence of the Raman G peak intensity on the angle.. On the other hand, the Raman 2D peak position, intensity, and width show a much more complicated dependence on the angle.. We account for all of these effects, including dependence on the incoming photon energy, in good agreement with the experimental data. We find that it is sufficient to include the interaction between the graphene layers on the electronic degrees of freedom (resulting in the occurrence of Van Hove singularities in the density of states). We assume that the phonon degrees of freedom are unaffected by the interaction between the layers. Furthermore, we decompose the Raman 2D peak into two components having very different linewidths; these widths are almost independent of the angle.. The change in the intensity and the peak position of one of these two components gives insight into the dependence of the overall Raman 2D peak features as a function of the angle.. Furthermore, we study the influence of the coherence on the Raman signal, and we separately study the influence of the interaction between the layers on the electron wave functions and energies. Additionally, we show regions in the phonon spectrum giving rise to the Raman 2D peak signal. This work provides an insight into the interplay between the mechanical degree of freedom (angle.) and the electronic degrees of freedom (singularities in the density of states) in rotated double-layer graphene. Additionally, this work provides a way to establish experimentally the value of the rotation angle. using Raman spectroscopy measurement. This procedure becomes even more robust if one repeats the Raman spectroscopy measurement with a different incoming photon energy. C1 [Coh, Sinisa] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Coh, S (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM sinisa@civet.berkeley.edu OI Tan, Liang Z/0000-0003-4724-6369 FU Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy [DE-AC02-05CH11231]; National Science Foundation [DMR10-1006184]; Simons Foundation Fellowship in Theoretical Physics FX We thank G. Samsonidze for discussion and F. Mauri for sharing data on the calculated monolayer graphene phonon band structure. This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy under Contract No. DE-AC02-05CH11231 and by the National Science Foundation under Grant No. DMR10-1006184, which provided for continuum model calculations. S. G. L. acknowledges support of a Simons Foundation Fellowship in Theoretical Physics. Computational resources were provided by theNational Energy Research Scientific Computing Center, which is supported by the Office of Science of the U. S. Department of Energy. NR 33 TC 24 Z9 24 U1 10 U2 62 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 31 PY 2013 VL 88 IS 16 AR 165431 DI 10.1103/PhysRevB.88.165431 PG 15 WC Physics, Condensed Matter SC Physics GA 244LN UT WOS:000326390000006 ER PT J AU Garcia-Lekue, A Sanchez-Portal, D Arnau, A Wang, LW AF Garcia-Lekue, A. Sanchez-Portal, D. Arnau, A. Wang, L. W. TI Plane-wave based electron tunneling through field emission resonance states SO PHYSICAL REVIEW B LA English DT Article ID IMAGE-POTENTIAL STATES; METAL-SURFACES; INTERFEROMETRY; IDENTIFICATION; EXCITATIONS; INTERFACE; BARRIER; DECAY AB Field emission resonances (FERs) on Cu(100) surface are investigated by means of tunneling regime simulations performed with a plane-wave based transport calculation method. FERs are located near the surface and decay into the vacuum, and their accurate simulation requires a faithful description of vacuum states. This type of simulations is thus not possible using the popular transport methods based on atom-centered localized basis sets and the use of plane waves becomes important. We introduce a procedure to treat self-consistently (SC) the finite bias nonequilibrium problem in tunneling regime. Image potential effects are included in a semiempirical way within the SC calculation. Tunneling through FERs is studied following a practical strategy to approximate the inelastic transmission for states lying in the band gap of the surface. As our approach permits the use of any tip geometry, tip effects on the energy and wave functions of FERs are explored. The method reported here provides an ideal tool for the simulation of FERs aimed at the understanding of experimental STS (scanning tunneling spectroscopy) observations. C1 [Garcia-Lekue, A.; Sanchez-Portal, D.; Arnau, A.] Donostia Int Phys Ctr, E-20018 San Sebastian, Spain. [Garcia-Lekue, A.] Basque Fdn Sci, IKERBASQUE, E-48011 Bilbao, Spain. [Sanchez-Portal, D.; Arnau, A.] Ctr Mixto CSIC UPV, Ctr Fis Mat CFM MPC, San Sebastian, Spain. [Arnau, A.] Univ Basque Country, Fac Quim, Dpto Fis Mat, San Sebastian, Spain. [Wang, L. W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. RP Garcia-Lekue, A (reprint author), Donostia Int Phys Ctr, Paseo Manuel Lardizabal 4, E-20018 San Sebastian, Spain. RI Sanchez-Portal, Daniel /E-5858-2010; DONOSTIA INTERNATIONAL PHYSICS CTR., DIPC/C-3171-2014; arnau, andres/H-7901-2012; CSIC-UPV/EHU, CFM/F-4867-2012 OI arnau, andres/0000-0001-5281-3212; FU Basque Departamento de Educacion and the UPV/EHU [IT-756-13]; Spanish Ministerio de Ciencia e Innovacioon [FIS2010-19609-C02-00]; ETORTEK program; Basque Departamento de Industria and the Diputacion Foral de Gipuzkoa; National Energy Research Scientific Computing Center (NERSC); US DOE/SC/BES [DE-AC02-05CH11231] FX We acknowledge support from the Basque Departamento de Educacion and the UPV/EHU (Grant No. IT-756-13), the Spanish Ministerio de Ciencia e Innovacioon (Grant No. FIS2010-19609-C02-00), and the ETORTEK program funded by the Basque Departamento de Industria and the Diputacion Foral de Gipuzkoa. It used the resources of the National Energy Research Scientific Computing Center (NERSC). L. W. Wang is supported by the US DOE/SC/BES under contract No. DE-AC02-05CH11231. NR 49 TC 1 Z9 1 U1 2 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 31 PY 2013 VL 88 IS 15 AR 155441 DI 10.1103/PhysRevB.88.155441 PG 9 WC Physics, Condensed Matter SC Physics GA 244LL UT WOS:000326389800007 ER PT J AU Rincon, J Garcia, DJ Hallberg, K Vojta, M AF Rincon, Julian Garcia, Daniel J. Hallberg, K. Vojta, Matthias TI Quantum phase transition between one-channel and two-channel Kondo polarons SO PHYSICAL REVIEW B LA English DT Article ID DENSITY-MATRIX RENORMALIZATION; DIMENSIONAL ELECTRON-GAS; IMPURITY; STATE; METALS; MODEL AB For a mobile spin-1/2 impurity, coupled antiferromagnetically to a one-dimensional gas of fermions, perturbative ideas have been used to argue in favor of two-channel Kondo behavior of the impurity spin. Here we combine general considerations and extensive numerical simulations to show that the problem displays a novel quantum phase transition between two-channel and one-channel Kondo screening upon increasing the Kondo coupling. We construct a ground-state phase diagram and discuss the various nontrivial crossovers as well as possible experimental realizations. C1 [Rincon, Julian] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Garcia, Daniel J.; Hallberg, K.] Comis Nacl Energia Atom, Ctr Atom Bariloche, Inst Balseiro, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina. [Garcia, Daniel J.; Hallberg, K.] Consejo Nacl Invest Cient & Tecn, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina. [Vojta, Matthias] Tech Univ Dresden, Inst Theoret Phys, D-01062 Dresden, Germany. RP Rincon, J (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RI Vojta, Matthias/B-2298-2012; OI Garcia, Daniel Julio/0000-0001-6777-9184 FU DFG [FG 960]; German-Israeli Foundation; Early Career Research Program of US DOE; Heinrich-Hertz-Stiftung NRW FX We thank B. Alascio, P. Cornaglia, A. Feiguin, E. Fradkin, T. Giamarchi, and C. Vojta for discussions. This research was supported by the DFG (FG 960), the German-Israeli Foundation, and the Early Career Research Program of US DOE. M.V. also acknowledges support by the Heinrich-Hertz-Stiftung NRW and the hospitality of the Centro Atomico Bariloche, where part of this work was performed. NR 26 TC 1 Z9 1 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 31 PY 2013 VL 88 IS 14 AR 140407 DI 10.1103/PhysRevB.88.140407 PG 4 WC Physics, Condensed Matter SC Physics GA 244LH UT WOS:000326389400001 ER PT J AU Schumacher, D Steffen, A Voigt, J Schubert, J Bruckel, T Ambaye, H Lauter, V AF Schumacher, D. Steffen, A. Voigt, J. Schubert, J. Brueckel, Th. Ambaye, H. Lauter, V. TI Inducing exchange bias in La0.67Sr0.33MnO3-delta/SrTiO3 thin films by strain and oxygen deficiency SO PHYSICAL REVIEW B LA English DT Article ID MAGNETORESISTANCE; MANGANITES; STOICHIOMETRY; ANISOTROPY; OXIDES AB We present an exchange bias (EB) effect of variable size in La0.67Sr0.33MnO3-delta single and La0.67Sr0.33MnO3-delta/SrTiO3 (LSMO/STO) bilayers grown on STO substrates. Samples have been prepared by pulsed laser deposition (PLD) and high-pressure sputter deposition (HSD) in oxygen atmosphere at different oxygen pressures. Increased out-of-plane lattice parameters of the LSMO layers and reduced Curie temperatures indicate oxygen deficiencies in the samples grown at lower oxygen pressures. We found an increase of the EB and the coercive fields with decreasing oxygen pressure, whereas the growth at high pressures does not lead to an EB effect. The depth-sensitive method of polarized neutron reflectometry (PNR) reveals a region with drastically reduced, maybe even completely vanishing net magnetization in the LSMO layer at the interface to STO in the exchange-biased samples, but not in the non-exchanged-biased one. It is suggested that an antiferromagnetic structure is formed in this part of the LSMO thin film, which causes the EB effect in this system. An explanation based on the strain-doping phase diagram of LSMO is provided. Thus our findings open a route for tuning the EB effect by changing the oxygen vacancy concentrations. C1 [Schumacher, D.; Steffen, A.; Voigt, J.; Schubert, J.; Brueckel, Th.; Ambaye, H.; Lauter, V.] Julich Ctr Neutron Sci JCNS, D-52425 Julich, Germany. [Schumacher, D.; Steffen, A.; Voigt, J.; Schubert, J.; Brueckel, Th.; Ambaye, H.; Lauter, V.] JARA FIT, Peter Grunberg Inst PGI, D-52425 Julich, Germany. [Schumacher, D.; Steffen, A.; Voigt, J.; Schubert, J.; Brueckel, Th.; Ambaye, H.; Lauter, V.] Forschungszentrum Julich, D-52425 Julich, Germany. [Ambaye, H.; Lauter, V.] Oak Ridge Natl Lab, Neutron Sci Directorate, Spallat Neutron Source, Oak Ridge, TN 37831 USA. RP Schumacher, D (reprint author), Julich Ctr Neutron Sci JCNS, D-52425 Julich, Germany. RI Bruckel, Thomas/J-2968-2013; Schubert, Jurgen/K-9543-2013; Ambaye, Haile/D-1503-2016; OI Bruckel, Thomas/0000-0003-1378-0416; Schubert, Jurgen/0000-0003-0185-6794; Ambaye, Haile/0000-0002-8122-9952; Voigt, Jorg/0000-0002-6556-4961; Steffen, Alexandra/0000-0002-9802-438X NR 27 TC 15 Z9 15 U1 11 U2 103 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD OCT 31 PY 2013 VL 88 IS 14 AR 144427 DI 10.1103/PhysRevB.88.144427 PG 7 WC Physics, Condensed Matter SC Physics GA 244LH UT WOS:000326389400002 ER PT J AU Allmond, JM AF Allmond, J. M. TI Simple correlations between electric quadrupole moments of atomic nuclei SO PHYSICAL REVIEW C LA English DT Article ID MULTIPLE COULOMB-EXCITATION; EVEN-EVEN NUCLEI; PT-OS NUCLEI; OSMIUM ISOTOPES; HEXADECAPOLE VIBRATIONS; ROTATIONAL STATES; SHAPES; TRANSITION; PT-196; BEAM AB Measurements of nonyrast electric quadrupole moments (i.e., diagonal E2 matrix elements) of atomic nuclei are becoming widely available from multiple-step Coulomb excitation. It is shown that, where quadrupole-moment data exist, < 2(1)(+) parallel to E2 parallel to 2(1)(+) > + < 2(2)(+) parallel to E2 parallel to 2(2)(+) > approximate to 0 is observed across a wide range of masses, deformations, and first 2(+) energies. Nearly all of these quadrupole-moment data, particularly < 2(2)(+) parallel to E2 parallel to|2(2)(+), are from the past two decades with half of the data from the past decade. In addition, < 4(1)(+) parallel to E2 parallel to|4(1)(+)> + < 4(2)(+) parallel to E2 parallel to 4(2)(+) > parallel to + < 4(3)(+) parallel to E2 parallel to 4(3)(+)> approximate to 0 is observed within two standard deviations for three of the four existing measurements. Despite many and varying complexities in the structure details of the individual nuclei, the correlations in the quadrupole moments appear simple. C1 Oak Ridge Natl Lab, Joint Inst Heavy Ion Res, Oak Ridge, TN 37831 USA. RP Allmond, JM (reprint author), Oak Ridge Natl Lab, Joint Inst Heavy Ion Res, Oak Ridge, TN 37831 USA. OI Allmond, James Mitchell/0000-0001-6533-8721 FU Office of Nuclear Physics, U.S. Department of Energy; U.S. Department of Energy FX The author would like to thank D. G. Jenkins, T. Papenbrock, D. C. Radford, D. J. Rowe, A. E. Stuchbery, and J. L. Wood for fruitful discussions and useful comments on the manuscript. Research sponsored by the Office of Nuclear Physics, U.S. Department of Energy. The Joint Institute for Heavy Ion Research has as member institutions the University of Tennessee, Vanderbilt University, and the Oak Ridge National Laboratory; it is supported by the members and by the U.S. Department of Energy. NR 68 TC 4 Z9 4 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 31 PY 2013 VL 88 IS 4 AR 041307 DI 10.1103/PhysRevC.88.041307 PG 6 WC Physics, Nuclear SC Physics GA 244LR UT WOS:000326390500001 ER PT J AU Nag, S Singh, AK Ragnarsson, I Hubel, H Al-Khatib, A Bringel, P Engelhardt, C Neusser-Neffgen, A Hagemann, GB Herskind, B Sletten, G Carpenter, MP Janssens, RVF Khoo, TL Lauritsen, T Clark, RM Fallon, P Benzoni, G Bracco, A Camera, F Chowdhury, P AF Nag, Somnath Singh, A. K. Ragnarsson, I. Huebel, H. Al-Khatib, A. Bringel, P. Engelhardt, C. Neusser-Neffgen, A. Hagemann, G. B. Herskind, B. Sletten, G. Carpenter, M. P. Janssens, R. V. F. Khoo, T. L. Lauritsen, T. Clark, R. M. Fallon, P. Benzoni, G. Bracco, A. Camera, F. Chowdhury, P. TI Collective and noncollective excitations in Te-122 SO PHYSICAL REVIEW C LA English DT Article ID HIGH-SPIN STATES; ROTATIONAL BANDS; SMOOTH TERMINATION; HOLE EXCITATIONS; OBLATE STATES; NUCLEI; COEXISTENCE; REGION AB High-spin states in Te-122 were populated in the reaction Se-82(Ca-48, alpha 4n) Te-122 at a beam energy of 200 MeV and gamma-ray coincidences weremeasured with the Gammasphere spectrometer. The previously known level scheme was extended to considerably higher spin. Maximally aligned states and several high-energy transitions feeding into some of these levels were observed. In addition, seven collective high-spin bands were discovered for the first time in this nucleus. The experimental results are compared with cranked Nilsson-Strutinsky model calculations and possible configuration assignments to the new high-spin structures are discussed. C1 [Nag, Somnath; Singh, A. K.] Indian Inst Technol, Dept Phys & Meteorol, IN-721302 Kharagpur, W Bengal, India. [Ragnarsson, I.] Lund Univ, Div Math Phys, LTH, S-221 Lund, Sweden. [Huebel, H.; Al-Khatib, A.; Bringel, P.; Engelhardt, C.; Neusser-Neffgen, A.] Univ Bonn, Helmholtz Inst Strahlen & Kernphys, D-53115 Bonn, Germany. [Hagemann, G. B.; Herskind, B.; Sletten, G.] Niels Bohr Inst, DK-2100 Copenhagen O, Denmark. [Carpenter, M. P.; Janssens, R. V. F.; Khoo, T. L.; Lauritsen, T.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Clark, R. M.; Fallon, P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Benzoni, G.; Bracco, A.; Camera, F.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Bracco, A.; Camera, F.] Univ Milan, Dipartimento Fis, I-20133 Milan, Italy. [Chowdhury, P.] Univ Massachusetts Lowell, Dept Phys, Lowell, MA 01854 USA. RP Nag, S (reprint author), Indian Inst Technol, Dept Phys & Meteorol, IN-721302 Kharagpur, W Bengal, India. RI Carpenter, Michael/E-4287-2015; OI Carpenter, Michael/0000-0002-3237-5734; Camera, Franco/0000-0003-1731-4834; benzoni, giovanna/0000-0002-7938-0338 FU CSIR, India [09/081(0704)/2009-EMR-I]; DST, India [SR/S2/HEP-09/2005]; Swedish Science Research Council; German BMBF [06 BN 109]; Danish FNU Council for Natural Sciences; U.S. Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357, DE-AC03-76SF00098] FX The authors would like to thank the ATLAS and Gammasphere operations staff for their support. S. N. acknowledges financial support from CSIR, India, under Contract No. 09/081(0704)/2009-EMR-I and help from Dr. P. Singh. This work was supported by the DST, India, under Project No. SR/S2/HEP-09/2005, by the Swedish Science Research Council, by the German BMBF under Contract No. 06 BN 109, by the Danish FNU Council for Natural Sciences, and by the U.S. Department of Energy, Office of Nuclear Physics, under Contracts No. DE-AC02-06CH11357 and No. DE-AC03-76SF00098. NR 36 TC 4 Z9 4 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 31 PY 2013 VL 88 IS 4 AR 044335 DI 10.1103/PhysRevC.88.044335 PG 13 WC Physics, Nuclear SC Physics GA 244LR UT WOS:000326390500005 ER PT J AU Wiringa, RB Pastore, S Pieper, SC Miller, GA AF Wiringa, R. B. Pastore, S. Pieper, Steven C. Miller, Gerald A. TI Charge-symmetry breaking forces and isospin mixing in Be-8 SO PHYSICAL REVIEW C LA English DT Article ID PROTON ELASTIC-SCATTERING; LIGHT-NUCLEI; PRECISION-MEASUREMENT; MONTE-CARLO; ASYMMETRY; VIOLATION AB We report Green's function Monte Carlo calculations of isospin-mixing (IM) matrix elements for the 2(+), 1(+), and 3(+) T = 0 and 1 pairs of states at 16-19 MeV excitation in Be-8. The realistic Argonne nu(18) (AV18) two-nucleon and Illinois-7 three-nucleon potentials are used to generate the nuclear wave functions. Contributions from the full electromagnetic interaction and strong class III charge-symmetry breaking (CSB) components of the AV18 potential are evaluated. We also examine two theoretically more complete CSB potentials based on rho-omega mixing, tuned to give the same neutron-neutron scattering length as AV18. The contribution of these different CSB potentials to the H-3-He-3, Li-7-Be-7, and Li-8-B-8 isovector energy differences is evaluated and reasonable agreement with experiment is obtained. Finally, for the Be-8 IM calculation we add the small class IV CSB terms coming from one-photon, one-pion, and one-rho exchange, as well as rho-omega mixing. The expectation values of the three CSB models vary by up to 20% in the isovector energy differences, but only by 10% or less in the IM matrix element. The total matrix element gives 85-90% of the experimental IM value of -145 keV for the 2(+) doublet, with about two thirds coming from the Coulomb interaction. We also report the IM matrix element to the first 2(+) state at 3 MeV excitation, which is the final state for various tests of the standard model for beta decay. C1 [Wiringa, R. B.; Pieper, Steven C.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Pastore, S.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Miller, Gerald A.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. RP Wiringa, RB (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. EM wiringa@anl.gov; pastores@mailbox.sc.edu; spieper@anl.gov; miller@phys.washington.edu RI Wiringa, Robert/M-4970-2015 FU US DOE, Office of Nuclear Physics [DE-AC02-06CH11357]; NUCLEI SciDAC program; US NSF [PHY-1068305]; US DOE [DE-FG02-97ER41014] FX We thank I. Brida for valuable input. The many-body calculations were performed on the parallel computers of the Laboratory Computing Resource Center, Argonne National Laboratory. The work of R.B.W. and S.C.P. is supported by the US DOE, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357, and by the NUCLEI SciDAC program, that of S. P. is supported by the US NSF under Grant No. PHY-1068305, and that of G. A. M. is supported by the US DOE under Contract No. DE-FG02-97ER41014. NR 37 TC 7 Z9 7 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD OCT 31 PY 2013 VL 88 IS 4 AR 044333 DI 10.1103/PhysRevC.88.044333 PG 8 WC Physics, Nuclear SC Physics GA 244LR UT WOS:000326390500003 ER PT J AU Adamson, P Barr, G Bishai, M Blake, A Bock, GJ Bogert, D Cao, SV Cherdack, D Childress, S Coelho, JAB Corwin, L Cronin-Hennessy, D de Jong, JK Devan, AV Devenish, NE Diwan, MV Escobar, CO Evans, JJ Falk, E Feldman, GJ Frohne, MV Gallagher, HR Gomes, RA Goodman, MC Gouffon, P Graf, N Gran, R Grzelak, K Habig, A Hartnell, J Hatcher, R Himmel, A Holin, A Hylen, J Irwin, GM Isvan, Z James, C Jensen, D Kafka, T Kasahara, SMS Koizumi, G Kordosky, M Kreymer, A Lang, K Ling, J Litchfield, PJ Lucas, P Mann, WA Marshak, ML Mathis, M Mayer, N Medeiros, MM Mehdiyev, R Meier, JR Messier, MD Miller, WH Mishra, SR Sher, SM Moore, CD Mualem, L Mufson, S Musser, J Naples, D Nelson, JK Newman, HB Nichol, RJ Nowak, JA Oliver, WP Orchanian, M Pahlka, RB Paley, J Patterson, RB Pawloski, G Phan-Budd, S Plunkett, RK Qiu, X Radovic, A Rebel, B Rosenfeld, C Rubin, HA Sanchez, MC Schneps, J Schreckenberger, A Schreiner, P Sharma, R Sousa, A Tagg, N Talaga, RL Thomas, J Thomson, MA Toner, R Torretta, D Tzanakos, G Urheim, J Vahle, P Viren, B Weber, A Webb, RC White, C Whitehead, L Wojcicki, SG Zwaska, R AF Adamson, P. Barr, G. Bishai, M. Blake, A. Bock, G. J. Bogert, D. Cao, S. V. Cherdack, D. Childress, S. Coelho, J. A. B. Corwin, L. Cronin-Hennessy, D. de Jong, J. K. Devan, A. V. Devenish, N. E. Diwan, M. V. Escobar, C. O. Evans, J. J. Falk, E. Feldman, G. J. Frohne, M. V. Gallagher, H. R. Gomes, R. A. Goodman, M. C. Gouffon, P. Graf, N. Gran, R. Grzelak, K. Habig, A. Hartnell, J. Hatcher, R. Himmel, A. Holin, A. Hylen, J. Irwin, G. M. Isvan, Z. James, C. Jensen, D. Kafka, T. Kasahara, S. M. S. Koizumi, G. Kordosky, M. Kreymer, A. Lang, K. Ling, J. Litchfield, P. J. Lucas, P. Mann, W. A. Marshak, M. L. Mathis, M. Mayer, N. Medeiros, M. M. Mehdiyev, R. Meier, J. R. Messier, M. D. Miller, W. H. Mishra, S. R. Sher, S. Moed Moore, C. D. Mualem, L. Mufson, S. Musser, J. Naples, D. Nelson, J. K. Newman, H. B. Nichol, R. J. Nowak, J. A. Oliver, W. P. Orchanian, M. Pahlka, R. B. Paley, J. Patterson, R. B. Pawloski, G. Phan-Budd, S. Plunkett, R. K. Qiu, X. Radovic, A. Rebel, B. Rosenfeld, C. Rubin, H. A. Sanchez, M. C. Schneps, J. Schreckenberger, A. Schreiner, P. Sharma, R. Sousa, A. Tagg, N. Talaga, R. L. Thomas, J. Thomson, M. A. Toner, R. Torretta, D. Tzanakos, G. Urheim, J. Vahle, P. Viren, B. Weber, A. Webb, R. C. White, C. Whitehead, L. Wojcicki, S. G. Zwaska, R. CA MINOS Collaboration TI Search for flavor-changing non-standard neutrino interactions by MINOS SO PHYSICAL REVIEW D LA English DT Article ID LEPTON CHARGE; OSCILLATIONS AB We report new constraints on flavor-changing non-standard neutrino interactions from the MINOS experiment, in which neutrino versus antineutrino interactions can be distinguished on an event-by-event basis. We analyzed a combined set of beam neutrino and antineutrino data from the well-understood NuMI beam, and found no evidence for deviations from standard neutrino mixing. The observed energy spectra constrain the non-standard neutrino interactions parameter to the range -0.20 < epsilon(mu tau) < 0.07 (90%C.L.). C1 [Goodman, M. C.; Paley, J.; Phan-Budd, S.; Sanchez, M. C.; Schreiner, P.; Talaga, R. L.] Argonne Natl Lab, Argonne, IL 60439 USA. [Tzanakos, G.] Univ Athens, Dept Phys, GR-15771 Athens, Greece. [Bishai, M.; Diwan, M. V.; Isvan, Z.; Ling, J.; Viren, B.; Whitehead, L.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Himmel, A.; Mualem, L.; Newman, H. B.; Orchanian, M.; Patterson, R. B.] CALTECH, Lauritsen Lab, Pasadena, CA 91125 USA. [Blake, A.; Thomson, M. A.; Toner, R.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Coelho, J. A. B.; Escobar, C. O.] Univ Estadual Campinas, IFGW UNICAMP, BR-13083970 Campinas, SP, Brazil. [Sousa, A.] Univ Cincinnati, Dept Phys, Cincinnati, OH 45221 USA. [Adamson, P.; Bock, G. J.; Bogert, D.; Childress, S.; Hatcher, R.; Hylen, J.; James, C.; Jensen, D.; Koizumi, G.; Kreymer, A.; Lucas, P.; Sher, S. Moed; Moore, C. D.; Pahlka, R. B.; Plunkett, R. K.; Rebel, B.; Sharma, R.; Torretta, D.; Zwaska, R.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Gomes, R. A.; Medeiros, M. M.] Univ Fed Goias, Inst Fis, BR-74001970 Goiania, Go, Brazil. [Feldman, G. J.; Sousa, A.; Toner, R.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Frohne, M. V.] Coll Holy Cross, Notre Dame, IN 46556 USA. [Whitehead, L.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Graf, N.; Rubin, H. A.; White, C.] IIT, Dept Phys, Chicago, IL 60616 USA. [Corwin, L.; Mayer, N.; Messier, M. D.; Mufson, S.; Musser, J.; Urheim, J.] Indiana Univ, Bloomington, IN 47405 USA. [Sanchez, M. C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Evans, J. J.; Holin, A.; Nichol, R. J.; Radovic, A.; Thomas, J.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Evans, J. J.] Univ Manchester, Sch Phys & Astron, Manchester M13 9PL, Lancs, England. [Cronin-Hennessy, D.; Kasahara, S. M. S.; Litchfield, P. J.; Marshak, M. L.; Meier, J. R.; Miller, W. H.; Nowak, J. A.; Pawloski, G.; Schreckenberger, A.] Univ Minnesota, Minneapolis, MN 55455 USA. [Gran, R.; Habig, A.] Univ Minnesota, Dept Phys, Duluth, MN 55812 USA. [Tagg, N.] Otterbein Coll, Westerville, OH 43081 USA. [Barr, G.; de Jong, J. K.; Weber, A.] Univ Oxford, Subdept Particle Phys, Oxford OX1 3RH, England. [Isvan, Z.; Naples, D.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Litchfield, P. J.; Weber, A.] Sci & Technol Facil Council, Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Gouffon, P.] Univ Sao Paulo, Inst Fis, BR-05315970 Sao Paulo, Brazil. [Mishra, S. R.; Rosenfeld, C.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Irwin, G. M.; Pawloski, G.; Qiu, X.; Wojcicki, S. G.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Devenish, N. E.; Falk, E.; Hartnell, J.] Univ Sussex, Dept Phys & Astron, Brighton BN1 9QH, E Sussex, England. [Webb, R. C.] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Cao, S. V.; Lang, K.; Mehdiyev, R.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Cherdack, D.; Coelho, J. A. B.; Gallagher, H. R.; Kafka, T.; Mann, W. A.; Mayer, N.; Oliver, W. P.; Schneps, J.] Tufts Univ, Dept Phys, Medford, MA 02155 USA. [Grzelak, K.] Univ Warsaw, Dept Phys, PL-00681 Warsaw, Poland. [Devan, A. V.; Kordosky, M.; Mathis, M.; Nelson, J. K.; Vahle, P.] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. RP Adamson, P (reprint author), Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RI Gomes, Ricardo/B-6899-2008; Coelho, Joao/D-3546-2013; Evans, Justin/P-4981-2014; Gouffon, Philippe/I-4549-2012; Nowak, Jaroslaw/P-2502-2016; Ling, Jiajie/I-9173-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017 OI Weber, Alfons/0000-0002-8222-6681; Cao, Son/0000-0002-9046-5324; Hartnell, Jeffrey/0000-0002-1744-7955; Cherdack, Daniel/0000-0002-3829-728X; Gomes, Ricardo/0000-0003-0278-4876; Evans, Justin/0000-0003-4697-3337; Gouffon, Philippe/0000-0001-7511-4115; Nowak, Jaroslaw/0000-0001-8637-5433; Ling, Jiajie/0000-0003-2982-0670; FU U.S. DOE; United Kingdom STFC; U.S. NSF; State of Minnesota; University of Athens, Greece; Brazil's FAPESP; Brazil's CNPq; Brazil's CAPES; University of Minnesota FX This work was supported by the U.S. DOE; the United Kingdom STFC; the U.S. NSF; the State and University of Minnesota; the University of Athens, Greece; and Brazil's FAPESP, CNPq and CAPES. We are grateful to the Minnesota Department of Natural Resources, the crew of the Soudan Underground Lab, and the personnel of Fermilab for their contribution to this effort. NR 40 TC 20 Z9 20 U1 0 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 31 PY 2013 VL 88 IS 7 AR 072011 DI 10.1103/PhysRevD.88.072011 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 244LY UT WOS:000326391400002 ER PT J AU Bae, T Jang, YC Jeong, H Jung, C Kim, HJ Kim, J Kim, J Kim, K Kim, S Lee, W Leem, J Sharpe, SR Yoon, B AF Bae, Taegil Jang, Yong-Chull Jeong, Hwancheol Jung, Chulwoo Kim, Hyung-Jin Kim, Jangho Kim, Jongjeong Kim, Kwangwoo Kim, Sunghee Lee, Weonjong Leem, Jaehoon Sharpe, Stephen R. Yoon, Boram CA SWME Collaboration TI Neutral kaon mixing from new physics: Matrix elements in N-f=2+1 lattice QCD SO PHYSICAL REVIEW D LA English DT Article ID OPERATORS; DELTA-S=2 AB We present results for matrix elements of Delta S = 2 four-fermion operators arising generically in models of new physics. These are needed to constrain such models using the measured values of epsilon(K) and Delta M-K. We use lattice QCD with 2 + 1 flavors of improved staggered fermions on lattices generated by the MILC Collaboration. We extrapolate to the continuum from three lattice spacings ranging down to a approximate to 0.045 fm. Total errors are similar to 5%-6%, arising primarily from our use of one-loop matching between lattice and continuum operators. For two of the matrix elements, our results disagree significantly from those obtained using different fermion discretizations. C1 [Bae, Taegil] Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. [Jang, Yong-Chull; Jeong, Hwancheol; Kim, Jangho; Kim, Jongjeong; Kim, Kwangwoo; Kim, Sunghee; Lee, Weonjong; Leem, Jaehoon; Yoon, Boram] Seoul Natl Univ, FPRD, Lattice Gauge Theory Res Ctr, Seoul 151747, South Korea. [Jang, Yong-Chull; Jeong, Hwancheol; Kim, Jangho; Kim, Jongjeong; Kim, Kwangwoo; Kim, Sunghee; Lee, Weonjong; Leem, Jaehoon; Yoon, Boram] Seoul Natl Univ, CTP, Dept Phys & Astron, Seoul 151747, South Korea. [Jung, Chulwoo; Kim, Hyung-Jin] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Sharpe, Stephen R.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. RP Bae, T (reprint author), Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. FU Creative Research Initiatives Progam of the NRF [2013-003454]; Korean government (MSIP); U.S. DOE [DE-AC02-98CH10886, DE-FG02-96ER40956]; KISTI supercomputing center [KSC-2012-G3-08]; Office of Science of the U.S. DOE FX We thank Claude Bernard for providing unpublished information. We thank Peter Boyle, Nicolas Garron, and Vittorio Lubicz for helpful discussion. W. L. is supported by the Creative Research Initiatives program (2013-003454) of the NRF grant funded by the Korean government (MSIP). C. J. and S. R. S. are supported in part by the U.S. DOE through Contract No. DE-AC02-98CH10886 and Grant No. DE-FG02-96ER40956, respectively. Computations for this work were carried out in part on the QCDOC computer of the USQCD Collaboration, funded by the Office of Science of the U.S. DOE. W. L. acknowledges support from the KISTI supercomputing center through the strategic support program (No. KSC-2012-G3-08). NR 25 TC 7 Z9 7 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 31 PY 2013 VL 88 IS 7 AR 071503 DI 10.1103/PhysRevD.88.071503 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 244LY UT WOS:000326391400001 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, M Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Yushkov, AN Kirkby, D Lankford, AJ Mandelkern, M Dey, B Gary, JW Long, O Vitug, GM Campagnari, C Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Martinez, AJ Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Ongmongkolkul, P Porter, FC Andreassen, R Huard, Z Meadows, BT Sokoloff, MD Sun, L Bloom, PC Ford, WT Gaz, A Nauenberg, U Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Schubert, KR Schwierz, R Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Baldini-Ferroli, R Calcaterra, A de Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Guido, E Lo Vetere, M Monge, MR Passaggio, S Patrignani, C Robutti, E Bhuyan, B Prasad, V Morii, M Adametz, A Uwer, U Lacker, HM Dauncey, PD Mallik, U Chen, C Cochran, J Meyer, WT Prell, S Rubin, AE Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Bougher, J Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Prencipe, E Barlow, RJ Lafferty, GD Behn, E Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Dujmic, D Sciolla, G Cheaib, R Patel, PM Robertson, SH Biassoni, P Neri, N Palombo, F Cremaldi, L Godang, R Sonnek, P Summers, DJ Nguyen, X Simard, M Taras, P De Nardo, G Monorchio, D Onorato, G Sciacca, C Martinelli, M Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Brau, J Frey, R Sinev, NB Strom, D Torrence, E Feltresi, E Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Sitt, S Biasini, M Manoni, E Pacetti, S Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Cervelli, A Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Perez, A Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Gioi, LL Piredda, G Bunger, C Grunberg, O Hartmann, T Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S de Monchenault, GH Vasseur, G Yeche, C Anulli, F Aston, D Bard, DJ Benitez, JF Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Gabareen, AM Graham, MT Hast, C Innes, WR Kim, P Kocian, ML Leith, DWGS Lewis, P Lindemann, D Lindquist, B Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Nelson, S Perl, M Pulliam, T Ratcliff, BN Roodman, A Salnikov, AA Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wagner, AP Wang, WF Wisniewski, WJ Wittgen, M Wright, DH Wulsin, HW Ziegler, V Park, W Purohit, MV White, RM Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Miyashita, TS Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Ruland, AM Schwitters, RF Wray, BC Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Zambito, S Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Villanueva-Perez, P Ahmed, H Albert, J Banerjee, S Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lee, M. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Yushkov, A. N. Kirkby, D. Lankford, A. J. Mandelkern, M. Dey, B. Gary, J. W. Long, O. Vitug, G. M. Campagnari, C. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Martinez, A. J. Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Ongmongkolkul, P. Porter, F. C. Andreassen, R. Huard, Z. Meadows, B. T. Sokoloff, M. D. Sun, L. Bloom, P. C. Ford, W. T. Gaz, A. Nauenberg, U. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Schubert, K. R. Schwierz, R. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Baldini-Ferroli, R. Calcaterra, A. de Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Guido, E. Lo Vetere, M. Monge, M. R. Passaggio, S. Patrignani, C. Robutti, E. Bhuyan, B. Prasad, V. Morii, M. Adametz, A. Uwer, U. Lacker, H. M. Dauncey, P. D. Mallik, U. Chen, C. Cochran, J. Meyer, W. T. Prell, S. Rubin, A. E. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Bougher, J. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Prencipe, E. Barlow, R. J. Lafferty, G. D. Behn, E. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Dujmic, D. Sciolla, G. Cheaib, R. Patel, P. M. Robertson, S. H. Biassoni, P. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Sonnek, P. Summers, D. J. Nguyen, X. Simard, M. Taras, P. De Nardo, G. Monorchio, D. Onorato, G. Sciacca, C. Martinelli, M. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Brau, J. Frey, R. Sinev, N. B. Strom, D. Torrence, E. Feltresi, E. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph. Marchiori, G. Ocariz, J. Sitt, S. Biasini, M. Manoni, E. Pacetti, S. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Cervelli, A. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Perez, A. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Gioi, L. Li Piredda, G. Buenger, C. Gruenberg, O. Hartmann, T. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. de Monchenault, G. Hamel Vasseur, G. Yeche, Ch. Anulli, F. Aston, D. Bard, D. J. Benitez, J. F. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Gabareen, A. M. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Kocian, M. L. Leith, D. W. G. S. Lewis, P. Lindemann, D. Lindquist, B. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Nelson, S. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Salnikov, A. A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wagner, A. P. Wang, W. F. Wisniewski, W. J. Wittgen, M. Wright, D. H. Wulsin, H. W. Ziegler, V. Park, W. Purohit, M. V. White, R. M. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Miyashita, T. S. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Ruland, A. M. Schwitters, R. F. Wray, B. C. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Zambito, S. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Villanueva-Perez, P. Ahmed, H. Albert, J. Banerjee, Sw. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BaBar Collaboration TI Measurement of an excess of (B)over-bar -> D-(*) tau(-)(v)over-bar(tau) decays and implications for charged Higgs bosons SO PHYSICAL REVIEW D LA English DT Article ID HIGH-ENERGY-PHYSICS; B-MESON DECAYS; BABAR DETECTOR; FORM-FACTORS; MODEL AB Based on the full BABAR data sample, we report improved measurements of the ratios R(D) = B((B) over bar -> D tau(-)(v) over bar (tau))/B((B) over bar -> Dl(-)(v) over bar (l)) and R(D*) = B((B) over bar -> D*tau(-)(v) over bar (tau))/B((B) over bar -> D*l(-)(v) over bar (l)), where l refers to either an electron or muon. These ratios are sensitive to new physics contributions in the form of a charged Higgs boson. We measure R(D) = 0.440 +/- 0.058 +/- 0.042 and R(D*) = 0.332 +/- 0.024 +/- 0.018, which exceed the standard model expectations by 2.0 sigma and 2.7 sigma, respectively. Taken together, the results disagree with these expectations at the 3.4 sigma level. This excess cannot be explained by a charged Higgs boson in the type II two-Higgs-doublet model. Kinematic distributions presented here exclude large portions of the more general type III two-Higgs-doublet model, but there are solutions within this model compatible with the results. C1 [Lees, J. P.; Poireau, V.; Tisserand, V.] Univ Savoie, CNRS, IN2P3, Lab Annecy Le Vieux Phys Particules, F-74941 Annecy Le Vieux, France. [Grauges, E.] Univ Barcelona, Dept ECM, Fac Fis, E-08028 Barcelona, Spain. [Palano, A.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Palano, A.] Univ Bari, Dipartimento Fis, I-70126 Bari, Italy. 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[Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Cervelli, A.; Forti, F.; Giorgi, M. A.; Oberhof, B.; Paoloni, E.; Rizzo, G.] Univ Pisa, Dipartimento Fis, I-56127 Pisa, Italy. [Lusiani, A.] Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Pegna, D. Lopes; Olsen, J.; Smith, A. J. S.] Princeton Univ, Princeton, NJ 08544 USA. [Faccini, R.; Ferrarotto, F.; Ferroni, F.; Gaspero, M.; Gioi, L. Li; Piredda, G.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Faccini, R.; Ferroni, F.; Gaspero, M.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Buenger, C.; Gruenberg, O.; Hartmann, T.; Leddig, T.; Voss, C.; Waldi, R.] Univ Rostock, D-18051 Rostock, Germany. [Adye, T.; Olaiya, E. O.; Wilson, F. F.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Emery, S.; de Monchenault, G. Hamel; Vasseur, G.; Yeche, Ch.] CEA, Irfu, SPP, Ctr Saclay, F-91191 Gif Sur Yvette, France. [Anulli, F.; Aston, D.; Bard, D. J.; Benitez, J. F.; Cartaro, C.; Convery, M. R.; Dorfan, J.; Dubois-Felsmann, G. P.; Dunwoodie, W.; Ebert, M.; Field, R. C.; Fulsom, B. G.; Gabareen, A. M.; Graham, M. T.; Hast, C.; Innes, W. R.; Kim, P.; Kocian, M. L.; Leith, D. W. G. S.; Lewis, P.; Lindemann, D.; Lindquist, B.; Luitz, S.; Luth, V.; Lynch, H. L.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Nelson, S.; Perl, M.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Salnikov, A. A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wagner, A. P.; Wang, W. F.; Wisniewski, W. J.; Wittgen, M.; Wright, D. H.; Wulsin, H. W.; Ziegler, V.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Park, W.; Purohit, M. V.; White, R. M.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Miyashita, T. S.; Puccio, E. M. T.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.] SUNY Albany, New York, NY 12222 USA. [Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Ruland, A. M.; Schwitters, R. F.; Wray, B. C.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; De Mori, F.; Filippi, A.; Gamba, D.; Zambito, S.] Ist Nazl Fis Nucl, Sez Torino, Turin, Italy. [Bianchi, F.; De Mori, F.; Gamba, D.; Zambito, S.] Univ Turin, Dipartimento Fis Sperimentale, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.; Villanueva-Perez, P.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Ahmed, H.; Albert, J.; Banerjee, Sw.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Godang, R.] Univ S Alabama, Mobile, AL 36688 USA. RP Lees, JP (reprint author), Univ Savoie, CNRS, IN2P3, Lab Annecy Le Vieux Phys Particules, F-74941 Annecy Le Vieux, France. RI Morandin, Mauro/A-3308-2016; Lusiani, Alberto/A-3329-2016; Di Lodovico, Francesca/L-9109-2016; Calcaterra, Alessandro/P-5260-2015; Frey, Raymond/E-2830-2016; Lo Vetere, Maurizio/J-5049-2012; Lusiani, Alberto/N-2976-2015; Patrignani, Claudia/C-5223-2009; Monge, Maria Roberta/G-9127-2012; Forti, Francesco/H-3035-2011; Oyanguren, Arantza/K-6454-2014; Luppi, Eleonora/A-4902-2015; White, Ryan/E-2979-2015; Kravchenko, Evgeniy/F-5457-2015; Calabrese, Roberto/G-4405-2015; Martinez Vidal, F*/L-7563-2014; Kolomensky, Yury/I-3510-2015 OI Morandin, Mauro/0000-0003-4708-4240; Lusiani, Alberto/0000-0002-6876-3288; Di Lodovico, Francesca/0000-0003-3952-2175; Calcaterra, Alessandro/0000-0003-2670-4826; Frey, Raymond/0000-0003-0341-2636; Lo Vetere, Maurizio/0000-0002-6520-4480; Lusiani, Alberto/0000-0002-6876-3288; Patrignani, Claudia/0000-0002-5882-1747; Monge, Maria Roberta/0000-0003-1633-3195; Forti, Francesco/0000-0001-6535-7965; Oyanguren, Arantza/0000-0002-8240-7300; Luppi, Eleonora/0000-0002-1072-5633; White, Ryan/0000-0003-3589-5900; Calabrese, Roberto/0000-0002-1354-5400; Martinez Vidal, F*/0000-0001-6841-6035; Kolomensky, Yury/0000-0001-8496-9975 FU Natural Sciences and Engineering Research Council (Canada); Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany); Istituto Nazionale di Fisica Nucleare (Italy); Foundation for Fundamental Research on Matter (Netherlands); Research Council of Norway; Ministry of Education and Science of the Russian Federation; Science and Technology Facilities Council (United Kingdom); Marie-Curie IEF program (European Union); A. P. Sloan Foundation (USA); U.S. Department of Energy and National Science Foundation; Ministerio de Economia y Competitividad (Spain) FX The concept for this analysis is to a large degree based on earlier BABAR work and we acknowledge the guidance provided by M. Mazur. The authors consulted with theorists A. Datta, S. Westhoff, S. Fajfer, J. Kamenik, and I. Nisandzic on the calculations of the charged Higgs contributions to the decay rates. We are grateful for the extraordinary contributions of our PEP-II colleagues in achieving the excellent luminosity and machine conditions that have made this work possible. The success of this project also relied critically on the expertise and dedication of the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and the kind hospitality extended to them. This work is supported by the U.S. Department of Energy and National Science Foundation, the Natural Sciences and Engineering Research Council (Canada), the Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France), the Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany), the Istituto Nazionale di Fisica Nucleare (Italy), the Foundation for Fundamental Research on Matter (Netherlands), the Research Council of Norway, the Ministry of Education and Science of the Russian Federation, Ministerio de Economia y Competitividad (Spain), and the Science and Technology Facilities Council (United Kingdom). Individuals have received support from the Marie-Curie IEF program (European Union) and the A. P. Sloan Foundation (USA). NR 47 TC 90 Z9 90 U1 1 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD OCT 31 PY 2013 VL 88 IS 7 AR 072012 DI 10.1103/PhysRevD.88.072012 PG 30 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 244LY UT WOS:000326391400003 ER PT J AU Griest, K Cieplak, AM Lehner, MJ AF Griest, Kim Cieplak, Agnieszka M. Lehner, Matthew J. TI New Limits on Primordial Black Hole Dark Matter from an Analysis of Kepler Source Microlensing Data SO PHYSICAL REVIEW LETTERS LA English DT Article ID GALACTIC HALO; MAGELLANIC CLOUDS; MACHO PROJECT; STARS AB We present new limits on the allowed masses of a dark matter (DM) halo consisting of primordial black holes (PBH) (or any other massive compact halo object). We analyze two years of data from the Kepler satellite, searching for short-duration bumps caused by gravitational microlensing. After removing background events consisting of variable stars, flare events, and comets or asteroids moving through the Kepler field, we find no microlensing candidates. We measure the efficiency of our selection criteria by adding millions of simulated microlensing lensing events into the Kepler light curves. We find that PBH DM with masses in the range 2 x 10(-9)M(circle dot) to 10(-7)M(circle dot) cannot make up the entirety of the DM in the Milky Way. At the low-mass end, this decreases the allowed mass range by more than an order of magnititude. C1 [Griest, Kim; Cieplak, Agnieszka M.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Lehner, Matthew J.] Acad Sinica, Inst Astron & Astrophys, Taipei 106, Taiwan. [Lehner, Matthew J.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Cieplak, Agnieszka M.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Griest, K (reprint author), Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. EM kgriest@ucsd.edu; acieplak@ucsd.edu; mlehner@asiaa.sinica.edu.tw OI Lehner, Matthew/0000-0003-4077-0985 FU DOE [DE-FG03-97ER40546, DE-SC0009919]; National Science Foundation Graduate Research Fellowship [DGE0707423]; NASA [NAS5-26555]; NASA Office of Space Science [NNX09AF08G] FX K. G. and A. M. C. were supported in part by the DOE under Grants No. DE-FG03-97ER40546 and No. DE-SC0009919. A. M. C. was supported in part by the National Science Foundation Graduate Research Fellowship under Grant No. DGE0707423. Some of the data presented in this Letter were obtained from the Multimission Archive at the Space Telescope Science Institute (MAST). STScI is operated by the Association of Universities for Research in Astronomy, Inc., under NASA Contract No. NAS5-26555. Support for MAST for non-HST data is provided by the NASA Office of Space Science via Grant No. NNX09AF08G and by other grants and contracts. NR 29 TC 26 Z9 26 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 31 PY 2013 VL 111 IS 18 AR 181302 DI 10.1103/PhysRevLett.111.181302 PG 5 WC Physics, Multidisciplinary SC Physics GA 244ML UT WOS:000326393000004 PM 24237504 ER PT J AU Plechaty, C Presura, R Esaulov, AA AF Plechaty, C. Presura, R. Esaulov, A. A. TI Focusing of an Explosive Plasma Expansion in a Transverse Magnetic Field SO PHYSICAL REVIEW LETTERS LA English DT Article ID LASER-PRODUCED PLASMA; HYBRID-DRIFT INSTABILITY; JETS; MECHANISM; MOTION; SPACE AB The dynamics of a laser ablation plasma expanding in an external magnetic field have been investigated with imaging interferometry and shadowgraphy. The diagnostics reveal a new interaction mechanism, namely, the redirection of the explosive plasma expansion into a converging flow. A comparison with three-dimensional ideal magnetohydrodynamic simulation results supports the observation that the efficient lateral plasma confinement causes the plasma to converge on the axis and initiate a directed flow. The resulting collimated flow propagates across the magnetic field in a kinetic regime, which cannot be modeled within the same framework. C1 [Plechaty, C.; Presura, R.; Esaulov, A. A.] Univ Nevada, Reno, NV 89557 USA. RP Plechaty, C (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM plechaty5@llnl.gov; presura@unr.edu; esaulov@unr.edu FU U.S. DOE [DE-FC52-06NA27616] FX The authors would like to thank Dr. Sandra Stein, Leela O'Brien, Showera Haque, and Matthew Tooth for their help during the experiment, and Dr. Gennady Sarkisov for designing the interferometry and shadow diagnostics. This work was performed at the Nevada Terawatt Facility and supported by the U.S. DOE under Cooperative Agreement No. DE-FC52-06NA27616. NR 25 TC 11 Z9 11 U1 4 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 31 PY 2013 VL 111 IS 18 AR 185002 DI 10.1103/PhysRevLett.111.185002 PG 5 WC Physics, Multidisciplinary SC Physics GA 244ML UT WOS:000326393000009 PM 24237528 ER PT J AU Hu, Q Xu, DH Zhou, Y Peng, RW Fan, RH Fang, NX Wang, QJ Huang, XR Wang, M AF Hu, Qing Xu, Di-Hu Zhou, Yu Peng, Ru-Wen Fan, Ren-Hao Fang, Nicholas X. Wang, Qian-Jin Huang, Xian-Rong Wang, Mu TI Position-sensitive spectral splitting with a plasmonic nanowire on silicon chip SO SCIENTIFIC REPORTS LA English DT Article ID GRATING COUPLERS; ON-INSULATOR; SILVER NANOWIRES; WAVE-GUIDES; LIGHT; PROPAGATION; TECHNOLOGY; DETECTOR; MICROSCOPY; PHOTONICS AB On-chip nanophotonics serves as the foundation for the new generation of information technology, but it is challenged by the diffraction limit of light. With the capabilities of confining light into (deep) subwavelength volumes, plasmonics makes it possible to dramatically miniaturize optical devices so as to integrate them into silicon chips. Here we demonstrate that by cascading nano-corrugation gratings with different periodicities on silver nanowires atop silicon, different colors can be spatially separated and chronologically released at different grating junctions. The released light frequency depends on the grating arrangement and corrugation periodicities. Hence the nanowire acts as a spectral splitter for sorting/demultiplexing photons at different nano-scale positions with a ten-femtosecond-level interval. Such nanowires can be constructed further into compact 2D networks or circuits. We believe that this study provides a new and promising approach for realizing spatiotemporal-sensitive spectral splitting and optical signal processing on nanoscales, and for general integration of nanophotonics with microelectronics. C1 [Hu, Qing; Xu, Di-Hu; Zhou, Yu; Peng, Ru-Wen; Fan, Ren-Hao; Wang, Qian-Jin; Wang, Mu] Nanjing Univ, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. [Hu, Qing; Xu, Di-Hu; Zhou, Yu; Peng, Ru-Wen; Fan, Ren-Hao; Wang, Qian-Jin; Wang, Mu] Nanjing Univ, Dept Phys, Nanjing 210093, Jiangsu, Peoples R China. [Hu, Qing; Fang, Nicholas X.] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Huang, Xian-Rong] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Wang, M (reprint author), Nanjing Univ, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. EM rwpeng@nju.edu.cn; muwang@nju.edu.cn RI Fang, Nicholas/A-5856-2008; Arumugam, Thirumagal/C-3408-2014 OI Fang, Nicholas/0000-0001-5713-629X; FU Ministry of Science and Technology of China [2012CB921502, 2010CB630705]; National Science Foundation of China [11034005, 61077023, 11021403]; Ministry of Education of China [20100091110029]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; NSF [CMMI-1120724] FX This work was supported by the Ministry of Science and Technology of China (Grant Nos. 2012CB921502 and 2010CB630705), the National Science Foundation of China (Grant Nos. 11034005, 61077023, and 11021403), and partly by the Ministry of Education of China (20100091110029). XRH was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NXF acknowledges partial support by NSF Grant no. CMMI-1120724. NR 57 TC 16 Z9 17 U1 4 U2 52 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 31 PY 2013 VL 3 AR 3095 DI 10.1038/srep03095 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 243QZ UT WOS:000326333300004 PM 24172838 ER PT J AU Ma, CR Liu, M Chen, CL Lin, Y Li, YR Horwitz, JS Jiang, JC Meletis, EI Zhang, QY AF Ma, Chunrui Liu, Ming Chen, Chonglin Lin, Yuan Li, Yanrong Horwitz, J. S. Jiang, Jiechao Meletis, E. I. Zhang, Qingyu TI The Origin of Local Strain in Highly Epitaxial Oxide Thin Films SO SCIENTIFIC REPORTS LA English DT Article ID DIELECTRIC-PROPERTIES; TRANSPORT-PROPERTIES; 001 MGO; MAGNETORESISTANCE; FERROELECTRICITY; SRTIO3; HETEROSTRUCTURES; SURFACES AB The ability to control the microstructures and physical properties of hetero-epitaxial functional oxide thin films and artificial structures is a long-sought goal in functional materials research. Normally, only the lattice misfit between the film and the substrate is considered to govern the physical properties of the epitaxial films. In fact, the mismatch of film unit cell arrangement and the Surface-Step-Terrace (SST) dimension of the substrate, named as "SST residual matching", is another key factor that significantly influence the properties of the epitaxial film. The nature of strong local strain induced from both lattice mismatch and the SST residual matching on ferroelectric (Ba,Sr)TiO3 and ferromagnetic (La,Ca) MnO3 thin films are systematically investigated and it is demonstrated that this combined effect has a dramatic impact on the physical properties of highly epitaxial oxide thin films. A giant anomalous magnetoresistance effect (similar to 10(10)) was achieved from the as-designed vicinal surfaces. C1 [Ma, Chunrui; Chen, Chonglin] Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA. [Liu, Ming] Xi An Jiao Tong Univ, Minist Educ, Key Lab, Elect Mat Res Lab, Xian 710049, Peoples R China. [Liu, Ming] Xi An Jiao Tong Univ, Int Ctr Dielect Res, Xian 710049, Peoples R China. [Chen, Chonglin] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Lin, Yuan; Li, Yanrong] Univ Elect Sci & Technol China, State Key Lab Elect Thin Films & Integrated Devic, Chengdu 610054, Sichuan, Peoples R China. [Horwitz, J. S.] US DOE, Germantown, MD 20585 USA. [Jiang, Jiechao; Meletis, E. I.] Univ Texas Arlington, Arlington, TX 76019 USA. [Zhang, Qingyu] Dalian Univ Technol, Key Lab Mat Modificat Laser, Dalian 116024, Peoples R China. RP Chen, CL (reprint author), Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA. EM cl.chen@utsa.edu RI lin, yuan/B-9955-2013; Zhang, Qingyu/O-8472-2015 FU National Science Foundation [NSF-NIRT-0709293]; Natural Science Foundation of China [11329402, 18110225]; Department of Energy [DE-FE0003780]; State of Texas through the Texas Center for Superconductivity at the University of Houston; China Scholarship Council FX This research was partially supported by the National Science Foundation under NSF-NIRT-0709293, the Natural Science Foundation of China under 11329402 and 18110225, the Department of Energy under DE-FE0003780, and the State of Texas through the Texas Center for Superconductivity at the University of Houston. We would like to thank Dr. HD Wu for the dielectric property measurements of the BSTO films. Also, Dr. Ming Liu and Dr. Chunrui Ma would like to acknowledge the support from the "China Scholarship Council" for the program of national study-abroad project for the postgraduates of high level universities at UTSA. NR 30 TC 8 Z9 8 U1 5 U2 81 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 31 PY 2013 VL 3 AR 3092 DI 10.1038/srep03092 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 243QZ UT WOS:000326333300001 PM 24172706 ER PT J AU Di Leo, RA Marschilok, AC Takeuchi, KJ Takeuchi, ES AF Di Leo, Roberta A. Marschilok, Amy C. Takeuchi, Kenneth J. Takeuchi, Esther S. TI Battery electrolytes based on saturated ring ionic liquids: Physical and electrochemical properties SO ELECTROCHIMICA ACTA LA English DT Article DE Ionic liquid; Lithium battery; Electrolyte; Conductivity; High voltage stability ID LITHIUM BATTERY; CONDUCTIVITY; VISCOSITY; STABILITY; CARBONATE; MIXTURES; CELLS AB Physical and electrochemical properties of mixtures of ionic liquids based on saturated ring systems with carbonate based solvents were investigated. The conductivity and electrochemical stability of two series of ionic liquids based on piperidinium and pyrrolidinium cations with tetrafluoroborate and bis(trifluorosulfonylimide) anions were evaluated. The effects of the ionic liquid cation, substituent chain length of the cation function group, and the anion type on conductivity and electrochemical stability as determined by cyclic voltammetry were studied. The conductivity was influenced by the substituent chain length of the ionic liquid cation and the solvent carbonate type, where higher conductivities were observed with shorter substituent chains and EC versus PC. The saturated ring ionic liquid-carbonate mixtures may show particular promise for implementation as battery electrolytes due to notable high voltage stabilities, where stability >5.5 V was maintained in the presence of lithium salt. This study should promote development of future safe, high voltage lithium ion battery systems. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Di Leo, Roberta A.; Marschilok, Amy C.; Takeuchi, Kenneth J.; Takeuchi, Esther S.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Di Leo, Roberta A.; Marschilok, Amy C.; Takeuchi, Esther S.] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. [Takeuchi, Esther S.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Marschilok, AC (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM amy.marschilok@stonybrook.edu; kenneth.takeuchi.1@stonybrook.edu; esther.takeuchi@stonybrook.edu RI Takeuchi, Esther/D-1825-2014; Marschilok, Amy/D-1821-2014 FU Intelligence Community Postdoctoral Research Fellowship Program through Office of the Director of National Intelligence FX This project was supported by a grant from the Intelligence Community Postdoctoral Research Fellowship Program through funding from the Office of the Director of National Intelligence. NR 27 TC 10 Z9 10 U1 1 U2 28 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD OCT 30 PY 2013 VL 109 BP 27 EP 32 DI 10.1016/j.electacta.2013.07.041 PG 6 WC Electrochemistry SC Electrochemistry GA 266EN UT WOS:000328006300004 ER PT J AU Ren, K McConnell, CA Gan, YX Afjeh, AA Zhang, LH AF Ren, Kai McConnell, Courtney A. Gan, Yong X. Afjeh, Abdollah A. Zhang, Lihua TI Magnetic field enhanced photoelectrochemical response of a nanostructured titanium dioxide anode SO ELECTROCHIMICA ACTA LA English DT Article DE Photoelectrochemical fuel cell; Response to magnet field; Photon excitation; TiO2 nanotube ID TIO2 NANOTUBE ARRAYS; SENSITIZED SOLAR-CELLS; FUEL-CELLS; WASTE-WATER; FABRICATION; ELECTRODE; SEMICONDUCTOR; PERFORMANCE; PROGRESS; SENSORS AB The concept of permanent-magnet photoelectrochemical fuel cell is proposed. The fuel cell contains a TiO2 nanotube anode and a platinum cathode. Water was used as the fuel. The anode has a self-organized high aspect ratio TiO2 nanotube layer made through electrochemical oxidation of Ti. Photocatalysis and permanent magnetic field excitation experiments were performed. The photoelectrochemical responses of the anode to visible (Vis) and ultraviolet (UV) light were studied to examine the magnetic field effect. The open circuit voltages were 0.0564, 0.1625, 0.1898 and 0.376 V. under the excitation of Vis, UV, magnet and magnet + UV, respectively. Current density was measured under different linear potential scanning conditions. It reached a value of 5.23 mA/m(2) just under the excitation of the permanent magnet at a bias voltage of 2 V. Combining the magnetic action and the photovoltaic effect, the titanium dioxide photosensitive anode showed a maximum photocurrent density of 296.05 mA/m(2) at 2 V bias. It is concluded that the absolute value of open circuit voltage (OCV) of the fuel cell due to the exposure to the magnet field is much higher than that due to either UV or Vis light illumination. However, UV light excitation results in higher current density in the measurement. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Ren, Kai; Gan, Yong X.; Afjeh, Abdollah A.] Univ Toledo, Dept Mech Ind & Mfg Engn, Toledo, OH 43606 USA. [McConnell, Courtney A.; Gan, Yong X.] Calif State Polytech Univ Pomona, Dept Mech Engn, Pomona, CA 91768 USA. [Zhang, Lihua] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Gan, YX (reprint author), Calif State Polytech Univ Pomona, Dept Mech Engn, 3801 W Temple Ave, Pomona, CA 91768 USA. EM yxgan@csupomona.edu RI Zhang, Lihua/F-4502-2014 FU US Environmental Protection Agency [SU83529701]; Kellogg Foundation; US Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported in part by the US Environmental Protection Agency under Grant Number SU83529701 and the Kellogg Foundation. The electron microscopic research carried out in the Center for Functional Nanomaterials at Brookhaven National Laboratory is supported by the US Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. We appreciate Kathryn Rose for correcting English. NR 30 TC 4 Z9 4 U1 3 U2 26 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD OCT 30 PY 2013 VL 109 BP 162 EP 167 DI 10.1016/j.electacta.2013.07.081 PG 6 WC Electrochemistry SC Electrochemistry GA 266EN UT WOS:000328006300022 ER PT J AU Xiao, N Li, DY Cui, GF Li, N Tian, D Li, Q Wu, G AF Xiao, Ning Li, Deyu Cui, Guofeng Li, Ning Tian, Dong Li, Qing Wu, Gang TI An effective triblock copolymer as a suppressor for microvia filling via copper electrodeposition SO ELECTROCHIMICA ACTA LA English DT Article DE Microvia filling; Copper electroplating; Suppressor; Triblock copolymer; Adsorbing mechanism ID POLYETHYLENE-GLYCOL; CHLORIDE-ION; PEG; DEPOSITION; SPS; CU; CL; INHIBITION; ADSORPTION; KINETICS AB In this work, an effective suppressor was found in copper electroplating solution for microvia filling. The suppressor is a triblock copolymer comprised of ethylene oxide (EO)-propylene oxide (PO)-ethylene oxide (EO) with a molecular weight of 2900 (EPE 2900). In terms of the obtained filling performance evaluated by observing the obtained cross-sectional views of the microvias after electroplating, the electroplating solution was systematically studied as functions of Cl- concentration, EPE 2900 concentration, and convection conditions. It was found that filling performance was greatly dependent on these key factors. In the developed copper electroplating formulation, EPE 2900 was able to yield sufficient filling performance in a broad Cl- concentration ranging from 3 to 200 ppm, although the optimized value was determined to be about 30 ppm in terms of the best filling performance. During the microvia filling process, Cl- concentration, EPE 2900 concentration, and forced convection would affect each other. Their interactions were studied based on the anchor effect of Cl- on the adsorption of EPE 2900 on Cu substrates. In doing so, extensive electrochemical experiments including galvanostatic measurements, linear sweep voltammetry, electrochemical impedance spectroscopy and cyclic voltammetry were employed to study the adsorption behavior of EPE 2900 on the cathode during both the copper electrodeposition and dissolution processes. An adsorbing mechanism of EPE 2900 on cathode was proposed to elucidate the promotional role in improving the microvia filling performance. (C) 2013 Published by Elsevier Ltd. C1 [Xiao, Ning; Li, Deyu; Li, Ning; Tian, Dong] Harbin Inst Technol, Dept Appl Chem, Harbin 150001, Peoples R China. [Cui, Guofeng] Sun Yat Sen Univ, Sch Chem & Chem Engn, Guangzhou 510275, Guangdong, Peoples R China. [Li, Qing; Wu, Gang] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Li, N (reprint author), Harbin Inst Technol, Dept Appl Chem, Harbin 150001, Peoples R China. EM lininghit@263.net; wugang@lanl.gov RI Wu, Gang/E-8536-2010; Li, Qing/G-4502-2011 OI Wu, Gang/0000-0003-4956-5208; Li, Qing/0000-0003-4807-030X FU Highnic Group (China) FX This work was financially supported by Highnic Group (China). NR 34 TC 5 Z9 5 U1 5 U2 40 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD OCT 30 PY 2013 VL 109 BP 226 EP 232 DI 10.1016/j.electacta.2013.07.127 PG 7 WC Electrochemistry SC Electrochemistry GA 266EN UT WOS:000328006300032 ER PT J AU Komanicky, V Hennessy, DC Iddir, H Zapol, P You, H AF Komanicky, Vladimir Hennessy, Daniel C. Iddir, Hakim Zapol, Peter You, Hoydoo TI Electrocatalytic activity of surface oxides on platinum nanofacets and surfaces SO ELECTROCHIMICA ACTA LA English DT Article DE Platinum catalysts; CO electrooxidation; Bifunctional catalysts; X-rays, DFT ID DENSITY-FUNCTIONAL THEORY; X-RAY-SCATTERING; OXYGEN REDUCTION; PT(100) SURFACE; PT(111); CO; ELECTRODES; OXIDATION; COVERAGE; PT(311) AB We investigated electrochemical behavior of surface oxides of platinum formed by annealing in air. We studied the catalytic activity for CO electrooxidation using electrochemical, X-ray, and DFT methods. We find that all oxidized platinum surfaces are highly active initially for CO electrooxidation reaction in so-called preignition region. While the high activity of the monolayer oxide formed on extended Pt surfaces decreases after the initial CO-oxidation cycle, bilayer oxide formed on nanoscaled facets sustain the high CO electrooxidation activity. DFT calculations show that OH binds, as strongly to bilayer surface oxides as to metallic surface while CO does not, suggesting the bifunctional property of the bilayer oxide surface. Published by Elsevier Ltd. C1 [Komanicky, Vladimir] Safarik Univ, Fac Sci, Kosice 04001, Slovakia. [Hennessy, Daniel C.; Iddir, Hakim; Zapol, Peter; You, Hoydoo] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Komanicky, V (reprint author), Safarik Univ, Fac Sci, Kosice 04001, Slovakia. EM vladimir.komanicky@upjs.sk; hyou@anl.gov RI Zapol, Peter/G-1810-2012; You, Hoydoo/A-6201-2011 OI Zapol, Peter/0000-0003-0570-9169; You, Hoydoo/0000-0003-2996-9483 FU U.S. DOE, BES [DE-AC02-06CH11357]; Slovak grant [VEGA 1/0782/12]; ERDF EU [ITMS 26220120005] FX The work at ANL and the use of the APS were supported by the U.S. DOE, BES, under contract No. DE-AC02-06CH11357 and the work at Safarik University are supported by Slovak grant VEGA 1/0782/12 and ERDF EU grant under contract No. ITMS 26220120005. NR 22 TC 1 Z9 1 U1 1 U2 21 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD OCT 30 PY 2013 VL 109 BP 440 EP 446 DI 10.1016/j.electacta.2013.07.098 PG 7 WC Electrochemistry SC Electrochemistry GA 266EN UT WOS:000328006300062 ER PT J AU Datta, S Henry, MP Lin, YJ Fracaro, AT Millard, CS Snyder, SW Stiles, RL Shah, J Yuan, JW Wesoloski, L Dorner, RW Carlson, WM AF Datta, Saurav Henry, Michael P. Lin, YuPo J. Fracaro, Anthony T. Millard, Cynthia S. Snyder, Seth W. Stiles, Rebecca L. Shah, Jitendra Yuan, Jianwei Wesoloski, Lisa Dorner, Robert W. Carlson, Wayne M. TI Electrochemical CO2 Capture Using Resin-Wafer Electrodeionization SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID PRESSURE SWING ADSORPTION; CARBON-DIOXIDE CAPTURE; FLUE-GASES; IONIC LIQUID; TECHNOLOGY; SEPARATION; MEMBRANE; WATER; ELECTRODIALYSIS; EFFICIENT AB Energy-efficient capture of CO2 from power-plant flue gas is one of the grand challenges to reduce greenhouse gas (GHG) emissions. Current CO2-capture technologies are limited by parasitic energy loss, inefficient capture, and unfavorable process economics. We present a novel electrochemical method for CO2 capture from coal-fired power-plant flue gas. The method utilizes in-situ electrochemical pH control with a resin wafer electrodeionization (RW-EDI) device that continuously shifts the pH of the process fluid between basic and acidic in sequential chambers (pH swing). This pH swing enables capture of CO2 from flue gas in the basic chamber followed by release (recovery) of the captured CO2 (purified) in the acidic chamber of the same device. The approach is based on the sensitivity of the thermodynamic equilibrium of CO2 hydration/dehydration reactions over a narrow pH range. The method enables simultaneous absorption (capture) of CO2 from flue gas and desorption (release) at atmospheric pressure without heating, vacuum, or consumptive chemical usage. In other words, the method concentrates CO2 from similar to 15% in flue gas to >98% in the recovery stream. To the best of our knowledge, this is the first experimental study focusing on simultaneous capture and release (recovery) of CO2 using an electrochemical method. We describe the method, the role of operating parameters on CO2 recovery, and advancements in process design and engineering for improved efficiency. We report on a method to enhance gas/liquid mixing inside the RW-EDI, which significantly increased CO2 capture rates. We also discuss the importance of using an enzyme/catalyst in enhancing the reaction kinetics. CO2 capture was observed to be a strong function of gas and liquid flow rates and applied electrical field. Up to 80% of the CO2 was captured from a simulated flue gas stream with >98% purity. The results indicate that a narrow pH swing from 8 to 6 (near-neutral pH) could offer a viable pathway for energy-efficient CO2 capture if the reaction kinetics are enhanced. Carbonic anhydrase enzyme enhances the reaction kinetics at near-neutral pH; however, the enzyme lost activity due to the instability at the operating conditions. This observation highlighted the necessity of robust enzymes/catalysts to enhance kinetics of CO2 recovery nearneutral pH. C1 [Datta, Saurav; Henry, Michael P.; Lin, YuPo J.; Fracaro, Anthony T.; Millard, Cynthia S.; Snyder, Seth W.] Argonne Natl Lab, Argonne, IL 60439 USA. [Stiles, Rebecca L.; Shah, Jitendra; Yuan, Jianwei; Wesoloski, Lisa; Dorner, Robert W.; Carlson, Wayne M.] Nalco Co, Air Protect Technol, Naperville, IL 60563 USA. RP Snyder, SW (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM seth@anl.gov FU DOE Advanced Research Project Agency-Energy (ARPA-E) [DE-FOA-0000065]; DOE Fossil Energy program [DE-PS26-06NT42829-0]; U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX We acknowledge the DOE Advanced Research Project Agency-Energy (ARPA-E) for financial support of this research (Funding Opportunity Number DE-FOA-0000065). The discovery phase of this research was supported by the DOE Fossil Energy program (Funding Opportunity Number DE-PS26-06NT42829-0). The discovery phase work was led by Dr. Michael C. Trachtenberg, Carbozyme, Inc. We thank Dr. Manian Ramesh, Nalco (retired) for his guidance and leadership on assembling the team.; The submitted manuscript was created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 53 TC 7 Z9 7 U1 5 U2 55 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 EI 1520-5045 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD OCT 30 PY 2013 VL 52 IS 43 BP 15177 EP 15186 DI 10.1021/ie402538d PG 10 WC Engineering, Chemical SC Engineering GA 245TZ UT WOS:000326488000020 ER PT J AU Carboni, M Abney, CW Taylor-Pashow, KML Vivero-Escoto, JL Lin, WB AF Carboni, Michael Abney, Carter W. Taylor-Pashow, Kathryn M. L. Vivero-Escoto, Juan L. Lin, Wenbin TI Uranium Sorption with Functionalized Mesoporous Carbon Materials SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID SURFACE FUNCTIONALIZATION; HIGHLY EFFICIENT; AQUEOUS-SOLUTION; SEAWATER; RECOVERY; U(VI); ACID; PHOSPHONATE; ADSORPTION; EXTRACTION AB A series of functionalized mesoporous carbon (MC) materials were prepared by covalent grafting with amidoxime, carboxyl, and phosphoryl functional groups and screened for uranium (U) sorption from aqueous media. The MC materials were characterized by nitrogen adsorption measurements and thermogravimetric analysis and investigated for U(VI) extraction from both acidic water (pH 4) and artificial seawater (pH 8.2). Under both conditions, a phosphoric acid-functionalized MC exhibited the highest U(VI) sorption, with a maximum sorption capacity of 97 mg of U(VI)/(g of sorbent) in acidic water and 67 mg of U(VI)/(g of sorbent) in artificial seawater. The effects of pH on U(VI) sorption, sorption kinetics, and sorption isotherms were obtained for the phosphoric acid-functionalized MC. Quantitative U(VI) removal from U(VI)-loaded sorbents was achieved by washing with HCl at concentrations higher than 0.01 M. These results indicate that functionalized MC provides a promising platform for the development of novel sorbents for efficient U(VI) extraction. C1 [Carboni, Michael; Abney, Carter W.; Lin, Wenbin] Univ Chicago, Dept Chem, Chicago, IL 60637 USA. [Taylor-Pashow, Kathryn M. L.] Savannah River Natl Lab, Aiken, SC 29808 USA. [Vivero-Escoto, Juan L.] Univ N Carolina, Dept Chem, Charlotte, NC 28223 USA. RP Lin, WB (reprint author), Univ Chicago, Dept Chem, 929 E 57th St, Chicago, IL 60637 USA. EM wenbinlin@uchicago.edu RI Lin, Wenbin/B-4151-2010; Vivero-Escoto, Juan/I-8015-2014; OI Lin, Wenbin/0000-0001-7035-7759; Abney, Carter/0000-0002-1809-9577 FU DOE Office of Nuclear Energy's Nuclear Energy University Program [20, 120427, 3151] FX This work was supported by the DOE Office of Nuclear Energy's Nuclear Energy University Program (Subcontract 20 #120427, Project #3151). NR 62 TC 29 Z9 29 U1 11 U2 98 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD OCT 30 PY 2013 VL 52 IS 43 BP 15187 EP 15197 DI 10.1021/ie402646r PG 11 WC Engineering, Chemical SC Engineering GA 245TZ UT WOS:000326488000021 ER PT J AU Isacoff, EY Jan, LY Minor, DL AF Isacoff, Ehud Y. Jan, Lily Y. Minor, Daniel L., Jr. TI Conduits of Life's Spark: A Perspective on Ion Channel Research since the Birth of Neuron SO NEURON LA English DT Review ID GATED SODIUM-CHANNEL; SHAKER K+ CHANNEL; NICOTINIC ACETYLCHOLINE-RECEPTOR; VOLTAGE-SENSING DOMAIN; X-RAY-STRUCTURE; HOMEOSTATIC SYNAPTIC PLASTICITY; ACTIVITY-DEPENDENT REGULATION; PROTEIN-COUPLED RECEPTORS; CELL-SURFACE EXPRESSION; EARLY SECRETORY PATHWAY AB Heartbeats, muscle twitches, and lightning-fast thoughts are all manifestations of bioelectricity and rely on the activity of a class of membrane proteins known as ion channels. The basic function of an ion channel can be distilled into, "The hole opens. Ions go through. The hole closes." Studies of the fundamental mechanisms by which this process happens and the consequences of such activity in the setting of excitable cells remains the central focus of much of the field. One might wonder after so many years of detailed poking at such a seemingly simple process, is there anything left to learn? C1 [Isacoff, Ehud Y.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Isacoff, Ehud Y.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Jan, Lily Y.; Minor, Daniel L., Jr.] Univ Calif San Francisco, Dept Biochem & Biophys, San Francisco, CA 94158 USA. [Jan, Lily Y.] Univ Calif San Francisco, Dept Physiol, San Francisco, CA 94158 USA. [Jan, Lily Y.] Univ Calif San Francisco, Dept Physiol, San Francisco, CA 94158 USA. [Jan, Lily Y.] Univ Calif San Francisco, Howard Hughes Med Inst, San Francisco, CA 94158 USA. [Minor, Daniel L., Jr.] Univ Calif San Francisco, Dept Cellular & Mol Pharmacol, San Francisco, CA 94158 USA. [Minor, Daniel L., Jr.] Univ Calif San Francisco, Cardiovasc Res Inst, San Francisco, CA 94158 USA. [Minor, Daniel L., Jr.] Univ Calif San Francisco, Calif Inst Quantitat Biomed Res, San Francisco, CA 94158 USA. [Isacoff, Ehud Y.; Minor, Daniel L., Jr.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Minor, DL (reprint author), Univ Calif San Francisco, Dept Biochem & Biophys, San Francisco, CA 94158 USA. EM daniel.minor@ucsf.edu FU NIH [R01-HL080050, R01-DC007664, R01-MH093603, U54-GM094625, R01 NS35549, R37MH065334, R01NS069229]; Howard Hughes Medical Institute FX We thank B. Hille and W.A. Catterall for assistance with the figures and K. Brejc for critical comments on the manuscript. We thank Francesco Tombola for helpful discussion. This work was supported by grants to D.L.M. from NIH R01-HL080050, R01-DC007664, R01-MH093603, and U54-GM094625 to E.Y.I. from NIH R01 NS35549, and to L.Y.J. from NIH R37MH065334, R01NS069229, and the Howard Hughes Medical Institute. NR 280 TC 12 Z9 12 U1 2 U2 28 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0896-6273 EI 1097-4199 J9 NEURON JI Neuron PD OCT 30 PY 2013 VL 80 IS 3 BP 658 EP 674 DI 10.1016/j.neuron.2013.10.040 PG 17 WC Neurosciences SC Neurosciences & Neurology GA 247IA UT WOS:000326609900012 PM 24183018 ER PT J AU Pepper, SE Ogden, MD AF Pepper, Sarah E. Ogden, Mark D. TI Perrhenate extraction studies by Cyphos 101-IL; screening for implementation in technetium removal SO SEPARATION AND PURIFICATION TECHNOLOGY LA English DT Article DE Anion exchange; Ionic liquid; Perrhenate; Solvent extraction; Technetium analogue ID HYDROCHLORIC-ACID SOLUTIONS; PHOSPHONIUM IONIC LIQUID; CHLORIDE SOLUTIONS; BIOPOLYMER CAPSULES; PICKLING SOLUTIONS; IRON IONS; RECOVERY; ZINC(II); IL-101; PALLADIUM(II) AB The solvent extraction of rhenium (VII) from chloride solutions by Cyphos 101-IL in toluene has been studied. Distribution values for the extraction of perrhenate are extremely high leading to almost quantitative extraction. From slope analysis, an anion exchange extraction mechanism is proposed, with formation of a ReO4- association with one Cyphos IL-101 cation. The extraction kinetics are fast, with complete equilibration occurring within 60 s. Under identical conditions, distribution coefficients for Cyphos 101-IL are greater than for Aliquat-336. Extraction of the perrhenate anion does not seem to be negatively impacted by common environmental contaminants including iron, sulphate and nitrate at the pH values tested. (C) 2013 Elsevier B.V. All rights reserved. C1 [Pepper, Sarah E.] Idaho Natl Lab, Idaho Falls, ID 83514 USA. [Ogden, Mark D.] ANSTO Minerals, Kirrawee Dc, NSW 2232, Australia. RP Ogden, MD (reprint author), ANSTO Minerals, Locked Bag 2001, Kirrawee Dc, NSW 2232, Australia. EM mark.ogden@ansto.gov.au FU United States Department of Energy, Office of Nuclear Energy, Science and Technology; INL Laboratory Directed Research and Development (LDRD) Program Under DOE-NE Idaho Operations Office [DE-AC07-051D14517] FX This work was supported by the United States Department of Energy, Office of Nuclear Energy, Science and Technology and the INL Laboratory Directed Research and Development (LDRD) Program Under DOE-NE Idaho Operations Office contract DE-AC07-051D14517. The authors also thank Byron White for ICP-MS data analysis. NR 42 TC 4 Z9 4 U1 4 U2 30 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1383-5866 EI 1873-3794 J9 SEP PURIF TECHNOL JI Sep. Purif. Technol. PD OCT 30 PY 2013 VL 118 BP 847 EP 852 DI 10.1016/j.seppur.2013.08.029 PG 6 WC Engineering, Chemical SC Engineering GA 252HA UT WOS:000326994500104 ER PT J AU Townson, JL Lin, YS Agola, JO Carnes, EC Leong, HS Lewis, JD Haynes, CL Brinker, CJ AF Townson, Jason L. Lin, Yu-Shen Agola, Jacob O. Carnes, Eric C. Leong, Hon S. Lewis, John D. Haynes, Christy L. Brinker, C. Jeffrey TI Re-examining the Size/Charge Paradigm: Differing in Vivo Characteristics of Size- and Charge-Matched Mesoporous Silica Nanoparticles SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CANCER-CELLS; SYSTEM AB The combination of nanoparticle (NP) size, charge, and surface chemistry (e.g., extent of modification with polyethylene glycol (PEG)) is accepted as a key determinant of NP/cellular interactions. However, the influence of spatial arrangement and accessibility of the charged molecules on the NP surface vis-a-vis the average surface charge (zeta (zeta) potential) is incompletely understood. Here we demonstrate that two types of mesoporous silica nanoparticles (MSNP) that are matched in terms of primary and hydrodynamic particle size, shape, pore structure, colloidal stability, and zeta potential, but differ in surface chemistry, viz, the spatial arrangement and relative exposure of surface amines, have profoundly different interactions with cells and tissues when evaluated in vitro and in vivo. While both particles are similar to 50 nm in diameter, PEGylated, and positively charged (zeta = +40 mV), PEG-PEI (MSNPs modified with exposed poly-amines), but not PEG-NMe3+ (MSNP modified with distributed, obstructed amines) rapidly bind serum proteins, diverse cells types in vitro, and endothelial and white blood cells in vivo (ex ovo chick embryo model). This finding helps elucidate the relative role of surface exposure of charged molecules vs zeta potential in otherwise physicochemically matched MSNP and highlights protein corona neutrality as an important design consideration when synthesizing cationic NPs for biological applications. C1 [Townson, Jason L.; Lin, Yu-Shen; Agola, Jacob O.; Brinker, C. Jeffrey] Univ New Mexico, Ctr Microengn Mat, Albuquerque, NM 87131 USA. [Brinker, C. Jeffrey] Univ New Mexico, Dept Chem Engn, Albuquerque, NM 87131 USA. [Carnes, Eric C.] Sandia Natl Labs, Nanobiol Dept, Albuquerque, NM 87185 USA. [Brinker, C. Jeffrey] Sandia Natl Labs, Self Assembled Mat Dept, Albuquerque, NM 87185 USA. [Leong, Hon S.] London Reg Canc Program, London, England. [Lewis, John D.] Univ Alberta, Dept Oncol, Edmonton, AB, Canada. [Haynes, Christy L.] Univ Minnesota, Dept Chem, Minneapolis, MN 55455 USA. RP Brinker, CJ (reprint author), Univ New Mexico, Ctr Microengn Mat, Albuquerque, NM 87131 USA. EM cjbrink@sandia.gov OI Leong, Hon/0000-0001-7801-1402 FU NIH [UO1 CA151792-01]; Gabrielle's Angel foundation; UNM CNTC; U.S. DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Sandia National Laboratories' LDRD program; AFOSR [FA 9550-10-1-0054]; NSF; EPA FX We thank Walker Wharton and Katharine Epler for helpful discussions and experimental assistance. This work was funded by NIH Grant UO1 CA151792-01. J.L.T. was supported by a Young Investigators Award from Gabrielle's Angel foundation. Y.S.L. was funded by a fellowship from The UNM CNTC. C.J.B acknowledges additional support from U.S. DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, Sandia National Laboratories' LDRD program, AFOSR grant FA 9550-10-1-0054, NSF and EPA. NR 15 TC 35 Z9 35 U1 2 U2 96 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 EI 1520-5126 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 30 PY 2013 VL 135 IS 43 BP 16030 EP 16033 DI 10.1021/ja4082414 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 245TX UT WOS:000326487800017 PM 24107191 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, MJ Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Yushkov, AN Kirkby, D Lankford, AJ Mandelkern, M Dey, B Gary, JW Long, O Vitug, GM Campagnari, C Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Ongmongkolkul, P Porter, FC Andreassen, R Huard, Z Meadows, BT Pappenheimer, C Pushpawela, BG Sokoloff, MD Sun, L Bloom, PC Ford, WT Gaz, A Nauenberg, U Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Schwierz, R Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Baldini-Ferroli, R Calcaterra, A de Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Guido, E Lo Vetere, M Monge, MR Passaggio, S Patrignani, C Robutti, E Bhuyan, B Prasad, V Morii, M Adametz, A Uwer, U Lacker, HM Dauncey, PD Mallik, U Chen, C Cochran, J Meyer, WT Prell, S Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Bougher, J Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Prencipe, E Schubert, KR Barlow, RJ Lafferty, GD Behn, E Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Dujmic, D Sciolla, G Cheaib, R Patel, PM Robertson, SH Biassoni, P Neri, N Palombo, F Cremaldi, L Godang, R Sonnek, P Summers, DJ Simard, M Taras, P De Nardo, G Monorchio, D Onorato, G Sciacca, C Martinelli, M Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Brau, J Frey, R Sinev, NB Strom, D Torrence, E Feltresi, E Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Sitt, S Biasini, M Manoni, E Pacetti, S Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Cervelli, A Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Perez, A Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Li Gioi, L Piredda, G Bunger, C Grunberg, O Hartmann, T Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S de Monchenault, GH Vasseur, G Yeche, C Anulli, F Aston, D Bard, DJ Benitez, JF Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Gabareen, AM Graham, MT Hast, C Innes, WR Kim, P Kocian, ML Leith, DWGS Lewis, P Lindemann, D Lindquist, B Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Nelson, S Perl, M Pulliam, T Ratcliff, BN Roodman, A Salnikov, AA Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wagner, AP Wang, WF Wisniewski, WJ Wittgen, M Wright, DH Wulsin, HW Ziegler, V Park, W Purohit, MV White, RM Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Miyashita, TS Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Ruland, AM Schwitters, RF Wray, BC Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Zambito, S Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Villanueva-Perez, P Ahmed, H Albert, J Banerjee, S Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lee, M. J. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Yushkov, A. N. Kirkby, D. Lankford, A. J. Mandelkern, M. Dey, B. Gary, J. W. Long, O. Vitug, G. M. Campagnari, C. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Ongmongkolkul, P. Porter, F. C. Andreassen, R. Huard, Z. Meadows, B. T. Pappenheimer, C. Pushpawela, B. G. Sokoloff, M. D. Sun, L. Bloom, P. C. Ford, W. T. Gaz, A. Nauenberg, U. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Schwierz, R. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Baldini-Ferroli, R. Calcaterra, A. de Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Guido, E. Lo Vetere, M. Monge, M. R. Passaggio, S. Patrignani, C. Robutti, E. Bhuyan, B. Prasad, V. Morii, M. Adametz, A. Uwer, U. Lacker, H. M. Dauncey, P. D. Mallik, U. Chen, C. Cochran, J. Meyer, W. T. Prell, S. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Bougher, J. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Prencipe, E. Schubert, K. R. Barlow, R. J. Lafferty, G. D. Behn, E. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Dujmic, D. Sciolla, G. Cheaib, R. Patel, P. M. Robertson, S. H. Biassoni, P. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Sonnek, P. Summers, D. J. Simard, M. Taras, P. De Nardo, G. Monorchio, D. Onorato, G. Sciacca, C. Martinelli, M. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Brau, J. Frey, R. Sinev, N. B. Strom, D. Torrence, E. Feltresi, E. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph. Marchiori, G. Ocariz, J. Sitt, S. Biasini, M. Manoni, E. Pacetti, S. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Cervelli, A. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Perez, A. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Li Gioi, L. Piredda, G. Buenger, C. Gruenberg, O. Hartmann, T. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. de Monchenault, G. Hamel Vasseur, G. Yeche, Ch. Anulli, F. Aston, D. Bard, D. J. Benitez, J. F. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Gabareen, A. M. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Kocian, M. L. Leith, D. W. G. S. Lewis, P. Lindemann, D. Lindquist, B. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Nelson, S. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Salnikov, A. A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wagner, A. P. Wang, W. F. Wisniewski, W. J. Wittgen, M. Wright, D. H. Wulsin, H. W. Ziegler, V. Park, W. Purohit, M. V. White, R. M. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Miyashita, T. S. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Ruland, A. M. Schwitters, R. F. Wray, B. C. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Zambito, S. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Villanueva-Perez, P. Ahmed, H. Albert, J. Banerjee, Sw. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BABAR Collaboration TI Measurement of the mass of the D-0 meson SO PHYSICAL REVIEW D LA English DT Article ID BABAR DETECTOR AB We report a measurement of the D-0 meson mass using the decay chain D* (2010) + -> D-0 pi(+) with D-0 -> K-K-K+pi(+). The data were recorded with the BABAR detector at center-of-mass energies at and near the Upsilon(4S) resonance, and correspond to an integrated luminosity of approximately 477 fb(-1). We obtain m(D-0) (1864: 841 +/- 0: 048 +/- 0: 063) MeV, where the quoted errors are statistical and systematic, respectively. 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G. S.; Lewis, P.; Lindemann, D.; Lindquist, B.; Luitz, S.; Luth, V.; Lynch, H. L.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Nelson, S.; Perl, M.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Salnikov, A. A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wagner, A. P.; Wang, W. F.; Wisniewski, W. J.; Wittgen, M.; Wright, D. H.; Wulsin, H. W.; Ziegler, V.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Park, W.; Purohit, M. V.; White, R. M.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Miyashita, T. S.; Puccio, E. M. T.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.; Gorodeisky, R.] SUNY Albany, Albany, NY 12222 USA. [Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Ruland, A. M.; Schwitters, R. F.; Wray, B. C.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; De Mori, F.; Filippi, A.; Gamba, D.; Zambito, S.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; De Mori, F.; Gamba, D.; Zambito, S.] Univ Turin, Dipartimento Fis, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartmento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.; Villanueva-Perez, P.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Ahmed, H.; Albert, J.; Banerjee, Sw.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Anulli, F.] Univ Sassari, I-07100 Sassari, Italy. RP Lees, JP (reprint author), Univ Savoie, CNRS, IN2P3, Lab Annecy Le Vieux Phys Particules LAPP, F-74941 Annecy Le Vieux, France. RI Forti, Francesco/H-3035-2011; Oyanguren, Arantza/K-6454-2014; Luppi, Eleonora/A-4902-2015; White, Ryan/E-2979-2015; Kravchenko, Evgeniy/F-5457-2015; Calabrese, Roberto/G-4405-2015; Martinez Vidal, F*/L-7563-2014; Kolomensky, Yury/I-3510-2015; Lo Vetere, Maurizio/J-5049-2012; Lusiani, Alberto/N-2976-2015; Patrignani, Claudia/C-5223-2009; Monge, Maria Roberta/G-9127-2012; Rizzo, Giuliana/A-8516-2015; Morandin, Mauro/A-3308-2016; Lusiani, Alberto/A-3329-2016; Di Lodovico, Francesca/L-9109-2016; Calcaterra, Alessandro/P-5260-2015; Frey, Raymond/E-2830-2016; OI Forti, Francesco/0000-0001-6535-7965; Oyanguren, Arantza/0000-0002-8240-7300; Luppi, Eleonora/0000-0002-1072-5633; White, Ryan/0000-0003-3589-5900; Calabrese, Roberto/0000-0002-1354-5400; Martinez Vidal, F*/0000-0001-6841-6035; Kolomensky, Yury/0000-0001-8496-9975; Lo Vetere, Maurizio/0000-0002-6520-4480; Lusiani, Alberto/0000-0002-6876-3288; Patrignani, Claudia/0000-0002-5882-1747; Monge, Maria Roberta/0000-0003-1633-3195; Cibinetto, Gianluigi/0000-0002-3491-6231; Pacetti, Simone/0000-0002-6385-3508; Rizzo, Giuliana/0000-0003-1788-2866; Faccini, Riccardo/0000-0003-2613-5141; Bellis, Matthew/0000-0002-6353-6043; Morandin, Mauro/0000-0003-4708-4240; Lusiani, Alberto/0000-0002-6876-3288; Di Lodovico, Francesca/0000-0003-3952-2175; Calcaterra, Alessandro/0000-0003-2670-4826; Frey, Raymond/0000-0003-0341-2636; Martinelli, Maurizio/0000-0003-4792-9178; Lanceri, Livio/0000-0001-8220-3095; Sciacca, Crisostomo/0000-0002-8412-4072; Ebert, Marcus/0000-0002-3014-1512; Paoloni, Eugenio/0000-0001-5969-8712; Bettarini, Stefano/0000-0001-7742-2998 FU U.S. Department of Energy and National Science Foundation,; Natural Sciences and Engineering Research Council (Canada); Commissariat a l'Energie Atomique and Institut National de Physique Nucle aire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany); Istituto Nazionale di Fisica Nucleare (Italy); Foundation for Fundamental Research on Matter (The Netherlands); Research Council of Norway; Ministry of Education and Science of the Russian Federation; Ministerio de Ciencia e Innovacion (Spain); Science and Technology Facilities Council (United Kingdom); Marie-Curie IEF program (European Union); WISE (Women in Science and Engineering) fellowship; A. P. Sloan Foundation (USA) FX We are grateful for the extraordinary contributions of our PEP- II colleagues in achieving the excellent luminosity and machine conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and the kind hospitality extended to them. This work is supported by the U.S. Department of Energy and National Science Foundation, the Natural Sciences and Engineering Research Council (Canada), the Commissariat a l'Energie Atomique and Institut National de Physique Nucle aire et de Physique des Particules (France), the Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany), the Istituto Nazionale di Fisica Nucleare (Italy), the Foundation for Fundamental Research on Matter (The Netherlands), the Research Council of Norway, the Ministry of Education and Science of the Russian Federation, Ministerio de Ciencia e Innovacion (Spain), and the Science and Technology Facilities Council (United Kingdom). Individuals have received support from the Marie-Curie IEF program (European Union) and the A. P. Sloan Foundation (USA). The University of Cincinnati is gratefully acknowledged for its support of this research through a WISE (Women in Science and Engineering) fellowship to C. Pappenheimer. NR 16 TC 6 Z9 6 U1 1 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 30 PY 2013 VL 88 IS 7 AR 071104 DI 10.1103/PhysRevD.88.071104 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 242WQ UT WOS:000326276100001 ER PT J AU Aaltonen, T Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Apollinari, G Appel, JA Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Auerbach, B Aurisano, A Azfar, F Badgett, W Bae, T Barbaro-Galtieri, A Barnes, VE Barnett, BA Barria, P Bartos, P Bauce, M Bedeschi, F Behari, S Bellettini, G Bellinger, J Benjamin, D Beretvas, A Bhatti, A Bland, KR Blumenfeld, B Bocci, A Bodek, A Bortoletto, D Boudreau, J Boveia, A Brigliadori, L Bromberg, C Brucken, E Budagov, J Budd, HS Burkett, K Busetto, G Bussey, P Butti, P Buzatu, A Calamba, A Camarda, S Campanelli, M Canelli, F Carls, B Carlsmith, D Carosi, R Carrillo, S Casal, B Casarsa, M Castro, A Catastini, P Cauz, D Cavaliere, V Cavalli-Sforza, M Cerri, A Cerrito, L Chen, YC Chertok, M Chiarelli, G Chlachidze, G Cho, K Chokheli, D Clark, A Clarke, C Convery, ME Conway, J Corbo, M Cordelli, M Cox, CA Cox, DJ Cremonesi, M Cruz, D Cuevas, J Culbertson, R d'Ascenzo, N Datta, M De Barbaro, P Demortier, L Deninno, M D'Errico, M Devoto, F Di Canto, A Di Ruzza, B Dittmann, JR Donati, S D'Onofrio, M Dorigo, M Driutti, A Ebina, K Edgar, R Elagin, A Erbacher, R Errede, S Esham, B Farrington, S Ramos, JPF Field, R Flanagan, G Forrest, R Franklin, M Freeman, JC Frisch, H Funakoshi, Y Galloni, C Garfinkel, AF Garosi, P Gerberich, H Gerchtein, E Giagua, S Giakoumopoulou, V Gibson, K Ginsburg, CM Giokaris, N Giromini, P Giurgiu, G Glagolev, V Glenzinski, D Gold, M Goldin, D Golossanov, A Gomez, G Gomez-Ceballos, G Goncharov, M Lopez, OG Gorelov, I Goshaw, AT Goulianos, K Gramellinia, E Grinstein, S Grosso-Pilcher, C Group, RC da Costa, JG Hahn, SR Han, JY Happacher, F Hara, K Hare, M Harr, RF Harrington-Taber, T Hatakeyama, K Hays, C Heinrich, J Herndon, M Hocker, A Hong, Z Hopkins, W Hou, S Hughes, RE Husemann, U Hussein, M Huston, J Introzzi, G Iori, M Ivanov, A James, E Jang, D Jayatilaka, B Jeon, EJ Jindariani, S Jones, M Joo, KK Jun, SY Junk, TR Kambeitz, M Kamon, T Karchin, PE Kasmi, A Kato, Y Ketchum, W Keung, J Kilminster, B Kim, DH Kim, HS Kim, JE Kim, MJ Kim, SH Kim, SB Kim, YJ Kim, YK Kimura, N Kirby, M Knoepfel, K Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kreps, M Kroll, J Kruse, M Kuhr, T Kurata, M Laasanen, AT Lammel, S Lancaster, M Lannon, K Latino, G Lee, HS Lee, JS Leo, S Leone, S Lewis, JD Limosani, A Lipeles, E Lister, A Liu, H Liu, Q Liu, T Lockwitz, S Loginov, A Lucchesi, D Luca, A Lueck, J Lujan, P Lukens, P Lungu, G Lys, J Lysak, R Madrak, R Maestro, P Malik, S Manca, G Manousakis-Katsikakis, A Marchese, L Margaroli, F Marino, P Martinez, M Matera, K Mattson, ME Mazzacane, A Mazzanti, P McNulty, R Mehta, A Mehtala, P Mesropian, C Miao, T Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Moon, CS Moore, R Morello, MJ Mukherjee, A Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nakano, I Napier, A Nett, J Neu, C Nigmanov, T Nodulman, L Noh, SY Norniella, O Oakes, L Oh, SH Oh, YD Oksuzian, I Okusawa, T Orava, R Ortolan, L Pagliaronea, C Palencia, E Palni, P Papadimitriou, V Parker, W Pauletta, G Paulini, M Paus, C Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pondrom, L Poprocki, S Potamianos, K Pranko, A Prokoshin, F Ptohos, F Punzi, G Ranjan, N Fernandez, IR Renton, P Rescigno, M Rimondi, F Ristori, L Robson, A Rodriguez, T Rolli, S Ronzani, M Roser, R Rosner, JL Ruffini, F Ruiz, A Russ, J Rusu, V Sakumoto, WK Sakurai, Y Santi, L Sato, K Saveliev, V Savoy-Navarro, A Schlabach, P Schmidt, EE Schwarz, T Scodellaro, L Scuri, F Seidel, S Seiya, Y Semenov, A Sforza, F Shalhout, SZ Shears, T Shepard, PF Shimojima, M Shochet, M Shreyber-Tecker, I Simonenko, A Sliwa, K Smith, JR Snider, FD Song, H Sorin, V Denis, RS Stancari, M Stentz, D Strologas, J Sudo, Y Sukhanov, A Suslov, I Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thomson, E Thukral, V Toback, D Tokar, S Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Ukegawa, F Uozumi, S Vazquez, F Velev, G Vellidis, C Vernieri, C Vidal, M Vilar, R Vizan, J Vogel, M Volpi, G Wagner, P Wallny, R Wang, SM Waters, D Wester, WC Whiteson, D Wicklund, AB Wilbur, S Williams, HH Wilson, JS Wilson, P Winer, BL Wittich, P Wolbers, S Wolfe, H Wright, T Wu, X Wu, Z Yamamoto, K Yamato, D Yang, T Yang, UK Yang, YC Yao, WM Yeh, GP Yi, K Yoh, J Yorita, K Yoshida, T Yu, GB Yu, I Zanetti, AM Zeng, Y Zhou, C Zucchelli, S AF Aaltonen, T. Amerio, S. Amidei, D. Anastassov, A. Annovi, A. Antos, J. Apollinari, G. Appel, J. A. Arisawa, T. Artikov, A. Asaadi, J. Ashmanskas, W. Auerbach, B. Aurisano, A. Azfar, F. Badgett, W. Bae, T. Barbaro-Galtieri, A. Barnes, V. E. Barnett, B. A. Barria, P. Bartos, P. Bauce, M. Bedeschi, F. Behari, S. Bellettini, G. Bellinger, J. Benjamin, D. Beretvas, A. Bhatti, A. Bland, K. R. Blumenfeld, B. Bocci, A. Bodek, A. Bortoletto, D. Boudreau, J. Boveia, A. Brigliadori, L. Bromberg, C. Brucken, E. Budagov, J. Budd, H. S. Burkett, K. Busetto, G. Bussey, P. Butti, P. Buzatu, A. Calamba, A. Camarda, S. Campanelli, M. Canelli, F. Carls, B. Carlsmith, D. Carosi, R. Carrillo, S. Casal, B. Casarsa, M. Castro, A. Catastini, P. Cauz, D. Cavaliere, V. Cavalli-Sforza, M. Cerri, A. Cerrito, L. Chen, Y. C. Chertok, M. Chiarelli, G. Chlachidze, G. Cho, K. Chokheli, D. Clark, A. Clarke, C. Convery, M. E. Conway, J. Corbo, M. Cordelli, M. Cox, C. A. Cox, D. J. Cremonesi, M. Cruz, D. Cuevas, J. 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CA CDF Collaboration TI Measurement of the Differential Cross Section d sigma/d(cos theta(t)) for Top-Quark Pair Production in p(p)over-bar Collisions at root s = 1.96 TeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID CHARGE ASYMMETRY; GENERAL-THEORY; DETECTOR; PHYSICS AB We report a measurement of the differential cross section d sigma = d(cos theta(t)) for top-quark pair production as a function of the top-quark production angle in proton-antiproton collisions at root s = 1.96 TeV. This measurement is performed using data collected with the CDF II detector at the Tevatron, corresponding to an integrated luminosity of 9.4 fb(-1). We employ the Legendre polynomials to characterize the shape of the differential cross section at the parton level. The observed Legendre coefficients are in good agreement with the prediction of the next-to-leading-order standard- model calculation, with the exception of an excess linear-term coefficient a(1) = 0.40 +/- 0.12, compared to the standard-model prediction of a(1) = 0.15(-0.03)(+0.07) C1 [Chen, Y. C.; Hou, S.; Mitra, A.; Teng, P. K.; Wang, S. M.] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Auerbach, B.; Nodulman, L.; Wicklund, A. B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Giakoumopoulou, V.; Giokaris, N.; Manousakis-Katsikakis, A.] Univ Athens, GR-15771 Athens, Greece. [Camarda, S.; Cavalli-Sforza, M.; Grinstein, S.; Martinez, M.; Ortolan, L.; Sorin, V.] Univ Autonoma Barcelona, Inst Fis Altes Energies, ICREA, E-08193 Bellaterra, Barcelona, Spain. [Bland, K. R.; Dittmann, J. R.; Hatakeyama, K.; Kasmi, A.; Wu, Z.] Baylor Univ, Waco, TX 76798 USA. [Gramellinia, E.; Marchese, L.; Mazzanti, P.; Moggi, N.; Mussini, M.; Rimondi, F.; Zucchelli, S.] Ist Nazl Fis Nucl, I-40127 Bologna, Italy. [Mussini, M.; Zucchelli, S.] Univ Bologna, I-40127 Bologna, Italy. [Chertok, M.; Conway, J.; Cox, C. A.; Cox, D. J.; Erbacher, R.; Forrest, R.; Ivanov, A.; Pilot, J.; Shalhout, S. Z.; Smith, J. R.; Wilbur, S.] Univ Calif Davis, Davis, CA 95616 USA. [Plager, C.] Univ Calif Los Angeles, Los Angeles, CA 90024 USA. [Casal, B.; Cuevas, J.; Gomez, G.; Palencia, E.; Ruiz, A.; Scodellaro, L.; Vilar, R.; Vizan, J.] CSIC Univ Cantabria, Inst Fis Cantabria, Santander 39005, Spain. [Calamba, A.; Jang, D.; Jun, S. Y.; Paulini, M.; Russ, J.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Boveia, A.; Canelli, F.; Frisch, H.; Grosso-Pilcher, C.; Ketchum, W.; Kim, Y. K.; Rosner, J. L.; Shochet, M.; Tang, J.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Antos, J.; Bartos, P.; Lysak, R.; Tokar, S.] Comenius Univ, Bratislava 84248, Slovakia. 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C.; Yu, I.] Kyungpook Natl Univ, Ctr High Energy Phys, Taegu 702701, South Korea. [Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. J.; Lee, H. S.; Lee, J. S.; Noh, S. Y.; Oh, Y. D.; Uozumi, S.; Yang, U. K.; Yang, Y. C.; Yu, I.] Seoul Natl Univ, Seoul 151742, South Korea. [Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. J.; Lee, H. S.; Lee, J. S.; Noh, S. Y.; Oh, Y. D.; Uozumi, S.; Yang, U. K.; Yang, Y. C.; Yu, I.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. J.; Lee, H. S.; Lee, J. S.; Noh, S. Y.; Oh, Y. D.; Uozumi, S.; Yang, U. K.; Yang, Y. C.; Yu, I.] Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. [Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. 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[Campanelli, M.; Cerrito, L.; Lancaster, M.; Waters, D.] UCL, London WC1E 6BT, England. [Ramos, J. P. Fernandez; Lopez, O. Gonzalez; Fernandez, I. Redondo] CIEMAT, E-28040 Madrid, Spain. [Gomez-Ceballos, G.; Goncharov, M.; Paus, C.] MIT, Cambridge, MA 02139 USA. [Amidei, D.; Edgar, R.; Mietlicki, D.; Schwarz, T.; Tecchio, M.; Wilson, J. S.; Wright, T.] Univ Michigan, Ann Arbor, MI 48109 USA. [Bromberg, C.; Hussein, M.; Huston, J.; Tollefson, K.] Michigan State Univ, E Lansing, MI 48824 USA. [Shreyber-Tecker, I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Gold, M.; Gorelov, I.; Palni, P.; Seidel, S.; Strologas, J.; Vogel, M.] Univ New Mexico, Albuquerque, NM 87131 USA. [Hughes, R. E.; Lannon, K.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Okayama 7008530, Japan. [Kato, Y.; Okusawa, T.; Seiya, Y.; Yamamoto, K.; Yamato, D.; Yoshida, T.] Osaka City Univ, Osaka 5588585, Japan. 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[Bellettini, G.; Butti, P.; Di Canto, A.; Donati, S.; Galloni, C.; Punzi, G.; Ronzani, M.; Sforza, F.] Univ Pisa, I-56127 Pisa, Italy. [Barria, P.; Garosi, P.; Latino, G.; Maestro, P.; Ruffini, F.] Univ Siena, I-27100 Pavia, Italy. [Marino, P.; Morello, M. J.; Trovato, M.; Vernieri, C.] Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Introzzi, G.] Ist Nazl Fis Nucl, I-27100 Pavia, Italy. [Introzzi, G.] Univ Pavia, I-27100 Pavia, Italy. [Boudreau, J.; Gibson, K.; Nigmanov, T.; Shepard, P. F.; Song, H.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Barnes, V. E.; Bortoletto, D.; Garfinkel, A. F.; Jones, M.; Laasanen, A. T.; Liu, Q.; Ranjan, N.; Vidal, M.] Purdue Univ, W Lafayette, IN 47907 USA. [Bodek, A.; Budd, H. S.; De Barbaro, P.; Han, J. Y.; Sakumoto, W. K.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10065 USA. [Giagua, S.; Iori, M.; Margaroli, F.; Rescigno, M.] Ist Nazl Fis Nucl, Sez Roma 1, I-00185 Rome, Italy. [Iori, M.] Univ Roma La Sapienza, I-00185 Rome, Italy. [Asaadi, J.; Aurisano, A.; Cruz, D.; Elagin, A.; Goldin, D.; Hong, Z.; Kamon, T.; Nett, J.; Thukral, V.; Toback, D.] Texas A&M Univ, Mitchell Inst Fundamental Phys & Astron, College Stn, TX 77843 USA. [Casarsa, M.; Cauz, D.; Dorigo, M.; Driutti, A.; Pagliaronea, C.; Pauletta, G.; Santi, L.; Zanetti, A. M.] Ist Nazl Fis Nucl, I-34127 Trieste, Italy. [Cauz, D.; Dorigo, M.; Driutti, A.; Pauletta, G.; Santi, L.] Grp Collegato Udine, I-33100 Udine, Italy. [Cauz, D.; Driutti, A.; Pauletta, G.; Santi, L.] Univ Udine, I-33100 Udine, Italy. Univ Trieste, I-34127 Trieste, Italy. [Hara, K.; Kim, S. H.; Kurata, M.; Miyake, H.; Nagai, Y.; Sato, K.; Shimojima, M.; Sudo, Y.; Takemasa, K.; Takeuchi, Y.; Tomura, T.; Ukegawa, F.] Univ Tsukuba, Tsukuba, Ibaraki 305, Japan. [Hare, M.; Napier, A.; Rolli, S.; Sliwa, K.] Tufts Univ, Medford, MA 02155 USA. [Group, R. C.; Liu, H.; Neu, C.; Oksuzian, I.] Univ Virginia, Charlottesville, VA 22906 USA. [Arisawa, T.; Ebina, K.; Funakoshi, Y.; Kimura, N.; Kondo, K.; Naganoma, J.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo 169, Japan. [Clarke, C.; Harr, R. F.; Karchin, P. E.; Mattson, M. E.] Wayne State Univ, Detroit, MI 48201 USA. [Bellinger, J.; Carlsmith, D.; Herndon, M.; Parker, W.; Pondrom, L.] Univ Wisconsin, Madison, WI 53706 USA. [Husemann, U.; Lockwitz, S.; Loginov, A.] Yale Univ, New Haven, CT 06520 USA. RP Aaltonen, T (reprint author), Univ Helsinki, Div High Energy Phys, Dept Phys, FIN-00014 Helsinki, Finland. RI Introzzi, Gianluca/K-2497-2015; Piacentino, Giovanni/K-3269-2015; Marino, Pietro/N-7030-2015; song, hao/I-2782-2012; Gorelov, Igor/J-9010-2015; Prokoshin, Fedor/E-2795-2012; Chiarelli, Giorgio/E-8953-2012; Kim, Soo-Bong/B-7061-2014; Robson, Aidan/G-1087-2011; maestro, paolo/E-3280-2010; Lysak, Roman/H-2995-2014; Moon, Chang-Seong/J-3619-2014; Scodellaro, Luca/K-9091-2014; Punzi, Giovanni/J-4947-2012; Grinstein, Sebastian/N-3988-2014; Paulini, Manfred/N-7794-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Cavalli-Sforza, Matteo/H-7102-2015 OI Introzzi, Gianluca/0000-0002-1314-2580; Piacentino, Giovanni/0000-0001-9884-2924; Marino, Pietro/0000-0003-0554-3066; song, hao/0000-0002-3134-782X; Gorelov, Igor/0000-0001-5570-0133; Prokoshin, Fedor/0000-0001-6389-5399; Chiarelli, Giorgio/0000-0001-9851-4816; maestro, paolo/0000-0002-4193-1288; Moon, Chang-Seong/0000-0001-8229-7829; Scodellaro, Luca/0000-0002-4974-8330; Punzi, Giovanni/0000-0002-8346-9052; Grinstein, Sebastian/0000-0002-6460-8694; Paulini, Manfred/0000-0002-6714-5787; Russ, James/0000-0001-9856-9155; FU U.S. Department of Energy and National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science, and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A. P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; Korean World Class University Program; National Research Foundation of Korea; Science and Technology Facilities Council; Royal Society, U. K.; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion and Programa Consolider-Ingenio, Spain; Slovak RD Agency; Academy of Finland; Australian Research Council (ARC); EU Community Marie Curie Fellowship [302103] FX We thank T. Tait, S. Jung, W. Bernreuther, and Z.-G. Si for their assistance in preparing the theoretical models and calculations used in this Letter, and T. Rizzo for helpful conversations. We also thank the development teams of SCIPY, PYTABLES, MATPLOTLIB, and IPYTHON for their useful tools [31]. We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the Ministry of Education, Culture, Sports, Science, and Technology of Japan; the Natural Sciences and Engineering Research Council of Canada; the National Science Council of the Republic of China; the Swiss National Science Foundation; the A. P. Sloan Foundation; the Bundesministerium fur Bildung und Forschung, Germany; the Korean World Class University Program and the National Research Foundation of Korea; the Science and Technology Facilities Council and the Royal Society, U. K.; the Russian Foundation for Basic Research; the Ministerio de Ciencia e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Slovak R&D Agency; the Academy of Finland; the Australian Research Council (ARC); and the EU Community Marie Curie Fellowship Contract No. 302103. NR 32 TC 18 Z9 18 U1 2 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 30 PY 2013 VL 111 IS 18 AR 182002 DI 10.1103/PhysRevLett.111.182002 PG 8 WC Physics, Multidisciplinary SC Physics GA 242XP UT WOS:000326279400004 PM 24237509 ER PT J AU Gopalakrishnan, S Martin, I Demler, EA AF Gopalakrishnan, Sarang Martin, Ivar Demler, Eugene A. TI Quantum Quasicrystals of Spin-Orbit-Coupled Dipolar Bosons SO PHYSICAL REVIEW LETTERS LA English DT Article ID ORDER; SUPERCONDUCTORS; SYMMETRY; PHASE; FIELD AB We study quasi-two-dimensional dipolar Bose gases in which the bosons experience a Rashba spin-orbit coupling. We show that the degenerate dispersion minimum due to the spin-orbit coupling, combined with the long-range dipolar interaction, can stabilize a number of quantum crystalline and quasicrystalline ground states. Coupling the bosons to a fermionic species can further stabilize these phases. We estimate that the crystalline and quasicrystalline phases should be detectable in realistic dipolar condensates, e.g., dysprosium, and discuss their symmetries and excitations. C1 [Gopalakrishnan, Sarang; Demler, Eugene A.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Martin, Ivar] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Gopalakrishnan, S (reprint author), Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC020-6CH11357]; Harvard-MIT CUA; DARPA OLE program; AFOSR MURI on Ultracold Molecules; ARO-MURI on Atomtronics FX We are grateful to A. Rosch, B. Lev, R. Wilson, and M. Knap for helpful discussions. S. G. was supported in part by the Harvard Quantum Optics Center. Work performed at Argonne National Laboratory (by I. M.) is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC020-6CH11357. E. A. D. acknowledges support from Harvard-MIT CUA, the DARPA OLE program, AFOSR MURI on Ultracold Molecules, and ARO-MURI on Atomtronics. NR 53 TC 24 Z9 24 U1 2 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 30 PY 2013 VL 111 IS 18 AR 185304 DI 10.1103/PhysRevLett.111.185304 PG 5 WC Physics, Multidisciplinary SC Physics GA 242XP UT WOS:000326279400008 ER PT J AU Fan, ZS Jastrow, JD Liang, C Matamala, R Miller, RM AF Fan, Zhaosheng Jastrow, Julie D. Liang, Chao Matamala, Roser Miller, Raymond Michael TI Priming Effects in Boreal Black Spruce Forest Soils: Quantitative Evaluation and Sensitivity Analysis SO PLOS ONE LA English DT Article ID DISSOLVED ORGANIC-CARBON; INTERIOR ALASKA; HYDRAULIC CONDUCTIVITY; MATTER; DECOMPOSITION; TURNOVER; RESPIRATION; MECHANISMS; PEATLANDS; TRANSPORT AB Laboratory studies show that introduction of fresh and easily decomposable organic carbon (OC) into soil-water systems can stimulate the decomposition of soil OC (SOC) via priming effects in temperate forests, shrublands, grasslands, and agro-ecosystems. However, priming effects are still not well understood in the field setting for temperate ecosystems and virtually nothing is known about priming effects (e. g., existence, frequency, and magnitude) in boreal ecosystems. In this study, a coupled dissolved OC (DOC) transport and microbial biomass dynamics model was developed to simultaneously simulate co-occurring hydrological, physical, and biological processes and their interactions in soil pore-water systems. The developed model was then used to examine the importance of priming effects in two black spruce forest soils, with and without underlying permafrost. Our simulations showed that priming effects were strongly controlled by the frequency and intensity of DOC input, with greater priming effects associated with greater DOC inputs. Sensitivity analyses indicated that priming effects were most sensitive to variations in the quality of SOC, followed by variations in microbial biomass dynamics (i.e., microbial death and maintenance respiration), highlighting the urgent need to better discern these key parameters in future experiments and to consider these dynamics in existing ecosystem models. Water movement carries DOC to deep soil layers that have high SOC stocks in boreal soils. Thus, greater priming effects were predicted for the site with favorable water movement than for the site with limited water flow, suggesting that priming effects might be accelerated for sites where permafrost degradation leads to the formation of dry thermokarst. C1 [Fan, Zhaosheng; Jastrow, Julie D.; Liang, Chao; Matamala, Roser; Miller, Raymond Michael] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. RP Fan, ZS (reprint author), Argonne Natl Lab, Biosci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM zfan@anl.gov FU U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Climate and Environmental Science Division [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Climate and Environmental Science Division under contract DE-AC02-06CH11357. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 64 TC 2 Z9 2 U1 4 U2 56 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 30 PY 2013 VL 8 IS 10 AR e77880 DI 10.1371/journal.pone.0077880 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 243RL UT WOS:000326334500072 PM 24205010 ER PT J AU Bristowe, NC Stengel, M Littlewood, PB Artacho, E Pruneda, JM AF Bristowe, N. C. Stengel, Massimiliano Littlewood, P. B. Artacho, Emilio Pruneda, J. M. TI One-dimensional half-metallic interfaces of two-dimensional honeycomb insulators SO PHYSICAL REVIEW B LA English DT Article ID LOCALIZED WANNIER FUNCTIONS; BORON-NITRIDE; GRAPHENE; ELECTRONICS AB We study zigzag interfaces between insulating compounds that are isostructural to graphene, specifically II-VI, III-V, and IV-IV two-dimensional honeycomb insulators. We show that these one-dimensional interfaces are polar, with a net density of excess charge that can be simply determined by using the ideal (integer) formal valence charges, regardless of the predominant covalent character of the bonding in these materials. We justify this finding on fundamental physical grounds by analyzing the topology of the formal polarization lattice in the parent bulk materials. First-principles calculations elucidate an electronic compensation mechanism not dissimilar to oxide interfaces, which is triggered by a Zener-like charge transfer between interfaces of opposite polarity. In particular, we predict the emergence of one-dimensional electron and hole gases, which in some cases are ferromagnetic half metallic. C1 [Bristowe, N. C.; Littlewood, P. B.; Artacho, Emilio] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bristowe, N. C.] Univ Liege, B-4000 Sart Tilman Par Liege, Belgium. [Stengel, Massimiliano] Inst Catalana Recerca & Estudis Avancats, Barcelona 08010, Spain. [Stengel, Massimiliano] CSIC, Inst Ciencia Mat Barcelona, Bellaterra 08193, Spain. [Littlewood, P. B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Artacho, Emilio] CIC Nanogune & DIPC, San Sebastian 20018, Spain. [Artacho, Emilio] Basque Fdn Sci Ikerbasque, Bilbao 48011, Spain. [Pruneda, J. M.] ICN2 Inst Catala Nanociencia & Nanotecnol, Bellaterra, Barcelona, Spain. [Pruneda, J. M.] CSIC, Bellaterra 08193, Barcelona, Spain. RP Bristowe, NC (reprint author), Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. RI Pruneda, Miguel/A-4077-2008; Stengel, Massimiliano/E-2934-2010; Bristowe, Nicholas/B-2230-2013; Artacho, Emilio/G-2616-2015; DONOSTIA INTERNATIONAL PHYSICS CTR., DIPC/C-3171-2014; nanoGUNE, CIC/A-2623-2015 OI Pruneda, Miguel/0000-0002-3621-6095; Stengel, Massimiliano/0000-0003-4175-3888; Bristowe, Nicholas/0000-0003-1286-8440; Artacho, Emilio/0000-0001-9357-1547; FU EPSRC; MCINN [FIS2009-12721-C0-401, CSD2007-00041]; Spanish Supercomputer Network; HPC Europa; DOE [FWP 70069] FX We acknowledge I. Souza for valuable discussions, the support of EPSRC, MCINN (Grants No. FIS2009-12721-C0-401 and No. CSD2007-00041), and computing resources of CamGRID and Darwin at Cambridge, the Spanish Supercomputer Network, and HPC Europa. P.B.L. acknowledges DOE support under Grant No. FWP 70069. NR 40 TC 9 Z9 9 U1 2 U2 44 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 30 PY 2013 VL 88 IS 16 AR UNSP 161411 DI 10.1103/PhysRevB.88.161411 PG 5 WC Physics, Condensed Matter SC Physics GA 242VW UT WOS:000326273500001 ER PT J AU Liu, XH Wang, Y Burton, JD Tsymbal, EY AF Liu, Xiaohui Wang, Yong Burton, J. D. Tsymbal, Evgeny Y. TI Polarization-controlled Ohmic to Schottky transition at a metal/ferroelectric interface SO PHYSICAL REVIEW B LA English DT Article ID MULTIFERROIC TUNNEL-JUNCTIONS; FERROELECTRIC CONTROL; SPIN POLARIZATION; OXIDE INTERFACES; BIFEO3; HETEROSTRUCTURES; FILMS; PHYSICS; DIODE AB Ferroelectric polar displacements have recently been observed in conducting electron-doped BaTiO3 (n-BTO). The coexistence of a ferroelectric phase and conductivity opens the door to new functionalities that may provide a unique route for novel device applications. Using first-principles methods and electrostatic modeling, we explore the effect that the switchable polarization of n-BTO has on the electronic properties of the SrRuO3/n-BTO (001) interface. Ferroelectric polarization controls the accumulation or depletion of electron charge at the interface, and the associated bending of the n-BTO conduction band determines the transport regime across the interface. The interface exhibits a Schottky tunnel barrier for one polarization orientation, whereas an Ohmic contact is present for the opposite polarization orientation, leading to a large change in interface resistance associated with polarization reversal. Our calculations reveal a five orders of magnitude change in the interface resistance because of polarization switching. C1 [Liu, Xiaohui; Burton, J. D.; Tsymbal, Evgeny Y.] Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. [Liu, Xiaohui; Burton, J. D.; Tsymbal, Evgeny Y.] Univ Nebraska, Nebraska Ctr Mat & Nanosci, Lincoln, NE 68588 USA. [Wang, Yong] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Liu, XH (reprint author), Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. EM jdburton1@gmail.com; tsymbal@unl.edu RI Tsymbal, Evgeny/G-3493-2013; Burton, John/B-5875-2008 OI Burton, John/0000-0001-5535-2407 FU Nanoelectronics Research Initiative (NRI) through the Center for NanoFerroic Devices (CNFD); US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (DOE) [DE-SC0004876] FX This research was supported by the Nanoelectronics Research Initiative (NRI) through the Center for NanoFerroic Devices (CNFD) and US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (DOE Grant No. DE-SC0004876). Computations were performed at the University of Nebraska Holland Computing Center. NR 43 TC 25 Z9 25 U1 8 U2 112 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 30 PY 2013 VL 88 IS 16 AR 165139 DI 10.1103/PhysRevB.88.165139 PG 6 WC Physics, Condensed Matter SC Physics GA 242VW UT WOS:000326273500004 ER PT J AU Shin, CS Avalos, CE Butler, MC Wang, HJ Seltzer, SJ Liu, RB Pines, A Bajaj, VS AF Shin, Chang S. Avalos, Claudia E. Butler, Mark C. Wang, Hai-Jing Seltzer, Scott J. Liu, Ren-Bao Pines, Alexander Bajaj, Vikram S. TI Suppression of electron spin decoherence of the diamond NV center by a transverse magnetic field SO PHYSICAL REVIEW B LA English DT Article ID NITROGEN-VACANCY SPIN; COHERENT DYNAMICS; BATH; RESONANCE; MAGNETOMETRY; QUBITS; TIME AB We demonstrate that the spin decoherence of nitrogen vacancy (NV) centers in diamond can be suppressed by a transverse magnetic field if the electron spin bath is the primary decoherence source. The NV spin coherence, created in "a decoherence-free subspace," is protected by the transverse component of the zero-field splitting, increasing the spin-coherence time about twofold. The decoherence due to the electron spin bath is also suppressed at magnetic fields stronger than similar to 25 G when applied parallel to the NV symmetry axis. Our method can be used to extend the spin-coherence time of similar spin systems for applications in quantum computing, field sensing, and other metrologies. C1 [Shin, Chang S.; Avalos, Claudia E.; Butler, Mark C.; Wang, Hai-Jing; Seltzer, Scott J.; Pines, Alexander; Bajaj, Vikram S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Shin, Chang S.; Avalos, Claudia E.; Butler, Mark C.; Wang, Hai-Jing; Seltzer, Scott J.; Pines, Alexander; Bajaj, Vikram S.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Shin, Chang S.; Avalos, Claudia E.; Butler, Mark C.; Wang, Hai-Jing; Seltzer, Scott J.; Pines, Alexander; Bajaj, Vikram S.] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Liu, Ren-Bao] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Liu, Ren-Bao] Chinese Univ Hong Kong, Ctr Quantum Coherence, Shatin, Hong Kong, Peoples R China. RP Shin, CS (reprint author), Halliburton Energy Serv Inc, 3000 N Sam Houston Pkwy E, Houston, TX 77032 USA. EM vikbajaj@gmail.com RI Liu, Ren-Bao/B-3729-2011; OI Liu, Ren-Bao/0000-0002-0620-2370; Butler, Mark/0000-0002-1273-5771 FU Office of Science Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [CHE-0957655]; Hong Kong RGC-NSFC [N_CUHK403/11] FX The authors thank Ran Fischer and Dmitry Budker for useful discussions. This work was supported by the Director, Office of Science Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. M.B. acknowledges financial support from the National Science Foundation under Award No. CHE-0957655. R.L. acknowledges financial support from Hong Kong RGC-NSFC Project N_CUHK403/11. NR 39 TC 6 Z9 6 U1 0 U2 29 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 30 PY 2013 VL 88 IS 16 AR 161412 DI 10.1103/PhysRevB.88.161412 PG 5 WC Physics, Condensed Matter SC Physics GA 242VW UT WOS:000326273500002 ER PT J AU Hu, XF Wu, J Niu, DX Chen, L Morton, SA Scholl, A Huang, ZC Zhai, Y Zhang, W Will, I Xu, YB Zhang, R van der Laan, G AF Hu, X. F. Wu, J. Niu, D. X. Chen, L. Morton, S. A. Scholl, A. Huang, Z. C. Zhai, Y. Zhang, W. Will, I. Xu, Y. B. Zhang, R. van der Laan, G. TI Discontinuous properties of current-induced magnetic domain wall depinning SO SCIENTIFIC REPORTS LA English DT Article DE APPLIED PHYSICS; MAGNETIC DEVICES; SPINTRONICS; FERROMAGNETISM ID MOTION; NANOWIRES; DYNAMICS; STRIPS AB The current-induced motion of magnetic domain walls (DWs) confined to nanostructures is of great interest for fundamental studies as well as for technological applications in spintronic devices. Here, we present magnetic images showing the depinning properties of pulse-current-driven domain walls in well-shaped Permalloy nanowires obtained using photoemission electron microscopy combined with x-ray magnetic circular dichroism. In the vicinity of the threshold current density (Jth = 4.2 x 10(11) A.m(-2)) for the DW motion, discontinuous DW depinning and motion have been observed as a sequence of "Barkhausen jumps". A one-dimensional analytical model with a piecewise parabolic pinning potential has been introduced to reproduce the DW hopping between two nearest neighbour sites, which reveals the dynamical nature of the current-driven DW motion in the depinning regime. C1 [Hu, X. F.; Niu, D. X.; Zhang, W.; Will, I.; Xu, Y. B.] Univ York, Dept Elect, Spintron & Nanodevice Lab, York YO10 5DD, N Yorkshire, England. [Hu, X. F.; Wu, J.; Niu, D. X.; Xu, Y. B.; Zhang, R.] Nanjing Univ, Sch Elect Sci & Engn, Nanjing York Int Ctr Spintron, Nanjing 210093, Jiangsu, Peoples R China. [Wu, J.] Univ York, Dept Phys, York YO10 5DD, N Yorkshire, England. [Chen, L.] Univ Leeds, Dept Elect, Leeds LS2 9JT, W Yorkshire, England. [Morton, S. A.; Scholl, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Huang, Z. C.; Zhai, Y.] Southeast Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China. [van der Laan, G.] Magnet Spect Grp, Diamond Light Source, Didcot OX11 0DE, Oxon, England. RP Xu, YB (reprint author), Univ York, Dept Elect, Spintron & Nanodevice Lab, York YO10 5DD, N Yorkshire, England. EM yongbing.xu@york.ac.uk RI Scholl, Andreas/K-4876-2012; van der Laan, Gerrit/Q-1662-2015; Zhai, Ya/J-6991-2012; OI van der Laan, Gerrit/0000-0001-6852-2495; Zhai, Ya/0000-0002-9006-9575; Huang, Zhaocong/0000-0002-0190-2810 FU State Key Programme for Basic Research of China [2014CB921101]; NSFC [61274102]; PAPD project; UK EPSRC; STFC; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX This work is supported by the State Key Programme for Basic Research of China (Grants No. 2014CB921101), NSFC (Grants No. 61274102) and PAPD project, UK EPSRC and STFC. The Advanced Light Source at Lawrence Berkeley National Laboratory is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. XH would like to thank the York NanoCenter for samples fabrication support. NR 51 TC 3 Z9 3 U1 4 U2 53 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 30 PY 2013 VL 3 AR 3080 DI 10.1038/srep03080 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 243QR UT WOS:000326332500001 PM 24170087 ER PT J AU Nicholson, DM Ojha, M Egami, T AF Nicholson, D. M. Ojha, Madhusudan Egami, T. TI First-principles local stress in crystalline and amorphous metals SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID DENSITY; ENERGY AB Atomic size is perhaps the most commonly used concept to describe material properties. Advances in the understanding of materials are hindered by the available choices of simplifying concepts that can be used. However, the precise definition of atomic size is not easy, and often controversial. Atomic level stress provides a new interpretive tool that draws on the rich formalism of solid mechanics for use with density functional calculations to advance a deeper understanding of the properties of materials. We discuss atomic level stresses in liquids and glasses and make comparisons with ordered and disordered crystals. Somewhat surprisingly, even ordered compounds that are under no macroscopic stress and whose individual atoms are completely relaxed, i.e., no force acting on them, can have substantial atomic level stresses. On top of concepts such as the ionicity or covalency, the atomic level stresses add to the arsenal of analysis tools that are available to interpret the results of density functional calculations. C1 [Nicholson, D. M.; Ojha, Madhusudan; Egami, T.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Ojha, Madhusudan; Egami, T.] Univ Tennessee, Knoxville, TN 37996 USA. RP Nicholson, DM (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM nicholsondm@ornl.gov FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX Research at ORNL was supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 24 TC 3 Z9 3 U1 3 U2 29 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD OCT 30 PY 2013 VL 25 IS 43 AR 435505 DI 10.1088/0953-8984/25/43/435505 PG 11 WC Physics, Condensed Matter SC Physics GA 237UR UT WOS:000325896900012 PM 24107600 ER PT J AU Tomic, S Pinteric, M Ivek, T Sedlmeier, K Beyer, R Wu, D Schlueter, JA Schweitzer, D Dressel, M AF Tomic, S. Pinteric, M. Ivek, T. Sedlmeier, K. Beyer, R. Wu, D. Schlueter, J. A. Schweitzer, D. Dressel, M. TI Magnetic ordering and charge dynamics in kappa-(BEDT-TTF)(2)Cu [N(CN)(2)]Cl SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID ORGANIC CONDUCTORS; BEDT-TTF; DENSITY WAVES; BIS(ETHYLENEDITHIO)TETRATHIAFULVALENE; PHASE; RAMAN; VIBRATIONS; ANISOTROPY; MODEL; NMR AB The Mott insulator kappa-(BEDT-TTF)(2)Cu[N(CN)(2)]Cl consists of molecular dimers arranged on an anisotropic triangular lattice. At low temperatures a pronounced dielectric anomaly is observed, and eventually a canted antiferromagnetic ground state forms. Optical spectroscopy clearly rules out charge imbalance and the existence of quantum electric dipoles with a dipolar-spin coupling. Here we suggest a novel form of spin-charge coupling where the prominent in-plane dielectric response in kappa-(BEDT-TTF)(2)Cu[N(CN)(2)]Cl is explained by short-range discommensurations of the antiferromagnetic phase in the temperature range 30 K < T < 50 K, and by relaxation of charged domain walls in the ferromagnetic structure at lower temperatures. C1 [Tomic, S.; Pinteric, M.; Ivek, T.] Inst Fiziku, HR-10001 Zagreb, Croatia. [Pinteric, M.] Univ Maribor, Fac Civil Engn, SLO-2000 Maribor, Slovenia. [Ivek, T.; Sedlmeier, K.; Beyer, R.; Wu, D.; Schweitzer, D.; Dressel, M.] Univ Stuttgart, Inst Phys, D-70550 Stuttgart, Germany. [Schlueter, J. A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Tomic, S (reprint author), Inst Fiziku, POB 304, HR-10001 Zagreb, Croatia. EM stomic@ifs.hr RI Tomic, Silvia/D-5466-2011; Ivek, Tomislav/D-5298-2011; Dressel, Martin/D-3244-2012; Pinteric, Marko/D-5739-2011 FU Deutsche Forschungsgemeinschaft (DFG); Deutscher Akademische Auslandsdienst (DAAD); Croatian Ministry of Science, Education and Sports [035-0000000-2836] FX We thank C Hotta, K Kanoda, S Mazumdar, J-P. Pouget, E Rose, M Tanatar, E Tutis and T Yamamoto for helpful discussions. The project was supported by the Deutsche Forschungsgemeinschaft (DFG), the Deutscher Akademische Auslandsdienst (DAAD) and the Croatian Ministry of Science, Education and Sports under grant 035-0000000-2836. NR 50 TC 9 Z9 9 U1 1 U2 33 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD OCT 30 PY 2013 VL 25 IS 43 AR 436004 DI 10.1088/0953-8984/25/43/436004 PG 7 WC Physics, Condensed Matter SC Physics GA 237UR UT WOS:000325896900023 PM 24107640 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adye, T Aefsky, S Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmad, A Ahsan, M Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alam, MA Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amoroso, S Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arslan, O Artamonov, A Artoni, G Arutinov, D Asai, S Asbah, N Ask, S Asman, B Asquith, L Assamagan, K Astalos, R Astbury, A Atkinson, M Atlay, NB Auerbach, B Auge, E Augsten, K Aurousseau, M Avolio, G Axen, D Azuelos, G Azuma, Y Baak, MA Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartsch, V Basye, A Bates, RL Batkova, L Batley, JR Battistin, M Bauer, F Bawa, HS Beale, S Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becks, KH Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belloni, A Beloborodova, OL Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernard, C Bernat, P Bernhard, R Bernius, C Bernlochner, FU Berry, T Bertella, C Bertolucci, F Besana, MI Besjes, GJ Bessidskaia, O Besson, N Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Bittner, B Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blocki, J Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Boddy, CR Boehler, M Boek, J Boek, TT Boelaert, N Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Bolnet, NM Bomben, M Bona, M Boonekamp, M Bordoni, S Borer, C Borisov, A Borissov, G Borri, M Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Bouchami, J Boudreau, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozovic-Jelisavcic, I Bracinik, J Branchini, P Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Bremer, J Brendlinger, K Brenner, R Bressler, S Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Broggi, F Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brost, E Brown, G Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Bucci, F Buchanan, J Buchholz, P Buckingham, RM Buckley, AG Buda, SI Budagov, IA Budick, B Buehrer, F Bugge, L Bulekov, O Bundock, AC Bunse, M Buran, T Burckhart, H Burdin, S Burgess, T Burke, S Busato, E Uscher, VB Bussey, P Buszello, CP Butler, B Butler, JM Buttar, CM Butterworth, JM Buttinger, W Byszewski, M Urbaan, SC Caforio, D Cakir, O Calafiura, P Calderini, G Calfayan, P Calkins, R Caloba, LP Caloi, R Calvet, D Calvet, S Toro, RC Camarri, P Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Canale, V Canelli, F Canepa, A Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capriotti, D Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, AA Carter, JR Carvalho, J Casadei, D Casado, MP Caso, C Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Cataldi, G Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caughron, S Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, B Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, K Chang, P Chapleau, B Chapman, JD Chapman, JW Charlton, DG Chavda, V Barajas, CAC Cheatham, S Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, S Chen, X Chen, Y Cheng, Y Cheplakov, A El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiefari, G Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choudalakis, G Chouridou, S Chow, BKB Christidi, IA Christov, A Chromek-Burckhart, D Chu, ML Chudoba, J Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciocio, A Cirilli, M Cirkovic, P Citron, ZH Citterio, M Ciubancan, M Clark, A Clark, PJ Clarke, RN Clemens, JC Clement, B Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coelli, S Coffey, L Cogan, JG Coggeshall, J Colas, J Cole, B Cole, S Colijn, AP Collins-Tooth, C Collot, J Colombo, T Colon, G Compostella, G Muino, PC Coniavitis, E Conidi, MC Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cooper-Smith, NJ Copic, K Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Courneyea, L Cowan, G Cox, BE Cranmer, K Crepe-Renaudin, S Crescioli, F Cristinziani, M Crosetti, G Cuciuc, CM Almenar, CC Donszelmann, TC Cummings, J Curatolo, M Cuthbert, C Czirr, H Czodrowski, P Czyczula, Z D'Auria, S D'Onofrio, M D'Orazio, A De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dallaire, F Dallapiccola, C Dam, M Damiani, DS Daniells, AC Dao, V Darbo, G Darlea, GL Darmora, S Dassoulas, JA Davey, W David, C Davidek, T Davies, E Davies, M Davignon, O Davison, AR Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Castro, S De Cecco, S de Graat, J De Groot, N de 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Wotschack, J. Woudstra, M. J. Wozniak, K. W. Wraight, K. Wright, M. Wrona, B. Wu, S. L. Wu, X. Wu, Y. Wulf, E. Wynne, B. M. Xella, S. Xiao, M. Xu, C. Xu, D. Xu, L. Yabsley, B. Yacoob, S. Yamada, M. Yamaguchi, H. Yamaguchi, Y. Yamamoto, A. Yamamoto, K. Yamamoto, S. Yamamura, T. Yamanaka, T. Yamauchi, K. Yamazaki, Y. Yan, Z. Yang, H. Yang, H. Yang, U. K. Yang, Y. Yang, Z. Yanush, S. Yao, L. Yasu, Y. Yatsenko, E. Wong, K. H. Yau Ye, J. Ye, S. Yen, A. L. Yildirim, E. Yilmaz, M. Yoosoofmiya, R. Yorita, K. Yoshida, R. Yoshihara, K. Young, C. Young, C. J. S. Youssef, S. Yu, D. R. Yu, J. Yu, J. Yuan, L. Yurkewicz, A. Zabinski, B. Zaidan, R. Zaitsev, A. M. Zambito, S. Zanello, L. Zanzi, D. Zaytsev, A. Zeitnitz, C. Zeman, M. Zemla, A. Zenin, O. Zenis, T. Zerwas, D. della Porta, G. Zevi Zhang, D. Zhang, H. Zhang, J. Zhang, L. Zhang, X. Zhang, Z. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zibell, A. Zieminska, D. Zimin, N. I. Zimmermann, C. Zimmermann, R. Zimmermann, S. Zimmermann, S. Zinonos, Z. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zobernig, G. Zoccoli, A. Nedden, M. zur Zurzolo, G. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Search for direct third-generation squark pair production in final states with missing transverse momentum and two b-jets in root s=8 TeV pp collisions with the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering; Supersymmetry ID DYNAMICAL SYMMETRY-BREAKING; SUPERGAUGE TRANSFORMATIONS; SUPERSYMMETRY; MODEL; PARTICLE; CURRENTS; LEPTONS; MASSES; QUARKS; PIONS AB The results of a search for pair production of supersymmetric partners of the Standard Model third-generation quarks are reported. This search uses 20.1 fb(-1) of pp collisions at root s = 8 TeV collected by the ATLAS experiment at the Large Hadron Collider. The lightest bottom and top squarks ((b) over tilde (1) and (t) over tilde (1) respectively) are searched for in a final state with large missing transverse momentum and two jets identified as originating from b-quarks. No excess of events above the expected level of Standard Model background is found. The results are used to set upper limits on the visible cross section for processes beyond the Standard Model. Exclusion limits at the 95% confidence level on the masses of the third-generation squarks are derived in phenomenological supersymmetric R-parity-conserving models in which either the bottom or the top squark is the lightest squark. The (b) over tilde (1) is assumed to decay via (b) over tilde (1) -> b (chi) over tilde (0)(1) and the (t) over tilde (1) via (t) over tilde (1) b (chi) over tilde (+/-)(1), with undetectable products of the subsequent decay of the (chi) over tilde (+/-)(1) due to the small mass splitting between the (chi) over tilde (+/-)(1) and the (chi) over tilde (0)(1) C1 [Jackson, P.; Soni, N.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA, Australia. [Edson, W.; Ernst, J.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY USA. [Chan, K.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Sbrizzi, A.; Subramania, H. S.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran; Kuday, S.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Cakir, I. Turk] Turkish Atom Energy Commiss, Ankara, Turkey. 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[Alison, J.; Anderson, K. J.; Boveia, A.; Canelli, F.; Cheng, Y.; Choudalakis, G.; Fiascaris, M.; Gardner, R. W.; Plante, I. Jen-La; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Cottin, G.; Diaz, M. A.] Pontificia Univ Catolica Chile, Fac Fis, Santiago 22, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Feder Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Huang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Wang, J.; Xu, D.; Yao, L.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Xu, C.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Karpov, S. N.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Karpov, S. N.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Karpov, S. N.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. W.; Kohriki, T.; Metcalfe, J.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perepelitsa, D. V.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Boelaert, N.; Dam, M.; Galster, G.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Coll Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Zeuthen, Germany. [Buckley, A. G.; Bunse, M.; Esch, H.; Gossling, C.; Harrington, R. D.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Reisinger, I.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Grohs, J. P.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Ko, B. R.; Kotwal, A.; Kruse, M. K.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Korn, A.; Martin, V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Amoroso, S.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Christov, A.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Hartert, J.; Herten, G.; Jakobs, K.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; dit Latour, B. Martin; Mermod, P.; Herrera, C. Mora; Muenstermann, D.; Nektarijevic, S.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Caso, C.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Snow, J.; Denis, R. D. St.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Evangelakou, D.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Peters, R. F. Y.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytechn Grenoble, Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hofmann, J. I.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, D-69115 Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, D-69115 Heidelberg, Germany. [Kugel, A.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Halladjian, G.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Goestkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kazarinov, M. Y.; Kharchenko, D.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kondo, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Shiyakova, M.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Franz, S.; Ishino, M.; Sasao, N.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Keresevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Keresevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Gibson, S. M.; Goncalo, R.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Univ London Royal Holloway & Bedford New Coll, Dept Phys, Egham TW20 0EX, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.; Snidero, G.; Wielers, M.] Lund Univ, Fys Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Arnaez, O.; Blum, W.; Uscher, V. B.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Goeringer, C.; Handel, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howarth, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Fletcher, G.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dufour, M-A.; Klemetti, M.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Chapman, J. W.; Chelstowska, M. A.; Cirilli, M.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Qian, J.; Scheirich, D.; Searcy, J.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Hauser, R.; Hayden, D.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; True, P.; Warburton, A.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Coelli, S.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Bouchami, J.; Dallaire, F.; Davies, M.; Gauthier, L.; Giunta, M.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Smizanska, M.; Soldatov, E. Yu.; Timoshenko, S.] MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Snesarev, A. A.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Staude, A.; Walker, R.; Will, J. Z.; Wittkowski, J.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Giovannini, P.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. 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C.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Raas, M.; Salvucci, A.; Toms, K.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Oussoren, K. P.; Pani, P.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. 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V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Strang, M.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. 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Abdel; Auge, E.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Vivie De Regie, J. B.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Smith, K. M.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Larner, A.; Lewis, A.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Young, C. J. S.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Conta, C.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Colombo, T.; Conta, C.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. 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Amor; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Rybar, M.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. 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[Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Fac Sci Ain Chock, Reseau Univ Phys Hautes Energies, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Salvatore, D.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Taffard, A.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Kaczmarska, A.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Jamin, D. O.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Leney, K. J. C.; Garcia, B. R. Mellado; Quayle, W. B.; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Petridis, A.; Plucinski, P.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Petridis, A.; Plucinski, P.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Lee, C. A.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Akimoto, G.; Di Mattia, A.; Hanawa, K.; Kajomovitz, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; Teng, P. K.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Alhroob, M.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Farooque, T.; Fatholahzadeh, B.; Ilic, N.; Keung, J.; Krieger, P.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Fortin, D.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Losty, M. J.; Loureiro, K. F.; Navas, L. Mendoza; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Eschrich, I. Gough; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Coll Udine, Udine, Italy. [Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, IFIC, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, IMB CNM, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] CSIC, Valencia, Spain. [Axen, D.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Courneyea, L.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Mitani, T.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Castaneda-Miranda, E.; Chen, X.; Dos Anjos, A.; Castillo, L. R. Flores; Gutzwiller, O.; Hard, A. S.; Jared, R. C.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Morales, M. I. Pedraza; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Redelbach, A.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Barisonzi, M.; Becker, K.; Becks, K. H.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Sturm, P.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Bernlochner, F. U.; Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, IN2P3, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, Lisbon, Portugal. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Wemans, A. Do Valle] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Kono, T.; Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Pinamonti, M.] SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Tamsett, M. C.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Vickey, T.] Univ Oxford, Dept Phys, Oxford, England. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Doyle, Anthony/C-5889-2009; Ferrando, James/A-9192-2012; Solfaroli Camillocci, Elena/J-1596-2012; Lee, Jason/B-9701-2014; Robson, Aidan/G-1087-2011; Kuday, Sinan/C-8528-2014; Snesarev, Andrey/H-5090-2013; Warburton, Andreas/N-8028-2013; Turchikhin, Semen/O-1929-2013; Boyko, Igor/J-3659-2013; Smirnova, Oxana/A-4401-2013; Sukharev, Andrey/A-6470-2014; Gabrielli, Alessandro/H-4931-2012; Zimmermann, Claus/E-9598-2014; Fabbri, Laura/H-3442-2012; Brooks, William/C-8636-2013; Villa, Mauro/C-9883-2009; Nozka, Libor/G-5550-2014; Nemecek, Stanislav/G-5931-2014; Kepka, Oldrich/G-6375-2014; Lokajicek, Milos/G-7800-2014; Jakoubek, Tomas/G-8644-2014; Staroba, Pavel/G-8850-2014; Kupco, Alexander/G-9713-2014; de Groot, Nicolo/A-2675-2009; Hejbal, Jiri/H-1358-2014; Marcisovsky, Michal/H-1533-2014; Mikestikova, Marcela/H-1996-2014; Lysak, Roman/H-2995-2014; Tomasek, Lukas/G-6370-2014; Svatos, Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Moraes, Arthur/F-6478-2010; Peleganchuk, Sergey/J-6722-2014; Bosman, Martine/J-9917-2014; Castro, Nuno/D-5260-2011; Grinstein, Sebastian/N-3988-2014; Wemans, Andre/A-6738-2012; Gutierrez, Phillip/C-1161-2011; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Mir, Lluisa-Maria/G-7212-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Akimov, Andrey/N-1769-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Demirkoz, Bilge/C-8179-2014; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Gauzzi, Paolo/D-2615-2009; O'Shea, Val/G-1279-2010; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; McKee, Shawn/B-6435-2012; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; OI Doyle, Anthony/0000-0001-6322-6195; Ferrando, James/0000-0002-1007-7816; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Lee, Jason/0000-0002-2153-1519; Kuday, Sinan/0000-0002-0116-5494; Warburton, Andreas/0000-0002-2298-7315; Turchikhin, Semen/0000-0001-6506-3123; Boyko, Igor/0000-0002-3355-4662; Smirnova, Oxana/0000-0003-2517-531X; Gabrielli, Alessandro/0000-0001-5346-7841; Fabbri, Laura/0000-0002-4002-8353; Brooks, William/0000-0001-6161-3570; Villa, Mauro/0000-0002-9181-8048; Mikestikova, Marcela/0000-0003-1277-2596; Tomasek, Lukas/0000-0002-5224-1936; Svatos, Michal/0000-0002-7199-3383; Moraes, Arthur/0000-0002-5157-5686; Peleganchuk, Sergey/0000-0003-0907-7592; Bosman, Martine/0000-0002-7290-643X; Castro, Nuno/0000-0001-8491-4376; Grinstein, Sebastian/0000-0002-6460-8694; Wemans, Andre/0000-0002-9669-9500; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Gauzzi, Paolo/0000-0003-4841-5822; O'Shea, Val/0000-0001-7183-1205; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Karyukhin, Andrey/0000-0001-9087-4315; Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; McKee, Shawn/0000-0002-4551-4502; Doria, Alessandra/0000-0002-5381-2649; Veloso, Filipe/0000-0002-5956-4244; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Coccaro, Andrea/0000-0003-2368-4559 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF; DNSRC; Lundbeck Foundation, Denmark; EPLANET; ERC; NSRF; European Union; IN2P3-CNRS; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF; DFG; HGF; MPG; AvH Foundation, Germany FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZ. S, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America.; The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 77 TC 37 Z9 37 U1 7 U2 150 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 29 PY 2013 IS 10 AR 189 DI 10.1007/JHEP10(2013)189 PG 40 WC Physics, Particles & Fields SC Physics GA 243DM UT WOS:000326296900004 ER PT J AU Davis, JCS Lee, DH AF Davis, J. C. Seamus Lee, Dung-Hai TI Concepts relating magnetic interactions, intertwined electronic orders, and strongly correlated superconductivity SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE high-Tc superconductivity; strong correlations; fermiology ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; VALENCE BOND STATE; T-C SUPERCONDUCTOR; CUPRATE SUPERCONDUCTORS; PSEUDOGAP STATE; PHYSICS; INSTABILITY; TRANSITION; COMPLEXITY; ANISOTROPY AB Unconventional superconductivity (SC) is said to occur when Cooper pair formation is dominated by repulsive electron-electron interactions, so that the symmetry of the pair wave function is other than an isotropic s-wave. The strong, on-site, repulsive electron-electron interactions that are the proximate cause of such SC are more typically drivers of commensurate magnetism. Indeed, it is the suppression of commensurate antiferromagnetism (AF) that usually allows this type of unconventional superconductivity to emerge. Importantly, however, intervening between these AF and SC phases, intertwined electronic ordered phases (IP) of an unexpected nature are frequently discovered. For this reason, it has been extremely difficult to distinguish the microscopic essence of the correlated superconductivity from the often spectacular phenomenology of the IPs. Here we introduce a model conceptual framework within which to understand the relationship between AF electron-electron interactions, IPs, and correlated SC. We demonstrate its effectiveness in simultaneously explaining the consequences of AF interactions for the copper-based, iron-based, and heavy-fermion superconductors, as well as for their quite distinct IPs. C1 [Davis, J. C. Seamus] Cornell Univ, Dept Phys, Ithaca, NY 14853 USA. [Davis, J. C. Seamus] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Davis, J. C. Seamus] Univ St Andrews, Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland. [Davis, J. C. Seamus] Cornell Univ, Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA. [Lee, Dung-Hai] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Lee, Dung-Hai] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Davis, JCS (reprint author), Cornell Univ, Dept Phys, Ithaca, NY 14853 USA. EM jcdavis@ccmr.cornell.edu; dunghai@berkeley.edu FU US Department of Energy (DOE) [Grant DE-2009-BNL-PM015]; DOE Office of Basic Energy Sciences, Division of Materials Science [DE-AC02-05CH11231]; Center for Emergent Superconductivity, an Energy Frontier Research Center; Energy Frontier Research Center at Brookhaven National Laboratory FX We thank S. A. Kivelson for a most useful discussion on the Q = 0 instabilities in the cuprates. We also thank D. K. Morr, M. Norman, and S. Sachdev for helpful discussions and communications. J.C.S.D. is supported by the Center for Emergent Superconductivity, an Energy Frontier Research Center, headquartered at Brookhaven National Laboratory and funded by the US Department of Energy (DOE), under Grant DE-2009-BNL-PM015. D.-H.L. is supported by the DOE Office of Basic Energy Sciences, Division of Materials Science, under Grant DE-AC02-05CH11231. NR 59 TC 70 Z9 70 U1 6 U2 37 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 29 PY 2013 VL 110 IS 44 BP 17623 EP 17630 DI 10.1073/pnas.1316512110 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 242LJ UT WOS:000326243100019 PM 24114268 ER PT J AU Chakraborty, S Jackson, TL Ahmed, M Thiemens, MH AF Chakraborty, Subrata Jackson, Teresa L. Ahmed, Musahid Thiemens, Mark H. TI Sulfur isotopic fractionation in vacuum UV photodissociation of hydrogen sulfide and its potential relevance to meteorite analysis SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE chondrites; achondrites; isotope ID MULTIPHOTON IONIZATION SPECTROSCOPY; MASS-INDEPENDENT FRACTIONATION; SOLAR NEBULA; CARBONACEOUS CHONDRITES; NO2 ISOTOPOLOGUES; H2S MOLECULE; OXYGEN; SYSTEM; DYNAMICS; DISSOCIATION AB Select meteoritic classes possess mass-independent sulfur isotopic compositions in sulfide and organic phases. Photochemistry in the solar nebula has been attributed as a source of these anomalies. Hydrogen sulfide (H2S) is the most abundant gas-phase species in the solar nebula, and hence, photodissociation of H2S by solar vacuum UV (VUV) photons (especially by Lyman-alpha radiation) is a relevant process. Because of experimental difficulties associated with accessing VUV radiation, there is a paucity of data and a lack of theoretical basis to test the hypothesis of a photochemical origin of mass-independent sulfur. Here, we present multiisotopic measurements of elemental sulfur produced during the VUV photolysis of H2S. Mass-independent sulfur isotopic compositions are observed. The observed isotopic fractionation patterns are wavelength-dependent. VUV photodissociation of H2S takes place through several predissociative channels, and the measured mass-independent fractionation is most likely a manifestation of these processes. Meteorite sulfur data are discussed in light of the present experiments, and suggestions are made to guide future experiments and models. C1 [Chakraborty, Subrata; Jackson, Teresa L.; Thiemens, Mark H.] Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA. [Ahmed, Musahid] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Chakraborty, S (reprint author), Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA. EM s1chakraborty@ucsd.edu RI Ahmed, Musahid/A-8733-2009 FU Office of Science, Office of Basic Energy Sciences; Division of Chemical Sciences, Geosciences, and Biosciences of the US Department of Energy at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX S. C. thanks Ryan D. Davis for his help in performing experiments at Advanced Light Source. Support from Ms. Sarah Ferrell and Dr. Amir Golan (Chemical Dynamics Beamline at the Advanced Light Source) and Dr. Doug Taube (Chemistry Laboratory Manager of Advanced Light Source) is acknowledged. Two anonymous reviewers and the editor are acknowledged for comments that improved the manuscript. The work is funded through National Aeronautics and Space Administration's Origins and Cosmochemistry programs. M. A. and the Advanced Light Source are supported by the Director, Office of Science, Office of Basic Energy Sciences and the Division of Chemical Sciences, Geosciences, and Biosciences of the US Department of Energy at Lawrence Berkeley National Laboratory under Contract DE-AC02-05CH11231. NR 68 TC 6 Z9 6 U1 4 U2 29 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 29 PY 2013 VL 110 IS 44 BP 17650 EP 17655 DI 10.1073/pnas.1213150110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 242LJ UT WOS:000326243100023 PM 23431159 ER PT J AU Fan, Y Osetskiy, YN Yip, S Yildiz, B AF Fan, Yue Osetskiy, Yuri N. Yip, Sidney Yildiz, Bilge TI Mapping strain rate dependence of dislocation-defect interactions by atomistic simulations SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE structural materials; mechanical properties; low strain rate atomistic simulation ID STACKING-FAULT TETRAHEDRON; MOLECULAR-DYNAMICS SIMULATIONS; IRRADIATED ZIRCONIUM ALLOYS; ALPHA-ZIRCONIUM; OBSTACLE INTERACTIONS; EDGE DISLOCATIONS; DEFORMATION; METALS; SCALE; MECHANISMS AB Probing the mechanisms of defect-defect interactions at strain rates lower than 10(6) s(-1) is an unresolved challenge to date to molecular dynamics (MD) techniques. Here we propose an original atomistic approach based on transition state theory and the concept of a strain-dependent effective activation barrier that is capable of simulating the kinetics of dislocation-defect interactions at virtually any strain rate, exemplified within 10(-7) to 10(7) s(-1). We apply this approach to the problem of an edge dislocation colliding with a cluster of self-interstitial atoms (SIAs) under shear deformation. Using an activation-relaxation algorithm [Kushima A, et al. (2009) J Chem Phys 130:224504], we uncover a unique strain-rate-dependent trigger mechanism that allows the SIA cluster to be absorbed during the process, leading to dislocation climb. Guided by this finding, we determine the activation barrier of the trigger mechanism as a function of shear strain, and use that in a coarse-graining rate equation formulation for constructing a mechanism map in the phase space of strain rate and temperature. Our predictions of a crossover from a defect recovery at the low strain-rate regime to defect absorption behavior in the high strain-rate regime are validated against our own independent, direct MD simulations at 10(5) to 10(7) s(-1). Implications of the present approach for probing molecular-level mechanisms in strain-rate regimes previously considered inaccessible to atomistic simulations are discussed. C1 [Fan, Yue; Yip, Sidney; Yildiz, Bilge] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA. [Yip, Sidney] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Osetskiy, Yuri N.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Yildiz, B (reprint author), MIT, Dept Nucl Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM byildiz@mit.edu RI FAN, YUE/H-1737-2011; OI Osetskiy, Yury/0000-0002-8109-0030 FU Consortium for Advanced Simulation of Light Water Reactors; Energy Innovation Hub for Modeling and Simulation of Nuclear Reactors under US Department of Energy [DE-AC05-00OR22725]; Division of Materials Sciences and Engineering, US Department of Energy FX This work was supported by the Consortium for Advanced Simulation of Light Water Reactors, an Energy Innovation Hub for Modeling and Simulation of Nuclear Reactors under US Department of Energy Contract DE-AC05-00OR22725, and Y.N.O. was supported by the Division of Materials Sciences and Engineering, US Department of Energy. NR 50 TC 28 Z9 28 U1 5 U2 55 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 29 PY 2013 VL 110 IS 44 BP 17756 EP 17761 DI 10.1073/pnas.1310036110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 242LJ UT WOS:000326243100041 PM 24114271 ER PT J AU Zhao, JJ Chatterjee, U Ai, DF Hinks, DG Zheng, H Gu, GD Castellan, JP Rosenkranz, S Claus, H Norman, MR Randeria, M Campuzano, JC AF Zhao, Junjing Chatterjee, Utpal Ai, Dingfei Hinks, David G. Zheng, Hong Gu, G. D. Castellan, John-Paul Rosenkranz, Stephan Claus, Helmut Norman, Michael R. Randeria, Mohit Campuzano, Juan Carlos TI Universal features in the photoemission spectroscopy of high-temperature superconductors SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article ID T-C SUPERCONDUCTOR; UNDERDOPED BI2SR2CACU2O8+DELTA; QUASI-PARTICLES; GAP ANISOTROPY; NORMAL-STATE; ENERGY GAPS; PSEUDOGAP; SYMMETRY AB The energy gap for electronic excitations is one of the most important characteristics of the superconducting state, as it directly reflects the pairing of electrons. In the copper-oxide high-temperature superconductors (HTSCs), a strongly anisotropic energy gap, which vanishes along high-symmetry directions, is a clear manifestation of the d-wave symmetry of the pairing. There is, however, a dramatic change in the form of the gap anisotropy with reduced carrier concentration (underdoping). Although the vanishing of the gap along the diagonal to the square Cu-O bond directions is robust, the doping dependence of the large gap along the Cu-O directions suggests that its origin might be different from pairing. It is thus tempting to associate the large gap with a second-order parameter distinct from superconductivity. We use angle-resolved photoemission spectroscopy to show that the two-gap behavior and the destruction of well-defined electronic excitations are not universal features of HTSCs, and depend sensitively on how the underdoped materials are prepared. Depending on cation substitution, underdoped samples either show two-gap behavior or not. In contrast, many other characteristics of HTSCs, such as the dome-like dependence of T-c on doping, long-lived excitations along the diagonals to the Cu-O bonds, and an energy gap at the Brillouin zone boundary that decreases monotonically with doping while persisting above T-c (the pseudogap), are present in all samples, irrespective of whether they exhibit two-gap behavior or not. Our results imply that universal aspects of high-T-c superconductivity are relatively insensitive to differences in the electronic states along the Cu-O bond directions. C1 [Zhao, Junjing; Ai, Dingfei; Campuzano, Juan Carlos] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Zhao, Junjing; Chatterjee, Utpal; Hinks, David G.; Zheng, Hong; Castellan, John-Paul; Rosenkranz, Stephan; Claus, Helmut; Norman, Michael R.; Campuzano, Juan Carlos] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Gu, G. D.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Randeria, Mohit] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. RP Campuzano, JC (reprint author), Univ Illinois, Dept Phys, Chicago, IL 60607 USA. EM jcc@uic.edu RI Rosenkranz, Stephan/E-4672-2011; Norman, Michael/C-3644-2013 OI Rosenkranz, Stephan/0000-0002-5659-0383; FU Basic Energy Sciences (BES), Office of Science, US Department of Energy (DOE) [DE-AC02-06CH11357]; DOE-BES [DE-SC0005035]; DOE [DE-AC02-98CH10886]; University of Wisconsin-Madison FX We thank D. Robinson and J.P.C. Ruff for support with the high-energy X-ray diffraction measurements. Work at Argonne was supported by Basic Energy Sciences (BES), Office of Science, US Department of Energy (DOE) under Contract DE-AC02-06CH11357 (to J.Z., U.C., D.G. H., H.Z., S.R., H.C., M.R.N., and J.C.C.). M.R. was supported by the DOE-BES Grant DE-SC0005035. G.D.G. was supported by the DOE Contract No. DE-AC02-98CH10886. The Synchrotron Radiation Center is supported by the University of Wisconsin-Madison. NR 31 TC 5 Z9 5 U1 4 U2 19 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 29 PY 2013 VL 110 IS 44 BP 17774 EP 17777 DI 10.1073/pnas.1302932110 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 242LJ UT WOS:000326243100044 PM 24101464 ER PT J AU Edayathumangalam, R Wu, R Garcia, R Wang, YG Wang, W Kreinbring, CA Bach, A Liao, JL Stone, TA Terwilliger, TC Hoang, QQ Belitsky, BR Petsko, GA Ringe, D Liu, D AF Edayathumangalam, Raji Wu, Rui Garcia, Roman Wang, Yuguang Wang, Wei Kreinbring, Cheryl A. Bach, Alicia Liao, Jingling Stone, Todd A. Terwilliger, Thomas C. Hoang, Quyen Q. Belitsky, Boris R. Petsko, Gregory A. Ringe, Dagmar Liu, Dali TI Crystal structure of Bacillus subtilis GabR, an autorepressor and transcriptional activator of gabT SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article ID ASPARTATE-AMINOTRANSFERASE; DEPENDENT ENZYMES; FACTOR FADR; PROTEIN; DOMAINS; RECOGNITION; BINDING; FAMILY; MOCR AB Bacillus subtilis GabR is a transcription factor that regulates gamma-aminobutyric acid (GABA) metabolism. GabR is a member of the understudied MocR/GabR subfamily of the GntR family of transcription regulators. A typical MocR/GabR-type regulator is a chimeric protein containing a short N-terminal helix-turn-helix DNA-binding domain and a long C-terminal pyridoxal 5'-phosphate (PLP)-binding putative aminotransferase domain. In the presence of PLP and GABA, GabR activates the gabTD operon, which allows the bacterium to use GABA as nitrogen and carbon sources. GabR binds to its own promoter and represses gabR transcription in the absence of GABA. Here, we report two crystal structures of full-length GabR from B. subtilis: a 2.7-angstrom structure of GabR with PLP bound and the 2.55-angstrom apo structure of GabR without PLP. The quaternary structure of GabR is a head-to-tail domain-swap homodimer. Each monomer comprises two domains: an N-terminal winged-helix DNA-binding domain and a C-terminal PLP-binding type I aminotransferase-like domain. The winged-helix domain contains putative DNA-binding residues conserved in other GntR-type regulators. Together with sedimentation velocity and fluorescence polarization assays, the crystal structure of GabR provides insights into DNA binding by GabR at the gabR and gabT promoters. The absence of GabR-mediated aminotransferase activity in the presence of GABA and PLP, and the presence of an active site configuration that is incompatible with stabilization of the GABA external aldimine suggest that a GabR aminotransferase-like activity involving GABA and PLP is not essential to its primary function as a transcription regulator. C1 [Edayathumangalam, Raji] Harvard Univ, Sch Med, Ctr Neurol Dis, Boston, MA 02115 USA. [Edayathumangalam, Raji] Brigham & Womens Hosp, Boston, MA 02115 USA. [Edayathumangalam, Raji; Kreinbring, Cheryl A.; Bach, Alicia; Petsko, Gregory A.; Ringe, Dagmar] Brandeis Univ, Rosenstiel Basic Med Sci Res Ctr, Dept Biochem, Waltham, MA 02454 USA. [Wu, Rui; Garcia, Roman; Wang, Yuguang; Liu, Dali] Loyola Univ, Dept Chem & Biochem, Chicago, IL 60626 USA. [Wang, Wei; Liao, Jingling; Hoang, Quyen Q.] Indiana Univ, Sch Med, Stark Neurosci Res Inst, Dept Biochem & Mol Biol, Indianapolis, IN 46202 USA. [Stone, Todd A.] Indiana Univ, Dept Mol & Cellular Biochem, Bloomington, IN 47405 USA. [Terwilliger, Thomas C.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. [Belitsky, Boris R.] Tufts Univ, Sch Med, Dept Mol Biol & Microbiol, Boston, MA 02111 USA. RP Petsko, GA (reprint author), Brandeis Univ, Rosenstiel Basic Med Sci Res Ctr, Dept Biochem, Waltham, MA 02454 USA. EM petsko@brandeis.edu; ringe@brandeis.edu; dliu@luc.edu RI Terwilliger, Thomas/K-4109-2012 OI Terwilliger, Thomas/0000-0001-6384-0320 FU Loyola University Chicago; NSF [CHE-1308672, MCB-0110651]; National Institutes of Health FX We thank Boguslaw Nocek (Structural Biology Center, Sector 19) at Advance Photon Source, Argonne National Laboratory for help with data collection; Zbyszek Dauter, Eleanor Dodson, Frank DiMaio, Nathaniel Echols, Julia Klutkowski, Ruslan Sanishvili, Miguel Ballicora, and Janet Smith for helpful discussions, suggestions, and/or technical help. This work was funded by the start-up funds from Loyola University Chicago (to D.L.), an NSF subaward from Grant CHE-1308672 (to D.L.), NSF Grant MCB-0110651 (to B.R.B.), and a grant from the National Institutes of Health (to D.R. and G.A.P.). NR 19 TC 23 Z9 23 U1 2 U2 10 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 29 PY 2013 VL 110 IS 44 BP 17820 EP 17825 DI 10.1073/pnas.1315887110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 242LJ UT WOS:000326243100052 PM 24127574 ER PT J AU Parker, SCJ Stitzel, ML Taylor, DL Orozco, JM Erdos, MR Akiyama, JA van Bueren, KL Chines, PS Narisu, N Black, BL Visel, A Pennacchio, LA Collins, FS AF Parker, Stephen C. J. Stitzel, Michael L. Taylor, D. Leland Orozco, Jose Miguel Erdos, Michael R. Akiyama, Jennifer A. van Bueren, Kelly Lammerts Chines, Peter S. Narisu, Narisu Black, Brian L. Visel, Axel Pennacchio, Len A. Collins, Francis S. CA NISC Comparative Sequencing TI Chromatin stretch enhancer states drive cell-specific gene regulation and harbor human disease risk variants SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article ID SUPER-ENHANCERS; SNP RS6983267; HUMAN GENOME; DISCOVERY; ELEMENTS; DNA; ANNOTATION; EXPRESSION; COHESIN; ISLETS AB Chromatin-based functional genomic analyses and genomewide association studies (GWASs) together implicate enhancers as critical elements influencing gene expression and risk for common diseases. Here, we performed systematic chromatin and transcriptome profiling in human pancreatic islets. Integrated analysis of islet data with those from nine cell types identified specific and significant enrichment of type 2 diabetes and related quantitative trait GWAS variants in islet enhancers. Our integrated chromatin maps reveal that most enhancers are short (median = 0.8 kb). Each cell type also contains a substantial number of more extended (>= 3 kb) enhancers. Interestingly, these stretch enhancers are often tissue-specific and overlap locus control regions, suggesting that they are important chromatin regulatory beacons. Indeed, we show that (i) tissue specificity of enhancers and nearby gene expression increase with enhancer length; (ii) neighborhoods containing stretch enhancers are enriched for important cell type-specific genes; and (iii) GWAS variants associated with traits relevant to a particular cell type are more enriched in stretch enhancers compared with short enhancers. Reporter constructs containing stretch enhancer sequences exhibited tissue-specific activity in cell culture experiments and in transgenic mice. These results suggest that stretch enhancers are critical chromatin elements for coordinating cell type-specific regulatory programs and that sequence variation in stretch enhancers affects risk of major common human diseases. C1 [Parker, Stephen C. J.; Stitzel, Michael L.; Taylor, D. Leland; Orozco, Jose Miguel; Erdos, Michael R.; Chines, Peter S.; Narisu, Narisu; Collins, Francis S.; NISC Comparative Sequencing] Natl Human Genome Res Inst, NIH, Bethesda, MD 20892 USA. [Akiyama, Jennifer A.; Visel, Axel; Pennacchio, Len A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [van Bueren, Kelly Lammerts; Black, Brian L.] Univ Calif San Francisco, Cardiovasc Res Inst, San Francisco, CA 95158 USA. [Visel, Axel; Pennacchio, Len A.] Joint Genome Inst, Dept Energy, Walnut Creek, CA 94598 USA. RP Collins, FS (reprint author), Natl Human Genome Res Inst, NIH, Bethesda, MD 20892 USA. EM collinsf@od.nih.gov RI Visel, Axel/A-9398-2009; OI Visel, Axel/0000-0002-4130-7784; Black, Brian/0000-0002-6664-8913; Taylor, Leland/0000-0001-6498-6970 FU Postdoctoral Research Associate (PRAT) fellowship [1ZIAHG000024, K99DK092251, K99DK099240, R01HL64658, R01DE019118]; E.O. Lawrence Berkeley National Laboratory [R01HG003988]; Department of Energy, University of California [DEAC02-05CH11231] FX We thank the Finland United States Investigation of NIDDM Genetics Consortium and National Institutes of Health (NIH) Chromatin community for valuable critiques and discussion. We thank Lori Bonnycastle, Laura Elnitski, Andrea Ramirez, Mario Morken, and Adam Woolfe for helpful comments. Human islets were obtained from organ donors through the ICR Basic Science Islet Distribution Program (Universities of Illinois, Washington, Miami, and Alabama at Birmingham) and the National Disease Research Interchange. We thank the reviewers for excellent feedback and suggestions. This work was supported by Postdoctoral Research Associate (PRAT) fellowship (to S.C.J.P.); Grants 1ZIAHG000024 (to F.S.C.), K99DK092251 (to M.L.S.), K99DK099240 (to S.C.J.P.), R01HL64658 (to B.L.B.), and R01DE019118 (to B.L.B.). A.V. and L.A.P. are supported by Grant R01HG003988 and conducted research at the E.O. Lawrence Berkeley National Laboratory, performed under Department of Energy Contract DEAC02-05CH11231, University of California. NR 33 TC 150 Z9 150 U1 2 U2 23 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 29 PY 2013 VL 110 IS 44 BP 17921 EP 17926 DI 10.1073/pnas.1317023110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 242LJ UT WOS:000326243100069 PM 24127591 ER PT J AU Chung, M Collura, MG Flanagan, G Freemire, B Hanlet, PM Jana, MR Johnson, RP Kaplan, DM Leonova, M Moretti, A Popovic, M Schwarz, T Tollestrup, A Torun, Y Yonehara, K AF Chung, M. Collura, M. G. Flanagan, G. Freemire, B. Hanlet, P. M. Jana, M. R. Johnson, R. P. Kaplan, D. M. Leonova, M. Moretti, A. Popovic, M. Schwarz, T. Tollestrup, A. Torun, Y. Yonehara, K. TI Pressurized H-2 rf Cavities in Ionizing Beams and Magnetic Fields SO PHYSICAL REVIEW LETTERS LA English DT Article ID HYDROGEN; ELECTRONS; GASES; IONS AB A major technological challenge in building a muon cooling channel is operating rf cavities in multitesla external magnetic fields. We report the first proof-of-principle experiment of a high pressure gas-filled rf cavity for use with intense ionizing beams and strong external magnetic fields. rf power consumption by beam-induced plasma is investigated with hydrogen and deuterium gases with pressures between 20 and 100 atm and peak rf gradients between 5 and 50 MV/m. The low pressure case agrees well with an analytical model based on electron and ion mobilities. Varying concentrations of oxygen gas are investigated to remove free electrons from the cavity and reduce the rf power consumption. Measurements of the electron attachment time to oxygen and rate of ion-ion recombination are also made. Additionally, we demonstrate the operation of the gas-filled rf cavity in a solenoidal field of up to 3 T, finding no major magnetic field dependence. All these results indicate that a high pressure gas-filled cavity is a viable technology for muon ionization cooling. C1 [Chung, M.; Collura, M. G.; Jana, M. R.; Leonova, M.; Moretti, A.; Popovic, M.; Schwarz, T.; Tollestrup, A.; Yonehara, K.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Flanagan, G.; Johnson, R. P.] Muons Inc, Batavia, IL 60134 USA. [Freemire, B.; Hanlet, P. M.; Kaplan, D. M.; Torun, Y.] IIT, Chicago, IL 60616 USA. RP Chung, M (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. FU Fermi Research Alliance, LLC [DE-AC02-07CH11359]; U.S. Department of Energy; U.S. Department of Energy STTR [DE-C00006266]; U.S. Muon Accelerator Program (MAP) FX The authors would like to thank R. Johnsen (University of Pittsburgh) for helpful comments and discussions. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the U.S. Department of Energy. This work was partially supported by U.S. Department of Energy STTR Grant No. DE-C00006266 and by grants from the U.S. Muon Accelerator Program (MAP) to Illinois Institute of Technology. NR 30 TC 4 Z9 4 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 29 PY 2013 VL 111 IS 18 AR 184802 DI 10.1103/PhysRevLett.111.184802 PG 5 WC Physics, Multidisciplinary SC Physics GA 242XM UT WOS:000326279100012 PM 24237526 ER PT J AU Hay, MJ Valeo, EJ Fisch, NJ AF Hay, Michael J. Valeo, Ernest J. Fisch, Nathaniel J. TI Geometrical Optics of Dense Aerosols: Forming Dense Plasma Slabs SO PHYSICAL REVIEW LETTERS LA English DT Article ID EXPANSIONS; BEAMS AB Assembling a freestanding, sharp-edged slab of homogeneous material that is much denser than gas, but much more rarefied than a solid, is an outstanding technological challenge. The solution may lie in focusing a dense aerosol to assume this geometry. However, whereas the geometrical optics of dilute aerosols is a well-developed field, the dense aerosol limit is mostly unexplored. Yet controlling the geometrical optics of dense aerosols is necessary in preparing such a material slab. Focusing dense aerosols is shown here to be possible, but the finite particle density reduces the effective Stokes number of the flow, a critical result for controlled focusing. C1 [Hay, Michael J.; Fisch, Nathaniel J.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Valeo, Ernest J.; Fisch, Nathaniel J.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Hay, MJ (reprint author), Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. EM hay@princeton.edu FU DOE [DE-AC02-09CH11466]; DOE NNSA SSGF [DE-FC52-08NA28752] FX This work was performed under DOE Contract No. DE-AC02-09CH11466. M.J.H. was supported by the DOE NNSA SSGF under Grant No. DE-FC52-08NA28752. NR 10 TC 3 Z9 3 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 29 PY 2013 VL 111 IS 18 AR 188301 DI 10.1103/PhysRevLett.111.188301 PG 5 WC Physics, Multidisciplinary SC Physics GA 242XM UT WOS:000326279100022 PM 24237567 ER PT J AU Mahler, DH Rozema, LA Darabi, A Ferrie, C Blume-Kohout, R Steinberg, AM AF Mahler, D. H. Rozema, Lee A. Darabi, Ardavan Ferrie, Christopher Blume-Kohout, Robin Steinberg, A. M. TI Adaptive Quantum State Tomography Improves Accuracy Quadratically SO PHYSICAL REVIEW LETTERS LA English DT Article ID DISTANCE AB We introduce a simple protocol for adaptive quantum state tomography, which reduces the worst-case infidelity [1 - F((rho) over cap, rho)] between the estimate and the true state from O(1/root N) to O(1/N). It uses a single adaptation step and just one extra measurement setting. In a linear optical qubit experiment, we demonstrate a full order of magnitude reduction in infidelity (from 0.1% to 0.01%) for a modest number of samples (N approximate to 3 x 10(4)). C1 [Mahler, D. H.; Rozema, Lee A.; Darabi, Ardavan; Steinberg, A. M.] Univ Toronto, Ctr Quantum Informat & Quantum Control, Dept Phys, Toronto, ON M5S 1A7, Canada. [Mahler, D. H.; Rozema, Lee A.; Darabi, Ardavan; Steinberg, A. M.] Univ Toronto, Inst Opt Sci, Toronto, ON M5S 1A7, Canada. [Mahler, D. H.; Rozema, Lee A.; Darabi, Ardavan; Steinberg, A. M.] Canadian Inst Adv Res, Toronto, ON M5G 1Z8, Canada. [Ferrie, Christopher] Univ New Mexico, Ctr Quantum Informat & Control, Albuquerque, NM 87131 USA. [Blume-Kohout, Robin] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Mahler, DH (reprint author), Univ Toronto, Ctr Quantum Informat & Quantum Control, Dept Phys, 60 St George St, Toronto, ON M5S 1A7, Canada. EM dmahler@physics.utoronto.ca RI Ferrie, Christopher/C-8330-2014; Steinberg, Aephraim/C-3226-2008; OI Ferrie, Christopher/0000-0003-2736-9943 FU NSF [PHY-1212445, PHY-1005540]; LDRD program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; NSERC PDF FX D.H. M., L.A. R., A.D., and A.M.S. thank NSERC and CIFAR for support, and Alan Stummer for designing the coincidence circuit. C.F. was supported in part by NSF Grants No. PHY-1212445 and No. PHY-1005540 and an NSERC PDF. R.B.K. was supported by the LDRD program at Sandia National Laboratories, a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 29 TC 25 Z9 25 U1 1 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 29 PY 2013 VL 111 IS 18 AR 183601 DI 10.1103/PhysRevLett.111.183601 PG 5 WC Physics, Multidisciplinary SC Physics GA 242XM UT WOS:000326279100011 PM 24237518 ER PT J AU Rodriguez, AW Reid, MTH Intravaia, F Woolf, A Dalvit, DAR Capasso, F Johnson, SG AF Rodriguez, Alejandro W. Reid, M. T. Homer Intravaia, Francesco Woolf, Alexander Dalvit, Diego A. R. Capasso, Federico Johnson, Steven G. TI Geometry-Induced Casimir Suspension of Oblate Bodies in Fluids SO PHYSICAL REVIEW LETTERS LA English DT Article ID FORCES AB We predict that a low-permittivity oblate body (disk-shaped object) above a thin metal substrate (plate with a hole) immersed in a fluid of intermediate permittivity will experience a metastable equilibrium (restoring force) near the center of the hole. Stability is the result of a geometry-induced transition in the sign of the force, from repulsive to attractive, that occurs as the disk approaches the hole-in planar or nearly planar geometries, the same material combination yields a repulsive force at all separations, in accordance with the Dzyaloshinskii-Lifshitz-Pitaevskii condition of fluid-induced repulsion between planar bodies. We explore the stability of the system with respect to rotations and lateral translations of the disks and demonstrate interesting transitions (bifurcations) in the rotational stability of the disks as a function of their size. Finally, we consider the reciprocal situation in which the disk-plate materials are interchanged and find that in this case the system also exhibits metastability. The forces in the system are sufficiently large to be observed in experiments and should enable measurements based on the diffusion dynamics of the suspended bodies. C1 [Rodriguez, Alejandro W.] Princeton Univ, Dept Elect Engn, Princeton, NJ 08540 USA. [Reid, M. T. Homer; Johnson, Steven G.] MIT, Dept Math, Cambridge, MA 02139 USA. [Woolf, Alexander; Capasso, Federico] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Intravaia, Francesco; Dalvit, Diego A. R.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Intravaia, Francesco] Univ Nottingham, Sch Phys & Astron, Nottingham NG7 2RD, England. RP Rodriguez, AW (reprint author), Princeton Univ, Dept Elect Engn, Princeton, NJ 08540 USA. RI Intravaia, Francesco/E-6500-2010 OI Intravaia, Francesco/0000-0001-7993-4698 FU DARPA [N66001-09-1-2070-DOD]; AFOSR Multidisciplinary Research Program of the University Research Initiative (MURI) for Complex and Robust On-chip Nanophotonics [FA9550-09-1-0704]; U.S. Army Research Office [W911NF-07-D-0004, W911NF-13-D-0001] FX This work was supported by DARPA Contract No. N66001-09-1-2070-DOD, by the AFOSR Multidisciplinary Research Program of the University Research Initiative (MURI) for Complex and Robust On-chip Nanophotonics, Grant No. FA9550-09-1-0704, and by the U.S. Army Research Office under Contracts No. W911NF-07-D-0004 and No. W911NF-13-D-0001. NR 33 TC 3 Z9 3 U1 2 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 29 PY 2013 VL 111 IS 18 AR UNSP 180402 DI 10.1103/PhysRevLett.111.180402 PG 5 WC Physics, Multidisciplinary SC Physics GA 242XM UT WOS:000326279100003 PM 24237491 ER PT J AU Gori, S Jung, S Wang, LT AF Gori, Stefania Jung, Sunghoon Wang, Lian-Tao TI Cornering electroweakinos at the LHC SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry Phenomenology ID MASS-DEGENERATE; LIGHTEST NEUTRALINO; SEARCH; SUPERSYMMETRY; CHARGINOS; COLLISIONS AB Squeezed supersymmetric spectra are challenging for the LHC searches based on a sizable missing energy and hard visible particles. One such scenario consists of chargino/second-lightest neutralino NLSPs and a lightest neutralino LSP with a relatively small mass gap (m(chi(NLSP)) - m(chi(LSP)) equivalent to Delta similar to (10 - 50) GeV). In this note, we explore search strategies to better probe this parameter space. We focus on the 3l + E-T(miss) channel arising from the chargino/second-lightest neutralino associated production, and we investigate the role of a relatively hard initial state radiation (ISR) jet. In addition to typical kinematic variables, such as the minimum lepton pair invariant mass, we propose an angular separation variable and two ratio variables which capitalize on the main kinematic features; leptons stay relatively soft under the boost from ISR and a sizable missing energy arises only in tight correlation with the ISR boost. With 300/fb of data at the 14 TeV LHC, we expect to probe electroweakinos up to 320 (700) GeV with Delta similar to 30 GeV and up to 220 (620) GeV with Delta similar to 20 GeV if gauginos decay via gauge bosons (light sleptons). We emphasize that the 3l channel is technically challenging for mass gaps below similar to 12 GeV. C1 [Gori, Stefania; Jung, Sunghoon; Wang, Lian-Tao] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Gori, Stefania; Jung, Sunghoon; Wang, Lian-Tao] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Gori, Stefania] Argonne Natl Lab, HEP Div, Argonne, IL 60439 USA. [Jung, Sunghoon] Korea Inst Adv Study, Sch Phys, Seoul 130722, South Korea. [Wang, Lian-Tao] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. RP Gori, S (reprint author), Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. EM goris@uchicago.edu; nejsh21@kias.re.kr; liantaow@uchicago.edu FU DOE [de-sc0003930, DE-AC02-06CH11357, DE-FGO2-96-ER40956]; National Science Foundation [NSF PHY11-25915] FX S.G. and L.T.W would like to thank KITP for its hospitality during some part of this work has been carried out. S.J. is grateful to Chicago 2012 LHC workshop where part of this work is carried out. SJ thanks KIAS Center for Advanced Computation for providing computing resources. L. T. W. is supported by the DOE Early Career Award under grant de-sc0003930. This work is supported in part by DOE under Contract No. DE-AC02-06CH11357 (ANL), DE-FGO2-96-ER40956 (U. Chicago) and by the National Science Foundation under Grant No. NSF PHY11-25915 (KITP). NR 43 TC 27 Z9 27 U1 0 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 29 PY 2013 IS 10 AR 191 DI 10.1007/JHEP10(2013)191 PG 20 WC Physics, Particles & Fields SC Physics GA 243DP UT WOS:000326297300001 ER PT J AU Armstrong, GSJ Colgan, J Pindzola, MS AF Armstrong, G. S. J. Colgan, J. Pindzola, M. S. TI Angular distributions for the electron-impact single ionization of sodium and magnesium SO PHYSICAL REVIEW A LA English DT Article ID COLLISIONS AB We present angular distributions for the electron-impact single ionization of sodium and magnesium at intermediate incident electron energies. The results are obtained from a full-dimensionality solution of the two-active-electron time-dependent Schrodinger equation using the time-dependent close-coupling method. We compare calculated angular distributions with existing measurements. We find good overall agreement with measurements over a range of incident electron energies in both cases. We also calculate angular distributions for ejection configurations in which no measurements are currently available. C1 [Armstrong, G. S. J.; Colgan, J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Pindzola, M. S.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. RP Armstrong, GSJ (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Colgan, James/0000-0003-1045-3858 FU National Nuclear Security Administration of the U. S. Department of Energy [DE-AC5206NA25396]; U. S. DOE; U. S. NSF FX The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the National Nuclear Security Administration of the U. S. Department of Energy under Contract No. DE-AC5206NA25396. Computational work was carried out at Los Alamos National Laboratory through the provision of an Institutional Computing Resources award. This work was supported in part by grants from the U. S. DOE and U. S. NSF to Auburn University. We thank K. L. Nixon and A. J. Murray for useful discussions. NR 30 TC 3 Z9 4 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD OCT 29 PY 2013 VL 88 IS 4 AR UNSP 042713 DI 10.1103/PhysRevA.88.042713 PG 7 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 242VH UT WOS:000326271000006 ER PT J AU Colby, R Qiao, L Zhang, KHL Shutthanandan, V Ciston, J Kabius, B Chambers, SA AF Colby, R. Qiao, L. Zhang, K. H. L. Shutthanandan, V. Ciston, J. Kabius, B. Chambers, S. A. TI Cation intermixing and electronic deviations at the insulating LaCrO3/SrTiO3(001) interface SO PHYSICAL REVIEW B LA English DT Article ID ENERGY-LOSS SPECTROSCOPY; OXIDE INTERFACES; STOICHIOMETRY; CHROMIUM; SRTIO3; GROWTH; CHARGE; TEM AB The interface between polar perovskite LaCrO3 and nonpolar SrTiO3(001) grown by molecular beam epitaxy is examined using a combination of electron microscopy, spectroscopy, and Rutherford backscattering spectrometry. The A-site cations of these ABO(3) perovskites are found to diffuse across the interface to a greater extent than the B-site cations, based on high-angle annular dark-field scanning transmission electron microscopy, energy-dispersive x-ray spectroscopy, and electron-energy-loss spectroscopy (EELS). The B-site cation valences are shown to be partially reduced near the interface by analysis of EELS near-edge structures. The location and direction of these electronic modifications do not intuitively compensate the charge imbalance imposed by uneven cation interdiffusion, and yet both the film and interface are insulating. These results highlight the importance of considering both the physical and electronic structure of such complex interfaces in determining their characteristics. C1 [Colby, R.; Shutthanandan, V.; Kabius, B.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Qiao, L.; Zhang, K. H. L.; Chambers, S. A.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Ciston, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. RP Colby, R (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RI Qiao, Liang/A-8165-2012; Zhang, Kelvin/F-5434-2014; Foundry, Molecular/G-9968-2014 FU US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [10122 (MBE and RBS)]; Department of Energy's Office of Biological and Environmental Research at Pacific Northwest National Laboratory; National Center for Electron Microscopy, Lawrence Berkeley National Laboratory; DOE BES [DE-AC02-05CH11231]; EMSL William Wiley Postdoctoral Fellowship program FX Thanks are extended to T. Droubay for useful discussions. This work was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award No. 10122 (MBE and RBS), and the EMSL William Wiley Postdoctoral Fellowship program. The work was performed in the Environmental Molecular Sciences Laboratory, a national science user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. The authors also acknowledge support of the National Center for Electron Microscopy, Lawrence Berkeley National Laboratory, which is supported by the DOE BES under Contract No. DE-AC02-05CH11231. NR 42 TC 9 Z9 9 U1 8 U2 47 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 29 PY 2013 VL 88 IS 15 AR UNSP 155325 DI 10.1103/PhysRevB.88.155325 PG 9 WC Physics, Condensed Matter SC Physics GA 242VN UT WOS:000326272000003 ER PT J AU de la Figuera, J Novotny, Z Setvin, M Liu, TJ Mao, ZQ Chen, G N'Diaye, AT Schmid, M Diebold, U Schmid, AK Parkinson, GS AF de la Figuera, Juan Novotny, Zbynek Setvin, Martin Liu, Tijiang Mao, Zhiqiang Chen, Gong N'Diaye, Alpha T. Schmid, Michael Diebold, Ulrike Schmid, Andreas K. Parkinson, Gareth S. TI Real-space imaging of the Verwey transition at the (100) surface of magnetite SO PHYSICAL REVIEW B LA English DT Article ID ENERGY-ELECTRON MICROSCOPY; LOW-TEMPERATURE PHASE; FE3O4; POLARIZATION; PERSPECTIVE AB Effects of the Verwey transition on the (100) surface of magnetite were studied using scanning tunneling microscopy and spin polarized low-energy electron microscopy. On cooling through the transition temperature TV, the initially flat surface undergoes a rooflike distortion with a periodicity of similar to 0.5 mu m due to ferroelastic twinning within monoclinic domains of the low-temperature monoclinic structure. The monoclinic c axis orients in the surface plane, along the [001](c) directions. At the atomic scale, the charge-ordered (root 2 x root 2)R45 degrees reconstruction of the (100) surface is unperturbed by the bulk transition, and is continuous over the twin boundaries. Time resolved low-energy electron microscopy movies reveal the structural transition to be first order at the surface, indicating that the bulk transition is not an extension of the Verwey-like (root 2 x root 2)R45 degrees reconstruction. Although conceptually similar, the charge-ordered phases of the (100) surface and sub-T-V bulk of magnetite are unrelated phenomena. C1 [de la Figuera, Juan] CSIC, Inst Quim Fis Rocasolano, Madrid 28006, Spain. [Novotny, Zbynek; Setvin, Martin; Schmid, Michael; Diebold, Ulrike; Parkinson, Gareth S.] Vienna Univ Technol, Inst Appl Phys, A-1040 Vienna, Austria. [Liu, Tijiang; Mao, Zhiqiang] Tulane Univ, New Orleans, LA 70119 USA. [Chen, Gong; N'Diaye, Alpha T.; Schmid, Andreas K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP de la Figuera, J (reprint author), CSIC, Inst Quim Fis Rocasolano, Madrid 28006, Spain. EM juan.delafiguera@iqfr.csic.es RI Setvin, Martin/G-5629-2014; de la Figuera, Juan/E-7046-2010; Diebold, Ulrike/A-3681-2010; Chen, Gong/H-3074-2015; Foundry, Molecular/G-9968-2014; Setvin, Martin/G-4879-2016; OI Setvin, Martin/0000-0001-8636-921X; de la Figuera, Juan/0000-0002-7014-4777; Diebold, Ulrike/0000-0003-0319-5256; Setvin, Martin/0000-0002-1210-7740; Schmid, Michael/0000-0003-3373-9357; Parkinson, Gareth/0000-0003-2457-8977 FU Spanish Government [MAT2009-14578-C03-01, MAT2012-38045-C04-01]; Office of Basic Energy Sciences, Division of Materials and Engineering Sciences, US Department of Energy [AC0205CH11231]; Centre for Atomic-Level Catalyst Design, an Energy Frontier Research Centre; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001058]; NSF [DMR-1205469]; Austrian Science Fund [P24925-N20] FX This research was supported by the Spanish Government through Projects No. MAT2009-14578-C03-01 and No. MAT2012-38045-C04-01, by the Office of Basic Energy Sciences, Division of Materials and Engineering Sciences, US Department of Energy under Contract No. AC0205CH11231, and by the Centre for Atomic-Level Catalyst Design, an Energy Frontier Research Centre funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001058. The work at Tulane is supported by the NSF under Grant No. DMR-1205469. G.S.P. acknowledges support from the Austrian Science Fund Project No. P24925-N20. NR 40 TC 9 Z9 9 U1 2 U2 38 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 29 PY 2013 VL 88 IS 16 AR 161410 DI 10.1103/PhysRevB.88.161410 PG 5 WC Physics, Condensed Matter SC Physics GA 242VQ UT WOS:000326272400004 ER PT J AU Kadau, K Cherne, FJ Ravelo, R Germann, TC AF Kadau, Kai Cherne, Frank J. Ravelo, Ramon Germann, Timothy C. TI Shock-induced phase transformations in gallium single crystals by atomistic methods SO PHYSICAL REVIEW B LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; EMBEDDED-ATOM METHOD; TRANSITIONS; IMPURITIES; POTENTIALS; SURFACES; HUGONIOT; METALS; NICKEL; WAVES AB Utilizing a modified embedded atom method potential, we performed large-scale classical molecular dynamics simulations (with up to 50 million atoms) to investigate the response of Ga single crystals to shock compression along the three major orientations of the orthorhombic A11 ground state, i. e., [001], [010], and [100]. For weak shocks with particle velocity u(p) < 300 m/s, these defect-free single crystals respond elastically, but for stronger shocks, they undergo a structural phase transformation and then (for even stronger shocks) melt. For intermediate shock strengths (300 m/s < u(p) < 1.2 km/s) a split shock wave is formed, with an elastic precursor (uniaxial compression wave) leading the slower transformation wave. The transformed region consists of a mixed phase, with stripes of the product phase embedded into the uniaxially compressed parent phase, with the ratio of product to parent phase increasing with increasing shock strength, much like in martensitic phase transformations. Upon shock release from the free surface at the end of the sample, the transformation is reversed, leaving only some defects behind, which makes it difficult to experimentally investigate the structural transformation in shock-recovered samples. We investigated the structure produced by the shock and found it to be similar to the beta phase of Ga which is obtained by supercooling from the liquid state. However, the product phase shows only half the period along [100] in the calculated diffraction pattern. Further investigation showed that this is due to a different stacking sequence in this direction, namely ABCD instead of AB for the beta phase. C1 [Kadau, Kai; Germann, Timothy C.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Cherne, Frank J.] Los Alamos Natl Lab, Weapons Expt Div, Los Alamos, NM 87545 USA. [Ravelo, Ramon] Univ Texas El Paso, Dept Phys, El Paso, TX 79968 USA. RP Kadau, K (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM kadaukai@yahoo.com; cherne@lanl.gov; rravelo@utep.edu; tcg@lanl.gov OI Germann, Timothy/0000-0002-6813-238X; Cherne, Frank/0000-0002-8589-6058 FU National Nuclear Security Administration; U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; Advanced Simulation and Computing (ASC) program FX We would like to thank Brad Lee Holian (Los Alamos) for many interesting discussions. This work was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under contract No. DE-AC52-06NA25396, with funding by the Advanced Simulation and Computing (ASC) program. NR 42 TC 7 Z9 7 U1 4 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD OCT 29 PY 2013 VL 88 IS 14 AR 144108 DI 10.1103/PhysRevB.88.144108 PG 10 WC Physics, Condensed Matter SC Physics GA 242VL UT WOS:000326271700002 ER PT J AU Kawano-Furukawa, H DeBeer-Schmitt, L Kikuchi, H Cameron, AS Holmes, AT Heslop, RW Forgan, EM White, JS Kihou, K Lee, CH Iyo, A Eisaki, H Saito, T Fukazawa, H Kohori, Y Gavilano, JL AF Kawano-Furukawa, H. DeBeer-Schmitt, Lisa Kikuchi, H. Cameron, A. S. Holmes, A. T. Heslop, R. W. Forgan, E. M. White, J. S. Kihou, K. Lee, C. H. Iyo, A. Eisaki, H. Saito, T. Fukazawa, H. Kohori, Y. Gavilano, J. L. TI Probing the anisotropic vortex lattice in the Fe-based superconductor KFe2As2 using small-angle neutron scattering SO PHYSICAL REVIEW B LA English DT Article AB Using small angle neutron scattering, the anisotropy of the magnetic vortex lattice (VL), in the heavily hole-doped pnictide superconductor KFe2As2, was studied. Well-ordered VL scattering patterns were measured with fields applied in directions between B parallel to c and the basal plane, rotating either towards [100] or [110]. Slightly distorted hexagonal patterns were observed when B parallel to c. However, the scattering pattern distorted more strongly as the field was rotated away from the c axis. At low field, the arrangement of vortices is affected by the anisotropy of penetration depth in the plane perpendicular to the field. By fitting the distortion with the anisotropic London model, we obtain an estimate of similar to 3.4 for the anisotropy factor gamma between the in-plane and c-axis penetration depths at the lowest temperature studied. The results further reveal VL phase transitions as a function of field direction. We discuss these transitions using the "hairy ball" theorem. C1 [Kawano-Furukawa, H.] Ochanomizu Univ, GSHS, Dept Phys, Tokyo 112, Japan. [DeBeer-Schmitt, Lisa] Oak Ridge Natl Lab, Instrument Source Div, Oak Ridge, TN USA. [Kikuchi, H.] Ochanomizu Univ, Dept Phys, Tokyo, Japan. [Cameron, A. S.; Holmes, A. T.; Heslop, R. W.; Forgan, E. M.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [White, J. S.; Gavilano, J. L.] PSI, Neutron Scattering Lab, CH-5232 Villigen, Switzerland. [White, J. S.] Ecole Polytech Fed Lausanne, Lab Quantum Magnetism, CH-1015 Lausanne, Switzerland. [Kihou, K.; Lee, C. H.; Iyo, A.; Eisaki, H.] AIST, Tsukuba, Ibaraki, Japan. [Kihou, K.; Lee, C. H.; Iyo, A.; Eisaki, H.; Fukazawa, H.; Kohori, Y.] TRIP, JST, Chiyoda, Tokyo, Japan. [Saito, T.; Fukazawa, H.; Kohori, Y.] Chiba Univ, Dept Phys, Chiba, Japan. RP Kawano-Furukawa, H (reprint author), Ochanomizu Univ, GSHS, Dept Phys, Tokyo 112, Japan. EM furukawa.hazuki@ocha.ac.jp RI White, Jonathan/G-2742-2010; DeBeer-Schmitt, Lisa/I-3313-2015; Holmes, Alexander/B-5485-2013; Kawano-Furukawa, Hazuki/M-7646-2016; Kawano-Furukawa, Hazuki/M-7695-2016 OI White, Jonathan/0000-0001-7738-0150; DeBeer-Schmitt, Lisa/0000-0001-9679-3444; Holmes, Alexander/0000-0002-3069-3069; Kawano-Furukawa, Hazuki/0000-0003-4713-3727; Kawano-Furukawa, Hazuki/0000-0003-4713-3727 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; EPSRC; MaNEP; European Commission; Ministry of Education, Culture, Sports, Science, and Technology, Japan [20102006]; Mitsubishi Foundation; US-Japan Cooperative Program on Neutron Scattering; JSPS Institutional Program for Young Researcher Overseas Visits at Ochanomizu University FX We thank M. Zolliker for invaluable assistance in setting up the dilution refrigerator at PSI, and M. Laver for discussions about the application of the HB theorem to KFe2As2. We acknowledge financial support for the part of the research conducted at ORNL's High Flux Isotope Reactor, which was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy, also the EPSRC, MaNEP and the European Commission under the 6th Framework Programme. This work was partially supported by a Grant-in-Aid for Scientific Research on Innovative Areas "Heavy Electrons" (No. 20102006) of The Ministry of Education, Culture, Sports, Science, and Technology, Japan and the Mitsubishi Foundation. The experiment using the CG2 SANS spectrometer at Oak Ridge National Laboratory was supported by the US-Japan Cooperative Program on Neutron Scattering. H. K. was supported by the JSPS Institutional Program for Young Researcher Overseas Visits at Ochanomizu University. NR 33 TC 2 Z9 2 U1 0 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 29 PY 2013 VL 88 IS 13 AR 134524 DI 10.1103/PhysRevB.88.134524 PG 8 WC Physics, Condensed Matter SC Physics GA 242VK UT WOS:000326271500003 ER PT J AU Li, Q Cao, GX Okamoto, S Yi, JY Lin, WZ Sales, BC Yan, JQ Arita, R Kunes, J Kozhevnikov, AV Eguiluz, AG Imada, M Gai, Z Pan, MH Mandrus, DG AF Li, Qing Cao, Guixin Okamoto, Satoshi Yi, Jieyu Lin, Wenzhi Sales, Brian C. Yan, Jiaqiang Arita, Ryotaro Kunes, Jan Kozhevnikov, Anton V. Eguiluz, Adolfo G. Imada, Masatoshi Gai, Zheng Pan, Minghu Mandrus, David G. TI Atomically resolved spectroscopic study of Sr2IrO4: Experiment and theory SO SCIENTIFIC REPORTS LA English DT Article ID AUGMENTED-WAVE METHOD; TUNNELING SPECTROSCOPY; SUPERCONDUCTORS; FERROMAGNETISM; TRANSITION; DENSITY; SURFACE AB Particularly in Sr2IrO4, the interplay between spin-orbit coupling, bandwidth and on-site Coulomb repulsion stabilizes a J(eff) = 1/2 spin-orbital entangled insulating state at low temperatures. Whether this insulating phase is Mott- or Slater-type, has been under intense debate. We address this issue via spatially resolved imaging and spectroscopic studies of the Sr2IrO4 surface using scanning tunneling microscopy/spectroscopy (STM/S). STS results clearly illustrate the opening of an insulating gap (150 similar to 250 meV) below the Neel temperature (T-N), in qualitative agreement with our density-functional theory (DFT) calculations. More importantly, the temperature dependence of the gap is qualitatively consistent with our DFT 1 dynamical mean field theory (DMFT) results, both showing a continuous transition from a gapped insulating ground state to a non-gap phase as temperatures approach TN. These results indicate a significant Slater character of gap formation, thus suggesting that Sr2IrO4 is a uniquely correlated system, where Slater and Mott-Hubbard-type behaviors coexist. C1 [Li, Qing; Lin, Wenzhi; Gai, Zheng; Pan, Minghu] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Cao, Guixin; Yi, Jieyu; Yan, Jiaqiang; Mandrus, David G.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Cao, Guixin; Okamoto, Satoshi; Yi, Jieyu; Sales, Brian C.; Yan, Jiaqiang; Mandrus, David G.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Arita, Ryotaro; Imada, Masatoshi] Univ Tokyo, Dept Appl Phys, Bunkyo Ku, Tokyo 1138656, Japan. [Arita, Ryotaro; Imada, Masatoshi] JST CREST, Bunkyo Ku, Tokyo 1138656, Japan. [Kunes, Jan] Acad Sci Czech Republic, Inst Phys, Prague 16253 6, Czech Republic. [Kozhevnikov, Anton V.] ETH, Inst Theoret Phys, CH-8093 Zurich, Switzerland. [Eguiluz, Adolfo G.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Li, Qing] Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Suzhou 215123, Jiangsu, Peoples R China. RP Pan, MH (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM panm@ornl.gov; dmandrus@utk.edu RI Okamoto, Satoshi/G-5390-2011; Kunes, Jan/B-4484-2008; Arita, Ryotaro/D-5965-2012; Gai, Zheng/B-5327-2012; Mandrus, David/H-3090-2014; Cao, Guixin/G-4452-2015 OI Okamoto, Satoshi/0000-0002-0493-7568; Kunes, Jan/0000-0001-9682-7640; Arita, Ryotaro/0000-0001-5725-072X; Gai, Zheng/0000-0002-6099-4559; Cao, Guixin/0000-0002-9252-1158 FU U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; MEXT Japan; MEXT; Computational Materials Science Initiative (CMSI), Japan; Grant Agency of the Czech Republic [13-25251S]; ASCR; BES of the U.S. DOE; NSF [OCI-0904972] FX This research was conducted (MP, QL, ZG) at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Research was supported (GXC, SO, WL, JYY, BCS, JQY, DGM) by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. RA and MI were supported by MEXT Japan and Strategic Programs for Innovative Research (SPIRE), MEXT, and the Computational Materials Science Initiative (CMSI), Japan. JK was supported by the Grant No. 13-25251S of the Grant Agency of the Czech Republic. AVK acknowledges the computational resources of the CSCS and of the NCCS and the CNMS at ORNL, which are sponsored by the respective facilities divisions of the offices of ASCR and BES of the U.S. DOE. AGE was supported by NSF Grant No. OCI-0904972. NR 48 TC 24 Z9 24 U1 5 U2 88 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 29 PY 2013 VL 3 AR 3073 DI 10.1038/srep03073 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 243QF UT WOS:000326331200001 PM 24166292 ER PT J AU Petzold, CJ Schwarz, RI AF Petzold, Christopher J. Schwarz, Richard I. TI Cells determine cell density using a small protein bound to a unique tissue-specific phospholipid SO PEERJ LA English DT Article DE Cell density signaling; Tendon morphogenesis; Bone morphogenesis; Membrane signaling; Growth plate formation AB Cell density is the critical parameter controlling tendon morphogenesis. Knowing its neighbors allows a cell to regulate correctly its proliferation and collagen production. A missing link to understanding this process is a molecular description of the sensing mechanism. Previously, this mechanism was shown in cell culture to rely on a diffusible factor (SNZR [sensor]) with an affinity for the cell layer. This led to purifying conditioned medium over 4 columns and analyzing the final column fractions for band intensity on SDS gels versus biological activity - a 16 kD band strongly correlated between assays. N-terminal sequencing - EPLAVVDL - identified a large gene (424 AA), extremely conserved between chicken and human. In this paper we probe whether this is the correct gene. Can the predicted large protein be cleaved to a smaller protein? EPLAVVDL occurs towards the C-terminus and cleavage would create a small 94 AA protein. This protein would run at similar to 10 kD, so what modifications or cofactor binding accounts for its running at 16 kD on SDS gels? This protein has no prominent hydrophobic regions, so can it be secreted? To validate its role, the chicken cDNA for this gene was tagged with myc and his and transfected into a human osteosarcoma cell line (U2OS). U2OS cells expressed the gene but not passively: differentiating into structures resembling spongy bone and expressing alkaline phosphatase, an early bone marker. Intracellularly, two bands were observed byWestern blotting: the full length protein and a smaller form (26 kD). Outside the cell, a small band (28 kD) was detected, although it was 40% larger than expected, as well asmultiple larger bands. These larger forms could be converted to the predicted smaller protein (94 AA C tags) by changing salt concentrations and ultrafiltering - releasing a cofactor to the filtrate while leaving a protein factor in the retentate. Using specific degradative enzymes and mass spectrometry, the bone cofactor was identified as a lipid containing a ceramide phosphate, a single chained glycerol lipid and a linker. Tendon uses a different cofactor made up of two fatty acid chains linked directly to the phosphate yielding a molecule about half the size. Moreover, adding the tendon factor/cofactor to osteosarcoma cells causes themto stop growing, which is opposite to its role with tendon cells. Thus, the cofactor is cell type specific both in composition and in the triggered response. Further support of its proposed role came from frozen sections from 5 week old mice where an antibody to the factor stained strongly at the growing ends of the tendon as predicted. In conclusion, the molecule needed for cell density signaling is a small protein bound to a unique, tissue-specific phospholipid yielding a membrane associated but diffusible molecule. Signal transduction is postulated to occur by an increased ordering of the plasma membrane as the concentration of this protein/lipid increases with cell density. C1 [Petzold, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Berkeley, CA 94720 USA. [Schwarz, Richard I.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Schwarz, RI (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. EM rischwarz@lbl.gov FU CRADA [BG92-106]; N.I.H. [R37CA064786]; Breast Cancer Research Foundation FX This work was supported in part by a CRADA BG92-106, N.I.H. grant R37CA064786, and a grant from The Breast Cancer Research Foundation. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 32 TC 0 Z9 0 U1 1 U2 1 PU PEERJ INC PI LONDON PA 341-345 OLD ST, THIRD FLR, LONDON, EC1V 9LL, ENGLAND SN 2167-8359 J9 PEERJ JI PeerJ PD OCT 29 PY 2013 VL 1 AR e192 DI 10.7717/peerj.192 PG 35 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA V36CL UT WOS:000209190900003 PM 24244914 ER PT J AU Seagle, CT Cottrell, E Fei, YW Hummer, DR Prakapenka, VB AF Seagle, Christopher T. Cottrell, Elizabeth Fei, Yingwei Hummer, Daniel R. Prakapenka, Vitali B. TI Electrical and thermal transport properties of iron and iron-silicon alloy at high pressure SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID DIAMOND-ANVIL CELL; CORE CONDITIONS; EARTHS CORE; RESISTIVITY; CONDUCTIVITY; TRANSITION; NICKEL; GPA; COMPRESSION; RESISTANCE AB The efficiency of heat transfer by conduction in the Earth's core controls the dynamics of convection and limits the power available for the geodynamo. We have measured the room temperature electrical resistivity of iron and iron-silicon alloy to 60 GPa and present a new model of the resistivity at high pressures and temperatures relevant to the Earth's core. The model is compared with available shock wave data and theoretical studies. For a power law and linear temperature dependence of electrical resistivity, the calculated thermal conductivity at the core-mantle boundary is similar to 67-145W/m/K for pure Fe and similar to 41-60 W/m/K for Fe-9wt % Si. Impurities in the core have a strong effect on the transport properties of iron that could significantly impact core thermal models. The models describing the data indicate higher thermal conductivity at core pressure than previously suggested, requiring additional energy sources in the past to operate the geodynamo. C1 [Seagle, Christopher T.; Cottrell, Elizabeth] Smithsonian Inst, Natl Museum Nat Hist, Washington, DC 20560 USA. [Seagle, Christopher T.; Fei, Yingwei; Hummer, Daniel R.] Carnegie Inst Sci, Geophys Lab, Washington, DC USA. [Prakapenka, Vitali B.] Univ Chicago, Ctr Adv Radiat Sources, Chicago, IL 60637 USA. RP Seagle, CT (reprint author), Sandia Natl Labs, POB 5800,MS 1189, Albuquerque, NM 87185 USA. EM ctseagl@sandia.gov RI Fei, Yingwei/F-3709-2011 OI Fei, Yingwei/0000-0001-9955-5353 FU National Science Foundation (Earth Sciences) [EAR-0622171]; Department of Energy (Geosciences) [DE-FG02-94ER14466]; State of Illinois; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; NSF [EAR-0738654, EAR-0738741] FX Portions of this work were performed at GeoSoilEnviroCARS (Sector 13), Advanced Photon Source (APS), Argonne National Laboratory. GeoSoilEnviroCARS is supported by the National Science Foundation (Earth Sciences) under grant EAR-0622171, the Department of Energy (Geosciences) under grant DE-FG02-94ER14466, and the State of Illinois. Use of the APS was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract DE-AC02-06CH11357. This research was supported by NSF grant EAR-0738654 to E.C. and NSF grant EAR-0738741 to Y.F. NR 35 TC 20 Z9 21 U1 2 U2 32 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD OCT 28 PY 2013 VL 40 IS 20 BP 5377 EP 5381 DI 10.1002/2013GL057930 PG 5 WC Geosciences, Multidisciplinary SC Geology GA 301DY UT WOS:000330514200009 ER PT J AU Weijer, W Zharkov, V Nof, D Dijkstra, HA de Ruijter, WPM van Scheltinga, AT Wubs, F AF Weijer, Wilbert Zharkov, Volodymyr Nof, Doron Dijkstra, Henk A. de Ruijter, Wilhelmus P. M. van Scheltinga, Arjen Terwisscha Wubs, Fred TI Agulhas ring formation as a barotropic instability of the retroflection SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID ATLANTIC OVERTURNING CIRCULATION; SEPARATING MEANDERING CURRENTS; FULLY-IMPLICIT MODEL; OCEAN CIRCULATION; STEADINESS; DYNAMICS; VARIABILITY; EXCHANGE; SYSTEMS; PHYSICS AB Agulhas Leakage is an important link in the global ocean circulation, as it transfers a significant volume of relatively warm and salty water from the Indian Ocean to the Atlantic Ocean. The main route of this transfer is through the shedding of large Agulhas rings from the Agulhas retroflection. In this paper we study the dynamics of the ring formation process by analyzing the stability of the Indian/Atlantic supergyre in a reduced gravity model. We show that the ring-shedding process results from a barotropic instability of the steady circulation in the Agulhas retroflection region. The destabilizing mode appears to be linked to a Rossby basin mode of the combined South Indian/Atlantic basin, which is localized in the retroflection region by the background flow. C1 [Weijer, Wilbert] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Zharkov, Volodymyr] Ctr Ocean Atmospher Predict Studies, Tallahassee, FL USA. [Nof, Doron] Florida State Univ, Tallahassee, FL 32306 USA. [Dijkstra, Henk A.; de Ruijter, Wilhelmus P. M.] Inst Marine & Atmospher Res Utrecht, Utrecht, Netherlands. [van Scheltinga, Arjen Terwisscha] Univ Bristol, Bristol, Avon, England. [Wubs, Fred] Univ Groningen, Groningen, Netherlands. RP Weijer, W (reprint author), Los Alamos Natl Lab, CCS-2,MS B214, Los Alamos, NM 87545 USA. EM wilbert@lanl.gov RI Weijer, Wilbert/A-7909-2010; Dijkstra , Henk /H-2559-2016; de Ruijter, Wilhelmus/I-2541-2016 FU Institute for Geophysics and Planetary Physics at the Los Alamos National Laboratory; Regional and Global Climate Modeling Program of the U.S. Department of Energy Office of Science; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; COMPLEXITY project PreKurs; Netherlands Organization for Scientific Research FX This research was supported by the Institute for Geophysics and Planetary Physics at the Los Alamos National Laboratory and the Regional and Global Climate Modeling Program of the U.S. Department of Energy Office of Science. Los Alamos National Laboratory is operated by the Los Alamos National Security, LLC for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. H.D. acknowledges support from the COMPLEXITY project PreKurs, which was funded by the Netherlands Organization for Scientific Research. We thank Joe LaCasce and an anonymous reviewer for their constructive comments. NR 30 TC 3 Z9 3 U1 0 U2 1 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD OCT 28 PY 2013 VL 40 IS 20 BP 5435 EP 5438 DI 10.1002/2013GL057751 PG 4 WC Geosciences, Multidisciplinary SC Geology GA 301DY UT WOS:000330514200019 ER PT J AU Tang, Q Hess, PG Brown-Steiner, B Kinnison, DE AF Tang, Qi Hess, Peter G. Brown-Steiner, Benjamin Kinnison, Douglas E. TI Tropospheric ozone decrease due to the Mount Pinatubo eruption: Reduced stratospheric influx SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID HETEROGENEOUS CHEMISTRY; TROPICAL OZONE; MT-PINATUBO; AEROSOL; TRENDS; MODEL; MIDLATITUDES; VARIABILITY; CIRCULATION; IMPACT AB We quantify the relationship between Mount Pinatubo eruption in June 1991 and tropospheric ozone abundances. The ozone reduction in the stratosphere and troposphere following the eruption is simulated by the Whole Atmosphere Community Climate Model and is in good agreement with the ozonesonde observations. Simulated anomalies in the global stratosphere-troposphere flux of ozone following the eruption are well correlated with those in the tropospheric ozone column. Both are at their minimum in late 1992 to early 1993 (-70 Tg yr(-1) in January 1993 for the flux and -1.9 Dobson Unit in November 1992 for tropospheric ozone) and recover after 1995. Therefore, this study identifies the reduced stratosphere-to-troposphere ozone flux as an important driver of the ozone decline in the troposphere following the eruption. A large fraction (67%) of the decrease in the flux is compensated by an increase in tropospheric photochemical ozone production. While both the strength of the residual circulation and the decrease in stratospheric ozone reduce the stratospheric ozone flux, the ozone reduction is identified as the dominant cause. C1 [Tang, Qi; Hess, Peter G.; Brown-Steiner, Benjamin] Cornell Univ, Dept Biol & Environm Engn, Ithaca, NY 14853 USA. [Tang, Qi] Lawrence Livermore Natl Lab, Livermore, CA USA. [Kinnison, Douglas E.] Natl Ctr Atmospher Res, Div Atmospher Chem, Boulder, CO 80307 USA. RP Tang, Q (reprint author), Cornell Univ, Dept Biol & Environm Engn, Ithaca, NY 14853 USA. EM tang30@llnl.gov RI Tang, Qi/C-1032-2011; Hess, Peter/M-3145-2015 OI Hess, Peter/0000-0003-2439-3796 FU NSF [AGS-1042787]; National Science Foundation; U.S. Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Atmospheric Radiation Measurement Program of the Office of Science at the U.S. Department of Energy FX We acknowledge anonymous reviewers and the science team producing the World Ozone and Ultraviolet Radiation Data Centre (WOUDC) ozonesonde data. This work is funded by NSF grant (AGS-1042787) to Cornell University. The National Center for Atmospheric Research is operated by the University Corporation for Atmospheric Research under sponsorship of the National Science Foundation. Work at LLNL was performed under the auspices of the U.S. Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344 and supported by the Atmospheric Radiation Measurement Program of the Office of Science at the U.S. Department of Energy. NR 25 TC 4 Z9 4 U1 1 U2 14 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD OCT 28 PY 2013 VL 40 IS 20 BP 5553 EP 5558 DI 10.1002/2013GL056563 PG 6 WC Geosciences, Multidisciplinary SC Geology GA 301DY UT WOS:000330514200040 ER PT J AU Fu, DY Zhou, J Tongay, S Liu, K Fan, W Liu, TJK Wu, JQ AF Fu, Deyi Zhou, Jian Tongay, Sefaattin Liu, Kai Fan, Wen Liu, Tsu-Jae King Wu, Junqiao TI Mechanically modulated tunneling resistance in monolayer MoS2 SO APPLIED PHYSICS LETTERS LA English DT Article ID SURFACE AB We report on the modulation of tunneling resistance in MoS2 monolayers using a conductive atomic force microscope (AFM). The resistance between the conductive AFM probe and the bottom electrode separated by a monolayer MoS2 is reversibly reduced by up to 4 orders of magnitude, which is attributed to enhanced quantum tunneling when the monolayer is compressed by the tip force. Under the Wentzel-Kramers-Brillouim approximation, the experimental data are quantitatively explained by using the metal-insulator-metal tunneling diode model. As an ideal tunneling medium, the defect-free, nanometer-thick MoS2 monolayer can serve as the active layer for non-impacting nano-electro-mechanical switches. (C) 2013 AIP Publishing LLC. C1 [Fu, Deyi; Zhou, Jian; Tongay, Sefaattin; Liu, Kai; Fan, Wen; Wu, Junqiao] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Liu, Kai; Wu, Junqiao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Liu, Tsu-Jae King] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. RP Fu, DY (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM wuj@berkeley.edu RI Liu, Kai/A-4754-2012; Wu, Junqiao/G-7840-2011; Fu, Deyi/C-6624-2011 OI Liu, Kai/0000-0002-0638-5189; Wu, Junqiao/0000-0002-1498-0148; Fu, Deyi/0000-0003-1365-8963 FU NSF Center for Energy Efficient Electronics Science (NSF) [ECCS-0939514] FX This work was supported by the NSF Center for Energy Efficient Electronics Science (NSF Award No. ECCS-0939514). We are grateful to Professor Eli Yablonovitch for helpful discussions. NR 18 TC 15 Z9 15 U1 1 U2 36 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 28 PY 2013 VL 103 IS 18 AR 183105 DI 10.1063/1.4827301 PG 3 WC Physics, Applied SC Physics GA 263NT UT WOS:000327816000040 ER PT J AU Liu, S Mahony, TS Bender, DA Sinclair, MB Brener, I AF Liu, Sheng Mahony, Thomas S. Bender, Daniel A. Sinclair, Michael B. Brener, Igal TI Mid-infrared time-domain spectroscopy system with carrier-envelope phase stabilization SO APPLIED PHYSICS LETTERS LA English DT Article ID FIELD-RESOLVED DETECTION; QUANTUM CASCADE LASER; REPETITION-RATE; FEMTOSECOND PULSES; GENERATION; GASE; METAMATERIAL; TRANSIENTS; THZ AB We built a mid-infrared time-domain spectroscopy (TDS) system optimized for the 8-12 mu m spectral range based on a compact ultrafast Erbium: fiber laser that enables measurements of phase-resolved optical field transients directly in the time domain with high stability and spectral brightness. We achieved long term (>10 h) stability of the TDS signal by using a carrier-envelope-phase locking technique to reduce the timing jitter caused by environmental changes. Time domain measurements of the mid-infrared beam were achieved via electro-optic sampling in a GaSe crystal, using an ultrashort (similar to 15 fs) output of the fiber laser. Here, we present a full characterization of our TDS system including the dependence of the amplitude and pulse shape of the detected infrared waveforms on the thickness of the GaSe crystals. (C) 2013 AIP Publishing LLC. C1 [Liu, Sheng; Mahony, Thomas S.; Bender, Daniel A.; Sinclair, Michael B.; Brener, Igal] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Liu, Sheng; Mahony, Thomas S.; Brener, Igal] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. RP Liu, S (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM snliu@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors thank R. Huber and A. Leitenstorfer for their help through useful discussions and initial training. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U. S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 25 TC 6 Z9 6 U1 5 U2 27 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 28 PY 2013 VL 103 IS 18 AR 181111 DI 10.1063/1.4827885 PG 5 WC Physics, Applied SC Physics GA 263NT UT WOS:000327816000076 ER PT J AU Roberts, AT Mohanta, A Everitt, HO Leach, JH Van den Broeck, D Hosalli, AM Paskova, T Bedair, SM AF Roberts, A. T. Mohanta, A. Everitt, H. O. Leach, J. H. Van den Broeck, D. Hosalli, A. M. Paskova, T. Bedair, S. M. TI Spectroscopic investigation of coupling among asymmetric InGaN/GaN multiple quantum wells grown on non-polar a-plane GaN substrates SO APPLIED PHYSICS LETTERS LA English DT Article ID LIGHT-EMITTING-DIODES; EMISSION; NITRIDE; EXCITONS AB Low defect density asymmetric multiple quantum wells (MQWs) of InGaN/GaN grown on non-polar a-plane GaN substrates were investigated using time-integrated and time-resolved photoluminescence spectroscopy. Comparison of these spectra with the predicted emission energies reveals that these QWs may be spectrally resolved at low temperatures. However, a combination of thermal activation and resonant tunneling of carriers increasingly coupled the QWs, favoring emission from the lowest energy QWs with increasing temperature in a manner analogous to MQWs composed of other non-polar semiconductor materials but unlike most InGaN MQWs grown on polar substrates and influenced by the strong polarization-dependent effects. (C) 2013 AIP Publishing LLC. C1 [Roberts, A. T.; Everitt, H. O.] US Army, Aviat & Missile Res Dev & Engn Ctr, Redstone Arsenal, AL 35898 USA. [Mohanta, A.] US Army, Aviat & Missile Res Dev & Engn Ctr, Oak Ridge Inst Sci & Educ, Res Participat Program, Redstone Arsenal, AL 35898 USA. [Everitt, H. O.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Leach, J. H.] Kyma Technol, Raleigh, NC 27617 USA. [Van den Broeck, D.; Hosalli, A. M.; Paskova, T.; Bedair, S. M.] N Carolina State Univ, Dept Elect & Comp Engn, Raleigh, NC 27695 USA. RP Paskova, T (reprint author), N Carolina State Univ, Dept Elect & Comp Engn, Raleigh, NC 27695 USA. EM tmpaskov@ncsu.edu RI Everitt, Henry/L-7118-2013 OI Everitt, Henry/0000-0002-8141-3768 FU National Science Foundation [DMR-1105842, DMR-1207075] FX This research was supported in part by appointment of A.M. to the Postgraduate Research Participation Program at the U.S. Army Aviation and Missile Research, Development and Engineering Center administered by the Oak Ridge Institute for Science and Education through an interagency agreement with the U.S. Department of Energy, as well as by National Science Foundation (Nos. DMR-1105842 and DMR-1207075). NR 26 TC 2 Z9 2 U1 1 U2 29 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 28 PY 2013 VL 103 IS 18 AR 181106 DI 10.1063/1.4827536 PG 4 WC Physics, Applied SC Physics GA 263NT UT WOS:000327816000049 ER PT J AU Luppi, E Head-Gordon, M AF Luppi, Eleonora Head-Gordon, Martin TI The role of Rydberg and continuum levels in computing high harmonic generation spectra of the hydrogen atom using time-dependent configuration interaction SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID CORRELATED MOLECULAR CALCULATIONS; ELECTRONIC OPTICAL-RESPONSE; DENSITY-FUNCTIONAL THEORY; GAUSSIAN-BASIS SETS; TD-CI SIMULATION; ULTRAFAST SCIENCE; LASER FIELDS; EOM-CCSD; ATTOSECOND; STATES AB We study the role of Rydberg bound-states and continuum levels in the field-induced electronic dynamics associated with the High-Harmonic Generation (HHG) spectroscopy of the hydrogen atom. Time-dependent configuration-interaction (TD-CI) is used with very large atomic orbital (AO) expansions (up to L = 4 with sextuple augmentation and off-center functions) to describe the bound Rydberg levels, and some continuum levels. To address the lack of ionization losses in TD-CI with finite AO basis sets, we employed a heuristic lifetime for energy levels above the ionization potential. The heuristic lifetime model is compared against the conventional atomic orbital treatment (infinite lifetimes), and a third approximation which is TD-CI using only the bound levels (continuum lifetimes go to zero). The results suggest that spectra calculated using conventional TD-CI do not converge with increasing AO basis set size, while the zero lifetime and heuristic lifetime models converge to qualitatively similar spectra, with implications for how best to apply bound state electronic structure methods to simulate HHG. The origin of HHG spectral features including the cutoff and extent of interference between peaks is uncovered by separating field-induced coupling between different types of levels (ground state, bound Rydberg levels, and continuum) in the simulated electronic dynamics. Thus the origin of deviations between the predictions of the semi-classical three step model and the full simulation can be associated with particular physical contributions, which helps to explain both the successes and the limitations of the three step model. (C) 2013 AIP Publishing LLC. C1 [Luppi, Eleonora] Univ Paris 06, Lab Chim Theor, F-75005 Paris, France. [Head-Gordon, Martin] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Head-Gordon, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Luppi, E (reprint author), Univ Paris 06, Lab Chim Theor, F-75005 Paris, France. FU Department of Energy (DOE) through the USXL program at Lawrence Berkeley National Laboratory; National Science Foundation (NSF) [CHE-1048789] FX Funding for this research has been provided by the Department of Energy (DOE) through the USXL program at Lawrence Berkeley National Laboratory. We acknowledge computational resources obtained under National Science Foundation (NSF) Award No. CHE-1048789. NR 59 TC 9 Z9 9 U1 0 U2 27 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 28 PY 2013 VL 139 IS 16 AR 164121 DI 10.1063/1.4824482 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 247RP UT WOS:000326637500024 PM 24182018 ER PT J AU Sistrunk, E Grilj, J McFarland, BK Rohlen, J Aguilar, A Guhr, M AF Sistrunk, E. Grilj, J. McFarland, B. K. Rohlen, J. Aguilar, A. Guehr, M. TI Resonant photoemission at the iron M-edge of Fe(CO)(5) SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID PHOTOELECTRON-SPECTRA; ELECTRON-SPECTROSCOPY; METAL HEXACARBONYLS; TRANSITION-METALS; CROSS-SECTIONS; PHOTON ENERGY; PHOTOIONIZATION; PENTACARBONYL; RESOLUTION; ABSORPTION AB High resolution electron kinetic energy spectra of iron pentacarbonyl (Fe(CO)(5)) are studied in the photon energy range of 40-90 eV. The relative yield of photolines associated with the Fe 3d level shows a Fano line shape at photon energies of 61 eV. The increase in signal from the 3d level is indicative of resonant photoemission involving 3p-3d transitions at the M edge of iron. The signature of this resonance is also present in photolines typically attributed to be mostly CO in character. We use the modulation depth of the Fano resonances to reinterpret the photoelectron lines in the literature. (C) 2013 AIP Publishing LLC. C1 [Sistrunk, E.; Grilj, J.; McFarland, B. K.; Guehr, M.] SLAC Natl Accelerator Lab, PULSE Inst, Menlo Pk, CA 94025 USA. [Rohlen, J.; Aguilar, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Rohlen, J.] Univ Gothenburg, Dept Phys, SE-41296 Gothenburg, Sweden. RP Guhr, M (reprint author), SLAC Natl Accelerator Lab, PULSE Inst, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. EM mguehr@stanford.edu RI Guehr, Markus/B-7446-2015 OI Guehr, Markus/0000-0002-9111-8981 FU AMOS program within the Chemical Sciences, Geosciences, and Biosciences Division of the Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy; Office of Science Early Career Research Program through the Office of Basic Energy Sciences, U.S. Department of Energy; European Research Agency via the FP-7 PEOPLE Program (Marie Curie Action) [298210]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors would like to thank the scientists and support staff at the ALS beam line 10 for their aid in setting up and performing the experiment, and Markus Koch and Kelly Gaffney for fruitful discussion. This work was supported by the AMOS program within the Chemical Sciences, Geosciences, and Biosciences Division of the Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy. M. G. acknowledges funding via the Office of Science Early Career Research Program through the Office of Basic Energy Sciences, U.S. Department of Energy. J.G. would like to acknowledge support by the European Research Agency via the FP-7 PEOPLE Program (Marie Curie Action 298210). The experiments were carried out at the Advanced Light Source, which is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 35 TC 2 Z9 2 U1 0 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 28 PY 2013 VL 139 IS 16 AR 164318 DI 10.1063/1.4827093 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 247RP UT WOS:000326637500046 PM 24182040 ER PT J AU Welch, PM AF Welch, P. M. TI The escape of a charged dendrimer from an oppositely charged planar surface SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID ANGLE NEUTRON-SCATTERING; RESPONSIVE CONFORMATIONAL-CHANGES; POLY(PROPYLENE IMINE) DENDRIMERS; PAMAM DENDRIMERS; MOLECULAR-DYNAMICS; POLY(AMIDOAMINE) DENDRIMERS; POLYELECTROLYTE DENDRIMERS; AQUEOUS-SOLUTIONS; STARBURST DENDRIMER; HYDRODYNAMIC RADII AB Many of the envisioned applications of dendrimers revolve around placing these molecules at and removing them from charged interfaces. Herein, we provide a prescription for the conditions needed to release a charged dendrimer from an oppositely charged flat substrate. Identifying an effective segment step length that reflects the intramolecular repulsions due to excluded volume and electrostatics, as well as the dendrimer's branching, provides the essential concept leading to an analytical prediction for the boundary between captured and free molecules. We find that this effective step length obeys trends similar to those predicted for linear chains, but is modified by the dendrimer's connectivity. Moreover, the boundary predicted for the capture of linear chains holds for dendrimers once this effective step length is employed. Monte Carlo computer simulations of coarse-grained model dendrimers escaping from charged surfaces validate these findings. The simulations consider generations 2 through 6 with a range of lengths between the branch points, as well as a range of solution ionic strengths and surface charge densities. (C) 2013 AIP Publishing LLC. C1 Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Welch, PM (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Welch, Paul/0000-0001-5614-2065 FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; U.S. Department of Energy Office of Biological and Environmental Research [SCFY081004]; Los Alamos National Laboratory Directed Research and Development program FX This work was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. Financial support provided by the U.S. Department of Energy Office of Biological and Environmental Research under Proposal SCFY081004 and the Los Alamos National Laboratory Directed Research and Development program. Computing time was provided by Los Alamos National Laboratory's Institutional Computing. We thank Kim Rasmussen and Boian Alexandrov for many insightful discussions of the issues addressed herein. NR 61 TC 1 Z9 1 U1 2 U2 22 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 28 PY 2013 VL 139 IS 16 AR 164906 DI 10.1063/1.4826575 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 247RP UT WOS:000326637500084 PM 24182078 ER PT J AU Barkov, F Romanenko, A Trenikhina, Y Grassellino, A AF Barkov, F. Romanenko, A. Trenikhina, Y. Grassellino, A. TI Precipitation of hydrides in high purity niobium after different treatments SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID HYDROGEN SYSTEM; ELECTRON-MICROSCOPE; TEMPERATURE; TANTALUM; ALLOYS AB Precipitation of lossy non-superconducting niobium hydrides represents a known problem for high purity niobium in superconducting applications. Using cryogenic optical and laser confocal scanning microscopy, we have directly observed surface precipitation and evolution of niobium hydrides in samples after different treatments used for superconducting RF cavities for particle acceleration. Precipitation is shown to occur throughout the sample volume, and the growth of hydrides is well described by the fast diffusion-controlled process in which almost all hydrogen is precipitated at T = 140 K within similar to 30 min. 120 degrees C baking and mechanical deformation are found to affect hydride precipitation through their influence on the number of nucleation and trapping centers. (C) 2013 Author(s). C1 [Barkov, F.; Romanenko, A.; Trenikhina, Y.; Grassellino, A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Trenikhina, Y.] IIT, Dept Phys, Chicago, IL 60616 USA. RP Romanenko, A (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM aroman@fnal.gov FU DOE Office of Nuclear Physics; United States Department of Energy [DE-AC02-07CH11359] FX We are thankful to M. Bossert, R. Schuessler, and D. Hicks for their help with sample preparation, to S. Shishkin for the help with digital processing of the images, and to H. Padamsee for useful discussions. This work was partially funded by the DOE Office of Nuclear Physics. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 38 TC 8 Z9 8 U1 2 U2 9 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 28 PY 2013 VL 114 IS 16 AR 164904 DI 10.1063/1.4826901 PG 9 WC Physics, Applied SC Physics GA 247SE UT WOS:000326639200121 ER PT J AU Gao, X Nielsen, E Muller, RP Young, RW Salinger, AG Bishop, NC Lilly, MP Carroll, MS AF Gao, X. Nielsen, E. Muller, R. P. Young, R. W. Salinger, A. G. Bishop, N. C. Lilly, M. P. Carroll, M. S. TI Quantum computer aided design simulation and optimization of semiconductor quantum dots SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID FERMI-DIRAC INTEGRALS; SCHRODINGER-POISSON EQUATIONS; SELF-CONSISTENT SOLUTION; SILICON DIOXIDE; ELECTRON-STATES; DEVICES; TRANSPORT; ACCURATE; WIRES; SPIN AB We present the Quantum Computer Aided Design (QCAD) simulator that targets modeling multi-dimensional quantum devices, particularly silicon multi-quantum dots (QDs) developed for quantum bits (qubits). This finite-element simulator has three differentiating features: (i) its core contains nonlinear Poisson, effective mass Schrodinger, and Configuration Interaction solvers that have massively parallel capability for high simulation throughput and can be run individually or combined self-consistently for 1D/2D/3D quantum devices; (ii) the core solvers show superior convergence even at near-zero-Kelvin temperatures, which is critical for modeling quantum computing devices; and (iii) it interfaces directly with the full-featured optimization engine Dakota. In this work, we describe the capabilities and implementation of the QCAD simulation tool and show how it can be used to both analyze existing experimental QD devices through capacitance calculations and aid in the design of few-electron multi-QDs. In particular, we observe that computed capacitances are in rough agreement with experiment, and that quantum confinement increases capacitance when the number of electrons is fixed in a quantum dot. Coupling of QCAD with the optimizer Dakota allows for rapid identification and improvement of device layouts that are likely to exhibit few-electron quantum dot characteristics. (C) 2013 AIP Publishing LLC. C1 [Gao, X.; Nielsen, E.; Muller, R. P.; Young, R. W.; Salinger, A. G.; Bishop, N. C.; Lilly, M. P.; Carroll, M. S.] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Gao, X (reprint author), Sandia Natl Labs, 1515 Eubank SE, Albuquerque, NM 87123 USA. EM xngao@sandia.gov FU Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories. Sandia is a Multiprogram Laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 53 TC 8 Z9 8 U1 0 U2 21 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 28 PY 2013 VL 114 IS 16 AR 164302 DI 10.1063/1.4825209 PG 19 WC Physics, Applied SC Physics GA 247SE UT WOS:000326639200080 ER PT J AU Johnson-Wilke, RL Tinberg, DS Yeager, C Qu, WG Fong, DD Fister, TT Streiffer, SK Han, YS Reaney, IM Trolier-McKinstry, S AF Johnson-Wilke, Raegan L. Tinberg, Daniel S. Yeager, C. Qu, Weiguo Fong, Dillon D. Fister, Timothy T. Streiffer, Stephen K. Han, Yisong Reaney, Ian M. Trolier-McKinstry, Susan TI Coherently strained epitaxial Pb(Zr1-xTix)O-3 thin films SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID PIEZOELECTRIC PROPERTIES; PEROVSKITES; THICKNESS; LATTICE; BATIO3; LAYER; SITU; LEAD AB Coherently strained Pb(Zr1-xTix)O-3, 0.2 <= x <= 0.35, thin films were grown by pulsed laser deposition on (001) and (111) oriented SrTiO3 substrates. A buffer layer of Pb(Zr0.6Ti0.4)O-3 was used to improve the lattice matching and induce compressive strain in Zr-rich compositions. The (001)(pc) (pc = pseudocubic) films showed an increased ferroelectric transition temperature, T-C, compared to bulk ceramics, but the transition from an untilted to a tilted ferroelectric (T-Tilt) exhibited only a modest increase in temperature. This suggests that it may be possible to enlarge the untilted ferroelectric phase field by compressive strain. Consistent with previous work on relaxed PZT films, coherently strained PZT films do not exhibit an abrupt transition from an untilted to a tilted state; rather, a region of non-zero tilt exists above T-Tilt. (111)(pc) films also showed an increased ferroelectric transition temperature with a weak strain dependence on TTilt. The compressive strain in (111)(pc) films induced a preferred domain structure with only 180 degrees domain walls, in contrast to bulk materials and relaxed films which are polydomain. (C) 2013 AIP Publishing LLC. C1 [Johnson-Wilke, Raegan L.; Tinberg, Daniel S.; Yeager, C.; Qu, Weiguo; Trolier-McKinstry, Susan] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Fong, Dillon D.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Fister, Timothy T.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Streiffer, Stephen K.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Han, Yisong] Univ Cambridge, Dept Mat Sci & Met, Cambridge CB3 0FS, England. [Reaney, Ian M.] Univ Sheffield, Dept Mat Sci & Engn, Sheffield S1 3JD, S Yorkshire, England. RP Johnson-Wilke, RL (reprint author), Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. OI Trolier-McKinstry, Susan/0000-0002-7267-9281 FU National Science Foundation [DMR-0602770, DMR-0820404]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX R.L.J.-W., D. S. T., C.Y., and S.T.-M. were funded through Grants DMR-0602770 and DMR-0820404 from the National Science Foundation. D. D. F., T. T. F., and S. K. S. were supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. The use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We would like to thank Dr. Jenia Karapetrova at Sector 33BM and Peter Baldo at Argonne National Laboratory for their assistance during the synchrotron diffraction experiments. NR 24 TC 4 Z9 4 U1 3 U2 37 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 28 PY 2013 VL 114 IS 16 AR 164104 DI 10.1063/1.4825215 PG 10 WC Physics, Applied SC Physics GA 247SE UT WOS:000326639200074 ER PT J AU Mahanta, NK Abramson, AR Howe, JY AF Mahanta, Nayandeep K. Abramson, Alexis R. Howe, Jane Y. TI Thermal conductivity measurements on individual vapor-grown carbon nanofibers and graphene nanoplatelets SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ELECTRICAL-CONDUCTIVITY; PYROLYTIC-GRAPHITE; PHONON TRANSPORT; LAYER GRAPHENE; NANOTUBES; COMPOSITES; FIBERS; CONDUCTANCE; THERMOPOWER; RESISTANCE AB The thermal flash technique was utilized for measuring the thermal conductivity of vapor-grown carbon nanofibers and graphene nanoplatelets. The vapor-grown carbon nanofibers with stacked-cone morphology and heat treated to 1100 degrees C and 3000 degrees C were measured to have thermal conductivities of 1130 W/m K and 1715 W/m K, respectively. The physical dimensions of the constitutive cones determining the mean free path due to static phonon scattering were estimated to be similar to 128 nm and similar to 176 nm for the low and high heat treatment temperatures, respectively. Static scattering lengths shorter than the Umklapp scattering length indicate ballistic transport within individual cones and limit the thermal conductivities of the nanofibers. Additionally, nanoplatelets of few-layer oxygen intercalated graphene and multi-layer reduced graphene exhibited thermal conductivities of 776 W/m K and 2275 W/m K, respectively. The lower thermal conductivity of few-layer (similar to 3 layers) graphene is attributed to the presence of intercalating oxygen atoms which introduce covalent character to the interlayer interactions, acting as phonon scattering centers and hence reducing the phonon mean free path. The thermal conductivity measured for multi-layer graphene with similar to 30-45 layers lies within range of the thermal conductivities previously reported for bulk graphite. (C) 2013 AIP Publishing LLC. C1 [Mahanta, Nayandeep K.; Abramson, Alexis R.] Case Western Reserve Univ, Dept Mech & Aerosp Engn, Cleveland, OH 44106 USA. [Howe, Jane Y.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Abramson, AR (reprint author), Case Western Reserve Univ, Dept Mech & Aerosp Engn, 2123 Martin Luther King Jr Dr, Cleveland, OH 44106 USA. EM alexis.abramson@case.edu RI Howe, Jane/G-2890-2011 FU U. S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Program; State of Ohio FX The authors would like to thank Max L. Lake and other staff at Applied Sciences, Inc. for the invaluable discussions regarding the synthesis and microstructure of the carbon nanofibers. Part of this research at the Oak Ridge National Laboratory's High Temperature Materials Laboratory was sponsored by the U. S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Program. This work was made possible in part through financial support from the State of Ohio. The content reflects the views of the authors and does not purport to reflect the views of the State of Ohio. NR 45 TC 3 Z9 3 U1 2 U2 25 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 28 PY 2013 VL 114 IS 16 AR 163528 DI 10.1063/1.4827378 PG 8 WC Physics, Applied SC Physics GA 247SE UT WOS:000326639200040 ER PT J AU Negotia, M Hodges, MPP Bryan, MT Fry, PW Im, MY Fischer, P Allwood, DA Hayward, TJ AF Negotia, M. Hodges, M. P. P. Bryan, M. T. Fry, P. W. Im, M. -Y. Fischer, P. Allwood, D. A. Hayward, T. J. TI Linear transport of domain walls confined to propagating 1-D potential wells SO JOURNAL OF APPLIED PHYSICS LA English DT Article AB We present a method of controllably propagating domain walls (DWs) in magnetic nanowires over extended linear distances by confining them to geometrically defined energy minima. Using simple models, magnetic transmission soft x-ray microscopy and magneto-optic Kerr effect measurements, we show that the technique allows DWs to be moved at arbitrary, user-defined velocities and be positioned with micrometer precision. Our approach is expected to be of utility in applications where the precise transport and positioning of DWs take precedent over the absolute speed of propagation, for example, where the fields produced by DWs are used to trap and transport magnetized particles. (C) 2013 AIP Publishing LLC. C1 [Negotia, M.; Hodges, M. P. P.; Bryan, M. T.; Allwood, D. A.; Hayward, T. J.] Univ Sheffield, Dept Mat Sci & Engn, Sheffield S10 2TN, S Yorkshire, England. [Fry, P. W.] Univ Sheffield, Nanosci & Technol Ctr, Sheffield S10 2TN, S Yorkshire, England. [Im, M. -Y.; Fischer, P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Xray Opt, Berkeley, CA 94720 USA. RP Negotia, M (reprint author), Univ Sheffield, Dept Mat Sci & Engn, Sheffield S10 2TN, S Yorkshire, England. RI Fischer, Peter/A-3020-2010 OI Fischer, Peter/0000-0002-9824-9343 FU EPSRC [EP/J002275/1, EP/F025459/1]; Berkeley Lab's program on Magnetic Materials; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy FX This work was supported by the EPSRC (Grant Nos. EP/J002275/1 and EP/F025459/1). P. F. and M.-Y. Im acknowledge support by Berkeley Lab's program on Magnetic Materials, funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. Portions of this work were performed as a User project at the Advanced Light Source, supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy. NR 20 TC 0 Z9 0 U1 1 U2 9 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 28 PY 2013 VL 114 IS 16 AR 163901 DI 10.1063/1.4825044 PG 6 WC Physics, Applied SC Physics GA 247SE UT WOS:000326639200056 ER PT J AU Sullivan, KT Bastea, S Kuntz, JD Gash, AE AF Sullivan, K. T. Bastea, S. Kuntz, J. D. Gash, A. E. TI A pressure-driven flow analysis of gas trapping behavior in nanocomposite thermite films SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID NANOSCALE AL/MOO3 THERMITE; REACTION PROPAGATION; COMBUSTION; AL/CUO; NANOALUMINUM; OXYGEN AB This article is in direct response to a recently published article entitled Electrophoretic deposition and mechanistic studies of nano-Al/CuO thermites (K. T. Sullivan et al., J. Appl. Phys., 112(2), 2012), in which we introduced a non-dimensional parameter as the ratio of gas production to gas escape within a thin porous thermite film. In our original analysis, we had treated the problem as Fickian diffusion of gases through the porous network. However, we believe a more physical representation of the problem is to treat this as pressure-driven flow of gases in a porous medium. We offer a new derivation of the non-dimensional parameter which calculates gas velocity using the well-known Poiseuille's Law for pressure-driven flow in a pipe. This updated analysis incorporates the porosity, gas viscosity, and pressure gradient into the equation. (C) 2013 AIP Publishing LLC. C1 [Sullivan, K. T.; Bastea, S.; Kuntz, J. D.; Gash, A. E.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Sullivan, KT (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344 NR 16 TC 3 Z9 3 U1 1 U2 21 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 28 PY 2013 VL 114 IS 16 AR 164907 DI 10.1063/1.4826617 PG 4 WC Physics, Applied SC Physics GA 247SE UT WOS:000326639200124 ER PT J AU Duhovic, S Oria, JV Odoh, SO Schreckenbach, G Batista, ER Diaconescu, PL AF Duhovic, Selma Oria, Jeremy V. Odoh, Samuel O. Schreckenbach, Georg Batista, Enrique R. Diaconescu, Paula L. TI Investigation of the Electronic Structure of Mono(1,1 '-Diamidoferrocene) Uranium(IV) Complexes SO ORGANOMETALLICS LA English DT Article ID TRANSITION-METAL-COMPLEXES; FERROCENE DIAMIDE LIGAND; ALKYL COMPLEXES; ABSORPTION-SPECTRA; POLYMERIZATION CATALYST; AROMATIC HETEROCYCLES; ACTINIDE COMPLEXES; REDOX CONTROL; BOND; ACTIVATION AB The electronic structure of several mono(1,1'-diamidoferrocene) uranium complexes (NNR)UX2 (NNR = fc(NR)(2), fc = 1,1'-ferrocenediyl, R = SiMe3, (SiBuMe2)-Bu-t, SiMe2Ph, X = I, CH2Ph), (NNTBS)UI(OAr) (OAr = 2,6-di-tert-butylphenoxide), and (NNTBS)U(CH2Ph)(OAr) was investigated by electrochemistry, electronic absorption and vibrational spectroscopy, and DFT calculations. Similar metrical parameters were observed for (NNTBS)U(CH2Ph)(2) and (NNDMP)U(CH2Ph)(2) (and also for the previously reported (NNTBS)UI2(THF), (NNTBS)UI2(THF), and (NNTBS)U(CH2Ph)(OAr)) that translate in similar DFT parameters (bond orders, metal charges) despite some small differences observed by electrochemistry and IR or electronic absorption spectroscopy. C1 [Duhovic, Selma; Oria, Jeremy V.; Diaconescu, Paula L.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Odoh, Samuel O.; Schreckenbach, Georg] Univ Manitoba, Dept Chem, Winnipeg, MB R3T 2N2, Canada. [Batista, Enrique R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Diaconescu, PL (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, 607 Charles E Young Dr East, Los Angeles, CA 90095 USA. EM pld@chem.ucla.edu FU U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry program [ER15984, 2012LANLE372]; LANL; Natural Sciences and Engineering Council of Canada (NSERC); Seaborg Institute for Transactinium Sciences at Los Alamos National Laboratory through a Seaborg Summer Research Fellowship FX The experimental and part of the computational work (S.D., J.V.O., P.L.D.) were supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry program under Grant No. ER15984 (to PLD), and the Sloan Foundation. The rest of the computational work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry program under Grant No. 2012LANLE372 (to ERB). J.V.O. was supported by an LANL graduate student research fellowship during the summer of 2013. G.S. acknowledges funding from the Natural Sciences and Engineering Council of Canada (NSERC). S.O.O. has been funded by the Seaborg Institute for Transactinium Sciences at Los Alamos National Laboratory through a Seaborg Summer Research Fellowship. NR 76 TC 14 Z9 14 U1 4 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD OCT 28 PY 2013 VL 32 IS 20 BP 6012 EP 6021 DI 10.1021/om400521k PG 10 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA 244CY UT WOS:000326365900038 ER PT J AU Bessas, D Rushchanskii, KZ Kachlik, M Disch, S Gourdon, O Bednarcik, J Maca, K Sergueev, I Kamba, S Lezaic, M Hermann, RP AF Bessas, D. Rushchanskii, K. Z. Kachlik, M. Disch, S. Gourdon, O. Bednarcik, J. Maca, K. Sergueev, I. Kamba, S. Lezaic, M. Hermann, R. P. TI Lattice instabilities in bulk EuTiO3 SO PHYSICAL REVIEW B LA English DT Article ID X-RAY-DIFFRACTION; ATOMIC DISPLACEMENTS; MAGNETIC PROPERTIES; POWDER DIFFRACTION; SCATTERING; PEROVSKITES; RESONANCE; TITANATE; ELECTRON; CRYSTAL AB The phase purity and the lattice dynamics in bulk EuTiO3 were investigated both microscopically, using x-ray and neutron diffraction, Eu-151-Mossbauer spectroscopy, and Eu-151 nuclear inelastic scattering, and macroscopically using calorimetry, resonant ultrasound spectroscopy, and magnetometry. Furthermore, our investigations were corroborated by ab initio theoretical studies. The perovskite symmetry, Pm (3) over barm, is unstable at the M- and R-points of the Brillouin zone. The lattice instabilities are lifted when the structure relaxes in one of the symmetries: I4/mcm, Imma, R (3) over barc with relative relaxation energy around -25 meV. Intimate phase analysis confirmed phase purity of our ceramics. A prominent peak in the Eu specific density of phonon states at 11.5 meV can be modeled in all candidate symmetries. A stiffening on heating around room temperature is indicative of a phase transition similar to the one observed in SrTiO3, however, although previous studies reported the structural phase transition to the tetragonal I4/mcm phase our detailed sample purity analysis and thorough structural studies using complementary techniques did not confirm a direct phase transition. Instead, in the same temperature range, Eu delocalization is observed which might explain the lattice dynamical instabilities. C1 [Bessas, D.; Disch, S.; Sergueev, I.; Hermann, R. P.] JCNS, D-52425 Julich, Germany. [Bessas, D.; Disch, S.; Sergueev, I.; Hermann, R. P.] Forschungszentrum Julich GmbH, JARA FIT, PGI, F-38043 Grenoble, France. [Bessas, D.; Hermann, R. P.] Univ Liege, Fac Sci, B-4000 Liege, Belgium. [Rushchanskii, K. Z.; Lezaic, M.] Forschungszentrum Julich, Peter Grunberg Inst, F-38043 Grenoble, France. [Rushchanskii, K. Z.; Lezaic, M.] JARA, F-38043 Grenoble, France. [Kachlik, M.; Maca, K.] Brno Univ Technol, CEITEC, Brno 61600, Czech Republic. [Disch, S.] Inst Laue Langevin, F-38042 Grenoble, France. [Gourdon, O.] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. [Gourdon, O.] Oak Ridge Natl Lab, JCNS, Oak Ridge, TN 37831 USA. [Bednarcik, J.] Deutsch Elect Synchrotron, D-22607 Hamburg, Germany. [Sergueev, I.] European Synchrotron Radiat Facil, F-38043 Grenoble, France. [Kamba, S.] Acad Sci Czech Republic, Inst Phys, Prague 18221, Czech Republic. RP Bessas, D (reprint author), European Synchrotron Radiat Facil, BP 220, F-38043 Grenoble, France. EM r.hermann@fz-juelich.de RI Lezaic, Marjana/H-8510-2013; Sergueev, Ilya/N-6591-2013; Hermann, Raphael/F-6257-2013; Kamba, Stanislav/G-5332-2014; Maca, Karel/D-7520-2012; Kachlik, Martin/D-6865-2012; Bessas, Dimitrios/I-5262-2013; Disch, Sabrina/K-7185-2013 OI Lezaic, Marjana/0000-0002-7318-9444; Sergueev, Ilya/0000-0002-7614-2238; Hermann, Raphael/0000-0002-6138-5624; Kamba, Stanislav/0000-0003-4699-869X; Kachlik, Martin/0000-0002-0619-4032; Bessas, Dimitrios/0000-0003-0240-2540; Disch, Sabrina/0000-0002-4565-189X FU Helmholtz Association of German research centers [VH NG-407, VH NG-409]; Czech Science Foundation [P204/12/1163]; MEYS [LD 11035, LD 12026 - COST MP0904]; ERDF [CEITEC - CZ.1.05/1.1.00/02.0068] FX The Helmholtz Association of German research centers is acknowledged for funding (VH NG-407 "Lattice dynamics in emerging functional materials" and VH NG-409 "Computational Nanoferronics Laboratory"). The European Synchrotron Radiation Facility, the Advanced Photon Source, the PETRAIII, and the Spallation Neutron Source are acknowledged for provision of synchrotron radiation and neutron beam time at ID22N, 6-ID-D, P02.1, POW-GEN, and NOMAD, respectively. The work in the Czech Republic has been supported by the Czech Science Foundation (Project No. P204/12/1163), MEYS (LD 11035 and LD 12026 - COST MP0904), and the ERDF (CEITEC - CZ.1.05/1.1.00/02.0068). We are grateful to Dr. D. Robinson, Dr. M. Feygenson, and Dr. J. Neuefeind for help during data acquisition and Julich Supercomputing Center for support. NR 66 TC 10 Z9 10 U1 2 U2 66 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD OCT 28 PY 2013 VL 88 IS 14 AR 144308 DI 10.1103/PhysRevB.88.144308 PG 9 WC Physics, Condensed Matter SC Physics GA 241IF UT WOS:000326159200002 ER PT J AU Korgul, A Rykaczewski, KP Grzywacz, R Sliwinska, H Batchelder, JC Bingham, C Borzov, IN Brewer, N Cartegni, L Fijalkowska, A Gross, CJ Hamilton, JH Jost, C Karny, M Krolas, W Liu, S Mazzocchi, C Madurga, M Mendez, AJ Miernik, K Miller, D Padgett, S Paulauskas, S Shapira, D Stracener, D Sieja, K Winger, JA Wolinska-Cichocka, M Zganjar, EF AF Korgul, A. Rykaczewski, K. P. Grzywacz, R. Sliwinska, H. Batchelder, J. C. Bingham, C. Borzov, I. N. Brewer, N. Cartegni, L. Fijalkowska, A. Gross, C. J. Hamilton, J. H. Jost, C. Karny, M. Krolas, W. Liu, S. Mazzocchi, C. Madurga, M. Mendez, A. J., II Miernik, K. Miller, D. Padgett, S. Paulauskas, S. Shapira, D. Stracener, D. Sieja, K. Winger, J. A. Wolinska-Cichocka, M. Zganjar, E. F. TI Experimental study of the beta-gamma and beta-n gamma decay of the neutron-rich nucleus Ga-85 SO PHYSICAL REVIEW C LA English DT Article ID SHELL-MODEL; SPECTROSCOPY AB The beta-decay properties of neutron-rich Ga-85 produced in proton-induced fission of U-238 were studied at the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory. Data consisted of beta - gamma and beta - gamma - gamma coincidences were collected at the Low-energy Radioactive Ion Beam Spectroscopy Station after high-resolution on-line mass separation. For the first time, the excited states in the N = 53 isotone Ge-85 were established from beta-delayed gamma decay of Ga-85. The level scheme of the N = 52 isotone Ge-84 was improved and includes now 0(+), 2(+), (2)(+), 4(+), and (0)(+) states populated in the beta-delayed-neutron-gamma decay of Ga-85. Advanced shell-model calculations were used to analyze experimental data on Ge-85 and Ge-84. C1 [Korgul, A.; Fijalkowska, A.; Karny, M.; Mazzocchi, C.; Miernik, K.] Univ Warsaw, Fac Phys, PL-00681 Warsaw, Poland. [Korgul, A.; Borzov, I. N.] Joint Inst Heavy Ion Res, Oak Ridge, TN 37831 USA. [Rykaczewski, K. P.; Grzywacz, R.; Bingham, C.; Gross, C. J.; Mendez, A. J., II; Miernik, K.; Shapira, D.; Stracener, D.; Wolinska-Cichocka, M.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Grzywacz, R.; Bingham, C.; Cartegni, L.; Madurga, M.; Miller, D.; Padgett, S.; Paulauskas, S.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Sliwinska, H.; Sieja, K.] Univ Strasbourg, IPHC, CNRS, UMR7178, F-67037 Strasbourg, France. [Batchelder, J. C.; Jost, C.; Liu, S.] Oak Ridge Associated Univ, UNIRIB, Oak Ridge, TN 37831 USA. [Borzov, I. N.] Joint Inst Nucl Res, Bogoliubov Lab Theoret Phys, Dubna 141980, Russia. [Brewer, N.; Hamilton, J. H.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Jost, C.; Liu, S.; Wolinska-Cichocka, M.] Oak Ridge Associated Univ, ORAU, Oak Ridge, TN 37831 USA. [Krolas, W.] Polish Acad Sci, Inst Nucl Phys, PL-31342 Krakow, Poland. [Winger, J. A.] Mississippi State Univ, Dept Phys & Astron, Mississippi State, MS 39762 USA. [Wolinska-Cichocka, M.] Warsaw Univ, Heavy Ion Lab, PL-02093 Warsaw, Poland. [Zganjar, E. F.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. RP Korgul, A (reprint author), Univ Warsaw, Fac Phys, PL-00681 Warsaw, Poland. RI Krolas, Wojciech/N-9391-2013; Miller, David/B-5372-2012 OI Miller, David/0000-0002-0426-974X FU Office of Nuclear Physics, U.S. Department of Energy; U.S. DOE [DE-AC05-00OR22725, DE-FG02-96ER41006, DE-FG02-96ER40983, DE-AC05-06OR23100, DE-FG02-96ER40978, DE-FG05-88ER40407]; National Nuclear Security Administration [DEFC03-03NA00143]; National Science Centre of the Polish Ministry of Science and Higher Education [2011/01/B/ST2/02476]; Helmholtz Alliance EMMI; IN2P3-RFBR [110291054]; U.S. Department of Energy [DE-AC05-00OR22725] FX We wish to acknowledge the Holifield Radioactive Ion Beam Facility (HRIBF) staff for their assistance with the experiments and for providing excellent quality neutron-rich radioactive beams. This research was sponsored by the Office of Nuclear Physics, U.S. Department of Energy, and supported under U.S. DOE Grants No. DE-AC05-00OR22725, No. DE-FG02-96ER41006, No. DE-FG02-96ER40983, No. DE-AC05-06OR23100, No. DE-FG02-96ER40978, and No. DE-FG05-88ER40407; National Nuclear Security Administration Grant No. DEFC03-03NA00143; National Science Centre of the Polish Ministry of Science and Higher Education Grant No. 2011/01/B/ST2/02476. I.N.B. was partially supported by Helmholtz Alliance EMMI and a grant from IN2P3-RFBR under Agreement No. 110291054. K.M.'s research was performed as a Eugene P. Wigner fellow and staff member at the Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. NR 36 TC 9 Z9 9 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 28 PY 2013 VL 88 IS 4 AR 044330 DI 10.1103/PhysRevC.88.044330 PG 6 WC Physics, Nuclear SC Physics GA 241IV UT WOS:000326161000002 ER PT J AU Marsh, JC Ma, WC Hagemann, GB Janssens, RVF Bengtsson, R Ryde, H Carpenter, MP Gurdal, G Hartley, DJ Hoffman, CR Ijaz, QA Kondev, FG Lauritsen, T Mukhopadhyay, S Riedinger, LL Yadav, RB Zhu, S AF Marsh, J. C. Ma, W. C. Hagemann, G. B. Janssens, R. V. F. Bengtsson, R. Ryde, H. Carpenter, M. P. Guerdal, G. Hartley, D. J. Hoffman, C. R. Ijaz, Q. A. Kondev, F. G. Lauritsen, T. Mukhopadhyay, S. Riedinger, L. L. Yadav, R. B. Zhu, S. TI Identification of triaxial strongly deformed bands in Hf-164 SO PHYSICAL REVIEW C LA English DT Article ID HIGH-SPIN; WOBBLING EXCITATIONS; SPECTROSCOPY; NUCLEI; MODE AB Two new rotational bands of distinct character have been identified in Hf-164. They are suggested to correspond to the long-anticipated triaxial strongly deformed (TSD) bands predicted by theoretical studies. The bands have been linked to known states, and the level spins and energies could be determined. The bands are also substantially stronger in intensity and are located at lower spins than the previously observed TSD bands in Hf-168, hereby making Hf-164 the best even-even system so far for the study of TSD structures in the A similar to 160 mass region. Cranking calculations based on the modified-oscillator model suggest that the bands are associated with four-quasiparticle configurations that involve high-j intruder (i(13/2))(2) proton orbitals. C1 [Marsh, J. C.; Ma, W. C.; Ijaz, Q. A.; Yadav, R. B.] Mississippi State Univ, Dept Phys & Astron, Mississippi State, MS 39762 USA. [Hagemann, G. B.] Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Janssens, R. V. F.; Carpenter, M. P.; Hoffman, C. R.; Lauritsen, T.; Zhu, S.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Bengtsson, R.] Lund Inst Technol, Dept Math Phys, S-22100 Lund, Sweden. [Ryde, H.] Lund Univ, Dept Nucl Phys, S-22100 Lund, Sweden. [Guerdal, G.; Kondev, F. G.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Hartley, D. J.] US Naval Acad, Dept Phys, Annapolis, MD 21402 USA. [Mukhopadhyay, S.] Bhabha Atom Res Ctr, Div Nucl Phys, Bombay 400085, Maharashtra, India. [Riedinger, L. L.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Marsh, JC (reprint author), Mississippi State Univ, Dept Phys & Astron, Mississippi State, MS 39762 USA. RI Carpenter, Michael/E-4287-2015; Hoffman, Calem/H-4325-2016 OI Carpenter, Michael/0000-0002-3237-5734; Hoffman, Calem/0000-0001-7141-9827 FU U.S. Department of Energy, Office of Nuclear Physics [DE-FG02-95ER40939, DE-AC02-06CH11357]; National Science Foundation [PHY-1203100] FX The authors thank the ANL operations at Gammasphere and gratefully acknowledge the efforts of J. P. Green for the target preparation. This work was supported by the U.S. Department of Energy, Office of Nuclear Physics, under Grants No. DE-FG02-95ER40939 (MSU) and No. DE-AC02-06CH11357 (ANL) and the National Science Foundation under Grant No. PHY-1203100 (USNA). NR 30 TC 5 Z9 5 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 28 PY 2013 VL 88 IS 4 AR 041306 DI 10.1103/PhysRevC.88.041306 PG 5 WC Physics, Nuclear SC Physics GA 241IV UT WOS:000326161000001 ER PT J AU Wiranata, A Koch, V Prakash, M Wang, XN AF Wiranata, Anton Koch, Volker Prakash, Madappa Wang, Xin Nian TI Shear viscosity of hadrons with K-matrix cross sections SO PHYSICAL REVIEW C LA English DT Article ID KINETIC GAS THEORY; HEAVY-ION COLLISIONS; PB-PB COLLISIONS; TRANSPORT-COEFFICIENTS; STATISTICAL-MECHANICS; GLUON PLASMA; TEMPERATURE; QCD AB Shear viscosity eta and entropy density s of a hadronic resonance gas are calculated using the Chapman-Enskog and virial expansion methods using the K-matrix parametrization of hadronic cross sections which preserves the unitarity of the T matrix. In the pi-K-N-eta mixture considered, a total of 57 resonances up to 2 GeV were included. Comparisons are also made to results with other hadronic cross sections such as the Breit-Wigner (BW) and, where available, experimental phase shift parameterizations. Hadronic interactions forming resonances are shown to decrease the shear viscosity and increase the entropy density leading to a substantial reduction of eta/s as the QCD phase transition temperature is approached. C1 [Wiranata, Anton; Wang, Xin Nian] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. [Wiranata, Anton; Wang, Xin Nian] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. [Wiranata, Anton; Koch, Volker; Wang, Xin Nian] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Prakash, Madappa] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. RP Wiranata, A (reprint author), Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. EM awiranata@lbl.gov; vkoch@lbl.gov; prakash@phy.ohiou.edu; xnwang@lbl.gov RI Prakash, Madappa/D-9820-2016; OI Wang, Xin-Nian/0000-0002-9734-9967 FU NSFC [11221504]; US DOE [DE-AC02-05CH11231, DE-FG02-93ER-40756] FX This work is supported by the NSFC under Grant No. 11221504, and by the US DOE under Contracts No. DE-AC02-05CH11231 and No. DE-FG02-93ER-40756. NR 67 TC 9 Z9 9 U1 0 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 28 PY 2013 VL 88 IS 4 AR 044917 DI 10.1103/PhysRevC.88.044917 PG 14 WC Physics, Nuclear SC Physics GA 241IV UT WOS:000326161000005 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, MJ Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Yushkov, AN Kirkby, D Lankford, AJ Mandelkern, M Dey, B Gary, JW Long, O Vitug, GM Campagnari, C Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Ongmongkolkul, P Porter, FC Andreassen, R Huard, Z Meadows, BT Pushpawela, BG Sokoloff, MD Sun, L Bloom, PC Ford, WT Gaz, A Nauenberg, U Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Schwierz, R Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Baldini-Ferroli, R Calcaterra, A de Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Guido, E Lo Vetere, M Monge, MR Passaggio, S Patrignani, C Robutti, E Bhuyan, B Prasad, V Morii, M Adametz, A Uwer, U Lacker, HM Dauncey, PD Mallik, U Chen, C Cochran, J Meyer, WT Prell, S Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Bougher, J Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Prencipe, E Schubert, KR Barlow, RJ Lafferty, GD Behn, E Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Dujmic, D Sciolla, G Cheaib, R Patel, PM Robertson, SH Biassoni, P Neri, N Palombo, F Cremaldi, L Godang, R Sonnek, P Summers, DJ Simard, M Taras, P De Nardo, G Monorchio, D Onorato, G Sciacca, C Martinelli, M Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Brau, J Frey, R Sinev, NB Strom, D Torrence, E Feltresi, E Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Sitt, S Biasini, M Manoni, E Pacetti, S Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Cervelli, A Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Perez, A Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Gioi, LL Piredda, G Bunger, C Grunberg, O Hartmann, T Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S de Monchenault, GH Vasseur, G Yeche, C Anulli, F Aston, D Bard, DJ Benitez, JF Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Gabareen, AM Graham, MT Hast, C Innes, WR Kim, P Kocian, ML Leith, DWGS Lewis, P Lindemann, D Lindquist, B Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Nelson, S Perl, M Pulliam, T Ratcliff, BN Roodman, A Salnikov, AA Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wagner, AP Wang, WF Wisniewski, WJ Wittgen, M Wright, DH Wulsin, HW Ziegler, V Park, W Purohit, MV White, RM Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Miyashita, TS Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Ruland, AM Schwitters, RF Wray, BC Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Zambito, S Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Villanueva-Perez, P Ahmed, H Albert, J Banerjee, S Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lee, M. J. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Yushkov, A. N. Kirkby, D. Lankford, A. J. Mandelkern, M. Dey, B. Gary, J. W. Long, O. Vitug, G. M. Campagnari, C. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Ongmongkolkul, P. Porter, F. C. Andreassen, R. Huard, Z. Meadows, B. T. Pushpawela, B. G. Sokoloff, M. D. Sun, L. Bloom, P. C. Ford, W. T. Gaz, A. Nauenberg, U. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Schwierz, R. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Baldini-Ferroli, R. Calcaterra, A. de Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Guido, E. Lo Vetere, M. Monge, M. R. Passaggio, S. Patrignani, C. Robutti, E. Bhuyan, B. Prasad, V. Morii, M. Adametz, A. Uwer, U. Lacker, H. M. Dauncey, P. D. Mallik, U. Chen, C. Cochran, J. Meyer, W. T. Prell, S. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Bougher, J. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Prencipe, E. Schubert, K. R. Barlow, R. J. Lafferty, G. D. Behn, E. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Dujmic, D. Sciolla, G. Cheaib, R. Patel, P. M. Robertson, S. H. Biassoni, P. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Sonnek, P. Summers, D. J. Simard, M. Taras, P. De Nardo, G. Monorchio, D. Onorato, G. Sciacca, C. Martinelli, M. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Brau, J. Frey, R. Sinev, N. B. Strom, D. Torrence, E. Feltresi, E. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph. Marchiori, G. Ocariz, J. Sitt, S. Biasini, M. Manoni, E. Pacetti, S. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Cervelli, A. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Perez, A. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Gioi, L. Li Piredda, G. Buenger, C. Gruenberg, O. Hartmann, T. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. de Monchenault, G. Hamel Vasseur, G. Yeche, Ch. Anulli, F. Aston, D. Bard, D. J. Benitez, J. F. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Gabareen, A. M. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Kocian, M. L. Leith, D. W. G. S. Lewis, P. Lindemann, D. Lindquist, B. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Nelson, S. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Salnikov, A. A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wagner, A. P. Wang, W. F. Wisniewski, W. J. Wittgen, M. Wright, D. H. Wulsin, H. W. Ziegler, V. Park, W. Purohit, M. V. White, R. M. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Miyashita, T. S. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Ruland, A. M. Schwitters, R. F. Wray, B. C. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Zambito, S. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Villanueva-Perez, P. Ahmed, H. Albert, J. Banerjee, Sw. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. TI Measurement of the e(+)e(-) -> p(p)over-bar cross section in the energy range from 3.0 to 6.5 GeV SO PHYSICAL REVIEW D LA English DT Article ID LARGE MOMENTUM-TRANSFER; HADRONIC FORM-FACTORS; QUANTUM CHROMODYNAMICS; RADIATIVE-CORRECTIONS; BHABHA SCATTERING; BABAR DETECTOR; MONTE-CARLO AB The e(+)e(-) -> p (p) over bar cross section and the proton magnetic form factor have been measured in the center-of-mass energy range from 3.0 to 6.5 GeV using the initial-state radiation technique with an undetected photon. This is the first measurement of the form factor at energies higher than 4.5 GeV. The analysis is based on 469 fb-1 of integrated luminosity collected with the BABAR detector at the PEP-II collider at e(+)e(-) center-of-mass energies near 10.6 GeV. The branching fractions for the decays J/psi -> p (p) over bar and psi(2S) -> p (p) over bar have also been measured. C1 [Lees, J. P.; Poireau, V.; Tisserand, V.] Univ Savoie, CNRS, IN2P3, Lab Annecy Le Vieux Phys Particules, F-74941 Annecy Le Vieux, France. [Grauges, E.] Univ Barcelona, Fac Fis, Dept ECM, E-08028 Barcelona, Spain. [Palano, A.] Ist Nazl Fis Nucl, Sez Bari, I-70125 Bari, Italy. [Palano, A.] Univ Bari, Dipartmento Fis, I-70126 Bari, Italy. [Eigen, G.; Stugu, B.] Univ Bergen, Inst Phys, N-5007 Bergen, Norway. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu. G.; Lee, M. J.; Lynch, G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu. G.; Lee, M. J.; Lynch, G.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Koch, H.; Schroeder, T.] Ruhr Univ Bochum, Inst Expt Phys 1, D-44780 Bochum, Germany. [Hearty, C.; Mattison, T. S.; McKenna, J. A.; So, R. Y.] Univ British Columbia, Vancouver, BC V6T 1Z1, Canada. [Khan, A.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Blinov, V. E.; Buzykaev, A. R.; Druzhinin, V. P.; Golubev, V. B.; Kravchenko, E. A.; Onuchin, A. P.; Serednyakov, S. I.; Skovpen, Yu. I.; Solodov, E. P.; Todyshev, K. Yu.; Yushkov, A. N.] RAS, Budker Inst Nucl Phys, SB, Novosibirsk 630090, Russia. [Druzhinin, V. P.; Golubev, V. B.; Kravchenko, E. A.; Serednyakov, S. I.; Skovpen, Yu. I.; Solodov, E. P.; Todyshev, K. Yu.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Blinov, V. E.; Onuchin, A. P.] Novosibirsk State Tech Univ, Novosibirsk 630090, Russia. [Kirkby, D.; Lankford, A. J.; Mandelkern, M.] Univ Calif Irvine, Irvine, CA 92697 USA. [Dey, B.; Gary, J. W.; Long, O.; Vitug, G. M.] Univ Calif Riverside, Riverside, CA 92521 USA. [Campagnari, C.; Sevilla, M. Franco; Hong, T. M.; Kovalskyi, D.; Richman, J. D.; West, C. A.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Eisner, A. M.; Lockman, W. S.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Inst Particle Phys, Santa Cruz, CA 95064 USA. [Chao, D. S.; Cheng, C. H.; Echenard, B.; Flood, K. T.; Hitlin, D. G.; Ongmongkolkul, P.; Porter, F. C.] CALTECH, Pasadena, CA 91125 USA. [Andreassen, R.; Huard, Z.; Meadows, B. T.; Pushpawela, B. G.; Sokoloff, M. D.; Sun, L.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Bloom, P. C.; Ford, W. T.; Gaz, A.; Nauenberg, U.; Smith, J. G.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Ayad, R.; Toki, W. H.] Colorado State Univ, Ft Collins, CO 80523 USA. [Spaan, B.] Tech Univ, Fak Phys, D-44221 Dortmund, Germany. [Schwierz, R.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Bernard, D.; Verderi, M.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. 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[Lusiani, A.] Scuola Normale Superiore Pisa, I-56127 Pisa, Italy. [Pegna, D. Lopes; Olsen, J.; Smith, A. J. S.] Princeton Univ, Princeton, NJ 08544 USA. [Faccini, R.; Ferrarotto, F.; Ferroni, F.; Gaspero, M.; Gioi, L. Li; Piredda, G.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Faccini, R.; Ferroni, F.; Gaspero, M.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Buenger, C.; Gruenberg, O.; Hartmann, T.; Leddig, T.; Voss, C.; Waldi, R.] Univ Rostock, D-18051 Rostock, Germany. [Adye, T.; Olaiya, E. O.; Wilson, F. F.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Emery, S.; de Monchenault, G. Hamel; Vasseur, G.; Yeche, Ch.] CEA, Ctr Saclay, SPP, Irfu, F-91191 Gif Sur Yvette, France. [Anulli, F.; Aston, D.; Bard, D. J.; Benitez, J. F.; Cartaro, C.; Convery, M. R.; Dorfan, J.; Dubois-Felsmann, G. P.; Dunwoodie, W.; Ebert, M.; Field, R. C.; Fulsom, B. G.; Gabareen, A. M.; Graham, M. T.; Hast, C.; Innes, W. R.; Kim, P.; Kocian, M. L.; Leith, D. W. G. S.; Lewis, P.; Lindemann, D.; Lindquist, B.; Luitz, S.; Luth, V.; Lynch, H. L.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Nelson, S.; Perl, M.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Salnikov, A. A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wagner, A. P.; Wang, W. F.; Wisniewski, W. J.; Wittgen, M.; Wright, D. H.; Wulsin, H. W.; Ziegler, V.] SLAC, Natl Accelerator Lab, Stanford, CA 94309 USA. [Park, W.; Purohit, M. V.; White, R. M.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Miyashita, T. S.; Puccio, E. M. T.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.] SUNY Albany, Albany, NY 12222 USA. [Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Ruland, A. M.; Schwitters, R. F.; Wray, B. C.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; De Mori, F.; Filippi, A.; Gamba, D.; Zambito, S.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; De Mori, F.; Gamba, D.; Zambito, S.] Univ Turin, Dipartimento Fis, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartmento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.; Villanueva-Perez, P.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Ahmed, H.; Albert, J.; Banerjee, Sw.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. RP Lees, JP (reprint author), Univ Savoie, CNRS, IN2P3, Lab Annecy Le Vieux Phys Particules, F-74941 Annecy Le Vieux, France. RI Morandin, Mauro/A-3308-2016; Lusiani, Alberto/A-3329-2016; Di Lodovico, Francesca/L-9109-2016; Calcaterra, Alessandro/P-5260-2015; Frey, Raymond/E-2830-2016; Patrignani, Claudia/C-5223-2009; Lo Vetere, Maurizio/J-5049-2012; Lusiani, Alberto/N-2976-2015; Monge, Maria Roberta/G-9127-2012; Forti, Francesco/H-3035-2011; Oyanguren, Arantza/K-6454-2014; Luppi, Eleonora/A-4902-2015; White, Ryan/E-2979-2015; Kravchenko, Evgeniy/F-5457-2015; Calabrese, Roberto/G-4405-2015; Martinez Vidal, F*/L-7563-2014; Kolomensky, Yury/I-3510-2015 OI Morandin, Mauro/0000-0003-4708-4240; Lusiani, Alberto/0000-0002-6876-3288; Di Lodovico, Francesca/0000-0003-3952-2175; Calcaterra, Alessandro/0000-0003-2670-4826; Frey, Raymond/0000-0003-0341-2636; Patrignani, Claudia/0000-0002-5882-1747; Lo Vetere, Maurizio/0000-0002-6520-4480; Lusiani, Alberto/0000-0002-6876-3288; Monge, Maria Roberta/0000-0003-1633-3195; Forti, Francesco/0000-0001-6535-7965; Oyanguren, Arantza/0000-0002-8240-7300; Luppi, Eleonora/0000-0002-1072-5633; White, Ryan/0000-0003-3589-5900; Calabrese, Roberto/0000-0002-1354-5400; Martinez Vidal, F*/0000-0001-6841-6035; Kolomensky, Yury/0000-0001-8496-9975 FU U.S. Department of Energy; National Science Foundation; Natural Sciences and Engineering Research Council (Canada); Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany); Istituto Nazionale di Fisica Nucleare (Italy); Foundation for Fundamental Research on Matter (Netherlands) FX We are grateful for the extraordinary contributions of our PEP-II colleagues in achieving the excellent luminosity and machine conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and the kind hospitality extended to them. This work is supported by the U.S. Department of Energy and National Science Foundation, the Natural Sciences and Engineering Research Council (Canada), the Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France), the Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany), the Istituto Nazionale di Fisica Nucleare (Italy), the Foundation for Fundamental Research on Matter (Netherlands), the Research Council of Norway, the Ministry of Education and Science of the Russian Federation, Ministerio de Ciencia e Innovacion (Spain), and the Science and Technology Facilities Council (United Kingdom). Individuals have received support from the Marie-Curie IEF program (European Union) and the A. P. Sloan Foundation (U. S.). NR 27 TC 18 Z9 21 U1 0 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 28 PY 2013 VL 88 IS 7 AR 072009 DI 10.1103/PhysRevD.88.072009 PG 12 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 241JE UT WOS:000326161900001 ER PT J AU Zheng, JX Wang, L Katsiev, K Losovyj, Y Vescovo, E Goodman, DW Dowben, PA Lu, J Mei, WN AF Zheng, Jiaxin Wang, Lu Katsiev, Khabibulakh Losovyj, Yaroslav Vescovo, Elio Goodman, D. Wayne Dowben, Peter A. Lu, Jing Mei, Wai-Ning TI Adsorption configurations of carbon monoxide on gold monolayer supported by graphene or monolayer hexagonal boron nitride: a first-principles study SO EUROPEAN PHYSICAL JOURNAL B LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; AU NANOPARTICLES; BAND-STRUCTURE; BASIS-SET; OXIDATION; MECHANISM; SURFACES; CLUSTERS; SYSTEMS AB Using density functional theory with a semiempirical van der Waals approach proposed by Grimme, the adsorption behavior of carbon monoxide on a gold monolayer supported by graphene or monolayer hexagonal boron nitride has been investigated. Based on the changes in the Dirac cone of graphene and a Bader charge analysis, we observe that the Au(111) monolayer gains a small charge from graphene and monolayer h-BN. The adsorbed CO molecule adopts similar adsorption configurations on Au(111)/graphene and Au(111)/h-BN with Au-C distance 2.17-2.50 angstrom and Au-C-O angle of 123.9 degrees-139.6 degrees. Moreover, we found that for low CO coverages, bonding to the gold surface is surprisingly energy-favorable. Yet the CO adsorption binding energy diminishes at high coverage due to the repulsive van der Waals interactions between CO molecules. C1 [Zheng, Jiaxin; Wang, Lu; Mei, Wai-Ning] Univ Nebraska, Dept Phys, Omaha, NE 68182 USA. [Zheng, Jiaxin; Lu, Jing] Peking Univ, State Key Lab Mesoscop Phys, Beijing 100871, Peoples R China. [Zheng, Jiaxin; Lu, Jing] Peking Univ, Dept Phys, Beijing 100871, Peoples R China. [Katsiev, Khabibulakh; Goodman, D. Wayne] Texas A&M Univ, Dept Chem, College Stn, TX 77842 USA. [Losovyj, Yaroslav] Louisiana State Univ, J Bennett Johnston Sr Ctr Adv Microstruct & Devic, Baton Rouge, LA 70806 USA. [Losovyj, Yaroslav; Dowben, Peter A.] Univ Nebraska, Nebraska Ctr Mat & Nanosci, Dept Phys & Astron, Lincoln, NE 68588 USA. [Vescovo, Elio] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. RP Zheng, JX (reprint author), Univ Nebraska, Dept Phys, Omaha, NE 68182 USA. EM lukewl@gmail.com RI Wang, Lu/D-2528-2011; Lu, Jing/H-4248-2013 FU Nebraska Research Initiative; NSF [EPS-1010674]; DOE [DE-EE0003174]; Semiconductor Research Corporation, Division of Nanomanufacturing Sciences [2123.001]; Center for Atomic-Level Catalyst Design, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001058]; United States Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76CH00016]; Louisiana Board of Regents FX This work was supported by Nebraska Research Initiative, NSF EPS-1010674, DOE DE-EE0003174 and by the Semiconductor Research Corporation, Division of Nanomanufacturing Sciences, task ID 2123.001. The University of Nebraska Holland Computing Center provided the computational resources with the associated USCMS Tier-2 site at the University of Nebraska-Lincoln. Part of the experimental work was supported as part of the Center for Atomic-Level Catalyst Design, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number #DE-SC0001058. The NSLS is supported by the United States Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-76CH00016. The J. Bennett Johnston Sr. Center for Advanced Microstructures and Devices is supported by the Louisiana Board of Regents. The authors would like to acknowledge substantive discussions leading up to the paper with Nataliya Lozova, Ivan Yakovkin, and Axel Enders. NR 40 TC 1 Z9 1 U1 4 U2 50 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6028 EI 1434-6036 J9 EUR PHYS J B JI Eur. Phys. J. B PD OCT 28 PY 2013 VL 86 IS 10 AR 441 DI 10.1140/epjb/e2013-40171-7 PG 7 WC Physics, Condensed Matter SC Physics GA 244IU UT WOS:000326382200002 ER PT J AU Nomura, Y Varela, J Weinberg, SJ AF Nomura, Yasunori Varela, Jaime Weinberg, Sean J. TI Black holes or firewalls: A theory of horizons SO PHYSICAL REVIEW D LA English DT Article ID INFLATIONARY UNIVERSE; EVAPORATION; PERTURBATIONS; INFORMATION; CREATION; GRAVITY; ENTROPY AB We present a quantum theory of black hole (and other) horizons, in which the standard assumptions of complementarity are preserved without contradicting information theoretic considerations. After the scrambling time, the quantum mechanical structure of a black hole becomes that of an eternal black hole at the microscopic level. In particular, the stretched horizon degrees of freedom and the states entangled with them can be mapped into the near-horizon modes in the two exterior regions of an eternal black hole, whose mass is taken to be that of the evolving black hole at each moment. Salient features arising from this picture include (i) the number of degrees of freedom needed to describe a black hole is e(.A/2l2)P, where A is the area of the horizon; (ii) black hole states having smooth horizons, however, span only an e(A/4l2)P-dimensional subspace of the relevant e(A/2l2)P-dimensional Hilbert space; (iii) internal dynamics of the horizon is such that an infalling observer finds a smooth horizon with a probability of 1 if a state stays in this subspace. We identify the structure of local operators responsible for describing semiclassical physics in the exterior and interior spacetime regions and show that this structure avoids the arguments for firewalls-the horizon can keep being smooth throughout the evolution. We discuss the fate of infalling observers under various circumstances, especially when the observers manipulate degrees of freedom before entering the horizon, and we find that an observer can never see a firewall by making a measurement on early Hawking radiation. We also consider the presented framework from the viewpoint of an infalling reference frame and argue that Minkowski-like vacua are not unique. In particular, the number of true Minkowski vacua is infinite, although the label discriminating these vacua cannot be accessed in usual nongravitational quantum field theory. An application of the framework to de Sitter horizons is also discussed. C1 [Nomura, Yasunori] Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Dept Phys, Berkeley, CA 94720 USA. Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Nomura, Y (reprint author), Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Dept Phys, Berkeley, CA 94720 USA. OI Nomura, Yasunori/0000-0002-1497-1479 FU Office of Science, Office of High Energy and Nuclear Physics, of the U. S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [PHY-1214644] FX We thank Juan Maldacena for useful conversations. This work was supported in part by the Director, Office of Science, Office of High Energy and Nuclear Physics, of the U. S. Department of Energy under Contract No. DE-AC02-05CH11231, and in part by the National Science Foundation under Grant No. PHY-1214644. NR 47 TC 8 Z9 8 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD OCT 28 PY 2013 VL 88 IS 8 AR 084052 DI 10.1103/PhysRevD.88.084052 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 241JK UT WOS:000326162700010 ER PT J AU Barai, P Nukala, PKVV Alava, MJ Zapperi, S AF Barai, Pallab Nukala, Phani K. V. V. Alava, Mikko J. Zapperi, Stefano TI Role of the sample thickness in planar crack propagation SO PHYSICAL REVIEW E LA English DT Article ID HETEROGENEOUS MATERIALS; FUSE NETWORKS; FRACTURE; DYNAMICS; STRENGTH; MODELS; MEDIA; FRONT; PAPER; BLOCK AB We study the effect of the sample thickness in planar crack front propagation in a disordered elastic medium using the random fuse model. We employ different loading conditions and we test their stability with respect to crack growth. We show that the thickness induces characteristic lengths in the stress enhancement factor in front of the crack and in the stress transfer function parallel to the crack. This is reflected by a thickness-dependent crossover scale in the crack front morphology that goes from from multiscaling to self-affine with exponents, in agreement with line depinning models and experiments. Finally, we compute the distribution of crack avalanches, which is shown to depend on the thickness and the loading mode. C1 [Barai, Pallab] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. [Nukala, Phani K. V. V.] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. [Alava, Mikko J.] Aalto Univ, Dept Appl Phys, COMP Ctr Excellence, FIN-00076 Espoo, Finland. [Zapperi, Stefano] IENI, CNR, I-20125 Milan, Italy. [Zapperi, Stefano] ISI Fdn, I-10126 Turin, Italy. RP Barai, P (reprint author), Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. RI Alava, Mikko/G-2202-2013; Zapperi, Stefano/C-9473-2009 OI Alava, Mikko/0000-0001-9249-5079; Zapperi, Stefano/0000-0001-5692-5465 FU European Research Council; Aalto University School of Science; Aalto Science Institute; Academy of Finland through the COMP Center of Excellence; Mathematical, Information, and Computational Sciences Division, Office of Advanced Scientific Computing Research, U.S. Department of Energy [DE-AC05-00OR22725]; UTBattelle, LLC FX S.Z. is supported by the European Research Council Advanced Grant 2011, SIZEFFECTS, and is grateful for the support of the visiting professor program of Aalto University School of Science and the Aalto Science Institute. M.J.A. is grateful for support from the Academy of Finland through the COMP Center of Excellence. P.K.V.V.N. acknowledges support received from the Mathematical, Information, and Computational Sciences Division, Office of Advanced Scientific Computing Research, U.S. Department of Energy, under Contract No. DE-AC05-00OR22725 with UTBattelle, LLC. NR 41 TC 3 Z9 3 U1 0 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD OCT 28 PY 2013 VL 88 IS 4 AR 042411 DI 10.1103/PhysRevE.88.042411 PG 7 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 241JU UT WOS:000326163800008 PM 24229193 ER PT J AU Bzdak, A Skokov, V AF Bzdak, Adam Skokov, Vladimir TI Decisive Test of Color Coherence in Proton-Nucleus Collisions at the LHC SO PHYSICAL REVIEW LETTERS LA English DT Article ID HIGH-ENERGY; GLUON PRODUCTION; SCATTERING; GLASS; QCD AB Proton-nucleus collisions (p + A) at LHC energies provide a rigorous test of color glass condensate (CGC), a model proposed to describe the high energy limit of quantum chromodynamics. In the CGC the average multiplicity of charged particles at midrapidity in p + A collisions depends logarithmically on the number of participants, N-part. In contrast, the wounded nucleon model of independent nucleon-nucleon scatterings, verified at RHIC energies, predicts that multiplicity in p + A depends linearly on N-part. We argue that the dependence of mean multiplicity on N-part in p + A collisions at LHC energies can single out a model of particle production, thus offering a stringent test of the CGC and the wounded nucleon model. Based on this observation we propose a novel experimental test of color coherence in p + A collisions. C1 [Bzdak, Adam] Brookhaven Natl Lab, RIKEN, BNL Res Ctr, Upton, NY 11973 USA. [Skokov, Vladimir] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Skokov, Vladimir] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA. RP Bzdak, A (reprint author), Brookhaven Natl Lab, RIKEN, BNL Res Ctr, Upton, NY 11973 USA. EM ABzdak@bnl.gov; VSkokov@quark.phy.bnl.gov OI Skokov, Vladimir/0000-0001-7619-1796 FU RIKEN-BNL Research Center; U.S. Department of Energy [DE-AC02-98CH10886] FX We thank Adrian Dumitru, Larry McLerran, and Al Mueller for valuable comments and in-depth discussions. We acknowledge Bjoern Schenke for providing us with the IP-Glasma results. Comments by Robert Pisarski, Bjoern Schenke, Paul Sorensen, and Raju Venugopalan are acknowledged. A. B. is supported through the RIKEN-BNL Research Center. V. S. is supported by the U.S. Department of Energy under Contract No. DE-AC02-98CH10886. NR 30 TC 14 Z9 14 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 28 PY 2013 VL 111 IS 18 AR 182301 DI 10.1103/PhysRevLett.111.182301 PG 5 WC Physics, Multidisciplinary SC Physics GA 241KD UT WOS:000326164800004 PM 24237511 ER PT J AU Firmo, IA Lederer, S Lupien, C Mackenzie, AP Davis, JC Kivelson, SA AF Firmo, I. A. Lederer, S. Lupien, C. Mackenzie, A. P. Davis, J. C. Kivelson, S. A. TI Evidence from tunneling spectroscopy for a quasi-one-dimensional origin of superconductivity in Sr2RuO4 SO PHYSICAL REVIEW B LA English DT Article ID SPIN-TRIPLET SUPERCONDUCTIVITY; PARTICLE INTERFERENCE; MAGNETIC-FIELDS; FERMI-SURFACE; GAP STRUCTURE; CONDUCTIVITY; FLUCTUATION; DEPENDENCE; SCATTERING; SYMMETRY AB To establish the mechanism of unconventional superconductivity in Sr2RuO4, a prerequisite is direct information concerning the momentum-space structure of the energy gaps Delta(i) (k), and in particular whether the pairing strength is stronger ("dominant") on the quasi-one-dimensional (alpha and beta) or on the quasi-two-dimensional (gamma) Fermi surfaces. We present scanning tunneling microscopy measurements of the density of states spectra in the superconducting state of Sr2RuO4 for 0.1T(c) < T < T-c and analyze them along with published thermodynamic data using a simple phenomenological model. We show that our observation of a single superconducting gap scale with maximum value 2 Delta approximate to 5T(c) along with a spectral shape indicative of line nodes is consistent, within a weak-coupling model, with magnetically mediated odd-parity superconductivity generated by dominant, near-nodal, Cooper pairing on the alpha and beta bands. C1 [Firmo, I. A.; Davis, J. C.] Cornell Univ, Dept Phys, Solid State Phys Lab, Ithaca, NY 14853 USA. [Firmo, I. A.; Davis, J. C.] Brookhaven Natl Lab, CMPMS Dept, Upton, NY 11973 USA. [Lederer, S.; Kivelson, S. A.] Stanford Univ, Dept Phys, Stanford, CA 96305 USA. [Lupien, C.] Univ Sherbrooke, Dept Phys, Sherbrooke, PQ J1K 2R1, Canada. [Lupien, C.] Univ Sherbrooke, RQMP, Sherbrooke, PQ J1K 2R1, Canada. [Mackenzie, A. P.; Davis, J. C.] Univ St Andrews, Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland. [Mackenzie, A. P.] Max Planck Inst Chem Phys Solids, D-01187 Dresden, Germany. [Davis, J. C.] Cornell Univ, Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA. RP Firmo, IA (reprint author), Cornell Univ, Dept Phys, Solid State Phys Lab, Ithaca, NY 14853 USA. RI Mackenzie, Andrew/K-6742-2015 FU Office of Naval Research [N00014-13-1-0047]; Royal Society-Wolfson Research Merit Award; EPSRC; Fundacao para a Ciencia e a Tecnologia, Portugal [SFRH/BD/60952/2009]; [DE-AC02-76SF00515] FX We especially acknowledge and thank Y. Maeno for access to his high-quality Sr2RuO4 crystals and for many constructive comments. We thank M. Aprili, S.-B. Chung, A. Damascelli, F. Mark Fischer, E.-A. Kim, I. Mazin, S. Raghu, Jean-Philippe Reid, T. M. Rice, and A. M. Rost for helpful discussions and communications. Studies at Cornell University were supported by the Office of Naval Research under Award N00014-13-1-0047, and at Stanford under DE-AC02-76SF00515. A. P. M. acknowledges the receipt of a Royal Society-Wolfson Research Merit Award and the support of EPSRC through the Programme Grant "Topological Protection and Non-Equilibrium States in Correlated Electron Systems". I. A. F. acknowledges support from Fundacao para a Ciencia e a Tecnologia, Portugal under Fellowship No. SFRH/BD/60952/2009. C. L., I. A. F., and S. L. carried out the spectroscopic imaging STM experiments plus the data preparation and analysis; Y. M. synthesized and characterized the samples; A. P. M., J.C.D., and S. A. K. supervised the project, and wrote the paper with key contributions from S. L. and I. A. F. The manuscript reflects contribution and ideas of all authors. NR 63 TC 20 Z9 20 U1 2 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 28 PY 2013 VL 88 IS 13 AR 134521 DI 10.1103/PhysRevB.88.134521 PG 10 WC Physics, Condensed Matter SC Physics GA 241ID UT WOS:000326159000004 ER PT J AU Lv, B Zhu, XY Lorenz, B Wei, FY Xue, YY Yin, ZP Kotliar, G Chu, CW AF Lv, B. Zhu, X. Y. Lorenz, B. Wei, F. Y. Xue, Y. Y. Yin, Z. P. Kotliar, G. Chu, C. W. TI Superconductivity in the Mn5Si3-type Zr5Sb3 system SO PHYSICAL REVIEW B LA English DT Article ID INTERSTITIAL CHEMISTRY; PHASES AB We report the discovery of superconductivity at 2.3 K in Zr5Sb3, the first superconducting member in the large compound family of the Mn5Si3-type structure. Transport, magnetic, and calorimetric measurements clearly demonstrate bulk superconductivity for Zr5Sb3 and suggest it to be a possible phonon-mediated BCS superconductor with a relatively large density of states at the Fermi level associated with the d electrons of Zr and substantially larger electron-phonon coupling compared to the Sn counterpart compound Zr5Sn3 from band structure calculations. More superconductors with even higher transition temperatures are expected to be found in this family of compounds. C1 [Lv, B.; Zhu, X. Y.; Lorenz, B.; Wei, F. Y.; Xue, Y. Y.; Chu, C. W.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Lv, B.; Zhu, X. Y.; Lorenz, B.; Wei, F. Y.; Xue, Y. Y.; Chu, C. W.] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Yin, Z. P.; Kotliar, G.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Chu, C. W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Lv, B (reprint author), Univ Houston, Dept Phys, Houston, TX 77204 USA. EM blv@uh.edu; cwchu@uh.edu FU US Air Force Office of Scientific Research (AFOSR) [FA9550-09-1-0656]; T.L.L. Temple Foundation; John J. and Rebecca Moores Endowment; State of Texas through the Texas Center for Superconductivity at the University of Houston; US Air Force Office of Scientific Research Multidisciplinary University Research Initiative program FX The work in Houston is supported in part by US Air Force Office of Scientific Research (AFOSR) Grant No. FA9550-09-1-0656, the T.L.L. Temple Foundation, the John J. and Rebecca Moores Endowment, and the State of Texas through the Texas Center for Superconductivity at the University of Houston. Z.P.Y. and G. K. are supported by the US Air Force Office of Scientific Research Multidisciplinary University Research Initiative program. NR 14 TC 2 Z9 2 U1 5 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 28 PY 2013 VL 88 IS 13 AR 134520 DI 10.1103/PhysRevB.88.134520 PG 5 WC Physics, Condensed Matter SC Physics GA 241ID UT WOS:000326159000003 ER PT J AU Mayes, RL Allen, MS Kammer, DC AF Mayes, Randy L. Allen, Mathew S. Kammer, Daniel C. TI Correcting indefinite mass matrices due to substructure uncoupling SO JOURNAL OF SOUND AND VIBRATION LA English DT Article AB The transmission simulator method of experimental dynamic substructuring captures the interface forces and motions through a fixture called a transmission simulator. The transmission simulator method avoids the need to measure connection point rotations, facilitates substructuring for systems with continuous connections and enriches the modal basis of the substructure model. To use this approach, one first attaches the transmission simulator to the experimental substructure and then measures the free modes of the assembly. A finite element model of the transmission simulator is then used to subtract the transmission simulator and to couple the experimental substructure to the assembly of interest. Unfortunately, in several cases the process of subtracting the transmission simulator has caused the mass matrix for the experimental substructure to become indefinite, making the substructure model difficult or impossible to use and potentially leading to erroneous results. The authors previously developed metrics that could be used to identify which modes of the experimental model led to the indefinite mass matrix. This work presents a method that utilizes those metrics with a sensitivity analysis to adjust the transmission simulator mass matrix so that the subtraction does not produce an indefinite mass matrix. A second method is presented in which the mass matrix is made positive definite by coupling additional mass to the substructure. The methods are evaluated using both numerical and experimental test cases, showing promising results. (c) 2013 Elsevier Ltd. All rights reserved. C1 [Mayes, Randy L.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Allen, Mathew S.; Kammer, Daniel C.] Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. RP Allen, MS (reprint author), Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. EM rlmayes@sandia.gov; msallen@engr.wisc.edu; kammer@engr.wisc.edu FU Sandia National Laboratories; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by, and some of this work was performed at Sandia National Laboratories. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 18 TC 4 Z9 4 U1 0 U2 5 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-460X J9 J SOUND VIB JI J. Sound Vibr. PD OCT 28 PY 2013 VL 332 IS 22 BP 5856 EP 5866 DI 10.1016/j.jsv.2013.05.025 PG 11 WC Acoustics; Engineering, Mechanical; Mechanics SC Acoustics; Engineering; Mechanics GA 204JG UT WOS:000323361000013 ER PT J AU Lai, C Sun, X AF Lai, C. Sun, X. TI Predicting flaw-induced resonance spectrum shift with theoretical perturbation analysis SO JOURNAL OF SOUND AND VIBRATION LA English DT Article ID DAMAGE DETECTION; PLATES AB Resonance inspection is an emerging non-destructive evaluation (NDE) technique used by the automotive casting industry which uses the resonance spectra differences between the good part population and the flawed parts to identify anomalous parts. It was previously established that finite-element (FE)-based modal analysis can be used to predict the resonance spectrum for an engineering scale part with relatively good accuracy. However, FE-based simulations can be time consuming in examining the spectrum shifts induced by all possible structural flaws. This paper aims at developing a computationally efficient perturbation technique to quantify the frequency shifts induced by small structural flaws, based on the FE simulated resonance spectrum for the perfect part. A generic automotive connecting rod is used as the example part for our study. The results demonstrate that the linear perturbation theory provides a very promising way in predicting frequency changes induced by small structural flaws. As the flaw size increases, the discrepancy between the perturbation analysis and the actual FE simulation results increases due to nonlinearity, yet the perturbation analysis is still able to predict the right trend in frequency shift. Published by Elsevier Ltd. C1 [Lai, C.; Sun, X.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Sun, X (reprint author), 902 Battelle Blvd,POB 999,MSIN K7-90, Richland, WA 99352 USA. EM xin.sun@pnl.gov FU United States Department of Energy [DE-ACO5-76RL01830]; EED LDRD program at the Pacific Northwest National Laboratory FX Pacific Northwest National Laboratory is operated by Battelle for the United States Department of Energy under Contract DE-ACO5-76RL01830. This study is partially supported by the EED LDRD program at the Pacific Northwest National Laboratory. NR 19 TC 1 Z9 1 U1 1 U2 5 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-460X J9 J SOUND VIB JI J. Sound Vibr. PD OCT 28 PY 2013 VL 332 IS 22 BP 5953 EP 5964 DI 10.1016/j.jsv.2013.05.024 PG 12 WC Acoustics; Engineering, Mechanical; Mechanics SC Acoustics; Engineering; Mechanics GA 204JG UT WOS:000323361000020 ER PT J AU Chorin, AJ Morzfeld, M AF Chorin, Alexandre J. Morzfeld, Matthias TI Conditions for successful data assimilation SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article AB [1] We show, using idealized models, that numerical data assimilation can be successful only if an effective dimension of the problem is not excessive. This effective dimension depends on the noise in the model and the data, and in physically reasonable problems, it can be moderate even when the number of variables is huge. We then analyze several data assimilation algorithms, including particle filters and variational methods. We show that well-designed particle filters can solve most of those data assimilation problems that can be solved in principle and compare the conditions under which variational methods can succeed to the conditions required of particle filters. We also discuss the limitations of our analysis. C1 [Chorin, Alexandre J.; Morzfeld, Matthias] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. [Chorin, Alexandre J.; Morzfeld, Matthias] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Morzfeld, M (reprint author), Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM mmo@math.lbl.gov FU Office of Science, Computational and Technology Research, U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [DMS-1217065] FX We thank P. Bickel of UC Berkeley for many interesting discussions, for making our thoughts more rigorous (where possible), and for helping us recognize the limitations of our analysis. We thank R. Miller of Oregon State University for very helpful discussions and help with the literature. We thank J. Weare for an interesting discussion. This work was supported in part by the Director, Office of Science, Computational and Technology Research, U.S. Department of Energy under contract DE-AC02-05CH11231 and by the National Science Foundation under grant DMS-1217065. NR 45 TC 7 Z9 7 U1 0 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 27 PY 2013 VL 118 IS 20 BP 11522 EP 11533 DI 10.1002/2013JD019838 PG 12 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA V45WS UT WOS:000209847300004 ER PT J AU Davies, L Jakob, C May, P Kumar, VV Xie, S AF Davies, L. Jakob, C. May, P. Kumar, V. V. Xie, S. TI Relationships between the large-scale atmosphere and the small-scale convective state for Darwin, Australia SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article AB [1] A persistent problem for numerical weather and climate models is the representation of tropical convective precipitation which for the most part occurs on spatial and temporal scales too small and too short to be explicitly resolved. Given that model parameterizations represent this subgrid convection as a function of the large-scale atmospheric state, an understanding of the strongest relationships between the two scales is needed. This study introduces a method to create two concurrent long-term data sets that describe both the large-scale atmosphere and the characteristics of the small-scale convection. Important relationships between these two scales are then investigated. It is found that convective precipitation, through convective precipitation area, has the strongest relationship with dynamical variables such as moisture convergence and vertical velocity at midlevels. The magnitude of the fluctuations of convective strength about the mean is found to be anticorrelated with the strength of the large-scale variables, indicating a more stochastic behavior of tropical convection in weakly than strongly forced regimes, respectively. Atmospheric stability related variables are not found to be positively related to either convective precipitation area or convective precipitation intensity, which is often an assumption made in convective parameterization. On the contrary, in a more unstable atmosphere, there is lower convective precipitation. C1 [Davies, L.] Monash Univ, Sch Math, Melbourne, Vic, Australia. [Jakob, C.] Monash Univ, ARC Ctr Excellence Climate Syst Sci, Melbourne, Vic, Australia. [May, P.; Kumar, V. V.] Bur Meteorol, Ctr Australian Weather & Climate Res, Melbourne, Vic, Australia. [Xie, S.] Lawrence Livermore Natl Lab, Atmospher Sci Div, Livermore, CA USA. RP Davies, L (reprint author), Univ Melbourne, Sch Earth Sci, Melbourne, Vic 3010, Australia. EM laura.davies@unimelb.edu.au FU Office of Science (BER), U.S. Department of Energy [DE-SC0002731] FX Davies and Jakob are supported by the Office of Science (BER), U.S. Department of Energy under grant DE-SC0002731. NR 45 TC 20 Z9 20 U1 0 U2 0 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 27 PY 2013 VL 118 IS 20 BP 11534 EP 11545 DI 10.1002/jgrd.50645 PG 12 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA V45WS UT WOS:000209847300005 ER PT J AU Matsui, H Koike, M Takegawa, N Kondo, Y Takami, A Takamura, T Yoon, S Kim, SW Lim, HC Fast, JD AF Matsui, H. Koike, M. Takegawa, N. Kondo, Y. Takami, A. Takamura, T. Yoon, S. Kim, S. -W. Lim, H. -C. Fast, J. D. TI Spatial and temporal variations of new particle formation in East Asia using an NPF-explicit WRF-chem model: North-south contrast in new particle formation frequency SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article AB [1] A recently developed new particle formation (NPF)-explicit version of the Weather Research and Forecasting Chemistry (WRF-chem) model can explicitly calculate the growth and sink of nucleated clusters with 20 aerosol size bins from 1 nm to 10 mu m in diameter. In this study, the model was used to investigate spatial and temporal variations in NPF event frequency and the concentrations of aerosols (condensation nuclei, CN) and cloud condensation nuclei (CCN) within the boundary layer in East Asia in spring 2009. We found a distinct north-south contrast in the NPF frequency and mechanism in East Asia. NPF occurred mainly during limited periods over certain regions between 30 degrees and 45 degrees N (northeast China, Korea, and Japan, including regions around the active volcanoes Miyakejima and Sakurajima). In these latitudes, NPF was suppressed by high concentrations of preexisting particles under stagnant air conditions associated with high-pressure systems, although nucleation occurred more extensively during most of the simulation period. In contrast, south of 30 degrees N, nucleation and NPF were both infrequent because of low SO2 emissions and H2SO4 concentrations. The period-averaged NPF frequency at 30 degrees-45 degrees N was three times that at 20 degrees-30 degrees N. This north-south contrast in NPF frequency was validated by surface measurements in outflow regions of East Asia. The simulated period-and domain-averaged contribution of secondary particles was estimated to be 44% for CN (>10 nm) and 26% for CCN at a supersaturation of 1.0%, though the contribution was highly sensitive to the amount and size distribution of primary aerosol emissions and the rate coefficient of the nucleation parameterization. C1 [Matsui, H.; Koike, M.; Kondo, Y.] Univ Tokyo, Grad Sch Sci, Dept Earth & Planetary Sci, Tokyo, Japan. [Matsui, H.] Japan Agcy Marine Earth Sci & Technol, Res Inst Global Change, Kanagawa, Japan. [Takegawa, N.] Univ Tokyo, Res Ctr Adv Sci & Technol, Tokyo, Japan. [Takami, A.] Natl Inst Environm Studies, Tsukuba, Ibaraki, Japan. [Takamura, T.] Chiba Univ, Ctr Environm Remote Sensing, Chiba, Japan. [Yoon, S.; Kim, S. -W.] Seoul Natl Univ, Sch Earth & Environm Sci, Seoul, South Korea. [Lim, H. -C.] Korea Meteorol Adm, Climate Sci Bur, Korea Global Atmospher Watch Ctr, Taean Gun, South Korea. [Fast, J. D.] Pacific Northwest Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. RP Matsui, H (reprint author), Japan Agcy Marine Earth Sci & Technol, Res Inst Global Change, Kanazawa Ku, 3173-25 Showa Machi, Yokohama, Kanagawa 2360001, Japan. EM matsui@jamstec.go.jp RI Kondo, Yutaka/D-1459-2012 FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT); Japan Science and Technology Agency (JST); Japanese Ministry of the Environment [A-0803, A-1101, B-1006]; Alliance for Global Sustainability (AGS) project, University of Tokyo; U.S. Department of Energy's (DoE) Atmospheric System Research program [DE-AC06-76RLO 1830]; School of Earth and Environmental Sciences, Seoul National University; Korea Meteorological Administration Research and Development Program [CATER 2012-3020] FX This work was supported by the Ministry of Education, Culture, Sports, Science, and Technology (MEXT), the strategic international cooperative program of the Japan Science and Technology Agency (JST), the global environment research fund of the Japanese Ministry of the Environment (A-0803, A-1101, and B-1006), and by the Alliance for Global Sustainability (AGS) project, University of Tokyo. This study was conducted as a part of the Mega-Cities: Asia Task under the framework of the International Global Atmospheric Chemistry (IGAC) project. Support for MOSAIC and WRF-Chem was provided by the U.S. Department of Energy's (DoE) Atmospheric System Research program under Contract DE-AC06-76RLO 1830 at PNNL. PNNL is operated for the U.S. DoE by the Battelle Memorial Institute. For a part of the simulations, we used the HA8000 computer system operated by the Supercomputing Division, Information Technology Center, University of Tokyo. S.-C. Yoon and S.-W. Kim were supported by the BK21 program of the School of Earth and Environmental Sciences, Seoul National University, and by the Korea Meteorological Administration Research and Development Program under Grant CATER 2012-3020. NR 118 TC 14 Z9 14 U1 4 U2 31 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 27 PY 2013 VL 118 IS 20 BP 11647 EP 11663 DI 10.1002/jgrd.50821 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA V45WS UT WOS:000209847300014 ER PT J AU Song, C Gyawali, M Zaveri, RA Shilling, JE Arnott, WP AF Song, Chen Gyawali, Madhu Zaveri, Rahul A. Shilling, John E. Arnott, W. Patrick TI Light absorption by secondary organic aerosol from alpha-pinene: Effects of oxidants, seed aerosol acidity, and relative humidity SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article AB [1] It is well known that light absorption from dust and black carbon aerosols has a warming effect on climate while light scattering from sulfate, nitrate, and sea salt aerosols has a cooling effect. However, there are large uncertainties associated with light absorption and scattering by different types of organic aerosols, especially in the near-UV and UV spectral regions. In this paper, we present the results from a systematic laboratory study focused on measuring light absorption by secondary organic aerosols (SOAs) generated from dark alpha-pinene + O-3 and alpha-pinene + NOx + O-3 systems in the presence of neutral and acidic sulfate seed aerosols. Light absorption was monitored using photoacoustic spectrometers at four different wavelengths: 355, 405, 532, and 870 nm. Significant light absorption at 355 and 405 nm was observed for the SOA formed from alpha-pinene + O-3 + NO3 system only in the presence of highly acidic sulfate seed aerosols under dry conditions. In contrast, no absorption was observed when the relative humidity was elevated to greater than 27% or in the presence of neutral sulfate seed aerosols. Organic nitrates in the SOA formed in the presence of neutral sulfate seed aerosols were found to be nonabsorbing, while the light-absorbing compounds are speculated to be aldol condensation oligomers with nitroxy organosulfate groups that are formed in highly acidic sulfate aerosols. Overall, these results suggest that dark alpha-pinene + O-3 and alpha-pinene + NOx + O-3 systems do not form light-absorbing SOA under typical atmospheric conditions. C1 [Song, Chen; Zaveri, Rahul A.; Shilling, John E.] Pacific Northwest Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Gyawali, Madhu; Arnott, W. Patrick] Univ Nevada Reno, Dept Phys, Nevada Syst Higher Educ, Reno, NV USA. RP Song, C (reprint author), RJ Reynolds Tobacco Co, 401 N Main St, Winston Salem, NC 27101 USA. EM songc@rjrt.com; rahul.zaveri@pnnl.gov OI Zaveri, Rahul/0000-0001-9874-8807 FU U.S. Department of Energy's (DOE) Atmospheric System Research (ASR) program; Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility - DOE's Office of Biological and Environmental Research; U.S. Department of Energy [DE-AC06-76RLO1830] FX We thank Alexander Laskin (PNNL) for thoughtful suggestions. Funding for this research was provided by the U.S. Department of Energy's (DOE) Atmospheric System Research (ASR) program and by the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at PNNL. Pacific Northwest National Laboratory is operated for the U.S. Department of Energy by Battelle Memorial Institute under contract DE-AC06-76RLO1830. NR 75 TC 13 Z9 14 U1 1 U2 1 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 27 PY 2013 VL 118 IS 20 BP 11741 EP 11749 DI 10.1002/jgrd.50767 PG 9 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA V45WS UT WOS:000209847300020 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Clerbaux, B De Lentdecker, G Favart, L Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Selvaggi, M Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Jorge, LS Sznajder, A Manganote, EJT Pereira, AV Anjos, TS Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Marinho, F Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, J Wang, X Wang, Z Xiao, H Xu, M Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, S Wang, D Zhang, L Zou, W Avila, C Montoya, CAC Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Plestina, R Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Duric, S Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Assran, Y Kamel, AE Mahmoud, MA Mahrous, A Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Korpela, A Tuuva, T Besancon, M Choudhury, S Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Millischer, L Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Benhabib, L Bianchini, L Bluj, M Busson, P Charlot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Florent, A de Cassagnac, RG Haguenauer, M Mine, P Mironov, C Naranjo, I Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Veelken, C Zabi, A Agram, JL Andrea, J Bloch, D Bodin, D Brom, JM Chabert, EC Collard, C Conte, E Drouhin, F Fontaine, JC Gele, D Goerlach, U Goetzmann, C Juillot, P Le Bihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Brochet, S Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Sgandurra, L Sordini, V Tschudi, Y Vander Donckt, M Verdier, P Viret, S Tsamalaidze, Z Autermann, C Beranek, S 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Oberst, O Ott, J Quast, G Rabbertz, K Ratnikov, F Rocker, S Schilling, FP Schott, G Simonis, HJ Stober, FM Ulrich, R Wagner-Kuhr, J Wayand, S Weiler, T Zeise, M Anagnostou, G Daskalakis, G Geralis, T Kesisoglou, S Kyriakis, A Loukas, D Markou, A Markou, C Ntomari, E Gouskos, L Mertzimekis, TJ Panagiotou, A Saoulidou, N Stiliaris, E Aslanoglou, X Evangelou, I Flouris, G Foudas, C Kokkas, P Manthos, N Papadopoulos, I Paradas, E Bencze, G Hajdu, C Hidas, P Horvath, D Radics, B Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Molnar, J Palinkas, J Szillasi, Z Karancsi, J Raics, P Trocsanyi, ZL Ujvari, B Swain, SK Beri, SB Bhatnagar, V Dhingra, N Gupta, R Kaur, M Mehta, MZ Mittal, M Nishu, N Saini, LK Sharma, A Singh, JB Kumar, A Kumar, A Ahuja, S Bhardwaj, A Choudhary, BC Malhotra, S Naimuddin, M Ranjan, K Saxena, P Sharma, V Shivpuri, RK Banerjee, S Bhattacharya, S Chatterjee, K Dutta, S Gomber, B Jain, S Jain, S Khurana, R Modak, A Mukherjee, S Roy, D Sarkar, S 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CA CMS Collaboration TI Measurement of the W+W- cross section in pp collisions at and limits on anomalous WW gamma and WWZ couplings SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID GAUGE-BOSON COUPLINGS; PARTON DISTRIBUTIONS; ATLAS DETECTOR; ROOT-S=7 TEV; HIGGS-BOSON; LHC; SEARCH; LEP AB A measurement of W+W- production in pp collisions at is presented. The data were collected with the CMS detector at the LHC, and correspond to an integrated luminosity of 4.92 +/- 0.11 fb(-1). The W+W- candidates consist of two oppositely charged leptons, electrons or muons, accompanied by large missing transverse energy. The W+W- production cross section is measured to be 52.4 +/- 2.0 (stat.)+/- 4.5 (syst.)+/- 1.2 (lum.) pb. This measurement is consistent with the standard model prediction of 47.0 +/- 2.0 pb at next-to-leading order. Stringent limits on the WW gamma and WWZ anomalous triple gauge-boson couplings are set. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. 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[Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. 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T.; Montecassiano, F.; Passaseo, M.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bellan, P.; Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; D'Agnolo, R. T.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Fanelli, C.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Fanelli, C.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Dellacasa, G.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Casasso, S.; Costa, M.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Z. J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Trocniz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; d'Enterria, D.; Dabrowski, A.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hegner, B.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Magini, N.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Polese, G.; Quertenmont, L.; Racz, A.; Reece, W.; Rolandi, G.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Taroni, S.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Gunaydin, Y. O.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Mall, O.; Miceli, T.; Nelson, R.; Pellett, D.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Hanson, G.; Liu, H.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, San Diego, CA 92103 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kalavase, P.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Williams, G.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Pegna, D. Lopes; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Koybasi, O.; Kress, M.; Leonardo, N.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Wang, F.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Rose, K.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Jeong, C.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Anderson, M.; Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Friis, E.; Grogg, K. S.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Kaadze, K.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Loveless, R.; Mohapatra, A.; Mozer, M. U.; Ojalvo, I.; Pierro, G. A.; Ross, I.; Savin, A.; Smith, W. H.; Swanson, J.] Univ Wisconsin, Madison, WI 53706 USA. [Fabjan, C.; Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Assran, Y.] Suez Canal Univ, Suez, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Mahrous, A.] Helwan Univ, Cairo, Egypt. [Radi, A.] British Univ Egypt, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Arfaei, H.; Fahim, A.] Sharif Univ Technol, Tehran, Iran. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Martini, L.] Univ Siena, I-53100 Siena, Italy. [Heredia-de La Cruz, I.] Univ Michoacana, Morelia, Michoacan, Mexico. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, G.] Scuola Normale Super Pisa, Ist Nazl Fis Nucl, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Ozkorucuklu, S.] Suleyman Demirel Univ, TR-32200 Isparta, Turkey. [Sonmez, N.] Ege Univ, Izmir, Turkey. [Bahtiyar, H.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Gunaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, TR-46050 Kahramanmaras, Turkey. [Belyaev, A.; Basso, L.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. [Adzic, P.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Andreev, Vladimir/M-8665-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Ragazzi, Stefano/D-2463-2009; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Benussi, Luigi/O-9684-2014; Russ, James/P-3092-2014; Leonidov, Andrey/P-3197-2014; vilar, rocio/P-8480-2014; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Cerrada, Marcos/J-6934-2014; Venturi, Andrea/J-1877-2012; Calderon, Alicia/K-3658-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Wolszczak, Weronika/N-3113-2013; Montanari, Alessandro/J-2420-2012; Gribushin, Andrei/J-4225-2012; Petrushanko, Sergey/D-6880-2012; Marlow, Daniel/C-9132-2014; de Jesus Damiao, Dilson/G-6218-2012; Janssen, Xavier/E-1915-2013; Novaes, Sergio/D-3532-2012; Bartalini, Paolo/E-2512-2014; Ligabue, Franco/F-3432-2014; Wulz, Claudia-Elisabeth/H-5657-2011; Dudko, Lev/D-7127-2012; Lokhtin, Igor/D-7004-2012 OI Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Ragazzi, Stefano/0000-0001-8219-2074; Rovelli, Tiziano/0000-0002-9746-4842; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Cerrada, Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Montanari, Alessandro/0000-0003-2748-6373; de Jesus Damiao, Dilson/0000-0002-3769-1680; Novaes, Sergio/0000-0003-0471-8549; Ligabue, Franco/0000-0002-1549-7107; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Dudko, Lev/0000-0002-4462-3192; FU BMWF (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MEYS (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER [SF0690030s09]; ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Republic of Korea); WCU (Republic of Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MSTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter (Thailand); IPST (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU, Regional Development Fund; Thalis programme; Aristeia programme; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MEYS (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MON, RosAtom, RAS and RFBR (Russia); MSTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 48 TC 22 Z9 22 U1 4 U2 107 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD OCT 26 PY 2013 VL 73 IS 10 AR 2610 DI 10.1140/epjc/s10052-013-2610-8 PG 22 WC Physics, Particles & Fields SC Physics GA 244KE UT WOS:000326386200001 ER PT J AU Kilgore, WB AF Kilgore, William B. TI The two-loop infrared structure of amplitudes with mixed gauge groups SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID JET CROSS-SECTIONS; QCD CORRECTIONS; GLUON SCATTERING; ORDER; QUARK; ALGORITHM AB The infrared structure of (multi-loop) scattering amplitudes is determined entirely by the identities of the external particles participating in the scattering. The two-loop infrared structure of pure QCD amplitudes has been known for some time. By computing the two-loop amplitudes for (f) over barf -> X and (f) over barf -> V1V2 scattering in an SU(N) x SU(M) x U(1) gauge theory, I determine the anomalous dimensions which govern the infrared structure for any massless two-loop amplitude. C1 Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Kilgore, WB (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. EM kilgore@bnl.gov FU U.S. Department of Energy [DE-AC02-98CH10886] FX This research was supported by the U.S. Department of Energy under Contract No. DE-AC02-98CH10886. NR 39 TC 0 Z9 0 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD OCT 25 PY 2013 VL 73 IS 10 AR 2603 DI 10.1140/epjc/s10052-013-2603-7 PG 8 WC Physics, Particles & Fields SC Physics GA AC0JC UT WOS:000332179600001 ER PT J AU Li, CL Tanjore, D He, W Wong, J Gardner, JL Sale, KL Simmons, BA Singh, S AF Li, Chenlin Tanjore, Deepti He, Wei Wong, Jessica Gardner, James L. Sale, Kenneth L. Simmons, Blake A. Singh, Seema TI Scale-up and evaluation of high solid ionic liquid pretreatment and enzymatic hydrolysis of switchgrass SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Scale-up; Pretreatment; Saccharification; Ionic liquid; High solid loading; Viscosity; Inhibition ID WHEAT-STRAW; DILUTE-ACID; CORN STOVER; LIGNOCELLULOSIC BIOMASS; SACCHARIFICATION; EXTRACTION; LIGNIN; SUGARS; RECALCITRANCE; FERMENTATION AB Background: Ionic liquid (IL) pretreatment is receiving significant attention as a potential process that enables fractionation of lignocellulosic biomass and produces high yields of fermentable sugars suitable for the production of renewable fuels. However, successful optimization and scale up of IL pretreatment involves challenges, such as high solids loading, biomass handling and transfer, washing of pretreated solids and formation of inhibitors, which are not addressed during the development stages at the small scale in a laboratory environment. As a first in the research community, the Joint BioEnergy Institute, in collaboration with the Advanced Biofuels Process Demonstration Unit, a Department of Energy funded facility that supports academic and industrial entities in scaling their novel biofuels enabling technologies, have performed benchmark studies to identify key challenges associated with IL pretreatment using 1-ethyl-3-methylimidazolium acetate and subsequent enzymatic saccharification beyond bench scale. Results: Using switchgrass as the model feedstock, we have successfully executed 600-fold, relative to the bench scale (6 L vs 0.01 L), scale-up of IL pretreatment at 15% (w/w) biomass loading. Results show that IL pretreatment at 15% biomass generates a product containing 87.5% of glucan, 42.6% of xylan and only 22.8% of lignin relative to the starting material. The pretreated biomass is efficiently converted into monosaccharides during subsequent enzymatic hydrolysis at 10% loading over a 150-fold scale of operations (1.5 L vs 0.01 L) with 99.8% fermentable sugar conversion. The yield of glucose and xylose in the liquid streams were 94.8% and 62.2%, respectively, and the hydrolysate generated contains high titers of fermentable sugars (62.1 g/L of glucose and 5.4 g/L cellobiose). The overall glucan and xylan balance from pretreatment and saccharification were 95.0% and 77.1%, respectively. Enzymatic inhibition by [C(2)mim][OAc] at high solids loadings requires further process optimization to obtain higher yields of fermentable sugars. Conclusion: Results from this initial scale up evaluation indicate that the IL-based conversion technology can be effectively scaled to larger operations and the current study establishes the first scaling parameters for this conversion pathway but several issues must be addressed before a commercially viable technology can be realized, most notably reduction in water consumption and efficient IL recycle. C1 [Li, Chenlin; Tanjore, Deepti; He, Wei; Wong, Jessica; Gardner, James L.] Lawrence Berkeley Natl Lab, Adv Biofuels Proc Demonstrat Unit, Emeryville, CA USA. [Sale, Kenneth L.; Simmons, Blake A.; Singh, Seema] Joint BioEnergy Inst, Deconstruct Div, Emeryville, CA USA. [Sale, Kenneth L.; Simmons, Blake A.; Singh, Seema] Sandia Natl Labs, Biol & Mat Sci Ctr, Livermore, CA USA. RP Singh, S (reprint author), Joint BioEnergy Inst, Deconstruct Div, Emeryville, CA USA. EM seesing@sandia.gov OI Li, Chenlin/0000-0002-0793-0505 FU Office of Biomass Program within the US DOE's Office of Energy Efficiency and Renewable Energy; American Recovery and Reinvestment Act; US DOE's Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231] FX ABPDU would like to acknowledge the funding support from Office of Biomass Program within the US DOE's Office of Energy Efficiency and Renewable Energy, and also the funding support from the American Recovery and Reinvestment Act. JBEI would like to acknowledge the funding support from US DOE's Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the US DOE. The authors would like to thank the Laboratory of Dr. Daniel Putnam from the University of California at Davis for providing the switchgrass, and Novozymes for the gift of the enzyme cocktails used in this work. NR 52 TC 21 Z9 21 U1 6 U2 73 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD OCT 25 PY 2013 VL 6 AR 154 DI 10.1186/1754-6834-6-154 PG 13 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA 247WH UT WOS:000326653100001 PM 24160440 ER PT J AU Rao, RR Roberts, SA Noble, DR Anderson, PD Hetu, JF AF Rao, Rekha R. Roberts, S. A. Noble, David R. Anderson, Patrick D. Hetu, Jean-Francois TI USNCCM-11: Computational fluid mechanics for free and moving boundary problems SO COMPUTERS & FLUIDS LA English DT Editorial Material C1 [Rao, Rekha R.; Roberts, S. A.; Noble, David R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Anderson, Patrick D.] Eindhoven Univ Technol, NL-5600 MB Eindhoven, Netherlands. [Hetu, Jean-Francois] Natl Res Council Canada, Boucherville, PQ J4B 6Y4, Canada. RP Rao, RR (reprint author), Sandia Natl Labs, MS 0836, Albuquerque, NM 87185 USA. EM rrrao@sandia.gov RI Anderson, Patrick/E-6046-2011; OI Anderson, Patrick/0000-0001-9157-0858 NR 13 TC 0 Z9 0 U1 0 U2 7 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD OCT 25 PY 2013 VL 87 SI SI BP 1 EP 1 DI 10.1016/j.compfluid.2013.09.023 PG 1 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA 244AX UT WOS:000326360600001 ER PT J AU Roberts, SA Noble, DR Benner, EM Schunk, PR AF Roberts, Scott A. Noble, David R. Benner, Eric M. Schunk, P. Randall TI Multiphase hydrodynamic lubrication flow using a three-dimensional shell finite element model SO COMPUTERS & FLUIDS LA English DT Article DE Lubrication theory; Finite-element method; Shell elements; Level-set method; Multiphase flow ID THERMAL-ELASTOHYDRODYNAMIC LUBRICATION; FLASH IMPRINT LITHOGRAPHY; SLIDE-ROLL RATIOS; POWER-LAW FLUID; JOURNAL-BEARING; LEVEL SET; CONTACT SOLUTION; SURFACE-TENSION; 2-PHASE FLOWS; LINE CONTACT AB Reynolds' lubrication theory has been widely used to study thin-region fluid flows for a variety of scientific and manufacturing applications. In this work, we set forth an extension of this theory to model the effect of free fluid interfaces and fluid-structural interactions in lubrication films. This model is implemented using curvilinear shell elements in a general three-dimensional finite element code, allowing the study of lubrication flows in arbitrarily complex geometries. This implementation also allows coupling with continuum mechanics, such as solid body deformation, through lubrication-based and fluid-structural interactions. Simulations using this model are compared to analytical solutions and experimental results for a number of model problems. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Roberts, Scott A.; Noble, David R.] Sandia Natl Labs, Thermal & Fluid Proc Dept, Albuquerque, NM 87185 USA. [Benner, Eric M.; Schunk, P. Randall] Sandia Natl Labs, Nanoscale & React Proc Dept, Albuquerque, NM 87185 USA. RP Roberts, SA (reprint author), Sandia Natl Labs, Thermal & Fluid Proc Dept, POB 5800,MS-0836, Albuquerque, NM 87185 USA. EM sarober@sandia.gov RI Roberts, Scott/C-1158-2009 OI Roberts, Scott/0000-0002-4196-6771 FU US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors acknowledge Sandia National Laboratories' Laboratory Directed Research and Development program. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 76 TC 3 Z9 3 U1 1 U2 26 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD OCT 25 PY 2013 VL 87 SI SI BP 12 EP 25 DI 10.1016/j.compfluid.2012.08.009 PG 14 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA 244AX UT WOS:000326360600003 ER PT J AU Kapahi, A Sambasivan, S Udaykumar, HS AF Kapahi, A. Sambasivan, S. Udaykumar, H. S. TI Simulation of collapse and fragmentation phenomena in a sharp interface Eulerian setting SO COMPUTERS & FLUIDS LA English DT Article DE Eulerian; Sharp interface method; Level set method; Ghost Fluid Method (GFM); Void collapse; Fragmentation Least squares method ID GHOST FLUID METHOD; VOID COLLAPSE; MULTIMATERIAL FLOWS; ENERGETIC MATERIAL; LEVEL SET; PART 1; IMPACT; EXPLOSIVES; PENETRATION; SCHEMES AB Sharp interface Eulerian methods are used to develop a technique for handling high speed material dynamics leading to collapse and fragmentation. Two problems are of primary interest, viz, void collapse in energetic materials and fragmentation of solids under impact; in the first case the sharp interface reconnects to itself, while in the second the sharp interface is torn apart. The challenge is to simulate using a sharp interface Eulerian approach through these topological changes and to apply boundary conditions on the immersed interfaces. Level set interface representations are combined with a modified Ghost Fluid Method to solve sharp interface dynamics in the presence of elasto-plastically deforming solid materials. A unified method of populating ghost field is developed using an adaptive least squares approach and demonstrated to be robust for severe interface deformations, including changes in topology. A parallel algorithm is used to enable solutions of large scale problems. The embedded material interfaces undergoing severe deformation while moving at a very high speed are handled efficiently and accurately in a multi-processor setting. Validation exercises, examples and benchmark calculations are presented to demonstrate the accuracy of the approach. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Kapahi, A.; Udaykumar, H. S.] Univ Iowa, Dept Mech & Ind Engn, Iowa City, IA 52242 USA. [Sambasivan, S.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Udaykumar, HS (reprint author), Univ Iowa, Dept Mech & Ind Engn, 3131 Seamans Ctr, Iowa City, IA 52242 USA. EM hs-kumar@uiowa.edu FU AFOSR; AFRL-RWPC (Computational Mechanics Branch, Eglin AFB) FX This work was performed under grants from the AFOSR Computational Mathematics program (Program Manager: Dr. Fariba Fahroo) and from the AFRL-RWPC (Computational Mechanics Branch, Eglin AFB, Program Manager: Dr. Michael E. Nixon). NR 48 TC 1 Z9 1 U1 1 U2 10 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD OCT 25 PY 2013 VL 87 SI SI BP 26 EP 40 DI 10.1016/j.compfluid.2012.09.007 PG 15 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA 244AX UT WOS:000326360600004 ER PT J AU Clausen, JR AF Clausen, Jonathan R. TI Using the suspension balance model in a finite-element flow solver SO COMPUTERS & FLUIDS LA English DT Article DE Suspensions; Suspension balance; Multiphase flow ID STOKESIAN DYNAMICS SIMULATION; COMPUTATIONAL FLUID-DYNAMICS; SHEAR-INDUCED MIGRATION; PRESSURE-DRIVEN FLOW; CONCENTRATED SUSPENSIONS; PARTICLE MIGRATION; NORMAL STRESSES; RIGID SPHERES; NONCOLLOIDAL SUSPENSIONS; COLLOIDAL SUSPENSIONS AB A suspension balance model (SBM) is implemented to describe the shear-driven migration of particles in noncolloidal suspensions in the context of a finite element (FE) solver. Before developing the FE methodology, the SBM is analyzed in the context of a rigorous two-phase averaging procedure, in which the traditional SBM model can be thought of as an approximate closure relationship for the rigorous two-phase equations. It is shown that the standard SBM equations are inconsistent, which is demonstrated analytically for the case of Couette flow. A FE model is developed using a corrected set of SBM equations, and the numerical techniques needed to handle the anisotropic Q-tensor and FE stabilization are detailed. The resultant FE-SBM method is tested using a Couette geometry and compared with existing models and experiments. A high level of sensitivity of the particle migration to the chosen viscosity model is noted, as well as the influence of excess diffusion caused by the FE stabilization procedure. The FE-SBM method is also used in conjunction with an arbitrary Lagrangian-Eulerian formulation to simulate the deflection of the free surface in a Couette cell. Secondary flows are observed in the free-surface simulation results, and the underlying mechanisms driving these secondary flows are explored. (C) 2013 Elsevier Ltd. All rights reserved. C1 Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Clausen, JR (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM jclause@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 60 TC 2 Z9 2 U1 4 U2 9 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD OCT 25 PY 2013 VL 87 SI SI BP 67 EP 78 DI 10.1016/j.compfluid.2012.12.004 PG 12 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA 244AX UT WOS:000326360600008 ER PT J AU Francois, MM Carlson, NN AF Francois, Marianne M. Carlson, Neil N. TI The global embedded interface formulation for interfacial mass transfer within a volume tracking framework SO COMPUTERS & FLUIDS LA English DT Article DE Volume tracking; Mass transfer; Interfacial flow; Droplet dynamics ID NUMERICAL-SIMULATION; SURFACE-TENSION; FLOW; BUBBLES AB Interfacial flow with mass transfer is particularly challenging to compute because the position of the interface between the fluids and the interface physics needs to be predicted as part of the solution of the flow equations. In addition, the discontinuity in fluid density, viscosity and species concentration at the interface present additional numerical challenges. In this work, we extend our balanced-force volume-tracking algorithm for modeling interfacial flow with surface tension force [10] to include mass transfer. We propose a global embedded interface formulation to model the interfacial conditions of the species concentration at an interface in thermodynamic equilibrium. To verify our formulation, we perform simulations of a pure diffusion problem with species concentration discontinuity at the interface. Then we present two and three-dimensional simulations of droplets rising by buoyancy with mass transfer. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Francois, Marianne M.; Carlson, Neil N.] Los Alamos Natl Lab, Computat Phys & Methods Grp CCS 2, Los Alamos, NM 87545 USA. RP Francois, MM (reprint author), Los Alamos Natl Lab, Computat Phys & Methods Grp CCS 2, POB 1663, Los Alamos, NM 87545 USA. EM mmfran@lanl.gov OI Francois, Marianne/0000-0003-3062-6234 FU National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; Nuclear Energy Office of the Department of Energy FX This work was performed under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. This work is supported by the Nuclear Energy Office of the Department of Energy. The authors thank Boonthanome Nouanesengsy and John Patchett of the paraview team for their help with post-processing the data for the nine droplets test cases and Matthew Wagner, summer student in CCS-2 for his help with the simulations presented in Section 5.1. NR 25 TC 2 Z9 2 U1 0 U2 5 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD OCT 25 PY 2013 VL 87 SI SI BP 102 EP 114 DI 10.1016/j.compfluid.2013.02.016 PG 13 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA 244AX UT WOS:000326360600011 ER PT J AU Li, G Zhang, Q Rhodes, D Zeng, B Goswami, P Baumbach, RE Tobash, PH Ronning, F Thompson, JD Bauer, ED Balicas, L AF Li, G. Zhang, Q. Rhodes, D. Zeng, B. Goswami, P. Baumbach, R. E. Tobash, P. H. Ronning, F. Thompson, J. D. Bauer, E. D. Balicas, L. TI Bulk evidence for a time-reversal symmetry broken superconducting state in URu2Si2 SO PHYSICAL REVIEW B LA English DT Article ID HIDDEN-ORDER; FIELD; EXCITATIONS; TRANSITION; LATTICE; WAVE AB URu2Si2 is claimed to be a chiral d-wave superconductor with a k(z) (k(x) +/- ik(y)) time-reversal symmetry broken orbital component for the Cooper pair wave function, which contains both nodal points and lines of nodes. To study the magnetic response of such an unconventional state through a bulk, thermodynamic probe, we measured the magnetic torque t in very high-quality, well-characterized URu2Si2 single crystals at high magnetic fields H and at very low temperatures T. The magnetization M(H) proportional to tau(H)/H of URu2Si2, in its superconducting state and for angles within 15. from the ab plane, reveals a change in its sign for H approaching H-c2: from a clear diamagnetic response dominated by the pinning of vortices to a state with a smaller but "paramagneticlike" hysteretic response which disappears at H-c2, thus implying that it is intrinsically related to the superconducting state. We argue that this anomalous, angular-dependent behavior is evidence for a time-reversal symmetry broken superconducting state in URu2Si2, although not necessarily for the k(z) (k(x) +/- ik(y)) state. C1 [Li, G.; Zhang, Q.; Rhodes, D.; Zeng, B.; Goswami, P.; Balicas, L.] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Baumbach, R. E.; Tobash, P. H.; Ronning, F.; Thompson, J. D.; Bauer, E. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Li, G (reprint author), Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. EM balicas@magnet.fsu.edu RI Zeng, Bin/O-3370-2013; Rhodes, Daniel/H-3423-2013; Li, Gang/E-3033-2015; OI Zeng, Bin/0000-0002-0090-4371; Ronning, Filip/0000-0002-2679-7957; Bauer, Eric/0000-0003-0017-1937 FU NSF [NSF-DMR-0084173]; State of Florida; DOE-BES [DE-SC0002613]; US DOE, Office of Science FX We acknowledge discussions with N. Harrison. The NHMFL is supported by NSF through Grant No. NSF-DMR-0084173 and the State of Florida. L. B. is supported by DOE-BES through award DE-SC0002613. The work at the LANL is carried out under the auspices of the US DOE, Office of Science. NR 38 TC 13 Z9 13 U1 2 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 25 PY 2013 VL 88 IS 13 AR 134517 DI 10.1103/PhysRevB.88.134517 PG 7 WC Physics, Condensed Matter SC Physics GA 240KK UT WOS:000326094500005 ER PT J AU Nisoli, C Abraham, D Lookman, T Saxena, A AF Nisoli, Cristiano Abraham, Douglas Lookman, Turab Saxena, Avadh TI Quasi-one-dimensional thermal breakage SO PHYSICAL REVIEW E LA English DT Article ID 2-DIMENSIONAL ISING-MODEL; SI(001) SURFACE; NANOWIRES; GROWTH; TRANSITION; MICROSCOPY; POLYMERS; DNA AB Breakage is generally understood in mechanical terms, yet nanostructures can rupture not only under external loads but also via thermal activation. Here we treat in a general framework the statistical mechanics of thermally induced breakage at the nanoscale for one-dimensional systems. We test it on a simple approximation and find that the probability of breakage controls distinct regimes, characterized by sharp crossovers and narrow peaks in the thermal fluctuations and specific heat. Our work provides predictions on clustering of new phases, of relevance in nanofabrication. C1 [Nisoli, Cristiano; Abraham, Douglas; Lookman, Turab; Saxena, Avadh] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Nisoli, Cristiano; Abraham, Douglas; Lookman, Turab; Saxena, Avadh] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Abraham, Douglas] Rudolf Peierls Ctr Theoret Phys, Oxford OX1 3NP, England. RP Nisoli, C (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Nisoli, Cristiano/0000-0003-0053-1023 FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DEAC52-06NA25396] FX This work was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DEAC52-06NA25396. NR 34 TC 0 Z9 0 U1 0 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD OCT 25 PY 2013 VL 88 IS 4 AR 042409 DI 10.1103/PhysRevE.88.042409 PG 7 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 240SZ UT WOS:000326118600005 PM 24229191 ER PT J AU Brown, RS Deng, ZD Cook, KV Pflugrath, BD Li, XY Fu, T Martinez, JJ Li, HD Trumbo, BA Ahmann, ML Seaburg, AG AF Brown, Richard S. Deng, Z. Daniel Cook, Katrina V. Pflugrath, Brett D. Li, Xinya Fu, Tao Martinez, Jayson J. Li, Huidong Trumbo, Bradly A. Ahmann, Martin L. Seaburg, Adam G. TI A Field Evaluation of an External and Neutrally Buoyant Acoustic Transmitter for Juvenile Salmon: Implications for Estimating Hydroturbine Passage Survival SO PLOS ONE LA English DT Article ID HYDRO-TURBINE PASSAGE; CHINOOK SALMON; SWIMMING PERFORMANCE; SNAKE RIVER; COLUMBIA RIVER; TELEMETRY TRANSMITTERS; ATTACHED TRANSMITTERS; ANADROMOUS SALMONIDS; AVIAN PREDATION; SMALLMOUTH BASS AB Turbine-passed fish are exposed to rapid decreases in pressure which can cause barotrauma. The presence of an implanted telemetry tag increases the likelihood of injury or death from exposure to pressure changes, thus potentially biasing studies evaluating survival of turbine-passed fish. Therefore, a neutrally buoyant externally attached tag was developed to eliminate this bias in turbine passage studies. This new tag was designed not to add excess mass in water or take up space in the coelom, having an effective tag burden of zero with the goal of reducing pressure related biases to turbine survival studies. To determine if this new tag affects fish performance or susceptibility to predation, it was evaluated in the field relative to internally implanted acoustic transmitters (JSATS; Juvenile Salmon Acoustic Telemetry System) used widely for survival studies of juvenile salmonids. Survival and travel time through the study reach was compared between fish with either tag type in an area of high predation in the Snake and Columbia rivers, Washington. An additional group of fish affixed with neutrally-buoyant dummy external tags were implanted with passive integrated transponder (PIT) tags and recovered further downstream to assess external tag retention and injury. There were no significant differences in survival to the first detection site, 12 river kilometers (rkm) downstream of release. Travel times were also similar between groups. Conversely, externally-tagged fish had reduced survival (or elevated tag loss) to the second detection site, 65 rkm downstream. In addition, the retention study revealed that tag loss was first observed in fish recaptured approximately 9 days after release. Results suggest that this new tag may be viable for short term (< 8 days) single-dam turbine-passage studies and under these situations, may alleviate the turbine passage-related bias encountered when using internal tags, however further research is needed to confirm this. C1 [Brown, Richard S.; Cook, Katrina V.; Pflugrath, Brett D.] Pacific NW Natl Lab, Ecol Grp, Richland, WA 99352 USA. [Deng, Z. Daniel; Li, Xinya; Fu, Tao; Martinez, Jayson J.; Li, Huidong] Pacific NW Natl Lab, Hydrol Grp, Richland, WA 99352 USA. [Trumbo, Bradly A.; Ahmann, Martin L.] US Army, Corps Engineers, Walla Walla, WA USA. [Seaburg, Adam G.] Univ Washington, Sch Aquat & Fishery Sci, Seattle, WA 98195 USA. RP Brown, RS (reprint author), Pacific NW Natl Lab, Ecol Grp, Richland, WA 99352 USA. EM rich.brown@pnnl.gov RI Deng, Daniel/A-9536-2011 OI Deng, Daniel/0000-0002-8300-8766 FU U.S. Army corps of Engineers, Walla Walla district (Walla Walla Washington State) [W912EF-08-D-0004] FX This study was funded by the U.S. Army corps of Engineers, Walla Walla district (Walla Walla Washington State) under contract number W912EF-08-D-0004. Funders were involved in study design and preparation of the manuscript (authors BAT and MLA). NR 55 TC 3 Z9 3 U1 3 U2 25 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 25 PY 2013 VL 8 IS 10 AR e77744 DI 10.1371/journal.pone.0077744 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 241GW UT WOS:000326155400054 PM 24204947 ER PT J AU Reddy, AP Simmons, CW D'haeseleer, P Khudyakov, J Burd, H Hadi, M Simmons, BA Singer, SW Thelen, MP VanderGheynst, JS AF Reddy, Amitha P. Simmons, Christopher W. D'haeseleer, Patrik Khudyakov, Jane Burd, Helcio Hadi, Masood Simmons, Blake A. Singer, Steven W. Thelen, Michael P. VanderGheynst, Jean S. TI Discovery of Microorganisms and Enzymes Involved in High-Solids Decomposition of Rice Straw Using Metagenomic Analyses SO PLOS ONE LA English DT Article ID SP-NOV.; LIGNOCELLULOSIC BIOFUELS; KOREAN GINSENG; BINDING MODULE; GEN. NOV.; CELLULOSE; SOIL; COMMUNITY; RESOURCE; SYSTEM AB High-solids incubations were performed to enrich for microbial communities and enzymes that decompose rice straw under mesophilic (35 degrees C) and thermophilic (55 degrees C) conditions. Thermophilic enrichments yielded a community that was 7.5 times more metabolically active on rice straw than mesophilic enrichments. Extracted xylanase and endoglucanse activities were also 2.6 and 13.4 times greater, respectively, for thermophilic enrichments. Metagenome sequencing was performed on enriched communities to determine community composition and mine for genes encoding lignocellulolytic enzymes. Proteobacteria were found to dominate the mesophilic community while Actinobacteria were most abundant in the thermophilic community. Analysis of protein family representation in each metagenome indicated that cellobiohydrolases containing carbohydrate binding module 2 (CBM2) were significantly overrepresented in the thermophilic community. Micromonospora, a member of Actinobacteria, primarily housed these genes in the thermophilic community. In light of these findings, Micromonospora and other closely related Actinobacteria genera appear to be promising sources of thermophilic lignocellulolytic enzymes for rice straw deconstruction under high-solids conditions. Furthermore, these discoveries warrant future research to determine if exoglucanases with CBM2 represent thermostable enzymes tolerant to the process conditions expected to be encountered during industrial biofuel production. C1 [Reddy, Amitha P.; Simmons, Christopher W.; D'haeseleer, Patrik; Khudyakov, Jane; Burd, Helcio; Hadi, Masood; Simmons, Blake A.; Singer, Steven W.; Thelen, Michael P.; VanderGheynst, Jean S.] Joint BioEnergy Inst, Emeryville, CA USA. [Reddy, Amitha P.; Simmons, Christopher W.; VanderGheynst, Jean S.] Univ Calif Davis, Davis, CA 95616 USA. [Singer, Steven W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [D'haeseleer, Patrik; Khudyakov, Jane; Thelen, Michael P.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA USA. [Hadi, Masood; Simmons, Blake A.] Sandia Natl Labs, Biol & Mat Sci Ctr, Livermore, CA USA. [Burd, Helcio] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP VanderGheynst, JS (reprint author), Joint BioEnergy Inst, Emeryville, CA USA. EM jsvander@ucdavis.edu RI Thelen, Michael/C-6834-2008; Khudyakov, Jane/C-1213-2014; Thelen, Michael/G-2032-2014; OI Thelen, Michael/0000-0002-2479-5480; Thelen, Michael/0000-0002-2479-5480; Khudyakov, Jane/0000-0001-7038-102X FU University of California Laboratory Fees Research Program [12-LR-237496]; DOE Joint BioEnergy Institute; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; U.S. Department of Energy FX This work was supported by the University of California Laboratory Fees Research Program #12-LR-237496 and performed as part of the DOE Joint BioEnergy Institute (http://www.jbei.org) supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U.S. Department of Energy. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 60 TC 12 Z9 12 U1 7 U2 36 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 25 PY 2013 VL 8 IS 10 AR e77985 DI 10.1371/journal.pone.0077985 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 241GW UT WOS:000326155400065 PM 24205054 ER PT J AU Wen, HD Guo, L Barnes, E Lee, JH Walko, DA Schaller, RD Moyer, JA Misra, R Li, YL Dufresne, EM Schlom, DG Gopalan, V Freeland, JW AF Wen, Haidan Guo, Lu Barnes, Eftihia Lee, June Hyuk Walko, Donald A. Schaller, Richard D. Moyer, Jarrett A. Misra, Rajiv Li, Yuelin Dufresne, Eric M. Schlom, Darrell G. Gopalan, Venkatraman Freeland, John W. TI Structural and electronic recovery pathways of a photoexcited ultrathin VO2 film SO PHYSICAL REVIEW B LA English DT Article ID METAL-INSULATOR TRANSITIONS; PHASE-TRANSITION; RUTILE TIO2; EXCITATION; MANGANITE AB The structural and electronic recovery pathways of a photoexcited ultrathin vanadium dioxide (VO2) film at nanosecond time scales have been studied using time-resolved x-ray diffraction and transient optical absorption techniques. The recovery pathways from the tetragonal metallic phase to the monoclinic insulating phase are highly dependent on the optical pump fluence. At pump fluences higher than the saturation fluence of 14.7 mJ/cm(2), we observed a transient structural state with lattice parameter larger than that of the tetragonal phase, which is decoupled from the metal-to-insulator phase transition. Subsequently, the photoexcited VO2 film recovered to the ground state at characteristic times dependent upon the pump fluence as a result of heat transport from the film to the substrate. We present a procedure to measure the time-resolved film temperature by correlating photoexcited and temperature-dependent x-ray diffraction measurements. A thermal transport model that incorporates changes of the thermal parameters across the phase transition reproduces the observed recovery dynamics. The optical excitation and fast recovery of ultrathin VO2 films provides a practical method to reversibly switch between the monoclinic insulating and tetragonal metallic state at nanosecond time scales. C1 [Wen, Haidan; Lee, June Hyuk; Walko, Donald A.; Li, Yuelin; Dufresne, Eric M.; Freeland, John W.] Argonne Natl Lab, Argonne, IL 60439 USA. [Guo, Lu; Barnes, Eftihia; Gopalan, Venkatraman] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Schaller, Richard D.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Schaller, Richard D.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Moyer, Jarrett A.] Univ Illinoi Urbana Champaign, Dept Phys, Urbana, IL 61801 USA. [Misra, Rajiv] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Schlom, Darrell G.] Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. [Schlom, Darrell G.] Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA. RP Wen, HD (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM wen@aps.anl.gov; vxg8@psu.edu; freeland@aps.anl.gov FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Office of Naval Research (ONR) [N00014-11-1-0665] FX Work at Argonne was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. D.G.S. and V.G. would like to acknowledge funding from the Office of Naval Research (ONR) Award No. N00014-11-1-0665. The transport measurements were performed in Peter Schiffer's laboratory. NR 48 TC 14 Z9 14 U1 1 U2 45 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 25 PY 2013 VL 88 IS 16 AR 165424 DI 10.1103/PhysRevB.88.165424 PG 8 WC Physics, Condensed Matter SC Physics GA 240KQ UT WOS:000326095200006 ER PT J AU Ban, CM Xie, M Sun, X Travis, JJ Wang, GK Sun, HT Dillon, AC Lian, J George, SM AF Ban, Chunmei Xie, Ming Sun, Xiang Travis, Jonathan J. Wang, Gongkai Sun, Hongtao Dillon, Anne C. Lian, Jie George, Steven M. TI Atomic layer deposition of amorphous TiO2 on graphene as an anode for Li-ion batteries SO NANOTECHNOLOGY LA English DT Article ID BINARY REACTION SEQUENCE; HIGH AREAL CAPACITY; LITHIUM-STORAGE; ANATASE TIO2; PHOTOCATALYTIC ACTIVITY; CARBON NANOTUBES; THIN-FILMS; OXIDE; GRAPHITE; NANOPARTICLES AB Atomic layer deposition (ALD) was used to deposit TiO2 anode material on high surface area graphene (reduced graphene oxide) sheets for Li-ion batteries. An Al2O3 ALD ultrathin layer was used as an adhesion layer for conformal deposition of the TiO2 ALD films at 120 degrees C onto the conducting graphene sheets. The TiO2 ALD films on the Al2O3 ALD adhesion layer were nearly amorphous and conformal to the graphene sheets. These nanoscale TiO2 coatings minimized the effect of the low diffusion coefficient of lithium ions in bulk TiO2. The TiO2 ALD films exhibited stable capacities of similar to 120 mAh g(-1) and similar to 100 mAh g(-1) at high cycling rates of 1 A g(-1) and 2 A g(-1), respectively. The TiO2 ALD films also displayed excellent cycling stability with similar to 95% of the initial capacity remaining after 500 cycles. These results illustrate that ALD can provide a useful method to deposit electrode materials on high surface area substrates for Li-ion batteries. C1 [Ban, Chunmei; Dillon, Anne C.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Xie, Ming; Travis, Jonathan J.; George, Steven M.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Xie, Ming; Travis, Jonathan J.; George, Steven M.] Univ Colorado, Dept Chem & Biol Engn, Boulder, CO 80309 USA. [Sun, Xiang; Wang, Gongkai; Sun, Hongtao; Lian, Jie] Rensselaer Polytech Inst, Dept Mech Aerosp & Nucl Engn, Troy, NY 12180 USA. RP Ban, CM (reprint author), Natl Renewable Energy Lab, 1617 Cole Blvd, Golden, CO 80401 USA. EM ming.xie@colorado.edu; lianj@rpi.edu; steven.george@colorado.edu RI xie, ming/A-1438-2012; Sun, Hongtao/N-6597-2013; George, Steven/O-2163-2013; Wang, Gongkai/A-6504-2015 OI Sun, Hongtao/0000-0003-3259-6091; George, Steven/0000-0003-0253-9184; FU US Department of Energy Office of Vehicle Technologies; Defense Advanced Research Project Agency (DARPA); National Science Foundation [DMR-1151028] FX The research work at National Renewable Energy Laboratory was supported by the US Department of Energy Office of Vehicle Technologies through the Batteries for Advanced Transportation Technologies Program. The work at the University of Colorado was supported by the Defense Advanced Research Project Agency (DARPA). The work at Rensselaer Polytechnic Institute was supported by the National Science Foundation (DMR-1151028). Drs Chunmei Ban and Ming Xie contributed equally to this work. NR 49 TC 35 Z9 35 U1 11 U2 197 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 J9 NANOTECHNOLOGY JI Nanotechnology PD OCT 25 PY 2013 VL 24 IS 42 SI SI AR 424002 DI 10.1088/0957-4484/24/42/424002 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 227VE UT WOS:000325142600004 PM 24067324 ER PT J AU Dunn, B Liu, P Meng, S AF Dunn, Bruce Liu, Ping Meng, Shirley TI Nanoscience and nanotechnology in next generation lithium batteries SO NANOTECHNOLOGY LA English DT Editorial Material C1 [Dunn, Bruce] Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90024 USA. [Liu, Ping] US DOE, Adv Res Projects Agcy Energy, Washington, DC 20585 USA. [Meng, Shirley] Univ Calif San Diego, Dept Nanoengn, San Diego, CA 92103 USA. RP Dunn, B (reprint author), Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90024 USA. NR 0 TC 3 Z9 3 U1 7 U2 60 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 J9 NANOTECHNOLOGY JI Nanotechnology PD OCT 25 PY 2013 VL 24 IS 42 SI SI AR 420201 DI 10.1088/0957-4484/24/42/420201 PG 1 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 227VE UT WOS:000325142600001 PM 24195122 ER PT J AU Lee, E Persson, KA AF Lee, Eunseok y Persson, Kristin A. TI First-principles study of the nano-scaling effect on the electrochemical behavior in LiNi0.5Mn1.5O4 SO NANOTECHNOLOGY LA English DT Article ID LI-ION BATTERIES; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; JAHN-TELLER DISTORTION; AUGMENTED-WAVE METHOD; THIN-FILM ELECTRODES; CATHODE MATERIALS; CRYSTAL-SURFACES; BASIS-SET; SPINEL AB Nano-scaling of electrode materials is often used in battery applications to enhance performance, particularly relating to rate capability. However, for the high-voltage spinel LiNi0.5Mn1.5O4 conflicting results have been reported on the benefits of nano-scaling. In this study, we present first-principles calculations to investigate the effect of nano-scaling on LiNi0.5Mn1.5O4, specifically focusing on the roles and coupling between surface stability, cation ordering and phase behavior. We calculate and compare the surface energy for the low index facets (100), (110), and (111), and find that the most stable facet is dependent on the cation ordering at the surface layer. In this context, we predict a spontaneous surface reconstruction in the cation-ordered structure which leads to a deviation from the perfect surface cation ordering and results in an enhanced accessibility to solid solution behavior as a function of Li content. Our results imply that nano-scaling will be more beneficial for the cation-ordered structure, as compared to the disordered structure where the solid solution region is already intrinsically accessible for a broad range of Li concentrations. C1 [Lee, Eunseok y; Persson, Kristin A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Lee, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM eunseoklee@lbl.gov FU Office of Vehicle Technologies of the US Department of Energy [DE-AC02-05CH11231] FX Work at the Lawrence Berkeley National Laboratory was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the US Department of Energy, under Contract No. DE-AC02-05CH11231. We are also grateful to Cheonjoong Kim and Jordi Cabana for enlightening discussions on the high-voltage spinel. NR 40 TC 9 Z9 9 U1 2 U2 75 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 J9 NANOTECHNOLOGY JI Nanotechnology PD OCT 25 PY 2013 VL 24 IS 42 SI SI AR 424007 DI 10.1088/0957-4484/24/42/424007 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 227VE UT WOS:000325142600009 PM 24067535 ER PT J AU Wang, F Wu, LJ Ma, C Su, D Zhu, YM Graetz, J AF Wang, Feng Wu, Lijun Ma, Chao Su, Dong Zhu, Yimei Graetz, Jason TI Excess lithium storage and charge compensation in nanoscale Li4+xTi5O12 SO NANOTECHNOLOGY LA English DT Article ID RECHARGEABLE BATTERIES; CATHODE MATERIALS; SPINEL; LI4TI5O12; INSERTION; NANOPARTICLES; SITES AB Lithium titanate spinel (Li4Ti5O12; LTO) is a promising candidate for anodes in lithium-ion batteries due to its excellent cyclability and safety performance, and has been known as a 'zero-strain' material that allows reversible lithium insertion-deinsertion with little change in the lattice parameters. For a better understanding of lithium reaction mechanisms in this material, it has been of great interest to identify where lithium is inserted and how it migrates during charge and discharge, which is often difficult with x-ray and electron scattering techniques due to the low scattering power of lithium. In this study, we employed atomic-resolution annular bright-field imaging to directly image the lithium on interstitial sites in nanoscale LTO, and electron energy-loss spectroscopy to measure local lithium occupancy and electronic structure at different states of charge. During lithiation, charge compensation occurs primarily at O sites, rather than at Ti sites, and no significant change was found in the projected density of states (Ti 3d) until the voltage was lowered to similar to 50 mV or below. The Li K-edge spectra were simulated via ab initio calculations, providing a direct correlation between the near-edge fine structure and the local lithium coordination. During the initial states of discharge, lithium ions on 8a sites migrate to 16c sites (above 740 mV). Further lithiation causes the partial re-occupation of 8a sites, initially in the near-surface region at similar to 600 mV, and then in the bulk at lower voltages (similar to 50 mV). We attribute the enhanced capacity in nanostructured LTO to extra storage of lithium in the near-surface region, primarily at {111} facets. C1 [Wang, Feng; Wu, Lijun; Ma, Chao; Su, Dong; Zhu, Yimei; Graetz, Jason] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Wang, F (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM fwang@bnl.gov RI Ma, Chao/J-4569-2015; Wang, Feng/C-1443-2016; Su, Dong/A-8233-2013 OI Wang, Feng/0000-0003-4068-9212; Su, Dong/0000-0002-1921-6683 FU New York Battery and Energy Storage Technology (NY-BEST) Consortium [18509]; US DOE, Office of Science [DE-AC02-98CH10886] FX This work was partially supported by New York Battery and Energy Storage Technology (NY-BEST) Consortium, under Contract No. 18509. We thank Ganesh Venugopal and Andrew Hunt from nGimat for providing the Li4Ti5O12 samples. We thank Jian Hong, Joseph Woicik, and Daniel Fisher for help with sample processing and synchrotron XPS measurements. XPS measurement at the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the US DOE, Office of Science, under Contract No. DE-AC02-98CH10886. NR 31 TC 6 Z9 6 U1 2 U2 67 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 J9 NANOTECHNOLOGY JI Nanotechnology PD OCT 25 PY 2013 VL 24 IS 42 SI SI AR 424006 DI 10.1088/0957-4484/24/42/424006 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 227VE UT WOS:000325142600008 PM 24067496 ER PT J AU Wu, J Dathar, GKP Sun, CW Theivanayagam, MG Applestone, D Dylla, AG Manthiram, A Henkelman, G Goodenough, JB Stevenson, KJ AF Wu, Jing Dathar, Gopi Krishna Phani Sun, Chunwen Theivanayagam, Murali G. Applestone, Danielle Dylla, Anthony G. Manthiram, Arumugam Henkelman, Graeme Goodenough, John B. Stevenson, Keith J. TI In situ Raman spectroscopy of LiFePO4: size and morphology dependence during charge and self-discharge SO NANOTECHNOLOGY LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; LI-INSERTION/EXTRACTION; PARTICLE-SIZE; BATTERIES; ELECTRODES; LIXFEPO4; CATHODES AB Previous studies of the size dependent properties of LiFePO4 have focused on the diffusion rate or phase transformation pathways by bulk analysis techniques such as x-ray diffraction (XRD), neutron diffraction and electrochemistry. In this work, in situ Raman spectroscopy was used to study the surface phase change during charge and self-discharge on a more localized scale for three morphologies of LiFePO4: (1) 25 +/- 6 nm width nanorods, (2) 25 +/- 6 nm width nanorods and (3) similar to 2 mu m porous microspheres. Both the large nanorod and microsphere geometries showed incomplete delithiation at the end of charge, which was most likely caused by anti-site defects along the 1D diffusion channels in the bulk of the larger particles. Based on the in situ Raman measurements, all of the morphologies studied exhibited self-discharge with time. Among them, the smallest FePO4 particles self-discharged (lithiated) the fastest. While nanostructuring LiFePO4 can offer advantages in terms of lowering anti-site defects within particles, it also creates new problems due to high surface energies that allow self-discharge. The in situ Raman spectroscopy also showed that carbon coating did not provide significant improvement to the stability of the lithiated particles. C1 [Wu, Jing; Dylla, Anthony G.; Henkelman, Graeme; Stevenson, Keith J.] Univ Texas Austin, Dept Chem & Biochem, Austin, TX 78712 USA. [Dathar, Gopi Krishna Phani] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN USA. [Sun, Chunwen] Chinese Acad Sci, Inst Phys, Beijing 100080, Peoples R China. [Theivanayagam, Murali G.; Manthiram, Arumugam] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA. [Applestone, Danielle] Otherlab Inc, San Francisco, CA USA. [Goodenough, John B.] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. RP Stevenson, KJ (reprint author), Univ Texas Austin, Dept Chem & Biochem, Austin, TX 78712 USA. EM stevenson@cm.utexas.edu RI Sun, Chunwen/A-9860-2008 OI Sun, Chunwen/0000-0002-3610-9396 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001091]; Office of Science of the US Department of Energy [DE-AC02-05CH11231]; program 'Understanding Charge Separation and Transfer at Interfaces in Energy Materials (EFRC:CST)'; Energy Frontier Research Center FX This material is based upon work supported as part of the program 'Understanding Charge Separation and Transfer at Interfaces in Energy Materials (EFRC:CST)', an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001091. We also acknowledge the computational resources from National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 26 TC 10 Z9 12 U1 10 U2 106 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 J9 NANOTECHNOLOGY JI Nanotechnology PD OCT 25 PY 2013 VL 24 IS 42 SI SI AR 424009 DI 10.1088/0957-4484/24/42/424009 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 227VE UT WOS:000325142600011 PM 24067625 ER PT J AU Xiao, J Zheng, JM Li, XL Shao, YY Zhang, JG AF Xiao, Jie Zheng, Jianming Li, Xiaolin Shao, Yuyan Zhang, Ji-Guang TI Hierarchically structured materials for lithium batteries SO NANOTECHNOLOGY LA English DT Article ID RECHARGEABLE LI-O-2 BATTERIES; LI-AIR BATTERIES; ION BATTERIES; CATHODE MATERIALS; OXYGEN REDUCTION; OXIDE COMPOSITE; POROUS CARBON; SILICON ANODE; LONG-LIFE; ELECTRODES AB The lithium-ion battery (LIB) is one of the most promising power sources to be deployed in electric vehicles, including solely battery powered vehicles, plug-in hybrid electric vehicles, and hybrid electric vehicles. With the increasing demand for devices of high-energy densities (> 500 Wh kg(-1)), new energy storage systems, such as lithium-oxygen (Li-O-2) batteries and other emerging systems beyond the conventional LIB, have attracted worldwide interest for both transportation and grid energy storage applications in recent years. It is well known that the electrochemical performance of these energy storage systems depends not only on the composition of the materials, but also on the structure of the electrode materials used in the batteries. Although the desired performance characteristics of batteries often have conflicting requirements with the micro/nano-structure of electrodes, hierarchically designed electrodes can be tailored to satisfy these conflicting requirements. This work will review hierarchically structured materials that have been successfully used in LIB and Li-O-2 batteries. Our goal is to elucidate (1) how to realize the full potential of energy materials through the manipulation of morphologies, and (2) how the hierarchical structure benefits the charge transport, promotes the interfacial properties and prolongs the electrode stability and battery lifetime. C1 [Xiao, Jie; Zheng, Jianming; Li, Xiaolin; Shao, Yuyan; Zhang, Ji-Guang] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Xiao, J (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. EM jiguang.zhang@pnnl.gov RI Shao, Yuyan/A-9911-2008; Zheng, Jianming/F-2517-2014 OI Shao, Yuyan/0000-0001-5735-2670; Zheng, Jianming/0000-0002-4928-8194 FU US Department of Energy's Office of Energy Efficiency and Renewable Energy, Office of Vehicle Technologies FX We gratefully acknowledge the support provided by the US Department of Energy's Office of Energy Efficiency and Renewable Energy, Office of Vehicle Technologies. NR 48 TC 14 Z9 14 U1 8 U2 131 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD OCT 25 PY 2013 VL 24 IS 42 SI SI AR 424004 DI 10.1088/0957-4484/24/42/424004 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 227VE UT WOS:000325142600006 PM 24067410 ER PT J AU Attanasio, C Nord, AS Zhu, YW Blow, MJ Li, ZR Liberton, DK Morrison, H Plajzer-Frick, I Holt, A Hosseini, R Phouanenavong, S Akiyama, JA Shoukry, M Afzal, V Rubin, EM FitzPatrick, DR Ren, B Hallgrimsson, B Pennacchio, LA Visel, A AF Attanasio, Catia Nord, Alex S. Zhu, Yiwen Blow, Matthew J. Li, Zirong Liberton, Denise K. Morrison, Harris Plajzer-Frick, Ingrid Holt, Amy Hosseini, Roya Phouanenavong, Sengthavy Akiyama, Jennifer A. Shoukry, Malak Afzal, Veena Rubin, Edward M. FitzPatrick, David R. Ren, Bing Hallgrimsson, Benedikt Pennacchio, Len A. Visel, Axel TI Fine Tuning of Craniofacial Morphology by Distant-Acting Enhancers SO SCIENCE LA English DT Article ID GENOME-WIDE ASSOCIATION; CLEFT-LIP; GENE-EXPRESSION; NEURAL CREST; TOOTH DEVELOPMENT; SONIC HEDGEHOG; CRANIAL BASE; PALATE; MOUSE; MICE AB The shape of the human face and skull is largely genetically determined. However, the genomic basis of craniofacial morphology is incompletely understood and hypothesized to involve protein-coding genes, as well as gene regulatory sequences. We used a combination of epigenomic profiling, in vivo characterization of candidate enhancer sequences in transgenic mice, and targeted deletion experiments to examine the role of distant-acting enhancers in craniofacial development. We identified complex regulatory landscapes consisting of enhancers that drive spatially complex developmental expression patterns. Analysis of mouse lines in which individual craniofacial enhancers had been deleted revealed significant alterations of craniofacial shape, demonstrating the functional importance of enhancers in defining face and skull morphology. These results demonstrate that enhancers are involved in craniofacial development and suggest that enhancer sequence variation contributes to the diversity of human facial morphology. C1 [Attanasio, Catia; Nord, Alex S.; Zhu, Yiwen; Plajzer-Frick, Ingrid; Holt, Amy; Hosseini, Roya; Phouanenavong, Sengthavy; Akiyama, Jennifer A.; Shoukry, Malak; Afzal, Veena; Rubin, Edward M.; Pennacchio, Len A.; Visel, Axel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Blow, Matthew J.; Rubin, Edward M.; Pennacchio, Len A.; Visel, Axel] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. [Li, Zirong; Ren, Bing] Univ Calif San Diego, Sch Med, Ludwig Inst Canc Res, La Jolla, CA 92093 USA. [Li, Zirong; Ren, Bing] Univ Calif San Diego, Sch Med, Dept Cellular & Mol Med, La Jolla, CA 92093 USA. [Liberton, Denise K.; Hallgrimsson, Benedikt] Univ Calgary, Dept Cell Biol & Anat, McCaig Bone & Joint Inst, Calgary, AB T2N 4N1, Canada. [Morrison, Harris; FitzPatrick, David R.] Univ Edinburgh, MRC Inst Genet & Mol Med, MRC Human Genet Unit, Edinburgh EH4 2XU, Midlothian, Scotland. [FitzPatrick, David R.] Royal Hosp Sick Children, Edinburgh EH9 1LF, Midlothian, Scotland. [Hallgrimsson, Benedikt] Univ Calgary, Alberta Childrens Hosp, Res Inst, Calgary, AB T2N 4N1, Canada. RP Visel, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM avisel@lbl.gov RI Visel, Axel/A-9398-2009; Blow, Matthew/G-6369-2012; attanasio, catia/D-5042-2017; Hallgrimsson, Benedikt/A-9616-2008; OI Visel, Axel/0000-0002-4130-7784; Blow, Matthew/0000-0002-8844-9149; Hallgrimsson, Benedikt/0000-0002-7192-9103; FitzPatrick, David R./0000-0003-4861-969X FU NIDCR FaceBase grant [U01DE020060]; National Human Genome Research Institute [R01HG003988, U54HG006997]; Swiss National Science Foundation; F32 NIH/National Institute of General Medical Sciences National Research Service Award [GM105202]; NIH [U54HG006997, 1R01DE021708, 1R01DE01963, 1U01DE020054, R01HG003991]; Natural Sciences and Engineering Research Council of Canada [238992-11]; UK Medical Research Council; Ludwig Institute for Cancer Research; NIH; Department of Energy [DE-AC02-05CH11231] FX The authors thank J. Harkes and M. Satyanarayanan for development of the OPT viewer; S. Shen and H. Hochheiser for integration of the OPT viewer and data sets into FaceBase; and J. Murray, M. Marazita, J. Manak, B. Schutte, and all FaceBase members for help in the selection of relevant craniofacial intervals and comments on results. A. V. and L. A. P. were supported by NIDCR FaceBase grant U01DE020060 and by National Human Genome Research Institute grants R01HG003988 and U54HG006997. C. A. was supported by a Swiss National Science Foundation advanced researcher fellowship. A. S. N. was supported by a F32 NIH/National Institute of General Medical Sciences National Research Service Award fellowship GM105202. B. H. was supported by NIH 1R01DE021708, NIH 1R01DE01963, NIH 1U01DE020054, and Natural Sciences and Engineering Research Council of Canada #238992-11 grants. D. R. F. and H. M. were supported by a UK Medical Research Council core program grant. B. R. was supported by the Ludwig Institute for Cancer Research and NIH grants U54HG006997 and R01HG003991. B. H. was supported by NIH 1R01DE01963. Research was conducted at the E. O. Lawrence Berkeley National Laboratory and performed under Department of Energy contract DE-AC02-05CH11231, University of California. ChIP-Seq data are available through GEO (accession no. GSE49413) and FaceBase. org. In vivo reporter data are available through the Vista Enhancer Browser (http://enhancer.lbl.gov) and FaceBase. org. OPT data, including raw images and interactive 3D viewing option, is available through http://facebase.org. All enhancer reporter vectors, as well as archived surplus LacZ-stained embryos for selected enhancers, are available from the authors. Craniofacial enhancer knockout lines are available through the Mutant Mouse Regional Resource Centers (Delta hs1431, MMRRC 03895; Delta hs746, MMRRC 03888; and Delta hs586, MMRRCC 03894). NR 61 TC 77 Z9 79 U1 3 U2 20 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD OCT 25 PY 2013 VL 342 IS 6157 AR 1241006 DI 10.1126/science.1241006 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 239RH UT WOS:000326042600032 PM 24159046 ER PT J AU Rocha, C Calado, R Borrego, P Marcelino, JM Bartolo, I Rosado, L Cavaco-Silva, P Gomes, P Familia, C Quintas, A Skar, H Leitner, T Barroso, H Taveira, N AF Rocha, Cheila Calado, Rita Borrego, Pedro Marcelino, Jose Maria Bartolo, Ines Rosado, Lino Cavaco-Silva, Patricia Gomes, Perpetua Familia, Carlos Quintas, Alexandre Skar, Helena Leitner, Thomas Barroso, Helena Taveira, Nuno TI Evolution of the human immunodeficiency virus type 2 envelope in the first years of infection is associated with the dynamics of the neutralizing antibody response SO RETROVIROLOGY LA English DT Article DE Vertical HIV-2 infection; Evolution of the neutralizing antibody response; Escape from neutralization; Molecular evolution; Tropism ID PLASMA VIRAL LOAD; HIV-2 INFECTION; GUINEA-BISSAU; VERTICAL TRANSMISSION; PHYLOGENETIC ANALYSIS; CLINICAL PROGRESSION; CORECEPTOR USAGE; SWISS-MODEL; WEST-AFRICA; V3 LOOP AB Background: Differently from HIV-1, HIV-2 disease progression usually takes decades without antiretroviral therapy and the majority of HIV-2 infected individuals survive as elite controllers with normal CD4(+) T cell counts and low or undetectable plasma viral load. Neutralizing antibodies (Nabs) are thought to play a central role in HIV-2 evolution and pathogenesis. However, the dynamic of the Nab response and resulting HIV-2 escape during acute infection and their impact in HIV-2 evolution and disease progression remain largely unknown. Our objective was to characterize the Nab response and the molecular and phenotypic evolution of HIV-2 in association with Nab escape in the first years of infection in two children infected at birth. Results: CD4+ T cells decreased from about 50% to below 30% in both children in the first five years of infection and the infecting R5 viruses were replaced by X4 viruses within the same period. With antiretroviral therapy, viral load in child 1 decreased to undetectable levels and CD4(+) T cells recovered to normal levels, which have been sustained at least until the age of 12. In contrast, viral load increased in child 2 and she progressed to AIDS and death at age 9. Beginning in the first year of life, child 1 raised high titers of antibodies that neutralized primary R5 isolates more effectively than X4 isolates, both autologous and heterologous. Child 2 raised a weak X4-specific Nab response that decreased sharply as disease progressed. Rate of evolution, nucleotide and amino acid diversity, and positive selection, were significantly higher in the envelope of child 1 compared to child 2. Rates of R5-to-X4 tropism switch, of V1 and V3 sequence diversification, and of convergence of V3 to a beta-hairpin structure were related with rate of escape from the neutralizing antibodies. Conclusion: Our data suggests that the molecular and phenotypic evolution of the human immunodeficiency virus type 2 envelope are related with the dynamics of the neutralizing antibody response providing further support for a model in which Nabs play an important role in HIV-2 pathogenesis. C1 [Rocha, Cheila; Calado, Rita; Borrego, Pedro; Bartolo, Ines; Barroso, Helena; Taveira, Nuno] Fac Farm Lisboa, Ctr Patogenese Mol, Unidade Retrovirus Infeccoes Assoc, Lisbon, Portugal. [Rocha, Cheila; Calado, Rita; Borrego, Pedro; Bartolo, Ines; Cavaco-Silva, Patricia; Gomes, Perpetua; Familia, Carlos; Quintas, Alexandre; Barroso, Helena; Taveira, Nuno] Inst Super Ciencias Saude Egas Moniz, Ctr Invest Interdisciplinar Egas Moniz CiiEM, Monte De Caparica, Portugal. [Marcelino, Jose Maria] Univ Nova Lisboa, Inst Higiene & Med Trop, Unidade Microbiol Med, P-1200 Lisbon, Portugal. [Rosado, Lino] Hosp Dona Estefania, Unidade Imunohematol, Lisbon, Portugal. [Gomes, Perpetua] Ctr Hosp Lisboa Ocidental HEM, Serv Med Transfus, Lab Biol Mol, Lisbon, Portugal. [Gomes, Perpetua] Inst Super Higiene & Med Trop, Ctr Malaria & Outras Doencas Tropicais, Lisbon, Portugal. [Skar, Helena; Leitner, Thomas] Los Alamos Natl Lab, Los Alamos, NM USA. RP Taveira, N (reprint author), Fac Farm Lisboa, Ctr Patogenese Mol, Unidade Retrovirus Infeccoes Assoc, Lisbon, Portugal. EM ntaveira@ff.ul.pt RI iMed.ULisboa, EEPHIV /B-4222-2014; iMed.ULisboa, iMed.ULisboa/C-6292-2014; Bartolo, Ines/A-7477-2014; Rocha, Cheila/E-8776-2015; Gomes, Perpetua/I-5652-2012; Marcelino, Jose Maria/B-3374-2008; Familia, Carlos/A-4535-2013; Borrego, Pedro/H-6968-2013; Taveira, Nuno/A-6252-2014; Quintas, Alexandre/J-6436-2012 OI Barroso, Helena/0000-0003-4098-5433; Bartolo, Ines/0000-0002-2022-8921; Rocha, Cheila/0000-0002-0148-9405; Gomes, Perpetua/0000-0003-3271-8255; Montez, Patricia/0000-0002-2463-0176; Marcelino, Jose Maria/0000-0002-4597-1535; Familia, Carlos/0000-0001-5059-2487; Borrego, Pedro/0000-0002-1949-9484; Taveira, Nuno/0000-0003-0176-5585; Quintas, Alexandre/0000-0002-5188-0453 FU Fundacao para a Ciencia e Tecnologia (FCT), Portugal [PTDC/SAU-FAR/115290/2009, PTDC/SAU-EPI/122400/2010]; NIH [R01AI087520]; Collaborative HIV and Anti-HIV Drug Resistance Network (CHAIN); European Union; Fundacao para a Ciencia e Tecnologia, Portugal; Swedish Research Council [623-2011-1100] FX This work was supported by grants PTDC/SAU-FAR/115290/2009 and PTDC/SAU-EPI/122400/2010 from Fundacao para a Ciencia e Tecnologia (FCT) (http://www.fct.pt), Portugal, a NIH grant (R01AI087520), and by Collaborative HIV and Anti-HIV Drug Resistance Network (CHAIN), from the European Union. Cheila Rocha, Rita Calado, Pedro Borrego and Ines Bartolo were supported by PhD scholarships from Fundacao para a Ciencia e Tecnologia, Portugal. Helena Skar was supported by a postdoctoral fellowship from the Swedish Research Council (623-2011-1100). The following reagents were obtained through the AIDS Research and Reference Reagent Program, NR 74 TC 3 Z9 3 U1 2 U2 8 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1742-4690 J9 RETROVIROLOGY JI Retrovirology PD OCT 24 PY 2013 VL 10 AR 110 DI 10.1186/1742-4690-10-110 PG 14 WC Virology SC Virology GA 280PP UT WOS:000329043500002 PM 24156513 ER PT J AU Barouch, DH Stephenson, KE Borducchi, EN Smith, K Stanley, K McNally, AG Liu, JY Abbink, P Maxfield, LF Seaman, MS Dugast, AS Alter, G Ferguson, M Li, WJ Earl, PL Moss, B Giorgi, EE Szinger, JJ Eller, LA Billings, EA Rao, M Tovanabutra, S Sanders-Buell, E Weijtens, M Pau, MG Schuitemaker, H Robb, ML Kim, JH Korber, BT Michael, NL AF Barouch, Dan H. Stephenson, Kathryn E. Borducchi, Erica N. Smith, Kaitlin Stanley, Kelly McNally, Anna G. Liu, Jinyan Abbink, Peter Maxfield, Lori F. Seaman, Michael S. Dugast, Anne-Sophie Alter, Galit Ferguson, Melissa Li, Wenjun Earl, Patricia L. Moss, Bernard Giorgi, Elena E. Szinger, James J. Eller, Leigh Anne Billings, Erik A. Rao, Mangala Tovanabutra, Sodsai Sanders-Buell, Eric Weijtens, Mo Pau, Maria G. Schuitemaker, Hanneke Robb, Merlin L. Kim, Jerome H. Korber, Bette T. Michael, Nelson L. TI Protective Efficacy of a Global HIV-1 Mosaic Vaccine against Heterologous SHIV Challenges in Rhesus Monkeys SO CELL LA English DT Article ID SIMIAN IMMUNODEFICIENCY VIRUS; T-LYMPHOCYTE RESPONSES; NEUTRALIZING ANTIBODIES; IMMUNE CONTROL; REPLICATION; DIVERSITY; MACAQUES; BREADTH; AIDS; IMMUNOGENICITY AB The global diversity of HIV-1 represents a critical challenge facing HIV-1 vaccine development. HIV-1 mosaic antigens are bioinformatically optimized immunogens designed for improved coverage of HIV-1 diversity. However, the protective efficacy of such global HIV-1 vaccine antigens has not previously been evaluated. Here, we demonstrate the capacity of bivalent HIV-1 mosaic antigens to protect rhesus monkeys against acquisition of infection following heterologous challenges with the difficult-to-neutralize simian-human immunodeficiency virus SHIV-SF162P3. Adenovirus/poxvirus and adenovirus/adenovirus vector-based vaccines expressing HIV-1 mosaic Env, Gag, and Pol afforded a significant reduction in the per-exposure acquisition risk following repetitive, intrarectal SHIV-SF162P3 challenges. Protection against acquisition of infection correlated with vaccine-elicited binding, neutralizing, and functional nonneutralizing antibodies, suggesting that the coordinated activity of multiple antibody functions may contribute to protection against difficult-to-neutralize viruses. These data demonstrate the protective efficacy of HIV-1 mosaic antigens and suggest a potential strategy for the development of a global HIV-1 vaccine. C1 [Barouch, Dan H.; Stephenson, Kathryn E.; Borducchi, Erica N.; Smith, Kaitlin; Stanley, Kelly; McNally, Anna G.; Liu, Jinyan; Abbink, Peter; Maxfield, Lori F.; Seaman, Michael S.] Harvard Univ, Beth Israel Deaconess Med Ctr, Sch Med, Ctr Virol & Vaccine Res, Boston, MA 02215 USA. [Barouch, Dan H.; Dugast, Anne-Sophie; Alter, Galit] Ragon Inst MGH Massachusetts Inst Technol & Harva, Boston, MA 02114 USA. [Ferguson, Melissa] Alpha Genesis Inc, Yemassee, SC 29945 USA. [Li, Wenjun] Univ Massachusetts, Sch Med, Worcester, MA 01605 USA. [Earl, Patricia L.; Moss, Bernard] NIAID, Bethesda, MD 20892 USA. [Giorgi, Elena E.; Szinger, James J.; Korber, Bette T.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Eller, Leigh Anne; Billings, Erik A.; Rao, Mangala; Tovanabutra, Sodsai; Sanders-Buell, Eric; Robb, Merlin L.; Kim, Jerome H.; Michael, Nelson L.] Walter Reed Army Inst Res, US Mil HIV Res Program, Rockville, MD 20850 USA. [Weijtens, Mo; Pau, Maria G.; Schuitemaker, Hanneke] Crucell Holland BV, NL-2301 CA Leiden, Netherlands. RP Barouch, DH (reprint author), Harvard Univ, Beth Israel Deaconess Med Ctr, Sch Med, Ctr Virol & Vaccine Res, Boston, MA 02215 USA. EM dbarouch@bidmc.harvard.edu RI Li, Wenjun/F-5634-2015; Dugast, AnneSophie/L-9541-2015 OI Li, Wenjun/0000-0001-5335-7386; FU U.S. Military Research and Material Command; U.S. Military HIV Research Program [W81XWH-07-2-0067]; National Institutes of Health [AI052074, AI060354, AI078526, AI084794, AI095985, AI096040, AI100645]; NIAID Division of Intramural Research; Ragon Institute of MGH, MIT, and Harvard; Bill and Melinda Gates Foundation [OPP1033091, OPP1040741] FX We thank M. Pensiero, S. Blackmore, R. Bradsky, C. Cabral, A. Cheung, J. Goudsmit, R. Hamel, B. Hibl, S. Howell, M. Iampietro, K. Kelly, D. Lynch, M. Marovich, C. Miller, J. Nkolola, A. O'Sullivan, L. Parenteau, J. Perry, W. Rinaldi, J. Sadoff, A. SanMiguel, N. Simmons, J. Smith, F. Stephens, D. van Manen, G. Westergaard, and L. Wyatt for generous advice, assistance, and reagents. The HIV-1 PTE peptides were obtained from the NIH AIDS Research and Reference Reagent Program. We acknowledge support from the U.S. Military Research and Material Command and the U.S. Military HIV Research Program (W81XWH-07-2-0067); the National Institutes of Health (AI052074, AI060354, AI078526, AI084794, AI095985, AI096040, and AI100645); the NIAID Division of Intramural Research; the Ragon Institute of MGH, MIT, and Harvard; and the Bill and Melinda Gates Foundation (OPP1033091 and OPP1040741). M. W., M. G. P., and H. S. are employees of Crucell. Beth Israel Deaconess Medical Center and Los Alamos National Laboratory are co-owners of an HIV-1 mosaic antigen patent that has been licensed to Crucell. The opinions in this manuscript are those of the authors and do not reflect the views of the U.S. Department of the Army or the Department of Defense. NR 37 TC 103 Z9 103 U1 1 U2 12 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD OCT 24 PY 2013 VL 155 IS 3 BP 531 EP 539 DI 10.1016/j.cell.2013.09.061 PG 9 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA 246WQ UT WOS:000326571800009 PM 24243013 ER PT J AU Fang, XY Wang, JB O'Carroll, IP Mitchell, M Zuo, XB Wang, Y Yu, P Liu, Y Rausch, JW Dyba, MA Kjems, J Schwieters, CD Seifert, S Winans, RE Watts, NR Stahl, SJ Wingfield, PT Byrd, RA Le Grice, SFJ Rein, A Wang, YX AF Fang, Xianyang Wang, Jinbu O'Carroll, Ina P. Mitchell, Michelle Zuo, Xiaobing Wang, Yi Yu, Ping Liu, Yu Rausch, Jason W. Dyba, Marzena A. Kjems, Jorgen Schwieters, Charles D. Seifert, Soenke Winans, Randall E. Watts, Norman R. Stahl, Stephen J. Wingfield, Paul T. Byrd, R. Andrew Le Grice, Stuart F. J. Rein, Alan Wang, Yun-Xing TI An Unusual Topological Structure of the HIV-1 Rev Response Element SO CELL LA English DT Article ID SMALL-ANGLE SCATTERING; X-RAY-SCATTERING; GENE-EXPRESSION REQUIRES; RICH-BINDING MOTIF; BIOLOGICAL MACROMOLECULES; SECONDARY STRUCTURE; ZINC-FINGER; VIRION EXPRESSION; TRANS-ACTIVATOR; TARGET SEQUENCE AB Nuclear export of unspliced and singly spliced viral mRNA is a critical step in the HIV life cycle. The structural basis by which the virus selects its own mRNA among more abundant host cellular RNAs for export has been a mystery for more than 25 years. Here, we describe an unusual topological structure that the virus uses to recognize its own mRNA. The viral Rev response element (RRE) adopts an "A"-like structure in which the two legs constitute two tracks of binding sites for the viral Rev protein and position the two primary known Rev-binding sites similar to 55 angstrom apart, matching the distance between the two RNAbinding motifs in the Rev dimer. Both the legs of the "A" and the separation between them are required for optimal RRE function. This structure accounts for the specificity of Rev for the RRE and thus the specific recognition of the viral RNA. C1 [Fang, Xianyang; Wang, Jinbu; Zuo, Xiaobing; Yu, Ping; Liu, Yu; Wang, Yun-Xing] NCI, Prot Nucle Acid Interact Sect, Struct Biophys Lab, HIV Drug Resistance Program,Ctr Canc Res,NIH, Frederick, MD 21702 USA. [O'Carroll, Ina P.; Rein, Alan] NCI, Retroviral Assembly Sect, HIV Drug Resistance Program, Ctr Canc Res,NIH, Frederick, MD 21702 USA. [Mitchell, Michelle; Wang, Yi; Rausch, Jason W.; Le Grice, Stuart F. J.] NCI, RT Biochem Sect, HIV Drug Resistance Program, Ctr Canc Res,NIH, Frederick, MD 21702 USA. [Yu, Ping; Dyba, Marzena A.] SAIC Frederick, Struct Biophys Lab, Frederick, MD 21702 USA. [Kjems, Jorgen] Univ Aarhus, Dept Mol Biol, DK-8000 Aarhus C, Denmark. [Schwieters, Charles D.] NIH, Div Computat Biosci, Ctr Informat Technol, Bethesda, MD 20892 USA. [Seifert, Soenke; Winans, Randall E.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Watts, Norman R.; Stahl, Stephen J.; Wingfield, Paul T.] NIAMSD, Prot Express Lab, NIH, Bethesda, MD 20892 USA. [Byrd, R. Andrew] NCI, Macromol NMR Sect, Struct Biophys Lab, Ctr Canc Res,NIH, Frederick, MD 21702 USA. RP Rein, A (reprint author), NCI, Retroviral Assembly Sect, HIV Drug Resistance Program, Ctr Canc Res,NIH, Frederick, MD 21702 USA. EM reina@mail.nih.gov; wangyunx@mail.nih.gov RI Byrd, R. Andrew/F-8042-2015 OI Byrd, R. Andrew/0000-0003-3625-4232 FU Intramural Research Program of the National Institutes of Health, National Cancer Institute (NCI) Center for Cancer Research; National Institute of Arthritis, Musculoskeletal and Skin Diseases; Center for Information Technology; SAIC-Frederick [HHSN26120080001E]; U.S. DOE [DE-AC02-06CH11357] FX We thank Drs. Stephen Hughes, Alexander Wlodawer, and Prof. James Williamson for discussion. This work was supported in part by the Intramural Research Program of the National Institutes of Health, National Cancer Institute (NCI) Center for Cancer Research; National Institute of Arthritis, Musculoskeletal and Skin Diseases; Center for Information Technology; and SAIC-Frederick under contract HHSN26120080001E. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. The content of this publication does not necessarily reflect the views or policies of the Department of Health and Human Services, nor does mention of trade names, commercial products or organizations imply endorsement by the US Government. NR 57 TC 52 Z9 52 U1 3 U2 25 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD OCT 24 PY 2013 VL 155 IS 3 BP 594 EP 605 DI 10.1016/j.cell.2013.10.008 PG 12 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA 246WQ UT WOS:000326571800014 PM 24243017 ER PT J AU Zhao, J Scheibe, TD Mahadevan, R AF Zhao, Jiao Scheibe, T. D. Mahadevan, R. TI Model-based analysis of mixed uranium(VI) reduction by biotic and abiotic pathways during in situ bioremediation SO CHEMICAL GEOLOGY LA English DT Article DE Abiotic pathways; Biotic pathways; Field conditions; Mixed U(VI) reduction; Mackinawite ID SULFATE-REDUCING BACTERIA; MICROBIAL REDUCTION; CONTAMINATED AQUIFER; IRON(II); FE(III); U(VI); GROUNDWATER; SEDIMENTS; DYNAMICS; OXIDES AB Given the numerous unknowns and uncertainties in sediment systems, understanding of the mechanisms of U(VI) reduction is still at the stage of improvement. Recent studies have shown that reductive immobilization of U(VI) in the subsurface is not caused by purely biological or purely abiotic reactions but rather a group of interconnected abiotic-biotic pathways (e. g. via mackinawite and biomass). These new findings necessitate an update of the existing mathematical models that make simplifications typically involving a single reducing agent (e. g. indigenous bacteria) for in situ bioremediation of uranium-contaminated groundwater. In this study, a comprehensive model was constructed based on new experimental observations, including mixed U(VI) reduction by chemical and enzymatic reactions. Thermodynamic analysis was done to predict the feasibility of the potential pathways that affect mackinawite formation under field conditions. Model simulations indicate that low concentrations of the reactant species make the reaction of homogeneous Fe(II) oxidation coupled to U(VI) reduction unfavorable in the field. Instead, FeS precipitation is an important Fe(II) sequestration reaction once sulfate metabolism dominates. The subsequent reduction of U(VI) by FeS (mackinawite) contributes to the total U(VI) removal under a variety of U(VI) concentrations encountered at field sites, which is in accordance with experimental observations. The model suggests the potential for both competition and coordination between chemical and biological pathways on the cell surface, providing a possible explanation as to why U(VI) can be efficiently reduced at either low or high sulfate concentration during the process of in situ bioremediation. Further increase in the resolution of the model (e. g. across multiple scales such as genome-, micron- and pore-sale) is necessary for better understanding of the interactions between biotic and abiotic pathways. (C) 2013 Elsevier B.V. All rights reserved. C1 [Zhao, Jiao; Mahadevan, R.] Univ Toronto, Dept Chem Engn & Appl Chem, Biozone, Toronto, ON M5S 3E5, Canada. [Mahadevan, R.] Univ Toronto, Inst Biomat & Biomed Engn, Toronto, ON M5S 3G9, Canada. [Scheibe, T. D.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Zhao, J (reprint author), Univ Toronto, Dept Chem Engn & Appl Chem, 200 Coll St, Toronto, ON M5S 3E5, Canada. EM jiao.zhao@utoronto.ca RI Scheibe, Timothy/A-8788-2008; Mahadevan, Radhakrishnan/A-8502-2008 OI Scheibe, Timothy/0000-0002-8864-5772; Mahadevan, Radhakrishnan/0000-0002-1270-9063 FU Office of Science (BER), U.S. Department of Energy [DE-FG02-07ER64367, DE-FC02-02ER63446]; Office of Science (BER), U.S. Department of Energy from the Environmental Remediation Sciences Program FX This research was supported by the Office of Science (BER), U.S. Department of Energy from grant DE-FG02-07ER64367 from the Environmental Remediation Sciences Program and Cooperative Agreement DE-FC02-02ER63446. The Sun Grid Infrastructure was provided by Compute Canada National Resource Allocation Award 2011-2013. NR 35 TC 2 Z9 2 U1 4 U2 24 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD OCT 24 PY 2013 VL 357 BP 215 EP 222 DI 10.1016/j.chemgeo.2013.08.037 PG 8 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 246WT UT WOS:000326572300019 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Clerbaux, B De Lentdecker, G Favart, L Gay, 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CA CMS Collaboration TI Measurement of the production cross section for Z gamma -> nu(nu)over-bar gamma in pp collisions at root s=7 TeV and limits on ZZ gamma and Z gamma gamma triple gauge boson couplings SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID SECTOR; TEVATRON; LEP AB A measurement of the Z gamma -> nu(nu) over bar gamma cross section in pp collisions at root s = 7 TeV is presented, using data corresponding to an integrated luminosity of 5.0 fb(-1) collected with the CMS detector. This measurement is based on the observation of events with an imbalance of transverse energy in excess of 130 GeV and a single photon in the absolute pseudorapidity range vertical bar eta vertical bar < 1.4 with transverse energy above 145 GeV. The Z gamma -> nu<(nu)over bar>gamma production cross section is measured to be 21.1 +/- 4.2(stat.)+/- 4.3(syst.)+/- 0.5(lum.)fb, which agrees with the standard model prediction of 21.9 +/- 1.1 fb. The results are combined with the CMS measurement of Z gamma production in the l(+)l(-)gamma final state (where l is an electron or a muon) to yield the most stringent limits to date on triple gauge boson couplings. vertical bar h(3)(Z)vertical bar < 2.7 x 10(-3), vertical bar h(4)(Z)vertical bar < 1.3 x 10(-5) for ZZ gamma and vertical bar h(3)(gamma)vertical bar < 2.9 x 10(-3), vertical bar h(4)(gamma)vertical bar < 1.5 x 10(-5) for Z gamma gamma couplings. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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M.; Fahim, A.; Hesari, H.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Cufflani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cufflani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. 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T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Ventura, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; D'Agnolo, R. T.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Casasso, S.; Costa, M.; Migliore, E.; Monaco, V.; Ortona, G.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. C.; Gallinaro, M.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Laney, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Sanchez, F. J. Munoz; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Sharma, A.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Coarasa Perez, J. A.; Colafranceschi, S.; d'Enterria, D.; Dabrowski, A.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Lourenco, C.; Magini, N.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimia, M.; Piparo, D.; Plagge, M.; Polese, G.; Quertenmont, L.; Racz, A.; Reece, W.; Rolandi, G.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Taroni, S.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Gunaydin, Y. O.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Natl Sci Ctr, Kharkov Inst Phys & Technol, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Buchmuller, O.; Burton, D.; Ling, D. Col; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Mall, O.; Miceli, T.; Nelson, R.; Pellett, D.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Hanson, G.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kalavase, P.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Sen, N.; Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. 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Lopes; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Koybasi, O.; Kress, M.; Leonardo, N.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Wang, F.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Li, W.; Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Rose, K.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. 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RI Leonidov, Andrey/P-3197-2014; vilar, rocio/P-8480-2014; Dahms, Torsten/A-8453-2015; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Calderon, Alicia/K-3658-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Benussi, Luigi/O-9684-2014; Russ, James/P-3092-2014; Bartalini, Paolo/E-2512-2014; Wolszczak, Weronika/N-3113-2013; Petrushanko, Sergey/D-6880-2012; Ligabue, Franco/F-3432-2014; Wulz, Claudia-Elisabeth/H-5657-2011; Dudko, Lev/D-7127-2012; Lokhtin, Igor/D-7004-2012; Montanari, Alessandro/J-2420-2012; Cerrada, Marcos/J-6934-2014; Venturi, Andrea/J-1877-2012; Marlow, Daniel/C-9132-2014; de Jesus Damiao, Dilson/G-6218-2012; Janssen, Xavier/E-1915-2013; Novaes, Sergio/D-3532-2012; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Ragazzi, Stefano/D-2463-2009; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Mundim, Luiz/A-1291-2012; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017 OI Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Ligabue, Franco/0000-0002-1549-7107; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Dudko, Lev/0000-0002-4462-3192; Montanari, Alessandro/0000-0003-2748-6373; Cerrada, Marcos/0000-0003-0112-1691; de Jesus Damiao, Dilson/0000-0002-3769-1680; Novaes, Sergio/0000-0003-0471-8549; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Ragazzi, Stefano/0000-0001-8219-2074; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Mundim, Luiz/0000-0001-9964-7805; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; FU Austrian de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Research Promotion Foundation, Cyprus; Ministry of Education and Research [SF0690030s09]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Office for Research and Technology, Hungary; Department of Atomic Energy; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology; World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion; Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; National Science Council, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; Science and Technology Facilities Council, U.K.; US Department of Energy; US National Science Foundation; Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU, Regional Development Fund; Thalis and Aristeia programmes; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Recurrent financing contract SF0690030s09 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Office for Research and Technology, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the National Science Council, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the Science and Technology Facilities Council, U.K.; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 35 TC 3 Z9 3 U1 3 U2 94 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 24 PY 2013 IS 10 AR 164 DI 10.1007/JHEP10(2013)164 PG 30 WC Physics, Particles & Fields SC Physics GA 241TJ UT WOS:000326190500001 ER PT J AU Chen, L Alarcon-Llado, E Hettick, M Sharp, ID Lin, YJ Javey, A Ager, JW AF Chen, Le Alarcon-Llado, Esther Hettick, Mark Sharp, Ian D. Lin, Yongjing Javey, Ali Ager, Joel W. TI Reactive Sputtering of Bismuth Vanadate Photoanodes for Solar Water Splitting SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID VISIBLE-LIGHT IRRADIATION; PHOTOCATALYTIC PROPERTIES; BIVO4; EFFICIENT; OXIDATION; COMPOSITE; PHOTOELECTRODES; TEMPERATURE; DEPOSITION; MECHANISM AB Bismuth vanadate (BiVO4) has attracted increasing attention as a photoanode for photoelectrochemical (PEC) water splitting. It has a band gap in the visible light range (2.4-2.5 eV) and a valence band position suitable for driving water oxidation under illumination. While a number of methods have been used to make BiVO4 photoanodes, scalable thin film deposition has remained relatively underexplored. Here, we report the synthesis of BiVO4 thin films by reactive sputtering. The use of separate Bi and V sputtering targets allows control of the Bi/V ratio in the film. Under optimized, slightly V-rich conditions, monoclinic phase BiVO4 with photoactivity for water oxidation is obtained. The highest photocurrents, ca. 1 mA cm(-2) at the reversible O-2/H2O potential with simulated AM 1.5G illumination, are obtained with bilayer WO3/BiVO4, where the WO3 serves as a hole-blocking layer. C1 [Chen, Le; Alarcon-Llado, Esther; Hettick, Mark; Sharp, Ian D.; Lin, Yongjing; Javey, Ali; Ager, Joel W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Chen, Le; Alarcon-Llado, Esther; Hettick, Mark; Lin, Yongjing; Javey, Ali; Ager, Joel W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Sharp, Ian D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Alarcon-Llado, Esther] Ecole Polytech Fed Lausanne, Lausanne, Switzerland. [Hettick, Mark; Lin, Yongjing; Javey, Ali] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. RP Ager, JW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, MS62R0203,1 Cyclotron Rd, Berkeley, CA 94720 USA. EM JWAger@lbl.gov RI Sharp, Ian/I-6163-2015; Javey, Ali/B-4818-2013; OI Sharp, Ian/0000-0001-5238-7487; Ager, Joel/0000-0001-9334-9751; Alarcon Llado, Esther/0000-0001-7317-9863 FU Office of Science of the U.S. Department of Energy [DE-SC0004993]; Marie Curie Actions Program FX This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DE-SC0004993. E.A.L. also acknowledges fellowship support from Marie Curie Actions Program. NR 36 TC 52 Z9 52 U1 6 U2 101 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 24 PY 2013 VL 117 IS 42 BP 21635 EP 21642 DI 10.1021/jp406019r PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 242RP UT WOS:000326260000002 ER PT J AU Choi, WI Wood, BC Schwegler, E Ogitsu, T AF Choi, Woon Ih Wood, Brandon C. Schwegler, Eric Ogitsu, Tadashi TI Site-Dependent Free Energy Barrier for Proton Reduction on MoS2 Edges SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID HYDROGEN EVOLUTION; SOLAR-ENERGY; ELECTROCATALYSIS; NANOCATALYSTS; NANOPARTICLES; NANOCLUSTERS; CATALYST; CELLS AB We calculated the adiabatic free energy surface of the proton reduction reaction on catalytically active MoS2 edge atoms by combining density functional theory with the Anderson-Newns model, which accounts for solvent fluctuation and charge transfer in the context of Marcus theory. This framework combines three different contributions to the associated reaction energetics and kinetics, namely, the relevant electronic orbitals of the substrate, the possibility of surface relaxation upon adsorption, and the impact of solvation. Under the assumption of fixed edge geometry throughout the reaction, we calculate the free energy barriers on edge S and Mo sites to be 0.65 and 0 eV, respectively. However, if we consider surface relaxation, the barrier on the edge S site is reduced by more than half to 0.31 eV. On edge Mo sites, the d(z)(2) orbital is responsible not only for the strength of binding but also for the barrierless reaction. On edge S sites, the bound hydrogen atom always retains some finite positive charge, which indicates that it remains partially solvated even after surface binding. In this case, it is crucial to account for the solvation energy in addition to the gas-phase adsorption energy when assessing hydrogen catalysis. C1 [Choi, Woon Ih; Wood, Brandon C.; Schwegler, Eric; Ogitsu, Tadashi] Lawrence Livermore Natl Lab, Quantum Simulat Grp, Livermore, CA 94550 USA. RP Ogitsu, T (reprint author), Lawrence Livermore Natl Lab, Quantum Simulat Grp, Livermore, CA 94550 USA. EM ogitsu1@llnl.gov RI Schwegler, Eric/A-2436-2016; OI Schwegler, Eric/0000-0003-3635-7418; Choi, Woon Ih/0000-0002-7183-3400 FU U.S. Department of Energy Fuel Cell Technologies Program; Laboratory Directed Research and Development (LDRD) Program of Lawrence Livermore National Laboratory (LLNL); U.S. Department of Energy by LLNL [DE-AC52-07NA27344] FX The authors acknowledge helpful discussions with E. Santos (U. of Ulm, Germany). We also gratefully acknowledge funding support from the U.S. Department of Energy Fuel Cell Technologies Program and Laboratory Directed Research and Development (LDRD) Program of Lawrence Livermore National Laboratory (LLNL). Computing support came from the Lawrence Livermore National Laboratory (LLNL) Institutional Computing Grand Challenge program. This work was performed under the auspices of the U.S. Department of Energy by LLNL under Contract DE-AC52-07NA27344. NR 31 TC 11 Z9 13 U1 1 U2 43 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 EI 1932-7455 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 24 PY 2013 VL 117 IS 42 BP 21772 EP 21777 DI 10.1021/jp405354u PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 242RP UT WOS:000326260000017 ER PT J AU Alayoglu, S Beaumont, SK Melaet, G Lindeman, AE Musselwhite, N Brooks, CJ Marcus, MA Guo, JG Liu, Z Kruse, N Somorjai, GA AF Alayoglu, Selim Beaumont, Simon K. Melaet, Gerome Lindeman, Avery E. Musselwhite, Nathan Brooks, Christopher J. Marcus, Matthew A. Guo, Jingua Liu, Zhi Kruse, Norbert Somorjai, Gabor A. TI Surface Composition Changes of Redox Stabilized Bimetallic CoCu Nanoparticles Supported on Silica under H-2 and O-2 Atmospheres and During Reaction between CO2 and H-2: In Situ X-ray Spectroscopic Characterization SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID FISCHER-TROPSCH SYNTHESIS; METHANOL SYNTHESIS; PHOTOELECTRON-SPECTROSCOPY; SYNTHESIS CATALYSTS; COBALT CATALYSTS; HYDROGENATION; SELECTIVITY; KINETICS; SCIENCE; DESIGN AB In this paper, we report the colloidal synthesis and detailed characterization of 11 nm bimetallic CoCu nanoparticle catalysts. Presently Co and Cu is an attractive combination because of their respective properties for industrially important Fischer-Tropsch and methanol synthesis reactions of CO (and CO2) with H-2. We report the preparation of catalysts by deposition of bimetallic metal nanoparticles, both within mesoporous silica (MCF-17) and on the native oxide surface of a silicon wafer. Subsequent phase separation into phase-segregated (i.e., dimer) particles is found to occur upon redox treatment. These nanoparticle catalysts have then been investigated using an array of techniques including synchrotron-based ambient pressure X-ray photoelectron spectroscopy (APXPS) and in situ near edge and extended X-ray absorption fine structure (NEXAFS/EXAFS) spectroscopies. CO2 hydrogenation is used as a probe reaction. All three techniques combine to show that an oxygen atmosphere segregates copper to the surface. In doing so the oxygen produces oxides of both Co and Cu metals. Significant hydrogen pressure and temperature are required to fully rereduce both metals to a metallic state as demonstrated by NEXAFS spectroscopy. Under the conditions of the CO2/H-2 reaction monitored in situ using NEXAFS spectroscopy, both metals exist in a fully reduced state at 2.7 bar, 1:3 CO2:H-2, and 260 degrees C. C1 [Alayoglu, Selim; Beaumont, Simon K.; Melaet, Gerome; Lindeman, Avery E.; Musselwhite, Nathan; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94704 USA. [Alayoglu, Selim; Beaumont, Simon K.; Melaet, Gerome; Lindeman, Avery E.; Musselwhite, Nathan; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Brooks, Christopher J.] Honda Res Inst, Columbus, OH 43212 USA. [Marcus, Matthew A.; Guo, Jingua; Liu, Zhi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Kruse, Norbert] Univ Libre Bruxelles, B-1050 Brussels, Belgium. RP Somorjai, GA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94704 USA. EM somorjai@berkeley.edu RI Liu, Zhi/B-3642-2009; Melaet, Gerome/N-4879-2015; Foundry, Molecular/G-9968-2014; Beaumont, Simon/F-5272-2012 OI Liu, Zhi/0000-0002-8973-6561; Melaet, Gerome/0000-0003-1414-1683; Beaumont, Simon/0000-0002-1973-9783 FU Office of Energy Research, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Honda Research Institute, USA FX The user projects in the Advanced Light Source and Molecular Foundry at the Lawrence Berkeley National Laboratory were supported by the Director, Office of Energy Research, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract DE-AC02-05CH11231. We acknowledge Honda Research Institute, USA for the financial support. NR 36 TC 14 Z9 14 U1 3 U2 59 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 24 PY 2013 VL 117 IS 42 BP 21803 EP 21809 DI 10.1021/jp405745n PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 242RP UT WOS:000326260000021 ER PT J AU Wong, CY Penwell, SB Cotts, BL Noriega, R Wu, H Ginsberg, NS AF Wong, Cathy Y. Penwell, Samuel B. Cotts, Benjamin L. Noriega, Rodrigo Wu, Hao Ginsberg, Naomi S. TI Revealing Exciton Dynamics in a Small-Molecule Organic Semiconducting Film with Subdomain Transient Absorption Microscopy SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PUMP-PROBE SPECTROSCOPY; CHARGE-TRANSFER STATE; SOLAR-CELLS; FUNCTIONALIZED PENTACENE; SINGLET FISSION; ULTRAFAST DYNAMICS; QUANTUM EFFICIENCY; PHOTOVOLTAIC CELLS; POLYMER BLENDS; FREE-CARRIER AB The ultrafast spectroscopy of single domains of polycrystalline films of TIPS-pentacene, a small-molecule organic semiconductor of interest in electronic and photovoltaic applications, is investigated using transient absorption microscopy. Individual domains are distinguished by their different polarization-dependent linear and nonlinear optical responses. As compared to bulk measurements, we show that the nonlinear response within a given domain can be tied more concretely to specific physical processes that transfer exciton populations between specified electronic states. By use of this approach and a simple kinetic model, the signatures of singlet fission as well as vibrational relaxation of the initially excited singlet state are identified. As such, observing exciton dynamics within and comparing exciton dynamics between different TIPS-pentacene domains reveal the relationship between photophysics and film morphology needed to improve device performance. C1 [Wong, Cathy Y.; Penwell, Samuel B.; Cotts, Benjamin L.; Noriega, Rodrigo; Wu, Hao; Ginsberg, Naomi S.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Ginsberg, Naomi S.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Ginsberg, Naomi S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci & Mat Sci Div, Berkeley, CA 94720 USA. [Ginsberg, Naomi S.] Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. RP Ginsberg, NS (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM nsginsberg@berkeley.edu FU Defense Advanced Research Projects Agency Young Faculty Award [N66001-12-1-4228]; Natural Sciences and Engineering Research Council, Canada; Department of Energy Office of Science Graduate Research Fellowship [DE-AC05-060R23100]; National Science Foundation Graduate Research Fellowship [DGE 1106400]; Philomathia Foundation; David and Lucile Packard Foundation Fellowship for Science and Engineering FX This work has been supported by the Defense Advanced Research Projects Agency Young Faculty Award number N66001-12-1-4228. C.Y.W. thanks the Natural Sciences and Engineering Research Council, Canada, for a Postdoctoral Fellowship. S.B.P. acknowledges a Department of Energy Office of Science Graduate Research Fellowship, made possible in part by the American Recovery and Reinvestment Act of 2009, administered by ORISE-ORAU under contract no. DE-AC05-060R23100; B.L.C. acknowledges a National Science Foundation Graduate Research Fellowship (DGE 1106400); RN. acknowledges the Philomathia Foundation for support; and N.S.G. acknowledges a David and Lucile Packard Foundation Fellowship for Science and Engineering. We also thank V. Ho and R. Segalman for advice in sample preparation. NR 91 TC 24 Z9 24 U1 10 U2 97 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 EI 1932-7455 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 24 PY 2013 VL 117 IS 42 BP 22111 EP 22122 DI 10.1021/jp407645k PG 12 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 242RP UT WOS:000326260000059 ER PT J AU Petkov, V Shastri, S Shan, SY Joseph, P Luo, J Zhong, CJ Nakamura, T Herbani, Y Sato, S AF Petkov, Valeri Shastri, Sarvjit Shan, Shiyao Joseph, Pharrah Luo, Jin Zhong, Chuan-Jian Nakamura, Takahiro Herbani, Yuliati Sato, Shunichi TI Resolving Atomic Ordering Differences in Group 11 Nanosized Metals and Binary Alloy Catalysts by Resonant High-Energy X-ray Diffraction and Computer Simulations SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID INTERMETALLIC COMPOUNDS; SOLID-SOLUTIONS; SHORT-RANGE; NANOPARTICLES; PARTICLES; CRYSTALS; SIZE; NANOCLUSTERS; OXIDATION; SURFACES AB Resonant high-energy X-ray diffraction coupled to atomic pair distribution function analysis and computer simulations is used to study the atomic-scale structure of group 11 nanosized metals and binary alloy catalysts. We find that nanosized Cu is quite disordered structurally whereas nanosized Ag and especially Au exhibit a very good degree of crystallinity. We resolve CuCu and AgAg atomic correlations from Au-involving ones in AuCu and AuAg nanoalloys and show that depending on the synthetic route group 11 binary alloys may adopt structural states that obey or markedly violate Vegards law. In the latter case, Cu and Ag atoms undergo substantial size expansion and contraction by as much as 0.3 and 0.03 angstrom, respectively, while heavier Au atoms remain practically intact. The size change of Cu and Ag atoms does not follow Paulings rule of electronegativity predicting charge flow toward the more electronegative Au but occurs in a way such that Cu/Au and Ag/Au atomic size ratios in the nanoalloys become closer to one. Atomic size adjusting and the concurrent charge redistribution result in a synergistic effect of oxygen inactive Au and oxygen very active Cu and Ag leading to nanoalloys with very good activity for low-temperature oxidation of CO. C1 [Petkov, Valeri] Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. [Shastri, Sarvjit] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Shan, Shiyao; Joseph, Pharrah; Luo, Jin; Zhong, Chuan-Jian] SUNY Binghamton, Dept Chem, Binghamton, NY 13902 USA. [Nakamura, Takahiro; Sato, Shunichi] Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Aoba Ku, Sendai, Miyagi 9808577, Japan. [Herbani, Yuliati] Indonesian Inst Sci, Res Ctr Phys, Serpong 15314, Tangerang Bante, Indonesia. RP Petkov, V (reprint author), Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. EM petko1vg@cmich.edu RI Zhong, Chuan-Jian/D-3394-2013 FU DOE-BES [DE-SC0006877]; DOE [DEAC02-06CH11357] FX Work on this paper was supported by DOE-BES Grant DE-SC0006877. Work at the Advanced Photon Source was supported by DOE under Contract DEAC02-06CH11357. NR 44 TC 12 Z9 12 U1 4 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 24 PY 2013 VL 117 IS 42 BP 22131 EP 22141 DI 10.1021/jp408017v PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 242RP UT WOS:000326260000061 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Eroe, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T DeWolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, 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