FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Halverson, JD Lee, WB Grest, GS Grosberg, AY Kremer, K AF Halverson, Jonathan D. Lee, Won Bo Grest, Gary S. Grosberg, Alexander Y. Kremer, Kurt TI Molecular dynamics simulation study of nonconcatenated ring polymers in a melt. I. Statics SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID ARM STAR POLYMERS; CHROMOSOME TERRITORIES; TOPOLOGICAL CONSTRAINTS; COMPUTER-SIMULATION; ENTANGLEMENT LENGTH; CYCLIC POLYSTYRENE; FIXED OBSTACLES; MODEL; CHAIN; CONFORMATION AB Molecular dynamics simulations were conducted to investigate the structural properties of melts of nonconcatenated ring polymers and compared to melts of linear polymers. The longest rings were composed of N = 1600 monomers per chain which corresponds to roughly 57 entanglement lengths for comparable linear polymers. For the rings, the radius of gyration squared, < R-g(2)>, was found to scale as N-4/5 for an intermediate regime and N-2/3 for the larger rings indicating an overall conformation of a crumpled globule. However, almost all beads of the rings are "surface beads" interacting with beads of other rings, a result also in agreement with a primitive path analysis performed in the next paper [J. D. Halverson, W. Lee, G. S. Grest, A. Y. Grosberg, and K. Kremer, J. Chem. Phys. 134, 204905 (2011)]. Details of the internal conformational properties of the ring and linear polymers as well as their packing are analyzed and compared to current theoretical models. (C) 2011 American Institute of Physics. [doi:10.1063/1.3587137] C1 [Halverson, Jonathan D.; Lee, Won Bo; Kremer, Kurt] Max Planck Inst Polymer Res, D-55128 Mainz, Germany. [Lee, Won Bo] Sogang Univ, Dept Chem & Biomol Engn, Seoul, South Korea. [Grest, Gary S.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Grosberg, Alexander Y.] NYU, Dept Phys, New York, NY 10003 USA. RP Kremer, K (reprint author), Max Planck Inst Polymer Res, Ackermannweg 10, D-55128 Mainz, Germany. EM kremer@mpip-mainz.mpg.de RI Kremer, Kurt/G-5652-2011; MPIP, Theory/I-9884-2014; Grosberg, Alexander/O-2122-2015; OI Grosberg, Alexander/0000-0002-4230-8690; Lee, Won Bo/0000-0001-7801-083X FU Alexander von Humboldt Foundation; Ministry of Education, Science and Technology [2010-0007886]; Multiscale Materials Modeling (MMM) initiative of the Max Planck Society; Sandia National Laboratories; United States Department of Energy [DE-AC04-94AL85000] FX The authors are grateful to T. Vilgis, T. Vettorel, and V. Harmandaris for their comments on an early version of the manuscript. The ESPResSo development team is acknowledged for optimizing the simulation software on the IBM Blue Gene/P at the Rechenzentrum Garching in Munich, Germany. We thank Donghui Zhang for discussions and references relating to experimental studies on cyclic polymers. This project was in part funded by the Alexander von Humboldt Foundation through a research grant awarded to A.Y.G. A.Y.G. also acknowledges the hospitality of the Aspen Center for Physics where part of this work was done. W. B. L. acknowledges financial support from the Alexander von Humboldt Foundation and the Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science and Technology (2010-0007886). Additional funding was provided by the Multiscale Materials Modeling (MMM) initiative of the Max Planck Society. We thank the New Mexico Computing Application Center (NMCAC) for a generous allocation of computer time. This work is supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract No. DE-AC04-94AL85000. NR 77 TC 91 Z9 92 U1 6 U2 53 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 28 PY 2011 VL 134 IS 20 AR 204904 DI 10.1063/1.3587137 PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 770SD UT WOS:000291107900063 PM 21639474 ER PT J AU Meredith, NP Horne, RB Lam, MM Denton, MH Borovsky, JE Green, JC AF Meredith, Nigel P. Horne, Richard B. Lam, Mai Mai Denton, Michael H. Borovsky, Joseph E. Green, Janet C. TI Energetic electron precipitation during high-speed solar wind stream driven storms SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article ID COROTATING INTERACTION REGIONS; RECURRENT GEOMAGNETIC STORMS; OUTER RADIATION BELT; MAGNETIC STORMS; RELATIVISTIC ELECTRONS; PARTICLE-PRECIPITATION; PLASMASPHERIC HISS; CHORUS EMISSIONS; PLASMA SHEET; ACCELERATION AB Electron precipitation from the Earth's inner magnetosphere transmits solar variability to the Earth's upper atmosphere and may affect surface level climate. Here we conduct a superposed epoch analysis of energetic electrons observed by the NOAA POES spacecraft during 42 high-speed solar wind stream (HSS) driven geomagnetic storms to determine the temporal evolution and global distribution of the precipitating flux. The flux of trapped and precipitating E > 30 keV electrons increases immediately following storm onset and remains elevated during the passage of the HSS. In contrast, the trapped and precipitating relativistic electrons (E > 1 MeV) drop out following storm onset and subsequently increase during the recovery phase to levels which eventually exceed the prestorm levels. There is no evidence for enhanced precipitation of relativistic electrons during the MeV flux drop out, suggesting that flux drop outs during the main phase of HSS-driven storms are not due to precipitation to the atmosphere. On average, the flux of precipitating E > 30 keV electrons is enhanced by a factor of similar to 10 during the passage of the high-speed stream at all geographic longitudes. In contrast, the precipitating relativistic electron count rate is observed to peak in the region poleward of the South Atlantic Anomaly. During the passage of the high-speed stream, the flux of precipitating E > 30 keV electrons peaks in the region from 2100 to 1200 magnetic local time at low L (4 < L < 7) and in the prenoon sector at high L (7 < L < 9), suggesting that chorus waves are responsible for the precipitation of E > 30 keV electrons in both regions. C1 [Meredith, Nigel P.; Horne, Richard B.] British Antarctic Survey, NERC, Cambridge CB3 0ET, England. [Lam, Mai Mai] Univ Leicester, Dept Phys & Astron, Leicester LE1 7RH, Leics, England. [Denton, Michael H.] Univ Lancaster, Dept Phys, Lancaster LA1 4YW, England. [Borovsky, Joseph E.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Green, Janet C.] NOAA, Space Weather Predict Ctr, Boulder, CO 80305 USA. RP Meredith, NP (reprint author), British Antarctic Survey, NERC, Madingley Rd, Cambridge CB3 0ET, England. EM nmer@bas.ac.uk; r.horne@bas.ac.uk; mml9@ion.le.ac.uk; m.denton@lancaster.ac.uk; jborovsky@lanl.gov; janet.green@noaa.gov OI Horne, Richard/0000-0002-0412-6407; Meredith, Nigel/0000-0001-5032-3463; Denton, Michael/0000-0002-1748-3710 FU Natural Environment Research Council; STFC [ST/G002401/1/] FX We thank the NSSDC Omniweb for providing the geomagnetic indices and solar wind parameters used in this study. This work was supported, in part, by the Natural Environment Research Council. J.E.B. and M. H. D. would like to thank all at BAS for their hospitality during their visit in Spring 2010. Work at Lancaster was supported by STFC grant ST/G002401/1/. NR 84 TC 53 Z9 53 U1 0 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAY 28 PY 2011 VL 116 AR A05223 DI 10.1029/2010JA016293 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 770RX UT WOS:000291107300004 ER PT J AU Mishra, PK Neuman, SP AF Mishra, Phoolendra Kumar Neuman, Shlomo P. TI Saturated-unsaturated flow to a well with storage in a compressible unconfined aquifer SO WATER RESOURCES RESEARCH LA English DT Article ID HYDRAULIC CONDUCTIVITY; NUMERICAL INVERSION; PARTIAL PENETRATION; LAPLACE TRANSFORMS; DRAINAGE; WATER; MODEL; DIAMETER AB Mishra and Neuman (2010) developed an analytical solution for flow to a partially penetrating well of zero radius in a compressible unconfined aquifer that allows inferring its saturated and unsaturated hydraulic properties from responses recorded in the saturated and/or unsaturated zones. Their solution accounts for horizontal as well as vertical flows in each zone. It represents unsaturated zone constitutive properties in a manner that is at once mathematically tractable and sufficiently flexible to provide much improved fits to standard constitutive models. In this paper we extend the solution of Mishra and Neuman [2010] to the case of a finite diameter pumping well with storage; investigate the effects of storage in the pumping well and delayed piezometer response on drawdowns in the saturated and unsaturated zones as functions of position and time; validate our solution against numerical simulations of drawdown in a synthetic aquifer having unsaturated properties described by the van Genuchten [1980]-Mualem [1976] model; use our solution to analyze 11 transducer-measured drawdown records from a seven-day pumping test conducted by University of Waterloo researchers at the Canadian Forces Base Borden in Ontario, Canada; validate our parameter estimates against manually-measured drawdown records in 14 other piezometers at Borden; and compare (a) our estimates of aquifer parameters with those obtained on the basis of all these records by Moench [2008], (b) on the basis of 11 transducer-measured drawdown records by Endres et al. [2007], (c) our estimates of van Genuchten-Mualem parameters with those obtained on the basis of laboratory drainage data from the site by Akindunni and Gillham [1992], and (d) our corresponding prediction of how effective saturation varies with elevation above the initial water table under static conditions with a profile based on water contents measured in a neutron access tube at a radial distance of about 5 m from the center of the pumping well. We also use our solution to analyze 11 transducer-measured drawdown records from a 7 day pumping test conducted by University of Waterloo researchers at the Canadian Forces Base Borden in Ontario, Canada. We validate our parameter estimates against manually measured drawdown records in 14 other piezometers at Borden. We compare our estimates of aquifer parameters with those obtained on the basis of all these records by Moench (2008) and on the basis of 11 transducer-measured drawdown records by Endres et al. (2007), and we compare our estimates of van Genuchten-Mualem parameters with those obtained on the basis of laboratory drainage data from the site by Akindunni and Gillham (1992); finally, we compare our corresponding prediction of how effective saturation varies with elevation above the initial water table under static conditions with a profile based on water contents measured in a neutron access tube at a radial distance of about 5 m from the center of the pumping well. C1 [Mishra, Phoolendra Kumar; Neuman, Shlomo P.] Univ Arizona, Dept Hydrol & Water Resources, Tucson, AZ 85721 USA. RP Mishra, PK (reprint author), Los Alamos Natl Lab, Hydrol Geochem & Geol Grp, MS T003, Los Alamos, NM 87545 USA. EM neuman@hwr.arizona.edu RI Mishra, Phoolendra/A-1927-2012 FU Vanderbilt University under the Consortium of Risk Evaluation with Stakeholder Participation (CRESP) III; U.S. Department of Energy FX This research was supported in part through a contract with Vanderbilt University under the Consortium of Risk Evaluation with Stakeholder Participation (CRESP) III, funded by the U.S. Department of Energy. NR 29 TC 15 Z9 15 U1 2 U2 17 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 J9 WATER RESOUR RES JI Water Resour. Res. PD MAY 28 PY 2011 VL 47 AR W05553 DI 10.1029/2010WR010177 PG 15 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA 770TJ UT WOS:000291111100017 ER PT J AU Pindzola, MS Ludlow, JA Ballance, CP Robicheaux, F Colgan, J AF Pindzola, M. S. Ludlow, J. A. Ballance, C. P. Robicheaux, F. Colgan, J. TI Electron-impact double ionization of B+ SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article ID CROSS-SECTIONS; HELIUM; IONS AB Time-dependent close-coupling and time-independent distorted-wave methods are used to calculate the electron-impact double-ionization cross section for the 1s(2)2s(2) ground configuration of the B+ atomic ion. The direct double-ionization cross section is calculated using the non-perturbative close-coupling method between the direct double-ionization threshold of 63.1 eV and the 1s ionization threshold of 218.4 eV. The indirect single ionization-autoionization cross section is calculated using the perturbative distorted-wave method between the 1s ionization threshold of 218.4 and 750 eV. The double-ionization cross section calculated using the two methods is compared with a crossed-beam experiment over the entire energy range. C1 [Pindzola, M. S.; Ludlow, J. A.; Ballance, C. P.; Robicheaux, F.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Colgan, J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. RP Pindzola, MS (reprint author), Auburn Univ, Dept Phys, Auburn, AL 36849 USA. RI Robicheaux, Francis/F-4343-2014; OI Robicheaux, Francis/0000-0002-8054-6040; Colgan, James/0000-0003-1045-3858 FU US Department of Energy; US National Science Foundation FX We would like to thank Professor Alfred Muller of the University of Giessen for sending us the experimental data for the electron-impact double ionization of B+. This work was supported in part by grants from the US Department of Energy and the US National Science Foundation. Computational work was carried out at the National Energy Research Scientific Computing Center in Oakland, CA, and at the National Institute for Computational Sciences in Oak Ridge, TN. NR 12 TC 9 Z9 9 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD MAY 28 PY 2011 VL 44 IS 10 AR 105202 DI 10.1088/0953-4075/44/10/105202 PG 4 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 762DQ UT WOS:000290452900013 ER PT J AU Keeling, RF Manning, AC Dubey, MK AF Keeling, Ralph F. Manning, Andrew C. Dubey, Manvendra K. TI The atmospheric signature of carbon capture and storage SO PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES LA English DT Article DE carbon capture and storage; geosequestration; leak detection; atmospheric oxygen; carbon-13; carbon-14 ID GENERAL-CIRCULATION MODEL; BOX-DIFFUSION; CO2; DIOXIDE; OXYGEN; SINKS; O-2; VERIFICATION; GAS; AIR AB Compared with other industrial processes, carbon capture and storage (CCS) will have an unusual impact on atmospheric composition by reducing the CO2 released from fossil-fuel combustion plants, but not reducing the associated O-2 loss. CO2 that leaks into the air from below-ground CCS sites will also be unusual in lacking the O-2 deficit normally associated with typical land CO2 sources, such as from combustion or ecosystem exchanges. CCS may also produce distinct isotopic changes in atmospheric CO2. Using simple models and calculations, we estimate the impact of CCS or leakage on regional atmospheric composition. We also estimate the possible impact on global atmospheric composition, assuming that the technology is widely adopted. Because of its unique signature, CCS may be especially amenable to monitoring, both regionally and globally, using atmospheric observing systems. Measurements of the O-2/N-2 ratio and the CO2 concentration in the proximity of a CCS site may allow detection of point leaks of the order of 1000 ton CO2 yr(-1) from a CCS reservoir up to 1km from the source. Measurements of O-2/N-2 and CO2 in background air from a global network may allow quantification of global and hemispheric capture rates from CCS to the order of +/- 0.4 PgCyr(-1). C1 [Keeling, Ralph F.] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA. [Manning, Andrew C.] Univ E Anglia, Sch Environm Sci, Norwich NR4 7TJ, Norfolk, England. [Dubey, Manvendra K.] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. RP Keeling, RF (reprint author), Univ Calif San Diego, Scripps Inst Oceanog, 9500 Gilman Dr, La Jolla, CA 92093 USA. EM rkeeling@ucsd.edu RI Dubey, Manvendra/E-3949-2010; Manning, Andrew/D-4416-2011 OI Dubey, Manvendra/0000-0002-3492-790X; Manning, Andrew/0000-0001-6952-7773 FU UK NERC/QUEST [NE/C002504/1]; US NSF [ATM-0632770, ATM-0651834]; DoE [DE-FG02-07ER64362]; NOAA [2007-2000636] FX We thank David Bowling (University of Utah) and Elena Kozlova (University of East Anglia) for providing data shown in figures 2 and 3, respectively. We thank David Etheridge for providing access to the Otway modelling results and other helpful comments. A. C. M. is supported by a UK NERC/QUEST Advanced Fellowship (ref. no. NE/C002504/1). R. F. K. has been supported under grants from the US NSF (ATM-0632770, ATM-0651834), DoE (DE-FG02-07ER64362) and NOAA (2007-2000636). M. K. D. thanks LANL's Laboratory Directed Research and Development Program for nurturing his work in direct air capture of CO2 and CCS. NR 47 TC 10 Z9 10 U1 0 U2 26 PU ROYAL SOC PI LONDON PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND SN 1364-503X EI 1471-2962 J9 PHILOS T R SOC A JI Philos. Trans. R. Soc. A-Math. Phys. Eng. Sci. PD MAY 28 PY 2011 VL 369 IS 1943 BP 2113 EP 2132 DI 10.1098/rsta.2011.0016 PG 20 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 751LK UT WOS:000289619100016 PM 21502179 ER PT J AU Avci, S Chmaissem, O Goremychkin, EA Rosenkranz, S Castellan, JP Chung, DY Todorov, IS Schlueter, JA Claus, H Kanatzidis, MG Daoud-Aladine, A Khalyavin, D Osborn, R AF Avci, S. Chmaissem, O. Goremychkin, E. A. Rosenkranz, S. Castellan, J-P. Chung, D. Y. Todorov, I. S. Schlueter, J. A. Claus, H. Kanatzidis, M. G. Daoud-Aladine, A. Khalyavin, D. Osborn, R. TI Magnetoelastic coupling in the phase diagram of Ba1-xKxFe2As2 as seen via neutron diffraction SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC ORDER; SUPERCONDUCTIVITY; COEXISTENCE AB We report a high resolution neutron diffraction investigation of the coupling of structural and magnetic transitions in Ba1-xKxFe2As2. The tetragonal-orthorhombic and antiferromagnetic transitions are suppressed with potassium doping, falling to zero at x less than or similar to 0.24. However, unlike Ba(Fe1-xCox)(2)As-2, the two transitions are first order and coincident over the entire phase diagram, with a biquadratic coupling of the two order parameters. The phase diagram is refined showing that the onset of superconductivity is at x = 0.133 with all three phases coexisting until x <= 0.24. C1 [Avci, S.; Chmaissem, O.; Goremychkin, E. A.; Rosenkranz, S.; Castellan, J-P.; Chung, D. Y.; Todorov, I. S.; Schlueter, J. A.; Claus, H.; Kanatzidis, M. G.; Osborn, R.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Chmaissem, O.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Kanatzidis, M. G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Daoud-Aladine, A.; Khalyavin, D.] Rutherford Appleton Lab, ISIS Pulsed Neutron & Muon Facil, Didcot OX11 0QX, Oxon, England. RP Avci, S (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RI Osborn, Raymond/E-8676-2011; Rosenkranz, Stephan/E-4672-2011; Khalyavin, Dmitry/E-4335-2017 OI Osborn, Raymond/0000-0001-9565-3140; Rosenkranz, Stephan/0000-0002-5659-0383; Khalyavin, Dmitry/0000-0002-6724-7695 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We acknowledge valuable discussions with I. Paul and A. Cano. Work supported by US Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract No. DE-AC02-06CH11357. NR 30 TC 60 Z9 60 U1 1 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 27 PY 2011 VL 83 IS 17 AR 172503 DI 10.1103/PhysRevB.83.172503 PG 4 WC Physics, Condensed Matter SC Physics GA 769LP UT WOS:000291015400002 ER PT J AU Gates, JM Dullmann, CE Schadel, M Yakushev, A Turler, A Eberhardt, K Kratz, JV Ackermann, D Andersson, LL Block, M Bruchle, W Dvorak, J Essel, HG Ellison, PA Even, J Forsberg, U Gellanki, J Gorshkov, A Graeger, R Gregorich, KE Hartmann, W Herzberg, RD Hessberger, FP Hild, D Hubner, A Jager, E Khuyagbaatar, J Kindler, B Krier, J Kurz, N Lahiri, S Liebe, D Lommel, B Maiti, M Nitsche, H Omtvedt, JP Parr, E Rudolph, D Runke, J Schaffner, H Schausten, B Schimpf, E Semchenkov, A Steiner, J Thorle-Pospiech, P Uusitalo, J Wegrzecki, M Wiehl, N AF Gates, J. M. Duellmann, Ch E. Schaedel, M. Yakushev, A. Tuerler, A. Eberhardt, K. Kratz, J. V. Ackermann, D. Andersson, L. -L. Block, M. Bruechle, W. Dvorak, J. Essel, H. G. Ellison, P. A. Even, J. Forsberg, U. Gellanki, J. Gorshkov, A. Graeger, R. Gregorich, K. E. Hartmann, W. Herzberg, R. -D. Hessberger, F. P. Hild, D. Huebner, A. Jaeger, E. Khuyagbaatar, J. Kindler, B. Krier, J. Kurz, N. Lahiri, S. Liebe, D. Lommel, B. Maiti, M. Nitsche, H. Omtvedt, J. P. Parr, E. Rudolph, D. Runke, J. Schaffner, H. Schausten, B. Schimpf, E. Semchenkov, A. Steiner, J. Thoerle-Pospiech, P. Uusitalo, J. Wegrzecki, M. Wiehl, N. TI First superheavy element experiments at the GSI recoil separator TASCA: The production and decay of element 114 in the Pu-244(Ca-48,3-4n) reaction SO PHYSICAL REVIEW C LA English DT Article ID SPONTANEOUS-FISSION DECAY; CROSS-SECTIONS; MASS-DRIFT; NUCLEI; ISOTOPES; HEAVY; SYSTEMATICS; ISOMERS; TARGETS; NO-252 AB Experiments with the new recoil separator, Transactinide Separator and Chemistry Apparatus (TASCA), at the GSI were performed by using beams of Ca-48 to irradiate targets of Pb206-208, which led to the production of No252-254 isotopes. These studies allowed for evaluation of the performance of TASCA when coupled to a new detector and electronics system. By following these studies, the isotopes of element 114 ((288-291)114) were produced in irradiations of Pu-244 targets with Ca-48 beams at compound nucleus excitation energies around 41.7 and 37.5 MeV, demonstrating TASCA's ability to perform experiments with picobarn-level cross sections. A total of 15 decay chains were observed and were assigned to the decay of 288-291114. A new a-decay branch in (281)Ds was observed, leading to the new nucleus (277)Hs. C1 [Gates, J. M.; Duellmann, Ch E.; Schaedel, M.; Ackermann, D.; Block, M.; Bruechle, W.; Essel, H. G.; Hartmann, W.; Hessberger, F. P.; Huebner, A.; Jaeger, E.; Khuyagbaatar, J.; Kindler, B.; Krier, J.; Kurz, N.; Lommel, B.; Schaffner, H.; Schausten, B.; Schimpf, E.; Steiner, J.] GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany. [Gates, J. M.; Yakushev, A.; Tuerler, A.; Gorshkov, A.; Graeger, R.] Tech Univ Munich, D-85748 Garching, Germany. [Gates, J. M.; Dvorak, J.; Ellison, P. A.; Gregorich, K. E.; Nitsche, H.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Duellmann, Ch E.; Eberhardt, K.; Kratz, J. V.; Hild, D.; Liebe, D.; Runke, J.; Thoerle-Pospiech, P.; Wiehl, N.] Johannes Gutenberg Univ Mainz, D-55099 Mainz, Germany. [Duellmann, Ch E.] Helmholtz Inst Mainz, D-55099 Mainz, Germany. [Andersson, L. -L.; Herzberg, R. -D.; Parr, E.] Univ Liverpool, Liverpool L69 7ZE, Merseyside, England. [Forsberg, U.; Gellanki, J.; Rudolph, D.] Lund Univ, SE-22100 Lund, Sweden. [Lahiri, S.; Maiti, M.] Saha Inst Nucl Phys, Kolkata 700064, India. [Omtvedt, J. P.; Semchenkov, A.] Univ Oslo, NO-0315 Oslo, Norway. [Uusitalo, J.] Univ Jyvaskyla, FI-40014 Jyvaskyla, Finland. [Wegrzecki, M.] Inst Electr Mat Technol, PL-02668 Warsaw, Poland. RP Gates, JM (reprint author), GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany. EM jmgates@lbl.gov RI Rudolph, Dirk/D-4259-2009; Herzberg, Rolf-Dietmar/E-1558-2011; Omtvedt, Jon Petter/C-8194-2011; Block, Michael/I-2782-2015; Even, Julia/K-1186-2016; Turler, Andreas/D-3913-2014 OI Rudolph, Dirk/0000-0003-1199-3055; Omtvedt, Jon Petter/0000-0002-1822-7348; Block, Michael/0000-0001-9282-8347; Even, Julia/0000-0002-6314-9094; Turler, Andreas/0000-0002-4274-1056 FU German BMBF [06MT247I, 06MT248, 06MZ223I]; Research Center Elementary Forces and Mathematical Foundations (EMG); Swedish Science Council; U.S. D.O.E [DE-AC02-05CH11231]; NNSA [DE-FC52-08NA28752]; Norwegian Research Council [177538]; Government of India FX We thank the ECR ion source and UNILAC staffs for providing excellent and stable 48Ca beams. H. Brand and the GSI Experimental Electronics Department, H. Grosslhuber, G. Matheis, and R. Buhnemann from the machine shop at the Institute of Radiochemistry, TU Munich as well as V. Gorshkov, who provided technical support. L. Stavsetra provided preliminary BGS results for the 48Ca + 242Pu reaction prior to publication, which we gratefully acknowledge. This work was financially supported by the German BMBF (Grants No. 06MT247I, No. 06MT248, and No. 06MZ223I); the Research Center Elementary Forces and Mathematical Foundations (EMG); the GSI-F& E (MT/TUR, MZJVKR); the Swedish Science Council; the U.S. D.O.E. under Contract No. DE-AC02-05CH11231 and the NNSA under Contract No. DE-FC52-08NA28752; the Norwegian Research Council (Project No. 177538); and the Government of India-XIth 5-year plan project TADDS. NR 59 TC 69 Z9 71 U1 0 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAY 27 PY 2011 VL 83 IS 5 AR 054618 DI 10.1103/PhysRevC.83.054618 PG 17 WC Physics, Nuclear SC Physics GA 769LX UT WOS:000291016300005 ER PT J AU Song, HC Bass, SA Heinz, U AF Song, Huichao Bass, Steffen A. Heinz, Ulrich TI Elliptic flow in root s=200 GeV Au+Au collisions and root s=2.76 TeV Pb+Pb collisions: Insights from viscous hydrodynamics plus hadron cascade hybrid model SO PHYSICAL REVIEW C LA English DT Article ID HEAVY-ION COLLISIONS; QUARK-GLUON PLASMA; PB-PB COLLISIONS; ECCENTRICITY FLUCTUATIONS; NUCLEAR COLLISIONS; SUPPRESSION AB Using the newly developed hybrid model VISHNU, which connects viscous hydrodynamics with a hadron cascade model, we study the differential and integrated elliptic flow v(2) at different centrality bins for 200 A GeV Au + Au collisions and 2.76 A TeV Pb + Pb collisions. We find that the average quark-gluon plasma (QGP)-specific shear viscosity eta/s slightly increases from Relativistic Heavy Ion Collider to Large Hadron Collider (LHC) energies. However, a further study assuming different temperature dependencies for (eta/s)(QGP) shows that one cannot uniquely constrain the form of (eta/s)(QGP) (T) by fitting the spectra and v(2) alone. Based on our current understanding, the question whether the QGP fluid is more viscous or more perfect in the temperature regime reached by LHC energies is still open. C1 [Song, Huichao] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Bass, Steffen A.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Heinz, Ulrich] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. RP Song, HC (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM hsong@lbl.gov FU US Department of Energy [DE-AC02-05CH11231, DE-FG02-05ER41367, DE-SC0004286, DE-SC0004104] FX We gratefully acknowledge fruitful discussions with T. Hirano, P. Huovinen, H. Masui, H. Niemi, A. Poskanzer, C. Shen, R. Snellings, and X.-N. Wang. We especially thank T. Hirano for providing the new initial conditions at LHC energies, R. Snellings for the experimental data shown in Figs. 2 and 3, and H. Buesching for the ALICE data show in Fig. 1(a). This work was supported by the US Department of Energy under Grant Nos. DE-AC02-05CH11231, DE-FG02-05ER41367, DE-SC0004286, and (within the framework of the Jet Collaboration) DE-SC0004104. We gratefully acknowledge extensive computing resources provided to us by the Ohio Supercomputer Center. NR 66 TC 84 Z9 84 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAY 27 PY 2011 VL 83 IS 5 AR 054912 DI 10.1103/PhysRevC.83.054912 PG 6 WC Physics, Nuclear SC Physics GA 769LX UT WOS:000291016300006 ER PT J AU Bott, SC Haas, DM Madden, RE Ueda, U Eshaq, Y Collins, G Gunasekera, K Mariscal, D Peebles, J Beg, FN Mazarakis, M Struve, K Sharpe, R AF Bott, S. C. Haas, D. M. Madden, R. E. Ueda, U. Eshaq, Y. Collins, G. Gunasekera, K. Mariscal, D. Peebles, J. Beg, F. N. Mazarakis, M. Struve, K. Sharpe, R. TI 250 kA compact linear transformer driver for wire array z-pinch loads SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article AB We present the application of a short rise (similar to 150 ns) 250 kA linear transformer driver (LTD) to wire array z-pinch loads for the first time. The generator is a modification of a previous driver in which a new conical power feed provides a low inductance coupling to wire loads. Performance of the new design using both short circuit and plasma loads is presented and discussed. The final design delivers similar to 200 kA to a wire array load which is in good agreement with SCREAMER calculations using a simplified representative circuit. Example results demonstrate successful experiments using cylindrical, conical, and inverse wire arrays as well as previously published work on x-pinch loads. C1 [Bott, S. C.; Haas, D. M.; Madden, R. E.; Ueda, U.; Eshaq, Y.; Collins, G.; Gunasekera, K.; Mariscal, D.; Peebles, J.; Beg, F. N.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Mazarakis, M.; Struve, K.; Sharpe, R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Bott, SC (reprint author), Univ Calif San Diego, La Jolla, CA 92093 USA. FU Department of Energy [DE-SC-0001063] FX The UC San Diego team is grateful to Sandia National Laboratories and to Dr. Chris Deeney for both the loan of the generator and the technical support in completing its installation. The UCSD authors also thank Mr. Sean McGraw (Ashland University, Ohio) who helped with some of the laboratory testing during his National Undergraduate Fellowship (NUF) placement. This work was supported by the Department of Energy under Contract No. DE-SC-0001063. NR 26 TC 10 Z9 10 U1 1 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD MAY 27 PY 2011 VL 14 IS 5 AR 050401 DI 10.1103/PhysRevSTAB.14.050401 PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 769MO UT WOS:000291018200001 ER PT J AU Liu, XJ Lu, WC Wang, CZ Ho, KM AF Liu, Xiaojie Lu, Wen-Cai Wang, C. Z. Ho, K. M. TI Energetic and fragmentation stability of water clusters (H2O)(n), n=2-30 SO CHEMICAL PHYSICS LETTERS LA English DT Article ID HEXAMER CLUSTERS; AB-INITIO; BINDING-ENERGIES; SPECTRA; SPECTROSCOPY; FORM AB Ab initio calculations have been performed to study the structural trend, energetic stability, and fragmentation behavior of water clusters (H2O)(2-30). We show that as size increases, the cluster structures evolve from a mono-ring motif to multi-ring and ring-stacking motifs, and then to stuffed cage structures. We also show that losing water molecules one-by-one is the most favorable fragmentation channel with a dissociation energy of similar to 11.53 kcal/mol. Small water clusters such as water dimer, trimer, and tetramer, can also be observed in the fragmentation products since they often appear in the second best fragmentation channel. (C) 2011 Elsevier B. V. All rights reserved. C1 [Liu, Xiaojie; Lu, Wen-Cai] Jilin Univ, Inst Theoret Chem, State Key Lab Theoret & Computat Chem, Changchun 130021, Jilin, Peoples R China. [Lu, Wen-Cai] Qingdao Univ, Growing Base State Key Lab, Lab Fiber Mat & Modern Text, Qingdao 266071, Shandong, Peoples R China. [Lu, Wen-Cai] Qingdao Univ, Coll Phys, Qingdao 266071, Shandong, Peoples R China. [Liu, Xiaojie; Wang, C. Z.; Ho, K. M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Liu, Xiaojie; Wang, C. Z.; Ho, K. M.] US DOE, Ames Lab, Ames, IA 50011 USA. RP Lu, WC (reprint author), Jilin Univ, Inst Theoret Chem, State Key Lab Theoret & Computat Chem, Changchun 130021, Jilin, Peoples R China. EM wencailu@jlu.edu.cn FU National Natural Science Foundation of China [21043001, 20773047]; U.S. Department of Energy by Iowa State University [DE-AC02-07CH11358]; Office of Basic Energy Sciences, Division of Material Science and Engineering; China Scholarship Council [2009617104] FX This work was supported by the National Natural Science Foundation of China (Nos. 21043001 and 20773047). Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. This work was also supported by the Director for Energy Research, Office of Basic Energy Sciences, Division of Material Science and Engineering including a grant for computer time at the National Energy Research Supercomputing Center (NERSC) in Berkeley, CA. Xiaojie Liu acknowledges the support from China Scholarship Council (File No. 2009617104). NR 28 TC 15 Z9 15 U1 1 U2 18 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD MAY 27 PY 2011 VL 508 IS 4-6 BP 270 EP 275 DI 10.1016/j.cplett.2011.04.055 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 766AK UT WOS:000290750400017 ER PT J AU He, J Scott, JL Heroux, A Roy, S Lenoir, M Overduin, M Stahelin, RV Kutateladze, TG AF He, Ju Scott, Jordan L. Heroux, Annie Roy, Siddhartha Lenoir, Marc Overduin, Michael Stahelin, Robert V. Kutateladze, Tatiana G. TI Molecular Basis of Phosphatidylinositol 4-Phosphate and ARF1 GTPase Recognition by the FAPP1 Pleckstrin Homology (PH) Domain SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID STRUCTURAL BASIS; FYVE DOMAIN; MEMBRANE; BINDING; PROTEINS; ACIDIFICATION; PTDINS(4)P; MECHANISM; APOPTOSIS; SOFTWARE AB Four-phosphate-adaptor protein 1 (FAPP1) regulates secretory transport from the trans-Golgi network (TGN) to the plasma membrane. FAPP1 is recruited to the Golgi through binding of its pleckstrin homology (PH) domain to phosphatidylinositol 4-phosphate (PtdIns(4) P) and a small GTPase ADP-ribosylation factor 1 (ARF1). Despite the critical role of FAPP1 in membrane trafficking, the molecular basis of its dual function remains unclear. Here, we report a 1.9 angstrom resolution crystal structure of the FAPP1 PH domain and detail the molecular mechanisms of the PtdIns(4) P and ARF1 recognition. The FAPP1 PH domain folds into a seven-stranded beta-barrel capped by an beta-helix at one edge, whereas the opposite edge is flanked by three loops and the beta 4 and beta 7 strands that form a lipid-binding pocket within the beta-barrel. The ARF1-binding site is located on the outer side of the beta-barrel as determined by NMR resonance perturbation analysis, mutagenesis, and measurements of binding affinities. The two binding sites have little overlap, allowing FAPP1 PH to associate with both ligands simultaneously and independently. Binding to PtdIns(4) P is enhanced in an acidic environment and is required for membrane penetration and tubulation activity of FAPP1, whereas the GTP-bound conformation of the GTPase is necessary for the interaction with ARF1. Together, these findings provide structural and biochemical insight into the multivalent membrane anchoring by the PH domain that may augment affinity and selectivity of FAPP1 toward the TGN membranes enriched in both PtdIns(4) P and GTP-bound ARF1. C1 [Scott, Jordan L.; Stahelin, Robert V.] Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA. [He, Ju; Roy, Siddhartha; Kutateladze, Tatiana G.] Univ Colorado, Sch Med, Dept Pharmacol, Aurora, CO 80045 USA. [Scott, Jordan L.; Stahelin, Robert V.] Univ Notre Dame, Walther Ctr Canc Res, Notre Dame, IN 46556 USA. [Stahelin, Robert V.] Indiana Univ Sch Med, Dept Biochem & Mol Biol, South Bend, IN 46617 USA. [Heroux, Annie] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. [Lenoir, Marc; Overduin, Michael] Univ Birmingham, Sch Canc Sci, Birmingham B15 2TT, W Midlands, England. RP Stahelin, RV (reprint author), Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA. EM rstaheli@iupui.edu; Tatiana.Kutateladze@ucdenver.edu OI Overduin, Michael/0000-0002-3114-6585 FU National Institutes of Health [GM071424, CA95144]; American Heart Association; Indiana University Biomedical Research; American Cancer Society; Cancer Research UK; Offices of Biological and Environmental Research and of Basic Energy Sciences of the United States Department of Energy; National Center for Research Resources of the National Institutes of Health [P41RR012408] FX This work was supported, in whole or in part, by National Institutes of Health Grants GM071424 and CA95144 and the American Heart Association (to T. G. K.). This work was also supported by grants from Indiana University Biomedical Research and the American Cancer Society (to R. V. S.) and Cancer Research UK (to M. O.).; We thank Y. Gedle, M. Lemmon, C. Musselman, E. Odintsova, and R. Zhao for discussions and helping with experiments and R. Prekeris and S. Wakatsuki for providing cDNAs of wild type and ARF1 Q71L. X-ray crystallographic data were collected at beamline X25 of the NSLS. Financial support for NSLS comes from the Offices of Biological and Environmental Research and of Basic Energy Sciences of the United States Department of Energy and from the National Center for Research Resources of the National Institutes of Health (Grant P41RR012408). NR 38 TC 41 Z9 43 U1 0 U2 7 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 J9 J BIOL CHEM JI J. Biol. Chem. PD MAY 27 PY 2011 VL 286 IS 21 BP 18650 EP 18657 DI 10.1074/jbc.M111.233015 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 766ME UT WOS:000290785700037 PM 21454700 ER PT J AU Schushan, M Landau, M Padan, E Ben-Tal, N AF Schushan, Maya Landau, Meytal Padan, Etana Ben-Tal, Nir TI Two Conflicting NHE1 Model Structures: Compatibility with Experimental Data and Implications for the Transport Mechanism SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Letter ID ANTIPORTER C1 [Schushan, Maya; Ben-Tal, Nir] Tel Aviv Univ, George S Wise Fac Life Sci, Dept Biochem & Mol Biol, IL-69978 Ramat Aviv, Israel. [Landau, Meytal] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90024 USA. [Landau, Meytal] Univ Calif Los Angeles, UCLA DOE Inst Genom & Prote, Los Angeles, CA USA. [Padan, Etana] Hebrew Univ Jerusalem, Dept Biol Chem, Alexander Silberman Inst Life Sci, IL-91904 Jerusalem, Israel. RP Schushan, M (reprint author), Tel Aviv Univ, George S Wise Fac Life Sci, Dept Biochem & Mol Biol, IL-69978 Ramat Aviv, Israel. EM NirB@tauex.tau.ac.il RI landau, Meytal/J-3075-2012 NR 5 TC 5 Z9 5 U1 0 U2 1 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 J9 J BIOL CHEM JI J. Biol. Chem. PD MAY 27 PY 2011 VL 286 IS 21 AR le9 DI 10.1074/jbc.L110.159202 PG 1 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 766ME UT WOS:000290785700003 ER PT J AU Mendes, R Kruijt, M de Bruijn, I Dekkers, E van der Voort, M Schneider, JHM Piceno, YM DeSantis, TZ Andersen, GL Bakker, PAHM Raaijmakers, JM AF Mendes, Rodrigo Kruijt, Marco de Bruijn, Irene Dekkers, Ester van der Voort, Menno Schneider, Johannes H. M. Piceno, Yvette M. DeSantis, Todd Z. Andersen, Gary L. Bakker, Peter A. H. M. Raaijmakers, Jos M. TI Deciphering the Rhizosphere Microbiome for Disease-Suppressive Bacteria SO SCIENCE LA English DT Article ID PATHOGENS AB Disease-suppressive soils are exceptional ecosystems in which crop plants suffer less from specific soil-borne pathogens than expected owing to the activities of other soil microorganisms. For most disease-suppressive soils, the microbes and mechanisms involved in pathogen control are unknown. By coupling PhyloChip-based metagenomics of the rhizosphere microbiome with culture-dependent functional analyses, we identified key bacterial taxa and genes involved in suppression of a fungal root pathogen. More than 33,000 bacterial and archaeal species were detected, with Proteobacteria, Firmicutes, and Actinobacteria consistently associated with disease suppression. Members of the gamma-Proteobacteria were shown to have disease-suppressive activity governed by nonribosomal peptide synthetases. Our data indicate that upon attack by a fungal root pathogen, plants can exploit microbial consortia from soil for protection against infections. C1 [Mendes, Rodrigo; Kruijt, Marco; de Bruijn, Irene; Dekkers, Ester; van der Voort, Menno; Raaijmakers, Jos M.] Wageningen Univ, Phytopathol Lab, NL-6700 EE Wageningen, Netherlands. [Schneider, Johannes H. M.] Inst Sugar Beet Res, NL-4611 HL Bergen Op Zoom, Netherlands. [Piceno, Yvette M.; DeSantis, Todd Z.; Andersen, Gary L.] Lawrence Berkeley Natl Lab, Dept Ecol, Berkeley, CA 94720 USA. [DeSantis, Todd Z.] Second Genome Inc, San Francisco, CA 94158 USA. [Bakker, Peter A. H. M.] Univ Utrecht, Dept Biol, NL-3584 CH Utrecht, Netherlands. RP Raaijmakers, JM (reprint author), Wageningen Univ, Phytopathol Lab, Droevendaalsesteeg 1, NL-6700 EE Wageningen, Netherlands. EM jos.raaijmakers@wur.nl RI Bakker, Peter/B-9355-2011; Utrecht Univ., PMI/G-9549-2011; de Bruijn, Irene/A-7437-2014; Raaijmakers, Jos/D-1574-2014; Mendes, Rodrigo/F-1534-2010; Andersen, Gary/G-2792-2015; Piceno, Yvette/I-6738-2016 OI de Bruijn, Irene/0000-0002-4889-3253; Raaijmakers, Jos/0000-0003-1608-6614; Mendes, Rodrigo/0000-0002-9817-4118; Andersen, Gary/0000-0002-1618-9827; Piceno, Yvette/0000-0002-7915-4699 FU Netherlands Science Organisation (NWO) [838.06.101]; Netherlands Genomics Initiative-Ecogenomics, Netherlands; Lawrence Berkeley National Laboratory (LBNL) [DE-AC02-05CH11231]; U.S. Department of Energy FX We thank T. Bisseling for critical reading and valuable suggestions. We acknowledge assistance by L. Sibbel-Wagemakers, N. Pangesti, M. de Milliano, N. Sharma, R. de Vries, P. M. S. van Oorschot, A. H. L. Schoone, and Y. Bakker. This work was financially supported by grants from Netherlands Science Organisation (NWO)-ERGO (#838.06.101) and Netherlands Genomics Initiative-Ecogenomics, Netherlands. Additional work was performed at Lawrence Berkeley National Laboratory (LBNL) (contract DE-AC02-05CH11231 with the U.S. Department of Energy). The 16S rDNA sequences are available on GenBank under accessions HQ848634 to HQ848643, and the thaABCD sequences under accession HQ888764. LBNL has a patent on the PhyloChip assay and Second Genome has licensed this assay from LBNL. Although the G3 PhyloChip is under patent (and under exclusive license to Second Genome), the data generated from the use of the chip are not patented or restricted. T.Z.dS. owns stock in Second Genome valued at under $10,000. NR 14 TC 381 Z9 410 U1 58 U2 432 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 J9 SCIENCE JI Science PD MAY 27 PY 2011 VL 332 IS 6033 BP 1097 EP 1100 DI 10.1126/science.1203980 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 769FN UT WOS:000290996700048 PM 21551032 ER PT J AU Hwang, GS Kaviany, M Gostick, JT Kientiz, B Weber, AZ Kim, MH AF Hwang, Gi Suk Kaviany, Massoud Gostick, Jeffrey T. Kientiz, Brian Weber, Adam Z. Kim, Moo Hwan TI Role of water states on water uptake and proton transport in Nafion using molecular simulations and bimodal network SO POLYMER LA English DT Article DE Water uptake; Proton conductivity; Water diffusivity ID POLYMER-ELECTROLYTE MEMBRANES; FUEL-CELL MEMBRANES; EXCHANGE MEMBRANES; SCHROEDERS-PARADOX; X-RAY; MODEL; DIFFUSION; ACID; CONDUCTIVITY; HYDRATION AB Using molecular simulations and a bimodal-domain network, the role of water state on Nafion water uptake and water and proton transport is investigated. Although the smaller domains provide moderate transport pathways, their effectiveness remains low due to strong, resistive water molecules/domain surface interactions. The water occupancy of the larger domains yields bulk-like water, and causes the observed transition in the water uptake and significant increases in transport properties. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Hwang, Gi Suk; Kaviany, Massoud] Univ Michigan, Dept Mech Engn, Ann Arbor, MI 48109 USA. [Gostick, Jeffrey T.; Kientiz, Brian; Weber, Adam Z.] Univ Calif Berkeley, Lawrence Berkeley Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Kim, Moo Hwan] Pohang Univ Sci & Technol, Dept Mech Engn, Pohang 790874, Kyungbuk, South Korea. RP Kaviany, M (reprint author), Univ Michigan, Dept Mech Engn, Ann Arbor, MI 48109 USA. EM kaviany@umich.edu OI Weber, Adam/0000-0002-7749-1624 FU Ministry of Science and Technology, South Korea; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Fuel Cell Technologies; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX We are thankful for the sponsorship of Global Partnership Program ("Ministry of Science and Technology, South Korea), assistance by Drs. Alexander Hexemer and Cheng Wang (Lawrence Berkeley National Laboratory) on the SAXS measurements, and discussions with Professor Reinhard Hentschke (University of Wuppertal, Germany) on the GCMD-MC simulation. This work was partially supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Fuel Cell Technologies, and the Director, Office of Science, Office of Basic Energy Sciences (for support of the Advanced Light Source), of the U.S. Department of Energy under contract number DE-AC02-05CH11231. NR 74 TC 25 Z9 25 U1 0 U2 21 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 EI 1873-2291 J9 POLYMER JI Polymer PD MAY 26 PY 2011 VL 52 IS 12 BP 2584 EP 2593 DI 10.1016/j.polymer.2011.03.056 PG 10 WC Polymer Science SC Polymer Science GA 771BY UT WOS:000291133400017 ER PT J AU Kim, E Ahn, H Lee, H Lee, B Ryu, DY AF Kim, Eunhye Ahn, Hyungju Lee, Hoyeon Lee, Byeongdu Ryu, Du Yeol TI Ordering and microdomain orientation in block copolymer films by thermal deprotection SO POLYMER LA English DT Article DE Ordering; Microdomain orientation; Block copolymer films ID X-RAY-SCATTERING; THIN-FILMS; TRANSITION; SURFACES; CYLINDER; ARRAYS; TEMPLATES; SUBSTRATE; BEHAVIOR; DOMAINS AB Ordering and microdomain orientation for the films of symmetric polystyrene-b-poly(tert-butyl methacrylate)s (PS-b-PtBMAs) was investigated by in-situ grazing incidence small-angle X-ray scattering (GISAXS) and the electron microscopy. During thermal deprotection at higher temperature (200 degrees C), functional tert-butyl ester units in the PtBMA block component are integrated into inter- or intra-molecular anhydride linkages. It was observed that this process causes an increase in the Flory -Huggins interaction parameter (chi) between the two block components for disordered PS-b-PtBMA film, leading to a modulated nonequilibrium structure. Interestingly, for lamella-forming PS-b-PtBMA film, a significant chain stretching in lateral direction during thermal deprotection resulted in a characteristic strain-induced perpendicular orientation in the middle of the film confined between two parallel orientations of lamellar microdomains. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Kim, Eunhye; Ahn, Hyungju; Lee, Hoyeon; Ryu, Du Yeol] Yonsei Univ, Dept Chem & Biomol Engn, Seoul 120749, South Korea. [Lee, Byeongdu] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. RP Ryu, DY (reprint author), Yonsei Univ, Dept Chem & Biomol Engn, 262 Seongsanno, Seoul 120749, South Korea. EM dyryu@yonsei.ac.kr RI Ryu, Du Yeol/G-8278-2012; OI Lee, Byeongdu/0000-0003-2514-8805 FU Ministry of Education, Science & Technology (MEST), Korea [2009-0067295, 2010K001430, R11-2007-050-00000] FX This work was supported by NRF grants (2009-0067295), Converging Research Center Program (2010K001430), and APCPI ERC program (R11-2007-050-00000), which are funded by the Ministry of Education, Science & Technology (MEST), Korea. NR 39 TC 3 Z9 3 U1 0 U2 17 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 J9 POLYMER JI Polymer PD MAY 26 PY 2011 VL 52 IS 12 BP 2677 EP 2684 DI 10.1016/j.polymer.2011.04.031 PG 8 WC Polymer Science SC Polymer Science GA 771BY UT WOS:000291133400027 ER PT J AU Liu, C Lee, Y Kondo, T Mun, ED Caudle, M Harmon, BN Bud'ko, SL Canfield, PC Kaminski, A AF Liu, Chang Lee, Yongbin Kondo, Takeshi Mun, Eun Deok Caudle, Malinda Harmon, B. N. Bud'ko, Sergey L. Canfield, Paul C. Kaminski, Adam TI Metallic surface electronic state in half-Heusler compounds RPtBi (R = Lu, Dy, Gd) SO PHYSICAL REVIEW B LA English DT Article ID HGTE QUANTUM-WELLS; TOPOLOGICAL INSULATORS; TERNARY COMPOUNDS; TRANSPORT; TRANSITION; BI2TE3; PHASE AB Rare-earth platinum bismuth (RPtBi) has been proposed recently as a potential topological insulator. In this paper, we present measurements of the metallic surface electronic structure in three members of this family, using angle-resolved photoemission spectroscopy (ARPES). Our data show clear spin-orbit splitting of the surface bands and the Kramers' degeneracy of spins at the (Gamma) over bar and (M) over bar points, which is reproduced nicely with our full-potential linearized augmented plane wave calculation for a surface electronic state. Topologically nontrivial behavior is signified by band inversion in the calculated bulk electronic structures, yet no direct indication of such behavior is detected by ARPES except for a weak Fermi crossing detected in close proximity to the (Gamma) over bar point, making the total number of Fermi crossings odd. In the surface band calculation, however, this crossing is explained by a Kramers pair of bands that are very close to each other. The classification of this family of materials as topological insulators remains an open question. C1 [Liu, Chang; Lee, Yongbin; Kondo, Takeshi; Mun, Eun Deok; Caudle, Malinda; Harmon, B. N.; Bud'ko, Sergey L.; Canfield, Paul C.; Kaminski, Adam] Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. [Liu, Chang; Kondo, Takeshi; Mun, Eun Deok; Caudle, Malinda; Harmon, B. N.; Bud'ko, Sergey L.; Canfield, Paul C.; Kaminski, Adam] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Liu, C (reprint author), Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. RI Canfield, Paul/H-2698-2014; Kondo, Takeshi/H-2680-2016 FU Department of Energy-Basic Energy Sciences [DE-AC02-07CH11358]; US DOE [DE-AC03-76SF00098] FX We thank S.-C. Zhang and J. Schmalian for instructive discussions as well as Sung-Kwan Mo for grateful instrumental support at the ALS. Ames Laboratory was supported by the Department of Energy-Basic Energy Sciences under Contract No. DE-AC02-07CH11358. ALS is operated by the US DOE under Contract No. DE-AC03-76SF00098. NR 27 TC 37 Z9 37 U1 4 U2 49 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 26 PY 2011 VL 83 IS 20 AR 205133 DI 10.1103/PhysRevB.83.205133 PG 5 WC Physics, Condensed Matter SC Physics GA 769IH UT WOS:000291005600002 ER PT J AU Rahman, R Verduijn, J Kharche, N Lansbergen, GP Klimeck, G Hollenberg, LCL Rogge, S AF Rahman, R. Verduijn, J. Kharche, N. Lansbergen, G. P. Klimeck, G. Hollenberg, L. C. L. Rogge, S. TI Engineered valley-orbit splittings in quantum-confined nanostructures in silicon SO PHYSICAL REVIEW B LA English DT Article ID NEMO 3-D; SIMULATION; TRANSPORT; ATOM; DOTS AB An important challenge in silicon quantum electronics in the few electron regime is the potentially small energy gap between the ground and excited orbital states in 3D quantum confined nanostructures due to the multiple valley degeneracies of the conduction band present in silicon. Understanding the "valley-orbit" (VO) gap is essential for silicon qubits, as a large VO gap prevents leakage of the qubit states into a higher dimensional Hilbert space. The VO gap varies considerably depending on quantum confinement, and can be engineered by external electric fields. In this work we investigate VO splitting experimentally and theoretically in a range of confinement regimes. We report measurements of the VO splitting in silicon quantum dot and donor devices through excited state transport spectroscopy. These results are underpinned by large-scale atomistic tight-binding calculations involving over 1 million atoms to compute VO splittings as functions of electric fields, donor depths, and surface disorder. The results provide a comprehensive picture of the range of VO splittings that can be achieved through quantum engineering. C1 [Rahman, R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Verduijn, J.; Lansbergen, G. P.; Rogge, S.] Delft Univ Technol, Kavli Inst Nanosci, NL-2628 CJ Delft, Netherlands. [Verduijn, J.; Rogge, S.] Univ New S Wales, Sch Phys, Ctr Quantum Computat & Commun Technol, Sydney, NSW 2052, Australia. [Kharche, N.] Rensselaer Polytech Inst, Dept Phys, Computat Ctr Nanotechnol Innovat, Troy, NY 12180 USA. [Klimeck, G.] Purdue Univ, Network Computat Nanotechnol, W Lafayette, IN 47907 USA. [Hollenberg, L. C. L.] Univ Melbourne, Sch Phys, Ctr Quantum Computat & Commun Technol, Melbourne, Vic 3010, Australia. RP Rahman, R (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM rrahman@sandia.gov RI Lansbergen, Gabriel/A-7895-2011; Kharche, Neerav/F-4331-2015; Klimeck, Gerhard/A-1414-2012; Rogge, Sven/G-3709-2010; OI Kharche, Neerav/0000-0003-1014-6022; Klimeck, Gerhard/0000-0001-7128-773X; Rahman, Rajib/0000-0003-1649-823X FU United States Department of Energy [DEAC04-94AL85000]; NASA; Australian Research Council Centre of Excellence for Quantum Computation and Communication Technology [CE110001029]; NSA; ARO [W911NF-08-1-0527] FX Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Corporation, for the United States Department of Energy under Contract No. DEAC04-94AL85000. NEMO-3D was initially developed at JPL, Caltech under a contract with NASA. NCN/nanohub.org computational resources were used. This research was conducted by the Australian Research Council Centre of Excellence for Quantum Computation and Communication Technology (Project No. CE110001029), NSA and ARO Contract No. W911NF-08-1-0527). NR 32 TC 22 Z9 22 U1 2 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 26 PY 2011 VL 83 IS 19 AR 195323 DI 10.1103/PhysRevB.83.195323 PG 5 WC Physics, Condensed Matter SC Physics GA 769IG UT WOS:000291005500005 ER PT J AU Armijo, J Barnard, JJ AF Armijo, J. Barnard, J. J. TI Droplet evolution in expanding flow of warm dense matter SO PHYSICAL REVIEW E LA English DT Article ID MOLECULAR-DYNAMICS; LASER-ABLATION; LIQUID; EVAPORATION; SIMULATION; EQUATION; FRAGMENTATION; TEMPERATURE; EXPANSION; FACILITY AB We propose a simple, self-consistent kinetic model for the evolution of a mixture of droplets and vapor expanding adiabatically in vacuum after rapid, almost isochoric heating. We study the evolution of the two-phase fluid at intermediate times between the molecular and the hydrodynamic scales, focusing on out-of-equilibrium and surface effects. We use the van der Waals equation of state as a test bed to implement our model and study the phenomenology of the upcoming second neutralized drift compression experiment (NDCX-II) at Lawrence Berkeley National Laboratory (LBNL) that uses ion beams for target heating. We find an approximate expression for the temperature difference between the droplets and the expanding gas and we check it with numerical calculations. The formula provides a useful criterion to distinguish the thermalized and nonthermalized regimes of expansion. In the thermalized case, the liquid fraction grows in a proportion that we estimate analytically, whereas, in case of too rapid expansion, a strict limit for the evaporation of droplets is derived. The range of experimental situations is discussed. C1 [Armijo, J.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Barnard, J. J.] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Armijo, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. EM julienarmijo@gmail.com RI Armijo, Julien/I-5413-2013 FU Ecole Normale Superieure, France; US Department of Energy under University of California at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; US Department of Energy under University of California at Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We wish to thank R. M. More, F. M. Bieniosek, P. A. Seidl, B. G. Logan, and I. D. Kaganovich for helpful discussions. One of us (J.A.) was partially supported by Ecole Normale Superieure, France. Work performed under the auspices of the US Department of Energy under University of California Contract No. DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory and Contract No. DE-AC52-07NA27344 at Lawrence Livermore National Laboratory. NR 44 TC 3 Z9 3 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 J9 PHYS REV E JI Phys. Rev. E PD MAY 26 PY 2011 VL 83 IS 5 AR 051507 DI 10.1103/PhysRevE.83.051507 PN 1 PG 11 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 769IR UT WOS:000291006600002 PM 21728540 ER PT J AU Carlsten, BE Bishofberger, KA Duffy, LD Russell, SJ Ryne, RD Yampolsky, NA Dragt, AJ AF Carlsten, Bruce E. Bishofberger, Kip A. Duffy, Leanne D. Russell, Steven J. Ryne, Robert D. Yampolsky, Nikolai A. Dragt, Alex J. TI Arbitrary emittance partitioning between any two dimensions for electron beams SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID OPERATION AB The flat-beam transform (FBT) for round symmetric beams can be extended using the concept of eigenemittances. By tailoring the initial beam conditions at the cathode, including adding arbitrary correlations between any two dimensions, this extension can be used to provide greater freedom in controlling the beam's final emittances. In principle, this technique can be used to generate extraordinarily transversely bright electron beams. Examples are provided where an equivalent FBT is established between the horizontal and the longitudinal beam dimensions. C1 [Carlsten, Bruce E.; Bishofberger, Kip A.; Duffy, Leanne D.; Russell, Steven J.; Yampolsky, Nikolai A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Ryne, Robert D.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Dragt, Alex J.] Univ Maryland, College Pk, MD 20742 USA. RP Carlsten, BE (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RI Yampolsky, Nikolai/A-7521-2011; OI Duffy, Leanne/0000-0002-0123-6723; Carlsten, Bruce/0000-0001-5619-907X NR 22 TC 10 Z9 10 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD MAY 26 PY 2011 VL 14 IS 5 AR 050706 DI 10.1103/PhysRevSTAB.14.050706 PG 16 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 769IY UT WOS:000291007300001 ER PT J AU Hamidi, H Gustafason, D Pellegrini, M Gasson, J AF Hamidi, Habib Gustafason, Derek Pellegrini, Matteo Gasson, Judith TI Identification of Novel Targets of CSL-Dependent Notch Signaling in Hematopoiesis SO PLOS ONE LA English DT Article ID EMBRYONIC STEM-CELLS; ACUTE LYMPHOBLASTIC-LEUKEMIA; IN-VITRO DIFFERENTIATION; FACTOR-BINDING SITES; MODEL-BASED ANALYSIS; ZONE B-CELLS; RBP-J-KAPPA; T-CELLS; TRANSCRIPTION FACTORS; GENE-EXPRESSION AB Somatic activating mutations in the Notch1 receptor result in the overexpression of activated Notch1, which can be tumorigenic. The goal of this study is to understand the molecular mechanisms underlying the phenotypic changes caused by the overexpression of ligand independent Notch 1 by using a tetracycline inducible promoter in an in vitro embryonic stem (ES) cells/OP9 stromal cells coculture system, recapitulating normal hematopoiesis. First, an in silico analysis of the promoters of Notch regulated genes (previously determined by microarray analysis) revealed that the motifs recognized by regulatory proteins known to mediate hematopoiesis were overrepresented. Notch 1 does not bind DNA but instead binds the CSL transcription factor to regulate gene expression. The in silico analysis also showed that there were putative CSL binding sites observed in the promoters of 28 out of 148 genes. A custom ChIP-chip array was used to assess the occupancy of CSL in the promoter regions of the Notch1 regulated genes in vivo and showed that 61 genes were bound by activated Notch responsive CSL. Then, comprehensive mapping of the CSL binding sites genome-wide using ChIP-seq analysis revealed that over 10,000 genes were bound within 10 kb of the TSS (transcription start site). The majority of the targets discovered by ChIP-seq belong to pathways that have been shown by others to crosstalk with Notch signaling. Finally, 83 miRNAs were significantly differentially expressed by greater than 1.5-fold during the course of in vitro hematopoiesis. Thirty one miRNA were up-regulated and fifty two were down-regulated. Overexpression of Notch1 altered this pattern of expression of microRNA: six miRNAs were up-regulated and four were down regulated as a result of activated Notch1 overexpression during the course of hematopoiesis. Time course analysis of hematopoietic development revealed that cells with Notch 1 overexpression mimic miRNA expression of cells in a less mature stage, which is consistent with our previous biological characterization. C1 [Hamidi, Habib; Gasson, Judith] Univ Calif Los Angeles, David Geffen Sch Med, Dept Biol Chem, Los Angeles, CA 90095 USA. [Gustafason, Derek; Pellegrini, Matteo] Univ Calif Los Angeles, DOE Inst Genom & Prote, Los Angeles, CA USA. [Pellegrini, Matteo] Univ Calif Los Angeles, Dept Mol Cell & Dev Biol, Los Angeles, CA USA. [Gasson, Judith] Univ Calif Los Angeles, David Geffen Sch Med, Dept Med, Div Hematol Oncol, Los Angeles, CA 90095 USA. [Gasson, Judith] Univ Calif Los Angeles, David Geffen Sch Med, Dept Biol Chem, Los Angeles, CA 90095 USA. [Gasson, Judith] Univ Calif Los Angeles, David Geffen Sch Med, Jonsson Comprehens Canc Ctr, Los Angeles, CA 90095 USA. RP Hamidi, H (reprint author), Univ Calif Los Angeles, David Geffen Sch Med, Dept Biol Chem, Los Angeles, CA 90095 USA. EM jgasson@mednet.ucla.edu NR 118 TC 22 Z9 23 U1 0 U2 6 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 185 BERRY ST, STE 1300, SAN FRANCISCO, CA 94107 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 26 PY 2011 VL 6 IS 5 AR e20022 DI 10.1371/journal.pone.0020022 PG 19 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 769XS UT WOS:000291052200027 PM 21637838 ER PT J AU Weyman, PD Vargas, WA Tong, YK Yu, JP Maness, PC Smith, HO Xu, Q AF Weyman, Philip D. Vargas, Walter A. Tong, Yingkai Yu, Jianping Maness, Pin-Ching Smith, Hamilton O. Xu, Qing TI Heterologous Expression of Alteromonas macleodii and Thiocapsa roseopersicina [NiFe] Hydrogenases in Synechococcus elongatus SO PLOS ONE LA English DT Article ID BIDIRECTIONAL HYDROGENASE; ACCESSORY GENES; MUTAGENESIS; MATURATION; OXIDATION; CLONING; BBS; CYANOBACTERIA; BIOSYNTHESIS; ALCALIGENES AB Oxygen-tolerant [NiFe] hydrogenases may be used in future photobiological hydrogen production systems once the enzymes can be heterologously expressed in host organisms of interest. To achieve heterologous expression of [NiFe] hydrogenases in cyanobacteria, the two hydrogenase structural genes from Alteromonas macleodii Deep ecotype (AltDE), hynS and hynL, along with the surrounding genes in the gene operon of HynSL were cloned in a vector with an IPTG-inducible promoter and introduced into Synechococcus elongatus PCC7942. The hydrogenase protein was expressed at the correct size upon induction with IPTG. The heterologously-expressed HynSL hydrogenase was active when tested by in vitro H-2 evolution assay, indicating the correct assembly of the catalytic center in the cyanobacterial host. Using a similar expression system, the hydrogenase structural genes from Thiocapsa roseopersicina (hynSL) and the entire set of known accessory genes were transferred to S. elongatus. A protein of the correct size was expressed but had no activity. However, when the 11 accessory genes from AltDE were co-expressed with hynSL, the T. roseopersicina hydrogenase was found to be active by in vitro assay. This is the first report of active, heterologously-expressed [NiFe] hydrogenases in cyanobacteria. C1 [Weyman, Philip D.; Vargas, Walter A.; Tong, Yingkai; Smith, Hamilton O.; Xu, Qing] J Craig Venter Inst, Dept Synthet Biol & Bioenergy, Rockville, MD USA. [Yu, Jianping; Maness, Pin-Ching] Natl Renewable Energy Lab, Golden, CO USA. RP Weyman, PD (reprint author), J Craig Venter Inst, Dept Synthet Biol & Bioenergy, Rockville, MD USA. EM qxu2019@gmail.com OI Weyman, Philip/0000-0001-5787-0291 FU U.S. Department of Energy [DE-FG36-05GO15027] FX This work was supported by the U.S. Department of Energy, the Hydrogen, Fuel Cells, and Infrastructure Technology Program (DE-FG36-05GO15027). The funder had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 39 TC 16 Z9 16 U1 0 U2 18 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 26 PY 2011 VL 6 IS 5 AR e20126 DI 10.1371/journal.pone.0020126 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 769XS UT WOS:000291052200035 PM 21637846 ER PT J AU Li, HY Sivapalan, M AF Li, Hongyi Sivapalan, Murugesu TI Effect of spatial heterogeneity of runoff generation mechanisms on the scaling behavior of event runoff responses in a natural river basin SO WATER RESOURCES RESEARCH LA English DT Article ID ELEMENTARY WATERSHED APPROACH; FLOOD FREQUENCY; GEOMORPHOLOGICAL DISPERSION; KINEMATIC DISPERSION; HYDROLOGIC RESPONSE; CATCHMENT-SCALE; RESIDENCE TIME; COLD REGIONS; MODEL; NETWORK AB This paper presents a theoretical investigation of the effects of spatial heterogeneity of runoff generation on the scaling behavior of runoff timing responses. A previous modeling study on the Illinois River Basin in Oklahoma had revealed a systematic spatial trend in the relative dominance of different runoff generation mechanisms, attributable to corresponding systematic trends in landscape properties. Considering the differences in the timing of hillslope responses between the different runoff mechanisms, this paper explores their impacts on the catchment-scale runoff routing responses, including how they change with spatial scale. For this purpose we utilize a distributed, physically based hydrological model, with a fully hydraulic stream network routing component. The model is used to generate instantaneous response functions (IRF) for nested catchments of a range of sizes along the river network and quantitative measures of their shape, e. g., peak and time to peak. In order to separate the effects of soil heterogeneity from those due to basin geomorphology, the model simulations are carried out for three hypothetical cases that make assumptions regarding landscape properties (uniform, a systematic trend, and heterogeneity plus the trend), repeating these simulations under wet and dry antecedent conditions. The simulations produced expected and also surprising results. The power law relationship between the peak of the IRF and drainage area is shown to be flatter under wet conditions than under dry conditions, even though the (faster) saturation excess mechanism is more dominant under wet conditions. This result appears to be caused by partial area runoff generation: under wet conditions, the fraction of saturation area is about 30%, while under dry conditions it is less than 10% for the same input of rainfall. This means travel times associated with overland flow (which mostly contributes to the peak and time to peak) are, in fact, longer during wet conditions than during dry conditions. The power law relationship between peak and drainage area also exhibits a scaling break at around 1000 km(2), which can be shown to be related to the peculiar geomorphology of the catchment. C1 [Li, Hongyi; Sivapalan, Murugesu] Univ Illinois, Dept Civil & Environm Engn, Urbana, IL 61801 USA. [Sivapalan, Murugesu] Univ Illinois, Dept Geog, Urbana, IL 61801 USA. [Sivapalan, Murugesu] Delft Univ Technol, Dept Water Management, Fac Civil Engn & Geosci, Delft, Netherlands. RP Li, HY (reprint author), Pacific NW Natl Lab, Hydrol Tech Grp, POB 999, Richland, WA 99352 USA. EM hongyi.li@pnl.gov RI Sivapalan, Murugesu/A-3538-2008; Li, Hong-Yi/C-9143-2014 OI Sivapalan, Murugesu/0000-0003-3004-3530; Li, Hong-Yi/0000-0001-5690-3610 FU DMIP2 team at the National Weather Service, NOAA; University of Illinois; National Science Foundation [NSF EFRI-0835982] FX We are grateful to the DMIP2 team at the National Weather Service, NOAA, for providing most of the data used in this study and for providing financial support to attend DMIP2 meetings. The research was partly funded by financial support provided by the University of Illinois through the AESIS project (Barbara Minsker, PI) and by the National Science Foundation (NSF EFRI-0835982, Ximing Cai, PI). This support is gratefully acknowledged. We dedicate this paper to Steve Burges for his significant and diverse contributions to hydrology over an illustrious 40 year career. NR 30 TC 17 Z9 17 U1 2 U2 15 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 J9 WATER RESOUR RES JI Water Resour. Res. PD MAY 26 PY 2011 VL 47 AR W00H08 DI 10.1029/2010WR009712 PG 20 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA 770TH UT WOS:000291110900003 ER PT J AU Xiao, HY Weber, WJ AF Xiao, H. Y. Weber, W. J. TI Oxygen Vacancy Formation and Migration in CexTh1-xO2 Solid Solution SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID DENSITY-FUNCTIONAL CALCULATION; GROUND-STATE PROPERTIES; ELECTRONIC-STRUCTURE; 1ST PRINCIPLES; ACTINIDE DIOXIDES; THORIUM-DIOXIDE; CERIUM DIOXIDE; CEO2 SURFACES; BULK MODULUS; THO2 AB A local-density approximation with the Hubbard U correction (LDA+U) method has been employed to investigate oxygen vacancy formation and migration in CexTh1-xO2. The addition of CeO2 into ThO2 significantly decreases the oxygen vacancy formation and migration energies. ThO2 containing 50% CeO2 exhibits the lowest calculated formation energy, 3.7 eV, and the lowest calculated migration energy, 0.2 eV, occurs for a CeO2 content of 75%, suggesting that introducing CeO2 into ThO2 promotes the formation of mobile oxygen vacancies. If the ceria content is less than about 35%, the reduced CexTh1-xO2 becomes antiferromagnetic (AFM), whereas the ferromagnetic (FM) state dominates for x values above about 35%, which may allow the tailoring of magnetic properties by varying the CeO2 content. C1 [Xiao, H. Y.; Weber, W. J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Weber, W. J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Xiao, HY (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RI Xiao, Haiyan/A-1450-2012; Weber, William/A-4177-2008 OI Weber, William/0000-0002-9017-7365 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX This work was supported as part of the Materials Science of Actinides, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. The theoretical calculations were performed using the supercomputer resources at the Environmental Molecular Sciences Laboratory located at Pacific Northwest National Laboratory, and the National Energy Research Scientific Computing Center located at Lawrence Berkeley National Laboratory. NR 78 TC 29 Z9 29 U1 4 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 26 PY 2011 VL 115 IS 20 BP 6524 EP 6533 DI 10.1021/jp202016s PG 10 WC Chemistry, Physical SC Chemistry GA 764SE UT WOS:000290652100016 PM 21542655 ER PT J AU Han, SP van Duin, ACT Goddard, WA Strachan, A AF Han, Si-ping van Duin, Adri C. T. Goddard, William A., III Strachan, Alejandro TI Thermal Decomposition of Condensed-Phase Nitromethane from Molecular Dynamics from ReaxFF Reactive Dynamics SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID FORCE-FIELD; LIQUID NITROMETHANE; AB-INITIO; SIMULATIONS; DETONATION; MECHANISM; PRESSURE; HYDROCARBONS; KINETICS; OXIDE AB We studied the thermal decomposition and subsequent reaction of the energetic material nitromethane (CH3NO2) using molecular dynamics with ReaxFF, a first principles-based reactive force field. We characterize the chemistry of liquid and solid nitromethane at high temperatures (2000-3000 K) and density 1.97 g/cm(3) for times up to 200 ps. At T = 3000 K the first reaction in the decomposition of nitromethane is an intermolecular proton transfer leading to CH3NOOH and CH2NO2. For lower temperatures (T = 2500 and 2000 K) the first reaction during decomposition is often an isomerization reaction involving the scission of the C-N bond the formation of a C-O bond to form methyl nitrate (CH3ONO). Also at very early times we observe intramolecular proton transfer events. The main product of these reactions is H2O which starts forming following those initiation steps. The appearance of H2O marks the beginning of the exothermic chemistry. Recent quantum-mechanics-based molecular dynamics simulations on the chemical reactions and time scales for decomposition of a crystalline sample heated to T = 3000 K for a few picoseconds are in excellent agreement with our results, providing an important, direct validation of ReaxFF. C1 [Strachan, Alejandro] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. [Han, Si-ping] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Han, Si-ping; van Duin, Adri C. T.; Goddard, William A., III] CALTECH, Mat & Proc Simulat Ctr, Beckman Inst 139 74, Pasadena, CA 91125 USA. RP Strachan, A (reprint author), Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. EM strachan@purdue.edu FU Seaborg Institute; ASC Materials and Physics modeling project; DARPA; ONR [N00014-09-1-0634]; LANL [65287-001-08] FX S.H. would like to thank the Seaborg Institute for a summer fellowship, Jason Keith for preparation of the ReaxFF training set, and P.W.K. Rothemund for help in formatting the manuscript. Work at Los Alamos was supported by the ASC Materials and Physics modeling project and DARPA (program manager Carey Schwatz). Work at Caltech is supported by ONR (N00014-09-1-0634, program manager Cliff Bedford), LANL (65287-001-08, program manager Ed Kober), and DARPA (program manager Carey Schwatz). NR 31 TC 43 Z9 52 U1 6 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 26 PY 2011 VL 115 IS 20 BP 6534 EP 6540 DI 10.1021/jp1104054 PG 7 WC Chemistry, Physical SC Chemistry GA 764SE UT WOS:000290652100017 PM 21542572 ER PT J AU White, CE Provis, JL Proffen, T van Deventer, JSJ AF White, Claire E. Provis, John L. Proffen, Thomas van Deventer, Jannie S. J. TI Quantitative Mechanistic Modeling of Silica Solubility and Precipitation during the Initial Period of Zeolite Synthesis SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID MONTE-CARLO-SIMULATION; PRECURSOR NANOPARTICLES; HYDROTHERMAL SYNTHESIS; ALKALINE-SOLUTIONS; NETWORK FORMATION; DISSOLUTION; DIFFUSION; SYSTEM; CRYSTALLIZATION; CYCLIZATION AB The mechanistic details of the structural changes occurring during the initial stages of silica polymerization to form gels or zeolites remain largely unknown due mainly to the complexity of sol gel synthesis processes. Previous simulation studies have applied simple lattice models to qualitatively replicate spontaneous silica nanoparticle formation using fitted interaction energy parameters to replicate the behavior of real systems. This study moves for the first time to the use of quantum chemical-based interaction (dimerization) energies, determined through density functional theory computations, in a coarse-grained Monte Carlo simulation of the initial stages of gel/cluster formation in sodium silicate systems across a range of concentrations. The use of accurate dimerization energies as model inputs enables setniquantitatively accurate results to be obtained, as determined by comparisons with Si-29 nuclear magnetic resonance data. The most concentrated system simulated (9.36 m silica concentration) undergoes Ostwald ripening, whereby a single large cluster forms, indicative of colloidal silica formation. Furthermore, as the extent of the reaction progresses, this initial nonequilibrated cluster (known as the primary amorphous phase in the zeolite synthesis literature) is progressively transformed to the secondary amorphous phase via structural rearrangements, without significant changes in the overall size of the cluster. These results are in good agreement with previous experimental studies on the nature of the amorphous phase (s) present during silicate gelation and prior to zeolite crystallintion. Hence, this investigation demonstrates for the first time the successful application of multiscale simulation methodology to the coarse-grained Monte Carlo approach of a sot gel process, revealing important quantitative mechanistic information regarding complex silicate reaction processes. C1 [White, Claire E.; Provis, John L.; van Deventer, Jannie S. J.] Univ Melbourne, Dept Chem & Biomol Engn, Melbourne, Vic 3010, Australia. [White, Claire E.; Proffen, Thomas] Los Alamos Natl Lab, Lujan Neutron Scattering Ctr, Los Alamos, NM 87545 USA. RP Provis, JL (reprint author), Univ Melbourne, Dept Chem & Biomol Engn, Melbourne, Vic 3010, Australia. EM jprovis@unimelb.edu.au RI White, Claire/A-1722-2011; Lujan Center, LANL/G-4896-2012; Provis, John/A-7631-2008; Proffen, Thomas/B-3585-2009 OI White, Claire/0000-0002-4800-7960; Provis, John/0000-0003-3372-8922; Proffen, Thomas/0000-0002-1408-6031 FU Australian Research Council (ARC) via the Particulate Fluids Processing Centre, a Special Research Centre; Centre for Sustainable Resource Processing via the Geopolymer Alliance FX The authors would like to thank Dr. Daniel Riley, University of Melbourne/Australian Nuclear Science and Technology Organisation, for computational hardware support and insightful discussions. This work was funded in part by the Australian Research Council (ARC) (including some funding via the Particulate Fluids Processing Centre, a Special Research Centre of the ARC), and in part by a studentship paid to Claire White by the Centre for Sustainable Resource Processing via the Geopolymer Alliance. NR 44 TC 15 Z9 15 U1 4 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2011 VL 115 IS 20 BP 9879 EP 9888 DI 10.1021/jp2006217 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 764SF UT WOS:000290652200007 ER PT J AU Sasaki, K Kuttiyiel, KA Barrio, L Su, D Frenkel, AI Marinkovic, N Mahajan, D Adzic, RR AF Sasaki, Kotaro Kuttiyiel, Kurian A. Barrio, Laura Su, Dong Frenkel, Anatoly I. Marinkovic, Nebojsa Mahajan, Devinder Adzic, Radoslav R. TI Carbon-Supported IrNi Core-Shell Nanoparticles: Synthesis, Characterization, and Catalytic Activity SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; PLATINUM MONOLAYER; SURFACE SEGREGATION; ELECTROCATALYSTS; REDUCTION; EXAFS; TRANSITION; STABILITY; ALLOYS; GROWTH AB We synthesized carbon-supported IrNi core- shell nanoparticles by chemical reduction and subsequent thermal annealing in H(2), and verified the formation of Ir shells on IrNi solid solution alloy cores by various experimental methods. The EXAFS analysis is consistent with the model wherein the IrNi nanoparticles are composed of two-layer Ir shells and IrNi alloy cores. In situ XAS revealed that the Ir shells completely protect Ni atoms in the cores from oxidation or dissolution in an acid electrolyte under elevated potentials. The formation of Ir shell during annealing due to thermal segregation is monitored by time-resolved synchrotron XRD measurements, coupled with Rietveld refinement analyses. The H(2) oxidation activity of the IrNi nanoparticles was found to be higher than that of a commercial Pt/C catalyst. This is predominantly due to Ni-core-induced Ir shell contraction that makes the surface less reactive for IrOH formation, and the resulting more metallic Ir surface becomes more active for H(2) oxidation. This new class of core shell nanopartides appears promising for application as hydrogen anode fuel cell electrocatalysts. C1 [Sasaki, Kotaro; Kuttiyiel, Kurian A.; Barrio, Laura; Adzic, Radoslav R.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Mahajan, Devinder] Brookhaven Natl Lab, Dept Energy Sci, Upton, NY 11973 USA. [Frenkel, Anatoly I.] Yeshiva Univ, Dept Phys, New York, NY 10016 USA. [Marinkovic, Nebojsa] Univ Delaware, Dept Chem Engn, Newark, DE 19716 USA. RP Sasaki, K (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM ksasaki@bnl.gov RI Frenkel, Anatoly/D-3311-2011; Barrio, Laura/A-9509-2008; Su, Dong/A-8233-2013; Marinkovic, Nebojsa/A-1137-2016; OI Frenkel, Anatoly/0000-0002-5451-1207; Barrio, Laura/0000-0003-3496-4329; Su, Dong/0000-0002-1921-6683; Marinkovic, Nebojsa/0000-0003-3579-3453; Barrio, Laura/0000-0002-6919-6414 FU U.S. Department of Energy, Divisions of Chemical and Material Sciences [DE-AC02-98CH10886]; DOE BES [DE-FG02-03ER15476]; Synchrotron Catalysis Consortium, U.S. Department of Energy [DE-FG02-05ER15688] FX This work is supported by U.S. Department of Energy, Divisions of Chemical and Material Sciences under the Contract No. DE-AC02-98CH10886. A.I.F. acknowledges support by DOE BES Grant DE-FG02-03ER15476. Beamlines X19A and X18B at the NSLS are supported in part by the Synchrotron Catalysis Consortium, U.S. Department of Energy Grant No DE-FG02-05ER15688. NR 45 TC 17 Z9 17 U1 3 U2 54 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2011 VL 115 IS 20 BP 9894 EP 9902 DI 10.1021/jp200746j PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 764SF UT WOS:000290652200009 ER PT J AU Moon, HG Shim, YS Su, D Park, HH Yoon, SJ Jang, HW AF Moon, Hi Gyu Shim, Young-Seok Su, Dong Park, Hyung-Ho Yoon, Seok-Jin Jang, Ho Won TI Embossed TiO2 Thin Films with Tailored Links between Hollow Hemispheres: Synthesis and Gas-Sensing Properties SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SENSOR APPLICATIONS; HYDROGEN SENSOR; METAL-OXIDES; TEMPLATES; NANOBELTS; NANOWIRES; NANOSTRUCTURES; PERFORMANCE; FABRICATION; NANOFIBERS AB Embossed TiO2 thin films with high surface areas were achieved using soft templates composed of monolayer polystyrene beads. The structure of links between beads in the templates could be controlled by varying O-2 plasma etching time, resulting in a variety of templates with close-linked, nanolinked, or isolated beads. Room-temperature deposition of TiO2 on the plasma-treated templates and calcination at 550 degrees C resulted in embossed films with tailored links between anatase TiO2 hollow hemispheres. Although all embossed TiO2 films displayed a similar increase in the surface-to-volume ratio compared with a plain TiO2 thin film, the response of embossed TiO2 films with nanolinked hollow hemispheres to CO or ethanol gases was much higher than the response of films with close-linked or isolated. hollow hemispheres. The strong correlation between gas sensitivity and the structure of links between the TiO2 hollow hemispheres revealed the critical importance of tailoring links between individual oxide nanostructures for enhancing gas-sensing properties of the ensemble of the individual nanostructures. The facile and large-scale synthesis of embossed TiO2 films with nanolinked hollow hemispheres on Si substrates and the high sensitivity that is achieved without the aid of additives provide a sustainable competitive advantage over other methods for fabricating highly sensitive metal oxide gas sensors. C1 [Moon, Hi Gyu; Shim, Young-Seok; Yoon, Seok-Jin; Jang, Ho Won] Korea Inst Sci & Technol, Ctr Elect Mat, Seoul 136791, South Korea. [Moon, Hi Gyu; Park, Hyung-Ho] Yonsei Univ, Dept Mat Sci & Engn, Seoul 120749, South Korea. [Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Jang, HW (reprint author), Korea Inst Sci & Technol, Ctr Elect Mat, Seoul 136791, South Korea. EM hwjang@kist.re.kr RI Su, Dong/A-8233-2013; Jang, Ho Won/D-9866-2011 OI Su, Dong/0000-0002-1921-6683; Jang, Ho Won/0000-0002-6952-7359 FU Korea Ministry of Intelligence and Economy [K0004114]; KIST [2E22121]; U.S. Department of Energy, Office of Basic Energy Science [DE-AC02-98CH10886] FX This work was financially supported by the Core Technology of Materials Research and Development Program of the Korea Ministry of Intelligence and Economy (grant no. K0004114) and a KIST research program (grant no. 2E22121). We thank Mr. Kisslinger for his help with TEM sample preparation. The work of D.S. was supported by the U.S. Department of Energy, Office of Basic Energy Science, under contract no. DE-AC02-98CH10886. NR 43 TC 28 Z9 28 U1 2 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2011 VL 115 IS 20 BP 9993 EP 9999 DI 10.1021/jp2020325 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 764SF UT WOS:000290652200021 ER PT J AU Dolocan, A Acharya, DP Zahl, P Sutter, P Camillone, N AF Dolocan, A. Acharya, D. P. Zahl, P. Sutter, P. Camillone, N., III TI Two-Color Ultrafast Photoexcited Scanning Tunneling Microscopy SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RESOLVED 2-PHOTON PHOTOEMISSION; PHOTOELECTRON EMISSION; ELECTRON DYNAMICS; THERMAL-EXPANSION; PROBE MICROSCOPY; RESOLUTION; SURFACES; PULSE; RELAXATION; CU(110) AB We report on two-color two-photon photoexcitation of a metal surface driven by ultrafast laser pulses and detected with a scanning tunneling microscope (STM) tip as a proximate anode. Results are presented for two cases: (i) where the tip is retracted from the surface far enough to prohibit tunneling, and (ii) where the tip is within tunneling range of the surface. A delay-modulation technique is implemented to isolate the two-color photoemission from concurrent one-color two-photon photoemission and provide subpicosecond time-resolved detection. When applied with the tip in tunneling range, this approach effectively isolates the two-photon photoexcited current signal from the conventional tunneling current and enables subpicosecond time-resolved detection of the photoexcited surface electrons. The advantage of the two-color approach is highlighted by comparison with the one-color case where optical interference causes thermal modulation of the STM tip length, resulting in tunneling current modulations that are orders of magnitude larger than the current due to photoexcitation of surface electrons. By completely eliminating this interference, and thereby avoiding thermal modulation of the STM tip length, the two-color approach represents an important step toward the ultimate goal of simultaneous subnanometer and subpicosecond measurements of surface electron dynamics by ultrafast-laser-excited STM. C1 [Dolocan, A.; Camillone, N., III] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Acharya, D. P.; Zahl, P.; Sutter, P.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Camillone, N (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM nicholas@bnl.gov RI Zahl, Percy/B-1244-2008 OI Zahl, Percy/0000-0002-6629-7500 FU Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences [DE-AC02-98CH10886] FX We gratefully acknowledge M. G. White and J. Zhou for their help with frequency doubling. We also thank G. Hall and A. Harris for helpful discussions. The experiments were carried out at the Center for Functional Nanomaterials, a Nanoscale Science Research Center supported by the Office of Basic Energy Sciences, U.S. Department of Energy. The research was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, under Contract No. DE-AC02-98CH10886 as part of a Chemical Imaging initiative within the Catalysis Science Program. NR 43 TC 14 Z9 14 U1 3 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2011 VL 115 IS 20 BP 10033 EP 10043 DI 10.1021/jp111875f PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 764SF UT WOS:000290652200027 ER PT J AU Pan, YX Mei, DH Liu, CJ Ge, QF AF Pan, Yun-xiang Mei, Donghai Liu, Chang-jun Ge, Qingfeng TI Hydrogen Adsorption on Ga2O3 Surface: A Combined Experimental and Computational Study SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID GAMMA-ALUMINA SURFACES; AUGMENTED-WAVE METHOD; GALLIUM OXIDE; OXYGEN VACANCY; BETA-GA2O3; PHOTOCATALYST; POLYMORPHS; CO2; DECOMPOSITION; GAMMA-GA2O3 AB In the present work, hydrogen adsorption on the Ga2O3 surfaces was investigated using Fourier transform infrared spectroscopy (FTIR) measurements and periodic density functional theory (DFT) calculations. Both the FTIR and DFT studies suggest that H-2 dissociates on the Ga2O3 surfaces, producing OH and GaH species. The FTIR bands at 3730, 3700, 3630, and 3600 cm(-1) are attributed to the vibration of the OH species whereas those at 2070 and 1990 cm(-1) to the GaH species. The structures of the species detected in experiments are established through a comparison with the DFT calculated stretching frequencies. The O atom of the experimentally detected OH species is believed to originate from the three-coordinated surface O atom. However, the H adatom that binds the coordinately unsaturated Ga atom results in the experimentally detected GaH species. Dissociative adsorption of H-2 on the perfect Ga2O3 surface, with the formation of both OH and GaH species, is endothermic and has an energy barrier of 0.90 eV. In contrast, dissociative adsorption of H-2 on the defective Ga2O3 surface with oxygen vacancies, which mainly produces GaH species, is exothermic, with an energy barrier of 0.61 eV. Accordingly, presence of the oxygen vacancies promotes H-2 dissociation and production of GaH species on the Ga2O3 surfaces. Higher temperatures are expected to favor oxygen vacancy creation on the Ga2O3 surfaces and thereby benefit the production of GaH species. This analysis is consistent with the FTIR results that the bands assigned to GaH species become stronger at higher temperatures. C1 [Pan, Yun-xiang; Liu, Chang-jun] Tianjin Univ, Sch Chem Engn, Adv Nano Technol Ctr, Tianjin 300072, Peoples R China. [Mei, Donghai] Pacific NW Natl Lab, Inst Interfacial Catalysis, Richland, WA 99352 USA. [Ge, Qingfeng] So Illinois Univ, Dept Chem & Biochem, Carbondale, IL 62901 USA. RP Liu, CJ (reprint author), Tianjin Univ, Sch Chem Engn, Adv Nano Technol Ctr, Tianjin 300072, Peoples R China. EM ughg_cjl@yahoo.com; qge@chem.siu.edu RI Mei, Donghai/D-3251-2011; Ge, Qingfeng/A-8498-2009; Mei, Donghai/A-2115-2012; Pan, Yun-xiang/G-6904-2015; OI Ge, Qingfeng/0000-0001-6026-6693; Mei, Donghai/0000-0002-0286-4182; Liu, Chang-jun/0000-0001-9918-1638 FU National Natural Science Foundation of China [20990223]; Pacific Northwest National Laboratory (PNNL); National Energy Research Scientific Computing Center (NERSC) [752] FX We gratefully acknowledge the support from the National Natural Science Foundation of China (#20990223). D. Mei was supported by a Laboratory Directed Research and Development (LDRD) project at Pacific Northwest National Laboratory (PNNL). The computations were performed using the Molecular Science Computing Facility in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), which is a U.S. Department of Energy national scientific user facility located at PNNL in Richland, Washington. Part of the computing time was also granted by the National Energy Research Scientific Computing Center (NERSC) under project No. 752. NR 36 TC 18 Z9 19 U1 4 U2 62 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2011 VL 115 IS 20 BP 10140 EP 10146 DI 10.1021/jp2014226 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 764SF UT WOS:000290652200039 ER PT J AU Priyadarshini, D Kondratyuk, P Picard, YN Morreale, BD Gellman, AJ Miller, JB AF Priyadarshini, Deepika Kondratyuk, Petro Picard, Yoosuf N. Morreale, Bryan D. Gellman, Andrew J. Miller, James B. TI High-Throughput Characterization of Surface Segregation in CuxPd1-x Alloys SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID POLYCRYSTALLINE PD70CU30 ALLOY; SINGLE-CRYSTAL ALLOY; CU-PD SYSTEM; AG-AU ALLOYS; HYDROGEN SEPARATION; ELEVATED-TEMPERATURES; COMPOSITE MEMBRANES; COMPOSITION SPREADS; TERNARY ALLOYS; BINARY-ALLOYS AB A high throughput methodology for the study of surface segregation in alloys has been developed and applied to the CuxPd1-x system. A novel offset-filament deposition tool was used to prepare CuxPd1-x composition spread alloy films (CSAFs), high throughput sample libraries with continuous lateral composition variation spanning the range x = 0.05-0.95. Spatially resolved low energy ion scattering spectroscopy (LEISS) and X-ray photoelectron spectroscopy (XPS) were used to characterize the films' top-surface and near-surface compositions, respectively, as functions of alloy composition, x, and temperature. Electron backscatter diffraction (EBSD) was used to identify the bulk phases in the CSAF as a function of alloy composition, x. Films equilibrated by annealing at temperatures >= 700 K displayed preferential segregation of Cu to their top-surfaces at all bulk compositions; segregation patterns did not, however, depend on local structure. The Langmuir-McLean thermodynamic model was applied to segregation measurements made in the temperature range 700-900 K in order to estimate the enthalpy (Delta H-seg) and entropy (Delta S-seg) of segregation as a function of bulk CuxPd1-x composition. Segregation measurements at x = 0.30 on the CSAF compare well with results previously reported for a bulk, polycrystalline Cu0.30Pd0.70 alloy, demonstrating the utility of the CSAF as a high throughput library for study of segregation. C1 [Priyadarshini, Deepika; Kondratyuk, Petro; Morreale, Bryan D.; Gellman, Andrew J.; Miller, James B.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Priyadarshini, Deepika; Kondratyuk, Petro; Gellman, Andrew J.; Miller, James B.] Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA. [Picard, Yoosuf N.] Carnegie Mellon Univ, Dept Mat Sci & Engn, Pittsburgh, PA 15213 USA. RP Miller, JB (reprint author), US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. EM jbmiller@andrew.cmu.edu RI Gellman, Andrew/M-2487-2014; OI Gellman, Andrew/0000-0001-6618-7427; Picard, Yoosuf/0000-0002-2853-5213 FU National Energy Technology Laboratory's ongoing research in Computational and Basic Sciences under RDS [DE-AC26-04NT41817]; RDS [DE-FE0004000] FX This technical effort was performed in support of the National Energy Technology Laboratory's ongoing research in Computational and Basic Sciences under RDS Contract DE-AC26-04NT41817 and RDS contract DE-FE0004000. NR 72 TC 19 Z9 19 U1 5 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2011 VL 115 IS 20 BP 10155 EP 10163 DI 10.1021/jp201793d PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 764SF UT WOS:000290652200041 ER PT J AU Presiado, I Lal, J Mamontov, E Kolesnikov, AI Huppert, D AF Presiado, Itay Lal, Jyotsana Mamontov, Eugene Kolesnikov, Alexander I. Huppert, Dan TI Fast Proton Hopping Detection in Ice I-h by Quasi-Elastic Neutron Scattering SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DOPED ICE; HYDROCHLORIC-ACID; ISOTOPIC EXCHANGE; ELEMENTARY STEPS; LIQUID WATER; DIFFUSION; DYNAMICS; CONDUCTIVITY; MECHANISM; MOBILITY AB Quasi-elastic neutron scattering was employed on samples of HCl-doped polycrystalline ice I-h. The analysis of the scattering signal provides the excess proton hopping time, tau(hop), in the temperature range of 140-195 K. The hopping time strongly depends on the temperature of the sample, and the activation energy of a hopping step is 17 kJ/mol. The values of tau(hop) of the current experiment are in good agreement with calculated values derived from previous photochemical experiments,(1) in which we found that the proton hopping time at T > 242 K is on the order of 200 fs, roughly 10 times shorter than in liquid water at room temperature. C1 [Presiado, Itay; Huppert, Dan] Tel Aviv Univ, Raymond & Beverly Sackler Fac Exact Sci, Sch Chem, IL-69978 Tel Aviv, Israel. [Lal, Jyotsana] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Mamontov, Eugene; Kolesnikov, Alexander I.] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. RP Huppert, D (reprint author), Tel Aviv Univ, Raymond & Beverly Sackler Fac Exact Sci, Sch Chem, IL-69978 Tel Aviv, Israel. EM huppert@tulip.tau.ac.il RI Kolesnikov, Alexander/I-9015-2012; Mamontov, Eugene/Q-1003-2015 OI Kolesnikov, Alexander/0000-0003-1940-4649; Mamontov, Eugene/0000-0002-5684-2675 FU Israel Science Foundation; James-Franck German-Israeli Program; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy [DE-AC0500OR22725]; US DOE-BES [DE-AC02-06CH11357] FX This work was supported by grants from the Israel Science Foundation and from the James-Franck German-Israeli Program in Laser-Matter Interaction. The experiment at Oak Ridge National Laboratory's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; ORNL is managed by UT-Batelle, LLC, under contract DE-AC0500OR22725 for the U.S. Department of Energy. Work at ANL was performed under the auspices of the US DOE-BES under contract DE-AC02-06CH11357. NR 43 TC 17 Z9 17 U1 0 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2011 VL 115 IS 20 BP 10245 EP 10251 DI 10.1021/jp2008094 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 764SF UT WOS:000290652200052 ER PT J AU DiMaio, F Terwilliger, TC Read, RJ Wlodawer, A Oberdorfer, G Wagner, U Valkov, E Alon, A Fass, D Axelrod, HL Das, D Vorobiev, SM Iwai, H Pokkuluri, PR Baker, D AF DiMaio, Frank Terwilliger, Thomas C. Read, Randy J. Wlodawer, Alexander Oberdorfer, Gustav Wagner, Ulrike Valkov, Eugene Alon, Assaf Fass, Deborah Axelrod, Herbert L. Das, Debanu Vorobiev, Sergey M. Iwai, Hideo Pokkuluri, P. Raj Baker, David TI Improved molecular replacement by density- and energy-guided protein structure optimization SO NATURE LA English DT Article ID LOW-RESOLUTION; CRYSTALLOGRAPHIC REFINEMENT; SOFTWARE; PREDICTION; ACCURACY; ROSETTA AB Molecular replacement(1-4) procedures, which search for placements of a starting model within the crystallographic unit cell that best account for the measured diffraction amplitudes, followed by automatic chain tracing methods(5-8), have allowed the rapid solution of large numbers of protein crystal structures. Despite extensive work(9-14), molecular replacement or the subsequent rebuilding usually fail with more divergent starting models based on remote homologues with less than 30% sequence identity. Here we show that this limitation can be substantially reduced by combining algorithms for protein structure modelling with those developed for crystallographic structure determination. An approach integrating Rosetta structure modelling with Autobuild chain tracing yielded high-resolution structures for 8 of 13 X-ray diffraction data sets that could not be solved in the laboratories of expert crystallographers and that remained unsolved after application of an extensive array of alternative approaches. We estimate that the new method should allow rapid structure determination without experimental phase information for over half the cases where current methods fail, given diffraction data sets of better than 3.2 angstrom resolution, four or fewer copies in the asymmetric unit, and the availability of structures of homologous proteins with >20% sequence identity. C1 [Terwilliger, Thomas C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [DiMaio, Frank; Baker, David] Univ Washington, Dept Biochem, Seattle, WA 98195 USA. [DiMaio, Frank; Baker, David] Univ Washington, Howard Hughes Med Inst, Seattle, WA 98195 USA. [Read, Randy J.] Univ Cambridge, Dept Haematol, Cambridge Inst Med Res, Cambridge CB2 0XY, England. [Wlodawer, Alexander] NCI, Macromol Crystallog Lab, Frederick, MD 21702 USA. [Oberdorfer, Gustav; Wagner, Ulrike] Graz Univ, Inst Mol Biosci, A-8010 Graz, Austria. [Valkov, Eugene] Univ Cambridge, Dept Biochem, Cambridge CB2 1GA, England. [Alon, Assaf; Fass, Deborah] Weizmann Inst Sci, Dept Biol Struct, IL-76100 Rehovot, Israel. [Axelrod, Herbert L.; Das, Debanu] SLAC Natl Accelerator Lab, Joint Ctr Struct Genom, Menlo Pk, CA 94025 USA. [Axelrod, Herbert L.; Das, Debanu] SLAC Natl Accelerator Lab, SSRL, Menlo Pk, CA 94025 USA. [Vorobiev, Sergey M.] Columbia Univ, NE Struct Genom Consortium, New York, NY 10027 USA. [Iwai, Hideo] Univ Helsinki, Inst Biotechnol, FI-00014 Helsinki, Finland. [Pokkuluri, P. Raj] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. RP Terwilliger, TC (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM terwilliger@lanl.gov; dabaker@u.washington.edu RI Iwai, Hideo/A-6416-2009; Valkov, Eugene/C-1554-2010; Read, Randy/L-1418-2013; Terwilliger, Thomas/K-4109-2012; Baker, David/K-8941-2012 OI Iwai, Hideo/0000-0001-7376-5264; Read, Randy/0000-0001-8273-0047; Terwilliger, Thomas/0000-0001-6384-0320; Baker, David/0000-0001-7896-6217 FU NIH [5R01GM092802, P41RR002250]; Wellcome Trust; HHMI; Israel Science Foundation; DK Molecular Enzymology [W901]; Austrian Science Fund [P19858]; NIH, National Cancer Institute, Center for Cancer Research; academy of Finland [1131413]; Protein Structure Initiative of National Institute of General Medical Sciences [U54 GM074958]; US Department of Energy's Office of Science, Biological and Environmental Research [DE-AC02-06CH11357]; NIH, National Institutes of General Medical Sciences, Protein Structure Initiative [U54 GM094586, GM074898] FX R.J.R., T.C.T. and D.B. thank the NIH (5R01GM092802), the Wellcome Trust (R.J.R.), and HHMI (D.B.) for funding this research. F.D. acknowledges the NIH (P41RR002250) and HHMI. D.F. and A.A. acknowledge support from the Israel Science Foundation. G.O. thanks DK Molecular Enzymology (FWF-project W901) and the Austrian Science Fund (FWF-project P19858). The work of A.W. was supported by the Intramural Research Program of the NIH, National Cancer Institute, Center for Cancer Research. H.I. acknowledges support from the academy of Finland (1131413). S.M.V. was supported by a grant from the Protein Structure Initiative of National Institute of General Medical Sciences (U54 GM074958). The work of P.R.P. at Argonne National Laboratory was supported by the US Department of Energy's Office of Science, Biological and Environmental Research GTL programme under contract DE-AC02-06CH11357. We thank all members of the JCSG for their general contributions to the protein production and structural work. The JCSG is supported by the NIH, National Institutes of General Medical Sciences, Protein Structure Initiative (U54 GM094586 and GM074898). NR 29 TC 123 Z9 124 U1 2 U2 34 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAY 26 PY 2011 VL 473 IS 7348 BP 540 EP U149 DI 10.1038/nature09964 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 768QM UT WOS:000290951300047 PM 21532589 ER PT J AU Ilie, C Freese, K Spolyar, D AF Ilie, Cosmin Freese, Katherine Spolyar, Douglas TI Dark stars and boosted dark matter annihilation rates SO NEW JOURNAL OF PHYSICS LA English DT Article ID 1ST STARS; FERMI LAT; PAMELA; HALOS; EVOLUTION; POSITRON; MASS; UNIVERSE; TELESCOPE; OPACITIES AB Dark stars (DSs) may constitute the first phase of stellar evolution, powered by dark matter (DM) annihilation. We investigate here the properties of DSs, assuming that the DM particle has the properties required for explaining the excess positron and electron signals in the cosmic rays detected by the PAMELA and FERMI satellites. Any possible DM interpretation of these signals will require exotic DM candidates, with annihilation cross-sections a few orders of magnitude higher than the canonical value required for correct thermal relic abundance for weakly interacting DM candidates; additionally, in most models, the annihilation must be preferentially to leptons. Secondly, we study the dependence of DS properties on the concentration parameter of the initial DM density profile of the halos where the first stars are formed. We restrict our study to the DM in the star due to simple (versus extended) adiabatic contraction and minimal (versus extended) capture; this simple study is sufficient to illustrate dependence on the cross-section and concentration parameter. Our basic results are that the final stellar properties, once the star enters the main sequence, are always roughly the same, regardless of the value of the boosted annihilation or concentration parameter in the range between c = 2 and c = 5: stellar mass similar to 1000M(circle dot), luminosity similar to 10(7)L(circle dot) and lifetime similar to 10(6) years (for the minimal DM models considered here; additional DM would lead to more massive DSs). However, the lifetime, final mass and final luminosity of the DSs show some dependence on the boost factor and concentration parameter, as discussed in this paper. C1 [Ilie, Cosmin; Freese, Katherine] Univ Michigan, Dept Phys, Michigan Ctr Theoret Phys, Ann Arbor, MI 48109 USA. [Spolyar, Douglas] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA. RP Ilie, C (reprint author), Univ Michigan, Dept Phys, Michigan Ctr Theoret Phys, Ann Arbor, MI 48109 USA. EM cilie@umich.edu FU DOE; Michigan Center for Theoretical Physics at the University of Michigan; DOE at Fermilab FX We acknowledge support from the DOE and the Michigan Center for Theoretical Physics at the University of Michigan (to CI and KF) and the DOE at Fermilab (to DS). We thank Pearl Sandick for helpful conversations and the anonymous referees for helpful suggestions for the improvement of the manuscript. NR 123 TC 4 Z9 4 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD MAY 26 PY 2011 VL 13 AR 053050 DI 10.1088/1367-2630/13/5/053050 PG 27 WC Physics, Multidisciplinary SC Physics GA 782IW UT WOS:000292002700001 ER PT J AU Yu, XH Rawat, R Shanklin, J AF Yu, Xiao-Hong Rawat, Richa Shanklin, John TI Characterization and analysis of the cotton cyclopropane fatty acid synthase family and their contribution to cyclopropane fatty acid synthesis SO BMC PLANT BIOLOGY LA English DT Article ID ADENOSYLMETHIONINE-DEPENDENT METHYLTRANSFERASES; AGROBACTERIUM-MEDIATED TRANSFORMATION; MYCOBACTERIUM-TUBERCULOSIS; MYCOLIC ACIDS; STEARIC-ACID; SEED OIL; STERCULIA-FOETIDA; LIPID-COMPOSITION; SEQUENCE MOTIFS; HEN LIVER AB Background: Cyclopropane fatty acids (CPA) have been found in certain gymnosperms, Malvales, Litchi and other Sapindales. The presence of their unique strained ring structures confers physical and chemical properties characteristic of unsaturated fatty acids with the oxidative stability displayed by saturated fatty acids making them of considerable industrial interest. While cyclopropenoid fatty acids (CPE) are well-known inhibitors of fatty acid desaturation in animals, CPE can also inhibit the stearoyl-CoA desaturase and interfere with the maturation and reproduction of some insect species suggesting that in addition to their traditional role as storage lipids, CPE can contribute to the protection of plants from herbivory. Results: Three genes encoding cyclopropane synthase homologues GhCPS1, GhCPS2 and GhCPS3 were identified in cotton. Determination of gene transcript abundance revealed differences among the expression of GhCPS1, 2 and 3 showing high, intermediate and low levels, respectively, of transcripts in roots and stems; whereas GhCPS1 and 2 are both expressed at low levels in seeds. Analyses of fatty acid composition in different tissues indicate that the expression patterns of GhCPS1 and 2 correlate with cyclic fatty acid (CFA) distribution. Deletion of the N-terminal oxidase domain lowered GhCPS's ability to produce cyclopropane fatty acid by approximately 70%. GhCPS1 and 2, but not 3 resulted in the production of cyclopropane fatty acids upon heterologous expression in yeast, tobacco BY2 cell and Arabidopsis seed. Conclusions: In cotton GhCPS1 and 2 gene expression correlates with the total CFA content in roots, stems and seeds. That GhCPS1 and 2 are expressed at a similar level in seed suggests both of them can be considered potential targets for gene silencing to reduce undesirable seed CPE accumulation. Because GhCPS1 is more active in yeast than the published Sterculia CPS and shows similar activity when expressed in model plant systems, it represents a strong candidate gene for CFA accumulation via heterologous expression in production plants. C1 [Yu, Xiao-Hong; Rawat, Richa; Shanklin, John] SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA. [Shanklin, John] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. RP Shanklin, J (reprint author), SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA. EM shanklin@bnl.gov FU Office of Basic Energy Sciences of the U.S. Department of Energy; National Science Foundation [DBI 0701919] FX We thank Dr. Carl Andre at Brookhaven National Laboratory for critical reading of our manuscript, Prof. John Ohlorogge at Michigan State University for SfCPS gene, Prof. Kent Chapman at the University of North Texas for providing us with the cotton seeds, and Mr. Kevin Lutke from Donald Danforth Plant Science Center who helped with the BY2 transformation. This work was supported by the Office of Basic Energy Sciences of the U.S. Department of Energy (JS), and by the National Science Foundation (Grant DBI 0701919) (RR and X-HY). NR 48 TC 13 Z9 14 U1 1 U2 32 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2229 J9 BMC PLANT BIOL JI BMC Plant Biol. PD MAY 25 PY 2011 VL 11 AR 97 DI 10.1186/1471-2229-11-97 PG 10 WC Plant Sciences SC Plant Sciences GA 789ZN UT WOS:000292558400001 PM 21612656 ER PT J AU Hin, C Lepinoux, J Neaton, JB Dresselhaus, M AF Hin, Celine Lepinoux, Joel Neaton, Jeffrey B. Dresselhaus, Mildred TI From the interface energy to the solubility limit of aluminium in nickel from first-principles and Kinetic Monte Carlo calculations SO MATERIALS SCIENCE AND ENGINEERING B-ADVANCED FUNCTIONAL SOLID-STATE MATERIALS LA English DT Article DE Phase diagrams; First-principles calculations; Interface energy ID WAVE BASIS-SET; AL-NI SYSTEM; COHESIVE ENERGY; SURFACE-TENSION; BINARY-ALLOYS; METALS; PHASE; NI3AL; BOUNDARIES; MODEL AB We developed a way to predict the solubility limit of solute atoms in a binary alloy using a Kinetic Monte Carlo algorithm. The idea is to use the interface energies calculated by first-principles calculations to parameterize the pair interaction energies used in the Kinetic Monte Carlo algorithm. In order to validate this method, it was tested on a very well known case: the Ni-Al alloy. We found that the calculations are in very good agreement with the previously calculated phase diagrams. (C) 2011 Elsevier B.V. All rights reserved. C1 [Hin, Celine] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Lepinoux, Joel] UJF, CNRS, Grenoble INP, SIMaP, F-38402 St Martin Dheres, France. [Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Lab, Mol Foundry, Berkeley, CA 94720 USA. [Dresselhaus, Mildred] MIT, Dept Phys, Cambridge, MA 02139 USA. RP Hin, C (reprint author), MIT, Dept Mech Engn, Cambridge, MA 02139 USA. EM celine_hin@yahoo.fr RI Neaton, Jeffrey/F-8578-2015 OI Neaton, Jeffrey/0000-0001-7585-6135 FU Department of Energy [DE-FG02-08ER46516] FX We gratefully acknowledge useful and stimulating discussions with Professor W.C. Carter. The authors gratefully acknowledge the financial support of the Department of Energy under Grant DE-FG02-08ER46516. NR 45 TC 3 Z9 3 U1 3 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-5107 J9 MATER SCI ENG B-ADV JI Mater. Sci. Eng. B-Adv. Funct. Solid-State Mater. PD MAY 25 PY 2011 VL 176 IS 9 BP 767 EP 771 DI 10.1016/j.mseb.2011.02.023 PG 5 WC Materials Science, Multidisciplinary; Physics, Condensed Matter SC Materials Science; Physics GA 779DE UT WOS:000291757500014 ER PT J AU Li, ADQ Zhan, CL Hu, DH Wan, W Yao, JN AF Li, Alexander D. Q. Zhan, Chuanlang Hu, Dehong Wan, Wei Yao, Jiannian TI Photoswitchable Nanoprobes Offer Unlimited Brightness in Frequency-Domain Imaging SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID FLUORESCENCE; NANOPARTICLES; RECOVERY AB A single probe has limited brightness in time-domain imaging and such limitation frequently renders individual molecules undetectable in the presence of interference or complex cellular structures. However, a single photoswitchable probe produces a signal, which can be separated from interference or noise using photoswitching-enabled Fourier transformation (PFT). As a result, the light-modulated probes can be made super bright in the frequency domain simply by acquiring more cycles in the time domain. C1 [Li, Alexander D. Q.; Wan, Wei] Washington State Univ, Dept Chem, Pullman, WA 99164 USA. [Li, Alexander D. Q.; Wan, Wei] Washington State Univ, Ctr Mat Res, Pullman, WA 99164 USA. [Zhan, Chuanlang; Yao, Jiannian] Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China. [Hu, Dehong] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Li, ADQ (reprint author), Washington State Univ, Dept Chem, Pullman, WA 99164 USA. EM dequan@wsu.edu RI Zhan, Chuanlang/F-5247-2011; Yao, Jiannian/A-9773-2012; Hu, Dehong/B-4650-2010 OI Zhan, Chuanlang/0000-0001-5127-0973; Hu, Dehong/0000-0002-3974-2963 FU National Science Foundation [CHE-0805547] FX We acknowledge the support of National Science Foundation (CHE-0805547). A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 15 TC 23 Z9 23 U1 3 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 25 PY 2011 VL 133 IS 20 BP 7628 EP 7631 DI 10.1021/ja1108479 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 776ZN UT WOS:000291580400003 PM 21539363 ER PT J AU Bhandari, D Kravchenko, II Lavrik, NV Sepaniak, MJ AF Bhandari, Deepak Kravchenko, Ivan I. Lavrik, Nickolay V. Sepaniak, Michael J. TI Nanotransfer Printing Using Plasma Etched Silicon Stamps and Mediated by in Situ Deposited Fluoropolymer SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ELECTRICAL CONTACTS; FILMS; LITHOGRAPHY; NANOFABRICATION; FABRICATION; THIN AB This communication describes a simple method that uses a thin film of octafluorocyclobutane (OFCB) polymer for efficient nanoscale transfer printing (nTP). Plasma polymerization of OFCB produces a Teflon-like fluoropolymer which strongly adheres and conformally covers a 3-D inorganic stamp. The inherently low surface energy of in situ deposited OFCB polymer on nanoscale silicon features is demonstrated as a unique nanocomposite stamp to fabricate various test structures with improved nTP feature resolution down to sub-100 nm. C1 [Bhandari, Deepak; Sepaniak, Michael J.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Kravchenko, Ivan I.; Lavrik, Nickolay V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Sepaniak, MJ (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM msepaniak@utk.edu RI Kravchenko, Ivan/K-3022-2015; Lavrik, Nickolay/B-5268-2011 OI Kravchenko, Ivan/0000-0003-4999-5822; Lavrik, Nickolay/0000-0002-9543-5634 FU Scientific User Facilities Division, U.S. Department of Energy at Oak Ridge National Laboratory FX A portion of this research was conducted at the Center for Nanophase Materials Sciences (CNMS) and Shared Research Equipment (SHaRE) User Facility, which are sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, U.S. Department of Energy. We thank Dr. H. M. Meyer III for assistance with X-ray photoelectron spectroscopy. NR 20 TC 6 Z9 6 U1 1 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 25 PY 2011 VL 133 IS 20 BP 7722 EP 7724 DI 10.1021/ja201497a PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 776ZN UT WOS:000291580400027 PM 21526774 ER PT J AU Wu, HP Pan, SL Poeppelmeier, KR Li, HY Jia, DZ Chen, ZH Fan, XY Yang, Y Rondinelli, JM Luo, HS AF Wu, Hongping Pan, Shilie Poeppelmeier, Kenneth R. Li, Hongyi Jia, Dianzeng Chen, Zhaohui Fan, Xiaoyun Yang, Yun Rondinelli, James M. Luo, Haosu TI K3B6O10Cl: A New Structure Analogous to Perovskite with a Large Second Harmonic Generation Response and Deep UV Absorption Edge SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID NONLINEAR-OPTICAL CRYSTAL; AUGMENTED-WAVE METHOD; K2AL2B2O7 CRYSTALS; BORATE CRYSTALS; SINGLE-CRYSTALS; KBBF CRYSTAL; GROWTH; RB; POLAR; BI2ZNOB2O6 AB Introduction of the Cl anion in the borate systems generates a new perovskite-like phase, K3B6O10Cl, which exhibits a large second harmonic response, about four times that of KH2PO4 (KDP), and is transparent from the deep UV (180 nm) to middle-IR region. K3B6O10Cl crystallizes in the noncentrosymmetric and rhombohedral space group R3m. The structure consists of the A-site hexaborate [B6O10] groups and the BX3 Cl-centered octahedral [ClK6] groups linked together through vertices to form the perovskite framework represented by ABX(3). C1 [Wu, Hongping; Pan, Shilie; Li, Hongyi; Chen, Zhaohui; Fan, Xiaoyun; Yang, Yun] Chinese Acad Sci, Xinjiang Key Lab Elect Informat Mat & Devices, Xinjiang Tech Inst Phys & Chem, Urumqi 830011, Peoples R China. [Wu, Hongping; Jia, Dianzeng] Xinjiang Univ, Coll Chem & Chem Engn, Urumqi 830046, Peoples R China. [Poeppelmeier, Kenneth R.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Rondinelli, James M.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Luo, Haosu] Chinese Acad Sci, State Key Lab High Performance Ceram & Superfine, Shanghai Inst Ceram, Shanghai 201800, Peoples R China. RP Pan, SL (reprint author), Chinese Acad Sci, Xinjiang Key Lab Elect Informat Mat & Devices, Xinjiang Tech Inst Phys & Chem, 40-1 S Beijing Rd, Urumqi 830011, Peoples R China. EM slpan@ms.xjb.ac.cn; krp@northwestern.edu RI Rondinelli, James/A-2071-2009 OI Rondinelli, James/0000-0003-0508-2175 FU Chinese Academy of Sciences [KJCX2-EW-H03-03]; National Natural Science Foundation of China [50802110, 21001114]; "One Hundred Talents Project Foundation" of Chinese Academy of Sciences; "Western Light Joint Scholar Foundation" of Chinese Academy of Sciences; "High Technology Research and Development Program" of Xinjiang Uygur Autonomous Region of China [200816120]; Scientific Research Program of Urumqi of China [G09212001]; National Science Foundation [DMR-1005827]; U.S. DOE, Office of Science [DE-AC02-06CH11357] FX This work is supported by Main Direction Program of Knowledge Innovation of Chinese Academy of Sciences (Grant No. KJCX2-EW-H03-03), the "National Natural Science Foundation of China" (Grant Nos. 50802110, 21001114), the "One Hundred Talents Project Foundation Program" of Chinese Academy of Sciences, the "Western Light Joint Scholar Foundation" Program of Chinese Academy of Sciences, the "High Technology Research and Development Program" of Xinjiang Uygur Autonomous Region of China (Grant No. 200816120), and Scientific Research Program of Urumqi of China (Grant No. G09212001). K.R.P. acknowledges the National Science Foundation Solid State Chemistry Award No. DMR-1005827. J.M.R. was supported by the U.S. DOE, Office of Science, under Contract No. DE-AC02-06CH11357. Computations were carried out at the Laboratory Computing Resource Center (LCRC) at Argonne National Laboratory. NR 67 TC 224 Z9 228 U1 8 U2 109 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 25 PY 2011 VL 133 IS 20 BP 7786 EP 7790 DI 10.1021/ja111083x PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 776ZN UT WOS:000291580400034 PM 21534555 ER PT J AU Shi, X Yang, J Salvador, JR Chi, MF Cho, JY Wang, H Bai, SQ Yang, JH Zhang, WQ Chen, LD AF Shi, Xun Yang, Jiong Salvador, James R. Chi, Miaofang Cho, Jung Y. Wang, Hsin Bai, Shengqiang Yang, Jihui Zhang, Wenqing Chen, Lidong TI Multiple-Filled Skutterudites: High Thermoelectric Figure of Merit through Separately Optimizing Electrical and Thermal Transports SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID FILLING FRACTION; BULK MATERIALS; COSB3; PERFORMANCE; CONDUCTIVITY; CRYSTALS; DEVICES; BARIUM AB Skutterudites CoSb(3) with multiple cofillers Ba, La, and Yb were synthesized and very high thermoelectric figure of merit ZT = 1.7 at 850 K was realized. X-ray diffraction of the densified multiple-filled bulk samples reveals all samples are phase pure. High-resolution scanning transmission electron microscopy (STEM) and energy dispersive X-ray spectroscopy (EDS) analysis confirm that multiple guest fillers occupy the nanoscale-cages in the skutterudites. The fillers are further shown to be uniformly distributed and the Co-Sb skutterudite framework is virtually unperturbed from atomic scale to a few micrometers. Our results firmly show that high power factors can be realized by adjusting the total filling fraction of fillers with different charge states to reach the optimum carrier density, at the same time, lattice thermal conductivity can also be significantly reduced, to values near the glass limit of these materials, through combining filler species of different rattling frequencies to achieve broad-frequency phonon scattering. Therefore, partially filled skutterudites with multiple fillers of different chemical nature render unique structural characteristics for optimizing electrical and thermal transports in a relatively independent way, leading to continually enhanced ZT values from single- to double-, and finally to multiple-filled skutterudites. The idea of combining multiple fillers with different charge states and rattling frequencies for performance optimization is also expected to be valid for other caged TE compounds. C1 [Yang, Jihui] Gen Motors R&D Ctr, Electrochem Energy Res Lab, Warren, MI 48090 USA. [Shi, Xun; Yang, Jiong; Zhang, Wenqing] Chinese Acad Sci, State Key Lab High Performance Ceram & Superfine, Shanghai Inst Ceram, Shanghai 200050, Peoples R China. [Shi, Xun; Salvador, James R.; Cho, Jung Y.] Gen Motors R&D Ctr, Chem Sci & Mat Syst Lab, Warren, MI 48090 USA. [Chi, Miaofang; Wang, Hsin] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Bai, Shengqiang; Chen, Lidong] Chinese Acad Sci, CAS Key Lab Mat Energy Convers, Shanghai Inst Ceram, Shanghai 200050, Peoples R China. RP Yang, JH (reprint author), Gen Motors R&D Ctr, Electrochem Energy Res Lab, Warren, MI 48090 USA. EM jihui.yang@gm.com; wqzhang@mail.sic.ac.cn; dd@mail.sic.ac.cn RI shi, xun/B-4499-2009; Yang, Jihui/A-3109-2009; Chen, Lidong/F-2705-2010; Zhang, Wenqing/K-1236-2012; Yang, Jiong/K-6330-2014; Chi, Miaofang/Q-2489-2015; Wang, Hsin/A-1942-2013 OI shi, xun/0000-0002-3806-0303; Yang, Jiong/0000-0002-5862-5981; Chi, Miaofang/0000-0003-0764-1567; Wang, Hsin/0000-0003-2426-9867 FU GM; DOE [DE-FC26-04NT42278, DEAC05000OR22725]; National Basic Research Program of China (973-program) [2007CB607503]; NSFC [50825205, 50672118, 50821004, 50820145203, 10634070]; Office of BES, U.S. DOE FX This work is supported by GM and by DOE under corporate agreement DE-FC26-04NT42278, by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Transportation Technologies as part of the High Temperature Materials Laboratory User Program at Oak Ridge National Laboratory managed by the UT-Battelle LLC, for the Department of Energy under contract DEAC05000OR22725, and by National Basic Research Program of China (973-program) under Project No. 2007CB607503 and NSFC projects (50825205, 50672118, 50821004, 50820145203, and 10634070). Microscopy research is supported by ORNL's Shared Research Equipment (SHaRE) User Facility, which is sponsored by the Office of BES, U.S. DOE. NR 57 TC 454 Z9 462 U1 71 U2 398 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 25 PY 2011 VL 133 IS 20 BP 7837 EP 7846 DI 10.1021/ja111199y PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA 776ZN UT WOS:000291580400040 PM 21524125 ER PT J AU Liu, QQ Yu, XH Wang, XC Deng, Z Lv, YX Zhu, JL Zhang, SJ Liu, HZ Yang, WG Wang, L Mao, HW Shen, GY Lu, ZY Ren, Y Chen, ZQ Lin, ZJ Zhao, YS Jin, CQ AF Liu, Qingqing Yu, Xiaohui Wang, Xiancheng Deng, Zheng Lv, Yuxi Zhu, Jinlong Zhang, Sijia Liu, Haozhe Yang, Wenge Wang, Lin Mao, Hokwang Shen, Guoyin Lu, Zhong-Yi Ren, Yang Chen, Zhiqiang Lin, Zhijun Zhao, Yusheng Jin, Changqing TI Pressure-Induced Isostructural Phase Transition and Correlation of FeAs Coordination with the Superconducting Properties of 111-Type Na1-xFeAs SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID IRON ARSENIDE SUPERCONDUCTOR; 43 K; T-C; LIFEAS; COMPOUND AB The effect of pressure on the crystalline structure and superconducting transition temperature (T-c) of the 111-type Na1-xFeAs system using in situ high-pressure synchrotron X-ray powder diffraction and diamond anvil cell techniques is studied. A pressure-induced tetragonal to tetragonal isostructural phase transition was found. The systematic evolution of the FeAs4 tetrahedron as a function of pressure based on Rietveld refinements on the powder X-ray diffraction patterns was obtained. The nonmonotonic T-c(P) behavior of Na1-xFeAs is found to correlate with the anomalies of the distance between the anion (As) and the iron layer as well as the bond angle of As-Fe-As for the two tetragonal phases. This behavior provides the key structural information in understanding the origin of the pressure dependence of T-c for 111-type iron pnictide superconductors. A pressure-induced structural phase transition is also observed at 20 GPa. C1 [Liu, Qingqing; Yu, Xiaohui; Wang, Xiancheng; Deng, Zheng; Lv, Yuxi; Zhu, Jinlong; Zhang, Sijia; Jin, Changqing] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Yu, Xiaohui; Lin, Zhijun; Zhao, Yusheng] Los Alamos Natl Lab, Los Alamos Neutron Sci Ctr LANSCE, Los Alamos, NM 87545 USA. [Liu, Haozhe] Harbin Inst Technol, Nat Sci Res Ctr, Harbin 150080, Peoples R China. [Yang, Wenge; Wang, Lin; Shen, Guoyin] Carnegie Inst Sci, HPSynC, Argonne, IL 60439 USA. [Yang, Wenge; Wang, Lin; Shen, Guoyin] Carnegie Inst Sci, HPCAT, Geophys Lab, Argonne, IL 60439 USA. [Mao, Hokwang] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. [Lu, Zhong-Yi] Renmin Univ China, Dept Phys, Beijing 100872, Peoples R China. [Ren, Yang] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Chen, Zhiqiang] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Jin, CQ (reprint author), Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. EM Jin@iphy.ac.cn RI Liu, Haozhe/E-6169-2011; 石, 源/D-5929-2012; 上官, 敏慧/E-8964-2012; ruc, phy/E-4170-2012; Lujan Center, LANL/G-4896-2012; Yang, Wenge/H-2740-2012; chen, zhiqiang/C-9134-2013; WANG, LIN/G-7884-2012; Chen, Zonghai/K-8745-2013; Lin, Zhijun/A-5543-2010 FU National Science Foundation (NSF); Ministry of Science and Technology of China (MOST); U.S. Department of Energy (DOE) [DE-SC0001057]; DOE Office of Basic Energy Sciences; DOE National Nuclear Security Administration FX This work was supported by the National Science Foundation (NSF) and the Ministry of Science and Technology of China (MOST) through research projects. HPSynC is supported as part of EFree, an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE) under Award DE-SC0001057. HPCAT is supported by the DOE Office of Basic Energy Sciences, DOE National Nuclear Security Administration, and NSF. NR 42 TC 31 Z9 32 U1 8 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 25 PY 2011 VL 133 IS 20 BP 7892 EP 7896 DI 10.1021/ja2009949 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 776ZN UT WOS:000291580400046 PM 21528857 ER PT J AU Szigethy, G Raymond, KN AF Szigethy, Geza Raymond, Kenneth N. TI Hexadentate Terephthalamide(bis-hydroxypyridinone) Ligands for Uranyl Chelation: Structural and Thermodynamic Consequences of Ligand Variation SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID STEREOGNOSTIC COORDINATION CHEMISTRY; CATION-CATION COMPLEXES; SEQUESTERING AGENTS; CRYSTAL-STRUCTURE; SCHIFF-BASE; UO22+ COMPLEXES; METAL-COMPLEXES; IRON CHELATORS; ACTINIDES; ION AB Several linear, hexa- and tetradentate ligands incorporating a combination of 2,3-dihydroxy-terephthalamide (TAM) and hydroxypyridinone-amide (HOPO) moieties have been developed as uranyl chelating agents. Crystallographic analysis of several {UO2[TAM(HOPO)(2)]}(2-) complexes revealed a variable and crowded coordination geometry about the uranyl center. The TAM moiety dominates the bonding in hexadenate complexes, with linker rigidity dictating the equality of equatorial U-O bonding. Hexadentate TAM-(HOPO)(2) ligands demonstrated slow binding kinetics with uranyl affinities on average 6 orders of magnitude greater than those of similarly linked bis-HOPO ligands. Study of tetradentate TAM(HOPO) ligands revealed that the high uranyl affinity stems primarily from the presence of the TAM moiety and only marginally from increased ligand denticity. Uranyl affinities of TAM(HOPO)(2) ligands were within experimental error, with TAM-(o-phen-1,2-HOPO)(2) exhibiting the most consistent uranyl affinity at variable pH. C1 [Raymond, Kenneth N.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Lab, Div Chem Sci, Glenn T Seaborg Ctr, Berkeley, CA 94720 USA. RP Raymond, KN (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM raymond@socrates.berkeley.edu FU Office of Science, Office of Basic Energy Sciences; Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231] FX We thank Drs. Rebecca Abergel and Trisha Hoette for assistance with the titration measurements and data treatment. This research is supported by the Director, Office of Science, Office of Basic Energy Sciences, and the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. NR 76 TC 22 Z9 22 U1 6 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 25 PY 2011 VL 133 IS 20 BP 7942 EP 7956 DI 10.1021/ja201511u PG 15 WC Chemistry, Multidisciplinary SC Chemistry GA 776ZN UT WOS:000291580400051 PM 21542587 ER PT J AU Klug, DD Tse, JS Zhao, JY Sturhahn, W Alp, EE Tulk, CA AF Klug, D. D. Tse, J. S. Zhao, J. Y. Sturhahn, W. Alp, E. E. Tulk, C. A. TI Dynamics of Kr in dense clathrate hydrates SO PHYSICAL REVIEW B LA English DT Article ID SYNCHROTRON-RADIATION; THERMAL-CONDUCTIVITY; SCATTERING; NUCLEAR; DEPENDENCE; HYDROGEN; KRYPTON; MOTIONS; XENON AB The dynamics of Kr atoms as guests in dense clathrate hydrate structures are investigated using site specific (83)Kr nuclear resonant inelastic x-ray scattering (NRIXS) spectroscopy in combination with molecular dynamics simulations. The dense structure H hydrate and filled-ice structures are studied at high pressures in a diamond anvil high-pressure cell. The dynamics of Kr in the structure H clathrate hydrate quench recovered at 77 K is also investigated. The Kr phonon density of states obtained from the experimental NRIXS data are compared with molecular dynamics simulations. The temperature and pressure dependence of the phonon spectra provide details of the Kr dynamics in the clathrate hydrate cages. Comparison with the dynamics of Kr atoms in the low-pressure structure II obtained previously was made. The Lamb-Mossbauer factor obtained from NRIXS experiments and molecular dynamics calculations are in excellent agreement and are shown to yield unique information on the strength and temperature dependence of guest-host interactions. C1 [Klug, D. D.] Natl Res Council Canada, Steacie Inst Mol Sci, Ottawa, ON K1A 0R6, Canada. [Tse, J. S.] Univ Saskatchewan, Dept Phys & Engn Phys, Saskatoon, SK S7N 5E2, Canada. [Zhao, J. Y.; Sturhahn, W.; Alp, E. E.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Tulk, C. A.] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. RP Klug, DD (reprint author), Natl Res Council Canada, Steacie Inst Mol Sci, 100 Sussex Dr, Ottawa, ON K1A 0R6, Canada. RI Tulk, Chris/R-6088-2016 OI Tulk, Chris/0000-0003-3400-3878 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX A portion of this Research at Oak Ridge National Laboratory's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 24 TC 4 Z9 4 U1 3 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 25 PY 2011 VL 83 IS 18 AR 184116 DI 10.1103/PhysRevB.83.184116 PG 6 WC Physics, Condensed Matter SC Physics GA 768NP UT WOS:000290942100003 ER PT J AU Miura, M Maiorov, B Baily, SA Haberkorn, N Willis, JO Marken, K Izumi, T Shiohara, Y Civale, L AF Miura, M. Maiorov, B. Baily, S. A. Haberkorn, N. Willis, J. O. Marken, K. Izumi, T. Shiohara, Y. Civale, L. TI Mixed pinning landscape in nanoparticle-introduced YGdBa2Cu3Oy films grown by metal organic deposition SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTORS; IRREVERSIBILITY LINE; COATED CONDUCTORS; CRITICAL CURRENTS; COLUMNAR DEFECTS; FLUX-CREEP; YBA2CU3O7; WIRES; CRYSTALS AB We study the field (H) and temperature (T) dependence of the critical current density (J(c)) and irreversibility field (H-irr) at different field orientations in Y0.77Gd0.23Ba2Cu3Oy with randomly distributed BaZrO3 nanoparticles (YGdBCO + BZO) and YBa2Cu3Oy (YBCO) films. Both MOD films have large RE2Cu2O5 (225) nanoparticles (similar to 80 nm in diameter) and a high density of twin boundaries (TB). In addition, YGdBCO + BZO films have a high density of BZO nanoparticles (similar to 25 nm in diameter). At high temperatures (T > 40 K), the superconducting properties, such as J(c), H-irr, and flux creep rates, are greatly affected by the BZO nanoparticles, while at low temperatures the superconducting properties of both the YBCO and YGdBCO + BZO films show similar field and temperature dependencies. In particular, while the J(c) of YBCO films follow a power-law dependence (proportional to H-alpha) at all measured T, this dependence is only followed at low T for YGdBCO + BZO films. As a function of T, the YGdBCO + BZO film shows J(c) (T, 0.01T) similar to [1 -(T/T-c)(2)](n) with n similar to 1.24 +/- 0.05, which points to "delta T-c pinning." We analyze the role of different types of defects in the different temperature regimes and find that the strong pinning of the BZO nanoparticles yields a higher H-irr and improved J(c) along the c axis and at intermediate orientations at high T. The mixed pinning landscapes due to the presence of disorder of various dimensionalities have an important role in the improvement of in-field properties. C1 [Miura, M.; Maiorov, B.; Baily, S. A.; Haberkorn, N.; Willis, J. O.; Marken, K.; Civale, L.] Los Alamos Natl Lab, Superconduct Technol Ctr, Los Alamos, NM 87545 USA. [Baily, S. A.] Los Alamos Natl Lab, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA. [Izumi, T.; Shiohara, Y.] Int Superconduct Technol Ctr, Superconduct Res Lab, Koto Ku, Tokyo 1350062, Japan. RP Miura, M (reprint author), Los Alamos Natl Lab, Superconduct Technol Ctr, POB 1663, Los Alamos, NM 87545 USA. EM miura38ktgaj@gmail.com OI Maiorov, Boris/0000-0003-1885-0436; Civale, Leonardo/0000-0003-0806-3113 FU Los Alamos National Laboratory; by the US DOE, Office of Basic Energy Sciences (Division of Materials Sciences and Engineering); NHMFL-UCGP; State of Florida; US NSF; NEDO as a Collaborative Research FX We thank T. Kato for assistance with TEM observations. This work was supported by the Laboratory Directed Research and Development program at Los Alamos National Laboratory; by the US DOE, Office of Basic Energy Sciences (Division of Materials Sciences and Engineering); by NHMFL-UCGP, the State of Florida, and by the US NSF. Work at ISTEC-SRL was supported by NEDO as a Collaborative Research. NR 41 TC 55 Z9 55 U1 3 U2 36 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 25 PY 2011 VL 83 IS 18 AR 184519 DI 10.1103/PhysRevB.83.184519 PG 8 WC Physics, Condensed Matter SC Physics GA 768NP UT WOS:000290942100009 ER PT J AU Knorowski, C Burleigh, S Travesset, A AF Knorowski, C. Burleigh, S. Travesset, A. TI Dynamics and Statics of DNA-Programmable Nanoparticle Self-Assembly and Crystallization SO PHYSICAL REVIEW LETTERS LA English DT Article ID COLLOIDS AB DNA linker mediated self-assembly is emerging as a very general strategy for designing new materials. In this Letter, we characterize both the dynamics and thermodynamics of nanoparticle-DNA self-assembly by molecular dynamics simulations from a new coarse-grained model. We establish the general phase diagram and discuss the stability of a previously overlooked crystalline phase (D-bcc). We also characterize universal properties about the dynamics of crystallization. We point out the connection to f-star polymer systems and discuss the implications for ongoing experiments as well as for the general field of DNA mediated self-assembly. C1 [Knorowski, C.; Travesset, A.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Knorowski, C.; Travesset, A.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Burleigh, S.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. RP Knorowski, C (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. FU DOE through the Ames Lab [DE-AC02-07CH11358] FX We acknowledge discussions with J. Anderson, O. Gang, D. Nykypanchuk, and C. Philips. S. B. acknowledges a DOE SULI internship at the Ames Lab. This work is funded by DOE through the Ames Lab under Contract No. DE-AC02-07CH11358. NR 26 TC 59 Z9 60 U1 4 U2 68 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 25 PY 2011 VL 106 IS 21 AR 215501 DI 10.1103/PhysRevLett.106.215501 PG 4 WC Physics, Multidisciplinary SC Physics GA 768MY UT WOS:000290940200009 PM 21699312 ER PT J AU Anderson, I Scheuner, C Goker, M Mavromatis, K Hooper, SD Porat, I Klenk, HP Ivanova, N Kyrpides, N AF Anderson, Iain Scheuner, Carmen Goeker, Markus Mavromatis, Kostas Hooper, Sean D. Porat, Iris Klenk, Hans-Peter Ivanova, Natalia Kyrpides, Nikos TI Novel Insights into the Diversity of Catabolic Metabolism from Ten Haloarchaeal Genomes SO PLOS ONE LA English DT Article ID ENTNER-DOUDOROFF PATHWAY; EXTREMELY HALOPHILIC ARCHAEA; UNIVERSAL STRESS-PROTEIN; SP-NOV; HALOQUADRATUM-WALSBYI; HALORHABDUS-UTAHENSIS; HALOFERAX-VOLCANII; GEN. NOV.; DEAD-SEA; HALOARCULA-MARISMORTUI AB Background: The extremely halophilic archaea are present worldwide in saline environments and have important biotechnological applications. Ten complete genomes of haloarchaea are now available, providing an opportunity for comparative analysis. Methodology/Principal Findings: We report here the comparative analysis of five newly sequenced haloarchaeal genomes with five previously published ones. Whole genome trees based on protein sequences provide strong support for deep relationships between the ten organisms. Using a soft clustering approach, we identified 887 protein clusters present in all halophiles. Of these core clusters, 112 are not found in any other archaea and therefore constitute the haloarchaeal signature. Four of the halophiles were isolated from water, and four were isolated from soil or sediment. Although there are few habitat-specific clusters, the soil/sediment halophiles tend to have greater capacity for polysaccharide degradation, siderophore synthesis, and cell wall modification. Halorhabdus utahensis and Haloterrigena turkmenica encode over forty glycosyl hydrolases each, and may be capable of breaking down naturally occurring complex carbohydrates. H. utahensis is specialized for growth on carbohydrates and has few amino acid degradation pathways. It uses the non-oxidative pentose phosphate pathway instead of the oxidative pathway, giving it more flexibility in the metabolism of pentoses. Conclusions: These new genomes expand our understanding of haloarchaeal catabolic pathways, providing a basis for further experimental analysis, especially with regard to carbohydrate metabolism. Halophilic glycosyl hydrolases for use in biofuel production are more likely to be found in halophiles isolated from soil or sediment. C1 [Anderson, Iain; Mavromatis, Kostas; Hooper, Sean D.; Ivanova, Natalia; Kyrpides, Nikos] US DOE, Genome Biol Program, Joint Genome Inst, Walnut Creek, CA USA. [Scheuner, Carmen; Goeker, Markus; Klenk, Hans-Peter] Deutsch Sammlung Mikroorganismen & Zellkulturen, D-3300 Braunschweig, Germany. [Porat, Iris] INEOS Bio, Fayetteville, AR USA. RP Anderson, I (reprint author), US DOE, Genome Biol Program, Joint Genome Inst, Walnut Creek, CA USA. EM IJAnderson@lbl.gov RI Kyrpides, Nikos/A-6305-2014 OI Kyrpides, Nikos/0000-0002-6131-0462 FU Office of Science of the United States Department of Energy [DE-AC02-05CH112] FX This work was supported by the Office of Science of the United States Department of Energy (http://www.er.doe.gov/) under Contract No. DE-AC02-05CH112. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 90 TC 35 Z9 35 U1 2 U2 29 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 25 PY 2011 VL 6 IS 5 AR e20237 DI 10.1371/journal.pone.0020237 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 769IQ UT WOS:000291006500046 PM 21633497 ER PT J AU Voolstra, CR Sunagawa, S Matz, MV Bayer, T Aranda, M Buschiazzo, E DeSalvo, MK Lindquist, E Szmant, AM Coffroth, MA Medina, M AF Voolstra, Christian R. Sunagawa, Shinichi Matz, Mikhail V. Bayer, Till Aranda, Manuel Buschiazzo, Emmanuel DeSalvo, Michael K. Lindquist, Erika Szmant, Alina M. Coffroth, Mary Alice Medina, Monica TI Rapid Evolution of Coral Proteins Responsible for Interaction with the Environment SO PLOS ONE LA English DT Article ID ANEMONE AIPTASIA-PALLIDA; SYMBIOTIC SEA-ANEMONE; REEF-BUILDING CORALS; GENE-EXPRESSION; MONTASTRAEA-FAVEOLATA; DINOFLAGELLATE MUTUALISM; NUCLEOTIDE SUBSTITUTION; FLUORESCENT PROTEINS; POSITIVE SELECTION; ACROPORA-PALMATA AB Background: Corals worldwide are in decline due to climate change effects (e. g., rising seawater temperatures), pollution, and exploitation. The ability of corals to cope with these stressors in the long run depends on the evolvability of the underlying genetic networks and proteins, which remain largely unknown. A genome-wide scan for positively selected genes between related coral species can help to narrow down the search space considerably. Methodology/Principal Findings: We screened a set of 2,604 putative orthologs from EST-based sequence datasets of the coral species Acropora millepora and Acropora palmata to determine the fraction and identity of proteins that may experience adaptive evolution. 7% of the orthologs show elevated rates of evolution. Taxonomically-restricted (i.e. lineage-specific) genes show a positive selection signature more frequently than genes that are found across many animal phyla. The class of proteins that displayed elevated evolutionary rates was significantly enriched for proteins involved in immunity and defense, reproduction, and sensory perception. We also found elevated rates of evolution in several other functional groups such as management of membrane vesicles, transmembrane transport of ions and organic molecules, cell adhesion, and oxidative stress response. Proteins in these processes might be related to the endosymbiotic relationship corals maintain with dinoflagellates in the genus Symbiodinium. Conclusion/Relevance: This study provides a birds-eye view of the processes potentially underlying coral adaptation, which will serve as a foundation for future work to elucidate the rates, patterns, and mechanisms of corals' evolutionary response to global climate change. C1 [Voolstra, Christian R.; Bayer, Till; Aranda, Manuel] King Abdullah Univ Sci & Technol, Red Sea Res Ctr, Thuwal, Saudi Arabia. [Sunagawa, Shinichi] European Mol Biol Lab, Heidelberg, Germany. [Matz, Mikhail V.] Univ Texas Austin, Sch Biol Sci, Sect Integrat Biol, Austin, TX 78712 USA. [Buschiazzo, Emmanuel; Medina, Monica] Univ Calif Merced, Sch Nat Sci, Merced, CA USA. [DeSalvo, Michael K.] Univ Calif San Francisco, Dept Anesthesia, UCSF Sch Med, San Francisco, CA 94143 USA. [Lindquist, Erika] Joint Genome Inst, Dept Energy, Walnut Creek, CA USA. [Szmant, Alina M.] Univ N Carolina, Ctr Marine Sci, Wilmington, NC 28401 USA. [Coffroth, Mary Alice] SUNY Buffalo, Grad Program Evolut Ecol & Behav, Buffalo, NY 14260 USA. [Coffroth, Mary Alice] SUNY Buffalo, Dept Geol, Buffalo, NY 14260 USA. RP Voolstra, CR (reprint author), King Abdullah Univ Sci & Technol, Red Sea Res Ctr, Thuwal, Saudi Arabia. EM christian.voolstra@kaust.edu.sa; mmedina@ucmerced.edu RI Aranda Lastra, Manuel/D-9530-2011; Sunagawa, Shinichi/D-9715-2011; Buschiazzo, Emmanuel/B-5126-2011; Voolstra, Christian/H-7158-2014; Bayer, Till/H-6826-2016; OI Aranda Lastra, Manuel/0000-0001-6673-016X; Sunagawa, Shinichi/0000-0003-3065-0314; Voolstra, Christian/0000-0003-4555-3795; Bayer, Till/0000-0002-4704-2449; Matz, Mikhail/0000-0001-5453-9819 FU National Science Foundation [IOS-0644438, OCE-0313708]; Collaborative Travel Fund; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; [DEB-1054766] FX This work was supported by DEB-1054766 to M. V. M. and National Science Foundation grants IOS-0644438 and OCE-0313708 to M. M., and by a Collaborative Travel Fund to C. R. V. made by King Abdullah University of Science and Technology (KAUST). The work conducted by the U.S. Department of Energy Joint Genome Institute is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 79 TC 28 Z9 28 U1 3 U2 43 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 185 BERRY ST, STE 1300, SAN FRANCISCO, CA 94107 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 25 PY 2011 VL 6 IS 5 AR e20392 DI 10.1371/journal.pone.0020392 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 769IQ UT WOS:000291006500059 PM 21633702 ER PT J AU Volkow, ND Tomasi, D Vaska, P AF Volkow, Nora D. Tomasi, Dardo Vaska, Paul TI Cell Phone Activation and Brain Glucose Metabolism Reply SO JAMA-JOURNAL OF THE AMERICAN MEDICAL ASSOCIATION LA English DT Letter C1 [Volkow, Nora D.] NIDA, Bethesda, MD 20892 USA. [Tomasi, Dardo] NIAAA, Bethesda, MD USA. [Vaska, Paul] Brookhaven Natl Lab, Dept Med, Upton, NY 11973 USA. RP Volkow, ND (reprint author), NIDA, Bethesda, MD 20892 USA. EM nvolkow@nida.nih.gov RI Tomasi, Dardo/J-2127-2015 NR 3 TC 0 Z9 0 U1 0 U2 1 PU AMER MEDICAL ASSOC PI CHICAGO PA 330 N WABASH AVE, STE 39300, CHICAGO, IL 60611-5885 USA SN 0098-7484 EI 1538-3598 J9 JAMA-J AM MED ASSOC JI JAMA-J. Am. Med. Assoc. PD MAY 25 PY 2011 VL 305 IS 20 BP 2067 EP 2068 DI 10.1001/jama.2011.672 PG 2 WC Medicine, General & Internal SC General & Internal Medicine GA 768AC UT WOS:000290901700014 ER PT J AU Song, HC Bass, SA Heinz, U Hirano, T Shen, C AF Song, Huichao Bass, Steffen A. Heinz, Ulrich Hirano, Tetsufumi Shen, Chun TI Hadron spectra and elliptic flow for 200 A GeV Au plus Au collisions from viscous hydrodynamics coupled to a Boltzmann cascade SO PHYSICAL REVIEW C LA English DT Article ID ECCENTRICITY FLUCTUATIONS; NUCLEAR COLLISIONS AB It is shown that the recently developed hybrid code VISHNU, which couples a relativistic viscous fluid dynamical description of the quark-gluon plasma (QGP) with a microscopic Boltzmann cascade for the late hadronic rescattering stage, yields an excellent description of charged and identified hadron spectra and elliptic flow measured in 200 A GeV Au + Au collisions at the Relativistic Heavy-Ion Collider (RHIC). Using initial conditions that incorporate event-by-event fluctuations in the initial shape and orientation of the collision fireball and values eta/s for the specific shear viscosity of the quark-gluon plasma that were recently extracted from the measured centrality dependence of the eccentricity-scaled, p(T)-integrated charged hadron elliptic flow v(2,ch)/epsilon, we obtain universally good agreement between theory and experiment for the p(T) spectra and differential elliptic flow v(2)(p(T)) for both pions and protons at all collision centralities. C1 [Song, Huichao; Hirano, Tetsufumi] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Bass, Steffen A.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Heinz, Ulrich; Shen, Chun] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Hirano, Tetsufumi] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. RP Song, HC (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. FU US Department of Energy [DE-AC02-05CH11231, DE-FG02-05ER41367, DE-SC0004286, DE-SC0004104]; Japan Society for the Promotion of Science [22740151, 213383] FX We gratefully acknowledge fruitful discussions with P. Huovinen, H. Masui, A. Poskanzer, S. Voloshin, and A. Tang. We specifically thank A. Poskanzer for computing for us the a values listed in Table I and R. Snellings for providing some of the data shown in Fig. 6. This work was supported by the US Department of Energy under Grants No. DE-AC02-05CH11231, No. DE-FG02-05ER41367, No. DE-SC0004286, and (within the framework of the JET Collaboration) No. DE-SC0004104. T. H. acknowledges support through Grant-in-Aid for Scientific Research No. 22740151 and through the Excellent Young Researchers Oversea Visit Program (No. 213383) of the Japan Society for the Promotion of Science. We gratefully acknowledge extensive computing resources provided to us by the Ohio Supercomputer Center. NR 51 TC 77 Z9 77 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 J9 PHYS REV C JI Phys. Rev. C PD MAY 25 PY 2011 VL 83 IS 5 AR 054910 DI 10.1103/PhysRevC.83.054910 PG 12 WC Physics, Nuclear SC Physics GA 768OM UT WOS:000290944500001 ER PT J AU Musch, BU Hagler, P Negele, JW Schafer, A AF Musch, B. U. Haegler, Ph. Negele, J. W. Schaefer, A. TI Exploring quark transverse momentum distributions with lattice QCD SO PHYSICAL REVIEW D LA English DT Article ID GENERALIZED PARTON DISTRIBUTIONS; FINAL-STATE INTERACTIONS; DEEP-INELASTIC SCATTERING; GAUGE-THEORY; DRELL-YAN; FRAGMENTATION FUNCTIONS; SPIN ASYMMETRIES; HADRON STRUCTURE; PHASE-FACTORS; SINGLE-SPIN AB We discuss in detail a method to study transverse momentum dependent parton distribution functions (TMDs) using lattice QCD. To develop the formalism and to obtain first numerical results, we directly implement a bilocal quark-quark operator connected by a straight Wilson line, allowing us to study T-even, "process-independent'' TMDs. Beyond results for x-integrated TMDs and quark densities, we present a study of correlations in x and k(perpendicular to). Our calculations are based on domain wall valence quark propagators by the LHP Collaboration calculated on top of gauge configurations provided by the MILC Collaboration with N-f = 2 + 1 asqtad-improved staggered sea quarks. C1 [Musch, B. U.] Jefferson Lab, Ctr Theory, Newport News, VA 23606 USA. [Haegler, Ph.] Tech Univ Munich, Inst Theoret Phys T39, Dept Phys, D-85747 Garching, Germany. [Haegler, Ph.; Schaefer, A.] Univ Regensburg, Inst Theoret Phys, D-93040 Regensburg, Germany. [Negele, J. W.] MIT, Ctr Theoret Phys, Cambridge, MA 02139 USA. RP Musch, BU (reprint author), Jefferson Lab, Ctr Theory, Newport News, VA 23606 USA. EM bmusch@jlab.org; phaegler@ph.tum.de NR 107 TC 49 Z9 49 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 25 PY 2011 VL 83 IS 9 AR 094507 DI 10.1103/PhysRevD.83.094507 PG 37 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 768OR UT WOS:000290945000001 ER PT J AU Berry, JW Hendrickson, B LaViolette, RA Phillips, CA AF Berry, Jonathan W. Hendrickson, Bruce LaViolette, Randall A. Phillips, Cynthia A. TI Tolerating the community detection resolution limit with edge weighting SO PHYSICAL REVIEW E LA English DT Article ID NETWORKS AB Communities of vertices within a giant network such as the World Wide Web are likely to be vastly smaller than the network itself. However, Fortunato and Barthelemy have proved that modularity maximization algorithms for community detection may fail to resolve communities with fewer than root L/2 edges, where L is the number of edges in the entire network. This resolution limit leads modularity maximization algorithms to have notoriously poor accuracy on many real networks. Fortunato and Barthelemy's argument can be extended to networks with weighted edges as well, and we derive this corollary argument. We conclude that weighted modularity algorithms may fail to resolve communities with less than root W is an element of/2 total edge weight, where W is the total edge weight in the network and is an element of is the maximum weight of an intercommunity edge. If is an element of is small, then small communities can be resolved. Given a weighted or unweighted network, we describe how to derive new edge weights in order to achieve a low is an element of, we modify the Clauset, Newman, and Moore (CNM) community detection algorithm to maximize weighted modularity, and we show that the resulting algorithm has greatly improved accuracy. In experiments with an emerging community standard benchmark, we find that our simple CNM variant is competitive with the most accurate community detection methods yet proposed. C1 [Berry, Jonathan W.; Hendrickson, Bruce; LaViolette, Randall A.; Phillips, Cynthia A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Berry, JW (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM jberry@sandia.gov; bahendr@sandia.gov; randall.laviolette@science.doe.gov; caphill@sandia.gov FU Laboratory Directed Research and Development program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We thank Santo Fortunato (ISI), Joseph McCloskey (DoD), Cris Moore (UNM), Tamara Kolda (Sandia), Dan Nordman (Iowa State), and Alyson Wilson (Iowa State) for helpful discussions and comments. This work was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 30 TC 42 Z9 43 U1 0 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD MAY 25 PY 2011 VL 83 IS 5 AR 056119 DI 10.1103/PhysRevE.83.056119 PN 2 PG 9 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 768PH UT WOS:000290946900001 PM 21728617 ER PT J AU Webb, S Wang, G Litvinenko, V AF Webb, Stephen Wang, Gang Litvinenko, Vladimir TI Three-dimensional model of small signal free-electron lasers SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID GAIN AB Coherent electron cooling is an ultrahigh-bandwidth form of stochastic cooling which utilizes the charge perturbation from Debye screening as a seed for a free-electron laser. The amplified and frequency-modulated signal that results from the free-electron laser process is then used to give an energy-dependent kick on the hadrons in a bunch. In this paper, we present a theoretical description of a high-gain free-electron laser with applications to a complete theoretical description of coherent electron cooling. C1 [Webb, Stephen] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Webb, Stephen; Wang, Gang; Litvinenko, Vladimir] Brookhaven Natl Lab, Collider Accelerator Dept, Upton, NY 11973 USA. RP Webb, S (reprint author), SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. EM swebb@grad.physics.sunysb.edu; gawang@bnl.gov; vl@bnl.gov FU Brookhaven Science Associates, LLC, U.S. Department of Energy [DE-AC02-98CH10886] FX The authors would like to thank Michael Blaskiewicz and Evgeny Saldin for helpful discussion. This work was supported by Brookhaven Science Associates, LLC under Contract No. DE-AC02-98CH10886 with the U.S. Department of Energy. NR 18 TC 4 Z9 4 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD MAY 25 PY 2011 VL 14 IS 5 AR 051003 DI 10.1103/PhysRevSTAB.14.051003 PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 768PK UT WOS:000290947200001 ER PT J AU Hou, C Xiong, YJ Fu, N Jacquot, CC Squier, TC Cao, HS AF Hou, Chen Xiong, Yijia Fu, Na Jacquot, Caitlin C. Squier, Thomas C. Cao, Haishi TI Turn-on ratiometric fluorescent sensor for Pb2+ detection SO TETRAHEDRON LETTERS LA English DT Article DE Pb2+; Sensor; Pyrene ID EXCIMER FORMATION; IONS; PB(II); LEAD; CHEMOSENSORS; DERIVATIVES; PYRENE; SENSITIVITY; SELECTIVITY; PROBES AB We report a ratiometric lead fluorescent sensor (LFS-1) with high affinity to Pb2+ that shows considerable selectivity over 12 other physiological related metal cations in aqueous media. Binding induces excimer formation, providing a highly sensitive ratiometric measure of lead concentrations. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Hou, Chen; Jacquot, Caitlin C.; Cao, Haishi] Univ Nebraska, Dept Chem, Kearney, NE 68849 USA. [Xiong, Yijia; Fu, Na; Squier, Thomas C.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99354 USA. RP Cao, HS (reprint author), Univ Nebraska, Dept Chem, Kearney, NE 68849 USA. EM caoh1@unk.edu RI Fu, Na/C-8662-2011; Xiong, Yijia/C-1341-2011 FU University Research and Creative Activity in the University of Nebraska at Kearney FX This research is supported by Mini-Grant, Undergraduate Research Fellows Program, and University Research and Creative Activity in the University of Nebraska at Kearney. Authors would also like to acknowledge Sara Basiaga in University of Nebraska at Lincoln for her assistance in collecting fluorescence spectra. NR 46 TC 12 Z9 12 U1 3 U2 30 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0040-4039 J9 TETRAHEDRON LETT JI Tetrahedron Lett. PD MAY 25 PY 2011 VL 52 IS 21 BP 2692 EP 2696 DI 10.1016/j.tetlet.2011.03.075 PG 5 WC Chemistry, Organic SC Chemistry GA 764AZ UT WOS:000290602100020 ER PT J AU Huang, GY Wirth, BD AF Huang, Gui-Yang Wirth, Brian D. TI First-principles study of diffusion of interstitial and vacancy in alpha U-Zr SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID AUGMENTED-WAVE METHOD; GAS BUBBLES; URANIUM; METALS; ALLOYS; STRESS; SYSTEM; PHASE AB Metallic uranium-zirconium alloys are of interest for a variety of fast reactor designs, and there is substantial experience with the behavior of metallic fuels. Yet, there remain a number of questions regarding the mechanisms controlling fission-gas-driven swelling in these alloys. Here we present results of ab initio calculations of the diffusion behavior of interstitial and vacancy point defects in alpha U-Zr alloys. The formation energy and migration barrier of vacancy and interstitial defects, and the influence of Zr on these values, is obtained and compared with experimental results. Our results confirm that self-diffusion in pure alpha U is via a simple vacancy mechanism, and shows anisotropic character. The calculated values of activation energy are consistent with the experimental results in the literature. For interstitial diffusion, the kick-out mechanism was found to have the smallest energy barrier. The calculations of point defects, and later Xe, in U-Zr alloys will provide a foundation for computational modeling of fission gas bubble nucleation and growth. C1 [Huang, Gui-Yang; Wirth, Brian D.] Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA. [Wirth, Brian D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Huang, GY (reprint author), Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA. EM huangguiyang@gmail.com; bdwirth@utk.edu RI Huang, Guiyang/E-7746-2012; Wirth, Brian/O-4878-2015 OI Huang, Guiyang/0000-0003-0144-7376; Wirth, Brian/0000-0002-0395-0285 FU US Department of Energy, Office of Nuclear Energy through Nuclear Energy University [00091204, CFDA 81.049] FX This research has been funded by the US Department of Energy, Office of Nuclear Energy through the Nuclear Energy University Program, administered by Battelle Energy Alliance, LLC, subcontract no. 00091204, CFDA#81.049. NR 43 TC 13 Z9 13 U1 5 U2 18 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAY 25 PY 2011 VL 23 IS 20 AR 205402 DI 10.1088/0953-8984/23/20/205402 PG 9 WC Physics, Condensed Matter SC Physics GA 759AQ UT WOS:000290212300011 PM 21540501 ER PT J AU Spencer, EC Ross, NL Parker, SF Woodfield, BF Boerio-Goates, J Smith, SJ Olsen, RE Kolesnikov, AI Navrotsky, A Ma, C AF Spencer, E. C. Ross, N. L. Parker, S. F. Woodfield, B. F. Boerio-Goates, J. Smith, S. J. Olsen, R. E. Kolesnikov, A. I. Navrotsky, A. Ma, C. TI Determination of the magnetic contribution to the heat capacity of cobalt oxide nanoparticles and the thermodynamic properties of the hydration layers SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID INELASTIC NEUTRON-SCATTERING; COO NANOPARTICLES; METAL-OXIDES; TRANSITION; CO3O4; WATER; OXIDATION; EXCITATIONS; ICE AB We present low temperature (11 K) inelastic neutron scattering (INS) data on four hydrated nanoparticle systems: 10 nm CoO center dot 0.10H(2)O (1), 16 nmCo(3)O(4)center dot 0.40H(2)O (2), 25 nm Co3O4 center dot 0.30H(2)O (3) and 40 nmCo(3)O4 center dot 0.026H(2)O (4). The vibrational densities of states were obtained for all samples and from these the isochoric heat capacity and vibrational energy for the hydration layers confined to the surfaces of these nanoparticle systems have been elucidated. The results show that water on the surface of CoO nanoparticles is more tightly bound than water confined to the surface of Co3O4, and this is reflected in the reduced heat capacity and vibrational entropy for water on CoO relative to water on Co3O4 nanoparticles. This supports the trend, seen previously, for water to be more tightly bound in materials with higher surface energies. The INS spectra for the antiferromagnetic Co3O4 particles (2-4) also show sharp and intense magnetic excitation peaks at 5 meV, and from this the magnetic contribution to the heat capacity of Co3O4 nanoparticles has been calculated; this represents the first example of use of INS data for determining the magnetic contribution to the heat capacity of any magnetic nanoparticle system. C1 [Spencer, E. C.; Ross, N. L.] Virginia Tech, Dept Geosci, Blacksburg, VA 24061 USA. [Parker, S. F.] STFC Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Woodfield, B. F.; Boerio-Goates, J.; Smith, S. J.; Olsen, R. E.] Brigham Young Univ, Dept Chem & Biochem, Provo, UT 84602 USA. [Kolesnikov, A. I.] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. [Navrotsky, A.; Ma, C.] Univ Calif Davis, Peter A Rock Thermochem Lab, Davis, CA 95616 USA. [Navrotsky, A.; Ma, C.] Univ Calif Davis, NEAT ORU, Davis, CA 95616 USA. RP Ross, NL (reprint author), Virginia Tech, Dept Geosci, Blacksburg, VA 24061 USA. RI davidson, anne/A-5160-2012; Kolesnikov, Alexander/I-9015-2012; OI Kolesnikov, Alexander/0000-0003-1940-4649; Parker, Stewart/0000-0002-3228-2570 FU US Department of Energy, Office of Basic Energy Sciences (DOE-BES) [DE FG03 01ER15237]; DOE [DE-AC05-00OR22725] FX N L Ross, E C Spencer, and A Navrotsky acknowledge support from the US Department of Energy, Office of Basic Energy Sciences (DOE-BES), grant DE FG03 01ER15237. A I Kolesnikov wishes to acknowledge ORNL/SNS at Oak Ridge National Laboratory that is managed by UT-Battelle, LLC, for DOE under contract DE-AC05-00OR22725. The STFC Rutherford Appleton Laboratory is thanked for access to neutron beam facilities. NR 33 TC 7 Z9 7 U1 1 U2 29 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAY 25 PY 2011 VL 23 IS 20 AR 205303 DI 10.1088/0953-8984/23/20/205303 PG 6 WC Physics, Condensed Matter SC Physics GA 759AQ UT WOS:000290212300007 PM 21540512 ER PT J AU Zhang, J Lu, WC Zang, QJ Zhao, LZ Wang, CZ Ho, KM AF Zhang, Jing Lu, Wen-Cai Zang, Qing-Jun Zhao, Li-Zhen Wang, C. Z. Ho, K. M. TI An ab initio calculation study of silicon and carbon binary clusters C7Sin (n=1-7) SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID MOLECULAR-ORBITAL CALCULATIONS; STABILITY; SPECTRA; FRAGMENTATION; ENERGETICS; SI AB Binary C7Sin (n = 1-7) clusters are studied using density functional calculations at the level of B3LYP/6-311G(d). Lowest-energy structures have been determined theoretically and their properties such as binding energies, second differences in energy and highest-occupied and lowest-unoccupied molecular orbital gaps have been analyzed. It is found that the lowest-energy structures of the C7Sin (n = 1-7) clusters change from linear to planar when n >= 3, and in the planar structures C atoms prefer to form five-and six-membered rings surrounded by extra Si atoms in the form of the C2Si units. C1 [Zhang, Jing; Lu, Wen-Cai] Jilin Univ, Inst Theoret Chem, State Key Lab Theoret & Computat Chem, Changchun 130021, Jilin, Peoples R China. [Lu, Wen-Cai; Zang, Qing-Jun; Zhao, Li-Zhen] Qingdao Univ, Growing Base State Key Lab, Lab Fiber Mat & Modern Text, Qingdao 266071, Shandong, Peoples R China. [Lu, Wen-Cai; Zang, Qing-Jun; Zhao, Li-Zhen] Qingdao Univ, Growing Base State Key Lab, Coll Phys, Qingdao 266071, Shandong, Peoples R China. [Wang, C. Z.; Ho, K. M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Wang, C. Z.; Ho, K. M.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. RP Lu, WC (reprint author), Jilin Univ, Inst Theoret Chem, State Key Lab Theoret & Computat Chem, Changchun 130021, Jilin, Peoples R China. EM wencailu@jlu.edu.cn FU National Natural Science Foundation of China [20773047, 21043001]; US Department of Energy by Iowa State University [DE-AC02-07CH11358] FX This work was supported by the National Natural Science Foundation of China under grant nos. 20773047 and 21043001. Ames Laboratory is operated for the US Department of Energy by Iowa State University under contract no. DE-AC02-07CH11358. This work was also supported by the Director for Energy Research, Office of Basic Energy Sciences including a grant of computer time at the National Energy Research Supercomputing Center (NERSC) in Berkeley. NR 28 TC 2 Z9 2 U1 1 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAY 25 PY 2011 VL 23 IS 20 AR 205305 DI 10.1088/0953-8984/23/20/205305 PG 7 WC Physics, Condensed Matter SC Physics GA 759AQ UT WOS:000290212300009 PM 21540510 ER PT J AU Ku, SY Liman, CD Cochran, JE Toney, MF Chabinyc, ML Hawker, CJ AF Ku, Sung-Yu Liman, Christopher D. Cochran, Justin E. Toney, Michael F. Chabinyc, Michael L. Hawker, Craig J. TI Solution-Processed Nanostructured Benzoporphyrin with Polycarbonate Binder for Photovoltaics SO ADVANCED MATERIALS LA English DT Article ID ORGANIC SOLAR-CELLS; CARBON-DIOXIDE; EFFICIENT; POLYMERS; FILMS AB A new method to aid large-area solution processing of organic small molecule semiconductors is reported. A thermally degradable poly(propylene carbonate) (PC) binder is added to a solution of soluble precursor to a tetrabenzoporphyrin to increase its viscosity, allowing for the use of large-area methods such as inkjet printing, slot coating, or blade coating. This method is used to make bulk heterojunction solar cells with a p-i-n type structure. C1 [Ku, Sung-Yu; Liman, Christopher D.; Chabinyc, Michael L.; Hawker, Craig J.] Univ Calif Santa Barbara, Mat Res Lab, Dept Mat, Mitsubishi Chem Ctr Adv Mat, Santa Barbara, CA 93106 USA. [Cochran, Justin E.] Univ Calif Santa Barbara, Dept Chem & Biochem, Santa Barbara, CA 93106 USA. [Toney, Michael F.] Stanford Synchrotron Radiat Lab, Stanford, CA 94305 USA. RP Chabinyc, ML (reprint author), Univ Calif Santa Barbara, Mat Res Lab, Dept Mat, Mitsubishi Chem Ctr Adv Mat, Santa Barbara, CA 93106 USA. EM mchabinyc@engineering.ucsb.edu; hawker@mrl.ucsb.edu RI Chabinyc, Michael/E-2387-2011; Hawker, Craig/G-4971-2011 OI Hawker, Craig/0000-0001-9951-851X FU NSF [CHE-1035292]; Mitsubsihi Chemicals Center for Advanced Materials; UCSB MRSEC under NSF [DMR05-20415] FX We thank M. Guide, N. Treat, M. Burkhardt, J. Heo, and M. Dimitriou for their insights, N. Eisenmenger and C. Shuttle for assistance with OPV testing, and Eric Verploegen for assistance with the in-situ annealing. We thank the Mitsubishi Chemical Group Science and Technology Research Center, Inc. for sharing their insights and provision of CP and analytical data. Software for analyzing GIWAXS data was written by Stefan Mannsfeld (SSRL) and R. Joseph Kline (NIST). Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a national user facility operated by Stanford University on behalf of the U. S. Department of Energy, Office of Basic Energy Sciences. This work was supported by the NSF SOLAR program (CHE-1035292), Mitsubsihi Chemicals Center for Advanced Materials and the UCSB MRSEC Program under NSF award DMR05-20415. This article is part of the Special Issue on Materials Research at the University of California, Santa Barbara. NR 24 TC 25 Z9 25 U1 3 U2 43 PU WILEY-BLACKWELL PI MALDEN PA COMMERCE PLACE, 350 MAIN ST, MALDEN 02148, MA USA SN 0935-9648 J9 ADV MATER JI Adv. Mater. PD MAY 24 PY 2011 VL 23 IS 20 SI SI BP 2289 EP + DI 10.1002/adma.201100028 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 776OZ UT WOS:000291547600006 PM 21520461 ER PT J AU Feldman, DR Algieri, CA Ong, JR Collins, WD AF Feldman, Daniel R. Algieri, Chris A. Ong, Jonathan R. Collins, William D. TI CLARREO shortwave observing system simulation experiments of the twenty-first century: Simulator design and implementation SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID GENERAL-CIRCULATION MODELS; CLIMATE SYSTEM; RADIATIVE-TRANSFER; BIDIRECTIONAL REFLECTANCE; ATMOSPHERIC CORRECTION; FEEDBACK PROCESSES; OPTICAL-PROPERTIES; VERSION-3 CCSM3; SURFACE ALBEDO; CLOUD FEEDBACK AB Projected changes in the Earth system will likely be manifested in changes in reflected solar radiation. This paper introduces an operational Observational System Simulation Experiment (OSSE) to calculate the signals of future climate forcings and feedbacks in top-of-atmosphere reflectance spectra. The OSSE combines simulations from the Intergovernmental Panel on Climate Change (IPCC) Fourth Assessment Report for the NCAR Community Climate System Model (CCSM) with the MODTRAN radiative transfer code to calculate reflectance spectra for simulations of current and future climatic conditions over the 21st century. The OSSE produces narrowband reflectances and broadband fluxes, the latter of which have been extensively validated against archived CCSM results. The shortwave reflectance spectra contain atmospheric features including signals from water vapor, liquid and ice clouds, and aerosols. The spectra are also strongly influenced by the surface bidirectional reflectance properties of predicted snow and sea ice and the climatological seasonal cycles of vegetation. By comparing and contrasting simulated reflectance spectra based on emissions scenarios with increasing projected and fixed present-day greenhouse gas and aerosol concentrations, we find that prescribed forcings from increases in anthropogenic sulfate and carbonaceous aerosols are detectable and are spatially confined to lower latitudes. Also, changes in the intertropical convergence zone and poleward shifts in the subsidence zones and the storm tracks are all detectable along with large changes in snow cover and sea ice fraction. These findings suggest that the proposed NASA Climate Absolute Radiance and Refractivity Observatory (CLARREO) mission to measure shortwave reflectance spectra may help elucidate climate forcings, responses, and feedbacks. C1 [Feldman, Daniel R.; Collins, William D.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Algieri, Chris A.; Collins, William D.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Earth Sci, Climate Sci Dept, Berkeley, CA 94720 USA. [Ong, Jonathan R.] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. RP Feldman, DR (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, 307 McCone Hall,MC 4767, Berkeley, CA 94720 USA. EM daniel_r_feldman@berkeley.edu RI Feldman, Daniel/N-8703-2013; Collins, William/J-3147-2014; Richards, Amber/K-8203-2015 OI Feldman, Daniel/0000-0003-3365-5233; Collins, William/0000-0002-4463-9848; FU NASA [NNX08AT80G, NAS2-03144, NNX10AK27G, SMD-08-0999, SMD-09-1397, SMD-10-1799]; Contractor Supporting Research (CSR); Office of Science, of the U.S. Department of Energy [DE-AC02-05CH11231] FX Funding for this research was supported by the following NASA grants: NNX08AT80G, NAS2-03144, and NNX10AK27G. This work was also supported by Contractor Supporting Research (CSR) funding from Berkeley Laboratory, provided by the Director, Office of Science, of the U.S. Department of Energy under contract DE-AC02-05CH11231. Additionally, NASA High-End Computing grants SMD-08-0999, SMD-09-1397, and SMD-10-1799 provided computational resources produce the simulations. The following individuals also provided considerable assistance with this research: Don Anderson of NASA Headquarters; Tsengdar Lee of the NASA Science Mission Directorate; Gail Anderson of AFRL; Vincent Ross of Aerex Corp.; Lex Berk of Spectral Sciences, Inc.; David Young, Bruce Wielicki, Zhonghai Jin, and Rosemary Baize of NASA Langley Research Center; Crystal Schaaf and Zhousen Wang of Boston University; and the entire NASA High-End Computing technical support team of NASA User Services. We also wish to thank the three reviewers for their insightful comments and suggestions. NR 66 TC 14 Z9 14 U1 2 U2 12 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAY 24 PY 2011 VL 116 AR D10107 DI 10.1029/2010JD015350 PG 15 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 770PW UT WOS:000291102000005 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hammer, J Hansel, S Hoch, M Hormann, N Hrubec, J Jeitler, M Kasieczka, G Kiesenhofer, W Krammer, M Liko, D Mikulec, I Pernicka, M Rohringer, H Schofbeck, R Strauss, J Teischinger, F Wagner, P Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Benucci, L De Wolf, EA Janssen, X Maes, T Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Blekman, F Blyweert, S D'Hondt, J Devroede, O Suarez, RG Kalogeropoulos, A Maes, J Maes, M Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Charaf, O Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hammad, GH Hreus, T Marage, E Thomas, L Velde, CV Vanlaer, P Adler, V Cimmino, A Costantini, S Grunewald, M Klein, B Lellouch, J Marinov, A Mccartin, J Ryckbosch, D Thyssen, F Tytgat, M Vanelderen, L Verwilligen, P Walsh, S Zaganidis, N Basegmez, S Bruno, G Caudron, J Ceard, L Gil, EC De Jeneret, JD Delaere, C Favart, D Giammanco, A Gregoire, G Hollar, J Lemaitre, V Liao, J Militaru, O Ovyn, S Pagano, D Pin, A Piotrzkowski, K Schul, N Beliy, N Caebergs, T Daubie, E Alves, GA Damiao, DD Pol, ME Souza, MHG Carvalho, W Da Costa, EM Martins, CD De Souza, SF Mundim, L Nogima, H Oguri, V Da Silva, WLP Santoro, A Do Amaral, SMS Sznajder, A De Araujo, FTD Dias, FA Tomei, TRFP Gregores, EM Lagana, C Marinho, F Mercadante, PG Novaes, SF Padula, SS Darmenov, N Dimitrov, L Genchev, V Iaydjiev, P Piperov, S Rodozov, M Stoykova, S Sultanov, G Tcholakov, V Trayanov, R Vankov, I Dimitrov, A Hadjiiska, R Karadzhinova, A Kozhuharov, V Litov, L Mateev, M Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, J Wang, J Wang, X Wang, Z Xiao, H Xu, M Zang, J Zhang, Z Ban, Y Guo, S Guo, Y Li, W Mao, Y Qian, SJ Teng, H Zhang, L Zhu, B Zou, W Cabrera, A Moreno, BG Rios, AAO Oliveros, AFO Sanabria, JC Godinovic, N Lelas, D Lelas, K Plestina, R Polic, D Puljak, I Antunovic, Z Dzelalija, M Brigljevic, V Duric, S Kadija, K Morovic, S Attikis, A Galanti, M Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Assran, Y Khalil, S Mahmoud, MA Hektor, A Kadastik, M Muntel, M Raidal, M Rebane, L Azzolini, V Eerola, P Fedi, G Czellar, S Harkonen, J Heikkinen, A Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Tuominen, E Tuominiemi, J Tuovinen, E Ungaro, D Wendland, L Banzuzi, K Korpela, A Tuuva, T Sillou, D Besancon, M Choudhury, S Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Gentit, FX Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Marionneau, M Millischer, L Rander, J Rosowsky, A Shreyber, I Titov, 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Lungu, G. Malik, S. Mesropian, C. Yan, M. Atramentov, O. Barker, A. Duggan, D. Gershtein, Y. Gray, R. Halkiadakis, E. Hidas, D. Hits, D. Lath, A. Panwalkar, S. Patel, R. Richards, A. Rose, K. Schnetzer, S. Somalwar, S. Stone, R. Thomas, S. Cerizza, G. Hollingsworth, M. Spanier, S. Yang, Z. C. York, A. Asaadi, J. Eusebi, R. Gilmore, J. Gurrola, A. Kamon, T. Khotilovich, V. Montalvo, R. Nguyen, C. N. Osipenkov, I. Pakhotin, Y. Pivarski, J. Safonov, A. Sengupta, S. Tatarinov, A. Toback, D. Weinberger, M. Akchurin, N. Bardak, C. Damgov, J. Jeong, C. Kovitanggoon, K. Lee, S. W. Roh, Y. Sill, A. Volobouev, I. Wigmans, R. Yazgan, E. Appelt, E. Brownson, E. Engh, D. Florez, C. Gabella, W. Issah, M. Johns, W. Kurt, P. Maguire, C. Sheldon, A. Melo P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Balazs, M. Boutle, S. Cox, B. Francis, B. Hirosky, R. Ledovskoy, A. Lin, C. Neu, C. Yohay, R. Gollapinni, S. Harr, R. Karchin, P. E. Lamichhane, P. Mattson, M. Ne, C. Milste Sakharov, A. Anderson, M. Bachtis, M. Bellinger, J. N. Carlsmith, D. Dasu, S. Efron, J. Flood, K. Gray, L. Grogg, K. S. Grothe, M. Hall-Wilton, R. Herndon, M. Klabbers, P. Klukas, J. Lanaro, A. Lazaridis, C. Leonard, J. Loveless, R. Mohapatra, A. Palmonari, F. Reeder, D. Ross, I. Savin, A. Smith, W. H. Swanson, J. Weinberg, M. CA CMS Collaboration TI Search for Supersymmetry in pp Collisions at root s=7 TeV in Events with Two Photons and Missing Transverse Energy SO PHYSICAL REVIEW LETTERS LA English DT Article ID OF-MASS ENERGIES; E(+)E(-) COLLISIONS; BREAKING TOPOLOGIES; GRAVITINO; LEP AB A search for supersymmetry in the context of general gauge-mediated breaking with the lightest neutralino as the next-to-lightest supersymmetric particle and the gravitino as the lightest is presented. The data sample corresponds to an integrated luminosity of 36 pb(-1) recorded by the CMS experiment at the LHC. The search is performed by using events containing two or more isolated photons, at least one hadronic jet, and significant missing transverse energy. No excess of events at high missing transverse energy is observed. Upper limits on the signal cross section for general gauge-mediated supersymmetry between 0.3 and 1.1 pb at the 95% confidence level are determined for a range of squark, gluino, and neutralino masses, excluding supersymmetry parameter space that was inaccessible to previous experiments. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.; Zhukov, V.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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[Adler, V.; Cimmino, A.; Costantini, S.; Grunewald, M.; Klein, B.; Lellouch, J.; Marinov, A.; Mccartin, J.; Ryckbosch, D.; Thyssen, F.; Tytgat, M.; Vanelderen, L.; Verwilligen, P.; Walsh, S.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Charaf, O.; Clerbaux, B.; De Lentdecker, G.; Dero, V.; Gay, A. P. R.; Hammad, G. H.; Hreus, T.; Marage, E.; Thomas, L.; Velde, C. Vander; Vanlaer, P.] Univ Libre Brussels, Brussels, Belgium. [Basegmez, S.; Bruno, G.; Caudron, J.; Ceard, L.; Gil, E. Cortina; De Jeneret, J. De Favereau; Delaere, C.; Favart, D.; Giammanco, A.; Gregoire, G.; Hollar, J.; Lemaitre, V.; Liao, J.; Militaru, O.; Ovyn, S.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Schul, N.] Catholic Univ Louvain, B-1348 Louvain, Belgium. [Beliy, N.; Caebergs, T.; Daubie, E.] Univ Mons, B-7000 Mons, Belgium. [Alves, G. A.; De Jesus Damiao, D.; Pol, M. E.; Souza, M. H. G.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Carvalho, W.; Da Costa, E. 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[Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Della Ricca, G.; Montanino, D.] Univ Trieste, Trieste, Italy. [Belforte, S.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Montanino, D.; Penzo, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Heo, S. G.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Chung, J.; Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Park, H.; Ro, S. R.; Son, D.; Son, D. C.; Son, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, Zero; Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Hong, B.; Jeong, M. S.; Jo, M.; Kim, H.; Kim, J. H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.; Rhee, H. B.; Seo, E.; Shin, S.; Sim, K. S.] Korea Univ, Seoul, South Korea. [Choi, M.; Kang, S.; Kim, H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. 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A.; Khurshid, T.; Qazi, S.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Brona, G.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bluj, M.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Soltan Inst Nucl Studies, PL-00681 Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Musella, P.; Nayak, A.; Seixas, J.; Varela, J.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Belotelov, I.; Bunin, P.; Golutvin, I.; Kamenev, A.; Karjavin, V.; Kozlov, G.; Lanev, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Toropin, A.; Troitsky, S.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Kaftanov, V.; Kossov, M.; Krokhotin, A.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Katkov, I.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Sarycheva, L.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Azhgirey, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Slabospitsky, S.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.; Adzic, P.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Djordjevic, M.; Krpic, D.; Milosevic, J.; Aguilar-Benitez, M.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Djordjevic, M.; Krpic, D.; Milosevic, J.; Aguilar-Benitez, M.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Arce, P.; Battilana, C.; Calvo, E.; Cepeda, M.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Diez Pardos, C.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.] Univ Oviedo, Oviedo, Spain. [Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Vizan Garcia, J. M.; Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Jorda, C.; Lobelle Pardo, P.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Gomez, J. Piedra; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Hammer, J.; Delaere, C.; Darmenov, N.; Genchev, V.; Iaydjiev, P.; Jung, H.; Hajdu, C.; Sikler, F.; Mohanty, A. K.; Chiorboli, M.; De Guio, F.; Montoya, C. A. Carrillo; Iorio, A. O. M.; Lucaroni, A.; Taroni, S.; Boccali, T.; Tonelli, G.; Grassi, M.; Pandolfi, F.; Botta, C.; Graziano, A.; Kossov, M.; Grishin, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Baillon, P.; Ball, A. H.; Barney, D.; Bell, A. J.; Benedetti, D.; Bernet, C.; Bialas, W.; Bloch, P.; Bocci, A.; Bolognesi, S.; Bona, M.; Breuker, H.; Bunkowski, K.; Camporesi, T.; Cerminara, G.; Coarasa Perez, J. A.; Cure, B.; D'Enterria, D.; De Roeck, A.; Di Guida, S.; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Gaddi, A.; Gennai, S.; Georgiou, G.; Gerwig, H.; Gigi, D.; Gill, K.; Giordano, D.; Glege, F.; Gomez-Reino Garrido, R.; Gouzevitch, M.; Govoni, P.; Gowdy, S.; Guiducci, L.; Hansen, M.; Hartl, C.; Harvey, J.; Hegeman, J.; Hegner, B.; Hoffmann, H. F.; Honma, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Lecoq, P.; Lourenco, C.; Maeki, T.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Maurisset, A.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Nesvold, E.; Nguyen, M.; Orimoto, T.; Orsini, L.; Perez, E.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Polese, G.; Racz, A.; Rodrigues Antunes, J.; Rolandi, G.; Rommerskirchen, T.; Rovelli, C.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Segoni, I.; Sharma, A.; Siegrist, P.; Simon, M.; Sphicas, P.; Spiropulu, M.; Stoye, M.; Tropea, P.; Tsirou, A.; Vichoudis, P.; Voutilainen, M.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Starodumov, A.; Bortignon, P.; Caminada, L.; Marchica, C.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Caminada, L.; Chanon, N.; Chen, Z.; Cittolin, S.; Dissertori, G.; Dittmar, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Herve, A.; Hintz, W.; Lecomte, P.; Lustermann, W.; Marchica, C.; del Arbol, P. Martinez Ruiz; Meridiani, P.; Milenovic, P.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pape, L.; Pauss, F.; Punz, T.; Rizzi, A.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Sawley, M. -C.; Stieger, B.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, M.; Wehrli, L.; Weng, J.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aguilo, E.; Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Otiougova, P.; Regenfus, C.; Robmann, P.; Schmidt, A.; Snoek, H.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Volpe, R.; Wu, J. H.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Topaksu, A. Kayis; Nart, A.; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Uzun, D.; Vergili, L. N.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Deliomeroglu, M.; Demir, D.; Lmez, E. Gu; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Levchuk, L.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Bostock, F.; Brooke, J. J.; Cheng, T. L.; Clement, E.; Cussans, D.; Frazier, R.; Goldstein, J.; Grimes, M.; Hansen, M.; Hartley, D.; Heath, G. P.; Heath, H. F.; Jackson, J.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Ward, S.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Camanzi, B.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Ballin, J.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Lyons, L.; MacEvoy, B. C.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rompotis, N.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Tourneur, S.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Wardrope, D.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Barrett, M.; Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Martin, W.; Reid, I. D.; Teodorescu, L.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.] Baylor Univ, Waco, TX 76798 USA. [Bose, T.; Jarrin, E. Carrera; Fantasia, C.; Heister, A.; John, J. St.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Avetisyan, A.; Bhattacharya, S.; Chou, J. P.; Cutts, D.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Landsberg, G.; Narain, M.; Nguyen, D.; Segala, M.; Sinthuprasith, T.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Cox, P. T.; Dolen, J.; Erbacher, R.; Friis, E.; Ko, W.; Kopecky, A.; Lander, R.; Liu, H.; Maruyama, S.; Miceli, T.; Nikolic, M.; Pellett, D.; Robles, J.; Salur, S.; Schwarz, T.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez; Veelken, C.] Univ Calif Davis, Davis, CA 95616 USA. [Brochero Cifuentes, J. A.; Andreev, V.; Arisaka, K.; Cline, D.; Cousins, R.; Deisher, A.; Duris, J.; Erhan, S.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Tucker, J.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Chandra, A.; Clare, R.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Kao, S. C.; Liu, F.; Liu, H.; Long, O. R.; Luthra, A.; Nguyen, H.; Shen, B. C.; Stringer, R.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Dusinberre, E.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pi, H.; Pieri, M.; Ranieri, R.; Sani, M.; Sharma, V.; Simon, S.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; Vlimant, J. R.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Spiropulu, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Gataullin, M.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Shin, K.; Timciuc, V.; Traczyk, P.; Veverka, J.; Wilkinson, R.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Akgun, B.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Jun, S. Y.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Dinardo, M. E.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Gaz, A.; Heyburn, B.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.; Zang, S. L.] Univ Colorado, Boulder, CO 80309 USA. [Agostino, L.; Alexander, J.; Cassel, D.; Chatterjee, A.; Das, S.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Kaufman, G. Nicolas; Patterson, J. R.; Puigh, D.; Ryd, A.; Salvati, E.; Shi, X.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Biselli, A.; Cirino, G.; Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Atac, M.; Bakken, J. A.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Borcherding, F.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Cooper, W.; Eartly, D. P.; Elvira, V. D.; Esen, S.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Green, D.; Gunthoti, K.; Gutsche, O.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jensen, H.; Johnson, M.; Joshi, U.; Khatiwada, R.; Klima, B.; Kousouris, K.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Limon, P.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Mason, D.; McBride, P.; Miao, T.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Pordes, R.; Prokofyev, O.; Saoulidou, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Tan, P.; Taylor, L.; Tkaczyk, S.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Gomez, J. Piedra; Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Matchev, K.; Mitselmakher, G.; Muniz, L.; Prescott, C.; Remington, R.; Schmitt, M.; Scurlock, B.; Sellers, P.; Skhirtladze, N.; Snowball, M.; Wang, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Ceron, C.; Gaultney, V.; Kramer, L.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Mesa, D.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bandurin, D.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Quertenmont, L.; Sekmen, S.; Veeraraghavan, V.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Guragain, S.; Hohlmann, M.; Kalakhety, H.; Ralich, R.; Vodopiyanov, I.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Callner, J.; Cavanaugh, R.; Dragoiu, C.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kunde, G. J.; Lacroix, F.; Malek, M.; O'Brien, C.; Silvestre, C.; Smoron, A.; Strom, D.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Duru, F.; Lae, C. K.; McCliment, E.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Olson, J.; Onel, Y.; Ozok, F.; Sen, S.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bonato, A.; Eskew, C.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Rappoccio, S.; Swartz, M.; Tran, N. V.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Grachov, O.; Iii, R. P. Kenny; Murray, M.; Noonan, D.; Sanders, S.; Wood, J. S.; Zhukova, V.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Bolton, T.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.; Wan, Z.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Boutemeur, M.; Eno, S. C.; Ferencek, D.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kirn, M.; Lu, Y.; Mignerey, A. C.; Rossato, K.; Rumerio, P.; Santanastasio, F.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.; Twedt, E.] Univ Maryland, College Pk, MD 20742 USA. [Wyslouch, B.; Alver, B.; Bauer, G.; Bendavid, J.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Everaerts, P.; Ceballos, G. Gomez; Goncharov, M.; Hahn, K. A.; Harris, P.; Kim, Y.; Klute, M.; Lee, Y. -J.; Li, W.; Loizides, C.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Rudolph, M.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Wenger, E. A.; Xie, S.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.] MIT, Cambridge, MA 02139 USA. [Cooper, S. I.; Cushman, P.; Dahmes, B.; De Benedetti, A.; Dudero, P. R.; Franzoni, G.; Haupt, J.; Klapoetke, K.; Kubota, Y.; Mans, J.; Rekovic, V.; Rusack, R.; Sasseville, M.; Singovsky, A.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Godang, R.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, University, MS 38677 USA. [Bloom, K.; Bose, S.; Butt, J.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kelly, T.; Kravchenko, I.; Lazo-Flores, J.; Malbouisson, H.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Baur, U.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Shipkowski, S. P.; Smith, K.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Boeriu, O.; Chasco, M.; Reucroft, S.; Swain, J.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Kubik, A.; Odell, N.; Ofierzynski, R. 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JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MST (Russia); MAE (Russia); MSTD (Serbia); MICINN (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK (Turkey); TAEK (Turkey); STFC (United Kingdom); DOE (USA); NSF (USA) FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine. We thank the technical and administrative staff at CERN and other CMS institutes and acknowledge support from: FMSR (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences and NICPB (Estonia); Academy of Finland, ME, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MST and MAE (Russia); MSTD (Serbia); MICINN and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK and TAEK (Turkey); STFC (United Kingdom); DOE and NSF (USA). NR 30 TC 43 Z9 43 U1 1 U2 46 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 24 PY 2011 VL 106 IS 21 AR 211802 DI 10.1103/PhysRevLett.106.211802 PG 15 WC Physics, Multidisciplinary SC Physics GA 767YE UT WOS:000290895300002 PM 21699288 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hammer, J Hansel, S Hartl, C Hoch, M Hormann, N Hrubec, J Jeitler, M Kasieczka, G Kiesenhofer, W Krammer, M Liko, D Mikulec, I Pernicka, M Rohringer, H Schofbeck, R Strauss, J Teischinger, F Wagner, P Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Benucci, L De Wolf, EA Janssen, X Maes, T Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Blekman, F Blyweert, S D'Hondt, J Devroede, O Suarez, RG Kalogeropoulos, A Maes, J Maes, M Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Charaf, O Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hammad, GH Hreus, T Marage, PE Thomas, L Vander 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CA CMS Collaboration TI Study of Z Boson Production in PbPb Collisions at root s(NN)=2.76 TeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID HEAVY-ION COLLISIONS; LHC AB A search for Z bosons in the mu(+)mu(-) decay channel has been performed in PbPb collisions at root s(NN) = 2.76 TeV with the CMS detector at the LHC, in a 7.2 mu b(-1) data sample. The number of opposite-sign muon pairs observed in the 60-120 GeV/c(2) invariant mass range is 39, corresponding to a yield per unit of rapidity (y) and per minimum bias event of [33.8 +/- 5.5(stat) +/- 4.4(syst)] x 10(-8), in the vertical bar y vertical bar < 2.0 range. Rapidity, transverse momentum, and centrality dependencies are also measured. The results agree with next-to-leading order QCD calculations, scaled by the number of incoherent nucleon-nucleon collisions. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. 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M.; Caponeri, B.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Menichelli, M.; Nappi, A.; Santocchia, A.; Taroni, S.; Valdata, M.; Volpe, R.; Pioppi, M.] Univ Perugia, Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Palmonari, F.; Segneri, G.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bernardini, J.; Boccali, T.; Fiori, F.; Messineo, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Azzurri, P.; Broccolo, G.; D'Agnolo, R. T.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. 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[Amapane, N.; Argiro, S.; Botta, C.; Castello, R.; Costa, M.; Graziano, A.; Marone, M.; Migliore, E.; Mila, G.; Monaco, V.; Musich, M.; Pelliccioni, M.; Romero, A.; Sacchi, R.; Sola, V.; Solano, A.; Trocino, D.; Pereira, A. Vilela] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Montanino, D.; Penzo, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Della Ricca, G.; Montanino, D.] Univ Trieste, Trieste, Italy. [Heo, S. G.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Chung, J.; Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Park, H.; Ro, S. R.; Son, D.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, Zero; Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Hong, B.; Jeong, M. S.; Jo, M.; Kim, H.; Kim, J. H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.; Rhee, H. B.; Seo, E.; Shin, S.; Sim, K. S.] Korea Univ, Seoul, South Korea. [Choi, M.; Kang, S.; Kim, H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Martisiute, D.; Petrov, P.; Sabonis, T.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ahmed, I.; Asghar, M. I.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bluj, M.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Soltan Inst Nucl Studies, PL-00681 Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Musella, P.; Nayak, A.; Seixas, J.; Varela, J.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Belotelov, I.; Bunin, P.; Golutvin, I.; Kamenev, A.; Karjavin, V.; Kozlov, G.; Lanev, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Toropin, A.; Troitsky, S.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Kaftanov, V.; Kossov, M.; Krokhotin, A.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Zhukov, V.; Boos, E.; Demiyanov, A.; Ershov, A.; Gribushin, A.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Sarycheva, L.; Savrin, V.; Snigirev, A.; Vardanyan, I.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Azhgirey, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Slabospitsky, S.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Maestre, J. Alcaraz; Arce, P.; Battilana, C.; Calvo, E.; Cepeda, M.; Cerrada, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Diez Pardos, C.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Redondo, I.; Romero, L.; Santaolalla, J.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chamizo Llatas, M.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Jorda, C.; Lobelle Pardo, P.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria, E-39005 Santander, Spain. [Hammer, J.; Darmenov, N.; Genchev, V.; Iaydjiev, P.; Hajdu, C.; Mohanty, A. K.; Lusito, L.; Chiorboli, M.; Ghezzi, A.; Malberti, M.; Lucaroni, A.; Tonelli, G.; Venturi, A.; Pandolfi, F.; Botta, C.; Graziano, A.; Pelliccioni, M.; Pereira, A. Vilela; Kossov, M.; Grishin, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Baillon, P.; Ball, A. H.; Barney, D.; Bell, A. J.; Benedetti, D.; Bernet, C.; Bialas, W.; Bloch, P.; Bocci, A.; Bolognesi, S.; Bona, M.; Breuker, H.; Brona, G.; Bunkowski, K.; Camporesi, T.; Cerminara, G.; Perez, J. A. Coarasa; Cure, B.; D'Enterria, D.; De Roeck, A.; Di Guida, S.; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Gaddi, A.; Gennai, S.; Georgiou, G.; Gerwig, H.; Gigi, D.; Gill, K.; Giordano, D.; Glege, F.; Garrido, R. Gomez-Reino; Gouzevitch, M.; Govoni, P.; Gowdy, S.; Guiducci, L.; Hansen, M.; Harvey, J.; Hegeman, J.; Hegner, B.; Hoffmann, H. F.; Honma, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Lecoq, P.; Lourenco, C.; Maeki, T.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Nesvold, E.; Nguyen, M.; Orimoto, T.; Orsini, L.; Perez, E.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Polese, G.; Racz, A.; Antunes, J. Rodrigues; Rolandi, G.; Rommerskirchen, T.; Rovelli, C.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Segoni, I.; Sharma, A.; Siegrist, P.; Simon, M.; Sphicas, P.; Spiropulu, M.; Stoeckli, F.; Stoye, M.; Tropea, P.; Tsirou, A.; Vichoudis, P.; Voutilainen, M.; Zeuner, W. D.; Sharma, V.; Hall-Wilton, R.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Starodumov, A.; Caminada, L.; Marchica, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bortignon, P.; Caminada, L.; Chen, Z.; Cittolin, S.; Dissertori, G.; Dittmar, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Herve, A.; Hintz, W.; Lecomte, P.; Lustermann, W.; Marchica, C.; del Arbol, P. Martinez Ruiz; Meridiani, P.; Milenovic, P.; Moortgat, F.; Nef, P.; Nessi-Tedaldi, F.; Pape, L.; Pauss, F.; Punz, T.; Rizzi, A.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Sawley, M. -C.; Stieger, B.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, M.; Wehrli, L.; Weng, J.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aguilo, E.; Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Regenfus, C.; Robmann, P.; Schmidt, A.; Snoek, H.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, E. A.; Chen, K. H.; Chen, W. T.; Dutta, S.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, M. H.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Wu, J. H.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Demir, Z.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Topaksu, A. Kayis; Nart, A.; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Uzun, D.; Vergili, L. N.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Deliomeroglu, M.; Demir, D.; Guelmez, E.; Halu, A.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Levchuk, L.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Bell, P.; Bostock, F.; Brooke, J. J.; Cheng, T. L.; Clement, E.; Cussans, D.; Frazier, R.; Goldstein, J.; Grimes, M.; Hansen, M.; Hartley, D.; Heath, G. P.; Heath, H. F.; Huckvale, B.; Jackson, J.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Ward, S.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Camanzi, B.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Ballin, J.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Davies, G.; Della Negra, M.; Fulcher, J.; Futyan, D.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Karapostoli, G.; MacEvoy, B. C.; Magnan, A. -M.; Marrouche, J.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rompotis, N.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Barrett, M.; Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Martin, W.; Reid, I. D.; Teodorescu, L.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.] Baylor Univ, Waco, TX 76798 USA. [Bose, T.; Jarrin, E. Carrera; Fantasia, C.; Heister, A.; John, J. St.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Avetisyan, A.; Bhattacharya, S.; Chou, J. P.; Cutts, D.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Landsberg, G.; Narain, M.; Nguyen, D.; Segala, M.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Cox, P. T.; Dolen, J.; Erbacher, R.; Friis, E.; Ko, W.; Kopecky, A.; Lander, R.; Liu, H.; Maruyama, S.; Miceli, T.; Nikolic, M.; Pellett, D.; Robles, J.; Salur, S.; Schwarz, T.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez; Veelken, C.] Univ Calif Davis, Davis, CA 95616 USA. [Felcini, M.; Andreev, V.; Arisaka, K.; Cline, D.; Cousins, R.; Deisher, A.; Duris, J.; Erhan, S.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Tucker, J.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Chandra, A.; Clare, R.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Kao, S. C.; Liu, F.; Liu, H.; Long, O. R.; Luthra, A.; Nguyen, H.; Shen, B. C.; Stringer, R.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Dusinberre, E.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pi, H.; Pieri, M.; Ranieri, R.; Sani, M.; Sharma, V.; Simon, S.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Rthwein, F. Wu; Yagil, A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; Vlimant, J. R.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Spiropulu, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Gataullin, M.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Timciuc, V.; Traczyk, P.; Veverka, J.; Wilkinson, R.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Akgun, B.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Jun, S. Y.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Dinardo, M. E.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Gaz, A.; Heyburn, B.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.; Zang, S. L.] Univ Colorado, Boulder, CO 80309 USA. [Agostino, L.; Alexander, J.; Cassel, D.; Chatterjee, A.; Das, S.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Kaufman, G. Nicolas; Patterson, J. R.; Puigh, D.; Ryd, A.; Shi, X.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Biselli, A.; Cirino, G.; Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Atac, M.; Bakken, J. A.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Borcherding, F.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Cooper, W.; Eartly, D. P.; Elvira, V. D.; Esen, S.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Green, D.; Gunthoti, K.; Gutsche, O.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jensen, H.; Johnson, M.; Joshi, U.; Khatiwada, R.; Klima, B.; Kousouris, K.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Limon, P.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Mason, D.; McBride, P.; Miao, T.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Pordes, R.; Prokofyev, O.; Saoulidou, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Tan, P.; Taylor, L.; Tkaczyk, S.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Piedra Gomez, J.; Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Goldberg, S.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Matchev, K.; Mitselmakher, G.; Muniz, L.; Pakhotin, Y.; Prescott, C.; Remington, R.; Schmitt, M.; Scurlock, B.; Sellers, P.; Skhirtladze, N.; Wang, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Ceron, C.; Gaultney, V.; Kramer, L.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bandurin, D.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Quertenmont, L.; Sekmen, S.; Veeraraghavan, V.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Guragain, S.; Hohlmann, M.; Kalakhety, H.; Ralich, R.; Vodopiyanov, I.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Callner, J.; Cavanaugh, R.; Dragoiu, C.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kunde, G. J.; Lacroix, F.; Malek, M.; O'Brien, C.; Silvestre, C.; Smoron, A.; Strom, D.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Duru, F.; Lae, C. K.; McCliment, E.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Olson, J.; Onel, Y.; Ozok, F.; Sen, S.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bonato, A.; Eskew, C.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Rappoccio, S.; Swartz, M.; Tran, N. V.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. 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MST (Russia); MAE (Russia); MSTD (Serbia); MICINN (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK (Turkey); TAEK (Turkey); STFC (United Kingdom); DOE (USA); NSF (USA) FX We thank Bryon Neufeld, Hannu Paukkunen, Carlos Salgado, Ivan Vitev, and Ramona Vogt for fruitful theoretical inputs on the nuclear effects involved in Z production. We wish to congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine in 2010. We thank the technical and administrative staff at CERN and other CMS institutes, and acknowledge support from FMSR (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences and NICPB (Estonia); Academy of Finland, ME, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MST and MAE (Russia); MSTD (Serbia); MICINN and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK and TAEK (Turkey); STFC (United Kingdom); DOE and NSF (USA). NR 22 TC 63 Z9 63 U1 1 U2 47 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 24 PY 2011 VL 106 IS 21 AR 212301 DI 10.1103/PhysRevLett.106.212301 PG 14 WC Physics, Multidisciplinary SC Physics GA 767YE UT WOS:000290895300004 PM 21699291 ER PT J AU Nicholson, A Ge, WH Zhang, XT Riera, J Daghofer, M Oles, AM Martins, GB Moreo, A Dagotto, E AF Nicholson, Andrew Ge, Weihao Zhang, Xiaotian Riera, Jose Daghofer, Maria Oles, Andrzej M. Martins, George B. Moreo, Adriana Dagotto, Elbio TI Competing Pairing Symmetries in a Generalized Two-Orbital Model for the Pnictide Superconductors SO PHYSICAL REVIEW LETTERS LA English DT Article ID ELECTRONS AB We introduce and study an extended "t-U-J'' two-orbital model for the pnictides that includes Heisenberg terms deduced from the strong coupling expansion. Including these J terms explicitly allows us to enhance the strength of the (pi, 0)-(0, pi) spin order which favors the presence of tightly bound pairing states even in the small clusters that are here exactly diagonalized. The A(1g) and B-2g pairing symmetries are found to compete in the realistic spin-ordered and metallic regime. The dynamical pairing susceptibility additionally unveils low-lying B-1g states, suggesting that small changes in parameters may render any of the three channels stable. C1 [Nicholson, Andrew; Ge, Weihao; Zhang, Xiaotian; Moreo, Adriana; Dagotto, Elbio] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Nicholson, Andrew; Ge, Weihao; Zhang, Xiaotian; Moreo, Adriana; Dagotto, Elbio] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Riera, Jose] Univ Nacl Rosario, Inst Fis Rosario, RA-2000 Rosario, Santa Fe, Argentina. [Daghofer, Maria] IFW Dresden, D-01171 Dresden, Germany. [Oles, Andrzej M.] Max Planck Inst Festkorperforsch, D-70569 Stuttgart, Germany. [Oles, Andrzej M.] Jagiellonian Univ, M Smoluchowski Inst Phys, PL-30059 Krakow, Poland. [Martins, George B.] Oakland Univ, Dept Phys, Rochester, MI 48309 USA. RP Nicholson, A (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RI Daghofer, Maria/C-5762-2008; Riera, Jose/A-1234-2008; Martins, George/C-9756-2012 OI Daghofer, Maria/0000-0001-9434-8937; Riera, Jose/0000-0003-4546-1137; Martins, George/0000-0001-7846-708X FU U.S. DOE, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; CONICET, Argentina; DFG; Foundation for Polish Science (FNP); Polish government [N202 069639] FX This work was supported by the U.S. DOE, Office of Basic Energy Sciences, Materials Sciences and Engineering Division (A. N., W. G., X. Z., G. M., A. M., E. D.), CONICET, Argentina (J. R.), the DFG under the Emmy-Noether program (M. D.), and by the Foundation for Polish Science (FNP) and the Polish government Project N202 069639 (A. M. O.). Conversations with D.X. Yao and Thomas Prestel are acknowledged. NR 28 TC 40 Z9 40 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 24 PY 2011 VL 106 IS 21 AR 217002 DI 10.1103/PhysRevLett.106.217002 PG 4 WC Physics, Multidisciplinary SC Physics GA 767YE UT WOS:000290895300011 PM 21699330 ER PT J AU Ren, X Bray, I Fursa, DV Colgan, J Pindzola, MS Pfluger, T Senftleben, A Xu, S Dorn, A Ullrich, J AF Ren, X. Bray, I. Fursa, D. V. Colgan, J. Pindzola, M. S. Pflueger, T. Senftleben, A. Xu, S. Dorn, A. Ullrich, J. TI Electron-impact ionization of helium: A comprehensive experiment benchmarks theory SO PHYSICAL REVIEW A LA English DT Article ID DIFFERENTIAL CROSS-SECTIONS; ENERGY; HE AB Single ionization of helium by 70.6-eV electron impact is studied in a comprehensive experiment covering a major part of the entire collision kinematics and the full 4 pi solid angle for the emitted electron. The absolutely normalized triple-differential experimental cross sections are compared with results from the convergent close-coupling (CCC) and the time-dependent close-coupling (TDCC) theories. Whereas excellent agreement with the TDCC prediction is only found for equal energy sharing, the CCC calculations are in excellent agreement with essentially all experimentally observed dynamical features, including the absolute magnitude of the cross sections. C1 [Ren, X.; Pflueger, T.; Senftleben, A.; Xu, S.; Dorn, A.; Ullrich, J.] Max Planck Inst Nucl Phys, DE-69117 Heidelberg, Germany. [Bray, I.; Fursa, D. V.] Curtin Univ, ARC Ctr Antimatter Matter Studies, Perth, WA, Australia. [Colgan, J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Pindzola, M. S.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. RP Ren, X (reprint author), Max Planck Inst Nucl Phys, DE-69117 Heidelberg, Germany. EM Alexander.Dorn@mpi-hd.mpg.de RI Fursa, Dmitry/C-2301-2009; Bray, Igor/B-8586-2009; Xu, Shenyue/G-3907-2015; OI Fursa, Dmitry/0000-0002-3951-9016; Bray, Igor/0000-0001-7554-8044; Xu, Shenyue/0000-0001-9872-2244; Colgan, James/0000-0003-1045-3858; Senftleben, Arne/0000-0003-0932-9892 FU DFG [RE 2966/1-1]; Australian Research Council; Australian National Computational Infrastructure Facility and its Western Australian node iVEC; US Department of Energy [DE-AC5206NA25396]; DOE; NSF FX X.R. is grateful for support from DFG Project No. RE 2966/1-1. I.B. and D.V.F. are grateful for the support of the Australian Research Council and the Australian National Computational Infrastructure Facility and its Western Australian node iVEC. The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the National Nuclear Security Administration of the US Department of Energy under Contract No. DE-AC5206NA25396. A portion of this work was performed through DOE and NSF grants to Auburn University. NR 21 TC 26 Z9 26 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 J9 PHYS REV A JI Phys. Rev. A PD MAY 24 PY 2011 VL 83 IS 5 AR 052711 DI 10.1103/PhysRevA.83.052711 PG 6 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 767YF UT WOS:000290895400010 ER PT J AU Adekola, AS Bardayan, DW Blackmon, JC Brune, CR Chae, KY Domizioli, C Greife, U Heinen, Z Hornish, MJ Jones, KL Kozub, RL Livesay, RJ Ma, Z Massey, TN Moazen, B Nesaraja, CD Pain, SD Shriner, JF Smith, ND Smith, MS Thomas, JS Visser, DW Voinov, AV AF Adekola, A. S. Bardayan, D. W. Blackmon, J. C. Brune, C. R. Chae, K. Y. Domizioli, C. Greife, U. Heinen, Z. Hornish, M. J. Jones, K. L. Kozub, R. L. Livesay, R. J. Ma, Z. Massey, T. N. Moazen, B. Nesaraja, C. D. Pain, S. D. Shriner, J. F., Jr. Smith, N. D. Smith, M. S. Thomas, J. S. Visser, D. W. Voinov, A. V. TI First proton-transfer study of F-18 + p resonances relevant for novae SO PHYSICAL REVIEW C LA English DT Article ID GAMMA-RAY EMISSION; REACTION-RATES; NOVA; CYGNI AB The F-18(p, alpha)O-15 reaction is the predominant destruction mechanism in novae of the radionuclide F-18, a target of gamma-ray observatories. Thus, its rate is important for understanding F-18 production in novae. We have studied resonances in the F-18 + p system by making a measurement of a proton-transfer reaction F-18(d, n). We have observed 15 Ne-19 levels, 5 of which are below the proton threshold, including a subthreshold state, which has significant l(p) = 0 strength. Our data provide a direct determination of the spectroscopic strength of these states and new constraints on their spins and parities, thereby resolving a controversy, which involves the 8- and 38-keV resonances. The F-18(p, alpha)O-15 reaction rate is reevaluated, which takes the subthreshold resonance and other new information determined in this experiment into account. C1 [Adekola, A. S.; Brune, C. R.; Heinen, Z.; Hornish, M. J.; Massey, T. N.; Voinov, A. V.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Adekola, A. S.; Jones, K. L.; Pain, S. D.; Thomas, J. S.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Bardayan, D. W.; Blackmon, J. C.; Nesaraja, C. D.; Smith, M. S.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Chae, K. Y.; Domizioli, C.; Ma, Z.; Moazen, B.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Greife, U.; Livesay, R. J.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. [Kozub, R. L.; Shriner, J. F., Jr.; Smith, N. D.] Tennessee Technol Univ, Dept Phys, Cookeville, TN 38505 USA. [Visser, D. W.] Univ N Carolina, Dept Phys & Astron, Chapel Hill, NC 27599 USA. RP Adekola, AS (reprint author), Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. EM aadekola@physics.rutgers.edu RI Jones, Katherine/B-8487-2011; Pain, Steven/E-1188-2011; OI Jones, Katherine/0000-0001-7335-1379; Pain, Steven/0000-0003-3081-688X; Nesaraja, Caroline/0000-0001-5571-8341 FU U.S. Department of Energy [DE-FG02-88ER40387, DE-FG02-93ER40789, DE-FG02-96ER40990, DE-FG02-96ER40955]; National Nuclear Security Administration through the U.S. Department of Energy [DE-FG52-08NA28552]; National Nuclear Security Administration through the National Science Foundation FX We thank the staff of the HRIBF for making this experiment possible. This work was supported, in part, by the U.S. Department of Energy under Grants No. DE-FG02-88ER40387 (OU), No. DE-FG02-93ER40789 (CSM), No. DE-FG02-96ER40990, and No. DE-FG02-96ER40955 (TTU) and the National Nuclear Security Administration under the Stewardship Science Academic Alliances program through the U.S. Department of Energy Cooperative Agreement No. DE-FG52-08NA28552 and the National Science Foundation (RUTGERS). NR 29 TC 18 Z9 18 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 J9 PHYS REV C JI Phys. Rev. C PD MAY 24 PY 2011 VL 83 IS 5 AR 052801 DI 10.1103/PhysRevC.83.052801 PG 5 WC Physics, Nuclear SC Physics GA 767YM UT WOS:000290896300001 ER PT J AU Ichikawa, T Kanada-En'yo, Y Moller, P AF Ichikawa, Takatoshi Kanada-En'yo, Yoshiko Moeller, Peter TI Cluster formations in deformed states for Si-28 and S-32 SO PHYSICAL REVIEW C LA English DT Article ID HIGH-SPIN STATES; Z NUCLEI; FISSION-BARRIERS; UNSTABLE NUCLEI; MEAN-FIELD; SHELL; HEAVY; BANDS; DEFORMATIONS; SCATTERING AB We study cluster formation in strongly deformed states for Si-28 and S-32 using a macroscopic-microscopic model. The study is based on calculated total-energy surfaces, which are the sums of deformation-dependent macroscopic-microscopic potential-energy surfaces and rotational-energy contributions. We analyze the angular-momentum-dependent total-energy surfaces and identify the normal-and superdeformed states in Si-28 and S-32. We show that at sufficiently high angular momenta strongly deformed minima appear. The corresponding microscopic density distributions show cluster structures that closely resemble the O-16 + C-12 and O-16 + O-16 configurations. At still higher deformations, beyond the minima, valleys develop in the calculated surfaces. These valleys lead to mass divisions that correspond to the target-projectile configurations for which molecular resonance states have been observed. We discuss the relation between the one-body deformed minima and the two-body molecular-resonance states. C1 [Ichikawa, Takatoshi] Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan. [Kanada-En'yo, Yoshiko] Kyoto Univ, Dept Phys, Kyoto 6068502, Japan. [Moeller, Peter] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Ichikawa, T (reprint author), Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan. FU MEXT of Japan; JPSJ Kakenhi [22540275]; National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; University of Tennessee [DE-FG02-06ER41407] FX This work was done under the Yukawa International Project for Quark-Hadron Sciences (YIPQS) and was partly supported by the GCOE program "The Next Generation of Physics, Spun from Universality and Emergence" under MEXT of Japan. The work of Y.K.-E. was supported by JPSJ Kakenhi (Grant No. 22540275). P. M. acknowledges that this work was carried out under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396 and was also supported by a travel grant to the Japan-US Theory Institute for Physics with Exotic Nuclei (JUSTIPEN) under Grant No. DE-FG02-06ER41407 (University of Tennessee). The numerical calculations were carried out on Altix3700 BX2 at YITP at the Kyoto University. NR 42 TC 13 Z9 13 U1 0 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 J9 PHYS REV C JI Phys. Rev. C PD MAY 24 PY 2011 VL 83 IS 5 AR 054319 DI 10.1103/PhysRevC.83.054319 PG 7 WC Physics, Nuclear SC Physics GA 767YM UT WOS:000290896300003 ER PT J AU Abbasi, R Abdou, Y Abu-Zayyad, T Adams, J Aguilar, JA Ahlers, M Andeen, K Auffenberg, J Bai, X Baker, M Barwick, SW Bay, R Alba, JLB Beattie, K Beatty, JJ Bechet, S Becker, JK Becker, KH Benabderrahmane, ML BenZvi, S Berdermann, J Berghaus, P Berley, D Bernardini, E Bertrand, D Besson, DZ Bindig, D Bissok, M Blaufuss, E Blumenthal, J Boersma, DJ Bohm, C Bose, D Boser, S Botner, O Braun, J Brown, AM Buitink, S Carson, M Chirkin, D Christy, B Clem, J Clevermann, F Cohen, S Colnard, C Cowen, DF D'Agostino, MV Danninger, M Daughhetee, J Davis, JC De Clercq, C Demirors, L Denger, T Depaepe, O Descamps, F Desiati, P de Vries-Uiterweerd, G DeYoung, T Diaz-Velez, JC Dierckxsens, M Dreyer, J Dumm, JP Ehrlich, R Eisch, J Ellsworth, RW Engdegard, O Euler, S Evenson, PA Fadiran, O Fazely, AR Fedynitch, A Feusels, T Filimonov, K Finley, C Fischer-Wasels, T Foerster, MM Fox, BD Franckowiak, A Franke, R Gaisser, TK Gallagher, J Geisler, M Gerhardt, L Gladstone, L Glusenkamp, T Goldschmidt, A Goodman, JA Gora, D Grant, D Griesel, T Gross, A Grullon, S Gurtner, M Ha, C Hallgren, A Halzen, F Han, K Hanson, K Heinen, D Helbing, K Herquet, P Hickford, S Hill, GC Hoffman, KD Homeier, A Hoshina, K Hubert, D Huelsnitz, W Hulss, JP Hulth, PO Hultqvist, K Hussain, S Ishihara, A Jacobsen, J Japaridze, GS Johansson, H Joseph, JM Kampert, KH Kappes, A Karg, T Karle, A Kelley, JL Kenny, P Kiryluk, J Kislat, F Klein, SR Kohne, JH Kohnen, G Kolanoski, H Kopke, L Kopper, S Koskinen, DJ Kowalski, M Kowarik, T Krasberg, M Krings, T Kroll, G Kuwabara, T Labare, M Lafebre, S Laihem, K Landsman, H Larson, MJ Lauer, R Lunemann, J Madsen, J Majumdar, P Marotta, A Maruyama, R Mase, K Matis, HS Meagher, K Merck, M Meszaros, P Meures, T Middell, E Milke, N Miller, J Montaruli, T Morse, R Movit, SM Nahnhauer, R Nam, JW Naumann, U Niessen, P Nygren, DR Odrowski, S Olivas, A Olivo, M O'Murchadha, A Ono, M Panknin, S Paul, L Heros, CPD Petrovic, J Piegsa, A Pieloth, D Porrata, R Posselt, J Price, PB Przybylski, GT Rawlins, K Redl, P Resconi, E Rhode, W Ribordy, M Rizzo, A Rodrigues, JP Roth, P Rothmaier, F Rott, C Ruhe, T Rutledge, D Ruzybayev, B Ryckbosch, D Sander, HG Santander, M Sarkar, S Schatto, K Schmidt, T Schonwald, A Schukraft, A Schultes, A Schulz, O Schunck, M Seckel, D Semburg, B Seo, SH Sestayo, Y Seunarine, S Silvestri, A Slipak, A Spiczak, GM Spiering, C Stamatikos, M Stanev, T Stephens, G Stezelberger, T Stokstad, RG Stossl, A Stoyanov, S Strahler, EA Straszheim, T Stur, M Sullivan, GW Swillens, Q Taavola, H Taboada, I Tamburro, A Tepe, A Ter-Antonyan, S Tilav, S Toale, PA Toscano, S Tosi, D Turcan, D van Eijndhoven, N Vandenbroucke, J Van Overloop, A van Santen, J Vehring, M Voge, M Walck, C Waldenmaier, T Wallraff, M Walter, M Weaver, C Wendt, C Westerhoff, S Whitehorn, N Wiebe, K Wiebusch, CH Williams, DR Wischnewski, R Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, C Xu, XW Yodh, G Yoshida, S Zarzhitsky, P AF Abbasi, R. Abdou, Y. Abu-Zayyad, T. Adams, J. Aguilar, J. A. Ahlers, M. Andeen, K. Auffenberg, J. Bai, X. Baker, M. Barwick, S. W. Bay, R. Alba, J. L. Bazo Beattie, K. Beatty, J. J. Bechet, S. Becker, J. K. Becker, K. -H. Benabderrahmane, M. L. BenZvi, S. Berdermann, J. Berghaus, P. Berley, D. Bernardini, E. Bertrand, D. Besson, D. Z. Bindig, D. Bissok, M. Blaufuss, E. Blumenthal, J. Boersma, D. J. Bohm, C. Bose, D. Boeser, S. Botner, O. Braun, J. Brown, A. M. Buitink, S. Carson, M. Chirkin, D. Christy, B. Clem, J. Clevermann, F. Cohen, S. Colnard, C. Cowen, D. F. D'Agostino, M. V. Danninger, M. Daughhetee, J. Davis, J. C. De Clercq, C. Demiroers, L. Denger, T. Depaepe, O. Descamps, F. Desiati, P. de Vries-Uiterweerd, G. DeYoung, T. Diaz-Velez, J. C. Dierckxsens, M. Dreyer, J. Dumm, J. P. Ehrlich, R. Eisch, J. Ellsworth, R. W. Engdegard, O. Euler, S. Evenson, P. A. Fadiran, O. Fazely, A. R. Fedynitch, A. Feusels, T. Filimonov, K. Finley, C. Fischer-Wasels, T. Foerster, M. M. Fox, B. D. Franckowiak, A. Franke, R. Gaisser, T. K. Gallagher, J. Geisler, M. Gerhardt, L. Gladstone, L. Gluesenkamp, T. Goldschmidt, A. Goodman, J. A. Gora, D. Grant, D. Griesel, T. Gross, A. Grullon, S. Gurtner, M. Ha, C. Hallgren, A. Halzen, F. Han, K. Hanson, K. Heinen, D. Helbing, K. Herquet, P. Hickford, S. Hill, G. C. Hoffman, K. D. Homeier, A. Hoshina, K. Hubert, D. Huelsnitz, W. Huelss, J. -P. Hulth, P. O. Hultqvist, K. Hussain, S. Ishihara, A. Jacobsen, J. Japaridze, G. S. Johansson, H. Joseph, J. M. Kampert, K. -H. Kappes, A. Karg, T. Karle, A. Kelley, J. L. Kenny, P. Kiryluk, J. Kislat, F. Klein, S. R. Koehne, J. -H. Kohnen, G. Kolanoski, H. Koepke, L. Kopper, S. Koskinen, D. J. Kowalski, M. Kowarik, T. Krasberg, M. Krings, T. Kroll, G. Kuwabara, T. Labare, M. Lafebre, S. Laihem, K. Landsman, H. Larson, M. J. Lauer, R. Luenemann, J. Madsen, J. Majumdar, P. Marotta, A. Maruyama, R. Mase, K. Matis, H. S. Meagher, K. Merck, M. Meszaros, P. Meures, T. Middell, E. Milke, N. Miller, J. Montaruli, T. Morse, R. Movit, S. M. Nahnhauer, R. Nam, J. W. Naumann, U. Niessen, P. Nygren, D. R. Odrowski, S. Olivas, A. Olivo, M. O'Murchadha, A. Ono, M. Panknin, S. Paul, L. de los Heros, C. Perez Petrovic, J. Piegsa, A. Pieloth, D. Porrata, R. Posselt, J. Price, P. B. Przybylski, G. T. Rawlins, K. Redl, P. Resconi, E. Rhode, W. Ribordy, M. Rizzo, A. Rodrigues, J. P. Roth, P. Rothmaier, F. Rott, C. Ruhe, T. Rutledge, D. Ruzybayev, B. Ryckbosch, D. Sander, H. -G. Santander, M. Sarkar, S. Schatto, K. Schmidt, T. Schoenwald, A. Schukraft, A. Schultes, A. Schulz, O. Schunck, M. Seckel, D. Semburg, B. Seo, S. H. Sestayo, Y. Seunarine, S. Silvestri, A. Slipak, A. Spiczak, G. M. Spiering, C. Stamatikos, M. Stanev, T. Stephens, G. Stezelberger, T. Stokstad, R. G. Stoessl, A. Stoyanov, S. Strahler, E. A. Straszheim, T. Stuer, M. Sullivan, G. W. Swillens, Q. Taavola, H. Taboada, I. Tamburro, A. Tepe, A. Ter-Antonyan, S. Tilav, S. Toale, P. A. Toscano, S. Tosi, D. Turcan, D. van Eijndhoven, N. Vandenbroucke, J. Van Overloop, A. van Santen, J. Vehring, M. Voge, M. Walck, C. Waldenmaier, T. Wallraff, M. Walter, M. Weaver, Ch. Wendt, C. Westerhoff, S. Whitehorn, N. Wiebe, K. Wiebusch, C. H. Williams, D. R. Wischnewski, R. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, C. Xu, X. W. Yodh, G. Yoshida, S. Zarzhitsky, P. CA IceCube Collaboration TI Constraints on the extremely-high energy cosmic neutrino flux with the IceCube 2008-2009 data SO PHYSICAL REVIEW D LA English DT Article ID RAYS; SPECTRUM AB We report on a search for extremely-high energy neutrinos with energies greater than 10(6) GeV using the data taken with the IceCube detector at the South Pole. The data was collected between April 2008 and May 2009 with the half-completed IceCube array. The absence of signal candidate events in the sample of 333.5 days of live time significantly improves model-independent limits from previous searches and allows to place a limit on the diffuse flux of cosmic neutrinos with an E-2 spectrum in the energy range 2.0 x 10(6) - 6.3 x 10(9) GeV to a level of E-2 phi <= 3.6 x 10(-8) GeV cm(-2) sec(-1) sr(-1). C1 [Ishihara, A.; Mase, K.; Ono, M.; Yoshida, S.] Chiba Univ, Dept Phys, Chiba 2638522, Japan. [Bissok, M.; Blumenthal, J.; Boersma, D. J.; Euler, S.; Geisler, M.; Gluesenkamp, T.; Heinen, D.; Huelss, J. -P.; Krings, T.; Laihem, K.; Meures, T.; Paul, L.; Schukraft, A.; Schunck, M.; Vehring, M.; Wallraff, M.; Wiebusch, C. H.] Rhein Westfal TH Aachen, Inst Phys 3, D-52056 Aachen, Germany. [Toale, P. A.; Williams, D. R.; Zarzhitsky, P.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Rawlins, K.] Univ Alaska Anchorage, Dept Phys & Astron, Anchorage, AK 99508 USA. [Fadiran, O.; Japaridze, G. S.] USA Clark Atlanta Univ, CTSPS, Atlanta, GA 30314 USA. [Daughhetee, J.; Taboada, I.; Tepe, A.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Daughhetee, J.; Taboada, I.; Tepe, A.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Fazely, A. R.; Ter-Antonyan, S.; Xu, X. W.] Southern Univ, Dept Phys, Baton Rouge, LA 70813 USA. [Bay, R.; D'Agostino, M. V.; Filimonov, K.; Gerhardt, L.; Kiryluk, J.; Klein, S. R.; Porrata, R.; Price, P. B.; Vandenbroucke, J.; Woschnagg, K.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Beattie, K.; Buitink, S.; Gerhardt, L.; Goldschmidt, A.; Joseph, J. M.; Kiryluk, J.; Klein, S. R.; Matis, H. S.; Nygren, D. R.; Przybylski, G. T.; Stezelberger, T.; Stokstad, R. G.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Kappes, A.; Kolanoski, H.; Waldenmaier, T.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Becker, J. K.; Dreyer, J.; Fedynitch, A.; Olivo, M.] Ruhr Univ Bochum, Fac Phys & Astron, D-44780 Bochum, Germany. [Boeser, S.; Denger, T.; Franckowiak, A.; Homeier, A.; Kowalski, M.; Panknin, S.; Stuer, M.; Voge, M.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Seunarine, S.] Univ W Indies, Dept Phys, BB-11000 Bridgetown, Barbados. [Bechet, S.; Bertrand, D.; Dierckxsens, M.; Hanson, K.; Marotta, A.; Petrovic, J.; Swillens, Q.] Univ Libre Bruxelles, Fac Sci, B-1050 Brussels, Belgium. [Bose, D.; De Clercq, C.; Depaepe, O.; Hubert, D.; Labare, M.; Rizzo, A.; Strahler, E. A.; van Eijndhoven, N.] Vrije Univ Brussel, Dienst ELEM, B-1050 Brussels, Belgium. [Adams, J.; Brown, A. M.; Gross, A.; Hickford, S.] Univ Canterbury, Dept Phys & Astron, Christchurch 1, New Zealand. [Berley, D.; Blaufuss, E.; Christy, B.; Ehrlich, R.; Ellsworth, R. W.; Goodman, J. A.; Hoffman, K. D.; Huelsnitz, W.; Meagher, K.; Olivas, A.; Redl, P.; Roth, P.; Schmidt, T.; Straszheim, T.; Sullivan, G. W.; Turcan, D.; Wissing, H.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Beatty, J. J.; Davis, J. C.; Rott, C.; Stamatikos, M.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Beatty, J. J.; Davis, J. C.; Rott, C.; Stamatikos, M.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Beatty, J. J.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Clevermann, F.; Koehne, J. -H.; Milke, N.; Pieloth, D.; Rhode, W.; Ruhe, T.] TU Dortmund Univ, Dept Phys, D-44221 Dortmund, Germany. [Grant, D.; Wood, T. R.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2G7, Canada. [Abdou, Y.; Carson, M.; Descamps, F.; de Vries-Uiterweerd, G.; Feusels, T.; Ryckbosch, D.; Van Overloop, A.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [Colnard, C.; Gross, A.; Odrowski, S.; Resconi, E.; Schulz, O.; Sestayo, Y.; Wolf, M.] Max Planck Inst Kernphys, D-69177 Heidelberg, Germany. [Barwick, S. W.; Nam, J. W.; Silvestri, A.; Yodh, G.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Cohen, S.; Demiroers, L.; Ribordy, M.] Ecole Polytech Fed Lausanne, High Energy Phys Lab, CH-1015 Lausanne, Switzerland. [Besson, D. Z.; Kenny, P.] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. [Gallagher, J.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Abbasi, R.; Aguilar, J. A.; Andeen, K.; Baker, M.; BenZvi, S.; Berghaus, P.; Braun, J.; Chirkin, D.; Desiati, P.; Diaz-Velez, J. C.; Dumm, J. P.; Eisch, J.; Gladstone, L.; Grullon, S.; Halzen, F.; Hanson, K.; Hill, G. C.; Hoshina, K.; Jacobsen, J.; Karle, A.; Kelley, J. L.; Krasberg, M.; Landsman, H.; Maruyama, R.; Merck, M.; Montaruli, T.; Morse, R.; O'Murchadha, A.; Rodrigues, J. P.; Santander, M.; Toscano, S.; van Santen, J.; Weaver, Ch.; Wendt, C.; Westerhoff, S.; Whitehorn, N.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Griesel, T.; Koepke, L.; Kowarik, T.; Kroll, G.; Luenemann, J.; Piegsa, A.; Rothmaier, F.; Sander, H. -G.; Schatto, K.; Wiebe, K.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55099 Mainz, Germany. [Herquet, P.; Kohnen, G.] Univ Mons, B-7000 Mons, Belgium. [Bai, X.; Clem, J.; Evenson, P. A.; Gaisser, T. K.; Hussain, S.; Kuwabara, T.; Niessen, P.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Stoyanov, S.; Tilav, S.; Xu, C.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Bai, X.; Clem, J.; Evenson, P. A.; Gaisser, T. K.; Hussain, S.; Kuwabara, T.; Niessen, P.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Stoyanov, S.; Tilav, S.; Xu, C.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Ahlers, M.; Sarkar, S.] Univ Oxford, Dept Phys, Oxford OX1 3NP, England. [Abu-Zayyad, T.; Madsen, J.; Spiczak, G. M.; Tamburro, A.] Univ Wisconsin, Dept Phys, River Falls, WI 54022 USA. [Bohm, C.; Danninger, M.; Finley, C.; Hulth, P. O.; Hultqvist, K.; Johansson, H.; Seo, S. H.; Walck, C.] Stockholm Univ, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Bohm, C.; Danninger, M.; Finley, C.; Hulth, P. O.; Hultqvist, K.; Johansson, H.; Seo, S. H.; Walck, C.] Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden. [Cowen, D. F.; Meszaros, P.; Movit, S. M.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Cowen, D. F.; DeYoung, T.; Foerster, M. M.; Fox, B. D.; Ha, C.; Koskinen, D. J.; Lafebre, S.; Larson, M. J.; Meszaros, P.; Rutledge, D.; Slipak, A.; Stephens, G.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Botner, O.; Engdegard, O.; Hallgren, A.; Miller, J.; de los Heros, C. Perez; Taavola, H.] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden. [Auffenberg, J.; Becker, K. -H.; Bindig, D.; Fischer-Wasels, T.; Gurtner, M.; Helbing, K.; Kampert, K. -H.; Karg, T.; Kopper, S.; Naumann, U.; Posselt, J.; Schultes, A.; Semburg, B.] Univ Wuppertal, Dept Phys, D-42119 Wuppertal, Germany. [Alba, J. L. Bazo; Benabderrahmane, M. L.; Berdermann, J.; Bernardini, E.; Franke, R.; Gora, D.; Han, K.; Kislat, F.; Lauer, R.; Majumdar, P.; Middell, E.; Nahnhauer, R.; Schoenwald, A.; Spiering, C.; Stoessl, A.; Tosi, D.; Walter, M.; Wischnewski, R.] DESY, D-15735 Zeuthen, Germany. [Montaruli, T.] Univ Bari, I-70126 Bari, Italy. [Montaruli, T.] Sezione Ist Nazl Fis Nucl, Dipartimento Fis, I-70126 Bari, Italy. RP Ishihara, A (reprint author), Chiba Univ, Dept Phys, Chiba 2638522, Japan. EM aya@hepburn.s.chiba-u.ac.jp RI Taavola, Henric/B-4497-2011; Aguilar Sanchez, Juan Antonio/H-4467-2015; HAN, KyoungHoon/D-4588-2011; Wiebusch, Christopher/G-6490-2012; Maruyama, Reina/A-1064-2013; Kowalski, Marek/G-5546-2012; Sarkar, Subir/G-5978-2011; Beatty, James/D-9310-2011; Tamburro, Alessio/A-5703-2013; Botner, Olga/A-9110-2013; Hallgren, Allan/A-8963-2013; Tjus, Julia/G-8145-2012; Auffenberg, Jan/D-3954-2014; Koskinen, David/G-3236-2014 OI Ter-Antonyan, Samvel/0000-0002-5788-1369; Schukraft, Anne/0000-0002-9112-5479; Perez de los Heros, Carlos/0000-0002-2084-5866; Taavola, Henric/0000-0002-2604-2810; Buitink, Stijn/0000-0002-6177-497X; Carson, Michael/0000-0003-0400-7819; Hubert, Daan/0000-0002-4365-865X; Benabderrahmane, Mohamed Lotfi/0000-0003-4410-5886; Aguilar Sanchez, Juan Antonio/0000-0003-2252-9514; Wiebusch, Christopher/0000-0002-6418-3008; Maruyama, Reina/0000-0003-2794-512X; Sarkar, Subir/0000-0002-3542-858X; Beatty, James/0000-0003-0481-4952; Auffenberg, Jan/0000-0002-1185-9094; Koskinen, David/0000-0002-0514-5917 FU U.S. National Science Foundation-Office of Polar Programs; U.S. National Science Foundation-Physics Division; University of Wisconsin Almni Research Foundation; Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin Madison; Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy; National Energy Research Scientific Computing Center; Louisiana Optical Network Initiative (LONI) grid computing resources; National Science and Engineering Research Council of Canada; Swedish Research Council; Swedish Polar Research Secretariat; Swedish National Infrastructure for Computing (SNIC); Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF); Deutsche Forschungsgemeinschaft (DFG); Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO); FWO Odysseus programme; Flanders Institute to encourage scientific and technological research in industry (IWT); Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Japan Society for Promotion of Science (JSPS); Swiss National Science Foundation (SNSF), Switzerland; EU; Capes Foundation, Ministry of Education of Brazil FX We acknowledge the support from the following agencies: U.S. National Science Foundation-Office of Polar Programs, U.S. National Science Foundation-Physics Division, University of Wisconsin Almni Research Foundation, the Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin Madison, the Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy, and National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI) grid computing resources; National Science and Engineering Research Council of Canada; Swedish Research Council, Swedish Polar Research Secretariat, Swedish National Infrastructure for Computing (SNIC), and Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Deutsche Forschungsgemeinschaft (DFG), Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO), FWO Odysseus programme, Flanders Institute to encourage scientific and technological research in industry (IWT), Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Japan Society for Promotion of Science (JSPS); the Swiss National Science Foundation (SNSF), Switzerland; A. Gross acknowledges support by the EU Marie Curie OIF Program; J. P. Rodrigues acknowledges support by the Capes Foundation, Ministry of Education of Brazil. NR 41 TC 72 Z9 72 U1 1 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 24 PY 2011 VL 83 IS 9 AR 092003 DI 10.1103/PhysRevD.83.092003 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 767YS UT WOS:000290897000001 ER PT J AU Pauzauskie, PJ Crowhurst, JC Worsley, MA Laurence, TA Kilcoyne, ALD Wang, YM Willey, TM Visbeck, KS Fakra, SC Evans, WJ Zaug, JM Satcher, JH AF Pauzauskie, Peter J. Crowhurst, Jonathan C. Worsley, Marcus A. Laurence, Ted A. Kilcoyne, A. L. David Wang, Yinmin Willey, Trevor M. Visbeck, Kenneth S. Fakra, Sirine C. Evans, William J. Zaug, Joseph M. Satcher, Joe H., Jr. TI Synthesis and characterization of a nanocrystalline diamond aerogel SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE gigapascal; nanomaterials; phase transition; photonics; qubit ID MESOPOROUS COESITE; COHERENT DYNAMICS; CARBON; PRESSURE; SPIN; TEMPERATURE; COMPLEX; SILICA; PHASE AB Aerogel materials have myriad scientific and technological applications due to their large intrinsic surface areas and ultralow densities. However, creating a nanodiamond aerogel matrix has remained an outstanding and intriguing challenge. Here we report the high-pressure, high-temperature synthesis of a diamond aerogel from an amorphous carbon aerogel precursor using a laser-heated diamond anvil cell. Neon is used as a chemically inert, near-hydrostatic pressure medium that prevents collapse of the aerogel under pressure by conformally filling the aerogel's void volume. Electron and X-ray spectromicroscopy confirm the aerogel morphology and composition of the nanodiamond matrix. Time-resolved photoluminescence measurements of recovered material reveal the formation of both nitrogen- and silicon-vacancy point-defects, suggesting a broad range of applications for this nanocrystalline diamond aerogel. C1 [Pauzauskie, Peter J.; Crowhurst, Jonathan C.; Worsley, Marcus A.; Laurence, Ted A.; Wang, Yinmin; Willey, Trevor M.; Visbeck, Kenneth S.; Evans, William J.; Zaug, Joseph M.; Satcher, Joe H., Jr.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94551 USA. [Kilcoyne, A. L. David; Fakra, Sirine C.] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Pauzauskie, PJ (reprint author), Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA. EM peterpz@uw.edu RI Laurence, Ted/E-4791-2011; Willey, Trevor/A-8778-2011; Pauzauskie, Peter/A-1316-2014; Worsley, Marcus/G-2382-2014; Kilcoyne, David/I-1465-2013; Wang, Yinmin (Morris)/F-2249-2010 OI Laurence, Ted/0000-0003-1474-779X; Willey, Trevor/0000-0002-9667-8830; Worsley, Marcus/0000-0002-8012-7727; Wang, Yinmin (Morris)/0000-0002-7161-2034 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-05CH11231]; US Department of Energy by the Lawrence Livermore National Laboratory (LLNL) [DE-AC52-07NA27344]; LLNL FX The authors thank A. Goncharov for assistance in determining LHDAC temperatures from thermal emission data, as well as L. Hrubesh, L. Fried, D. Awschalom, M. Armstrong, C. Grant, T. Baumann, P. Weber, J. Bradley, I. Hutcheon, W. Goldstein, and G. Fox for valuable comments, and I. Hutcheon for access to SEM facilities. Use of the Advanced Light Source is supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-05CH11231. This work performed under the auspices of the US Department of Energy by the Lawrence Livermore National Laboratory (LLNL) under Contract DE-AC52-07NA27344. P.J.P. gratefully acknowledges funding from an E.O. Lawrence Fellowship at the LLNL. NR 33 TC 14 Z9 14 U1 3 U2 56 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 24 PY 2011 VL 108 IS 21 BP 8550 EP 8553 DI 10.1073/pnas.1010600108 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 768CB UT WOS:000290908000013 PM 21555550 ER PT J AU Lucks, JB Qi, L Mutalik, VK Wang, D Arkin, AP AF Lucks, Julius B. Qi, Lei Mutalik, Vivek K. Wang, Denise Arkin, Adam P. TI Versatile RNA-sensing transcriptional regulators for engineering genetic networks SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE gene networks; regulatory systems; orthogonal regulators ID ANTISENSE RNA; SYNTHETIC BIOLOGY; ESCHERICHIA-COLI; PLASMID PT181; IN-VIVO; EXPRESSION; RIBOREGULATORS; ATTENUATION; REPLICATION; ELEMENTS AB The widespread natural ability of RNA to sense small molecules and regulate genes has become an important tool for synthetic biology in applications as diverse as environmental sensing and metabolic engineering. Previous work in RNA synthetic biology has engineered RNA mechanisms that independently regulate multiple targets and integrate regulatory signals. However, intracellular regulatory networks built with these systems have required proteins to propagate regulatory signals. In this work, we remove this requirement and expand the RNA synthetic biology toolkit by engineering three unique features of the plasmid pT181 antisense-RNA-mediated transcription attenuation mechanism. First, because the antisense RNA mechanism relies on RNA-RNA interactions, we show how the specificity of the natural system can be engineered to create variants that independently regulate multiple targets in the same cell. Second, because the pT181 mechanism controls transcription, we show how independently acting variants can be configured in tandem to integrate regulatory signals and perform genetic logic. Finally, because both the input and output of the attenuator is RNA, we show how these variants can be configured to directly propagate RNA regulatory signals by constructing an RNA-meditated transcriptional cascade. The combination of these three features within a single RNA-based regulatory mechanism has the potential to simplify the design and construction of genetic networks by directly propagating signals as RNA molecules. C1 [Lucks, Julius B.; Qi, Lei; Wang, Denise; Arkin, Adam P.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Lucks, Julius B.] Miller Inst Basic Res Sci, Berkeley, CA 94720 USA. [Mutalik, Vivek K.; Arkin, Adam P.] Univ Calif Berkeley, Lawrence Berkeley Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Arkin, Adam P.] Calif Inst Quantitat Sci QB3, Berkeley, CA 94720 USA. RP Arkin, AP (reprint author), EO Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,MS Stanley 922, Berkeley, CA 94720 USA. EM aparkin@lbl.gov RI Arkin, Adam/A-6751-2008; Lucks, Julius/L-2801-2016; OI Arkin, Adam/0000-0002-4999-2931; Qi, Lei S/0000-0002-3965-3223; Mutalik, Vivek/0000-0001-7934-0400 FU Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231]; Synthetic Biology Engineering Research Center under National Science Foundation [04-570/0540879]; Miller Institute for Basic Research in Science FX The authors thank Richard Novick (Department of Microbiology, New York University School of Medicine, New York) for donating plasmid pT181; Ron Breaker, Blake Wiedenheft, and Vincent Rouilly for comments; Weston Whitaker and Jeff Skerker for discussions; and Richard Shan and Quintara Biosciences for assistance in plasmid sequencing. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract DE-AC02-05CH11231. This work was supported by the Synthetic Biology Engineering Research Center under National Science Foundation Grant 04-570/0540879. J.B.L. acknowledges the financial support of the Miller Institute for Basic Research in Science. NR 39 TC 106 Z9 106 U1 1 U2 27 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 24 PY 2011 VL 108 IS 21 BP 8617 EP 8622 DI 10.1073/pnas.1015741108 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 768CB UT WOS:000290908000025 PM 21555549 ER PT J AU Cipriano, R Kan, CE Graham, J Danielpour, D Stampfer, M Jackson, MW AF Cipriano, Rocky Kan, Charlene E. Graham, James Danielpour, David Stampfer, Martha Jackson, Mark W. TI TGF-beta signaling engages an ATM-CHK2-p53-independent RAS-induced senescence and prevents malignant transformation in human mammary epithelial cells SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE breast cancer; tumor suppressor ID ONCOGENE-INDUCED SENESCENCE; DNA-DAMAGE RESPONSE; BREAST-CANCER CELLS; GROWTH-FACTOR-BETA; C-MYC; CELLULAR-TRANSFORMATION; P16 INACTIVATION; P53; TUMORIGENESIS; ACTIVATION AB Oncogene-induced senescence (OIS), the proliferative arrest engaged in response to persistent oncogene activation, serves as an important tumor-suppressive barrier. We show here that finite lifespan human mammary epithelial cells (HMEC) undergo a p16/RB- and p53-independent OIS in response to oncogenic RAS that requires TGF-beta signaling. Suppression of TGF-beta signaling by expression of a dominant-negative TGF-beta type II receptor, use of a TGF-beta type I receptor inhibitor, or ectopic expression of MYC permitted continued proliferation upon RAS expression. Surprisingly, unlike fibroblasts, shRNA-mediated knockdown of ATM or CHK2 was unable to prevent RAS-mediated OIS, arguing that the DNA damage response is not required for OIS in HMEC. Abrogation of TGF-beta signaling not only allowed HMEC lacking p53 to tolerate oncogenic RAS but also conferred the capacity for anchorage-independent growth. Thus, the OIS engaged after dysregulated RAS expression provides an early barrier to malignant progression and is mediated by TGF-beta receptor activation in HMEC. Understanding the mechanisms that initiate and maintain OIS in epithelial cells may provide a foundation for future therapies aimed at reengaging this proliferative barrier as a cancer therapy. C1 [Cipriano, Rocky; Graham, James; Jackson, Mark W.] Case Western Reserve Univ, Dept Pathol, Cleveland, OH 44106 USA. [Kan, Charlene E.] Case Western Reserve Univ, Dept Genet, Cleveland, OH 44106 USA. [Danielpour, David; Jackson, Mark W.] Case Western Reserve Univ, Case Comprehens Canc Ctr, Cleveland, OH 44106 USA. [Stampfer, Martha] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Jackson, MW (reprint author), Case Western Reserve Univ, Dept Pathol, Cleveland, OH 44106 USA. EM mwj7@case.edu FU National Institutes of Health [T32CA059366]; Department of Defense [BC074072] FX This work was supported by National Institutes of Health Grant T32CA059366 (to R. C.) and Department of Defense Breast Cancer Research Program Grant BC074072 (to M.W.J). NR 42 TC 41 Z9 43 U1 3 U2 5 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 24 PY 2011 VL 108 IS 21 BP 8668 EP 8673 DI 10.1073/pnas.1015022108 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 768CB UT WOS:000290908000034 PM 21555587 ER PT J AU Schaefer, JK Rocks, SS Zheng, W Liang, LY Gu, BH Morel, FMM AF Schaefer, Jeffra K. Rocks, Sara S. Zheng, Wang Liang, Liyuan Gu, Baohua Morel, Francois M. M. TI Active transport, substrate specificity, and methylation of Hg(II) in anaerobic bacteria SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE mercury bioavailability; mercury detoxification ID SULFATE-REDUCING BACTERIA; HEAVY-METAL RESISTANCE; FRESH-WATER SEDIMENTS; MERCURY METHYLATION; ESCHERICHIA-COLI; DEGRADATION; ECOSYSTEMS; TOXICOLOGY; SALINITY; SAMPLES AB The formation of methylmercury (MeHg), which is biomagnified in aquatic food chains and poses a risk to human health, is effected by some iron-and sulfate-reducing bacteria (FeRB and SRB) in anaerobic environments. However, very little is known regarding the mechanism of uptake of inorganic Hg by these organisms, in part because of the inherent difficulty in measuring the intracellular Hg concentration. By using the FeRB Geobacter sulfurreducens and the SRB Desulfovibrio desulfuricans ND132 as model organisms, we demonstrate that Hg(II) uptake occurs by active transport. We also establish that Hg(II) uptake by G. sulfurreducens is highly dependent on the characteristics of the thiols that bind Hg(II) in the external medium, with some thiols promoting uptake and methylation and others inhibiting both. The Hg(II) uptake system of D. desulfuricans has a higher affinity than that of G. sulfurreducens and promotes Hg methylation in the presence of stronger complexing thiols. We observed a tight coupling between Hg methylation and MeHg export from the cell, suggesting that these two processes may serve to avoid the build up and toxicity of cellular Hg. Our results bring up the question of whether cellular Hg uptake is specific for Hg(II) or accidental, occurring via some essential metal importer. Our data also point at Hg(II) complexation by thiols as an important factor controlling Hg methylation in anaerobic environments. C1 [Schaefer, Jeffra K.; Rocks, Sara S.; Morel, Francois M. M.] Princeton Univ, Dept Geosci, Princeton, NJ 08544 USA. [Zheng, Wang; Liang, Liyuan; Gu, Baohua] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Morel, FMM (reprint author), Princeton Univ, Dept Geosci, Princeton, NJ 08544 USA. EM morel@princeton.edu RI Gu, Baohua/B-9511-2012; Liang, Liyuan/O-7213-2014 OI Gu, Baohua/0000-0002-7299-2956; Liang, Liyuan/0000-0003-1338-0324 FU Office of Biological and Environmental Research, Office of Science, US Department of Energy; US Department of Energy [DE-AC05-00OR22725] FX We thank C. Cobb-Adams for the analysis of Hg and MeHg at Princeton University. We also thank J. Jay and T. Barkay for helpful comments in review of this manuscript. This research was supported in part by the Office of Biological and Environmental Research, Office of Science, US Department of Energy, as part of the Mercury Science Focus Area Program at Oak Ridge National Laboratory, which is managed by UT-Battelle, LLC, for the US Department of Energy under contract DE-AC05-00OR22725. NR 33 TC 82 Z9 88 U1 5 U2 110 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 24 PY 2011 VL 108 IS 21 BP 8714 EP 8719 DI 10.1073/pnas.1105781108 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 768CB UT WOS:000290908000042 PM 21555571 ER PT J AU Kakar, S Sturms, R Tiffany, A Nix, JC DiSpirito, AA Hargrove, MS AF Kakar, Smita Sturms, Ryan Tiffany, Andrea Nix, Jay C. DiSpirito, Alan A. Hargrove, Mark S. TI Crystal Structures of Parasponia and Trema Hemoglobins: Differential Heme Coordination Is Linked to Quaternary Structure SO BIOCHEMISTRY LA English DT Article ID PLANT HEMOGLOBIN; HEXACOORDINATE HEMOGLOBINS; RESPIRATION; ADAPTATION; EXPRESSION; CYTOGLOBIN; EVOLUTION; HYPOXIA; SURFACE; NO AB Hemoglobins from the plants Parasponia andersonii (ParaHb) and Trema tomentosa (TremaHb) are 93% identical in primary structure but differ in oxygen binding constants in accordance with their distinct physiological functions. Additionally, these proteins are dimeric, and ParaHb exhibits the unusual property of having different heme redox potentials for each subunit. To investigate how these hemoglobins could differ in function despite their shared sequence identity and to determine the cause of subunit heterogeneity in ParaHb, we have measured their crystal structures in the ferric oxidation state. Furthermore, we have made a monomeric ParaHb mutant protein (I43N) and measured its ferrous/ferric heme redox potential to test the hypothesized link between quaternary structure and heme heterogeneity in wild-type ParaHb. Our results demonstrate that TremaHb is a symmetric dimeric hemoglobin similar to other class 1 nonsymbiotic plant hemoglobins but that ParaHb has structurally distinct heme coordination in each of its two subunits that is absent in the monomeric I43N mutant protein. A mechanism for achieving structural heterogeneity in ParaHb in which the Ile(101(F4)) side chain contacts the proximal His(105(F8)) in one subunit but not the other is proposed. These results are discussed in the context of the evolution of plant oxygen transport hemoglobins, and other potential functions of plant hemoglobins. C1 [Kakar, Smita; Sturms, Ryan; Tiffany, Andrea; DiSpirito, Alan A.; Hargrove, Mark S.] Iowa State Univ, Dept Biochem Biophys & Mol Biol, Ames, IA 50011 USA. [Nix, Jay C.] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Hargrove, MS (reprint author), Iowa State Univ, Dept Biochem Biophys & Mol Biol, Ames, IA 50011 USA. EM msh@iastate.edu NR 36 TC 7 Z9 7 U1 0 U2 4 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD MAY 24 PY 2011 VL 50 IS 20 BP 4273 EP 4280 DI 10.1021/bi2002423 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 763XW UT WOS:000290594000006 PM 21491905 ER PT J AU Harper, JC Lopez, DM Larkin, EC Economides, MK McIntyre, SK Alam, TM Tartis, MS Werner-Washburne, M Brinker, CJ Brozik, SM Wheeler, DR AF Harper, Jason C. Lopez, DeAnna M. Larkin, Elizabeth C. Economides, Megan K. McIntyre, Sarah K. Alam, Todd M. Tartis, Michaelann S. Werner-Washburne, Margaret Brinker, C. Jeffrey Brozik, Susan M. Wheeler, David R. TI Encapsulation of S. cerevisiae in Poly(glycerol) Silicate Derived Matrices: Effect of Matrix Additives and Cell Metabolic Phase on Long-Term Viability and Rate of Gene Expression SO CHEMISTRY OF MATERIALS LA English DT Article DE living hybrid biomaterials; bioencapsulation; glycerol modified silanes; cell viability; cell metabolic phase; whole-cell based biosensors ID RECOMBINANT ESCHERICHIA-COLI; SOL-GEL ENCAPSULATION; SACCHAROMYCES-CEREVISIAE; LIVING BACTERIA; SI-29 NMR; BIOSENSOR; YEAST; PERSPECTIVES; BIOMOLECULES; SELECTIVITY AB Bioencapsulation of living cells into silica materials derived from the sol gel process has resulted in novel hybrid living materials with exciting functionalities. Despite the many successes in this field, long-term viability and activity of the encapsulated cells remain a significant obstacle to producing practical and robust devices,.e.g., whole-cell-based biosensors. We report the first study on the effects of various media additives and the metabolic phase of encapsulated cells on long-term viability and the rate of inducible gene expression. Saccharomyces cerevisiae (S. cerevisiae) cells, genetically engineered to produce yellow fluorescent protein (YFP) in response to galactose, were encapsulated in poly(glycerol) silicate derived matrices. Surprisingly, we find that addition of media components to the glycerol-silica matrix adversely impacted long-term viability in all cases studied, with a 1.3, 1.4, or 5.4 fold decrease in viability after only 9 days of storage in matrices containing yeast peptone dextrose (YPD), yeast peptone (YP, no glucose), or Synthetic Complete (SC) +2% glucose media, respectively. These findings are attributed to the media components inducing exit of the cells from the more robust quiescent state, and the metabolic production of toxic byproducts. Encapsulated cells from exponential culture exhibited inducible reporter gene expression rates approximately 33% higher than cells from stationary cultures. Addition of media components to the silica matrix increased gene expression rates under certain conditions. These results further elaborate on other silica matrix encapsulated living cell studies, and provide important design parameters for developing effective living cell-based biosensors for case-specific detection applications. C1 [Harper, Jason C.; Economides, Megan K.; Brinker, C. Jeffrey; Brozik, Susan M.] Univ New Mexico, Dept Chem & Nucl Engn, Albuquerque, NM 87131 USA. [Werner-Washburne, Margaret; Brinker, C. Jeffrey] Univ New Mexico, Dept Mol Genet & Microbiol, Albuquerque, NM 87131 USA. [Larkin, Elizabeth C.; Tartis, Michaelann S.] New Mexico Inst Min & Technol, Dept Chem Engn, Socorro, NM 87801 USA. [Harper, Jason C.; Lopez, DeAnna M.; McIntyre, Sarah K.; Alam, Todd M.; Brinker, C. Jeffrey; Brozik, Susan M.; Wheeler, David R.] Sandia Natl Labs, Albuquerque, NM 87106 USA. RP Brinker, CJ (reprint author), Univ New Mexico, Dept Chem & Nucl Engn, Albuquerque, NM 87131 USA. EM cjbrink@sandia.gov; smbrozi@sandia.gov; drwheel@sandia.gov FU Defense Treat Reduction Agency (DTRA) [B0844671]; DoE NNSA Office for Nonproliferation Research and Development [NA-22]; Sandia Lab Directed Research and Development program; Air Force Office of Scientific Research [FA 9550-10-1-0054]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was funded by the Defense Treat Reduction Agency (DTRA) Chem. Bio. Basic Research Program grant B0844671, the DoE NNSA Office for Nonproliferation Research and Development (NA-22), and the Sandia Lab Directed Research and Development program. CJB acknowledges funding from the Air Force Office of Scientific Research grant FA 9550-10-1-0054, and the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 53 TC 16 Z9 16 U1 2 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 J9 CHEM MATER JI Chem. Mat. PD MAY 24 PY 2011 VL 23 IS 10 BP 2555 EP 2564 DI 10.1021/cm103525u PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 763YD UT WOS:000290594700009 ER PT J AU Babu, GS Valant, M Page, K Llobet, A Kolodiazhnyi, T Axelsson, AK AF Babu, Gunda Santosh Valant, Matjaz Page, Katharine Llobet, Anna Kolodiazhnyi, Taras Axelsson, Anna-Karin TI New (Bi1.88Fe0.12)(Fe1.42Te0.58)O-6.87 Pyrochlore with Spin-Glass Transition SO CHEMISTRY OF MATERIALS LA English DT Article DE Bi-pyrochlore; displacive disorder; Raman spectra; dielectric relaxation; spin glass ID X-RAY-DIFFRACTION; DIELECTRIC-PROPERTIES; DISPLACIVE DISORDER; CRYSTAL-CHEMISTRY; OXIDE PYROCHLORES; PHASE-FORMATION; RELAXATION; SPECTRA AB The synthesized (Bi1.88Fe0.12)(Fe1.42Te0.58)O-6.87 is characterized with so far the highest Fe content among pyrochlores. Consequently, it exhibits a strong spin-glass magnetic transition at around 20 K The dielectric relaxation in the same temperature range originates from multiwall hopping of the displaced ions on A and O' sites. The displacement was confirmed with the structural analysis of the pyrochlore using Rietveld refinement on joint neutron and X-ray diffraction data. At room temperature, the pyrochlore exhibits a cubic Fd (3) over barm symmetry (a = 10.38804 (13) angstrom) with Fe3+ ions sharing A and B structural sites. The refined results indicate on a displacive disorder with A-site positioned at 96g and O' positioned at 32e. The lattice vibrational analysis using Raman spectra is in agreement with the displacive disorder of the pyrochlore. C1 [Babu, Gunda Santosh; Valant, Matjaz] Univ Nova Gorica, Mat Res Lab, Nova Gorica 5000, Slovenia. [Page, Katharine; Llobet, Anna] Los Alamos Natl Lab, Lujan Neutron Scattering Ctr, Los Alamos, NM 87545 USA. [Kolodiazhnyi, Taras] Natl Inst Mat Sci, Tsukuba, Ibaraki 3050044, Japan. [Axelsson, Anna-Karin] Univ London Imperial Coll Sci Technol & Med, Dept Mat, London SW7 2AZ, England. RP Valant, M (reprint author), Univ Nova Gorica, Mat Res Lab, Vipavska 13, Nova Gorica 5000, Slovenia. EM matjaz.valant@ung.si RI gunda, santosh babu/B-1499-2010; Page, Katharine/C-9726-2009; Llobet, Anna/B-1672-2010; KOLODIAZHNYI, Taras/H-2860-2011; Lujan Center, LANL/G-4896-2012; axelsson, anna-karin/E-6884-2013; OI Page, Katharine/0000-0002-9071-3383; Valant, Matjaz/0000-0003-4842-5676; Kolodiazhnyi, Taras/0000-0002-9630-9461 FU DOE Office of Basic Energy Sciences; DOE [DE-AC52-06NA25396] FX The authors thank Hiroya Sakurai for valuable comments on spin-glass properties. This work has benefited from the use of HIPD at the Lujan Center at Los Alamos Neutron Science Center, funded by DOE Office of Basic Energy Sciences. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE Contract DE-AC52-06NA25396. NR 49 TC 14 Z9 14 U1 2 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAY 24 PY 2011 VL 23 IS 10 BP 2619 EP 2625 DI 10.1021/cm200281z PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 763YD UT WOS:000290594700017 ER PT J AU Schutz-Sikma, EA Joshi, HM Ma, Q MacRenaris, KW Eckermann, AL Dravid, VP Meade, TJ AF Schutz-Sikma, Elise A. Joshi, Hrushikesh M. Ma, Qing MacRenaris, Keith W. Eckermann, Amanda L. Dravid, Vinayak P. Meade, Thomas J. TI Probing the Chemical Stability of Mixed Ferrites: Implications for Magnetic Resonance Contrast Agent Design SO CHEMISTRY OF MATERIALS LA English DT Article DE MRI; ferrite; nanoparticle; leaching; magnetic properties ID IRON-OXIDE NANOPARTICLES; ABSORPTION FINE-STRUCTURE; MRI CONTRAST; BIOMEDICAL APPLICATIONS; MFE2O4 M; COBALT; SPINEL; SIZE; NANOCRYSTALS; MN AB Nanomaterials with mixed composition, in particular magnetic spinel ferrites, are emerging as efficient contrast agents for magnetic resonance imaging. Many factors, including size, composition, atomic structure, and surface properties, are crucial in the design of such nanoparticle-based probes because of their influence on the magnetic properties. Silica-coated iron oxide (IO-SiO(2)) and cobalt ferrite (CoIO-SiO(2)) nanoparticles were synthesized using standard high-temperature thermal decomposition and base-catalyzed water-in-oil microemulsion techniques. Under neutral aqueous conditions, it was found that 50-75% of the cobalt content in the CoIO-SiO(2) nanoparticles leached out the core structure. Leaching caused a 7.2-fold increase in the longitudinal relaxivity and an increase in the saturation magnetization from similar to 48 to similar to 65 emu/g of the core. X-ray absorption fine structure studies confirmed that the atomic structure of the ferrite core was altered following leaching, while transmission electron microscopy and dynamic light scattering confirmed that the morphology and size of the nanoparticle remained unchanged. The CoIO-SiO(2) nanoparticles converted from a partially inverted spinel cation arrangement (unleached state) to an inverse spine arrangement (leached state). The control IO-SiO(2) nanoparticles remained stable with no change in the structure and negligible changes in the magnetic behavior. This detailed analysis highlights how important understanding the properties of nanomaterials is in the development of reliable agents for diagnostic and therapeutic applications. C1 [Schutz-Sikma, Elise A.; MacRenaris, Keith W.; Eckermann, Amanda L.; Meade, Thomas J.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Joshi, Hrushikesh M.; Dravid, Vinayak P.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Ma, Qing] Northwestern Univ, Argonne Natl Lab, Synchrotron Res Ctr, DND CAT, Argonne, IL 60439 USA. RP Meade, TJ (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM tmeade@northwestern.edu RI Dravid, Vinayak/B-6688-2009; Eckermann, Amanda/A-3224-2013 FU Center for Cancer Nanotechnology Excellence (CCNE) initiative of the National Institutes of Health's National Cancer Institute [U54CA119341]; National Institute of Biomedical Imaging and Bioengineering [1RO1EB005866-01]; E. I. DuPont de Nemours Co.; Dow Chemical Co.; State of Illinois; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The work performed at Northwestern University was supported by the Center for Cancer Nanotechnology Excellence (CCNE) initiative of the National Institutes of Health's National Cancer Institute under Award U54CA119341 and the National Institute of Biomedical Imaging and Bioengineering under Award 1RO1EB005866-01. The DND-CAT located at the Advanced Photon Source (APS) is supported by E. I. DuPont de Nemours & Co., The Dow Chemical Co., and the State of Illinois. Use of the APS was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. The SQUID measurements were performed by Oleksandr Chernyashevskyy in the Magnetic and Physical Properties Measurement Facility at Northwestern University. TEM analysis was performed in the EPIC/NIFTI facility of the NUANCE Center at Northwestern University. Special thanks go to Collin Morris in the Chemistry Department at Northwestern University for help with the ferrite crystallographic models. NR 59 TC 29 Z9 29 U1 3 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 J9 CHEM MATER JI Chem. Mat. PD MAY 24 PY 2011 VL 23 IS 10 BP 2657 EP 2664 DI 10.1021/cm200509g PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 763YD UT WOS:000290594700022 PM 21603070 ER PT J AU Aad, G Abbott, B Abdallah, J Abdelalim, AA Abdesselam, A Abdinov, O Abi, B Abolins, M Abramowicz, H Abreu, H Acerbi, E Acharya, BS Adams, DL Addy, TN Adelman, J Aderholz, M Adomeit, S Adragna, P Adye, T Aefsky, S Aguilar-Saavedra, A Aharrouche, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akdogan, T Akesson, TP Akimoto, G Akimov, AV Akiyama, A Alam, MS Alam, MA Albrand, S Aleksa, M Aleksandrov, IN Aleppo, M Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Aliyev, M Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alviggi, MG Amako, K Amaral, P Amelung, C Ammosov, VV Amorim, A Amoros, G Amram, N Anastopoulos, C Andeen, T Anders, CF Anderson, KJ Andreazza, A Andrei, V Andrieux, ML Anduaga, XS Angerami, A Anghinolfi, F Anjos, N Annovi, A Antonaki, A Antonelli, M Antonelli, S Antonov, A Antos, J Anulli, F Aoun, S Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Archambault, JP Arfaoui, S Arguin, JF Arik, E Arik, M Armbruster, AJ Arnaez, O Arnault, C Artamonov, A Artoni, G Arutinov, D Asai, S Asfandiyarov, R Ask, S Asman, B Asquith, L Assamagan, K Astbury, A Astvatsatourov, A Atoian, G Aubert, B Auerbach, B Auge, E Augsten, K Aurousseau, M Austin, N Avramidou, R Axen, D Ay, C Azuelos, G Azuma, Y Baak, MA Baccaglioni, G Bacci, C Bach, AM Bachacou, H Bachas, K Bachy, G Backes, M Backhaus, M Badescu, E Bagnaia, P Bahinipati, S Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, MD Baker, S Pedrosa, FBD Banas, E Banerjee, P Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Barashkou, A Galtieri, AB Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barr, AJ Barreiro, F da Costa, JBG Barrillon, P Bartoldus, R Barton, AE Bartsch, D Bartsch, V Bates, RL Batkova, L Batley, JR Battaglia, A Battistin, M Battistoni, G Bauer, F Bawa, HS Beare, B Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Beckingham, M Becks, KH Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Begel, M Harpaz, SB Behera, PK Beimforde, M Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellina, F Bellomo, G Bellomo, M Belloni, A Beloborodova, O Belotskiy, K Beltramello, O Ben Ami, S Benary, O Benchekroun, D Benchouk, C Bendel, M Benedict, BH Benekos, N Benhammou, Y Benjamin, DP Benoit, M Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernardet, K Bernat, P Bernhard, R Bernius, C Berry, T Bertin, A Bertinelli, F Bertolucci, F Besana, MI Besson, N Bethke, S Bhimji, W Bianchi, RM Bianco, M Biebel, O Bieniek, SP Biesiada, J Biglietti, M Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biscarat, C Bitenc, U Black, KM Blair, RE Blanchard, JB Blanchot, G Blocker, C Blocki, J Blondel, A Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VB Bocci, A Boddy, CR Boehler, M Boek, J Boelaert, N Boser, S Bogaerts, JA Bogdanchikov, A Bogouch, A Bohm, C Boisvert, V Bold, T Boldea, V Bona, M Bondarenko, VG Boonekamp, M Boorman, G Booth, CN Booth, P Bordoni, S Borer, C Borisov, A Borissov, G Borjanovic, I Borroni, S Bos, K Boscherini, D Bosman, M Boterenbrood, H Botterill, D Bouchami, J Boudreau, J Bouhova-Thacker, EV Boulahouache, C Bourdarios, C Bousson, N Boveia, A Boyd, J Boyko, IR Bozhko, NI Bozovic-Jelisavcic, I Bracinik, J Braem, A Brambilla, E Branchini, P Brandenburg, GW Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brelier, B Bremer, J Brenner, R Bressler, S Breton, D Brett, ND Bright-Thomas, PG Britton, D Brochu, FM Brock, I Brock, R Brodbeck, TJ Brodet, E Broggi, F Bromberg, C Brooijmans, G Brooksb, WK Brown, G Brubaker, E de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Buanes, T Bucci, F Buchanan, J Buchanan, NJ Buchholz, P Buckingham, RM Buckley, AG Buda, SI Budagov, IA Budick, B Buescher, V Bugge, L Buira-Clark, D Buis, EJ Bulekov, O Bunse, M Buran, T Burckhart, H Burdin, S Burgess, T Burke, S Busato, E Bussey, P Buszello, CP Butin, F Butler, B Butler, JM Buttar, CM Butterworth, JM Buttinger, W Byatt, T Urban, SC Caccia, M Caforio, D Cakir, O Calafiura, P Calderini, G Calfayan, P Calkins, R Caloba, LP Caloi, R Calvet, D Calvet, S Toro, RC Camard, A Camarri, P Cambiaghi, M Cameron, D Cammin, J Campana, S Campanelli, M Canale, V Canelli, F Canepa, A Cantero, J Capasso, L Garrido, MDMC Caprini, I Caprini, M Capriotti, D Capua, M Caputo, R Caramarcu, C Cardarelli, R Carli, T Carlino, G Carminati, L Caron, B Caron, S Carpentieri, C Montoya, GDC Carter, AA Carter, JR Carvalho, J Casadei, D Casado, MP Cascella, M Caso, C Hernandez, AMC Castaneda-Miranda, E Gimenez, VC Castro, NF Cataldi, G Cataneo, F Catinaccio, A Catmore, JR Cattai, A Cattani, G Caughron, S Cauz, D Cavallari, A Cavalleri, P Cavalli, D Cavalli-Sforza, M Cavasinni, V Cazzato, A Ceradini, F Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cetin, SA Cevenini, F Chafaq, A Chakraborty, D Chan, K Chapleau, B Chapman, JD Chapman, JW Chareyre, E Charlton, DG Chavda, V Cheatham, S Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, L Chen, S Chen, T Chen, X Cheng, S Cheplakov, A Chepurnov, VF El Moursli, RC Chernyatin, V Cheu, E Cheung, SL Chevalier, L Chevallier, F Chiefari, G Chikovani, L Childers, JT Chilingarov, A Chiodini, G Chizhov, MV Choudalakis, G Chouridou, S Christidi, IA Christov, A Chromek-Burckhart, D Chu, ML Chudoba, J Ciapetti, G Ciba, K Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciobotaru, MD Ciocca, C Ciocio, A Cirilli, M Ciubancan, M Clark, A Clark, PJ Cleland, W Clemens, JC Clement, B Clement, C Clifft, RW Coadou, Y Cobal, M Coccaro, A Cochran, J Coe, P Cogan, JG Coggeshall, J Cogneras, E Cojocaru, CD Colas, J Colijn, AP Collard, C Collins, NJ Collins-Tooth, C Collot, J Colon, G Coluccia, R Comune, G Muino, PC Coniavitis, E Conidi, MC Consonni, M Constantinescu, S Conta, C Conventi, F Cook, J Cooke, M Cooper, BD Cooper-Sarkar, AM Cooper-Smith, NJ Copic, K Cornelissen, T Corradi, M Corriveau, F Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Costin, T Cote, D Torres, RC Courneyea, L Cowan, G Cowden, C Cox, BE Cranmer, K Crescioli, F Cristinziani, M Crosetti, G Crupi, R Crepe-Renaudin, S Almenar, CC Donszelmann, TC Cuneo, S Curatolo, M Curtis, CJ Cwetanski, P Czirr, H Czyczula, Z D'Auria, S D'Onofrio, M D'Orazio, A Mello, ADG Da Silva, PVM Da Via, C Dabrowski, W Dahlhoff, A Dai, T Dallapiccola, C Dallison, SJ Dam, M Dameri, M Damiani, DS Danielsson, HO Dankers, R Dannheim, D Dao, V Darbo, G Darlea, GL Daum, C Dauvergne, JP Davey, W Davidek, T Davidson, N Davidson, R Davies, M Davison, AR Dawe, E Dawson, I Dawson, JW Daya, RK De, K de Asmundis, R De Castro, S Salgado, PEDF De Cecco, S de Graat, J De Groot, N de Jong, P De La Taille, C De la Torre, H De Lotto, B De Mora, L De Nooij, L Branco, MD De Pedis, D De Saintignon, P De Salvo, A De Sanctis, U De Santo, A De Regie, JBD Dean, S Dedovich, DV Degenhardt, J Dehchar, M Deile, M Del Papa, C Del Peso, J Del Prete, T Dell'Acqua, A Dell'Asta, L Della Pietra, M Della Volpe, D Delmastro, M Delpierre, P Delruelle, N Delsart, PA Deluca, C Demers, S Demichev, M Demirkoz, B Deng, J Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Devetak, E Deviveiros, PO Dewhurst, A DeWilde, B Dhaliwal, S Dhullipudi, R Di Ciaccio, A Di Ciaccio, L Di Girolamo, A Di Girolamo, B Di Luise, S Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Diaz, MA Diblen, F Diehl, EB Dietl, H Dietrich, J Dietzsch, TA Diglio, S Yagci, KD Dingfelder, J Dionisi, C Dita, P Dita, S Dittus, F Djama, F Djilkibaev, R Djobava, T do Vale, B Wemans, ADV Doan, TKO Dobbs, M Dobinson, R Dobos, D Dobson, E Dobson, M 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Evangelakou, D Evans, H Fabbri, L Fabre, C Facius, K Fakhrutdinov, RM Falciano, S Falou, AC Fang, Y Fanti, M Farbin, A Farilla, A Farley, J Farooque, T Farrington, SM Farthouat, P Fasching, D Fassnacht, P Fassouliotis, D Fatholahzadeh, B Favareto, A Fayard, L Fazio, S Febbraro, R Federic, P Fedin, OL Fedorko, I Fedorko, W Fehling-Kaschek, M Feligioni, L Fellmann, D Felzmann, CU Feng, C Feng, EJ Fenyuk, AB Ferencei, J Ferland, J Fernandes, B Fernando, W Ferrag, S Ferrando, J Ferrara, V Ferrari, A Ferrari, P Ferrari, R Ferrer, A Ferrer, ML Ferrere, D Ferretti, C Parodi, AF Fiascaris, M Fiedler, F Filipcic, A Filippas, A Filthaut, F Fincke-Keeler, M Fiolhais, MCN Fiorini, L Firan, A Fischer, G Fischer, P Fisher, MJ Fisher, SM Flammer, J Flechl, M Fleck, I Fleckner, J Fleischmann, P Fleischmann, S Flick, T Castillo, LRF Flowerdew, MJ Fohlisch, F Fokitis, M Martin, TF Forbush, DA Formica, A Forti, A Fortin, D Foster, JM Fournier, D Foussat, A Fowler, AJ Fowler, K Fox, H Francavilla, P 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CA ATLAS Collaboration TI A search for new physics in dijet mass and angular distributions in pp collisions at root s=7 TeV measured with the ATLAS detector SO NEW JOURNAL OF PHYSICS LA English DT Article ID PARTON DISTRIBUTIONS; HADRON COLLIDERS; CHIRAL COLOR; QCD; QUARK AB A search for new interactions and resonances produced in LHC proton-proton (pp) collisions at a centre-of-mass energy root s = 7 TeV was performed with the ATLAS detector. Using a dataset with an integrated luminosity of 36 pb(-1), dijet mass and angular distributions were measured up to dijet masses of similar to 3.5 TeV and were found to be in good agreement with Standard Model predictions. This analysis sets limits at 95% CL on various models for new physics: an excited quark is excluded for mass between 0.60 and 2.64 TeV, an axigluon hypothesis is excluded for axigluon masses between 0.60 and 2.10 TeV and quantum black holes are excluded in models with six extra space-time dimensions for quantum gravity scales between 0.75 and 3.67 TeV. Production cross section limits as a function of dijet mass are set using a simplified Gaussian signal model to facilitate comparisons with other hypotheses. Analysis of the dijet angular distribution using a novel technique simultaneously employing the dijet mass excludes quark contact interactions with a compositeness scale 3 below 9.5 TeV. 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P.; Vazeille, F.; Viret, S.] Clermont Univ, Lab Phys Corpusculaire, Aubiere, France. [Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Febbraro, R.; Ghodbane, N.; Gris, P. L. Y.; Guicheney, C.; Pallin, D.; Podlyski, F.; Santoni, C.; Says, L. P.; Vazeille, F.; Viret, S.] Univ Clermont Ferrand, Aubiere, France. [Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Febbraro, R.; Ghodbane, N.; Gris, P. L. Y.; Guicheney, C.; Pallin, D.; Podlyski, F.; Santoni, C.; Says, L. P.; Vazeille, F.; Viret, S.] IN2P3, CNRS, Aubiere, France. [Angerami, A.; Brooijmans, G.; Dodd, J.; Guo, J.; Hughes, E. W.; Mateos, D. Lopez; Parsons, J. A.; Penson, A.; Spano, F.; Urbaniec, D.; Williams, E.; Wulf, E.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Dam, M.; Driouichi, C.; Facius, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Klinkby, E. B.; Lundquist, J.; Rensch, B.; Simonyan, M.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Mastroberardino, A.; Morello, G.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Cosenza, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Morello, G.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Bold, T.; Ciba, K.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Idzik, M.; Jelen, K.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Rulikowska-Zarebska, E.; Toczek, B.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa; Malecki, P.; Olszewski, A.; Olszowska, J.; Richter-Was, E.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Daya, R. 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F.; Prudent, X.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Ebenstein, W. L.; Fowler, A. J.; Ko, B. R.; Oh, S. H.; Wang, C.; Yamaoka, J.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; O'Brien, B. J.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Griesmayer, E.] Fachhsch Wiener Neustadt, Wiener Neustadt, Austria. [Annovi, A.; Antonelli, M.; Bilokon, H.; Cerutti, F.; Curatolo, M.; Esposito, B.; Ferrer, M. L.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.; Wen, M.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Bell, P. J.; Bell, W. H.; Berglund, E.; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Efthymiopoulos, I.; Ferrere, D.; Gadomski, S.; Navarro, J. E. 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G.] Georgian Acad Sci, Inst Phys, GE-380077 Tbilisi, Rep of Georgia. [Chikovani, L.; Djobava, T.; Khubua, J.; Magradze, E.; Mchedlidze, G.; Mosidze, M.; Tskhadadze, E. G.] Georgian Acad Sci, HEP Inst, GE-380060 Tbilisi, Rep of Georgia. [Chikovani, L.; Djobava, T.; Khubua, J.; Magradze, E.; Mchedlidze, G.; Mosidze, M.; Tskhadadze, E. G.] Tbilisi State Univ, GE-380086 Tbilisi, Rep of Georgia. [Astvatsatourov, A.; Dueren, M.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-6300 Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Gemmell, A.; Kenyon, M.; McGlone, H.; Moraes, A.; O'Shea, V.; Barrer, C. Oropeza; Pickford, A.; Robson, A.; Saxon, D. H.; Shaw, C.; Smith, K. M.; St Denis, R. D.; Steele, G.; Stewart, G. A.; Thompson, A. S.; Wraight, K.; Wright, C.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Ay, C.; Blumenschein, U.; Brandt, O.; Erdmann, J.; Evangelakou, D.; George, M.; Grosse-Knetter, J.; Guindon, S.; Haller, J.; Henrichs, A.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Mann, A.; Meyer, J.; Quadt, A.; Roe, A.; Shabalina, E.; Uhrmacher, M.; Weber, P.; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Andrieux, M-L; Clement, B.; Collot, J.; Crepe-Renaudin, S.; de Saintignon, P.; Delsart, P. A.; Donini, J.; Dzahini, D.; Hostachy, J-Y; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Martin, Ph; Polci, F.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Andrieux, M-L; Clement, B.; Collot, J.; Crepe-Renaudin, S.; de Saintignon, P.; Delsart, P. A.; Donini, J.; Dzahini, D.; Hostachy, J-Y; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Martin, Ph; Polci, F.; Stark, J.; Sun, X.; Trocme, B.] IN2P3, CNRS, Grenoble, France. [Albrand, S.; Andrieux, M-L; Clement, B.; Collot, J.; Crepe-Renaudin, S.; de Saintignon, P.; Delsart, P. A.; Donini, J.; Dzahini, D.; Hostachy, J-Y; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Martin, Ph; Polci, F.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Brandenburg, G. W.; Franklin, M.; Hurst, P.; Huth, J.; Jeanty, L.; Kagan, M.; Outschoorn, V. Martinez; Mercurio, K. M.; Mills, C.; Moed, S.; Morii, M.; Prasad, S.; Smith, B. C.; Zevi della Porta, G.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Childers, J. T.; Dietzsch, T. A.; Foehlisch, F.; Geweniger, C.; Hanke, P.; Henke, M.; Khomich, A.; Kluge, E-E; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H-C; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Radescu, V.; Schaetzel, S.; Schoening, A.] Heidelberg Univ, Inst Phys, D-6900 Heidelberg, Germany. [Abdesselam, A.; Kugel, A.; Maenner, R.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, D-6800 Mannheim, Germany. [Ohsugi, T.] Hiroshima Univ, Fac Sci, Hiroshima 730, Japan. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Jain, V.; Luehring, F.; Marino, C. P.; Ogren, H.; Penwell, J.; Price, D.; Rust, D. R.; Whittington, D.; Yang, Y.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Epp, B.; Jussel, P.; Kneringer, E.; Kuhn, D.; Rudolph, G.] Leopold Franzens Univ, Inst Astro Teilchenphys, Innsbruck, Austria. [Behera, P. K.; Limper, M.; Mallik, U.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; Dudziak, F.; Lebedev, A.; Mete, A. S.; Meyer, W. T.; Nelson, A.; Prell, S.; Rosenberg, E. I.; Ruiz-Martinez, A.; Triplett, N.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Barashkou, A.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chepurnov, V. F.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Gusakov, Y.; Huseynov, N.; Kalinovskaya, L. V.; Kazarinov, M. Y.; Kekelidze, G. D.; Kharchenko, D.; Khovanskiy, N.; Khramov, E.; Kolesnikov, V.; Kotov, Vm; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Lazarev, A. B.; Malyukov, S.; Manjavidze, I. D.; Minashvili, I. A.; Mineev, M.; Nikolaev, K.; Olchevski, A. G.; Peshekhonov, V. D.; Romanov, V. M.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Ishii, K.; Ishino, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Manabe, A.; Mitsui, S.; Morita, Y.; Murakami, K.; Nagano, K.; Nozaki, M.; Odaka, S.; Ohska, T. K.; Sasaki, O.; Sasaki, T.; Suzuki, Y.; Tanaka, S.; Terada, S.; Tojo, J.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Akiyama, A.; Hayakawa, T.; Homma, Y.; Ichimiya, R.; Ishikawa, A.; Kawagoe, K.; King, M.; Kiyamura, H.; Kurashige, H.; Matsushita, T.; Miyazaki, K.; Nishiyama, T.; Ochi, A.; Okada, S.; Omachi, C.; Suita, K.; Takeda, H.; Tani, K.; Tokunaga, K.; Yamazaki, Y.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Sasao, N.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Brodbeck, T. J.; Catmore, J. R.; Cheatham, S.; Chilingarov, A.; Davidson, R.; De Mora, L.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Ratoff, P. N.; Sloan, T. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Brambilla, E.; Cazzato, A.; Chiodini, G.; Coluccia, R.; Crupi, R.; Gorini, E.; Grancagnolo, F.; Guida, A.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Bianco, M.; Brambilla, E.; Cazzato, A.; Coluccia, R.; Crupi, R.; Gorini, E.; Guida, A.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Fis, Lecce, Italy. [Allport, P. P.; Austin, N.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Houlden, M. A.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Maxfield, S. J.; Mehta, A.; Migas, S.; Prichard, P. M.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wiglesworth, C.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Landon, M. P. J.; Lloyd, S. L.; Morin, J.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Stevenson, K.; Castanheira, M. Teixeira Dias; Traynor, D.] Queen Mary Univ London, Dept Phys, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Boorman, G.; Cooper-Smith, N. J.; Cowan, G.; Edwards, C. A.; George, S.; Goncalo, R.; Hayden, D.; Kilvington, G.; Misiejuk, A.; Rose, M.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Boeser, S.; Butterworth, J. M.; Byatt, T.; Campanelli, M.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dean, S.; Drohan, J. G.; Jansen, E.; Jones, T. W.; Konstantinidis, N.; Monk, J.; Nash, M.; Nurse, E.; Prabhu, R.; Richards, A.; Robinson, J. E. M.; Sherwood, P.; Simmons, B.; Taylor, C.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Beauchemin, P. H.; Bordoni, S.; Calderini, G.; Camard, A.; Cavalleri, P.; Chareyre, E.; De Cecco, S.; Derue, F.; Imbault, D.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lellouch, J.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph; Theveneaux-Pelzer, T.; Trincaz-Duvoid, S.; Trinh, T. N.; Vannucci, F.; Yuan, L.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beauchemin, P. H.; Bordoni, S.; Calderini, G.; Camard, A.; Cavalleri, P.; Chareyre, E.; De Cecco, S.; Derue, F.; Imbault, D.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lellouch, J.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph; Theveneaux-Pelzer, T.; Trincaz-Duvoid, S.; Trinh, T. N.; Vannucci, F.; Yuan, L.] Univ Paris Diderot, Paris, France. [Beauchemin, P. H.; Bordoni, S.; Calderini, G.; Camard, A.; Cavalleri, P.; Chareyre, E.; De Cecco, S.; Derue, F.; Imbault, D.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lellouch, J.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph; Theveneaux-Pelzer, T.; Trincaz-Duvoid, S.; Trinh, T. N.; Vannucci, F.; Yuan, L.] IN2P3, CNRS, Paris, France. [Akesson, T. P.; Alonso, A.; Groth-Jensen, J.; Hedberg, V.; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.] Lund Univ, Inst Fys, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Lagouri, T.; March, L.; Nebot, E.; Rodier, S.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Aharrouche, M.; Arnaez, O.; Bendel, M.; Blum, W.; Buescher, V.; Eckweiler, S.; Edmonds, K.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Ji, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Meyer, C.; Moreno, D.; Neusiedl, A.; Rieke, S.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Siragusa, G.; Tapprogge, S.; Anh, T. Vu] Johannes Gutenberg Univ Mainz, Inst Phys, D-6500 Mainz, Germany. [Almond, J.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Foster, J. M.; Howarth, J.; Hughes-Jones, R. E.; Ibbotson, M.; Jones, G.; Keates, J. R.; Kelly, M.; Kolya, S. D.; Lane, J. L.; Loebinger, F. K.; Marshall, R.; Martyniuk, A. C.; Marx, M.; Masik, J.; Miyagawa, P. S.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Plano, W. G.; Schwanenberger, C.; Snow, S. W.; Tevlin, C. M.; Watts, S.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aoun, S.; Arfaoui, S.; Bee, C. P.; Benchouk, C.; Bernardet, K.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Delpierre, P.; Djama, F.; Etienne, F.; Feligioni, L.; Henry-Couannier, F.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Monnier, E.; Odier, J.; Petit, E.; Pralavorio, P.; Qian, Z.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aoun, S.; Arfaoui, S.; Bee, C. P.; Benchouk, C.; Bernardet, K.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Delpierre, P.; Djama, F.; Etienne, F.; Feligioni, L.; Henry-Couannier, F.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Monnier, E.; Odier, J.; Petit, E.; Pralavorio, P.; Qian, Z.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] IN2P3, CNRS, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Thompson, E. N.; van Eldik, N.; Willocq, S.; Woudstra, M. J.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Chapleau, B.; Corriveau, F.; Dobbs, M.; Dufour, M-A; Guler, H.; Klemetti, M.; Robertson, S. H.; Schram, M.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Davey, W.; Davidson, N.; Felzmann, C. U.; Kazi, S. I.; Limosani, A.; Moorhead, G. F.; Phan, A.; Sevior, M. E.; Shao, Q. T.; Taylor, G. N.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Eppig, A.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, H.; Liu, J. B.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Purdham, J.; Qian, J.; Scheirich, D.; Strandberg, J.; Thun, R. P.; Walch, S.; Wilson, A.; Yang, H.; Zhou, B.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Comune, G.; Di Mattia, A.; Fedorko, W.; Hauser, R.; Heim, S.; Holzbauer, J. L.; Huston, J.; Koll, J.; Kraus, J.; Linnemann, J. T.; Mangeard, P. S.; Martin, B.; Miller, R. J.; Pope, B. G.; Ryan, P.; Schwienhorst, R.; Tollefson, K.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Acerbi, E.; Aleppo, M.; Alessandria, F.; Alimonti, G.; Andreazza, A.; Baccaglioni, G.; Battistoni, G.; Bellomo, G.; Besana, M. I.; Broggi, F.; Caccia, M.; Carminati, L.; Cavalli, D.; Dell'Asta, L.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Lazzaro, A.; Lombardo, V. P.; Mandelli, L.; Mazzanti, M.; Meroni, C.; Montesano, S.; Perini, L.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Rossi, L.; Sorbi, M.; Tartarellia, G. F.; Troncon, C.; Turra, R.; Vegni, G.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Acerbi, E.; Aleppo, M.; Andreazza, A.; Bellomo, G.; Besana, M. I.; Caccia, M.; Carminati, L.; Dell'Asta, L.; Fanti, M.; Favareto, A.; Lazzaro, A.; Montesano, S.; Perini, L.; Ragusa, F.; Rivoltella, G.; Rossi, L.; Sorbi, M.; Turra, R.; Vegni, G.] Univ Milan, Dipartimento Fis, Milan, Italy. [Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Gilewsky, V.; Kuzhir, P.; Rumiantsev, V.; Starovoitov, P.; Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Azuelos, G.; Banerjee, P.; Bouchami, J.; Davies, M.; Ferland, J.; Guler, H.; Gutierrez, A.; Lebel, C.; Leroy, C.; Goia, J. A. Macana; Martin, J. P.; Mehdiyev, R.; Scallon, O.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bondarenko, V. G.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Morozov, S. V.; Romaniouk, A.; Smirnov, S. Yu; Soldatov, E.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu; Smirnova, L. N.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Biebel, O.; Calfayan, P.; de Graat, J.; Deile, M.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Genest, M. H.; Hertenberger, R.; Kennedy, J.; Kummer, C.; Legger, F.; Lichtnecker, M.; Mameghani, R.; Mueller, T. A.; Nunnemann, T.; Rauscher, F.; Reznicek, P.; Ruckert, B.; Sanders, M. P.; Schaile, D.; Schieck, J.; Serfon, C.; Staude, A.; Walker, R.; Will, J. Z.; Zhuang, X.] Univ Munich, Fak Phys, Munich, Germany. [Aderholz, M.; Barillari, T.; Beimforde, M.; Bethke, S.; Capriotti, D.; Cortiana, G.; Dannheim, D.; Dietl, H.; Dubbert, J.; Ehrich, T.; Flowerdew, M. J.; Giovannini, P.; Goettfert, T.; Groh, M.; Haefner, P.; Hauff, D.; Hott, T.; Jantsch, A.; Kaiser, S.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Lutz, G.; Macchiolo, A.; Manz, A.; Menke, S.; Mohrdieck-Moeck, S.; Moser, H. G.; Nisius, R.; Oberlack, H.; Pospelov, G. E.; Potrap, I. N.; Rauter, E.; Richter, R.; Salihagic, D.; Schacht, P.; Seuster, R.; Stonjek, S.; Valderanis, C.; von der Schmitt, H.; von Loeben, J.; Weigell, P.; Zhuravlov, V.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.; Tanaka, Y.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Itoh, Y.; Ohshima, T.; Okumura, Y.; Sugimoto, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Cevenini, F.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Della Volpe, D.; Doria, A.; Giordano, R.; Iacobucci, G.; Izzo, V.; Merola, L.; Musto, E.; Patricelli, S.; Rossi, E.; Sekhniaidze, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Cevenini, F.; Chiefari, G.; Della Volpe, D.; Giordano, R.; Merola, L.; Musto, E.; Patricelli, S.; Rossi, E.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Metcalfe, J.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Chelstowska, M. A.; Consonni, M.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Koetsveld, F.; Magrath, A.; Ordonez, G.; Raas, M.; Timmermans, C. J. W. P.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Bentvelsen, S.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Buis, E. J.; Colijn, A. P.; Dankers, R.; Daum, C.; de Jong, P.; De Nooij, L.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Koutsman, A.; Lee, H.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Muijs, A.; Mussche, I.; Ottersbach, J. P.; Peters, O.; Reichold, A.; Rijpstra, M.; Ruckstuhl, N.; Salamanna, G.; Sandstroem, R.; Snuverink, J.; Ta, D.; Tsiakiris, M.; Turlay, E.; van der Graaf, H.; van der Kraaij, E.; van der Leeuw, R.; van der Poel, E.; Van Eijk, B.; van Kesteren, Z.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Bentvelsen, S.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Buis, E. J.; Colijn, A. P.; Dankers, R.; Daum, C.; de Jong, P.; De Nooij, L.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Koutsman, A.; Lee, H.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Muijs, A.; Mussche, I.; Ottersbach, J. P.; Peters, O.; Reichold, A.; Rijpstra, M.; Ruckstuhl, N.; Salamanna, G.; Sandstroem, R.; Snuverink, J.; Ta, D.; Tsiakiris, M.; Turlay, E.; van der Graaf, H.; van der Kraaij, E.; van der Leeuw, R.; van der Poel, E.; Van Eijk, B.; van Kesteren, Z.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; de Lima, J. G. Rocha; Suhr, C.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Beloborodova, O.; Bobrovnikov, V. B.; Bogdanchikov, A.; Kazanin, V. A.; Kolachev, G. M.; Korol, A.; Malyshev, V.; Maslennikov, A. L.; Maximov, D. A.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.; Zaytsev, A.] Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; Djilkibaev, R.; van Huysduynen, L. Hooft; Konoplich, R.; Krasznahorkay, A.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.; Shibata, A.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA. [Fernando, W.; Fisher, M. J.; Gan, K. K.; Kagan, H.; Kass, R. D.; Moss, J.; Rahimi, A. M.; Strang, M.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Huang, G. S.; Issever, C.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Kocnar, A.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Potter, C. T.; Ptacek, E.; Reinsch, A.; Robinson, M.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abreu, H.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Blanchard, J-B; Bourdarios, C.; Breton, D.; Collard, C.; De La Taille, C.; De Regie, J. B. De Vivie; Diglio, S.; Duflot, L.; Escalier, M.; Falou, A. C.; Fayard, L.; Fournier, D.; Grivaz, J-F; Heller, M.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lounis, A.; Makovec, N.; Matricon, P.; Nakahama, Y.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Veillet, J. J.; Vukotic, I.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Abreu, H.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Blanchard, J-B; Bourdarios, C.; Breton, D.; Collard, C.; De La Taille, C.; De Regie, J. B. De Vivie; Diglio, S.; Duflot, L.; Escalier, M.; Falou, A. C.; Fayard, L.; Fournier, D.; Grivaz, J-F; Heller, M.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lounis, A.; Makovec, N.; Matricon, P.; Nakahama, Y.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Veillet, J. J.; Vukotic, I.; Wicek, F.; Zerwas, D.; Zhang, Z.] IN2P3, CNRS, Orsay, France. [Hanagaki, K.; Hirose, M.; Meguro, T.; Nomachi, M.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Czyczula, Z.; Gjelsten, B. K.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Pylypchenko, Y.; Read, A. L.; Rohne, O.; Samset, B. H.; Stapnes, S.; Strandlie, A.; Taga, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Abdesselam, A.; Apolle, R.; Barr, A. J.; Boddy, C. R.; Brett, N. D.; Buchanan, J.; Buckingham, R. M.; Buira-Clark, D.; Coe, P.; Coniavitis, E.; Cooper-Sarkar, A. M.; Dehchar, M.; Doglioni, C.; Farrington, S. M.; Ferrando, J.; Gallas, E. J.; Gilbert, L. M.; Gwenlan, C.; Hawes, B. M.; Holmes, A.; Horton, K.; Howell, D. F.; Huffman, T. B.; Issever, C.; Karagoz, M.; King, R. S. B.; Kirsch, G. P.; Kundu, N.; Larner, A.; Lau, W.; Lavorato, A.; Liang, Z.; Livermore, S. S. A.; Loken, J.; Mattravers, C.; Mermod, P.; Nickerson, R. B.; Pinder, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Wooden, G.] Univ Oxford, Dept Phys, Oxford, England. [Bellomo, M.; Cambiaghi, M.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudioa, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Cambiaghi, M.; Conta, C.; Franchino, S.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.] Univ Pavia, Dipartimento Fis Nucl & Teor, I-27100 Pavia, Italy. [Alison, J.; Degenhardt, J.; Donega, M.; Dressnandt, N.; Fratina, S.; Hance, M.; Hines, E.; Jackson, B.; Kroll, J.; Kunkle, J.; LeGeyt, C.; Lipeles, E.; Martin, F. F.; Olivito, D.; Ospanov, R.; Reece, R.; Stahlman, J.; Thomson, E.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Nesterov, S. Y.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Zalite, Yo K.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Francavilla, P.; Giangiobbe, V.; Lupi, A.; Mazzoni, E.; Roda, C.; Sarri, F.; Zenonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Francavilla, P.; Giangiobbe, V.; Lupi, A.; Mazzoni, E.; Roda, C.; Sarri, F.; Zenonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Boudreau, J.; Boulahouache, C.; Cleland, W.; Kittelmann, T.; Mueller, J.; Paolone, V.; Prieur, D.; Savinov, V.; Tsulaia, V.; Wendler, S.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, A.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Wemans, A. Do Valle; Fernandes, B.; Fiolhais, M. C. N.; Gomes, A.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Magalhaes Martins, P. J.; Maio, A.; Maneira, J.; Morais, A.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Soares, M.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedra, A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, A.] Univ Granada, CAFPE, Granada, Spain. [Chudoba, J.; Gallus, P.; Gunther, J.; Hruska, I.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Kvasnicka, O.; Lipinsky, L.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Panuskova, M.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Davidek, T.; Dolejsi, J.; Dolezal, Z.; Drasal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Augsten, K.; Holy, T.; Horazdovsky, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Bozhko, N. I.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Gapienko, V. A.; Golovnia, S. N.; Gorokhov, S. A.; Goryachev, V. N.; Gushchin, V. N.; Ivashin, A. V.; Kabachenko, V. V.; Karyukhin, N.; Kholodenko, A. G.; Kiver, A. M.; Kopikov, S. V.; Koreshev, V.; Korotkov, V. A.; Kozhin, A. S.; Lapin, V. V.; Larionov, A. V.; Levitski, M. S.; Lokajicek, M.; Minaenko, A. A.; Mitrofanov, G. Y.; Moisseev, A. M.; Myagkov, A. G.; Nikolaenko, V.; Pleskach, A. V.; Ryadovikov, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Sviridov, Yu M.; Vorobiev, A. P.; Vovenko, A. S.; Zaets, V. G.; Zaitsev, A. M.; Zenin, A. V.; Zenin, O.; Zmouchko, V. V.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Botterill, D.; Burke, S.; Clifft, R. W.; Dallison, S. J.; Dewhurst, A.; Emeliyanov, D.; Fisher, S. M.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Greenfield, D.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Strube, J.; Tyndel, M.; Weber, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.; Ju, X.; Ming, Y.; Ortega, E. O.; Smit, G. V. Ybeles] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagnaia, P.; Bini, C.; Borroni, S.; Caloi, R.; Cavallari, A.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; Dionisi, C.; Falciano, S.; Gentile, S.; Giagu, S.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Maiani, C.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Spila, F.; Valente, P.; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma I, Rome, Italy. [Artoni, G.; Bagnaia, P.; Bini, C.; Borroni, S.; Caloi, R.; Cavallari, A.; Ciapetti, G.; D'Orazio, A.; Dionisi, C.; Gentile, S.; Giagu, S.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Maiani, C.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Spila, F.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Nardo, R.; Di Simone, A.; Liberti, B.; Marchese, F.; Paoloni, A.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Nardo, R.; Di Simone, A.; Marchese, F.; Paoloni, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Ruggieri, F.; Spiriti, E.; Stanescu, C.; Tonazzo, A.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Biglietti, M.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.; Ruggieri, F.; Tonazzo, A.] Univ Roma Tre, Dipartimento Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Goujdami, D.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Fac Sci Ain Chock, Reseau Univ Phys Hautes Energies, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. Univ Cadi Ayyad, Fac Sci, Semlalia Dept Phys, Marrakech 40000, Morocco. [Derkaoui, J. E.; Ouchrif, M.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Boonekamp, M.; Chevalier, L.; Chevallier, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Le Menedeu, E.; Legendre, M.; Lenzi, B.; Mansoulie, B.; Meyer, J-P; Morange, N.; Nicolaidou, R.; Ouraou, A.; Pomarede, D. M.; Resende, B.; Royon, C. R.; Schune, Ph; Schwindling, J.; Simard, O.; Virchaux, M.; Yu, J.] CEA, CEA Saclay, DSM, IRFU Inst Rech Lois Fondament Univers, Gif Sur Yvette, France. [Bangert, A.; Chouridou, S.; Damiani, D. S.; Dubbs, T.; Fowler, K.; Grillo, A. A.; Hare, G. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Forbush, D. A.; Goussiou, A. G.; Griffiths, J.; Harris, O. M.; Kuykendall, W.; Lubatti, H. J.; Mockett, P.; Policicchio, A.; Rothberg, J.; Ventura, D.; Verducci, M.; Wang, J. C.; Watts, G.; Zhao, T.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Abdesselam, A.; Anastopoulos, C.; Booth, C. N.; Booth, P.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Duxfield, R.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mayne, A.; Mcfayden, J. A.; Nicolas, L.; Owen, S.; Paganis, E.; Sutton, M. R.; Tovey, D. R.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Ohshita, H.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Sipica, V.; Stahl, T.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-5900 Siegen, Germany. [Dawe, E.; Gao, Y. S.; Godfrey, J.; Komaragiri, J. R.; O'Neil, D. C.; Petteni, M.; Schouten, D.; Stelzer, B.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Grenier, P.; Haas, A.; Hansson, P.; Horn, C.; Jackson, P.; Kenney, C. J.; Kim, P. C.; Kocian, M.; Koi, T.; Lowe, A. J.; Miller, D. W.; Mount, R.; Nelson, S.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Wilson, M. G.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Batkova, L.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.; Zilka, B.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Aurousseau, M.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Leney, C.; Vickey, T.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Asman, B.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Hidvegi, A.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Lesser, J.; Lundberg, J.; Milstead, D. A.; Moa, T.; Nordkvist, B.; Ohm, C. C.; Papadelis, A.; Ramstedt, M.; Sellden, B.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Asman, B.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Lundberg, J.; Milstead, D. A.; Moa, T.; Nordkvist, B.; Ohm, C. C.; Ramstedt, M.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Grahn, K-J; Lund-Jensen, B.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Caputo, R.; Deluca, C.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Khodinov, A.; McCarthy, L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.; Yurkewicz, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Potter, C. J.; Salvatore, F.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Lee, J. S. H.; Patel, N.; Saavedra, A. F.; Varvell, K. E.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Harpaz, S. Behar; Ben Ami, S.; Bressler, S.; Kajomovitz, E.; Landsman, H.; Lifshitz, R.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Brodet, E.; Etzion, E.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hershenhorn, A. D.; Hod, N.; Kreisel, A.; Mahalalel, Y.; Munwes, Y.; Oren, Y.; Reinherz-Aronis, E.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.; Urkovsky, E.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Imori, M.; Kanaya, N.; Kaneda, M.; Kataoka, Y.; Kawamoto, T.; Kessoku, K.; Kobayashi, T.; Kubota, T.; Mashimo, T.; Masubuchi, T.; Matsumoto, H.; Matsunaga, H.; Nakamura, K.; Ninomiya, Y.; Nomoto, H.; Oda, S.; Okuyama, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamamura, T.; Yamazaki, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Imori, M.; Kanaya, N.; Kaneda, M.; Kataoka, Y.; Kawamoto, T.; Kessoku, K.; Kobayashi, T.; Kubota, T.; Mashimo, T.; Masubuchi, T.; Matsumoto, H.; Matsunaga, H.; Nakamura, K.; Ninomiya, Y.; Nomoto, H.; Oda, S.; Okuyama, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamamura, T.; Yamazaki, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Jinnouchi, O.; Kanno, T.; Kuze, M.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [Bailey, D. C.; Bain, T.; Beau, T.; Brelier, B.; Cheung, S. L.; Deviveiros, P. O.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Jankowski, E.; Krieger, P.; Le Maner, C.; Martens, F. K.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Sandhu, P.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Caron, B.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Losty, M. J.; Nugent, I. M.; Oakham, F. G.; Oram, C. J.; Savard, P.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Hara, K.; Kim, S. H.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Inst Pure & Appl Sci, Ibaraki, Japan. [Hamilton, S.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.] Tufts Univ, Ctr Sci & Technol, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Rodriguez, D.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Benedict, B. H.; Bold, T.; Ciobotaru, M. D.; Deng, J.; Dobson, M.; Eschrich, I. Gough; Grabowska-Bold, I.; Hawkins, D.; Lankford, A. J.; Okawa, H.; Porter, R.; Scannicchio, D. A.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Wheeler-Ellis, S. J.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Cauz, D.; Cobal, M.; De Lotto, B.; De Sanctis, U.; Del Papa, C.; Pinamonti, M.; Shaw, K.; Suruliz, K.] Ist Nazl Fis Nucl, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Suruliz, K.] ICTP, Udine, Italy. [Cauz, D.; Cobal, M.; De Lotto, B.; De Sanctis, U.; Del Papa, C.; Pinamonti, M.; Shaw, K.] Univ Udine, Dipartimento Fis, I-33100 Udine, Italy. [Benekos, N.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Khandanyan, H.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Belanger-Champagne, C.; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Hansen, C. J.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Amoros, G.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Amoros, G.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, Dept Fis Atom, Valencia, Spain. [Amoros, G.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, IMB, CNM, Valencia, Spain. [Amoros, G.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] CSIC, Valencia, Spain. [Axen, D.; Gay, C.; Loh, C. W.; Mills, W. J.; Muir, A.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Astbury, A.; Banerjee, Sw; Bansal, V.; Berghaus, F.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R; McPherson, A.; Plamondon, M.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Kimura, N.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Duchovni, E.; Frank, T.; Gabizon, O.; Gross, E.; Klier, A.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Asfandiyarov, R.; Montoya, G. D. Carrillo; Hernandez, A. M. Castaneda; Castaneda-Miranda, E.; Chen, X.; Dos Anjos, A.; Fang, Y.; Fasching, D.; Castillo, L. R. Flores; Gonzalez, S.; Gutzwiller, O.; Ji, H.; Kashif, L.; Cheong, A. Leung Fook; Li, H.; Ma, L. L.; Mellado Garcia, B. R.; Pan, Y. B.; Pataraia, S.; Morales, M. I. Pedraza; Peng, H.; Poveda, J.; Quayle, W. B.; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Zhu, Y.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Meyer, J.; Redelbach, A.; Stroehmer, R.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, Wurzburg, Germany. [Barisonzi, M.; Becks, K. H.; Boek, J.; Braun, H. M.; Drees, J.; Fleischmann, S.; Flick, T.; Gerlach, P.; Glitza, K. W.; Gorfine, G.; Grah, C.; Hamacher, K.; Harenberg, T.; Henss, T.; Hirschbuehl, D.; Imhaeuser, M.; Kalinin, S.; Kersten, S.; Kootz, A.; Kuhl, T.; Lenz, T.; Lenzen, G.; Maettig, P.; Mechtel, M.; Sandhoff, M.; Sandvoss, S.; Sartisohn, G.; Schultes, J.; Siebel, A.; Sturm, P.; Thadome, J.; Voss, T. T.; Wagner, W.; Wahlen, H.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Atoian, G.; Auerbach, B.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Demers, S.; Garberson, F.; Golling, T.; Guest, D.; Hsu, P. J.; Kaplan, B.; Lee, L.; Lockwitz, S.; Loginov, A.; Martin, A. J.; Schmidt, M. P.; Sherman, D.; Thioye, M.; Tipton, P.; Wall, R.; Zeller, M.] Yale Univ, Dept Phys, New Haven, CT USA. [Grabski, V.; Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Biscarat, C.; Cogneras, E.; Rahal, G.] IN2P3, Ctr Calcul CNRS, Villeurbanne, France. [Amorim, A.; Fernandes, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Maio, A.; Morais, A.; Palma, A.; Pina, J.; Pinto, B.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amorim, A.; Fernandes, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Maio, A.; Morais, A.; Palma, A.; Pina, J.; Pinto, B.; Saraiva, J. G.; Silva, J.] Univ Lisbon, CFNUL, P-1699 Lisbon, Portugal. [Beare, B.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Carvalho, J.; Fiolhais, M. C. N.; Magalhaes Martins, P. J.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Kono, T.; Terwort, M.; Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mateos, D. Lopez; Marshall, Z.; Perez, K.] CALTECH, Pasadena, CA 91125 USA. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Park, W.; Purohit, M.; Trivedi, A.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Pasztor, G.; Toth, J.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Richter-Was, E.] Jagiellonian Univ, Inst Phys, Krakow, Poland. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Freiburg, Germany. RI valente, paolo/A-6640-2010; Fazio, Salvatore /G-5156-2010; Doyle, Anthony/C-5889-2009; Jakubek, Jan/E-6530-2011; Marti-Garcia, Salvador/F-3085-2011; Conde Muino, Patricia/F-7696-2011; collins-tooth, christopher/A-9201-2012; Stoicea, Gabriel/B-6717-2011; Robson, Aidan/G-1087-2011; Losada, Marta/B-2261-2010; Gutierrez, Phillip/C-1161-2011; Ferrando, James/A-9192-2012; Perrino, Roberto/B-4633-2010; De Cecco, Sandro/B-1016-2012; branchini, paolo/A-4857-2011; Wolter, Marcin/A-7412-2012; McKee, Shawn/B-6435-2012; Rotaru, Marina/A-3097-2011; Nemecek, Stanislav/C-3487-2012; Buttar, Craig/D-3706-2011; Takai, Helio/C-3301-2012; St.Denis, Richard/C-8997-2012; Britton, David/F-2602-2010; Li, Xuefei/C-3861-2012; Smirnova, Lidia/D-8089-2012; Smirnov, Sergei/F-1014-2011; Gladilin, Leonid/B-5226-2011; Kramarenko, Victor/E-1781-2012; Alexa, Calin/F-6345-2010; Moorhead, Gareth/B-6634-2009; Petrucci, Fabrizio/G-8348-2012; Wemans, Andre/A-6738-2012; Fabbri, Laura/H-3442-2012; Kurashige, Hisaya/H-4916-2012; Kuzhir, Polina/H-8653-2012; Delmastro, Marco/I-5599-2012; Weigell, Philipp/I-9356-2012; Veneziano, Stefano/J-1610-2012; Di Micco, Biagio/J-1755-2012; spagnolo, stefania/A-6359-2012; Andreazza, Attilio/E-5642-2011; Di Nardo, Roberto/J-4993-2012; Della Pietra, Massimo/J-5008-2012; Bergeaas Kuutmann, Elin/A-5204-2013; Cascella, Michele/B-6156-2013; messina, andrea/C-2753-2013; de Groot, Nicolo/A-2675-2009; Amorim, Antonio/C-8460-2013; Orlov, Ilya/E-6611-2012; Annovi, Alberto/G-6028-2012; Pina, Joao /C-4391-2012; Vanyashin, Aleksandr/H-7796-2013; La Rosa, Alessandro/I-1856-2013; Casadei, Diego/I-1785-2013; Moraes, Arthur/F-6478-2010; Boyko, Igor/J-3659-2013; Kuleshov, Sergey/D-9940-2013; Anjos, Nuno/I-3918-2013; Kartvelishvili, Vakhtang/K-2312-2013; Dawson, Ian/K-6090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Castro, Nuno/D-5260-2011; Wolters, Helmut/M-4154-2013; Warburton, Andreas/N-8028-2013; De, Kaushik/N-1953-2013; Sukharev, Andrey/A-6470-2014; O'Shea, Val/G-1279-2010; Lee, Jason/B-9701-2014; Morozov, Sergey/C-1396-2014; Villa, Mauro/C-9883-2009; Nemecek, Stanislav/G-5931-2014; Staroba, Pavel/G-8850-2014; Lokajicek, Milos/G-7800-2014; Kupco, Alexander/G-9713-2014; Marcisovsky, Michal/H-1533-2014; Mikestikova, Marcela/H-1996-2014; Snesarev, Andrey/H-5090-2013; Chudoba, Jiri/G-7737-2014; Peleganchuk, Sergey/J-6722-2014; Santamarina Rios, Cibran/K-4686-2014; Bosman, Martine/J-9917-2014; Lei, Xiaowen/O-4348-2014; Demirkoz, Bilge/C-8179-2014; Ventura, Andrea/A-9544-2015; Villaplana Perez, Miguel/B-2717-2015; Livan, Michele/D-7531-2012; Mitsou, Vasiliki/D-1967-2009; CARPENTIERI, CARMELA/E-2137-2015; Joergensen, Morten/E-6847-2015; Martins, Paulo/M-1844-2014; Mir, Lluisa-Maria/G-7212-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Cavalli-Sforza, Matteo/H-7102-2015; Ferrer, Antonio/H-2942-2015; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; Tikhomirov, Vladimir/M-6194-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Jones, Roger/H-5578-2011; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Carvalho, Joao/M-4060-2013; Booth, Christopher/B-5263-2016; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Smirnova, Oxana/A-4401-2013; Leyton, Michael/G-2214-2016; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Olshevskiy, Alexander/I-1580-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Morone, Maria Cristina/P-4407-2016; Goncalo, Ricardo/M-3153-2016; Canelli, Florencia/O-9693-2016; Battistoni, Giuseppe/B-5264-2012; Idzik, Marek/A-2487-2017; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; la rotonda, laura/B-4028-2016; OI valente, paolo/0000-0002-5413-0068; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Stoicea, Gabriel/0000-0002-7511-4614; Ferrando, James/0000-0002-1007-7816; Perrino, Roberto/0000-0002-5764-7337; McKee, Shawn/0000-0002-4551-4502; Rotaru, Marina/0000-0003-3303-5683; Takai, Helio/0000-0001-9253-8307; Britton, David/0000-0001-9998-4342; Smirnov, Sergei/0000-0002-6778-073X; Gladilin, Leonid/0000-0001-9422-8636; Moorhead, Gareth/0000-0002-9299-9549; Petrucci, Fabrizio/0000-0002-5278-2206; Wemans, Andre/0000-0002-9669-9500; Fabbri, Laura/0000-0002-4002-8353; Kuzhir, Polina/0000-0003-3689-0837; Delmastro, Marco/0000-0003-2992-3805; Veneziano, Stefano/0000-0002-2598-2659; spagnolo, stefania/0000-0001-7482-6348; Andreazza, Attilio/0000-0001-5161-5759; Della Pietra, Massimo/0000-0003-4446-3368; Cascella, Michele/0000-0003-2091-2501; Orlov, Ilya/0000-0003-4073-0326; Annovi, Alberto/0000-0002-4649-4398; Pina, Joao /0000-0001-8959-5044; Vanyashin, Aleksandr/0000-0002-0367-5666; La Rosa, Alessandro/0000-0001-6291-2142; Moraes, Arthur/0000-0002-5157-5686; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Castro, Nuno/0000-0001-8491-4376; Wolters, Helmut/0000-0002-9588-1773; Warburton, Andreas/0000-0002-2298-7315; De, Kaushik/0000-0002-5647-4489; O'Shea, Val/0000-0001-7183-1205; Lee, Jason/0000-0002-2153-1519; Morozov, Sergey/0000-0002-6748-7277; Villa, Mauro/0000-0002-9181-8048; Mikestikova, Marcela/0000-0003-1277-2596; Peleganchuk, Sergey/0000-0003-0907-7592; Santamarina Rios, Cibran/0000-0002-9810-1816; Bosman, Martine/0000-0002-7290-643X; Lei, Xiaowen/0000-0002-2564-8351; Ventura, Andrea/0000-0002-3368-3413; Villaplana Perez, Miguel/0000-0002-0048-4602; Livan, Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886; CARPENTIERI, CARMELA/0000-0002-2994-0317; Joergensen, Morten/0000-0002-6790-9361; Martins, Paulo/0000-0003-3753-3751; Mir, Lluisa-Maria/0000-0002-4276-715X; Riu, Imma/0000-0002-3742-4582; Ferrer, Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543; Grancagnolo, Sergio/0000-0001-8490-8304; Tikhomirov, Vladimir/0000-0002-9634-0581; Camarri, Paolo/0000-0002-5732-5645; Jones, Roger/0000-0002-6427-3513; Gorelov, Igor/0000-0001-5570-0133; Carvalho, Joao/0000-0002-3015-7821; Booth, Christopher/0000-0002-6051-2847; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Smirnova, Oxana/0000-0003-2517-531X; Leyton, Michael/0000-0002-0727-8107; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Olshevskiy, Alexander/0000-0002-8902-1793; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Morone, Maria Cristina/0000-0002-0200-0632; Goncalo, Ricardo/0000-0002-3826-3442; Canelli, Florencia/0000-0001-6361-2117; Battistoni, Giuseppe/0000-0003-3484-1724; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Maio, Amelia/0000-0001-9099-0009; Fiolhais, Miguel/0000-0001-9035-0335; Karyukhin, Andrey/0000-0001-9087-4315; Anjos, Nuno/0000-0002-0018-0633; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; Veloso, Filipe/0000-0002-5956-4244; Gomes, Agostinho/0000-0002-5940-9893; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Santos, Helena/0000-0003-1710-9291; Coccaro, Andrea/0000-0003-2368-4559; De Lotto, Barbara/0000-0003-3624-4480 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; ARTEMIS; European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNAS, Greece; ISF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, UK; Royal Society, UK; Leverhulme Trust, UK; DOE, USA; NSF, USA FX We thank CERN for the highly successful operation of the LHC and we also thank the support staff from our institutions without whom ATLAS could not have been operated efficiently. We acknowledge support from ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; ARTEMIS, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNAS, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, UK; DOE and NSF, USA. The crucial computing support from all WLCG partners is also acknowledged, in particular from CERN and not only the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway and Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) but also the Tier-2 facilities worldwide. NR 50 TC 62 Z9 62 U1 3 U2 71 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD MAY 24 PY 2011 VL 13 AR 053044 DI 10.1088/1367-2630/13/5/053044 PG 44 WC Physics, Multidisciplinary SC Physics GA 782IT UT WOS:000292002400004 ER PT J AU Ni, S Wang, YB Liao, XZ Figueiredo, RB Li, HQ Zhao, YH Lavernia, EJ Ringer, SP Langdon, TG Zhu, YT AF Ni, S. Wang, Y. B. Liao, X. Z. Figueiredo, R. B. Li, H. Q. Zhao, Y. H. Lavernia, E. J. Ringer, S. P. Langdon, T. G. Zhu, Y. T. TI Strain softening in nanocrystalline Ni-Fe alloy induced by large HPT revolutions SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Severe plastic deformation; Nanocrystalline materials; Strain softening; Dislocation density; Lomer-Cottrell locks ID HIGH-PRESSURE TORSION; MOLECULAR-DYNAMICS SIMULATION; GRAIN-GROWTH; MICROSTRUCTURAL EVOLUTION; PLASTIC-DEFORMATION; FCC METALS; DISLOCATION JUNCTIONS; STRENGTH; NICKEL; COPPER AB The influence of strain on the hardness of an electrochemically deposited nanocrystalline Ni-20 wt.% Fe alloy processed by high-pressure torsion (HFT) for 20 and 30 revolutions was investigated. Strain softening followed by a stable hardness value was observed. Structural investigations revealed that, while dislocation density was important, continuous grain growth played a major role in the strain softening. The stable hardness indicates that an equilibrium structure was achieved, supporting a dynamic balance between deformation-induced grain growth and grain refinement and between deformation-induced dislocation generation and dislocation annihilation. (C) 2011 Elsevier B.V. All rights reserved. C1 [Ni, S.; Wang, Y. B.; Liao, X. Z.] Univ Sydney, Sch Aerosp Mech & Mechatron Engn, Sydney, NSW 2006, Australia. [Figueiredo, R. B.] Univ Fed Minas Gerais, Dept Met & Mat Engn, BR-31270901 Belo Horizonte, MG, Brazil. [Li, H. Q.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Zhao, Y. H.; Lavernia, E. J.] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [Ringer, S. P.] Univ Sydney, Australian Ctr Microscopy & Microanal, Sydney, NSW 2006, Australia. [Langdon, T. G.] Univ So Calif, Dept Aerosp & Mech Engn, Los Angeles, CA 90089 USA. [Langdon, T. G.] Univ So Calif, Dept Mat Sci, Los Angeles, CA 90089 USA. [Langdon, T. G.] Univ Southampton, Sch Engn Sci, Mat Res Grp, Southampton SO17 1BJ, Hants, England. [Zhu, Y. T.] N Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27659 USA. RP Liao, XZ (reprint author), Univ Sydney, Sch Aerosp Mech & Mechatron Engn, Sydney, NSW 2006, Australia. EM xiaozhou.liao@sydney.edu.au RI Liao, Xiaozhou/B-3168-2009; Wang, Yanbo/B-3175-2009; Ni, Song/E-9484-2011; Figueiredo, Roberto/F-3451-2012; Lavernia, Enrique/I-6472-2013; Li, Hongqi/B-6993-2008; Zhu, Yuntian/B-3021-2008; Langdon, Terence/B-1487-2008; Zhao, Yonghao/A-8521-2009; Ringer, Simon/E-3487-2012; Lujan Center, LANL/G-4896-2012 OI Liao, Xiaozhou/0000-0001-8565-1758; Lavernia, Enrique/0000-0003-2124-8964; Zhu, Yuntian/0000-0002-5961-7422; Ringer, Simon/0000-0002-1559-330X; FU Australian Microscopy & Microanalysis Research Facility node at the University of Sydney; Australian Research Council [DP0772880]; Los Alamos National Laboratory; Office of Naval Research [N00014-08-1-0405]; National Science Foundation of the United States [DMR-0855009]; U.S. Army Research Office and Army Research Laboratory; China Scholarship Council FX The authors are grateful for scientific and technical input and support from the Australian Microscopy & Microanalysis Research Facility node at the University of Sydney. This project is supported by the Australian Research Council [Grant No. DP0772880 (S.N., Y.B.W., and X.Z.L.)], the LDRD program of Los Alamos National Laboratory (H.Q.L.), the Office of Naval Research [Grant No. N00014-08-1-0405 (Y.H.Z. and E.J.L.)], the National Science Foundation of the United States (Grant No. DMR-0855009, T.G.L.) and the U.S. Army Research Office and Army Research Laboratory (Y.T.Z.). S.N. also appreciates support from the China Scholarship Council. NR 42 TC 10 Z9 11 U1 1 U2 26 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD MAY 24 PY 2011 VL 528 IS 13-14 BP 4807 EP 4811 DI 10.1016/j.msea.2011.03.007 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA 756IF UT WOS:000290004200070 ER PT J AU Belof, JL Cioce, CR Xu, X Zhang, XP Space, B Woodcock, HL AF Belof, Jonathan L. Cioce, Christian R. Xu, Xue Zhang, X. Peter Space, Brian Woodcock, H. Lee TI Characterization of Tunable Radical Metal-Carbenes: Key Intermediates in Catalytic Cyclopropanation SO ORGANOMETALLICS LA English DT Article ID HIGHLY ENANTIOSELECTIVE CYCLOPROPANATION; RUTHENIUM PORPHYRIN COMPLEXES; DENSITY-FUNCTIONAL THEORY; ASYMMETRIC CYCLOPROPANATION; CHIRAL PORPHYRIN; INTRAMOLECULAR CYCLOPROPANATIONS; BENZODIAZEPINE-RECEPTOR; OLEFIN AZIRIDINATION; MOLECULAR-ORBITALS; AMINOBUTYRIC-ACID AB A new class of radical metal-carbene complex has been characterized as having Fischer-like orbital interactions and adjacent pi acceptor stabilization. Density functional theory along with natural bond orbital analysis and charge decomposition analysis has given insight into the electronics of this catalytic intermediate in an open-shell cobalt-porphyrin, [Co(Por)], system. The complex has a single bond from the metal to the carbene and has radical character with localized spin density on the carbene carbon. In addition, the carbene carbon is found to be nucleophilic and "tunable" through the introduction of different alpha-carbon substituents. Finally, based on these findings, rational design strategies are proposed that should lead to the enhancement of catalytic activity. C1 [Belof, Jonathan L.; Cioce, Christian R.; Xu, Xue; Zhang, X. Peter; Space, Brian; Woodcock, H. Lee] Univ S Florida, Dept Chem, Tampa, FL 33620 USA. [Belof, Jonathan L.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Woodcock, HL (reprint author), Univ S Florida, Dept Chem, 4202 Fowler Ave,CHE205, Tampa, FL 33620 USA. EM hlw@mail.usf.edu RI Zhang, Peter/B-7976-2011; Cioce, Christian/E-2875-2013; OI Zhang, Peter/0000-0001-7574-8409; Woodcock, Henry/0000-0003-3539-273X FU NIH [1K22HL088341-01A1]; University of South Florida; NCSA [TG-DMR090028]; NSF [CHE-0722887, CHE-0711024]; U.S. Department of Energy [DE0GG02-07ER46470]; U.S. Department of Defense [HDTRA1-08-C-0035]; Draper Laboratory [URAD2010187] FX H.L.W. would like to acknowledge NIH (1K22HL088341-01A1) and the University of South Florida (start-up) for funding. Computations were performed on the NCSA Cobalt supercomputer under a Teragrid Grant (Grant No. TG-DMR090028) to B.S., and also at the USF Research Computing Center, where NSF-funded computational resources (under Grant No. CHE-0722887) were greatly appreciated. B.S. and X.P.Z. acknowledge funding from the U.S. Department of Energy (Grant No. DE0GG02-07ER46470), the U.S. Department of Defense (Grant No. HDTRA1-08-C-0035), the National Science Foundation (Grant No. CHE-0711024), and Draper Laboratory (Grant No. URAD2010187). The authors also thank the Space Foundation (Basic and Applied Research) for partial support. NR 83 TC 32 Z9 32 U1 4 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 J9 ORGANOMETALLICS JI Organometallics PD MAY 23 PY 2011 VL 30 IS 10 BP 2739 EP 2746 DI 10.1021/om2001348 PG 8 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA 799TA UT WOS:000293307800015 PM 21643517 ER PT J AU Lavrik, NV Taylor, LT Sepaniak, MJ AF Lavrik, N. V. Taylor, L. T. Sepaniak, M. J. TI Nanotechnology and chip level systems for pressure driven liquid chromatography and emerging analytical separation techniques: A review SO ANALYTICA CHIMICA ACTA LA English DT Review DE Microfluidic; Pressure driven separation; HPLC; Pillar arrays; Liquid chromatography; Nanocolumns ID PILLAR-ARRAY COLUMNS; DETERMINISTIC LATERAL DISPLACEMENT; ELECTROSPRAY MASS-SPECTROMETRY; ENHANCED RAMAN-SCATTERING; HIGH-ASPECT-RATIO; ON-A-CHIP; CAPILLARY-ELECTROPHORESIS DEVICES; MONOLITHIC SILICA COLUMN; MICROFLUIDIC DEVICES; HPLC-CHIP AB Pressure driven liquid chromatography (LC) is a powerful and versatile separation technique particularly suitable for differentiating species present in extremely small quantities. This paper briefly reviews main historical trends and focuses on more recently developed technological approaches in miniaturization and on-chip integration of LC columns. The review emphasizes enabling technologies as well as main technological challenges specific to pressure driven separations and highlights emerging concepts that could ultimately overcome fundamental limitations of conventional LC columns. (C) 2011 Elsevier B.V. All rights reserved. C1 [Taylor, L. T.; Sepaniak, M. J.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Lavrik, N. V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37830 USA. RP Sepaniak, MJ (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM msepaniak@utk.edu RI Lavrik, Nickolay/B-5268-2011 OI Lavrik, Nickolay/0000-0002-9543-5634 FU Office of Basic Energy Sciences, U.S. Department of Energy; Office of Basic Energy Sciences; US Environmental Protection Agency [EPA-83274001]; University of Tennessee FX A portion of this work was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Office of Basic Energy Sciences, U.S. Department of Energy. NVL acknowledges support by the Office of Basic Energy Sciences. This research was also supported by the US Environmental Protection Agency STAR Program under grant EPA-83274001 with the University of Tennessee. NR 163 TC 36 Z9 37 U1 2 U2 77 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0003-2670 J9 ANAL CHIM ACTA JI Anal. Chim. Acta PD MAY 23 PY 2011 VL 694 IS 1-2 BP 6 EP 20 DI 10.1016/j.aca.2011.03.059 PG 15 WC Chemistry, Analytical SC Chemistry GA 772MZ UT WOS:000291239300002 PM 21565297 ER PT J AU Arnaldi, R Banicz, K Castor, J Chaurand, B Chen, W Cicalo, C Colla, A Cortese, P Damjanovic, S David, A de Falco, A Devaux, A Ducroux, L En'yo, H Fargeix, J Ferretti, A Floris, M Forster, A Force, P Guettet, N Guichard, A Gulkanian, H Heuser, JM Keil, M Li, Z Lourenco, C Lozano, J Manso, F Martins, P Masoni, A Neves, A Ohnishi, H Oppedisano, C Parracho, P Pillot, P Poghosyan, T Puddu, G Radermacher, E Ramalhete, P Rosinsky, P Scomparin, E Seixas, J Serci, S Shahoyan, R Sonderegger, P Specht, HJ Tieulent, R Uras, A Usai, G Veenhof, R Wohri, HK AF Arnaldi, R. Banicz, K. Castor, J. Chaurand, B. Chen, W. Cicalo, C. Colla, A. Cortese, P. Damjanovic, S. David, A. de Falco, A. Devaux, A. Ducroux, L. En'yo, H. Fargeix, J. Ferretti, A. Floris, M. Foerster, A. Force, P. Guettet, N. Guichard, A. Gulkanian, H. Heuser, J. M. Keil, M. Li, Z. Lourenco, C. Lozano, J. Manso, F. Martins, P. Masoni, A. Neves, A. Ohnishi, H. Oppedisano, C. Parracho, P. Pillot, P. Poghosyan, T. Puddu, G. Radermacher, E. Ramalhete, P. Rosinsky, P. Scomparin, E. Seixas, J. Serci, S. Shahoyan, R. Sonderegger, P. Specht, H. J. Tieulent, R. Uras, A. Usai, G. Veenhof, R. Woehri, H. K. CA NA60 Collaboration TI A comparative measurement of phi -> K+K- and phi -> mu(+)mu(-) in In-In collisions at the CERN SPS SO PHYSICS LETTERS B LA English DT Article DE Heavy ion collisions; phi puzzle ID HEAVY-ION COLLISIONS; MESON PRODUCTION; DECAYS; MATTER AB The NA60 experiment at the CERN SPS has studied phi meson production in In-In collisions at 158 AGeV via both the K+K- and the mu(+)mu(-) decay channels. The yields and inverse slope parameters of the m(T) spectra observed in the two channels are compatible within errors, different from the large discrepancies seen in Pb-Pb collisions between the hadronic (NA49) and dimuon (NA50) decay channels. Possible physics implications are discussed. (C) 2011 Elsevier B.V. All rights reserved. C1 [de Falco, A.; Floris, M.; Puddu, G.; Serci, S.; Uras, A.; Usai, G.; Woehri, H. K.] Univ Cagliari, Cagliari, Italy. [Arnaldi, R.; Oppedisano, C.; Scomparin, E.] Ist Nazl Fis Nucl, Sez Torino, Cagliari, Italy. [Banicz, K.; Damjanovic, S.; David, A.; Foerster, A.; Guettet, N.; Keil, M.; Lourenco, C.; Martins, P.; Parracho, P.; Radermacher, E.; Ramalhete, P.; Rosinsky, P.; Shahoyan, R.; Veenhof, R.] CERN, CH-1211 Geneva 23, Switzerland. [Banicz, K.; Damjanovic, S.; Specht, H. J.] Heidelberg Univ, Inst Phys, D-6900 Heidelberg, Germany. [Castor, J.; Devaux, A.; Fargeix, J.; Force, P.; Manso, F.] Univ Blaise Pascal, LPC, Clermont Ferrand, France. [Castor, J.; Devaux, A.; Force, P.; Guettet, N.] Univ Clermont Ferrand 2, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Chaurand, B.] Ecole Polytech, LLR, Palaiseau, France. [Chaurand, B.] CNRS, IN2P3, Palaiseau, France. [Chen, W.; Li, Z.] BNL, Upton, NY USA. [Cicalo, C.; Masoni, A.] Ist Nazl Fis Nucl, Sez Cagliari, Cagliari, Italy. [Colla, A.; Cortese, P.; Ferretti, A.] Univ Turin, I-10124 Turin, Italy. [David, A.; Keil, M.; Lozano, J.; Martins, P.; Neves, A.; Parracho, P.; Seixas, J.; Shahoyan, R.; Sonderegger, P.; Woehri, H. K.] Inst Super Tecn, Lisbon, Portugal. [Ducroux, L.; Guichard, A.; Pillot, P.; Tieulent, R.] Univ Lyon 1, IPN Lyon, F-69365 Lyon, France. [Ducroux, L.; Guichard, A.; Pillot, P.; Tieulent, R.] CNRS, IN2P3, Lyon, France. [En'yo, H.; Heuser, J. M.; Ohnishi, H.] RIKEN, Wako, Saitama, Japan. [Gulkanian, H.; Poghosyan, T.] Yerevan Phys Inst, Yerevan 375036, Armenia. RP de Falco, A (reprint author), Univ Cagliari, Cagliari, Italy. EM alessandro.de.falco@ca.infn.it RI En'yo, Hideto/B-2440-2015; Usai, Gianluca/E-9604-2015; Lozano-Bahilo, Julio/F-4881-2016; Ferretti, Alessandro/F-4856-2013; Tinoco Mendes, Andre David/D-4314-2011; Cortese, Pietro/G-6754-2012; Colla, Alberto/J-4694-2012 OI Usai, Gianluca/0000-0002-8659-8378; Lozano-Bahilo, Julio/0000-0003-0613-140X; Ferretti, Alessandro/0000-0001-9084-5784; Tinoco Mendes, Andre David/0000-0001-5854-7699; NR 18 TC 6 Z9 6 U1 0 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAY 23 PY 2011 VL 699 IS 5 BP 325 EP 329 DI 10.1016/j.physletb.2011.04.028 PG 5 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 771CK UT WOS:000291134600003 ER PT J AU Griggio, F Jesse, S Kumar, A Marincel, DM Tinberg, DS Kalinin, SV Trolier-McKinstry, S AF Griggio, F. Jesse, S. Kumar, A. Marincel, D. M. Tinberg, D. S. Kalinin, S. V. Trolier-McKinstry, S. TI Mapping piezoelectric nonlinearity in the Rayleigh regime using band excitation piezoresponse force microscopy SO APPLIED PHYSICS LETTERS LA English DT Article ID FERROELECTRIC THIN-FILMS; DYNAMICS AB Band excitation piezoresponse force microscopy enables local investigation of the nonlinear piezoelectric behavior of ferroelectric thin films. However, the presence of additional nonlinearity associated with the dynamic resonant response of the tip-surface junction can complicate the study of a material's nonlinearity. Here, the relative importance of the two nonlinearity sources was examined as a function of the excitation function. It was found that in order to minimize the effects of nonlinear tip-surface interactions but achieve good signal to noise level, an optimal excitation function must be used. (C) 2011 American Institute of Physics. [doi: 10.1063/1.3593138] C1 [Griggio, F.; Marincel, D. M.; Tinberg, D. S.; Trolier-McKinstry, S.] Penn State Univ, Dept Mat Sci & Engn, Mat Res Inst, Mat Res Lab, University Pk, PA 16802 USA. [Jesse, S.; Kumar, A.; Kalinin, S. V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Jesse, S.; Kumar, A.; Kalinin, S. V.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Trolier-McKinstry, S (reprint author), Penn State Univ, Dept Mat Sci & Engn, Mat Res Inst, Mat Res Lab, University Pk, PA 16802 USA. EM fxg14@psu.edu; stmckinstry@psu.edu RI Kumar, Amit/C-9662-2012; Kalinin, Sergei/I-9096-2012; Jesse, Stephen/D-3975-2016; OI Kumar, Amit/0000-0002-1194-5531; Kalinin, Sergei/0000-0001-5354-6152; Jesse, Stephen/0000-0002-1168-8483; Trolier-McKinstry, Susan/0000-0002-7267-9281 FU National Security Science and Engineering Faculty Fellowship; CNMS [CNMS2010-090]; Oak Ridge National Laboratory by the Office of Basic Energy Sciences, U. S. Department of Energy [DE-AC05-00OR22725] FX Support for this work was provided in part by the National Security Science and Engineering Faculty Fellowship and by CNMS user Proposal No. CNMS2010-090 (F. G. and S. T. M.). A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Office of Basic Energy Sciences, U. S. Department of Energy under contract DE-AC05-00OR22725. Thanks to Oleg Ovchinnikov for useful discussions on MATLAB coding. NR 14 TC 17 Z9 17 U1 1 U2 24 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 23 PY 2011 VL 98 IS 21 AR 212901 DI 10.1063/1.3593138 PG 3 WC Physics, Applied SC Physics GA 769TQ UT WOS:000291041600056 ER PT J AU Klaer, P Jenkins, CA Alijani, V Winterlik, J Balke, B Felser, C Elmers, HJ AF Klaer, P. Jenkins, C. A. Alijani, V. Winterlik, J. Balke, B. Felser, C. Elmers, H. J. TI Disentangling the Mn moments on different sublattices in the half-metallic ferrimagnet Mn3-xCoxGa SO APPLIED PHYSICS LETTERS LA English DT Article ID RAY CIRCULAR-DICHROISM AB Ferrimagnetic Mn3-xCoxGa compounds have been investigated by magnetic circular dichroism in x-ray absorption (XMCD). Compounds with x>0.5 crystallize in the CuHg2Ti structure. A tetragonal distortion of the cubic structure occurs for x <= 0.5. For the cubic phase, magnetometry reveals a linearly increasing magnetization of 2x Bohr magnetons per formula unit obeying the generalized Slater-Pauling rule. XMCD confirms the ferrimagnetic character with Mn atoms occupying two different sublattices with antiparallel spin orientation and different degrees of spin localization and identifies the region 0.6omega > I(2)) regime. We show that the energy spacing Delta E = E(1) - E(2) between the two emitted electrons provides the key parameter that controls both the energy and the angular distribution and reveals the universal features present in both the nonsequential and sequential regime. This universality, i.e., independence of (h) over bar omega, is a manifestation of the continuity across the threshold for sequential double ionization. For all photon energies considered, the energy distribution can be described by a universal shape function that contains only the spectral and temporal information entering second-order time-dependent perturbation theory. Angular correlations and distributions are found to be more sensitive to the value of (h) over bar omega. In particular, shake-up interferences have a large effect on the angular distribution. Energy spectra, angular distributions parametrized by the anisotropy parameters beta(j), and total cross sections presented in this paper are obtained by fully correlated time-dependent ab initio calculations. C1 [Pazourek, R.; Feist, J.; Nagele, S.; Persson, E.; Burgdoerfer, J.] Vienna Univ Technol, Inst Theoret Phys, A-1040 Vienna, Austria. [Feist, J.] Harvard Smithsonian Ctr Astrophys, ITAMP, Cambridge, MA 02138 USA. [Schneider, B. I.] Natl Sci Fdn, Div Phys, Off Cyberinfrastruct, Arlington, VA 22230 USA. [Collins, L. A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Pazourek, R (reprint author), Vienna Univ Technol, Inst Theoret Phys, A-1040 Vienna, Austria. EM renate.pazourek@tuwien.ac.at RI Nagele, Stefan/E-6938-2011; Feist, Johannes/J-7394-2012 OI Nagele, Stefan/0000-0003-1213-0294; Feist, Johannes/0000-0002-7972-0646 FU FWF-Austria [SFB016, P21141-N16]; NSF [TG-PHY090031]; US Department of Energy [DE-AC52-06NA25396] FX We thank I. Ivanov for sending us results in numerical form. R.P., J.F., S.N., E.P., and J.B. acknowledge support by the FWF-Austria, Grants No. SFB016 and No. P21141-N16. J.F. acknowledges support by the NSF through a grant to ITAMP. This research was supported in part by the National Science Foundation through TeraGrid resources provided by NICS and TACC under Grant No. TG-PHY090031. Additional computational time was provided by the Vienna Scientific Cluster (VSC) and under Institutional Computing at Los Alamos National Laboratory. The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the National Nuclear Security Administration of the US Department of Energy under Contract No. DE-AC52-06NA25396. NR 54 TC 29 Z9 30 U1 0 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 J9 PHYS REV A JI Phys. Rev. A PD MAY 20 PY 2011 VL 83 IS 5 AR 053418 DI 10.1103/PhysRevA.83.053418 PG 11 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 767MF UT WOS:000290860000009 ER PT J AU Koretsune, T Saito, S Cohen, ML AF Koretsune, Takashi Saito, Susumu Cohen, Marvin L. TI One-dimensional alkali-doped C-60 chains encapsulated in BN nanotubes SO PHYSICAL REVIEW B LA English DT Article ID BORON-NITRIDE NANOTUBES; ELECTRON-PHONON INTERACTIONS; CARBON NANOTUBE; SUPERCONDUCTIVITY; MICROTUBULES AB We study the energetics, electronic structures, and electron-phonon couplings of a one-dimensional potassium-doped C-60 chain encapsulated in a boron nitride nanotube using the framework of the density-functional theory. We demonstrate that the reaction of potassium doping is exothermic and the resulting material is one-dimensional metal where conducting electrons are only in the C-60 chain. Interestingly, the Fermi-level density of states has a peculiar pressure dependence and can be larger than those in the three-dimensional alkali-doped fullerene compounds, indicating the possibility of various phase transitions. We also discuss the electron-phonon couplings and the possibility of superconductivity. C1 [Koretsune, Takashi; Saito, Susumu] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan. [Cohen, Marvin L.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Cohen, Marvin L.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Koretsune, T (reprint author), Tokyo Inst Technol, Dept Phys, Meguro Ku, 2-12-1 Oh Okayama, Tokyo 1528551, Japan. RI Koretsune, Takashi/D-3209-2017 OI Koretsune, Takashi/0000-0002-5334-0792 FU National Science Foundation [DMR07-05941]; Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy [DE-AC02-05CH11231]; MEXT Japan [22740252, 22013005, 19054005]; Ishikawa Carbon Foundation; MEXT Japan through the Tokyo Institute of Technology FX We would like to thank J. Noffsinger for useful discussions. Numerical calculations were performed on TSUB-AME Grid Cluster at Global Scientific Information and Computing Center of the Tokyo Institute of Technology. This work was partially supported by National Science Foundation Grant No. DMR07-05941, by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy under Contract No. DE-AC02-05CH11231, by a Grant-in-Aid for Scientific Research (Contracts No. 22740252, No. 22013005, and No. 19054005) and Elements Science and Technology Project from MEXT Japan, by Ishikawa Carbon Foundation, and by the Global Center of Excellence Program by MEXT Japan through the "Nanoscience and Quantum Physics" Project of the Tokyo Institute of Technology. NR 31 TC 1 Z9 1 U1 1 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 20 PY 2011 VL 83 IS 19 AR 193406 DI 10.1103/PhysRevB.83.193406 PG 4 WC Physics, Condensed Matter SC Physics GA 767OC UT WOS:000290864900001 ER PT J AU Zaki, N Knox, K Johnson, PD Fujii, J Vobornik, I Panaccione, G Osgood, RM AF Zaki, N. Knox, K. Johnson, P. D. Fujii, J. Vobornik, I. Panaccione, G. Osgood, R. M. TI Surface states on vicinal Cu(775): STM and photoemission study SO PHYSICAL REVIEW B LA English DT Article ID STEP MODULATION; WAVE-FUNCTION; TERRACE AB We report angle-resolved photoemission spectroscopy (ARPES) and a set of in situ scanning tunneling microscopy (STM) measurements on a narrow-terrace-width vicinal Cu(111) crystal surface, Cu(775), whose vicinal cut lies close to the transition between terrace and step modulation. These measurements show sharp zone-folding (or umklapp) features with a periodicity in k(parallel to), indicating that the predominant reference plane is that of Cu(775), i.e., that the surface is predominately step-modulated. Our measurements also show variation in umklapp intensity with photon energy, which is consistent with prior ARPES experiments on other vicinal Cu(111) surfaces and in agreement with our designation of the state as being step-modulated. The measurements also show a weak terrace-modulated state, which, based on several characteristics, we attribute to the presence of terrace widths larger than the ideal terrace width. By measuring the intensity ratio of the two distinct surface-state modulations from photoemission and the terrace-width distribution from STM, we derive a value for the terrace width at which the surface state switches between the two modulations. C1 [Zaki, N.; Knox, K.; Osgood, R. M.] Columbia Univ, New York, NY 10027 USA. [Johnson, P. D.] Brookhaven Natl Lab, New York, NY 11973 USA. [Fujii, J.; Vobornik, I.; Panaccione, G.] Lab TASC, Ist Officina Mat Consiglio Nazl Ric IOM CNR, I-34149 Trieste, Italy. RP Zaki, N (reprint author), Columbia Univ, New York, NY 10027 USA. RI Vobornik, Ivana/B-9463-2015; Vobornik, Ivana/A-7461-2011; OI Vobornik, Ivana/0000-0001-9957-3535; Jun, Fujii/0000-0003-3208-802X FU Department of Energy [DE-FG 02-04-ER-46157, DE-AC02-98CH10886] FX This research was supported by the Department of Energy Contract No. DE-FG 02-04-ER-46157. Work at Brookhaven National Laboratory was supported by the Department of Energy under Contract No. DE-AC02-98CH10886. We thank Jerry Dadap, Mehmet Yilmaz, and Manolis Antonoyiannak for several useful comments and suggestions. We thank Peter Lucak for writing some of the step-width analysis code. NR 24 TC 7 Z9 7 U1 2 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 20 PY 2011 VL 83 IS 20 AR 205420 DI 10.1103/PhysRevB.83.205420 PG 7 WC Physics, Condensed Matter SC Physics GA 767OV UT WOS:000290866800007 ER PT J AU Yeoh, EY Zhu, SJ Hamilton, JH Li, K Ramayya, AV Liu, YX Hwang, JK Liu, SH Wang, JG Sun, Y Sheikh, JA Bhat, GH Luo, YX Rasmussen, JO Lee, IY Ding, HB Gu, L Xu, Q Xiao, ZG Ma, WC AF Yeoh, E. Y. Zhu, S. J. Hamilton, J. H. Li, K. Ramayya, A. V. Liu, Y. X. Hwang, J. K. Liu, S. H. Wang, J. G. Sun, Y. Sheikh, J. A. Bhat, G. H. Luo, Y. X. Rasmussen, J. O. Lee, I. Y. Ding, H. B. Gu, L. Xu, Q. Xiao, Z. G. Ma, W. C. TI High-spin structure and multiphonon gamma vibrations in very neutron-rich Ru-114 SO PHYSICAL REVIEW C LA English DT Article ID PROJECTED SHELL-MODEL; IDENTICAL BANDS; PARITY BANDS; RU-108,RU-110,RU-112; NUCLEI; ISOTOPES; STATES AB High-spin levels of the neutron-rich Ru-114 have been investigated by measuring the prompt. rays in the spontaneous fission of Cf-252. The ground-state band and one-phonon gamma-vibrational band have been extended up to 14(+) and 9(+), respectively. Two levels are proposed as the members of a two-phonon gamma-vibrational band. A back bending (band crossing) has been observed in the ground-state band at (h) over bar omega approximate to 0.40 MeV. Using the triaxial deformation parameters, the cranked shell model calculations indicate that this back bending in Ru-114 should originate from the alignment of a pair of h(11/2) neutrons. Triaxial projected shell model calculations for the gamma-vibrational band structures of Ru-114 are in good agreement with the experimental data. However, when using the oblate deformation parameters, both of the above-calculated results are not in agreement with the experimental data. C1 [Yeoh, E. Y.; Zhu, S. J.; Wang, J. G.; Ding, H. B.; Gu, L.; Xu, Q.; Xiao, Z. G.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Zhu, S. J.; Hamilton, J. H.; Li, K.; Ramayya, A. V.; Hwang, J. K.; Liu, S. H.; Luo, Y. X.] Vanderbilt Univ, Dept Phys, Nashville, TN 37235 USA. [Liu, Y. X.] Huzhou Teachers Coll, Sch Sci, Huzhou 313000, Peoples R China. [Liu, S. H.] UNIRIB Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. [Sun, Y.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200240, Peoples R China. [Sheikh, J. A.; Bhat, G. H.] Univ Kashmir, Dept Phys, Srinagar 190006, Jammu & Kashmir, India. [Luo, Y. X.; Rasmussen, J. O.; Lee, I. Y.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Ma, W. C.] Mississippi State Univ, Dept Phys, Mississippi State, MS 39762 USA. RP Yeoh, EY (reprint author), Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. EM zhushj@mail.tsinghua.edu.cn RI XIAO, Zhigang/C-3788-2015; Sun, Yang/P-2417-2015 FU National Natural Science Foundation of China [10975082, 10875077, 10975051, 11075103]; Major State Basic Research Development Program [2007CB815005]; Higher Education Science Foundation [20100002110077]; US Department of Energ [DE-FG05-88ER40407]; [DE-AC03-76SF00098] FX The work at Tsinghua University, Shanghai Jiao Tong University, and Huzhou Teachers College was supported by the National Natural Science Foundation of China under Grants No. 10975082, No. 10875077, No. 10975051, and No. 11075103, the Major State Basic Research Development Program under Grant No. 2007CB815005, and the Special Program of Higher Education Science Foundation under Grant No. 20100002110077, respectively. The work at Vanderbilt University and LBNL was supported by the US Department of Energy under Grant No. DE-FG05-88ER40407 and Contract No. DE-AC03-76SF00098, respectively. NR 28 TC 11 Z9 13 U1 0 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 J9 PHYS REV C JI Phys. Rev. C PD MAY 20 PY 2011 VL 83 IS 5 AR 054317 DI 10.1103/PhysRevC.83.054317 PG 6 WC Physics, Nuclear SC Physics GA 767RX UT WOS:000290874800001 ER PT J AU An, YQ Taylor, AJ Conradson, SD Trugman, SA Durakiewicz, T Rodriguez, G AF An, Yong Q. Taylor, Antoinette J. Conradson, Steven D. Trugman, Stuart A. Durakiewicz, Tomasz Rodriguez, George TI Ultrafast Hopping Dynamics of 5f Electrons in the Mott Insulator UO2 Studied by Femtosecond Pump-Probe Spectroscopy SO PHYSICAL REVIEW LETTERS LA English DT Article ID URANIUM-DIOXIDE; POLARON; CRYSTAL; PHONONS; ENERGY AB We describe a femtosecond pump-probe study of ultrafast hopping dynamics of 5f electrons in the Mott insulator UO2 following Mott-gap excitation at temperatures of 5-300 K. Hopping-induced response of the lattice and electrons is probed by transient reflectivity at mid- and above-gap photon energies, respectively. These measurements show an instantaneous hop, subsequent picosecond lattice deformation, followed by acoustic phonon emission and microsecond relaxation. Temperature-dependent studies indicate that the slow relaxation results from Hubbard excitons formed by U3+ - U5+ pairs. C1 [An, Yong Q.; Taylor, Antoinette J.; Conradson, Steven D.; Trugman, Stuart A.; Durakiewicz, Tomasz; Rodriguez, George] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP An, YQ (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM yqan@lanl.gov RI An, Yong/N-7479-2013; Rodriguez, George/G-7571-2012; OI Rodriguez, George/0000-0002-6044-9462; Durakiewicz, Tomasz/0000-0002-1980-1874; Trugman, Stuart/0000-0002-6688-7228 FU LDRD; BES FX We thank R. L. Martin, J. Demsar, Y.-S. Park, and M. T. Paffett for helpful contributions. This work was performed, in part, at CINT and supported by LDRD and BES core materials program. NR 23 TC 16 Z9 16 U1 3 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 207402 DI 10.1103/PhysRevLett.106.207402 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200025 PM 21668262 ER PT J AU Banerjee, P Haxton, WC Qian, YZ AF Banerjee, Projjwal Haxton, W. C. Qian, Yong-Zhong TI Long, Cold, Early r Process? Neutrino-Induced Nucleosynthesis in He Shells Revisited SO PHYSICAL REVIEW LETTERS LA English DT Article ID BLACK-HOLE FORMATION; STAR MERGERS; HELIUM SHELL; EARLY GALAXY; SUPERNOVAE; EVOLUTION; ELEMENTS; ABUNDANCES; DEPENDENCE; DYNAMICS AB We revisit a nu-driven r-process mechanism in the He shell of a core-collapse supernova, finding that it could succeed in early stars of metallicity Z less than or similar to 10(-3)Z(circle dot), at relatively low temperatures and neutron densities, producing A similar to 130 and 195 abundance peaks over similar to 10-20 s. The mechanism is sensitive to the nu emission model and to nu oscillations. We discuss the implications of an r process that could alter interpretations of abundance data from metal-poor stars, and point out the need for further calculations that include effects of the supernova shock. C1 [Banerjee, Projjwal; Qian, Yong-Zhong] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Haxton, W. C.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Haxton, W. C.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Banerjee, P (reprint author), Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. EM banerjee@physics.umn.edu; haxton@berkeley.edu; qian@physics.umn.edu FU U.S. DOE at UMN [DE-FG02-87ER40328]; U.S. DOE at Berkeley [DE-SC00046548] FX We thank Alexander Heger for discussions of massive stars and Frank Timmes and Rob Hoffman for help with the torch network. This work was supported in part by the U.S. DOE under DE-FG02-87ER40328 at UMN and DE-SC00046548 at Berkeley. NR 28 TC 35 Z9 35 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 201104 DI 10.1103/PhysRevLett.106.201104 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200007 PM 21668217 ER PT J AU Drut, JE Lahde, TA Ten, T AF Drut, Joaquin E. Lahde, Timo A. Ten, Timour TI Momentum Distribution and Contact of the Unitary Fermi Gas SO PHYSICAL REVIEW LETTERS LA English DT Article ID PHYSICS; MATTER; ATOMS AB We calculate the momentum distribution n(k) of the unitary Fermi gas by using quantum Monte Carlo calculations at finite temperature T/epsilon(F) as well as in the ground state. At large momenta k/k(F), we find that n(k) falls off as C/k(4), in agreement with the Tan relations. From the asymptotics of n(k), we determine the contact C as a function of T/epsilon(F) and present a comparison with theory. At low T/epsilon(F), we find that C increases with temperature, and we tentatively identify a maximum around T/epsilon(F) similar or equal to 0.4. Our calculations are performed on lattices of spatial extent up to N(x) = 14 with a particle number per unit volume of similar or equal to 0.03-0.07. C1 [Drut, Joaquin E.; Ten, Timour] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Drut, Joaquin E.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Lahde, Timo A.] Aalto Univ, Helsinki Inst Phys, FI-00076 Espoo, Finland. [Lahde, Timo A.] Aalto Univ, Dept Appl Phys, FI-00076 Espoo, Finland. [Ten, Timour] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. RP Drut, JE (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. FU U.S. DOE [DE-FG02-00ER41132, DE-AC02-05CH11231]; UNEDF SciDAC Collaboration [DE-FC02-09ER41586]; NSF [PHY-0653312]; Academy of Finland; Vilho, Yrjo, and Kalle Vaisala Foundation of the Finnish Academy of Science and Letters; Waldemar von Frenckell Foundation of the Finnish Society of Sciences and Letters; Magnus Ehrnrooth Foundation of the Finnish Society of Sciences and Letters FX We thank R. J. Furnstahl for encouragement and A. Bulgac, J. Carlson, S. Gandolfi, A. Gezerlis, and K. Schmidt for instructive discussions and comments. We are also grateful to T. Enss, H. Hu, and F. Palestini for giving us access to their respective results. We acknowledge support under U.S. DOE Grants No. DE-FG02-00ER41132 and No. DE-AC02-05CH11231, UNEDF SciDAC Collaboration Grant No. DE-FC02-09ER41586, and NSF Grant No. PHY-0653312. This study was supported, in part, by the Academy of Finland through its Centers of Excellence Program (2006-2011), the Vilho, Yrjo, and Kalle Vaisala Foundation of the Finnish Academy of Science and Letters, and the Waldemar von Frenckell and Magnus Ehrnrooth Foundations of the Finnish Society of Sciences and Letters. Part of this work was performed by using an allocation of computing time from the Ohio Supercomputer Center. NR 59 TC 38 Z9 38 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 205302 DI 10.1103/PhysRevLett.106.205302 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200016 PM 21668239 ER PT J AU Harvey-Thompson, AJ Lebedev, SV Burdiak, G Waisman, EM Hall, GN Suzuki-Vidal, F Bland, SN Chittenden, JP De Grouchy, P Khoory, E Pickworth, L Skidmore, J Swadling, G AF Harvey-Thompson, A. J. Lebedev, S. V. Burdiak, G. Waisman, E. M. Hall, G. N. Suzuki-Vidal, F. Bland, S. N. Chittenden, J. P. De Grouchy, P. Khoory, E. Pickworth, L. Skidmore, J. Swadling, G. TI Suppression of the Ablation Phase in Wire Array Z Pinches Using a Tailored Current Prepulse SO PHYSICAL REVIEW LETTERS LA English DT Article ID ENHANCEMENT; IMPLOSION; POWER AB A new wire array configuration has been used to create thin shell-like implosions in a cylindrical array. The setup introduces a similar to 5 kA, similar to 25 ns current prepulse followed by a similar to 140 ns current-free interval before the application of the main (similar to 1 MA) current pulse. The prepulse volumetrically heats the wires which expand to similar to 1 mm diameter leaving no dense wire core and without development of instabilities. The main current pulse then ionizes all the array mass resulting in suppression of the ablation phase, an accelerating implosion, and no trailing mass. Rayleigh-Taylor instability growth in the imploding plasma is inferred to be seeded by mu m-scale perturbations on the surface of the wires. The absence of wire cores is found to be the critical factor in altering the implosion dynamics. C1 [Harvey-Thompson, A. J.; Lebedev, S. V.; Burdiak, G.; Hall, G. N.; Suzuki-Vidal, F.; Bland, S. N.; Chittenden, J. P.; De Grouchy, P.; Khoory, E.; Pickworth, L.; Skidmore, J.; Swadling, G.] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, London SW7 2BW, England. [Waisman, E. M.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Harvey-Thompson, AJ (reprint author), Univ London Imperial Coll Sci Technol & Med, Blackett Lab, London SW7 2BW, England. RI Hall, Gareth/C-4179-2015; Swadling, George/S-5980-2016 OI Swadling, George/0000-0001-8370-8837 FU Sandia National Laboratories Albuquerque; NNSA under DOE [DE-F03-02NA00057] FX The authors are grateful to Dr. M. E. Cuneo and Dr. R. B. Spielman for many useful discussions. This research was sponsored by Sandia National Laboratories Albuquerque and the NNSA under DOE Cooperative Agreement No. DE-F03-02NA00057. NR 13 TC 26 Z9 28 U1 1 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 205002 DI 10.1103/PhysRevLett.106.205002 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200014 PM 21668237 ER PT J AU Lo, CC Lang, V George, RE Morton, JJL Tyryshkin, AM Lyon, SA Bokor, J Schenkel, T AF Lo, C. C. Lang, V. George, R. E. Morton, J. J. L. Tyryshkin, A. M. Lyon, S. A. Bokor, J. Schenkel, T. TI Electrically Detected Magnetic Resonance of Neutral Donors Interacting with a Two-Dimensional Electron Gas SO PHYSICAL REVIEW LETTERS LA English DT Article ID SPIN-RESONANCE; SILICON; SCATTERING AB We have measured the electrically detected magnetic resonance of donor-doped silicon field-effect transistors in resonant X- (9.7 GHz) and W-band (94 GHz) microwave cavities. The two-dimensional electron gas resonance signal increases by 2 orders of magnitude from X to W band, while the donor resonance signals are enhanced by over 1 order of magnitude. Bolometric effects and spin-dependent scattering are inconsistent with the observations. We propose that polarization transfer from the donor to the two-dimensional electron gas is the main mechanism giving rise to the spin resonance signals. C1 [Lo, C. C.; Bokor, J.] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Lang, V.; Morton, J. J. L.] Univ Oxford, Dept Mat, Oxford OX1 3PH, England. [George, R. E.; Morton, J. J. L.] Univ Oxford, Dept Phys, Clarendon Lab, CAESR, Oxford OX1 3PU, England. [Tyryshkin, A. M.; Lyon, S. A.] Princeton Univ, Dept Elect Engn, Princeton, NJ 08544 USA. [Schenkel, T.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Accelerator & Fus Res, Berkeley, CA 94720 USA. RP Lo, CC (reprint author), Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. EM cclo@eecs.berkeley.edu; volker.lang@materials.ox.ac.uk RI Morton, John/I-3515-2013; Bokor, Jeffrey/A-2683-2011 FU U.S. National Security Agency [100000080295]; DOE [DE-AC02-05CH11231 (LBNL)]; EPSRC [EP/D048559/1 (Oxford)]; NSF [DMR-0213706 (Princeton)]; Konrad-Adenauer-Stiftung e.V; Royal Society; St. John's College, Oxford FX We thank A. Ardavan, R. de Sousa, and T. Last for useful discussions, and the UC Berkeley Microlab staff for technical support in device fabrication. This work was supported by the U.S. National Security Agency under 100000080295. Additional support by the DOE under Contract No. DE-AC02-05CH11231 (LBNL), EPSRC through CAESR EP/D048559/1 (Oxford), and NSF through the Princeton MRSEC under Grant No. DMR-0213706 (Princeton) are also acknowledged. V. L. is supported by Konrad-Adenauer-Stiftung e.V. and EPSRC DTA. J.J.L.M. is supported by The Royal Society and St. John's College, Oxford. NR 31 TC 21 Z9 21 U1 1 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 207601 DI 10.1103/PhysRevLett.106.207601 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200026 PM 21668263 ER PT J AU Maris, P Vary, JP Navratil, P Ormand, WE Nam, H Dean, DJ AF Maris, P. Vary, J. P. Navratil, P. Ormand, W. E. Nam, H. Dean, D. J. TI Origin of the Anomalous Long Lifetime of C-14 SO PHYSICAL REVIEW LETTERS LA English DT Article ID EFFECTIVE-FIELD THEORY; MODEL-OPERATOR APPROACH; CHIRAL LAGRANGIANS; NUCLEAR-FORCES; SYSTEMS AB We report the microscopic origins of the anomalously suppressed beta decay of C-14 to N-14 using the ab initio no-core shell model with the Hamiltonian from the chiral effective field theory including three-nucleon force terms. The three-nucleon force induces unexpectedly large cancellations within the p shell between contributions to beta decay, which reduce the traditionally large contributions from the nucleon-nucleon interactions by an order of magnitude, leading to the long lifetime of C-14. C1 [Maris, P.; Vary, J. P.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Navratil, P.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Navratil, P.; Ormand, W. E.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Ormand, W. E.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Nam, H.; Dean, D. J.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Maris, P (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. FU U.S. DOE (UNEDF SciDAC Collaboration) [DE-FC02-09ER41582, DE-FG02-87ER40371]; DOE Office of Science [DE-AC05-00OR22725]; U.S. DOE [DE-AC05-00OR22725, DE-AC52-07NA27344] FX This work was supported in part by U.S. DOE Grants No. DE-FC02-09ER41582 (UNEDF SciDAC Collaboration) and No. DE-FG02-87ER40371 and by U.S. DOE Contracts No. DE-AC52-07NA27344 and No. DE-AC05-00OR22725. Computational resources were provided by Livermore Computing at LLNL and by the Oak Ridge Leadership Computing Facility at ORNL [21], which is supported by the DOE Office of Science under Contract No. DE-AC05-00OR22725. NR 34 TC 54 Z9 55 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 202502 DI 10.1103/PhysRevLett.106.202502 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200008 PM 21668224 ER PT J AU Velizhanin, KA Piryatinski, A AF Velizhanin, Kirill A. Piryatinski, Andrei TI Numerical Study of Carrier Multiplication Pathways in Photoexcited Nanocrystal and Bulk Forms of PbSe SO PHYSICAL REVIEW LETTERS LA English DT Article ID MULTIPLE EXCITON GENERATION; QUANTUM DOTS; SEMICONDUCTOR NANOCRYSTALS; MULTIEXCITON GENERATION; IMPACT IONIZATION; SOLAR-CELLS; EFFICIENCY AB Employing the interband exciton scattering model, we perform a numerical study of the direct photogeneration and population relaxation processes contributing to carrier multiplication (CM) in nanocrystalline and bulk PbSe. We argue that in both cases the impact ionization is the main mechanism of CM. This explains the weak contribution of the direct photogeneration to the total quantum efficiency (QE). An investigation of the size scaling of QE in nanocrystals and a comparison to the bulk limit provide microscopic insight into the experimentally observed trends. C1 [Velizhanin, Kirill A.; Piryatinski, Andrei] Los Alamos Natl Lab, Div Theoret, Ctr Nonlinear Studies CNLS, Los Alamos, NM 87545 USA. RP Velizhanin, KA (reprint author), Los Alamos Natl Lab, Div Theoret, Ctr Nonlinear Studies CNLS, Los Alamos, NM 87545 USA. EM apiryat@lanl.gov RI Piryatinski, Andrei/B-5543-2009; Velizhanin, Kirill/C-4835-2008 FU BES Office; DOE; Los Alamos LDRD; CNLS FX This work was supported by the BES Office, DOE, Los Alamos LDRD funds, and CNLS. We thank V. Klimov and D. Smith for stimulating discussions and comments on the manuscript. NR 27 TC 26 Z9 26 U1 0 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 207401 DI 10.1103/PhysRevLett.106.207401 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200024 PM 21668261 ER PT J AU Vieyra, HA Oeschler, N Seiro, S Jeevan, HS Geibel, C Parker, D Steglich, F AF Vieyra, H. A. Oeschler, N. Seiro, S. Jeevan, H. S. Geibel, C. Parker, D. Steglich, F. TI Determination of Gap Symmetry from Angle-Dependent Hc2 Measurements on CeCu2Si2 SO PHYSICAL REVIEW LETTERS LA English DT Article ID ANGULAR-DEPENDENCE; CRITICAL FIELDS; SUPERCONDUCTIVITY; MAGNETISM; CRYSTAL; STATE AB The tetragonal heavy-fermion compound CeCu2Si2 exhibits a superconducting ground state (S type, T-c = 0.67 K) close to a magnetic instability. Here, we present angle-resolved resistivity measurements of the upper critical field H-c2. In-plane rotation of S-type CeCu2Si2 single crystals reveals a fourfold oscillation of H-c2. An extended weak-coupling BCS model for a d-wave symmetry including strong Pauli-limiting effects confirms the aforementioned angular dependence and points towards d(xy) symmetry of the order parameter. C1 [Vieyra, H. A.; Oeschler, N.; Seiro, S.; Jeevan, H. S.; Geibel, C.; Steglich, F.] Max Planck Inst Chem Phys Solids, D-01187 Dresden, Germany. [Parker, D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Vieyra, HA (reprint author), Max Planck Inst Chem Phys Solids, Nothnitzer Str 40, D-01187 Dresden, Germany. EM Hugo.Vieyra@cpfs.mpg.de FU IMPRS-Dresden; U.S. Department of Energy, Basic Energy Sciences, Materials Science and Engineering FX We are grateful to Peter Thalmeier for helpful discussions. H. A. V. acknowledges support by the IMPRS-Dresden. Work at ORNL supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Science and Engineering. NR 32 TC 17 Z9 17 U1 2 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 207001 DI 10.1103/PhysRevLett.106.207001 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200021 PM 21668257 ER PT J AU Zhang, Y Ke, XZ Chen, CF Yang, JH Kent, PRC AF Zhang, Yi Ke, Xuezhi Chen, Changfeng Yang, Jihui Kent, Paul R. C. TI Nanodopant-Induced Band Modulation in AgPbmSbTe2+m-Type Thermoelectrics SO PHYSICAL REVIEW LETTERS LA English DT Article ID SOLID-SOLUTIONS; HIGH FIGURE; MERIT; PBTE; GAPS; SB; BI AB The structure-property relation is a key outstanding problem in the study of nanocomposite materials. Here we elucidate the fundamental physics of nanodopants in thermoelectric nanocomposites XPbmYTe2+m (X = Ag, Na; Y = Sb, Bi). First-principles calculations unveil a sizable band-gap widening driven by nanodopant-induced lattice strain and a band split-off mainly caused by the spin-orbit interaction in nanodopant. Boltzmann transport calculations on PbTe with modified band mimicking nanodopant-induced modulations show significant but competing effects on high-temperature electron transport behavior. These results offer insights for understanding experimental findings and optimizing thermoelectric properties of narrow band-gap semiconductor nanocomposites. C1 [Zhang, Yi; Ke, Xuezhi; Chen, Changfeng] Univ Nevada, Dept Phys, Las Vegas, NV 89154 USA. [Zhang, Yi; Ke, Xuezhi; Chen, Changfeng] Univ Nevada, HiPSEC, Las Vegas, NV 89154 USA. [Ke, Xuezhi] E China Normal Univ, Dept Phys, Shanghai 200062, Peoples R China. [Yang, Jihui] GM RD Ctr, Elect Energy Res Lab, Warren, MI 48090 USA. [Kent, Paul R. C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Zhang, Y (reprint author), Univ Nevada, Dept Phys, Las Vegas, NV 89154 USA. RI Zhang, Yi/C-9291-2011; Yang, Jihui/A-3109-2009; Kent, Paul/A-6756-2008 OI Kent, Paul/0000-0001-5539-4017 FU DOE [DE-FC52-06NA26274, DE-FC26-04NT42278]; GM; DOE Offices of Advanced Scientific Computing Research and Basic Energy Sciences; NSFC [11074074] FX This work was supported by DOE Grants No. DE-FC52-06NA26274, No. DE-FC26-04NT42278, and by GM, and used resources of NCCS and CNMS at ORNL, sponsored by DOE Offices of Advanced Scientific Computing Research and Basic Energy Sciences. X. K. is also supported by NSFC Grant No. 11074074. NR 30 TC 14 Z9 14 U1 0 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 206601 DI 10.1103/PhysRevLett.106.206601 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200019 PM 21668249 ER PT J AU Banks, JA Nishiyama, T Hasebe, M Bowman, JL Gribskov, M dePamphilis, C Albert, VA Aono, N Aoyama, T Ambrose, BA Ashton, NW Axtell, MJ Barker, E Barker, MS Bennetzen, JL Bonawitz, ND Chapple, C Cheng, CY Correa, LGG Dacre, M DeBarry, J Dreyer, I Elias, M Engstrom, EM Estelle, M Feng, L Finet, C Floyd, SK Frommer, WB Fujita, T Gramzow, L Gutensohn, M Harholt, J Hattori, M Heyl, A Hirai, T Hiwatashi, Y Ishikawa, M Iwata, M Karol, KG Koehler, B Kolukisaoglu, U Kubo, M Kurata, T Lalonde, S Li, KJ Li, Y Litt, A Lyons, E Manning, G Maruyama, T Michael, TP Mikami, K Miyazaki, S Morinaga, S Murata, T Mueller-Roeber, B Nelson, DR Obara, M Oguri, Y Olmstead, RG Onodera, N Petersen, BL Pils, B Prigge, M Rensing, SA Riano-Pachon, DM Roberts, AW Sato, Y Scheller, HV Schulz, B Schulz, C Shakirov, EV Shibagaki, N Shinohara, N Shippen, DE Sorensen, I Sotooka, R Sugimoto, N Sugita, M Sumikawa, N Tanurdzic, M Theissen, G Ulvskov, P Wakazuki, S Weng, JK Willats, WWGT Wipf, D Wolf, PG Yang, LX Zimmer, AD Zhu, QH Mitros, T Hellsten, U Loque, D Otillar, R Salamov, A Schmutz, J Shapiro, H Lindquist, E Lucas, S Rokhsar, D Grigoriev, IV AF Banks, Jo Ann Nishiyama, Tomoaki Hasebe, Mitsuyasu Bowman, John L. Gribskov, Michael dePamphilis, Claude Albert, Victor A. Aono, Naoki Aoyama, Tsuyoshi Ambrose, Barbara A. Ashton, Neil W. Axtell, Michael J. Barker, Elizabeth Barker, Michael S. Bennetzen, Jeffrey L. Bonawitz, Nicholas D. Chapple, Clint Cheng, Chaoyang Correa, Luiz Gustavo Guedes Dacre, Michael DeBarry, Jeremy Dreyer, Ingo Elias, Marek Engstrom, Eric M. Estelle, Mark Feng, Liang Finet, Cedric Floyd, Sandra K. Frommer, Wolf B. Fujita, Tomomichi Gramzow, Lydia Gutensohn, Michael Harholt, Jesper Hattori, Mitsuru Heyl, Alexander Hirai, Tadayoshi Hiwatashi, Yuji Ishikawa, Masaki Iwata, Mineko Karol, Kenneth G. Koehler, Barbara Kolukisaoglu, Uener Kubo, Minoru Kurata, Tetsuya Lalonde, Sylvie Li, Kejie Li, Ying Litt, Amy Lyons, Eric Manning, Gerard Maruyama, Takeshi Michael, Todd P. Mikami, Koji Miyazaki, Saori Morinaga, Shin-ichi Murata, Takashi Mueller-Roeber, Bernd Nelson, David R. Obara, Mari Oguri, Yasuko Olmstead, Richard G. Onodera, Naoko Petersen, Bent Larsen Pils, Birgit Prigge, Michael Rensing, Stefan A. Mauricio Riano-Pachon, Diego Roberts, Alison W. Sato, Yoshikatsu Scheller, Henrik Vibe Schulz, Burkhard Schulz, Christian Shakirov, Eugene V. Shibagaki, Nakako Shinohara, Naoki Shippen, Dorothy E. Sorensen, Iben Sotooka, Ryo Sugimoto, Nagisa Sugita, Mamoru Sumikawa, Naomi Tanurdzic, Milos Theissen, Guenter Ulvskov, Peter Wakazuki, Sachiko Weng, Jing-Ke Willats, William W. G. T. Wipf, Daniel Wolf, Paul G. Yang, Lixing Zimmer, Andreas D. Zhu, Qihui Mitros, Therese Hellsten, Uffe Loque, Dominique Otillar, Robert Salamov, Asaf Schmutz, Jeremy Shapiro, Harris Lindquist, Erika Lucas, Susan Rokhsar, Daniel Grigoriev, Igor V. TI The Selaginella Genome Identifies Genetic Changes Associated with the Evolution of Vascular Plants SO SCIENCE LA English DT Article ID SMALL RNAS; MESSENGER-RNAS; ARABIDOPSIS; MOELLENDORFFII; MECHANISM; LAND; PERSPECTIVE; SIRNAS AB Vascular plants appeared similar to 410 million years ago, then diverged into several lineages of which only two survive: the euphyllophytes (ferns and seed plants) and the lycophytes. We report here the genome sequence of the lycophyte Selaginella moellendorffii (Selaginella), the first nonseed vascular plant genome reported. By comparing gene content in evolutionarily diverse taxa, we found that the transition from a gametophyte- to a sporophyte-dominated life cycle required far fewer new genes than the transition from a nonseed vascular to a flowering plant, whereas secondary metabolic genes expanded extensively and in parallel in the lycophyte and angiosperm lineages. Selaginella differs in posttranscriptional gene regulation, including small RNA regulation of repetitive elements, an absence of the trans-acting small interfering RNA pathway, and extensive RNA editing of organellar genes. C1 [Banks, Jo Ann] Purdue Univ, Dept Bot & Plant Pathol, W Lafayette, IN 47907 USA. [Nishiyama, Tomoaki] Kanazawa Univ, Adv Sci Res Ctr, Kanazawa, Ishikawa 9200934, Japan. [Nishiyama, Tomoaki; Hasebe, Mitsuyasu; Cheng, Chaoyang; Hirai, Tadayoshi; Ishikawa, Masaki; Iwata, Mineko; Kubo, Minoru; Kurata, Tetsuya; Obara, Mari; Oguri, Yasuko; Onodera, Naoko; Sato, Yoshikatsu; Shinohara, Naoki; Sugimoto, Nagisa; Wakazuki, Sachiko] Japan Sci & Technol Agcy, ERATO, Okazaki, Aichi 4448585, Japan. [Hasebe, Mitsuyasu; Aono, Naoki; Aoyama, Tsuyoshi; Hiwatashi, Yuji; Miyazaki, Saori; Morinaga, Shin-ichi; Murata, Takashi; Sumikawa, Naomi] Natl Inst Nat Sci, Natl Inst Basic Biol, Okazaki, Aichi 4448585, Japan. [Hasebe, Mitsuyasu; Aoyama, Tsuyoshi; Hiwatashi, Yuji; Murata, Takashi] Grad Univ Adv Studies, Sch Life Sci, Dept Basic Sci, Okazaki, Aichi 4448585, Japan. [Bowman, John L.; Floyd, Sandra K.] Monash Univ, Sch Biol Sci, Melbourne, Vic 3800, Australia. [Bowman, John L.] Univ Calif Davis, Plant Biol Sect, Davis, CA 95616 USA. [Gribskov, Michael; Li, Kejie; Li, Ying] Purdue Univ, Dept Biol Sci, W Lafayette, IN 47907 USA. [dePamphilis, Claude; Axtell, Michael J.] Penn State Univ, Dept Biol, University Pk, PA 16802 USA. [dePamphilis, Claude; Axtell, Michael J.] Penn State Univ, Huck Inst Life Sci, University Pk, PA 16802 USA. [dePamphilis, Claude] Penn State Univ, Grad Program Plant Biol, University Pk, PA 16802 USA. [dePamphilis, Claude] Penn State Univ, Inst Mol Evolutionary Genet, University Pk, PA 16802 USA. [Albert, Victor A.] SUNY Buffalo, Dept Biol Sci, Buffalo, NY 14260 USA. [Ambrose, Barbara A.; Karol, Kenneth G.; Litt, Amy] New York Bot Garden, Bronx, NY 10458 USA. [Ashton, Neil W.; Barker, Elizabeth] Univ Regina, Dept Biol, Regina, SK S4S 0A2, Canada. [Barker, Michael S.] Univ Arizona, Dept Ecol & Evolutionary Biol, Tucson, AZ 85721 USA. [Bennetzen, Jeffrey L.; DeBarry, Jeremy; Yang, Lixing; Zhu, Qihui] Univ Georgia, Dept Genet, Athens, GA 30602 USA. [Bonawitz, Nicholas D.; Chapple, Clint; Weng, Jing-Ke] Purdue Univ, Dept Biochem, W Lafayette, IN 47907 USA. [Correa, Luiz Gustavo Guedes; Koehler, Barbara] Univ Potsdam, Dept Mol Biol, D-14476 Potsdam, Germany. [Dacre, Michael; Manning, Gerard] Salk Inst Biol Studies, Razavi Newman Ctr Bioinformat, La Jolla, CA 92037 USA. [Dreyer, Ingo] Univ Potsdam, Heisenberg Grp Biophys & Mol Plant Biol, D-14476 Potsdam, Germany. [Elias, Marek] Charles Univ Prague, Dept Bot, Fac Sci, Prague 12801 2, Czech Republic. [Elias, Marek] Univ Prague, Fac Sci, Ostrava 71000, Czech Republic. [Engstrom, Eric M.] Coll William & Mary, Dept Biol, Williamsburg, VA 23187 USA. [Estelle, Mark; Prigge, Michael] Univ Calif San Diego, Sect Cell & Dev Biol, La Jolla, CA 92093 USA. [Feng, Liang] Univ Georgia, Inst Bioinformat, Athens, GA 30602 USA. [Finet, Cedric] Ecole Normale Super Lyon, Lab Reprod & Dev Plantes, F-69364 Lyon, France. [Frommer, Wolf B.; Lalonde, Sylvie] Carnegie Inst Sci, Dept Plant Biol, Stanford, CA 94305 USA. [Fujita, Tomomichi] Hokkaido Univ, Fac Sci, Sapporo, Hokkaido 0600810, Japan. [Gramzow, Lydia; Theissen, Guenter] Univ Jena, Dept Genet, D-07743 Jena, Germany. [Gutensohn, Michael; Schulz, Burkhard] Purdue Univ, Dept Hort & Landscape Architecture, W Lafayette, IN 47907 USA. [Gutensohn, Michael] Univ Halle Wittenberg, Inst Biol, D-06120 Halle, Germany. [Harholt, Jesper; Petersen, Bent Larsen; Sorensen, Iben; Ulvskov, Peter; Willats, William W. G. T.] Univ Copenhagen, Dept Plant Biol & Biotechnol, DK-1871 Frederiksberg C, Denmark. [Hattori, Mitsuru; Sugita, Mamoru] Nagoya Univ, Ctr Gene Res, Nagoya, Aichi 4648602, Japan. [Hattori, Mitsuru] Univ Tokyo, Sch Sci, Dept Chem, Bunkyo Ku, Tokyo 1130033, Japan. [Heyl, Alexander] Free Univ Berlin, Dahlem Ctr Plant Sci, Inst Biol Appl Genet, D-14195 Berlin, Germany. [Hirai, Tadayoshi] Univ Tsukuba, Ctr Gene Res, Grad Sch Life & Environm Sci, Tsukuba, Ibaraki 3058572, Japan. [Kolukisaoglu, Uener] Univ Rostock, Ctr Life Sci Automat, D-18119 Rostock, Germany. [Kolukisaoglu, Uener] Univ Tubingen, Studiengangskoordinat Nanosci, D-72076 Tubingen, Germany. [Kurata, Tetsuya] Nara Inst Sci & Technol, Grad Sch Biol Sci, Plant Global Educ Project, Nara 6300192, Japan. [Li, Ying] Mayo Clin, Div Biomed Stat & Informat, Rochester, MN 55905 USA. [Lyons, Eric; Scheller, Henrik Vibe] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Maruyama, Takeshi] Hokkaido Univ, Grad Sch Life Sci, Sapporo, Hokkaido 0600810, Japan. [Michael, Todd P.] Rutgers State Univ, Dept Plant Biol & Pathol, Piscataway, NJ 08854 USA. [Michael, Todd P.] Waksman Inst Microbiol, Piscataway, NJ 08854 USA. [Michael, Todd P.] Monsanto Co, Genome Anal Ctr, St Louis, MO 63167 USA. [Mikami, Koji] Hokkaido Univ, Fac Fisheries Sci, Hakodate, Hokkaido 0418611, Japan. [Miyazaki, Saori] Natl Inst Genet, Mishima, Shizuoka 4118540, Japan. [Morinaga, Shin-ichi] Univ Tokyo, Grad Sch Arts & Sci, Tokyo 1538902, Japan. [Mueller-Roeber, Bernd] Bernd Max Planck Inst Mol Plant Physiol, D-14476 Potsdam, Germany. [Nelson, David R.] Univ Tennessee, Dept Microbiol Immunol & Biochem, Memphis, TN 38163 USA. [Obara, Mari] Japan Sci & Technol Agcy, Sapporo, Hokkaido 0600819, Japan. [Olmstead, Richard G.] Univ Washington, Dept Biol, Seattle, WA 98195 USA. [Onodera, Naoko] Dalhousie Univ, Dept Biochem & Mol Biol, Halifax, NS B3H 4R2, Canada. [Pils, Birgit] Wellcome Trust Ctr Human Genet, Oxford OX3 7BN, England. [Pils, Birgit] Sias AG, CH-8634 Hombrechtikon, Switzerland. [Rensing, Stefan A.; Zimmer, Andreas D.] Univ Freiburg, Fac Biol, D-79104 Freiburg, Germany. [Rensing, Stefan A.] Univ Freiburg, BIOSS Ctr Biol Signaling Studies, D-79104 Freiburg, Germany. [Rensing, Stefan A.] Univ Freiburg, Freiburg Initiat Syst Biol FRISYS, D-79104 Freiburg, Germany. [Mauricio Riano-Pachon, Diego] Max Planck Inst Mol Plant Physiol, Bioinformat Grp, GabiPD Team, D-14476 Potsdam, Germany. [Mauricio Riano-Pachon, Diego] Univ Los Andes, Dept Ciencias Biol, Bogota, Colombia. [Roberts, Alison W.] Univ Rhode Isl, Dept Biol Sci, Kingston, RI 02881 USA. [Scheller, Henrik Vibe; Loque, Dominique] Joint BioEnergy Inst, Feedstocks Div, Emeryville, CA 94608 USA. [Schulz, Christian] Ruhr Univ Bochum, Dept Evolut & Biodivers Plants, D-44780 Bochum, Germany. [Shakirov, Eugene V.; Shippen, Dorothy E.] Texas A&M Univ, Dept Biochem & Biophys, College Stn, TX 77843 USA. [Shibagaki, Nakako] Osaka Univ, Grad Sch Engn, Suita, Osaka 5650871, Japan. [Shinohara, Naoki; Sotooka, Ryo] Hokkaido Univ, Sch Sci, Sapporo, Hokkaido 0600810, Japan. [Sorensen, Iben] Cornell Univ, Dept Plant Biol, Ithaca, NY 14850 USA. [Tanurdzic, Milos] Cold Spring Harbor Lab, Cold Spring Harbor, NY 11724 USA. [Weng, Jing-Ke] Salk Inst Biol Studies, Jack H Skirball Ctr Chem Biol & Prote, La Jolla, CA 92037 USA. [Wipf, Daniel] Univ Bourgogne, INRA, UMR 1088, CNRS 5184, F-21065 Dijon, France. [Wolf, Paul G.] Utah State Univ, Dept Biol, Logan, UT 84322 USA. [Mitros, Therese; Rokhsar, Daniel] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Hellsten, Uffe; Otillar, Robert; Salamov, Asaf; Schmutz, Jeremy; Shapiro, Harris; Lindquist, Erika; Lucas, Susan; Rokhsar, Daniel; Grigoriev, Igor V.] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. RP Banks, JA (reprint author), Purdue Univ, Dept Bot & Plant Pathol, W Lafayette, IN 47907 USA. EM banksj@purdue.edu RI dePamphilis, Claude/P-6652-2016; Schmutz, Jeremy/N-3173-2013; Elias, Marek/D-6851-2014; Petersen, Bent/H-9437-2014; Ulvskov, Peter/I-1228-2014; Feng, Liang/I-5010-2014; Kolukisaoglu, Uener/J-8831-2014; Harholt, Jesper/F-6865-2014; Weng, Jing-Ke/A-6900-2015; Sato, Yoshikatsu/I-6129-2014; Loque, Dominique/A-8153-2008; Wolf, Paul/F-7664-2010; Dreyer, Ingo/N-4747-2014; Riano-Pachon, Diego/A-1755-2010; Dacre, Michael/C-1131-2008; Harholt, Jesper/F-3760-2011; Shakirov, Eugene/A-1363-2012; Tanurdzic, Milos/A-5712-2012; Mikami, Koji/A-9825-2012; Weng, Jing-Ke/E-7343-2013; Zhu, Qihui/N-2625-2013; Frommer, Wolf B/A-8256-2008; Ye, Mingli/G-4909-2012; Yang, Lixing/A-7073-2013; Li, Kejie/D-3595-2013 OI Nelson, David/0000-0003-0583-5421; Willats, William/0000-0003-2064-4025; Prigge, Michael/0000-0003-0671-2538; Scheller, Henrik/0000-0002-6702-3560; Nishiyama, Tomoaki/0000-0003-1279-7806; Bowman, John/0000-0001-7347-3691; Barker, Michael/0000-0001-7173-1319; Michael, Todd/0000-0001-6272-2875; DeBarry, Jeremy/0000-0001-5718-2675; Tanurdzic, Milos/0000-0002-7564-0868; Manning, Gerard/0000-0002-5087-9151; Gribskov, Michael/0000-0002-1718-0242; HIWATASHI, YUJI/0000-0002-3996-0549; Schmutz, Jeremy/0000-0001-8062-9172; Elias, Marek/0000-0003-0066-6542; Petersen, Bent/0000-0002-2004-9077; Ulvskov, Peter/0000-0003-3776-818X; Kolukisaoglu, Uener/0000-0002-8656-5963; Harholt, Jesper/0000-0002-7984-0066; Weng, Jing-Ke/0000-0003-3059-0075; Wolf, Paul/0000-0002-4317-6976; Riano-Pachon, Diego/0000-0001-9803-3465; Dacre, Michael/0000-0002-5561-1656; Shakirov, Eugene/0000-0003-2689-7410; Weng, Jing-Ke/0000-0003-1079-3668; FU Office of Science of the U.S. DOE [DE-AC02-05CH11231]; NSF [0844413, 0515435, 0519970, 0638595, 0922742, 1020443, 0607123, 0744800, 1020660, 1036466, 0735191, 0228660, 0421604]; Japan Society for the Promotion of Science; Ministry of Education, Culture, Sports, Science, and Technology, Japan; Australian Research Council [FF0561326]; Lewis B and Dorothy Cullman Program; Natural Sciences and Engineering Research Council of Canada (NSERC) [2982]; NIH [GM84051, T32 GM007757, T32-HG00035, GM065383]; Life Sciences Research Foundation; National Human Genome Research Institute (NHGRI) [HG004164]; German Science Foundation (Deutsche Forschungsgemeinschaft, DFG) [DR 430/4-2]; Czech Ministry of Education [21620828]; Jeffress Memorial Trust [J-938]; DOE [DE-FG02-04ER15542]; Danish Council for Independent Research, Technology and Production Sciences [009-066624/274-09-0314]; Villum Kann Rasmussen Foundation; U.S. Department of Agriculture (USDA) [DE-FG02-08ER64630]; Danish Council for Strategic Research [09-063090]; Marie Curie FP6 RTN ZOONET; DFG [RE 837/10-2, BMBF FRISYS 0313921]; Bundesministerium fuer Bildung und Forschung, Germany [0315046]; USDA NRI [2007-35318-18389]; Burgundy Regional Council [20100112095254682-1] FX Selaginella sequences were deposited at GenBank with the accession numbers GL377566 to GL378322.1 and HM173080. Genome sequencing and analysis were performed by the U.S. Department of Energy (DOE), Joint Genome Institute, supported by the Office of Science of the U.S. DOE, Contract DE-AC02-05CH11231 (I.V.G., U.H., D.L., E.L., S.L., T.M., R.O., D.R., A.S., J.S., H.V.S.). Support was provided by NSF 0844413 (J.A.B.); Japan Society for the Promotion of Science (M.H., T.N., T.F., K.M., T.M., M.S.); Ministry of Education, Culture, Sports, Science, and Technology, Japan (M.H., T.N., T.F.); NSF 0515435 and Australian Research Council FF0561326 (J.L.B.); NSF 0519970 (M.G.); NSF 0638595 (C.D.); NSF 0922742 (V.A.A.); The Lewis B and Dorothy Cullman Program (B.A.A., A.L.); NSF 1020443 (B.A.A.); Natural Sciences and Engineering Research Council of Canada (NSERC) 2982 (N.W.A.); NIH GM84051 (M.J.A.); NSERC (E.I.B.); NIH T32 GM007757 and NSERC PGS-D (M.S.B.); NSF 0607123 (J.L.B.); Life Sciences Research Foundation (NDB); National Human Genome Research Institute (NHGRI) HG004164 (M.D.); German Science Foundation (Deutsche Forschungsgemeinschaft, DFG) DR 430/4-2 (I.D.); Czech Ministry of Education 21620828 (M.E.); Jeffress Memorial Trust J-938 (E.M.E.); NSF 0744800 (M.E. and M.P.); DOE DE-FG02-04ER15542 (W.B.F. and S.L.); The Danish Council for Independent Research, Technology and Production Sciences 009-066624/274-09-0314 (J.H.); The Villum Kann Rasmussen Foundation (J.H., I.S., B.P., P.U., W.W.); NIH T32-HG00035, NSF 1020660, and NSF 1036466 (K.G.K.); NSF 0735191 (E.L.); NHGRI HG004164 (G.M); U.S. Department of Agriculture (USDA) DE-FG02-08ER64630 (T.P.M.); NSF 0228660 (R.G.O.); The Danish Council for Strategic Research 09-063090 (B.L.P. and P.U.); Marie Curie FP6 RTN ZOONET (B.P.); DFG RE 837/10-2, BMBF FRISYS 0313921 (S.A.R.); Bundesministerium fuer Bildung und Forschung, Germany, GABI-FUTURE grant 0315046 (D.M.R.); USDA NRI 2007-35318-18389 (A.W.R.); NSF 0421604 (C.S.); NIH GM065383 (D.E.S.); Burgundy Regional Council 20100112095254682-1 (D.W.); and DFG RE 837/10-2 (A.D.Z.). K. Wall, D. Hurley, and S. Hentel provided computational assistance. NR 25 TC 297 Z9 348 U1 18 U2 161 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 J9 SCIENCE JI Science PD MAY 20 PY 2011 VL 332 IS 6032 BP 960 EP 963 DI 10.1126/science.1203810 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 766FO UT WOS:000290766600042 PM 21551031 ER PT J AU Dunkle, JA Wang, LY Feldman, MB Pulk, A Chen, VB Kapral, GJ Noeske, J Richardson, JS Blanchard, SC Cate, JHD AF Dunkle, Jack A. Wang, Leyi Feldman, Michael B. Pulk, Arto Chen, Vincent B. Kapral, Gary J. Noeske, Jonas Richardson, Jane S. Blanchard, Scott C. Cate, Jamie H. Doudna TI Structures of the Bacterial Ribosome in Classical and Hybrid States of tRNA Binding SO SCIENCE LA English DT Article ID AMINOACYL-TRANSFER-RNA; CRYSTAL-STRUCTURE; RECYCLING FACTOR; 70S RIBOSOME; CRYO-EM; INTERMEDIATE STATES; TRANSLATION FACTORS; MESSENGER-RNA; TRANSLOCATION; DYNAMICS AB During protein synthesis, the ribosome controls the movement of tRNA and mRNA by means of large-scale structural rearrangements. We describe structures of the intact bacterial ribosome from Escherichia coli that reveal how the ribosome binds tRNA in two functionally distinct states, determined to a resolution of similar to 3.2 angstroms by means of x-ray crystallography. One state positions tRNA in the peptidyl-tRNA binding site. The second, a fully rotated state, is stabilized by ribosome recycling factor and binds tRNA in a highly bent conformation in a hybrid peptidyl/exit site. The structures help to explain how the ratchet-like motion of the two ribosomal subunits contributes to the mechanisms of translocation, termination, and ribosome recycling. C1 [Dunkle, Jack A.; Pulk, Arto; Noeske, Jonas; Cate, Jamie H. Doudna] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Dunkle, Jack A.; Pulk, Arto; Noeske, Jonas; Cate, Jamie H. Doudna] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Wang, Leyi; Feldman, Michael B.; Blanchard, Scott C.] Cornell Univ, Weill Cornell Med Coll, Dept Physiol & Biophys, New York, NY 10065 USA. [Feldman, Michael B.] Weill Cornell Rockefeller Univ Sloan Kettering Tr, New York, NY 10065 USA. [Chen, Vincent B.; Kapral, Gary J.; Richardson, Jane S.] Duke Univ, Med Ctr, Dept Biochem, Durham, NC 27710 USA. [Cate, Jamie H. Doudna] Univ Calif Berkeley, Lawrence Berkeley Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Cate, JHD (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. EM jcate@lbl.gov RI Blanchard, Scott/A-5804-2009; OI Pulk, Arto/0000-0001-8793-3038 FU National Institutes of Health [GM65050, GM079238, GM074127-04S1, GM088674, P01-GM63210, GM07739]; National Cancer Institute [CA92584]; National Center for Research Resources [RR-15301]; U.S. Department of Energy [DE-AC03 76SF00098, DE-AC02-06CH11357]; Human Frontiers in Science Program FX We thank K. Hamadani for purified RRF; K. Nierhaus for tRNAPhe overexpression plasmids; K. Frankel, S. Classen, and G. Meigs for help with data measurement at the SIBYLS and 8.3.1 beamlines at the Advanced Light Source (ALS); R. Kanagalaghatta, D. Neau, F. Murphy, and I. Kourinov for help with data measurement at ID-24 at the Advanced Photon Source (APS); J. Headd for help with Phenix refinement; and J. Holton for useful crystallographic discussions. We also thank J. Doudna and H. Noller for helpful comments on the manuscript. Atomic coordinates and structure factors are deposited in the Protein Data Bank (accession codes 3R8N and 3R8S for the fully rotated state RF, 3R8O and 3R8T for the unrotated state R0). This work was funded by the National Institutes of Health (GM65050 to J.H.D.C., GM079238 to S.C.B, and GM074127-04S1, GM088674, and P01-GM63210 project IV to J. S. R.), National Cancer Institute grant CA92584 for the SIBYLS and 8.3.1 beam lines at the ALS, and National Center for Research Resources grant RR-15301 for the Northeastern Collaborative Access Team beam lines at 24-ID at APS, and by the U.S. Department of Energy (DE-AC03 76SF00098 for the SIBYLS and 8.3.1 beamlines at the ALS, and DE-AC02-06CH11357 for the APS). M.B.F. is a trainee in the Weill Cornell/Rockefeller University/SloanKettering Tri-Institutional MD-PhD Program supported by NIH Medical Scientist Training Program grant GM07739. J.N. is supported by a Human Frontiers in Science Program Postdoctoral Fellowship. NR 47 TC 177 Z9 179 U1 2 U2 19 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 J9 SCIENCE JI Science PD MAY 20 PY 2011 VL 332 IS 6032 BP 981 EP 984 DI 10.1126/science.1202692 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 766FO UT WOS:000290766600048 PM 21596992 ER PT J AU Barman, TS Macintosh, B Konopacky, QM Marois, C AF Barman, Travis S. Macintosh, Bruce Konopacky, Quinn M. Marois, Christian TI CLOUDS AND CHEMISTRY IN THE ATMOSPHERE OF EXTRASOLAR PLANET HR8799b SO ASTROPHYSICAL JOURNAL LA English DT Article DE brown dwarfs; planetary systems; stars: atmospheres; stars: low-mass ID INTEGRAL FIELD SPECTROGRAPH; BROWN DWARF ATMOSPHERES; STAR ADAPTIVE OPTICS; ORBITING HR 8799; BINARY T DWARF; MODEL ATMOSPHERES; ULTRACOOL DWARFS; CARBON-MONOXIDE; MU-M; INFRARED-SPECTROSCOPY AB Using the integral field spectrograph OSIRIS, on the Keck II telescope, broad near-infrared H- and K-band spectra of the young exoplanet HR8799b have been obtained. In addition, six new narrowband photometric measurements have been taken across the H and K bands. These data are combined with previously published photometry for an analysis of the planet's atmospheric properties. Thick photospheric dust cloud opacity is invoked to explain the planet's red near-IR colors and relatively smooth near-IR spectrum. Strong water absorption is detected, indicating a hydrogen-rich atmosphere. Only weak CH4 absorption is detected at K band, indicating efficient vertical mixing and a disequilibrium CO/CH4 ratio at photospheric depths. The H-band spectrum has a distinct triangular shape consistent with low surface gravity. New giant planet atmosphere models are compared to these data with best-fitting bulk parameters, T-eff = 1100 K +/- 100 and log(g) = 3.5 +/- 0.5 (for solar composition). Given the observed luminosity (log L-obs/L-circle dot similar to -5.1), these values correspond to a radius of 0.75 R-Jup-0.12(+0.17) and a mass of similar to 0.72 M-Jup-0.6(+2.6)-strikingly inconsistent with interior/evolution models. Enhanced metallicity (up to similar to 10x that of the Sun) along with thick clouds and non-equilibrium chemistry are likely required to reproduce the complete ensemble of spectroscopic and photometric data and the low effective temperatures (< 1000 K) required by the evolution models. C1 [Barman, Travis S.] Lowell Observ, Flagstaff, AZ 86001 USA. [Macintosh, Bruce; Konopacky, Quinn M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Marois, Christian] Natl Res Council Canada, Herzberg Inst Astrophys, Victoria, BC V9E 2E7, Canada. RP Barman, TS (reprint author), Lowell Observ, 1400 W Mars Hill Rd, Flagstaff, AZ 86001 USA. EM barman@lowell.edu FU W.M. Keck Foundation; NSF; National Science Foundation (United States); Science and Technology Facilities Council (United Kingdom); National Research Council (Canada); CONICYT (Chile); Australian Research Council (Australia); Ministerio da Ciencia e Tecnologia (Brazil); Ministerio de Ciencia; Tecnologia e Innovacion Productiva (Argentina); NASA; U.S. Department of Energy, Lawrence Livermore National Laboratory [DE-AC52-07NA27344 (LLNL-JRNL-476433)] FX We thank the referee, Jonathan Fortney, for his careful review of our paper. Additional thanks go out to Shelley Wright, Jim Lyke, and James Larkin for their assistance with all things OSIRIS-related. We also thank Brad Hansen, Mark Marley, Didier Saumon, and Tristan Guillot for many useful discussions on the vagaries of planets and brown dwarfs. We are indebted to Jim Lyke, Al Conrad, Hien Tran, Scott Dahm, Randy Campbell, Terry Stickel, and the entire Keck staff for their assistance in maximizing our observing efficiency. T.B. acknowledges the Kavli Institute for Theoretical Physics and the participants of the 2010 workshop on Exoplanets for providing a stimulating environment. This research has benefited from the SpeX Prism Spectral Libraries, maintained by Adam Burgasser. The data presented herein were obtained at the W.M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California and the National Aeronautics and Space Administration. The Observatory was made possible by the generous financial support of the W.M. Keck Foundation. The authors wish to recognize and acknowledge the very significant cultural role and reverence that the summit of Mauna Kea has always had within the indigenous Hawaiian community. We are most fortunate to have the opportunity to conduct observations from this mountain. Observations were also obtained at the Gemini Observatory, which is operated by the Association of Universities for Research in Astronomy, Inc., under a cooperative agreement with the NSF on behalf of the Gemini partnership: the National Science Foundation (United States), the Science and Technology Facilities Council (United Kingdom), the National Research Council (Canada), CONICYT (Chile), the Australian Research Council (Australia), Ministerio da Ciencia e Tecnologia (Brazil) and Ministerio de Ciencia, Tecnologia e Innovacion Productiva (Argentina). Most of the numerical work was carried out at the NASA Advanced Supercomputing facilities. This research was supported by NASA Origins of Solar Systems grants to LLNL and Lowell Observatory. This research was also supported by JPL/NexSci RSA awards. Portions of this work were performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 (LLNL-JRNL-476433). We thank all these institutions for their support. NR 91 TC 141 Z9 141 U1 0 U2 9 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X J9 ASTROPHYS J JI Astrophys. J. PD MAY 20 PY 2011 VL 733 IS 1 AR 65 DI 10.1088/0004-637X/733/1/65 PG 18 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 760HE UT WOS:000290314600065 ER PT J AU Childress, M Aldering, G Aragon, C Antilogus, P Bailey, S Baltay, C Bongard, S Buton, C Canto, A Chotard, N Copin, Y Fakhouri, HK Gangler, E Kerschhaggl, M Kowalski, M Hsiao, EY Loken, S Nugent, P Paech, K Pain, R Pecontal, E Pereira, R Perlmutter, S Rabinowitz, D Runge, K Scalzo, R Thomas, RC Smadja, G Tao, C Weaver, BA Wu, C AF Childress, M. Aldering, G. Aragon, C. Antilogus, P. Bailey, S. Baltay, C. Bongard, S. Buton, C. Canto, A. Chotard, N. Copin, Y. Fakhouri, H. K. Gangler, E. Kerschhaggl, M. Kowalski, M. Hsiao, E. Y. Loken, S. Nugent, P. Paech, K. Pain, R. Pecontal, E. Pereira, R. Perlmutter, S. Rabinowitz, D. Runge, K. Scalzo, R. Thomas, R. C. Smadja, G. Tao, C. Weaver, B. A. Wu, C. TI KECK OBSERVATIONS OF THE YOUNG METAL-POOR HOST GALAXY OF THE SUPER-CHANDRASEKHAR-MASS TYPE Ia SUPERNOVA SN 2007if SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: dwarf; supernovae: general; supernovae: individual (SN 2007if) ID DIGITAL SKY SURVEY; STELLAR POPULATION SYNTHESIS; COMPACT DWARF GALAXIES; STAR-FORMING GALAXIES; TO-LIGHT RATIOS; METALLICITY RELATION; FACTORY OBSERVATIONS; LUMINOSITY FUNCTION; FORMATION RATES; DATA RELEASE AB We present Keck LRIS spectroscopy and g-band photometry of the metal-poor, low-luminosity host galaxy of the super-Chandrasekhar-mass Type Ia supernova SN 2007if. Deep imaging of the host reveals its apparent magnitude to be m(g) = 23.15 +/- 0.06, which at the spectroscopically measured redshift of z(helio) = 0.07450 +/- 0.00015 corresponds to an absolute magnitude of M-g = -14.45 +/- 0.06. Galaxy g - r color constrains the mass-to-light ratio, giving a host stellar mass estimate of log(M-*/M-circle dot) = 7.32 +/- 0.17. Balmer absorption in the stellar continuum, along with the strength of the 4000 angstrom break, constrains the age of the dominant starburst in the galaxy to be t(burst) = 123(-77)(+165) Myr, corresponding to a main-sequence turnoff mass of M/M-circle dot = 4.6(-1.4)(+2.6). Using the R-23 method of calculating metallicity from the fluxes of strong emission lines, we determine the host oxygen abundance to be 12 + log(O/H)(KK04) = 8.01 +/- 0.09, significantly lower than any previously reported spectroscopically measured Type Ia supernova host galaxy metallicity. Our data show that SN 2007if is very likely to have originated from a young, metal-poor progenitor. C1 [Childress, M.; Aldering, G.; Aragon, C.; Bailey, S.; Fakhouri, H. K.; Hsiao, E. Y.; Loken, S.; Perlmutter, S.; Runge, K.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Phys, Berkeley, CA 94720 USA. [Childress, M.; Fakhouri, H. K.; Perlmutter, S.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Antilogus, P.; Bongard, S.; Canto, A.; Pain, R.; Wu, C.] Univ Paris 07, Univ Paris 06, Lab Phys Nucl & Hautes Energies, CNRS IN2P3, F-75252 Paris 05, France. [Baltay, C.; Rabinowitz, D.; Scalzo, R.] Yale Univ, Dept Phys, New Haven, CT 06250 USA. [Buton, C.; Kerschhaggl, M.; Kowalski, M.; Paech, K.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Chotard, N.; Copin, Y.; Gangler, E.; Pereira, R.; Smadja, G.] Univ Lyon, F-69622 Villeurbanne, France. [Chotard, N.; Copin, Y.; Gangler, E.; Pereira, R.; Smadja, G.] Univ Lyon 1, F-69622 Villeurbanne, France. [Chotard, N.; Copin, Y.; Gangler, E.; Pereira, R.; Smadja, G.] CNRS, IN2P3, Inst Phys Nucl Lyon, F-75700 Paris, France. [Nugent, P.; Thomas, R. C.] Lawrence Berkeley Natl Lab, Computat Res Div, Computat Cosmol Ctr, Berkeley, CA 94611 USA. [Pecontal, E.] Univ Lyon 1, Ctr Rech Astron Lyon, F-69561 St Genis Laval, France. [Scalzo, R.] Australian Natl Univ, Mt Stromlo Observ, Res Sch Astron & Astrophys, Weston, ACT 2611, Australia. [Tao, C.] Ctr Phys Particules Marseille, F-13288 Marseille 09, France. [Tao, C.] Tsinghua Univ, Tsinghua Ctr Astrophys, Beijing 100084, Peoples R China. [Weaver, B. A.] NYU, Ctr Cosmol & Particle Phys, New York, NY 10003 USA. RP Childress, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Phys, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM mjchildress@lbl.gov RI Kowalski, Marek/G-5546-2012; Copin, Yannick/B-4928-2015; Perlmutter, Saul/I-3505-2015; OI Copin, Yannick/0000-0002-5317-7518; Perlmutter, Saul/0000-0002-4436-4661; Scalzo, Richard/0000-0003-3740-1214 FU Office of Science, Office of High Energy Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; Gordon & Betty Moore Foundation; CNRS/IN2P3; CNRS/INSU; PNC; National Natural Science Foundation of China [10903010]; National Science Foundation [ANI-0087344]; University of California, San Diego FX This work was supported by the Director, Office of Science, Office of High Energy Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, by a grant from the Gordon & Betty Moore Foundation, and in France by support from CNRS/IN2P3, CNRS/INSU, and PNC. C. W. acknowledges support from the National Natural Science Foundation of China grant 10903010. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Director, Office of Science, Office of Advanced Scientific Computing Research, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We thank them for a generous allocation of storage and computing time. HPWREN is funded by National Science Foundation Grant Number ANI-0087344, and the University of California, San Diego. NR 106 TC 13 Z9 13 U1 0 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X J9 ASTROPHYS J JI Astrophys. J. PD MAY 20 PY 2011 VL 733 IS 1 AR 3 DI 10.1088/0004-637X/733/1/3 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 760HE UT WOS:000290314600003 ER PT J AU Pai, AP Lara, P Pan, C Hillegonds, D AF Pai, A. P. Lara, P. Pan, C. Hillegonds, D. TI Direct measurement of calcium metabolism in patients with castration-resistant prostate cancer using a novel isotope tracing approach in urine. SO JOURNAL OF CLINICAL ONCOLOGY LA English DT Meeting Abstract C1 Univ Calif Davis, Med Ctr, Sacramento, CA 95817 USA. Univ Calif Davis, Sacramento, CA 95817 USA. Lawrence Livermore Natl Lab, Livermore, CA USA. NR 0 TC 0 Z9 0 U1 0 U2 1 PU AMER SOC CLINICAL ONCOLOGY PI ALEXANDRIA PA 2318 MILL ROAD, STE 800, ALEXANDRIA, VA 22314 USA SN 0732-183X EI 1527-7755 J9 J CLIN ONCOL JI J. Clin. Oncol. PD MAY 20 PY 2011 VL 29 IS 15 SU S MA e15083 PG 1 WC Oncology SC Oncology GA V31JQ UT WOS:000208880303786 PM 28020431 ER PT J AU Pan, C Wang, S White, RD Gandara, DR Lara, P Li, T Mack, P Rodriguez-Fahrni, A Lee, JS Malfatti, M Turteltaub, K Henderson, PT AF Pan, C. Wang, S. White, R. deVere Gandara, D. R. Lara, P. Li, T. Mack, P. Rodriguez-Fahrni, A. Lee, J. S. Malfatti, M. Turteltaub, K. Henderson, P. T. TI A phase 0 microdosing trial of an in vivo assay for predicting chemoresistance to platinum. SO JOURNAL OF CLINICAL ONCOLOGY LA English DT Meeting Abstract C1 Univ Calif Davis, Sacramento, CA 95817 USA. Lawrence Livermore Natl Lab, Livermore, CA USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU AMER SOC CLINICAL ONCOLOGY PI ALEXANDRIA PA 2318 MILL ROAD, STE 800, ALEXANDRIA, VA 22314 USA SN 0732-183X EI 1527-7755 J9 J CLIN ONCOL JI J. Clin. Oncol. PD MAY 20 PY 2011 VL 29 IS 15 SU S MA 2578 PG 1 WC Oncology SC Oncology GA V31JQ UT WOS:000208880301393 PM 28022281 ER PT J AU Leitner, T AF Leitner, Thomas TI Guidelines for HIV in court cases SO NATURE LA English DT Letter C1 Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Leitner, T (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM tkl@lanl.gov RI Brown, Jeremy/B-4544-2010 OI Brown, Jeremy/0000-0002-1447-8633 FU NIAID NIH HHS [R01 AI087520] NR 0 TC 3 Z9 3 U1 0 U2 2 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 J9 NATURE JI Nature PD MAY 19 PY 2011 VL 473 IS 7347 BP 284 EP 284 DI 10.1038/473284a PG 1 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 765QA UT WOS:000290722400019 PM 21593845 ER PT J AU Agakishiev, H Aggarwal, MM Ahammed, Z Alakhverdyants, AV Alekseev, I Alford, J Anderson, BD Anson, CD Arkhipkin, D Averichev, GS Balewski, J Beavis, DR Behera, NK Bellwied, R Betancourt, MJ Betts, RR Bhasin, A Bhati, AK Bichsel, H Bielcik, J Bielcikova, J Biritz, B Bland, LC Bordyuzhin, IG Borowski, W Bouchet, J Braidot, E Brandin, AV Bridgeman, A Brovko, SG Bruna, E Bueltmann, S Bunzarov, I Burton, TP Cai, XZ Caines, H Calderon, M Cebra, D Cendejas, R Cervantes, MC Chajecki, Z Chaloupka, P Chattopadhyay, S Chen, HF Chen, JH Chen, JY Chen, L Cheng, J Cherney, M Chikanian, A Choi, KE Christie, W Chung, P Codrington, MJM Corliss, R Cramer, JG Crawford, HJ Leyva, AD De Silva, LC Debbe, RR Dedovich, TG Derevschikov, AA de Souza, RD Didenko, L Djawotho, P Dogra, SM Dong, X Drachenberg, JL Draper, JE Dunlop, C Efimov, LG Elnimr, M Engelage, J Eppley, G Estienne, M Eun, L Evdokimov, O Fatemi, R Fedorisin, J Fersch, RG Filip, P Finch, E Fine, V Fisyak, Y Gagliardi, CA Gangadharan, DR Geurts, F Ghosh, P Gorbunov, YN Gordon, A Grebenyuk, OG Grosnick, D Guertin, SM Gupta, A Gupta, S Guryn, W Haag, B Hajkova, O Hamed, A Han, LX Harris, JW Hays-Wehle, JP Heinz, M Heppelmann, S Hirsch, A Hjort, E Hoffmann, GW Hofman, DJ Huang, B Huang, HZ Humanic, TJ Huo, L Igo, G Jacobs, P Jacobs, W Jena, C Jin, F Joseph, J Judd, EG Kabana, S Kang, K Kapitan, J Kauder, K Ke, HW Keane, D Kechechyan, A Kettler, D Kikola, DP Kiryluk, J Kisiel, A Kizka, V Klein, SR Knospe, AG Koetke, DD Kollegger, T Konzer, J Koralt, I Koroleva, L Korsch, W Kotchenda, L Kouchpil, V Kravtsov, P Krueger, K Krus, M Kumar, L Kurnadi, P Lamont, MAC Landgraf, JM LaPointe, S Lauret, J Lebedev, A Lednicky, R Lee, JH Leight, W LeVine, MJ Li, C Li, L Li, N Li, W Li, X Li, X Li, Y Li, ZM Lisa, MA Liu, F Liu, H Liu, J Ljubicic, T Llope, WJ Longacre, RS Love, WA Lu, Y Lukashov, EV Luo, X Ma, GL Ma, YG Mahapatra, DP Majka, R Mall, OI Manweiler, R Margetis, S Markert, C Masui, H Matis, HS Matulenko, YA McDonald, D McShane, TS Meschanin, A Milner, R Minaev, NG Mioduszewski, S Mitrovski, MK Mohammed, Y Mohanty, B Mondal, MM Morozov, B Morozov, DA Munhoz, MG Mustafa, MK Naglis, M Nandi, BK Nayak, TK Netrakanti, PK Nogach, LV Nurushev, SB Odyniec, G Ogawa, A Oh, K Ohlson, A Okorokov, V Oldag, EW Olson, D Pachr, M Page, BS Pal, SK Pandit, Y Panebratsev, Y Pawlak, T Pei, H Peitzmann, T Perkins, C Peryt, W Pile, P Planinic, M Ploskon, MA Pluta, J Plyku, D Poljak, N Porter, J Poskanzer, AM Potukuchi, BVKS Powell, CB Prindle, D Pruneau, C Pruthi, NK Pujahari, PR Putschke, J Qiu, H Raniwala, R Raniwala, S Ray, RL Redwine, R Reed, R Ritter, HG Roberts, JB Rogachevskiy, OV Romero, JL Ruan, L Rusnak, J Sahoo, NR Sakrejda, I Salur, S Sandweiss, J Sangaline, E Sarkar, A Schambach, J Scharenberg, RP Schmah, AM Schmitz, N Schuster, TR Seele, J Seger, J Selyuzhenkov, I Seyboth, P Shah, N Shahaliev, E Shao, M Sharma, M Shi, SS Shou, QY Sichtermann, EP Simon, F Singaraju, RN Skoby, MJ Smirnov, N Solanki, D Sorensen, P Spinka, HM Srivastava, B Stanislaus, TDS Staszak, D Steadman, SG Stevens, JR Stock, R Strikhanov, M Stringfellow, B Suaide, AAP Suarez, MC Subba, NL Sumbera, M Sun, XM Sun, Y Sun, Z Surrow, B Svirida, DN Symons, TJM de Toledo, AS Takahashi, J Tang, AH Tang, Z Tarini, LH Tarnowsky, T Thein, D Thomas, JH Tian, J Timmins, AR Tlusty, D Tokarev, M Trainor, TA Trentalange, S Tribble, RE Tribedy, P Tsai, OD Ullrich, T Underwood, DG Van Buren, G van Nieuwenhuizen, G Vanfossen, JA Varma, R Vasconcelos, GMS Vasiliev, AN Videbaek, F Viyogi, YP Vokal, S Voloshin, SA Wada, M Walker, M Wang, F Wang, G Wang, H Wang, JS Wang, Q Wang, XL Wang, Y Webb, G Webb, JC Westfall, GD Whitten, C Wieman, H Wissink, SW Witt, R Witzke, W Wu, YF Xiao, Z Xie, W Xu, H Xu, N Xu, QH Xu, W Xu, Y Xu, Z Xue, L Yang, Y Yang, Y Yepes, P Yip, K Yoo, IK Zawisza, M Zbroszczyk, H Zhan, W Zhang, JB Zhang, S Zhang, WM Zhang, XP Zhang, Y Zhang, ZP Zhao, F Zhao, J Zhong, C Zhou, W Zhu, X Zhu, YH Zoulkarneev, R Zoulkarneeva, Y AF Agakishiev, H. Aggarwal, M. M. Ahammed, Z. Alakhverdyants, A. V. Alekseev, I. Alford, J. Anderson, B. D. Anson, C. D. Arkhipkin, D. Averichev, G. S. Balewski, J. Beavis, D. R. Behera, N. K. Bellwied, R. Betancourt, M. J. Betts, R. R. Bhasin, A. Bhati, A. K. Bichsel, H. Bielcik, J. Bielcikova, J. Biritz, B. Bland, L. C. Bordyuzhin, I. G. Borowski, W. Bouchet, J. Braidot, E. Brandin, A. V. Bridgeman, A. Brovko, S. G. Bruna, E. Bueltmann, S. Bunzarov, I. Burton, T. P. Cai, X. Z. Caines, H. Calderon, M. Cebra, D. Cendejas, R. Cervantes, M. C. Chajecki, Z. Chaloupka, P. Chattopadhyay, S. Chen, H. F. Chen, J. H. Chen, J. Y. Chen, L. Cheng, J. Cherney, M. Chikanian, A. Choi, K. E. Christie, W. Chung, P. Codrington, M. J. M. Corliss, R. Cramer, J. G. Crawford, H. J. Leyva, A. Davila De Silva, L. C. Debbe, R. R. Dedovich, T. G. Derevschikov, A. A. Derradi de Souza, R. Didenko, L. Djawotho, P. Dogra, S. M. Dong, X. Drachenberg, J. L. Draper, J. E. Dunlop, C. Efimov, L. G. Elnimr, M. Engelage, J. Eppley, G. Estienne, M. Eun, L. Evdokimov, O. Fatemi, R. Fedorisin, J. Fersch, R. G. Filip, P. Finch, E. Fine, V. Fisyak, Y. Gagliardi, C. A. Gangadharan, D. R. Geurts, F. Ghosh, P. Gorbunov, Y. N. Gordon, A. Grebenyuk, O. G. Grosnick, D. Guertin, S. M. Gupta, A. Gupta, S. Guryn, W. Haag, B. Hajkova, O. Hamed, A. Han, L-X. Harris, J. W. Hays-Wehle, J. P. Heinz, M. Heppelmann, S. Hirsch, A. Hjort, E. Hoffmann, G. W. Hofman, D. J. Huang, B. Huang, H. Z. Humanic, T. J. Huo, L. Igo, G. Jacobs, P. Jacobs, W. Jena, C. Jin, F. Joseph, J. Judd, E. G. Kabana, S. Kang, K. Kapitan, J. Kauder, K. Ke, H. W. Keane, D. Kechechyan, A. Kettler, D. Kikola, D. P. Kiryluk, J. Kisiel, A. Kizka, V. Klein, S. R. Knospe, A. G. Koetke, D. D. Kollegger, T. Konzer, J. Koralt, I. Koroleva, L. Korsch, W. Kotchenda, L. Kouchpil, V. Kravtsov, P. Krueger, K. Krus, M. Kumar, L. Kurnadi, P. Lamont, M. A. C. Landgraf, J. M. LaPointe, S. Lauret, J. Lebedev, A. Lednicky, R. Lee, J. H. Leight, W. LeVine, M. J. Li, C. Li, L. Li, N. Li, W. Li, X. Li, X. Li, Y. Li, Z. M. Lisa, M. A. Liu, F. Liu, H. Liu, J. Ljubicic, T. Llope, W. J. Longacre, R. S. Love, W. A. Lu, Y. Lukashov, E. V. Luo, X. Ma, G. L. Ma, Y. G. Mahapatra, D. P. Majka, R. Mall, O. I. Manweiler, R. Margetis, S. Markert, C. Masui, H. Matis, H. S. Matulenko, Yu A. McDonald, D. McShane, T. S. Meschanin, A. Milner, R. Minaev, N. G. Mioduszewski, S. Mitrovski, M. K. Mohammed, Y. Mohanty, B. Mondal, M. M. Morozov, B. Morozov, D. A. Munhoz, M. G. Mustafa, M. K. Naglis, M. Nandi, B. K. Nayak, T. K. Netrakanti, P. K. Nogach, L. V. Nurushev, S. B. Odyniec, G. Ogawa, A. Oh, K. Ohlson, A. Okorokov, V. Oldag, E. W. Olson, D. Pachr, M. Page, B. S. Pal, S. K. Pandit, Y. Panebratsev, Y. Pawlak, T. Pei, H. Peitzmann, T. Perkins, C. Peryt, W. Pile, P. Planinic, M. Ploskon, M. A. Pluta, J. Plyku, D. Poljak, N. Porter, J. Poskanzer, A. M. Potukuchi, B. V. K. S. Powell, C. B. Prindle, D. Pruneau, C. K. Pruthi, N. Pujahari, P. R. Putschke, J. Qiu, H. Raniwala, R. Raniwala, S. Ray, R. L. Redwine, R. Reed, R. Ritter, H. G. Roberts, J. B. Rogachevskiy, O. V. Romero, J. L. Ruan, L. Rusnak, J. Sahoo, N. R. Sakrejda, I. Salur, S. Sandweiss, J. Sangaline, E. Sarkar, A. Schambach, J. Scharenberg, R. P. Schmah, A. M. Schmitz, N. Schuster, T. R. Seele, J. Seger, J. Selyuzhenkov, I. Seyboth, P. Shah, N. Shahaliev, E. Shao, M. Sharma, M. Shi, S. S. Shou, Q. Y. Sichtermann, E. P. Simon, F. Singaraju, R. N. Skoby, M. J. Smirnov, N. Solanki, D. Sorensen, P. Spinka, H. M. Srivastava, B. Stanislaus, T. D. S. Staszak, D. Steadman, S. G. Stevens, J. R. Stock, R. Strikhanov, M. Stringfellow, B. Suaide, A. A. P. Suarez, M. C. Subba, N. L. Sumbera, M. Sun, X. M. Sun, Y. Sun, Z. Surrow, B. Svirida, D. N. Symons, T. J. M. Szanto de Toledo, A. Takahashi, J. Tang, A. H. Tang, Z. Tarini, L. H. Tarnowsky, T. Thein, D. Thomas, J. H. Tian, J. Timmins, A. R. Tlusty, D. Tokarev, M. Trainor, T. A. Trentalange, S. Tribble, R. E. Tribedy, P. Tsai, O. D. Ullrich, T. Underwood, D. G. Van Buren, G. van Nieuwenhuizen, G. Vanfossen, J. A., Jr. Varma, R. Vasconcelos, G. M. S. Vasiliev, A. N. Videbaek, F. Viyogi, Y. P. Vokal, S. Voloshin, S. A. Wada, M. Walker, M. Wang, F. Wang, G. Wang, H. Wang, J. S. Wang, Q. Wang, X. L. Wang, Y. Webb, G. Webb, J. C. Westfall, G. D. Whitten, C., Jr. Wieman, H. Wissink, S. W. Witt, R. Witzke, W. Wu, Y. F. Xiao, Z. Xie, W. Xu, H. Xu, N. Xu, Q. H. Xu, W. Xu, Y. Xu, Z. Xue, L. Yang, Y. Yang, Y. Yepes, P. Yip, K. Yoo, I-K. Zawisza, M. Zbroszczyk, H. Zhan, W. Zhang, J. B. Zhang, S. Zhang, W. M. Zhang, X. P. Zhang, Y. Zhang, Z. P. Zhao, F. Zhao, J. Zhong, C. Zhou, W. Zhu, X. Zhu, Y. H. Zoulkarneev, R. Zoulkarneeva, Y. CA STAR Collaboration TI Observation of the antimatter helium-4 nucleus SO NATURE LA English DT Article ID QUARK-GLUON PLASMA; ANTIPROTONS; COLLISIONS; ELECTRON AB High-energy nuclear collisions create an energy density similar to that of the Universe microseconds after the Big Bang(1); in both cases, matter and antimatter are formed with comparable abundance. However, the relatively short-lived expansion in nuclear collisions allows antimatter to decouple quickly from matter, and avoid annihilation. Thus, a high-energy accelerator of heavy nuclei provides an efficient means of producing and studying antimatter. The antimatter helium-4 nucleus ((4)(He) over bar), also known as the anti-alpha ((alpha) over bar), consists of two antiprotons and two antineutrons (baryon number B = -4). It has not been observed previously, although the alpha-particle was identified a century ago by Rutherford and is present in cosmic radiation at the ten per cent level(2). Antimatter nuclei with B -1 have been observed only as rare products of interactions at particle accelerators, where the rate of antinucleus production in high-energy collisions decreases by a factor of about 1,000 with each additional antinucleon(3-5). Here we report the observation of (4)<(He) over bar, the heaviest observed antinucleus to date. In total, 18 (4)(He) over bar counts were detected at the STAR experiment at the Relativistic Heavy Ion Collider (RHIC; ref. 6) in 10(9) recorded gold-on-gold (Au+Au) collisions at centre-of-mass energies of 200 GeV and 62 GeV per nucleon-nucleon pair. The yield is consistent with expectations from thermodynamic(7) and coalescent nucleosynthesis(8) models, providing an indication of the production rate of even heavier antimatter nuclei and a benchmark for possible future observations of (4)(He) over bar in cosmic radiation. C1 [Agakishiev, H.; Alakhverdyants, A. V.; Averichev, G. S.; Bunzarov, I.; Dedovich, T. G.; Efimov, L. G.; Fedorisin, J.; Filip, P.; Kechechyan, A.; Kizka, V.; Lednicky, R.; Panebratsev, Y.; Rogachevskiy, O. V.; Shahaliev, E.; Tokarev, M.; Vokal, S.; Zoulkarneev, R.; Zoulkarneeva, Y.] Joint Inst Nucl Res, Dubna 141980, Russia. [Aggarwal, M. M.; Bhati, A. K.; K. Pruthi, N.] Panjab Univ, Chandigarh 160014, India. [Ahammed, Z.; Dong, X.; Grebenyuk, O. G.; Hjort, E.; Jacobs, P.; Kiryluk, J.; Klein, S. R.; Masui, H.; Matis, H. S.; Naglis, M.; Odyniec, G.; Olson, D.; Ploskon, M. A.; Porter, J.; Poskanzer, A. M.; Powell, C. B.; Ritter, H. G.; Sakrejda, I.; Schmah, A. M.; Sichtermann, E. P.; Sun, X. M.; Symons, T. J. M.; Thomas, J. H.; Wieman, H.; Zhang, Y.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Alekseev, I.; Bordyuzhin, I. G.; Koroleva, L.; Morozov, B.; Svirida, D. N.] Alikhanov Inst Theoret & Expt Phys, Moscow 117218, Russia. [Alford, J.; Anderson, B. D.; Bouchet, J.; Joseph, J.; Keane, D.; Kumar, L.; Margetis, S.; Pandit, Y.; Subba, N. L.; Vanfossen, J. A., Jr.; Zhang, W. M.] Kent State Univ, Kent, OH 44242 USA. [Anson, C. D.; Chajecki, Z.; Humanic, T. J.; Lisa, M. A.] Ohio State Univ, Columbus, OH 43210 USA. [Arkhipkin, D.; Beavis, D. R.; Bland, L. C.; Burton, T. P.; Christie, W.; Debbe, R. R.; Didenko, L.; Dunlop, C.; Fine, V.; Fisyak, Y.; Gordon, A.; Guryn, W.; Lamont, M. A. C.; Landgraf, J. M.; Lauret, J.; Lebedev, A.; Lee, J. H.; LeVine, M. J.; Ljubicic, T.; Longacre, R. S.; Love, W. A.; Mitrovski, M. K.; Ogawa, A.; Pile, P.; Ruan, L.; Sorensen, P.; Tang, A. H.; Ullrich, T.; Van Buren, G.; Videbaek, F.; Webb, J. C.; Xu, Z.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Balewski, J.; Betancourt, M. J.; Corliss, R.; Hays-Wehle, J. P.; Leight, W.; Milner, R.; Redwine, R.; Seele, J.; Steadman, S. G.; Surrow, B.; van Nieuwenhuizen, G.; Walker, M.] MIT, Cambridge, MA 02139 USA. [Behera, N. K.; Nandi, B. K.; Pujahari, P. R.; Sarkar, A.; Varma, R.] Indian Inst Technol, Bombay 400076, Maharashtra, India. [Bellwied, R.; De Silva, L. C.; Timmins, A. R.] Univ Houston, Houston, TX 77204 USA. [Betts, R. R.; Evdokimov, O.; Hofman, D. J.; Kauder, K.; Pei, H.; Suarez, M. C.] Univ Illinois, Chicago, IL 60607 USA. [Bhasin, A.; Dogra, S. M.; Gupta, A.; Gupta, S.; Potukuchi, B. V. K. S.] Univ Jammu, Jammu 180001, India. [Bichsel, H.; Cramer, J. G.; Kettler, D.; Prindle, D.; Trainor, T. A.] Univ Washington, Seattle, WA 98195 USA. [Bielcik, J.; Hajkova, O.; Krus, M.; Pachr, M.] Czech Tech Univ, FNSPE, Prague 11519, Czech Republic. [Bielcikova, J.; Chaloupka, P.; Chung, P.; Kapitan, J.; Kouchpil, V.; Rusnak, J.; Sumbera, M.; Tlusty, D.] Nucl Phys Inst AS CR, Rez 25068, Czech Republic. [Biritz, B.; Cendejas, R.; Gangadharan, D. R.; Guertin, S. M.; Huang, H. Z.; Igo, G.; Kurnadi, P.; Shah, N.; Staszak, D.; Trentalange, S.; Tsai, O. D.; Wang, G.; Whitten, C., Jr.; Xu, W.; Zhao, F.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Borowski, W.; Estienne, M.; Kabana, S.] SUBATECH, F-44307 Nantes, France. [Braidot, E.; Peitzmann, T.] NIKHEF, NL-1098 XG Amsterdam, Netherlands. [Braidot, E.; Peitzmann, T.] Univ Utrecht, NL-1098 XG Amsterdam, Netherlands. [Brandin, A. V.; Kotchenda, L.; Kravtsov, P.; Lukashov, E. V.; Okorokov, V.; Strikhanov, M.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Bridgeman, A.; Krueger, K.; Spinka, H. M.; Underwood, D. G.] Argonne Natl Lab, Argonne, IL 60439 USA. [Brovko, S. G.; Calderon, M.; Cebra, D.; Draper, J. E.; Haag, B.; Liu, H.; Mall, O. I.; Reed, R.; Romero, J. L.; Salur, S.; Sangaline, E.] Univ Calif Davis, Davis, CA 95616 USA. [Bruna, E.; Caines, H.; Chikanian, A.; Finch, E.; Harris, J. W.; Heinz, M.; Knospe, A. G.; Majka, R.; Ohlson, A.; Putschke, J.; Sandweiss, J.; Smirnov, N.] Yale Univ, New Haven, CT 06520 USA. [Bueltmann, S.; Koralt, I.; Plyku, D.] Old Dominion Univ, Norfolk, VA 23529 USA. [Cai, X. Z.; Chen, J. H.; Han, L-X.; Jin, F.; Li, W.; Ma, G. L.; Ma, Y. G.; Shou, Q. Y.; Tian, J.; Xue, L.; Zhang, S.; Zhao, J.; Zhong, C.; Zhu, Y. H.] Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Bhasin, A.; Cervantes, M. C.; Codrington, M. J. M.; Djawotho, P.; Drachenberg, J. L.; Gagliardi, C. A.; Hamed, A.; Huo, L.; Mioduszewski, S.; Mohammed, Y.; Pal, S. K.; Tribble, R. E.] Texas A&M Univ, College Stn, TX 77843 USA. [Bhasin, A.; Chattopadhyay, S.; Ghosh, P.; Mohanty, B.; Mondal, M. M.; Nayak, T. K.; Sahoo, N. R.; Singaraju, R. N.; Tribedy, P.; Viyogi, Y. P.] Variable Energy Cyclotron Ctr, Kolkata 700064, India. [Chen, H. F.; Huang, B.; Li, C.; Lu, Y.; Luo, X.; Shao, M.; Sun, Y.; Tang, Z.; Wang, X. L.; Xu, Y.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Chen, J. Y.; Chen, L.; Ke, H. W.; Li, N.; Li, Z. M.; Liu, F.; Shi, S. S.; Wu, Y. F.; Xu, N.; Yang, Y.; Zhang, J. B.] CCNU HZNU, Inst Particle Phys, Wuhan 430079, Peoples R China. [Cheng, J.; Kang, K.; Li, Y.; Wang, Y.; Xiao, Z.; Zhang, X. P.; Zhu, X.] Tsinghua Univ, Beijing 100084, Peoples R China. [Cherney, M.; Gorbunov, Y. N.; McShane, T. S.; Seger, J.] Creighton Univ, Omaha, NE 68178 USA. [Choi, K. E.; Oh, K.; Yoo, I-K.] Pusan Natl Univ, Pusan 609735, South Korea. [Leyva, A. Davila; Hoffmann, G. W.; Li, L.; Markert, C.; Oldag, E. W.; Ray, R. L.; Schambach, J.; Thein, D.; Wada, M.] Univ Texas Austin, Austin, TX 78712 USA. [Derevschikov, A. A.; Matulenko, Yu A.; Meschanin, A.; Minaev, N. G.; Morozov, D. A.; Nogach, L. V.; Nurushev, S. B.; Vasiliev, A. N.] Inst High Energy Phys, Protvino 142281, Russia. [Derradi de Souza, R.; Takahashi, J.; Vasconcelos, G. M. S.] Univ Estadual Campinas, BR-13083859 Sao Paulo, Brazil. [Elnimr, M.; LaPointe, S.; Pruneau, C.; Sharma, M.; Tarini, L. H.; Voloshin, S. A.] Wayne State Univ, Detroit, MI 48201 USA. [Eppley, G.; Geurts, F.; Llope, W. J.; McDonald, D.; Roberts, J. B.; Yepes, P.] Rice Univ, Houston, TX 77251 USA. [Eun, L.; Heppelmann, S.] Penn State Univ, University Pk, PA 16802 USA. [Fatemi, R.; Fersch, R. G.; Korsch, W.; Webb, G.; Witzke, W.] Univ Kentucky, Lexington, KY 40506 USA. [Grosnick, D.; Koetke, D. D.; Manweiler, R.; Stanislaus, T. D. S.] Valparaiso Univ, Valparaiso, IN 46383 USA. [Hirsch, A.; Kikola, D. P.; Konzer, J.; Li, X.; Mustafa, M. K.; Netrakanti, P. K.; Scharenberg, R. P.; Skoby, M. J.; Srivastava, B.; Stringfellow, B.; Wang, F.; Wang, Q.; Xie, W.] Purdue Univ, W Lafayette, IN 47907 USA. [Jacobs, W.; Page, B. S.; Selyuzhenkov, I.; Stevens, J. R.; Wissink, S. W.] Indiana Univ, Bloomington, IN 47408 USA. [Jena, C.; Mahapatra, D. P.] Inst Phys, Bhubaneswar 751005, Orissa, India. [Kisiel, A.; Pawlak, T.; Peryt, W.; Pluta, J.; Zawisza, M.; Zbroszczyk, H.] Warsaw Univ Technol, PL-00661 Warsaw, Poland. [Kollegger, T.; Schuster, T. R.; Stock, R.; Zhou, W.] Goethe Univ Frankfurt, D-60325 Frankfurt, Germany. [Li, X.; Xu, Q. H.] Shandong Univ, Jinan 250100, Shandong, Peoples R China. [Munhoz, M. G.; Suaide, A. A. P.; Szanto de Toledo, A.] Univ Sao Paulo, BR-05508090 Sao Paulo, Brazil. [Planinic, M.; Poljak, N.] Univ Zagreb, HR-10002 Zagreb, Croatia. [Qiu, H.; Sun, Z.; Wang, J. S.; Xu, H.; Yang, Y.; Zhan, W.] Inst Modern Phys, Lanzhou 730000, Peoples R China. [Raniwala, R.; Raniwala, S.; Solanki, D.] Univ Rajasthan, Jaipur 302004, Rajasthan, India. [Schmitz, N.; Seyboth, P.; Simon, F.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Tarnowsky, T.; Wang, H.; Westfall, G. D.] Michigan State Univ, E Lansing, MI 48824 USA. [Witt, R.] USN Acad, Annapolis, MD 21402 USA. RI Takahashi, Jun/B-2946-2012; Alekseev, Igor/J-8070-2014; Yoo, In-Kwon/J-6222-2012; Peitzmann, Thomas/K-2206-2012; Witt, Richard/H-3560-2012; Yip, Kin/D-6860-2013; Xue, Liang/F-8077-2013; Voloshin, Sergei/I-4122-2013; Pandit, Yadav/I-2170-2013; Lednicky, Richard/K-4164-2013; Yang, Yanyun/B-9485-2014; Rusnak, Jan/G-8462-2014; Bielcikova, Jana/G-9342-2014; Sumbera, Michal/O-7497-2014; Strikhanov, Mikhail/P-7393-2014; Xu, Wenqin/H-7553-2014; Bruna, Elena/C-4939-2014; Dogra, Sunil /B-5330-2013; Chaloupka, Petr/E-5965-2012; Huang, Bingchu/H-6343-2015; Derradi de Souza, Rafael/M-4791-2013; Suaide, Alexandre/L-6239-2016; Svirida, Dmitry/R-4909-2016; Inst. of Physics, Gleb Wataghin/A-9780-2017; Okorokov, Vitaly/C-4800-2017; Ma, Yu-Gang/M-8122-2013; OI Takahashi, Jun/0000-0002-4091-1779; Alekseev, Igor/0000-0003-3358-9635; Peitzmann, Thomas/0000-0002-7116-899X; Yip, Kin/0000-0002-8576-4311; Xue, Liang/0000-0002-2321-9019; Pandit, Yadav/0000-0003-2809-7943; Yang, Yanyun/0000-0002-5982-1706; Sumbera, Michal/0000-0002-0639-7323; Strikhanov, Mikhail/0000-0003-2586-0405; Xu, Wenqin/0000-0002-5976-4991; Bruna, Elena/0000-0001-5427-1461; Huang, Bingchu/0000-0002-3253-3210; Derradi de Souza, Rafael/0000-0002-2084-7001; Suaide, Alexandre/0000-0003-2847-6556; Okorokov, Vitaly/0000-0002-7162-5345; Ma, Yu-Gang/0000-0002-0233-9900; Fisyak, Yuri/0000-0002-3151-8377; Bhasin, Anju/0000-0002-3687-8179; Ke, Hongwei/0000-0003-1463-7291; Sorensen, Paul/0000-0001-5056-9391; Thomas, James/0000-0002-6256-4536 FU RHIC Operations Group; RACF at BNL; NERSC Center at LBNL; Open Science Grid consortium; Offices of NP and HEP within the US DOE Office of Science; US NSF; Sloan Foundation; DFG cluster of excellence 'Origin and Structure of the Universe' of Germany; CNRS/IN2P3; FAPESP; CNPq of Brazil; Ministry of Education and Science of the Russian Federation; NNSFC; CAS; MoST; MoE of China; GA and MSMT of the Czech Republic; FOM and NWO of the Netherlands; DAE, DST and CSIR of India; Polish Ministry of Science and Higher Education; Korea Research Foundation; Ministry of Science, Education and Sports of Croatia; RosAtom of Russia FX We thank the RHIC Operations Group and RACF at BNL, the NERSC Center at LBNL and the Open Science Grid consortium for providing resources and support. This work was supported in part by the Offices of NP and HEP within the US DOE Office of Science, the US NSF, the Sloan Foundation, the DFG cluster of excellence 'Origin and Structure of the Universe' of Germany, CNRS/IN2P3, FAPESP, CNPq of Brazil, the Ministry of Education and Science of the Russian Federation, NNSFC, CAS, MoST and MoE of China, GA and MSMT of the Czech Republic, FOM and NWO of the Netherlands, DAE, DST and CSIR of India, the Polish Ministry of Science and Higher Education, the Korea Research Foundation, the Ministry of Science, Education and Sports of Croatia, and RosAtom of Russia. NR 30 TC 56 Z9 57 U1 5 U2 68 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAY 19 PY 2011 VL 473 IS 7347 BP 353 EP 356 DI 10.1038/nature10079 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 765QA UT WOS:000290722400043 ER PT J AU Liu, HH AF Liu, Hui-Hai TI A note on equations for steady-state optimal landscapes SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID RIVER NETWORKS; ENERGY-DISSIPATION; DRAINAGE NETWORKS; MINIMUM ENERGY; MODEL; EVOLUTION; BASIN; HILLSLOPE AB Based on the optimality principle (that the global energy expenditure rate is at its minimum for a given landscape under steady state conditions) and calculus of variations, we have derived new governing equations for describing steady-state optimal landscapes. Other than building on the well-established Manning's equation, this work does not rely on any empirical relationships (such as those relating hydraulic parameters to local slopes). Using additional constraints, we also theoretically demonstrate that discharge is a power function of local slope, which is consistent with field data and previous studies. Citation: Liu, H.-H. (2011), A note on equations for steady-state optimal landscapes, Geophys. Res. Lett., 38, L10402, doi:10.1029/2011GL047619. C1 Univ Calif Berkeley, Lawrence Berkeley Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Liu, HH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Earth Sci, MS 90-1116, Berkeley, CA 94720 USA. EM hhliu@lbl.gov FU U.S. Department of Energy (DOE) [DE-AC02-05CH11231] FX We are indebted to Yingqi Zhang and Dan Hawkes at Lawrence Berkeley National Laboratory for their critical and careful review of a preliminary version of this manuscript. We also appreciate the constructive comments from Riccardo Rigon and an anonymous reviewer. This work was supported by the U.S. Department of Energy (DOE), under DOE contract DE-AC02-05CH11231. NR 25 TC 4 Z9 4 U1 2 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAY 19 PY 2011 VL 38 AR L10402 DI 10.1029/2011GL047619 PG 4 WC Geosciences, Multidisciplinary SC Geology GA 767QX UT WOS:000290872200006 ER PT J AU Soderholm, L Skanthakumar, S Wilson, RE AF Soderholm, L. Skanthakumar, S. Wilson, Richard E. TI Structural Correspondence between Uranyl Chloride Complexes in Solution and Their Stability Constants SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID X-RAY-SCATTERING; AQUEOUS-SOLUTION; DIOXOURANIUM(VI) ION; UO22+ ION; AQUA ION; COORDINATION; URANIUM(VI); CATION; EXAFS; SPECIATION AB Pair-distribution functions (PDF)s were obtained from high-energy X-ray scattering (HEXS) data on a series of uranyl solutions as a function of chloride ion concentration. Analyses reveal that chloride forms only inner-sphere complexes with the uranyl, replacing inner-sphere waters such that the total uranyl coordination number decreases from 4.7 waters at [Cl(-)] = 0 m to 4.4 (1.7 water and 2.7 Cl(-)) at [Cl(-)] = 6.8 m. Some of the second-coordination sphere waters reorient upon uranyl inner-sphere chloride complexation in order to hydrogen bond with the bound anion. Similar data obtained on a series of solutions maintained at constant ionic strength are used to confirm structural assignments through determining stability constants for the addition of chloride to uranyl and comparison with published values. The stability constants, beta(1) = 1.5(10) m(-1), beta(2) = 0.8(4) m(-2), and beta(3) = 0.4(1) m(-3), obtained in a series of solutions with constant ionic strength of 5.3 m, are in reasonable agreement with previously published results determined by solvent extraction. The agreement of s ability constants supports our peak assignments for the PDF and thus our structural model for uranyl chloride complexes in solution. Using coordination numbers and speciation determined here as a function of chloride ion concentration, the monochloro species is found to have four coordinating waters in the uranyl equatorial plane, the dichoro species is found to be an equilibrium of three and two coordinating waters, and the trichloro species has only a single water in the equatorial plane. These values correspond to total average coordination numbers of 5, 4.3, and 4 for the mono-, di-, and trichlorouranyl complexes. From the equilibrium value of the dichloro species, it can be further estimated that Delta G = -0.5 kcal/mol for the conversion of five to four coordinate species. Overall, the HEXS data support the assertion that uranyl chloride correlations do exist and the results are not simply the result of solvent-ion effects. C1 [Soderholm, L.; Skanthakumar, S.; Wilson, Richard E.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Soderholm, L (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ls@anl.gov RI Wilson, Richard/H-1763-2011 OI Wilson, Richard/0000-0001-8618-5680 FU U.S. DOE, OBES, Chemical Sciences, Geosciences, and Biosciences Division [DE- AC02-06CH11357]; OBES, Materials Sciences [DE- AC02-06CH11357] FX We acknowledge the Actinide Facility for technical support during synchrotron experiments. This work is supported by the U.S. DOE, OBES, Chemical Sciences, Geosciences, and Biosciences Division under Contract DE- AC02-06CH11357. The APS is supported by OBES, Materials Sciences, under the same contract number. NR 51 TC 22 Z9 22 U1 2 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 19 PY 2011 VL 115 IS 19 BP 4959 EP 4967 DI 10.1021/jp111551t PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 761UU UT WOS:000290427300012 PM 21526745 ER PT J AU Xu, Q Ban, CM Dillon, AC Wei, SH Zhao, YF AF Xu, Qiang Ban, Chunmei Dillon, Anne C. Wei, Su-Huai Zhao, Yufeng TI First-Principles Study of Lithium Borocarbide as a Cathode Material for Rechargeable Li ion Batteries SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID AB-INITIO; LIXBC; SUPERCONDUCTIVITY; ELECTRODES; CHEMISTRY; OXIDES; BC3 AB Computational simulations within density functional theory are performed to investigate the potential application of a lithium borocarbide (LiBC) compound as a unique material for lithium ion batteries. The graphene-like BC sheets are predicted to be Li+ intercalation hosts with the Li ion capacity surprisingly surpassing that of graphite. Here, the layered LixBC structure is preserved with x >= 0.5, indicating that half of the Li ions in the LiBC compound are rechargeable. Furthermore, the intercalation potential (equilibrium lithium-insertion voltage of 2.3-2.4 V relative to lithium metal) is significantly higher than that in graphite, allowing Li0.5BC to function as a cathode material. The reversible electrochemical reaction, LiBC reversible arrow Li0.5BC 0.5Li, enables a specific energy density of 1088 W h/kg and a volumetric energy density of 2463 Wh/L. The volume change is less than 3% during the charging and discharging process. This discovery could lead to the development of a unique high-capacity LiBC Li ion cathode material. C1 [Xu, Qiang; Ban, Chunmei; Dillon, Anne C.; Wei, Su-Huai; Zhao, Yufeng] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Zhao, YF (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM Yufeng.Zhao@nrel.gov FU U.S. Department of Energy through the DOE's Office of Energy Efficiency and Renewable Energy Office of the Vehicle Technologies [DE-AC36-08GO28308]; NREL FX This work was funded by the U.S. Department of Energy under Subcontract Number DE-AC36-08GO28308 through the DOE's Office of Energy Efficiency and Renewable Energy Office of the Vehicle Technologies Program and NREL's Laboratory Directed Research and Development Program. NR 35 TC 13 Z9 13 U1 4 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 19 PY 2011 VL 2 IS 10 BP 1129 EP 1132 DI 10.1021/jz200440m PG 4 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 767GQ UT WOS:000290843700004 PM 26295314 ER PT J AU Beckham, GT Peters, B AF Beckham, Gregg T. Peters, Baron TI Optimizing Nucleus Size Metrics for Liquid-Solid Nucleation from Transition Paths of Near-Nanosecond Duration SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID MONTE-CARLO SIMULATIONS; LENNARD-JONES SYSTEM; CRYSTAL-NUCLEATION; RATE CONSTANTS; MOLECULAR-DYNAMICS; REACTION COORDINATE; CROSS-NUCLEATION; PHASE FORMATION; ISING-MODEL; BARRIERS AB We determine the mechanism for the liquid-solid phase transition in the Lennard-Jones fluid close to coexistence with aimless shooting and likelihood maximization. The reaction coordinate for this process is a product of a structural descriptor and the size of the nascent solid nucleus and is quantitatively verified with the committor probability histogram test. This study identifies the first accurate scalar reaction coordinate for the liquid-solid nucleation process in Lennard-Jonesium, which will likely extend to nucleation processes in other spherically symmetric fluids. On the basis of our results, we propose a structural correction factor for the commonly cited nucleus size reaction coordinate from classical nucleation theory that enables connection of simulation data to stochastic models of nucleation kinetics. In addition, we show that aimless shooting is able to obtain reasonable acceptance rates for transitions with highly diffusive characteristics, which has been problematic for transition path sampling methods for diffusive processes such as nucleation and macromolecular transitions. C1 [Beckham, Gregg T.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. [Beckham, Gregg T.] Colorado Sch Mines, Dept Chem Engn, Golden, CO 80401 USA. [Peters, Baron] Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. [Peters, Baron] Univ Calif Santa Barbara, Dept Chem & Biochem, Santa Barbara, CA 93106 USA. RP Beckham, GT (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. EM gregg.beckham@nrel.gov FU NSF [0955502]; National Renewable Energy Laboratory FX B.P. was supported by NSF CAREER Award 0955502. We acknowledge Peter Bolhuis and Wolfgang Lechner for helpful discussions. Computational time for this research was supported in part by the Golden Energy Computing Organization at the Colorado School of Mines using resources acquired with financial assistance from the National Science Foundation and the National Renewable Energy Laboratory. NR 64 TC 27 Z9 27 U1 0 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 19 PY 2011 VL 2 IS 10 BP 1133 EP 1138 DI 10.1021/jz2002887 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 767GQ UT WOS:000290843700005 PM 26295315 ER PT J AU Wang, XB Xantheas, SS AF Wang, Xue-Bin Xantheas, Sotiris S. TI Photodetachment of Isolated Bicarbonate Anion: Electron Binding Energy of HCO3- SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID CARBON-DIOXIDE; WAVE-FUNCTIONS; CONFIGURATION-INTERACTION; COUPLED-CLUSTER; GAS-PHASE; PHOTOELECTRON-SPECTROSCOPY; AQUEOUS-SOLUTION; BASIS-SETS; CHEMISTRY; SYSTEM AB We report the first direct photodetachment photoelectron spectroscopy of HCO3- in the gas phase under low-temperature conditions. The observed photoelectron spectra are complicated due to excitations of manifolds in both vibrational and electronic states. A long and single vibrational progression with a frequency of 530 +/- 20 cm(-1) is partially resolved in the threshold of the T = 20 K, 266 nm spectrum. The adiabatic electron detachment energy (ADE) of HCO3-, or, in other words, the electron affinity (EA) of neutral HCO3, is experimentally determined from the (0,0) transition to be 3.680 +/- 0.015 eV. The computed values of the Franck-Condon integral and intensity are favorable for observing the (0,0) transition. High-level ab initio calculations at the CCSD-(T) level of theory produce an estimated anharmonic frequency of 546 cm(-1) for HCO3 and a value of 3.79 eV for the (0,0) transition, both in good agreement with the experimentally determined values. C1 [Wang, Xue-Bin; Xantheas, Sotiris S.] Pacific NW Natl Lab, Div Chem & Mat Sci, Richland, WA 99352 USA. [Wang, Xue-Bin] Washington State Univ, Dept Phys, Richland, WA 99354 USA. RP Wang, XB (reprint author), Pacific NW Natl Lab, Div Chem & Mat Sci, 902 Battelle Blvd,POB 999,MS K1-83, Richland, WA 99352 USA. EM xuebin.wang@pnl.gov; sotiris.xantheas@pnl.gov RI Xantheas, Sotiris/L-1239-2015 FU Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy (DOE); DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory; Department of Energy's Office of Biological and Environmental Research FX This work was supported by the Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy (DOE). Part of this work was performed at the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory, which is operated by Battelle for the DOE. This research was performed in part using the Molecular Science Computing Facility (MSCF) in the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research. Additional computer resources were provided by the Office of Basic Energy Sciences, U.S. Department of Energy at the National Energy Research Scientific Computing Center (NERSC), a U.S. Department of Energy Office of Science user facility at Lawrence Berkeley National Laboratory. NR 46 TC 4 Z9 4 U1 3 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 19 PY 2011 VL 2 IS 10 BP 1204 EP 1210 DI 10.1021/jz200327f PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 767GQ UT WOS:000290843700018 PM 26295327 ER PT J AU Jiang, DE Overbury, SH Dai, S AF Jiang, De-en Overbury, Steven H. Dai, Sheng TI Interaction of Gold Clusters with a Hydroxylated Surface SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID TEMPERATURE CO OXIDATION; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; SELECTIVE OXIDATION; AU CATALYSTS; NANOPARTICLES; NANOCLUSTERS; DENSITY; TITANIA; SILICA AB We explore the interaction between gold nanoclusters and a fully hydroxylated surface, Mg(OH)(2)'s basal plane, by using a density functional theory-enabled local basin-hopping technique for global-minimum search. We find strong interaction of gold nanoclusters with the surface hydroxyls via a short bond between edge Au atoms and O atoms of the -OH groups. We expect that this strong interaction is ubiquitous on hydroxylated support surfaces and helps the gold nanoclusters against sintering, thereby contributing to their CO-oxidation activity at low temperatures. C1 [Jiang, De-en; Overbury, Steven H.; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Overbury, Steven H.; Dai, Sheng] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Jiang, DE (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM jiangd@ornl.gov RI Jiang, De-en/D-9529-2011; Overbury, Steven/C-5108-2016; Dai, Sheng/K-8411-2015 OI Jiang, De-en/0000-0001-5167-0731; Overbury, Steven/0000-0002-5137-3961; Dai, Sheng/0000-0002-8046-3931 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 39 TC 19 Z9 20 U1 4 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 19 PY 2011 VL 2 IS 10 BP 1211 EP 1215 DI 10.1021/jz200420t PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 767GQ UT WOS:000290843700019 PM 26295328 ER PT J AU Ressler, JJ Burke, JT Escher, JE Angell, CT Basunia, MS Beausang, CW Bernstein, LA Bleuel, DL Casperson, RJ Goldblum, BL Gostic, J Hatarik, R Henderson, R Hughes, RO Munson, J Phair, LW Ross, TJ Scielzo, ND Swanberg, E Thompson, IJ Wiedeking, M AF Ressler, J. J. Burke, J. T. Escher, J. E. Angell, C. T. Basunia, M. S. Beausang, C. W. Bernstein, L. A. Bleuel, D. L. Casperson, R. J. Goldblum, B. L. Gostic, J. Hatarik, R. Henderson, R. Hughes, R. O. Munson, J. Phair, L. W. Ross, T. J. Scielzo, N. D. Swanberg, E. Thompson, I. J. Wiedeking, M. TI Surrogate measurement of the Pu-238(n, f) cross section SO PHYSICAL REVIEW C LA English DT Article ID NEUTRON FISSION AB The neutron-induced fission cross section of Pu-238 was determined using the surrogate ratio method. The (n, f) cross section over an equivalent neutron energy range 5-20 MeV was deduced from inelastic alpha-induced fission reactions on Pu-239, with U-235(alpha, alpha' f) and U-236(alpha, alpha' f) used as references. These reference reactions reflect U-234(n, f) and U-235(n, f) yields, respectively. The deduced Pu-238(n, f) cross section agrees well with standard data libraries up to similar to 10 MeV, although larger values are seen at higher energies. The difference at higher energies is less than 20%. C1 [Ressler, J. J.; Burke, J. T.; Escher, J. E.; Bernstein, L. A.; Bleuel, D. L.; Casperson, R. J.; Gostic, J.; Hatarik, R.; Henderson, R.; Scielzo, N. D.; Swanberg, E.; Thompson, I. J.; Wiedeking, M.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Angell, C. T.; Goldblum, B. L.; Munson, J.; Swanberg, E.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Basunia, M. S.; Hatarik, R.; Phair, L. W.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Beausang, C. W.; Hughes, R. O.; Ross, T. J.] Univ Richmond, Dept Phys, Richmond, VA 23173 USA. [Ross, T. J.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. RP Ressler, JJ (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM ressler2@llnl.gov RI Escher, Jutta/E-1965-2013; Burke, Jason/I-4580-2012 FU US Department of Energy [DE-AC52-07NA27344 (LLNL), DE-AC02-05CH11231 (LBNL)]; Department of Energy's NNSA, Office of Nonproliferation Research and Development [NA-22] FX The authors thank the 88-Inch Cyclotron operations and facilities staff for the support of this study. We would also like to thank the Department of Energy's NNSA, Office of Nonproliferation Research and Development (NA-22), for financial support. This work was performed under the auspices of the US Department of Energy under Contracts No. DE-AC52-07NA27344 (LLNL) and No. DE-AC02-05CH11231 (LBNL). NR 29 TC 23 Z9 23 U1 1 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAY 19 PY 2011 VL 83 IS 5 AR 054610 DI 10.1103/PhysRevC.83.054610 PG 7 WC Physics, Nuclear SC Physics GA 766DF UT WOS:000290760500002 ER PT J AU Cao, QH Damanik, A Ma, E Wegman, D AF Cao, Qing-Hong Damanik, Asan Ma, Ernest Wegman, Daniel TI Probing lepton flavor triality with Higgs boson decay SO PHYSICAL REVIEW D LA English DT Article AB If neutrino tribimaximal mixing is explained by a non-Abelian discrete symmetry such as A(4), T-7, Delta(27), etc., the charged-lepton Higgs sector has a Z(3) residual symmetry (lepton flavor triality), which may be observed directly in the decay chain H-0 -> psi(0)(2)(psi) over bar (0)(2), then psi(0)(2)(($) over bar (0)(2)) -> l(i)(+) l(j)(-) (i not equal j), where H-0 is a standard-model-like Higgs boson and psi(0)(2) is a scalar particle needed for realizing the original discrete symmetry. If kinematically allowed, this unusual and easily detectable decay is observable at the LHC with 1 fb(-1) for E-cm = 7 TeV. C1 [Cao, Qing-Hong] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Cao, Qing-Hong] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Damanik, Asan] Sanata Dharma Univ, Dept Phys, Yogyakarta, Indonesia. [Ma, Ernest; Wegman, Daniel] Univ Calif Riverside, Dept Phys & Astron, Riverside, CA 92521 USA. RP Cao, QH (reprint author), Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. RI lebert, thomas/H-4032-2011; OI Wegman, Daniel/0000-0002-8189-1313; Damanik, Asan/0000-0003-3241-0162 FU U.S. Department of Energy [DE-AC02-06CH11357, DE-FG03-94ER40837]; Argonne National Laboratory; University of Chicago Joint Theory Institute [03921-07-137]; Ministry of National Education, Indonesia FX Q. H. C. is supported in part by the U.S. Department of Energy under Grant No. DE-AC02-06CH11357 and the Argonne National Laboratory and University of Chicago Joint Theory Institute Grant No. 03921-07-137. A. D. is supported by the Program of Academic Recharging C (PAR-C), Ministry of National Education, Indonesia. E. M. and D. W. are supported in part by the U.S. Department of Energy under Grant No. DE-FG03-94ER40837. A. D. thanks the Department of Physics and Astronomy, University of California, Riverside for hospitality during his visit. NR 17 TC 17 Z9 17 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 19 PY 2011 VL 83 IS 9 AR 093012 DI 10.1103/PhysRevD.83.093012 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 766DI UT WOS:000290760800003 ER PT J AU Velizhanin, KA Chien, CC Dubi, Y Zwolak, M AF Velizhanin, Kirill A. Chien, Chih-Chun Dubi, Yonatan Zwolak, Michael TI Driving denaturation: Nanoscale thermal transport as a probe of DNA melting SO PHYSICAL REVIEW E LA English DT Article ID HEAT-CONDUCTION; NONLINEAR MODEL; DYNAMICS; CHAINS AB DNA denaturation has been a subject of intense study due to its relationship to DNA transcription and its fundamental importance as a nonlinear structural transition. Many aspects of this phenomenon, however, remain poorly understood. Existing models fit quite well with experimental results on the fraction of unbound base pairs versus temperature, but yield incorrect results for other essential quantities such as the base pair fluctuation time scales. Here we demonstrate that nanoscale thermal transport can serve as a sensitive probe of the underlying microscopic physics responsible for the dynamics of DNA denaturation. Specifically, we show that the heat transport properties of DNA are altered significantly as it denatures, and this alteration encodes detailed information on the dynamics of thermal fluctuations and their interaction along the strand. This finding allows for the discrimination between models of DNA denaturation and will help shed new light on the nonlinear vibrational dynamics of this important molecule. C1 [Velizhanin, Kirill A.; Chien, Chih-Chun; Dubi, Yonatan; Zwolak, Michael] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Velizhanin, Kirill A.] Los Alamos Natl Lab, CNLS, Los Alamos, NM 87545 USA. RP Velizhanin, KA (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM kirill@lanl.gov; mpz@lanl.gov RI Zwolak, Michael/G-2932-2013; Dubi, Yonatan/G-5304-2013; Velizhanin, Kirill/C-4835-2008 OI Zwolak, Michael/0000-0001-6443-7816; FU US Department of Energy; CNLS FX The authors would like to thank A. R. Bishop, K. Rasmussen, and B. Alexandrov for valuable discussions. This research is supported by the US Department of Energy through the LANL/LDRD Program. K. A. V. also acknowledges the support provided by CNLS. NR 31 TC 12 Z9 12 U1 0 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 J9 PHYS REV E JI Phys. Rev. E PD MAY 19 PY 2011 VL 83 IS 5 AR 050906 DI 10.1103/PhysRevE.83.050906 PN 1 PG 4 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 766DZ UT WOS:000290762500002 PM 21728482 ER PT J AU Lunin, A Yakovlev, V Grudiev, A AF Lunin, A. Yakovlev, V. Grudiev, A. TI Analytical solutions for transient and steady state beam loading in arbitrary traveling wave accelerating structures SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article AB Analytical solutions are derived for both transient and steady state gradient distributions in the traveling wave (TW) accelerating structures with arbitrary variation of parameters over the structure length. The results of the unloaded and beam loaded cases are presented. Finally, the exact analytical shape of the rf pulse waveform was found in order to apply the transient beam loading compensation scheme during the structure filling time. The obtained theoretical formulas were cross-checked by direct numerical simulations on the CLIC main linac accelerating structure and demonstrated a good agreement. The proposed methods provide a fast and reliable tool for the initial stage of the TW structure analysis. C1 [Lunin, A.; Yakovlev, V.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Grudiev, A.] CERN, CH-1211 Geneva 23, Switzerland. RP Lunin, A (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. NR 21 TC 3 Z9 3 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD MAY 19 PY 2011 VL 14 IS 5 AR 052001 DI 10.1103/PhysRevSTAB.14.052001 PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 766EJ UT WOS:000290763500001 ER PT J AU Vorobiev, A Major, J Dosch, H Mueller-Buschbaum, P Falus, P Felcher, GP Velthuis, SGET AF Vorobiev, A. Major, J. Dosch, H. Mueller-Buschbaum, P. Falus, P. Felcher, G. P. Velthuis, S. G. E. te TI Phase and Microphase Separation of Polymer Thin Films Dewetted from Silicon-A Spin-Echo Resolved Grazing Incidence Neutron Scattering Study SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID DIBLOCK COPOLYMER FILMS; X-RAY; ANGLE; DIFFRACTION; SIMULATION; SURFACES; REFLECTIVITY; TRANSITIONS; ORDER AB An understanding of the structure of ultrathin polymer films on solid substrates has scientific importance in applications as well as in fundamental studies of polymer diffusion or adsorption. We present studies of the organization of dewetted droplets of polymers on a silicon surface using a new neutron scattering technique, spin echo resolved grazing incidence scattering (SERGIS), that has the potential to address at the same time the droplet droplet correlations and the chemical configuration inside each droplet. For the seminal experiments, the polarized neutron reflectometer EVA at the Institut Laue-Langevin, Grenoble, France, was equipped with a spin echo setup, and measurements were taken on surface structures previously characterized by different techniques. The dewetted polymers used in our studies were pure polystyrene, a mixture of polystyrene and polyparamethylstyrene, and a diblock copolymer of the two homopolymers. Even with a provisional setup SERGIS, we were able to determine the correlation between the droplets, providing results in excellent agreement with those obtained by atomic force microscopy and grazing incidence small-angle X-ray and neutron scattering. In addition, it was confirmed that the correlation function for diblock copolymer droplets is more complex than for polymer mixtures, exhibiting partial ordering of the copolymer within each droplet. C1 [Vorobiev, A.; Major, J.; Dosch, H.] Max Planck Inst Metallforsch, D-70569 Stuttgart, Germany. [Mueller-Buschbaum, P.] Tech Univ Munich, Lehrstuhl Funkt Mat, Phys Dept E13, D-85747 Garching, Germany. [Falus, P.; Felcher, G. P.; Velthuis, S. G. E. te] Argonne Natl Lab, Argonne, IL 60439 USA. [Dosch, H.] DESY, D-2000 Hamburg, Germany. RP Vorobiev, A (reprint author), Max Planck Inst Metallforsch, Heisenbergstr 3, D-70569 Stuttgart, Germany. EM alexei.vorobiev@esrf.fr RI te Velthuis, Suzanne/I-6735-2013; Muller-Buschbaum, Peter/C-3397-2017 OI te Velthuis, Suzanne/0000-0002-1023-8384; Muller-Buschbaum, Peter/0000-0002-9566-6088 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-06CH11357]; Max Planck Society, Munich; DFG [SPP 1164, Mu1487/2] FX The support of the management and staff at the Institut Laue-Langevin, Grenoble, France, is gratefully acknowledged. This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under contract No. DE-AC02-06CH11357 (PF, SGEtV, and GPF) and by focused neutron research funding of the Max Planck Society, Munich. P.M.B. acknowledges funding by the DFG Schwerpunktprogramm SPP 1164 "Nano- and Microfluidics" (Mu1487/2). NR 50 TC 3 Z9 3 U1 2 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 19 PY 2011 VL 115 IS 19 BP 5754 EP 5765 DI 10.1021/jp1120756 PG 12 WC Chemistry, Physical SC Chemistry GA 761US UT WOS:000290427100007 PM 21504157 ER PT J AU Khodadadi, S Curtis, JE Sokolov, AP AF Khodadadi, S. Curtis, J. E. Sokolov, A. P. TI Nanosecond Relaxation Dynamics of Hydrated Proteins: Water versus Protein Contributions SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID METHYL-GROUP DYNAMICS; MOLECULAR-DYNAMICS; NEUTRON-SCATTERING; DIELECTRIC-SPECTROSCOPY; GLASS-TRANSITION; SIDE-CHAIN; LYSOZYME; SOLVENT; SIMULATIONS; PLASTOCYANIN AB We have studied picosecond to nanosecond dynamics of hydrated protein powders using dielectric spectroscopy and molecular dynamics (MD) simulations. Our analysis of hydrogen-atom single particle dynamics from MD simulations focused on "main" (tau(main) approximate to tens of picoseconds) and "slow" (tau(slow) approximate to nanosecond) relaxation processes that were observed in dielectric spectra of similar hydrated protein samples. Traditionally, the interpretation of these processes observed in dielectric spectra has been ascribed to the relaxation behavior of hydration water tightly bounded to a protein and not to protein atoms. Detailed analysis of the MD simulations and comparison to dielectric data indicate that the observed relaxation process in the nanosecond time range of hydrated protein spectra is mainly due to protein atoms. The relaxation processes involve the entire structure of protein including atoms in the protein backbone, side chains, and turns. Both surface and buried protein atoms contribute to the slow processes; however, surface atoms demonstrate slightly faster relaxation dynamics. Analysis of the water molecule residence and dipolar relaxation correlation behavior indicates that the hydration water relaxes at much shorter time scales. C1 [Khodadadi, S.; Curtis, J. E.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Sokolov, A. P.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Sokolov, A. P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Khodadadi, S (reprint author), NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. EM sheila.khodadadi@nist.gov FU NSF [DMR-1059562]; National Research Council FX We acknowledge the partial financial support from NSF (DMR-1059562). S.K. acknowledges the National Research Council for support. Certain commercial equipment, instruments, materials, suppliers, or software are identified in this paper to foster understanding. Such identification does not imply recommendation or endorsement by the National Institute of Standards and Technology, nor does it imply that the materials or equipment identified are necessarily the best available for the purpose. NR 44 TC 28 Z9 28 U1 1 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 19 PY 2011 VL 115 IS 19 BP 6222 EP 6226 DI 10.1021/jp1122213 PG 5 WC Chemistry, Physical SC Chemistry GA 761US UT WOS:000290427100056 PM 21513284 ER PT J AU Ishizaki, A Fleming, GR AF Ishizaki, Akihito Fleming, Graham R. TI On the Interpretation of Quantum Coherent Beats Observed in Two-Dimensional Electronic Spectra of Photosynthetic Light Harvesting Complexes SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID WAVE-PACKET INTERFEROMETRY; ENERGY-TRANSFER; PHYSIOLOGICAL TEMPERATURE; DYNAMICS; MODEL; DECOHERENCE; EXCITATION; VIBRATIONS; MOLECULES; SYSTEMS AB The observation of long-lived electronic quantum coherence in a photosynthetic light harvesting system [Engel et al. Nature 2007, 446, 782] has led to much effort being devoted to elucidation of the quantum mechanisms of the photosynthetic excitation energy transfer. In this paper we examine the question of whether the decay of the coherent beating signal is due to quantum mechanical decoherence or ensemble dephasing (also called "fake decoherence"). We compare results based on the quantum master equation description of the time-evolution of the reduced density matrix with a mixed quantum/classical approach where the ensemble average is calculated after the dynamics. The two methods show good agreement with results from the quantum master equation in terms of the decay of quantum coherent oscillations when ensemble average is considered for the mixed quantum/classical approach. However, the results also demonstrate it remains possible that the quantum coherent motion is robust under individual realizations of the environment-induced fluctuations contrary to intuition obtained from the reduced density matrices, indicating that the decay of the observed quantum coherence should be understood as ensemble dephasing. Our calculations imply that coherence is a property of the pigment-protein system, not simply the preparation method of the electronic excitation. C1 [Fleming, Graham R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Fleming, GR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM GRFleming@lbl.gov RI Ishizaki, Akihito/A-7069-2010 OI Ishizaki, Akihito/0000-0002-0246-4461 FU Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC03-76SF000098] FX We acknowledge an allocation of supercomputing time from the National Energy Research Scientific Computing Center. This work was supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract DE-AC02-05CH11231 and the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy through Grant DE-AC03-76SF000098. NR 59 TC 67 Z9 67 U1 3 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 19 PY 2011 VL 115 IS 19 BP 6227 EP 6233 DI 10.1021/jp112406h PG 7 WC Chemistry, Physical SC Chemistry GA 761US UT WOS:000290427100057 PM 21488648 ER PT J AU Green, J Tyrrell, Z Radosz, M Hong, K Mays, JW AF Green, Jade Tyrrell, Zachary Radosz, Maciej Hong, Kunlun Mays, Jimmy W. TI Nanostructure of Solid Precipitates Obtained by Expansion of Polystyrene-block-Polybutadiene Solutions in Near Critical Propane: Block Ratio and Micellar Solution Effects SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID COPOLYMER THIN-FILMS; ANIONIC-POLYMERIZATION; MODEL POLYDIENES; POLYISOPRENE; POLYOLEFINS; PRESSURE; SOLVENT; PHASE AB In contrast to incompressible liquid solutions, compressible near-critical solutions of block copolymers allow for controlling rapid structure transformations with pressure alone. For example, when dissolved in near-critical propane, polystyrene-block-polybutadiene can form a random molecular solution at high pressures, a micellar solution at moderate pressures, and a solvent-free precipitate at low pressures. In contrast to the unstructured virgin copolymer, such a propane-treated precipitate rapidly self-assembles toward structures characteristic of equilibrated block copolymers, such as lamellae, spheres, or cylinders, which depend on the block ratio rather than on the decompression rate or temperature, at least within the rate and temperature ranges investigated in this work. At lower temperatures, however, say below 40 degrees C, glass transition of the styrene-butadiene diblocks can inhibit independent structure formation, while crystallization of their hydrogenated-butadiene analogues can preserve the micellar-solution structure. C1 [Green, Jade; Tyrrell, Zachary; Radosz, Maciej] Univ Wyoming, Soft Mat Lab, Dept Chem & Petr Engn, Laramie, WY 82071 USA. [Hong, Kunlun; Mays, Jimmy W.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Green, J (reprint author), Univ Wyoming, Soft Mat Lab, Dept Chem & Petr Engn, Laramie, WY 82071 USA. RI Hong, Kunlun/E-9787-2015 OI Hong, Kunlun/0000-0002-2852-5111 FU National Science Foundation at the University of Wyoming [CTS-0625338]; NIH [P20 RR0-16474]; National Institutes of Health, Institute for Research Resources [P20 RR15640]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy [CNMS2006-114] FX The authors gratefully acknowledge the practical help and valuable advice by Dr. W. Winoto. This work is funded by a National Science Foundation Grant CTS-0625338 at the University of Wyoming. J.G.'s stipend is funded by NIH Grant #P20 RR0-16474 from the INBRE Program of the National Center for Research Resources. The TEM facility is funded by the National Institutes of Health, Institute for Research Resources, and Grant P20 RR15640 to the Neuroscience Center of Biomedical Research Excellence. The polymer samples used in this work were synthesized at Oak Ridge National Laboratory's Center for Nanophase Materials Sciences, sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy, through User Project CNMS2006-114. NR 17 TC 0 Z9 0 U1 0 U2 6 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 19 PY 2011 VL 115 IS 19 BP 9465 EP 9470 DI 10.1021/jp201762e PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 761UV UT WOS:000290427400020 PM 21686070 ER PT J AU Proslier, T Klug, JA Elam, JW Claus, H Becker, NG Pellin, MJ AF Proslier, Thomas Klug, Jeffrey A. Elam, Jeffrey W. Claus, Helmut Becker, Nicholas G. Pellin, Michael J. TI Atomic Layer Deposition and Superconducting Properties of NbSi Films SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID THIN-FILMS; SILICIDE FORMATION; SURFACE-REACTIONS; NIOBIUM; SI2H6; WF6; HYDROGEN; NB3SI; HEAT AB Atomic layer deposition was used to synthesize niobium suicide (NbSi) films with a 1:1 stoichiometry, using NbF5 and Si2H6 as precursors. The growth mechanism at 200 degrees C was examined by in-situ quartz crystal microbalance (QCM) and quadrupole mass spectrometer (QMS). This study revealed a self-limiting reaction with a growth rate of 4.5 angstrom/cycle. NbSi was found to grow only on oxide-free films prepared using halogenated precursors. The electronic properties, growth rate, chemical composition, and structure of the films were studied over the deposition temperature range 150-400 degrees C. For all temperatures, the films are found to be stoichiometric NbSi (1:1) with no detectable fluorine impurities, amorphous with a density of 6.65 g/cm(3), and metallic with a resistivity rho = 150 mu Omega.cm at 300 K for films thicker than 35 nm. The growth rate was nearly constant for deposition temperatures between 150 and 275 degrees C but increases above 300 degrees C, suggesting the onset of non-self-limiting growth. The electronic properties of the films were measured down to 1.2 K and revealed a superconducting transition at T-c = 3.1 K. To our knowledge, a superconducting niobium silicide film with a 1:1 stoichiometry has never been grown before by any technique. C1 [Proslier, Thomas; Klug, Jeffrey A.; Elam, Jeffrey W.; Claus, Helmut; Becker, Nicholas G.; Pellin, Michael J.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Proslier, T (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM prolier@anl.gov RI Pellin, Michael/B-5897-2008; Klug, Jeffrey/A-3653-2013 OI Pellin, Michael/0000-0002-8149-9768; FU U.S. Department of Energy, Office of Science [DE-AC02-06CH11357]; American Recovery and Reinvestment Act (ARRA) through the US Department of Energy, Office of High Energy Physics Department of Science FX The work was supported by the U.S. Department of Energy, Office of Science, under Contract DE-AC02-06CH11357 and by the American Recovery and Reinvestment Act (ARRA) through the US Department of Energy, Office of High Energy Physics Department of Science. The electron microscopy was accomplished at the Electron Microscopy Center for Materials Research at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated under Contract DE-AC02-06CH11357. NR 34 TC 7 Z9 7 U1 1 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 19 PY 2011 VL 115 IS 19 BP 9477 EP 9485 DI 10.1021/jp201873b PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 761UV UT WOS:000290427400022 ER PT J AU Li, ZJ Zhang, ZR Kay, BD Dohnalek, Z AF Li, Zhenjun Zhang, Zhenrong Kay, Bruce D. Dohnalek, Zdenek TI Polymerization of Formaldehyde and Acetaldehyde on Ordered (WO3)(3) Films on Pt(111) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SELECTIVE CATALYTIC-REDUCTION; ENERGY-LOSS SPECTROSCOPY; NITRIC-OXIDE; GAS-PHASE; V2O5-WO3/TIO2 CATALYSTS; METATHESIS ACTIVITY; TUNGSTEN-OXIDE; TITANIUM-OXIDE; WO3 CATALYSTS; ADSORPTION AB Polymerization of formaldehyde, H2CO, and acetaldehyde, CH3CHO, was studied under ultrahigh vacuum conditions on a model catalyst consisting of an ultrathin WO3 film supported on Pt(111). The onset of polymerization is observed at very low temperatures of 70 and 80 K for H2CO and CH3CHO, respectively, as documented by the evolution of the infrared reflection-absorption spectra. The amount of polymer increases with increasing coverage and saturates at 5 and 8 monolayers (ML) for the H2CO and CH3CHO multilayer films, respectively. Upon heating, the polymers decompose around 250 and 190 K for H2CO and CH3CHO, respectively, as evidenced mass spectrometrically by the desorption of their monomers and oligomers into the gas phase. The heats of H2CO and CH3CHO sublimation and polymerization determined on the basis of our experiments are in good agreement with previously published values. C1 [Li, Zhenjun; Zhang, Zhenrong; Kay, Bruce D.; Dohnalek, Zdenek] Pacific NW Natl Lab, Chem & Mat Sci Div, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Dohnalek, Z (reprint author), Pacific NW Natl Lab, Chem & Mat Sci Div, Fundamental & Computat Sci Directorate, POB 999,Mail Stop K8-88, Richland, WA 99352 USA. EM Bruce.Kay@pnl.gov; Dohnalek@pnl.gov RI Li, Zhenjun/F-4714-2010; OI Zhang, Zhenrong/0000-0003-3969-2326 FU U.S. Department of Energy Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences; Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory (PNNL); U.S. DOE by Battelle Memorial Institute [DE-AC06-76RLO 1830] FX This work was supported by the U.S. Department of Energy Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences, and was performed at EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory (PNNL). PNNL is operated for the U.S. DOE by Battelle Memorial Institute under contract no. DE-AC06-76RLO 1830. Computational resources were provided at EMSL and the National Energy Research Scientific Computing Center at Lawrence Berkeley National Laboratory. NR 53 TC 13 Z9 14 U1 2 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 19 PY 2011 VL 115 IS 19 BP 9692 EP 9700 DI 10.1021/jp202169x PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 761UV UT WOS:000290427400048 ER PT J AU Aad, G Abbott, B Abdallah, J Abdelalim, AA Abdesselam, A Abdinov, O Abi, B Abolins, M Abramowicz, H Abreu, H Acerbi, E Acharya, BS Ackers, M Adams, DL Addy, TN Adelman, J Aderholz, M Adomeit, S Adragna, P Adye, T Aefsky, S Aguilar-Saavedra, JA Aharrouche, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akdogan, T Akesson, TPA Akimoto, G Akimov, AV Alam, MS Alam, MA Albrand, S Aleksa, M Aleksandrov, IN Aleppo, M Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Aliyev, M Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, J Alviggi, MG Amako, K Amaral, P Amelung, C Ammosov, VV Amorim, A Amoros, G Amram, N Anastopoulos, C Andeen, T 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Cataneo, F Catinaccio, A Catmore, JR Cattai, A Cattani, G Caughron, S Cavallari, A Cavalleri, P Cavalli, D Cavalli-Sforza, M Cavasinni, V Cazzato, A Ceradini, F Cerna, C Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cetin, SA Cevenini, F Chafaq, A Chakraborty, D Chan, K Chapleau, B Chapman, JD Chapman, JW Chareyre, E Charlton, DG Chavda, V Cheatham, S Chekanov, S Chekulaev, SV Chelkov, GA Chen, H Chen, L Chen, S Chen, T Chen, X Cheng, S Cheplakov, A Chepurnov, VF El Moursli, RC Chernyatin, V Cheu, E Cheung, SL Chevalier, L Chevallier, F Chiefari, G Chikovani, L Childers, JT Chilingarov, A Chiodini, G Chizhov, MV Choudalakis, G Chouridou, S Christidi, IA Christov, A Chromek-Burckhart, D Chu, ML Chudoba, J Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciobotaru, MD Ciocca, C Ciocio, A Cirilli, M Ciubancan, M Clark, A Clark, PJ Cleland, W Clemens, JC Clement, B Clement, C Clifft, RW Coadou, Y Cobal, M Coccaro, A Cochran, J Coe, P Cogan, JG Coggeshall, J Cogneras, E Cojocaru, CD 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Zhang, D. Zhang, H. Zhang, J. Zhang, X. Zhang, Z. Zhao, L. Zhao, T. Zhao, Z. Zhemchugov, A. Zheng, S. Zhong, J. Zhou, B. Zhou, N. Zhou, Y. Zhu, C. G. Zhu, H. Zhu, Y. Zhuang, X. Zhuravlov, V. Zieminska, D. Zilka, B. Zimmermann, R. Zimmermann, S. Zimmermann, S. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zmouchko, V. V. Zobernig, G. Zoccoli, A. Zolnierowski, Y. Zsenei, A. zur Nedden, M. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Charged-particle multiplicities in pp interactions measured with the ATLAS detector at the LHC SO NEW JOURNAL OF PHYSICS LA English DT Article ID TRANSVERSE-MOMENTUM SPECTRA; SQUARE-ROOT-S; CM ENERGIES; DISTRIBUTIONS; COLLISIONS; COLLIDER; TEV AB Measurements are presented from proton-proton collisions at centre-of-mass energies of root s = 0.9, 2.36 and 7 TeV recorded with the ATLAS detector at the LHC. Events were collected using a single-arm minimum-bias trigger. The charged-particle multiplicity, its dependence on transverse momentum and pseudorapidity and the relationship between the mean transverse momentum and charged-particle multiplicity are measured. Measurements in different regions of phase space are shown, providing diffraction-reduced measurements as well as more inclusive ones. The observed distributions are corrected to well-defined phase-space regions, using model-independent corrections. The results are compared to each other and to various Monte Carlo (MC) models, including a new AMBT1 pythia6 tune. In all the kinematic regions considered, the particle multiplicities are higher than predicted by the MC models. The central charged-particle multiplicity per event and unit of pseudorapidity, for tracks with p(T) > 100 MeV, is measured to be 3.483 +/- 0.009 (stat) +/- 0.106 (syst) at root s = 0.9 TeV and 5.630 +/- 0.003 (stat) +/- 0.169 (syst) at root s = 7 TeV. 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[Demirkoz, B.; Helsens, C.; Osuna, C.; Pacheco Pages, A.; Padilla Aranda, C.; Perez Codina, E.] Univ Autonoma Barcelona, Inst Fis Altes Energies, IFAE, ES-08193 Bellaterra, Barcelona, Spain. [Borjanovic, I.; Krstic, J.; Popovic, D. S.; Reljic, D.; Sijacki, Dj; Simic, Lj; Vranjes, N.; Milosavljevic, M. Vranjes] Univ Belgrade, Inst Phys, Belgrade 11001, Serbia. [Bozovic-Jelisavcic, I.; Mamuzic, J.; Mudrinic, M.] Vinca Inst Nucl Sci, Belgrade 11000, Serbia. [Kastanas, A.; Lipniacka, A.; Mohn, B.; Stugu, B.; Tonoyan, A.] Univ Bergen, Dept Phys & Technol, NO-5007 Bergen, Norway. [Alonso, J.; Arguin, J-F; Bach, A. M.; Galtieri, A. Barbaro; Beringer, J.; Biesiada, J.; Ciocio, A.; Einsweiler, K.; Gaponenko, A.; Gilchriese, M.; Haber, C.; Heinemann, B.; Hinchliffe, I.; Joseph, J.; Korn, A.; Leggett, C.; Lys, J.; Quarrie, D. R.; Ruwiedel, C.; Siegrist, J.; Skinnari, L. A.; Stavropoulos, G.; Tompkins, L.; Varouchas, D.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Phys, Berkeley, CA 94720 USA. [Aliev, M.; Giorgi, F. M.; Grancagnolo, S.; Herrberg, R.; Kind, O.; Kolanoski, H.; Kwee, R.; Lacker, H.; Leyton, M.; Lohse, T.; Mandrysch, R.; Garcia, Y. Rodriguez; Schulz, H.; Sidoti, A.; zur Nedden, M.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Battaglia, A.; Beck, H. P.; Borer, C.; Ereditato, A.; Martin, T. Fonseca; Gallo, V.; Haug, S.; Kabana, S.; Topfel, C.; Venturi, N.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, High Energy Phys Lab, CH-3012 Bern, Switzerland. [Bansil, H. S.; Booth, J. R. A.; Bracinik, J.; Bright-Thomas, P. G.; Charlton, D. G.; Collins, N. J.; Curtis, C. J.; Dowell, J. D.; Garvey, J.; Hadley, D. R.; Harrison, K.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Homer, R. J.; Lilley, J. N.; Mahout, G.; Martin, T. A.; Mclaughlan, T.; McMahon, T. J.; Newman, P. R.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Typaldos, D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham B15 2TT, W Midlands, England. [Akdogan, T.; Arik, E.; Arik, M.; Dogan, O. B.; Istin, S.; Rador, T.] Bogazici Univ, Fac Sci, Dept Phys, TR-80815 Bebek, Turkey. [Cetin, S. A.] Dogus Univ, Fac Arts & Sci, Dept Phys, TR-34722 Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.; Diblen, F.] Gaziantep Univ, Fac Engn, Dept Engn Phys, TR-27310 Sehitkamil, Gaziantep, Turkey. Istanbul Tech Univ, Fac Arts & Sci, Dept Phys, TR-34469 Istanbul, Turkey. [Antonelli, S.; Bellagamba, L.; Bertin, A.; Bindi, M.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Ciocca, C.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Giacobbe, B.; Giusti, P.; Massa, I.; Mengarelli, A.; Monzani, S.; Piccinini, M.; Polini, A.; Rinaldi, L.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Spighi, R.; Valentinetti, S.; Villa, M.; Vitale, A.; Zoccoli, A.] INFN Sez Bologna, IT-40127 Bologna, Italy. Univ Bologna, Dipartimento Fis, IT-40127 Bologna, Italy. [Ackers, M.; Alhroob, M.; Anders, C. F.; Arutinov, D.; Barbero, M.; Bartsch, D.; Brock, I.; Cammin, J.; Cristinziani, M.; Desch, K.; Dingfelder, J.; Fischer, P.; Fleischmann, S.; Gaycken, G.; Geich-Gimbel, Ch; Gonella, L.; Hillert, S.; Huegging, F.; Ince, T.; Janus, M.; Khoriauli, G.; Koevesarki, P.; Kokott, T.; Kostyukhin, V. V.; Kroseberg, J.; Krueger, H.; Kruth, A.; Lapoire, C.; Lehmacher, M.; Loddenkoetter, T.; Mathes, M.; Mazur, M.; Meuser, S.; Moeser, N.; Mueller, K.; Nanava, G.; Nattermann, T.; Nuncio-Quiroz, A-E; Hanninger, G. Nunes; Peric, I.; Poghosyan, T.; Psoroulas, S.; Radics, B.; Rottlaender, I.; Runolfsson, O.; Schmieden, K.; Schmitz, M.; Schumacher, J. W.; Stockmanns, T.; Therhaag, J.; Treis, J.; Tsung, J-W; Uchida, K.; Uhlenbrock, M.; Vlasov, N.; Vogel, A.; von Toerne, E.; Wermes, N.; Wienemann, P.; Zendler, C.; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Ahlen, S. P.; Black, K. M.; Butler, J. M.; Harrington, R. D.; Hazen, E.; Lewandowska, M.; Love, J.; Marin, A.; Nation, N. R.; Posch, C.; Shank, J. T.; Whitaker, S. P.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Aefsky, S.; Amelung, C.; Bensinger, J. R.; Blocker, C.; Kirsch, L. E.; Pomeroy, D.; Skvorodnev, N.; Wellenstein, H.] Brandeis Univ, Dept Phys, Waltham, MA 02454 USA. [Caloba, L. P.; Cerqueira, A. S.; Torres, R. Coura; Gesualdi Mello, A. Da Rocha; Da Silva, P. V. M.; do Vale, M. A. B.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Perantoni, M.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, BR-21945970 Rio De Janeiro, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-05508900 Sao Paulo, Brazil. [Adams, D. L.; Armstrong, S. R.; Assamagan, K.; Begel, M.; Bernius, C.; Chen, H.; Chernyatin, V.; Dhullipudi, R.; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Greenwood, Z. D.; Hackenburg, R.; Klimentov, A.; Lanni, F.; Lynn, D.; Ma, H.; Maeno, T.; Majewski, S.; Nevski, P.; Nikolopoulos, K.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Park, W.; Pleier, M-A; Poblaguev, A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Rajagopalan, S.; Redlinger, G.; Sawyer, L.; Snyder, S.; Sondericker, J.; Steinberg, P.; Stumer, I.; Takai, H.; Tamsett, M. 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P.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Archambault, J. P.; Cojocaru, C. D.; Gillberg, D.; Heelan, L.; Khakzad, M.; Liu, C.; McCarthy, T. G.; Oakham, F. G.; Randrianarivony, K.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Braem, A.; Catinaccio, A.; Cattai, A.; Cerri, A.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dudarev, A.; Foussat, A.; Gonidec, A.; Gorini, B.; Correia, A. M. Henriques; Hoecker, A.; Koblitz, B.; La Rosa, A.; Mapelli, A.; Martin, B.; Messina, A.; Morley, A. K.; Nairz, A. M.; Nicquevert, B.; Petersen, B. A.; Poppleton, A.; Salzburger, A.; Sfyrla, A.; Szeless, B.; Tricoli, A.; Zsenei, A.] CERN, CH-1211 Geneva, Switzerland. [Anderson, K. J.; Boveia, A.; Brubaker, E.; Canelli, F.; Choudalakis, G.; Costin, T.; Feng, E. J.; Fiascaris, M.; Gardner, R. W.; Gupta, A.; Jen-La Plante, I.; Kapliy, A.; Melachrinos, C.; Merritt, F. S.; Onyisi, P. U. E.; Oreglia, M. J.; Pilcher, J. E.; Shochet, M. J.; Tuggle, J. M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Diaz, M. A.; Panes, B.; Quinonez, F.; Romero Maltrana, D.; Urrejola, P.] Pontificia Univ Catolica Chile, Fac Fis, Dept Fis, Santiago 4860, Chile. [Brooks, W. K.; Kuleshov, S.; Oyarzun, A.; Pezoa, R.; Prokoshin, F.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Cheng, S.; Han, H.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Tong, G.; Xie, Y.; Xu, G.; Yang, Y.; Yuan, L.; Zheng, S.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Gong, C.; Han, L.; Jiang, Y.; Jin, G.; Li, S.; Liu, M.; Liu, Y.; Wu, Y.; Xu, C.; Zhang, D.; Zhao, Z.] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, CN Anhui, Peoples R China. [Chen, S.; Chen, T.; Ping, J.; Yu, J.] Nanjing Univ, Dept Phys, Nanjing 210093, CN Jiangsu, Peoples R China. [Feng, C.; Ge, P.; He, M.; Miao, J.; Wang, J.; Zhan, Z.; Zhang, X.; Zhu, C. G.] Shandong Univ, High Energy Phys Grp, Jinan 250100, CN Shandong, Peoples R China. [Busato, E.; Calvet, D.; Calvet, S.; Cinca, D.; Febbraro, R.; Ghodbane, N.; Gris, P. L. Y.; Guicheney, C.; Pallin, D.; Podlyski, F.; Santoni, C.; Says, L. P.; Vazeille, F.; Viret, S.] Univ Clermont Ferrand, Lab Phys Corpusculaire, Clermont Univ, FR-63177 Aubiere, France. [Andeen, T.; Angerami, A.; Brooijmans, G.; Copic, K.; Dodd, J.; Grau, N.; Gray, H. M.; Guo, J.; Hughes, E. W.; Leltchouk, M.; Mateos, D. Lopez; Marshall, Z.; Parsons, J. A.; Penson, A.; Perez, K.; Reale, V. Perez; Spano, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY 10533 USA. [Boelaert, N.; Dam, M.; Driouichi, C.; Facius, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Jez, P.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Lundquist, J.; Mackeprang, R.; Petersen, T. C.; Rensch, B.; Simonyan, M.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen 0, Denmark. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Mastroberardino, A.; Morello, G.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Collegato Cosenza, IT-87036 Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Mastroberardino, A.; Morello, G.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, IT-87036 Arcavacata Di Rende, Italy. [Dabrowski, W.; Dwuznik, M.; Idzik, M.; Jelen, K.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Rulikowska-Zarebska, E.; Toczek, B.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, FPACS, AGH UST, PL-30059 Krakow, Poland. [Banas, E.; Blocki, J.; Bruckman de Renstrom, P. A.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa; Malecki, P.; Olszewski, A.; Olszowska, J.; Richter-Was, E.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Daya, R. K.; Yagci, K. Dindar; Firan, A.; Goldin, D.; Hadavand, H. K.; Hoffman, J.; Ilchenko, Y.; Ishmukhametov, R.; Joffe, D.; Kama, S.; Kasmi, A.; Kehoe, R.; Liang, Z.; Lu, L.; Renkel, P.; Rios, R. R.; Stroynowski, R.; Ye, J.; Zarzhitsky, P.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Galyaev, E.; Izen, J. M.; Lou, X.; Reeves, K.] Univ Texas Dallas, Richardson, TX 75080 USA. [Bechtle, P.; Kuutmann, E. Bergeaas; Boehler, M.; Brandt, G.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Gosdzik, B.; Gregor, I. M.; Hiller, K. H.; Hristova, I.; Husemann, U.; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Mehlhase, S.; Mijovic, L.; Moenig, K.; Naumann, T.; Nozicka, M.; Cavalcanti, T. Perez; Petschull, D.; Placakyte, R.; Rubinskiy, I.; Stelzer, H. J.; Terwort, M.; Vankov, P.; Wildt, M. A.; Zhu, H.] DESY, D-22603 Hamburg, Germany. [Bunse, M.; Dobos, D.; Goessling, C.; Hirsch, F.; Klaiber-Lodewigs, J.; Klingenberg, R.; Krasel, O.; Mass, M.; Muenstermann, D.; Rajek, S.; Reisinger, I.; Walbersloh, J.; Weber, J.; Wunstorf, R.] TU Dortmund, DE-44221 Dortmund, Germany. [Goepfert, T.; Kar, D.; Kobel, M.; Leonhardt, K.; Ludwig, A.; Mader, W. F.; Prudent, X.; Schaarschmidt, J.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01069 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Fowler, A. J.; Ko, B. R.; Oh, S. H.; Wang, C.; Yamaoka, J.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; O'Brien, B. J.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, Edinburgh EH9 3JZ, Midlothian, Scotland. [Griesmayer, E.] Fachhsch Wiener Neustadt, AT-2700 Wiener Neustadt, Austria. [Annovi, A.; Antonelli, M.; Bilokon, H.; Cerutti, F.; Curatolo, M.; Esposito, B.; Ferrer, M. L.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Ventura, S.; Vilucchi, E.; Wen, M.] INFN Lab Nazl Frascati, IT-00044 Frascati, Italy. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Bell, P. J.; Bell, W. H.; Berglund, E.; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Efthymiopoulos, I.; Ferrere, D.; Gadomski, S.; Navarro, J. E. Garcia; Gaumer, O.; Gonzalez-Sevilla, S.; Goulette, M. P.; Hamilton, A.; Leger, A.; Lister, A.; Macina, D.; Latour, B. Martin dit; Mikulec, B.; Moneta, L.; Herrera, C. Mora; Morone, M-C; Nektarijevic, S.; Orellana, F.; Pasztor, G.; Pohl, M.; Robichaud-Veronneau, A.; Rosselet, L.; Urquijo, P.; Wu, X.] Univ Geneva, Sect Phys, CH-1211 Geneva 4, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Coccaro, A.; Cornelissen, T.; Cuneo, S.; Dameri, M.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Morettini, P.; Odino, G. A.; Olcese, M.; Osculati, B.; Parodi, F.; Rossi, L. P.; Schiavi, C.] INFN Sez Genova, IT-16146 Genoa, Italy. Univ Genoa, Dipartimento Fis, IT-16146 Genoa, Italy. [Chikovani, L.; Djobava, T.; Khubua, J.; Magradze, E.; Mchedlidze, G.; Mosidze, M.; Tskhadadze, E. G.] Georgian Acad Sci, Inst Phys, GE-380077 Tbilisi, Rep of Georgia. [Chikovani, L.; Djobava, T.; Khubua, J.; Magradze, E.; Mchedlidze, G.; Mosidze, M.; Tskhadadze, E. G.] Tbilisi State Univ, HEP Inst, GE-380086 Tbilisi, Rep of Georgia. [Astvatsatourov, A.; Dueren, M.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35392 Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Gemmell, A.; Kenyon, M.; McGlone, H.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Pickford, A.; Robson, A.; Saxon, D. H.; Shaw, C.; Smith, K. M.; St Denis, R. D.; Steele, G.; Stewart, G. A.; Thompson, A. S.; Wraight, K.; Wright, C.] Univ Glasgow, Dept Phys & Astron, Glasgow G12 8QQ, Lanark, Scotland. [Ay, C.; Blumenschein, U.; Brandt, O.; Erdmann, J.; Evangelakou, D.; Grosse-Knetter, J.; Guindon, S.; Haller, J.; Henrichs, A.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Mann, A.; Meyer, J.; Morel, J.; Park, S. J.; Prell, S.; Quadt, A.; Roe, A.; Shabalina, E.; Uhrmacher, M.; Weber, P.; Weingarten, J.] Univ Gottingen, Inst Phys 2, D-37077 Gottingen, Germany. [Albrand, S.; Andrieux, M-L; Clement, B.; Collot, J.; Crepe-Renaudin, S.; de Saintignon, P.; Delsart, P. A.; Donini, J.; Dzahini, D.; Hostachy, J-Y; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Martin, Ph; Polci, F.; Stark, J.; Sun, X.; Trocme, B.] CNRS IN2P3, LPSC, FR-38026 Grenoble, France. [Albrand, S.; Andrieux, M-L; Clement, B.; Collot, J.; Crepe-Renaudin, S.; de Saintignon, P.; Delsart, P. A.; Donini, J.; Dzahini, D.; Hostachy, J-Y; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Martin, Ph; Polci, F.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, FR-38026 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Brandenburg, G. W.; Franklin, M.; Hurst, P.; Huth, J.; Jeanty, L.; Kagan, M.; Kashif, L.; Outschoorn, V. Martinez; Mills, C.; Moed, S.; Morii, M.; Prasad, S.; Smith, B. C.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Childers, J. T.; Dietzscha, T. A.; Foehlisch, F.; Geweniger, C.; Hanke, P.; Henke, M.; Khomich, A.; Kluge, E-E; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H-C; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, D-69120 Heidelberg, Germany. [Radescu, V.; Schaetzel, S.; Schoening, A.] Inst Phys, D-69120 Heidelberg, Germany. [Kugel, A.; Maenner, R.; Schroer, N.] ZITI Ruprecht Karls Univ Heidelberg, DE-68131 Mannheim, Germany. [Ohsugi, T.] Hiroshima Univ, Fac Sci, Higashihiroshima, JP Hiroshima 7398526, Japan. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Saeki Ku, Hiroshima, JP Hiroshima 7315193, Japan. [Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Jain, V.; Luehring, F.; Marino, C. P.; Ogren, H.; Penwell, J.; Price, D.; Rust, D. R.; Whittington, D.; Yang, Y.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. 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A.; Mineev, M.; Nikolaev, K.; Olchevski, A. G.; Peshekhonov, V. D.; Romanov, V. M.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.] Joint Inst Nucl Res, RU-141980 JINR Dubna, Moscow Region, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Ishii, K.; Ishino, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Manabe, A.; Mitsui, S.; Morita, Y.; Murakami, K.; Nagano, K.; Nozaki, M.; Odaka, S.; Ohska, T. K.; Sasaki, O.; Sasaki, T.; Suzuki, Y.; Tanaka, S.; Terada, S.; Tojo, J.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Org, KEK, Tsukuba, Ibaraki 3050801, Japan. [Hayakawa, T.; Homma, Y.; Ichimiya, R.; Ishikawa, A.; Kawagoe, K.; King, M.; Kiyamura, H.; Kurashige, H.; Matsushita, T.; Miyazaki, K.; Nishiyama, T.; Ochi, A.; Okada, S.; Omachi, C.; Suita, K.; Takeda, H.; Tani, K.; Tokunaga, K.; Yamazaki, Y.] Kobe Univ, Grad Sch Sci, Nada Ku, JP Kobe 6578501, Japan. [Takashima, R.] Kyoto Univ, Fushimi Ku, Kyoto, JP Kyoto 6128522, Japan. [Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, FCE, Dept Fis, IFLP CONICET UNLP, RA-1900 La Plata, Argentina. [Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Brodbeck, T. J.; Catmore, J. R.; Cheatham, S.; Chilingarov, A.; Davidson, R.; De Mora, L.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Ratoff, P. N.; Sloan, T. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster LA1 4YB, England. [Bianco, M.; Brambilla, E.; Cataldi, G.; Cazzato, A.; Chiodini, G.; Coluccia, R.; Crupi, R.; Gorini, E.; Grancagnolo, F.; Guida, A.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] INFN Sez Lecce, IT-73100 Lecce, Italy. [Allport, P. P.; Austin, N.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Houlden, M. A.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Maxfield, S. J.; Mehta, A.; Migas, S.; Prichard, P. M.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wiglesworth, C.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Bianco, M.; Brambilla, E.; Cazzato, A.; Coluccia, R.; Crupi, R.; Gorini, E.; Guida, A.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Fis, IT-73100 Lecce, Italy. [Cindro, V.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, SI-1000 Ljubljana, Slovenia. [Cindro, V.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Dept Phys, SI-1000 Ljubljana, Slovenia. [Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Cooper, B. D.; Eisenhandler, E.; Ellis, K.; Landon, M. P. J.; Lloyd, S. L.; Morin, J.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Stevenson, K.; Castanheira, M. Teixeira Dias; Traynor, D.] Queen Mary Univ London, Dept Phys, London E1 4NS, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Boorman, G.; Cooper-Smith, N. J.; Cowan, G.; Edwards, C. A.; George, S.; Goncalo, R.; Hayden, D.; Kilvington, G.; McMahon, T. R.; Misiejuk, A.; Rose, M.; Strong, J. A.; Teixeira-Dias, P.] Univ London, Dept Phys, Egham TW20 0EX, Surrey, England. [Baker, S.; Boeser, S.; Butterworth, J. M.; Byatt, T.; Campanelli, M.; Christidi, I. A.; Davison, A. R.; Dean, S.; Drohan, J. G.; Jansen, E.; Jones, T. W.; Konstantinidis, N.; Monk, J.; Nash, M.; Nurse, E.; Ozcan, V. E.; Prabhu, R.; Richards, A.; Robinson, J. E. M.; Sherwood, P.; Simmons, B.; Taylor, C.; Waugh, B. M.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Beau, T.; Bordoni, S.; Calderini, G.; Camard, A.; Cavalleri, P.; Chareyre, E.; De Cecco, S.; Derue, F.; Imbault, D.; Krasny, M. W.; Lacour, D.; Laforge, B.; Le Dortz, O.; Lellouch, J.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph; Theveneaux-Pelzer, T.; Trincaz-Duvoid, S.; Trinh, T. N.; Vannucci, F.] Univ Paris 07, Lab Phys Nucl & Hautes Energies, Univ Paris 06, CNRS IN2P3, F-75252 Paris 05, France. [Akesson, T. P. A.; Alonso, A.; Groth-Jensen, J.; Hedberg, V.; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.] Lund Univ, Fysiska Inst, SE-22100 Lund, Sweden. [Barreiro, F.; Cantero, J.; Del Peso, J.; Glasman, C.; Labarga, L.; Lagouri, T.; March, L.; Nebot, E.; Rodier, S.; Terron, J.] Univ Autonoma Madrid, Fac Ciencias, Dept Fis Teor, ES-28049 Madrid, Spain. [Aharrouche, M.; Arnaez, O.; Bendel, M.; Blum, W.; Buescher, V.; Eckweiler, S.; Edmonds, K.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Ji, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Meyer, C.; Moreno, D.; Neusiedl, A.; Rieke, S.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Siragusa, G.; Tapprogge, S.; Anh, T. Vu] Johannes Gutenberg Univ Mainz, Inst Phys, DE-55099 Mainz, Germany. [Almond, J.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Foster, J. M.; Howarth, J.; Hughes-Jones, R. E.; Ibbotson, M.; Jones, G.; Keates, J. R.; Kelly, M.; Kolya, S. D.; Lane, J. L.; Loebinger, F. K.; Marshall, R.; Martyniuk, A. C.; Marx, M.; Masik, J.; Miyagawa, P. S.; Nasteva, I.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Plano, W. G.; Schwanenberger, C.; Snow, S. W.; Tevlin, C. M.; Watts, S.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester M13 9PL, Lancs, England. [Aoun, S.; Bee, C.; Benchouk, C.; Bernardet, K.; Bousson, N.; Cerna, C.; Clemens, J. C.; Coadou, Y.; Correard, S.; Delpierre, P.; Djama, F.; Etienne, F.; Feligioni, L.; Henry-Couannier, F.; Hoffmann, D.; Hubaut, F.; Kuna, M.; Le Guirriec, E.; Leveque, J.; Li, B.; Monnier, E.; Odier, J.; Petit, E.; Pralavorio, P.; Qian, Z.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, CNRS IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Thompson, E. N.; van Eldik, N.; Willocq, S.; Woudstra, M. J.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Chapleau, B.; Corriveau, F.; Dobbs, M.; Dufour, M-A; Guler, H.; Klemetti, M.; Potter, C. T.; Robertson, S. 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[Aderholz, M.; Barillari, T.; Beimforde, M.; Bethke, S.; Capriotti, D.; Cortiana, G.; Dannheim, D.; Dedes, G.; Dietl, H.; Dubbert, J.; Ehrich, T.; Flowerdew, M. J.; Giovannini, P.; Goettfert, T.; Groh, M.; Haefner, P.; Hauff, D.; Hott, T.; Jantsch, A.; Kaiser, S.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Lutz, G.; Macchiolo, A.; Manz, A.; Menke, S.; Mohrdieck-Moeck, S.; Moser, H. G.; Nisius, R.; Oberlack, H.; Pospelov, G. E.; Potrap, I. N.; Rauter, E.; Richter, R.; Salihagic, D.; Schacht, P.; Seuster, R.; Stonjek, S.; Valderanis, C.; von der Schmitt, H.; von Loeben, J.; Zhuravlov, V.] Werner Heisenberg Inst, Max Planck Inst Phys, D-80805 Munich, Germany. [Shimojima, M.; Tanaka, Y.] Nagasaki Inst Appl Sci, JP Nagasaki 8510193, Japan. [Hasegawa, S.; Itoh, Y.; Ohshima, T.; Okumura, Y.; Sugimoto, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Grad Sch Sci, Chikusa Ku, Nagoya, Aichi 4648602, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Cevenini, F.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Doria, A.; Giordano, R.; Iacobucci, G.; Izzo, V.; Merola, L.; Musto, E.; Patricelli, S.; Rossi, E.; Sekhniaidze, G.] INFN Sez Napoli, IT-80126 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Cevenini, F.; Chiefari, G.; della Volpe, D.; Giordano, R.; Merola, L.; Musto, E.; Patricelli, S.; Rossi, E.] Univ Naples Federico II, Dipartimento Sci Fis, IT-80126 Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Metcalfe, J.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Consonni, M.; De Groot, N.; Filthaut, F.; Klok, P. F.; Konig, A. C.; Koetsveld, F.; Magrath, C. A.; Ordonez, G.; Raas, M.; Timmermans, C. J. W. P.] Radboud Univ Nijmegen, NIKHEF, Dept Expt High Energy Phys, NL-6525 AJ Nijmegen, Netherlands. [Bentvelsen, S.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Buis, E. J.; Colijn, A. P.; Dankers, R.; Daum, C.; de Jong, P.; De Nooij, L.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Koutsman, A.; Lee, H.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Muijs, A.; Mussche, I.; Ottersbach, J. P.; Peters, O.; Reichold, A.; Rijpstra, M.; Ruckstuhl, N.; Salamanna, G.; Sandstroem, R.; Snuverink, J.; Ta, D.; Tsiakiris, M.; Turlay, E.; van der Graaf, H.; van der Kraaij, E.; van der Poel, E.; Van Eijk, B.; van Kesteren, Z.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.] Nikhef Natl Inst Subat Phys, NL-1098 XG Amsterdam, Netherlands. [Bentvelsen, S.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Buis, E. J.; Colijn, A. P.; Dankers, R.; Daum, C.; de Jong, P.; De Nooij, L.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Koutsman, A.; Lee, H.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Muijs, A.; Mussche, I.; Ottersbach, J. P.; Peters, O.; Reichold, A.; Rijpstra, M.; Ruckstuhl, N.; Salamanna, G.; Sandstroem, R.; Snuverink, J.; Ta, D.; Tsiakiris, M.; Turlay, E.; van der Graaf, H.; van der Kraaij, E.; van der Poel, E.; Van Eijk, B.; van Kesteren, Z.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.] Univ Amsterdam, NL-1098 XG Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; de Lima, J. G. Rocha; Suhr, C.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Bobrovnikov, V. B.; Bogdanchikov, A.; Kazanin, V. A.; Kolachev, G. M.; Korol, A.; Malyshev, V.; Maslennikov, A. L.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.; Zaytsev, A.] Budker Inst Nucl Phys BINP, RU Novosibirsk 630090, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; Djilkibaev, R.; Konoplich, R.; Krasznahorkay, A.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Shibata, A.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA. [Arms, K. E.; Fernando, W.; Fisher, M. J.; Gan, K. K.; Kagan, H.; Kass, R. D.; Moss, J.; Rahimi, A. M.; Strang, M.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 7008530, Japan. [Abbott, B.; Gutierrez, P.; Huang, G. S.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Kocnar, A.] Palacky Univ, Olomouc 77207, Czech Republic. [Brau, J. E.; Ptacek, E.; Reinsch, A.; Robinson, M.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abreu, H.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Bernat, P.; Blanchard, J-B; Bourdarios, C.; Breton, D.; Collard, C.; De La Taille, C.; De Regie, J. B. De Vivie; Diglio, S.; Dudziak, F.; Duflot, L.; Escalier, M.; Falou, A. C.; Fayard, L.; Fournier, D.; Grivaz, J-F; Heller, M.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lounis, A.; Makovec, N.; Matricon, P.; Nakahama, Y.; Niedercorn, F.; Perus, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Veillet, J. J.; Vukotic, I.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, CNRS, IN2P3, Orsay, France. [Hanagaki, K.; Hirose, M.; Meguro, T.; Nomachi, M.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka 5600043, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Czyczula, Z.; Gjelsten, B. K.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Pylypchenko, Y.; Read, A. L.; Rohne, O.; Samset, B. H.; Stapnes, S.; Strandlie, A.; Taga, A.] Univ Oslo, Dept Phys, NO-0316 Oslo 3, Norway. [Abdesselam, A.; Apolle, R.; Barr, A. J.; Beauchemin, P. H.; Boddy, C. R.; Brett, N. D.; Buchanan, J.; Buckingham, R. M.; Buira-Clark, D.; Coe, P.; Coniavitis, E.; Cooper-Sarkar, A. M.; Dennis, C.; Doglioni, C.; Farrington, S. M.; Ferrando, J.; Gallas, E. J.; Gilbert, L. M.; Gwenlan, C.; Hawes, B. M.; Holmes, A.; Horton, K.; Howell, D. F.; Huffman, T. B.; Issever, C.; Karagoz, M.; King, R. S. B.; Kirsch, G. P.; Kundu, N.; Larner, A.; Lau, W.; Lavorato, A.; Liang, Z.; Livermore, S. S. A.; Loken, J.; Mattravers, C.; Mermod, P.; Mitra, A.; Nickerson, R. B.; Pinder, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Wooden, G.] Univ Oxford, Dept Phys, Oxford OX1 3RH, England. [Bellomo, M.; Cambiaghi, M.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesi, V.] INFN Sez Pavia, IT-27100 Pavia, Italy. [Cambiaghi, M.; Conta, C.; Franchino, S.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.] Univ Pavia, Dipartimento Fis Nucl & Teor, IT-27100 Pavia, Italy. [Alison, J.; Degenhardt, J.; Donega, M.; Dressnandt, N.; Fratina, S.; Hance, M.; Hines, E.; Jackson, B.; Kroll, J.; Kunkle, J.; LeGeyt, B. C.; Lipeles, E.; Martin, F. F.; Olivito, D.; Ospanov, R.; Reece, R.; Stahlman, J.; Thomson, E.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, High Energy Phys Grp, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Nesterov, S. Y.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Zalite, Yo K.] Petersburg Nucl Phys Inst, RU-188300 Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Francavilla, P.; Giangiobbe, V.; Lupi, A.; Mazzoni, E.; Roda, C.; Sarri, F.; Zenonos, Z.] INFN Sez Pisa, IT-56127 Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Francavilla, P.; Giangiobbe, V.; Lupi, A.; Mazzoni, E.; Roda, C.; Sarri, F.; Zenonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, IT-56127 Pisa, Italy. [Boudreau, J.; Boulahouache, C.; Cleland, W.; Kittelmann, T.; Mueller, J.; Paolone, V.; Prieur, D.; Savinov, V.; Tsulaia, V.; Wendler, S.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Amorim, A.; Anjos, N.; Carvalho, J.; Conde Muino, P.; Do Valle Wemans, A.; Fernandes, B.; Fiolhais, M. C. N.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Magalhaes Martins, P. J.; Maio, A.; Maneira, J.; Morais, A.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Soares, M.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000149 Lisbon, Portugal. [Aguilar-Saavedra, J. A.; Castro, N. F.] Univ Granada, Dept Fis Teor & Cosmos, E-18071 Granada, Spain. [Aguilar-Saavedra, J. A.; Castro, N. F.] CAFPE, E-18071 Granada, Spain. [Chudoba, J.; Gallus, P.; Gunther, J.; Havranek, M.; Hruska, I.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Kvasnicka, O.; Lipinsky, L.; Lokajicek, M.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Panuskova, M.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, CZ-18221 Prague 8, Czech Republic. [Davidek, T.; Dolejsi, J.; Dolezal, Z.; Drasal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Inst Particle & Nucl Phys, CZ-18000 Prague 8, Czech Republic. [Augsten, K.; Holy, T.; Horazdovsky, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.] Czech Tech Univ, CZ-16635 Prague 6, Czech Republic. [Ammosov, V. V.; Borisov, A.; Bozhko, N. I.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Gapienko, V. A.; Golovnia, S. N.; Gorokhov, S. A.; Goryachev, V. N.; Gushchin, V. N.; Ivashin, A. V.; Kabachenko, V. V.; Karyukhin, A. N.; Kholodenko, A. G.; Kiver, A. M.; Kopikov, S. V.; Koreshev, V.; Korotkov, V. A.; Kozhin, A. S.; Lapin, V. V.; Larionov, A. V.; Levitski, M. S.; Minaenko, A. A.; Mitrofanov, G. Y.; Moisseev, A. M.; Myagkov, A. G.; Nikolaenko, V.; Pleskach, A. V.; Ryadovikov, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Sviridov, Yu M.; Vorobiev, A. P.; Vovenko, A. S.; Zaets, V. G.; Zaitsev, A. M.; Zenin, A. V.; Zenin, O.; Zmouchko, V. V.] State Res Ctr Inst High Energy Phys, Moscow 142281, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Botterill, D.; Burke, S.; Clifft, R. W.; Dallison, S. J.; Dewhurst, A.; Emeliyanov, D.; Fisher, S. M.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Greenfield, D.; Hart, J. C.; Haywood, S. J.; Kirk, J.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Strube, J.; Tyndel, M.; Weber, M.; Wickens, F. J.; Wielers, M.; Zajacova, Z.] Sci & Technol Facil Council, Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Benslama, K.; Ju, X.; Ming, Y.; Ortega, E. O.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Shiga 5258577, Japan. [Anulli, F.; Artoni, G.; Bagnaia, P.; Biglietti, M.; Bini, C.; Borroni, S.; Caloi, R.; Cavallari, A.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvoa, A.; Dionisi, C.; Falciano, S.; Gentile, S.; Giagu, S.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Maiani, C.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Tehrani, F. Safai; Camillocci, E. Solfaroli; Spila, F.; Valente, P.; Vari, R.; Veneziano, S.; Zanello, L.] INFN Sez Roma, IT-00185 Rome, Italy. [Artoni, G.; Bagnaia, P.; Biglietti, M.; Bini, C.; Borroni, S.; Caloi, R.; Cavallari, A.; Ciapetti, G.; D'Orazio, A.; Dionisi, C.; Gentile, S.; Giagu, S.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Maiani, C.; Tehrani, F. Safai; Camillocci, E. Solfaroli; Spila, F.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, IT-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Nardo, R.; Di Simone, A.; Liberti, B.; Marchese, F.; Paoloni, A.; Salamon, A.; Santonico, R.] INFN Sez Roma Tor Vergata, IT-00133 Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Nardo, R.; Di Simone, A.; Marchese, F.; Paoloni, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, IT-00133 Rome, Italy. [Bacci, C.; Baroncelli, A.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Spiriti, E.; Stanescu, C.; Tonazzo, A.] INFN Sez Roma Tre, IT-00146 Rome, Italy. [Bacci, C.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.; Tonazzo, A.] Univ Roma Tre, Dipartimento Fis, IT-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Goujdami, D.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies RUPHE, Fac Sci Ain Chock, MA Casablanca, Morocco. Ctr Natl Energie Sci Tech Nucl CNESTEN, Rabat 10001, Morocco. [Derkaoui, J. E.; Ouchrif, M.] Univ Mohamed Premier, LPTPM, Fac Sci, Oujda 60000, Morocco. [El Moursli, R. Cherkaoui; Ghazlane, H.] Univ Mohammed 5, Fac Sci, Rabat 10000, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Boonekamp, M.; Chevalier, L.; Chevallier, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Le Menedeu, E.; Legendre, M.; Lenzi, B.; Mansoulie, B.; Meyer, J-P; Morange, N.; Nicolaidou, R.; Ouraou, A.; Pomarede, D. M.; Resende, B.; Royon, C. R.; Schune, Ph; Schwindling, J.; Virchaux, M.] CEA, DSM IRFU, Ctr Etudes Saclay, FR-91191 Gif Sur Yvette, France. [Bangert, A.; Chouridou, S.; Damiani, D. S.; Dubbs, T.; Fowler, K.; Grillo, A. A.; Hare, G. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W; Schumm, B. A.; Seiden, A.; Taylor, G.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys SCIPP, Santa Cruz, CA 95064 USA. [Forbush, D. A.; Goussiou, A. G.; Griffiths, J.; Harris, O. M.; Kuykendall, W.; Lubatti, H. J.; Mockett, P.; Policicchio, A.; Rosati, S.; Rothberg, J.; Ventura, D.; Verducci, M.; Wang, J. C.; Watts, G.; Zhao, T.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Booth, C. N.; Booth, P.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Duxfield, R.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Lehto, M.; Mayne, A.; Mcfayden, J. A.; Nicolas, L.; Owen, S.; Paganis, E.; Sutton, M. R.; Tovey, D. R.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield S3 7RH, S Yorkshire, England. [Hasegawa, Y.; Ohshita, H.; Takeshita, T.] Shinshu Univ, Dept Phys, Fac Sci, Matsumoto, JP Nagano 3908621, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Sipica, V.; Stahl, T.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Komaragiri, J. R.; O'Neil, D. C.; Petteni, M.; Schouten, D.; Stelzer, B.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Gao, Y. S.; Grenier, P.; Haas, A.; Hansson, P.; Horn, C.; Jackson, P.; Kenney, C. J.; Kim, P. C.; Kocian, M.; Koi, T.; Lowe, A. J.; Miller, D. W.; Mount, R.; Nelson, S.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Wilson, M. G.; Wittgen, M.; Young, C.] Stanford Linear Accelerator Ctr, Accelerator Lab, Stanford, CA 94309 USA. [Batkova, L.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.; Zilka, B.] Comenius Univ, Fac Math Phys & Informat, SK-84248 Bratislava, Slovakia. [Antos, J.; Brunckob, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, SK-04353 Kosice, Slovakia. Univ Johannesburg, Dept Phys, ZA-2006 Johannesburg, South Africa. [Leney, K. J. C.; Vickey, T.] Univ Witwatersrand, Sch Phys, ZA-2050 Johannesburg, South Africa. [Asman, B.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Hidvegi, A.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Lesser, J.; Lundberg, J.; Milstead, D. A.; Moa, T.; Nordkvist, B.; Ohm, C. C.; Papadelis, A.; Ramstedt, M.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden. [Asman, B.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Lundberg, J.; Milstead, D. A.; Moa, T.; Nordkvist, B.; Ohm, C. C.; Ramstedt, M.; Sellden, B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Grahn, K-J; Lund-Jensen, B.] Royal Inst Technol KTH, Dept Phys, SE-10691 Stockholm, Sweden. [Ahmad, A.; Caputo, R.; Deluca, C.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Grimm, K.; Hobbs, J.; Jia, J.; Khodinov, A.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.; Yurkewicz, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [De Santo, A.; Potter, C. J.; Salvatore, F.] Univ Sussex, Dept Phys & Astron, Brighton BN1 9QH, E Sussex, England. [Lee, J. S. H.; Patel, N.; Saavedra, A. F.; Varvell, K. E.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, AU Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Meng, Z.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhong, J.; Zhou, Y.] Acad Sinica, Inst Phys, TW Taipei 11529, Taiwan. [Harpaz, S. Behar; Ben Ami, S.; Bressler, S.; Hershenhorn, A. D.; Kajomovitz, E.; Landsman, H.; Lifshitz, R.; Rozen, Y.; Tarem, S.; Tennenbaum-Katan, Y. D.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Technion, IL Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Brodet, E.; Etzion, E.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hod, N.; Kreisel, A.; Mahalalel, Y.; Munwes, Y.; Oren, Y.; Reinherz-Aronis, E.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.; Urkovsky, E.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 IL Tel Aviv, Israel. [Iliadis, D.; Kordas, K.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Fac Sci, Dept Phys, Div Nucl & Particle Phys, GR-54124 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Imori, M.; Isobe, T.; Kanaya, N.; Kaneda, M.; Kataoka, Y.; Kawamoto, T.; Kessoku, K.; Kobayashi, T.; Kubota, T.; Mashimo, T.; Masubuchi, T.; Matsumoto, H.; Matsunaga, H.; Nakamura, K.; Ninomiya, Y.; Nomoto, H.; Oda, S.; Okuyama, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamamura, T.; Yamazaki, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Bunkyo Ku, JP Tokyo 1130033, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Imori, M.; Isobe, T.; Kanaya, N.; Kaneda, M.; Kataoka, Y.; Kawamoto, T.; Kessoku, K.; Kobayashi, T.; Kubota, T.; Mashimo, T.; Masubuchi, T.; Matsumoto, H.; Matsunaga, H.; Nakamura, K.; Ninomiya, Y.; Nomoto, H.; Oda, S.; Okuyama, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamamura, T.; Yamazaki, T.] Dept Phys, Bunkyo Ku, JP Tokyo 1130033, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 1920397, Japan. [Jinnouchi, O.; Kanno, T.; Kuze, M.] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan. [Bailey, D. C.; Bain, T.; Beare, B.; Brelier, B.; Montero, S. Carron; Cheung, S. L.; Deviveiros, P. O.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Jankowski, E.; Joo, K. K.; Krieger, P.; Le Maner, C.; Martens, F. K.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Sandhu, P.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada. [Canepa, A.; Caron, B.; Chekulaev, S. V.; Fortin, D.; Losty, M. J.; Nugent, I. M.; Oram, C. J.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Taylor, W.] York Univ, Dept Phys & Astron, N York, ON M3J 1P3, Canada. [Hara, K.; Kim, S. H.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Inst Pure & Appl Sci, Tsukuba, JP Ibaraki 3058571, Japan. [Hamilton, S.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.] Tufts Univ, Ctr Sci & Technol, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Rodriguez, D.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Benedict, B. H.; Bold, T.; Ciobotaru, M. D.; Deng, J.; Dobson, M.; Eschrich, I. Gough; Grabowska-Bold, I.; Hawkins, D.; Lankford, A. J.; Okawa, H.; Porter, R.; Scannicchio, D. A.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Wheeler-Ellis, S. J.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Acharya, B. S.; Cobal, M.; De Lotto, B.; De Sanctis, U.; Del Papa, C.; Pinamonti, M.; Shaw, K.; Suruliz, K.] INFN Grp Collegato Udine, IT-33100 Udine, Italy. [Acharya, B. S.; Cobal, M.; Suruliz, K.] Abdus Salaam Int Ctr Theoret Phys, IT-34014 Trieste, Italy. [De Lotto, B.; De Sanctis, U.; Del Papa, C.; Pinamonti, M.; Shaw, K.] Univ Udine, Dipartimento Fis, IT-33100 Udine, Italy. [Benekos, N.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Khandanyan, H.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Belanger-Champagne, C.; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Hansen, C. J.] Uppsala Univ, Dept Phys & Astron, SE-75120 Uppsala, Sweden. [Amoros, G.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Ctr Mixto UVEG CSIC, Inst Fis Corpuscular IFIC, ES-46071 Valencia, Spain. [Amoros, G.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, Dept Fis Mol & Nucl, Dept Ing Elect, Bellaterra 08193, Spain. [Amoros, G.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Inst Microelect Barcelona IMB CNM CSIC, Bellaterra 08193, Spain. [Axen, D.; Gay, C.; Loh, C. W.; Mills, W. J.; Muir, A.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC V6T 1Z1, Canada. [Astbury, A.; Banerjee, Sw; Bansal, V.; Berghaus, F.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R; McPherson, R. A.; Plamondon, M.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC V8W 3P6, Canada. [Kimura, N.; Yorita, K.] Waseda Univ, WISE, Shinjuku Ku, Tokyo 1698555, Japan. [Alon, R.; Barak, L.; Duchovni, E.; Frank, T.; Gabizon, O.; Gross, E.; Klier, A.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Asfandiyarov, R.; Montoya, G. D. Carrillo; Hernandez, A. M. Castaneda; Castaneda-Miranda, E.; Chen, X.; Dos Anjos, A.; Fang, Y.; Fasching, D.; Ferguson, D.; Castillo, L. R. Flores; Gonzalez, S.; Gutzwiller, O.; Ji, H.; Cheong, A. Leung Fook; Li, H.; Ma, L. L.; Garcia, B. R. Mellado; Pan, Y. B.; Pataraia, S.; Morales, M. I. Pedraza; Peng, H.; Poveda, J.; Quayle, W. B.; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Zhu, Y.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Meyer, J.; Redelbach, A.; Stroehmer, R.; Trefzger, T.] Univ Wurzburg, Inst Phys, D-97074 Wurzburg, Germany. [Barisonzi, M.; Becks, K. H.; Boek, J.; Braun, H. M.; Dopke, J.; Drees, J.; Flick, T.; Gerlach, P.; Glitza, K. 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RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hermann Herder Str 3, D-79104 Freiburg Ibr, Germany. RI Di Nardo, Roberto/J-4993-2012; Della Pietra, Massimo/J-5008-2012; Bergeaas Kuutmann, Elin/A-5204-2013; Cascella, Michele/B-6156-2013; messina, andrea/C-2753-2013; de Groot, Nicolo/A-2675-2009; Amorim, Antonio/C-8460-2013; Orlov, Ilya/E-6611-2012; Annovi, Alberto/G-6028-2012; Brooks, William/C-8636-2013; Pina, Joao /C-4391-2012; Vanyashin, Aleksandr/H-7796-2013; Gladilin, Leonid/B-5226-2011; Kramarenko, Victor/E-1781-2012; Alexa, Calin/F-6345-2010; Moorhead, Gareth/B-6634-2009; Petrucci, Fabrizio/G-8348-2012; Wemans, Andre/A-6738-2012; Fabbri, Laura/H-3442-2012; Kurashige, Hisaya/H-4916-2012; Kuzhir, Polina/H-8653-2012; Delmastro, Marco/I-5599-2012; Veneziano, Stefano/J-1610-2012; spagnolo, stefania/A-6359-2012; Andreazza, Attilio/E-5642-2011; Perrino, Roberto/B-4633-2010; De Cecco, Sandro/B-1016-2012; branchini, paolo/A-4857-2011; Wolter, Marcin/A-7412-2012; McKee, Shawn/B-6435-2012; Rotaru, Marina/A-3097-2011; Nemecek, Stanislav/C-3487-2012; Buttar, Craig/D-3706-2011; Takai, Helio/C-3301-2012; 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Gavrilenko, Igor/M-8260-2015; Jones, Roger/H-5578-2011; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Booth, Christopher/B-5263-2016; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Smirnova, Oxana/A-4401-2013; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Samset, Bjorn H./B-9248-2012; Olshevskiy, Alexander/I-1580-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Morone, Maria Cristina/P-4407-2016; Goncalo, Ricardo/M-3153-2016; Canelli, Florencia/O-9693-2016; Battistoni, Giuseppe/B-5264-2012; Idzik, Marek/A-2487-2017; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Monzani, Simone/D-6328-2017; Fullana Torregrosa, Esteban/A-7305-2016; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; la rotonda, laura/B-4028-2016; OI Della Pietra, Massimo/0000-0003-4446-3368; Cascella, Michele/0000-0003-2091-2501; Orlov, Ilya/0000-0003-4073-0326; Annovi, Alberto/0000-0002-4649-4398; Brooks, William/0000-0001-6161-3570; Pina, Joao /0000-0001-8959-5044; Vanyashin, Aleksandr/0000-0002-0367-5666; Gladilin, Leonid/0000-0001-9422-8636; Moorhead, Gareth/0000-0002-9299-9549; Petrucci, Fabrizio/0000-0002-5278-2206; Wemans, Andre/0000-0002-9669-9500; Fabbri, Laura/0000-0002-4002-8353; Kuzhir, Polina/0000-0003-3689-0837; Delmastro, Marco/0000-0003-2992-3805; Veneziano, Stefano/0000-0002-2598-2659; spagnolo, stefania/0000-0001-7482-6348; Andreazza, Attilio/0000-0001-5161-5759; Perrino, Roberto/0000-0002-5764-7337; McKee, Shawn/0000-0002-4551-4502; Rotaru, Marina/0000-0003-3303-5683; Takai, Helio/0000-0001-9253-8307; Britton, David/0000-0001-9998-4342; Smirnov, Sergei/0000-0002-6778-073X; valente, paolo/0000-0002-5413-0068; Stoicea, Gabriel/0000-0002-7511-4614; Ferrando, James/0000-0002-1007-7816; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; La Rosa, Alessandro/0000-0001-6291-2142; Moraes, Arthur/0000-0002-5157-5686; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Castro, Nuno/0000-0001-8491-4376; Wolters, Helmut/0000-0002-9588-1773; Warburton, Andreas/0000-0002-2298-7315; De, Kaushik/0000-0002-5647-4489; O'Shea, Val/0000-0001-7183-1205; Lee, Jason/0000-0002-2153-1519; Villa, Mauro/0000-0002-9181-8048; Mikestikova, Marcela/0000-0003-1277-2596; Peleganchuk, Sergey/0000-0003-0907-7592; Santamarina Rios, Cibran/0000-0002-9810-1816; Bosman, Martine/0000-0002-7290-643X; Nasteva, Irina/0000-0001-7115-7214; Grinstein, Sebastian/0000-0002-6460-8694; Lei, Xiaowen/0000-0002-2564-8351; Ventura, Andrea/0000-0002-3368-3413; Villaplana Perez, Miguel/0000-0002-0048-4602; Livan, Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886; CARPENTIERI, CARMELA/0000-0002-2994-0317; Joergensen, Morten/0000-0002-6790-9361; Martins, Paulo/0000-0003-3753-3751; Mir, Lluisa-Maria/0000-0002-4276-715X; Riu, Imma/0000-0002-3742-4582; Ferrer, Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543; Grancagnolo, Sergio/0000-0001-8490-8304; Tikhomirov, Vladimir/0000-0002-9634-0581; Camarri, Paolo/0000-0002-5732-5645; Jones, Roger/0000-0002-6427-3513; Gorelov, Igor/0000-0001-5570-0133; Booth, Christopher/0000-0002-6051-2847; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Smirnova, Oxana/0000-0003-2517-531X; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Samset, Bjorn H./0000-0001-8013-1833; Olshevskiy, Alexander/0000-0002-8902-1793; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Morone, Maria Cristina/0000-0002-0200-0632; Goncalo, Ricardo/0000-0002-3826-3442; Canelli, Florencia/0000-0001-6361-2117; Battistoni, Giuseppe/0000-0003-3484-1724; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Troncon, Clara/0000-0002-7997-8524; Bailey, David C/0000-0002-7970-7839; Fullana Torregrosa, Esteban/0000-0003-3082-621X; Nielsen, Jason/0000-0002-9175-4419; Grancagnolo, Francesco/0000-0002-9367-3380; CACCIA, MASSIMO/0000-0002-9499-678X; Dell'Asta, Lidia/0000-0002-9601-4225; Cataldi, Gabriella/0000-0001-8066-7718; Sawyer, Lee/0000-0001-8295-0605; Korol, Aleksandr/0000-0001-8448-218X; Maio, Amelia/0000-0001-9099-0009; Fiolhais, Miguel/0000-0001-9035-0335; Karyukhin, Andrey/0000-0001-9087-4315; Anjos, Nuno/0000-0002-0018-0633; Begel, Michael/0000-0002-1634-4399; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Capua, Marcella/0000-0002-2443-6525; Vari, Riccardo/0000-0002-2814-1337; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Nisati, Aleandro/0000-0002-5080-2293; Gray, Heather/0000-0002-5293-4716; Doria, Alessandra/0000-0002-5381-2649; Veloso, Filipe/0000-0002-5956-4244; Gomes, Agostinho/0000-0002-5940-9893; Mincer, Allen/0000-0002-6307-1418; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Adye, Tim/0000-0003-0627-5059; Santos, Helena/0000-0003-1710-9291; Evans, Harold/0000-0003-2183-3127; Coccaro, Andrea/0000-0003-2368-4559; De Lotto, Barbara/0000-0003-3624-4480; Cristinziani, Markus/0000-0003-3893-9171; Chromek-Burckhart, Doris/0000-0003-4243-3288; Qian, Jianming/0000-0003-4813-8167; Haas, Andrew/0000-0002-4832-0455; Della Volpe, Domenico/0000-0001-8530-7447; Cranmer, Kyle/0000-0002-5769-7094; Romero-Maltrana, Diego/0000-0003-2550-5243; Vos, Marcel/0000-0001-8474-5357; Casadei, Diego/0000-0002-3343-3529; Mendes Saraiva, Joao Gentil/0000-0002-7006-0864; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Weber, Michele/0000-0002-2770-9031; Strube, Jan/0000-0001-7470-9301; Beck, Hans Peter/0000-0001-7212-1096; Salamanna, Giuseppe/0000-0002-0861-0052; Prokofiev, Kirill/0000-0002-2177-6401; Lacasta, Carlos/0000-0002-2623-6252; Price, Darren/0000-0003-2750-9977; Filthaut, Frank/0000-0003-3338-2247; abi, babak/0000-0001-7036-9645; Carvalho, Joao/0000-0002-3015-7821; Quinonez Granados, Fernando Andres/0000-0002-0153-6160; Paoloni, Alessandro/0000-0002-4141-7799; Belanger-Champagne, Camille/0000-0003-2368-2617; Pomarede, Daniel/0000-0003-2038-0488 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq; FAPESP, Brazil; NSERC; NRC; CFI, Canada; CERN; CONICYT, Chile; CAS; MOST; NSFC, China; COLCIENCIAS, Colombia; MSMT CR; MPO CR; VSC CR, Czech Republic; DNRF; DNSRC; Lundbeck Foundation, Denmark; ARTEMIS; European Union; IN2P3-CNRS; CEA-DSM/IRFU, France; GNAS, Georgia; BMBF; DFG; HGF; MPG; AvH Foundation, Germany; GSRT, Greece; ISF; MINERVA; GIF; DIP; Benoziyo Center, Israel; INFN, Italy; MEXT; JSPS, Japan; CNRST, Morocco; FOM; NWO, the Netherlands; RCN, Norway; MNiSW, Poland; GRICES; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS; MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC; Wallenberg Foundation, Sweden; SER; SNSF; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC; Royal Society and Leverhulme Trust, UK; DOE; NSF, USA FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; ARTEMIS, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNAS, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, the Netherlands; RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, UK; DOE and NSF, USA. The crucial computing support from all WLCG partners is acknowledged, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway and Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (the Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and the Tier-2 facilities worldwide. We thank Peter Skands for useful discussions concerning the AMBT1 tune. NR 51 TC 111 Z9 111 U1 6 U2 90 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD MAY 19 PY 2011 VL 13 AR 053033 DI 10.1088/1367-2630/13/5/053033 PG 68 WC Physics, Multidisciplinary SC Physics GA 782IQ UT WOS:000292002100003 ER PT J AU Hu, HF Zuo, JM Wen, JS Xu, ZJ Lin, ZW Li, Q Gu, GD Park, WK Greene, LH AF Hu, Hefei Zuo, Jian-Min Wen, Jinsheng Xu, Zhijun Lin, Zhiwei Li, Qiang Gu, Genda Park, Wan Kyu Greene, Laura H. TI Phase separation in the iron chalcogenide superconductor Fe1+yTexSe1-x SO NEW JOURNAL OF PHYSICS LA English DT Article ID FESE AB We present direct evidence for phase separation and chemical inhomogeneity in Fe1+yTexSe1-x single crystals from scanning transmission electron microscopy (STEM) and electron energy-loss spectroscopy (EELS) data. In STEM, images recorded using a high-angle annular dark field (HAADF) detector show characteristic nanometer-scale patterns of phase separation from the Z-dependent image contrast. The separation was observed both in non-superconducting samples with excess iron and in superconducting samples. Using EELS, we determined similar to 20% (or lower) fluctuation in Te concentration from the average local compositions by integrating the intensity of the Te-M-4,M-5 edge. The energy-loss near-edge structure (ELNES) of the Fe-L-2,L-3 edge changes with varying composition, especially the L-3/L-2 white-line intensity ratio, which is sensitive to the d-state occupancy of the Fe. The results suggest a miscibility gap in the Fe1+yTexSe1-x system and changes in the d-electron states at the nanometer scale from the separated phases. C1 [Zuo, Jian-Min] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA. [Hu, Hefei; Park, Wan Kyu; Greene, Laura H.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Hu, Hefei; Zuo, Jian-Min; Park, Wan Kyu; Greene, Laura H.] Univ Illinois, Frederick Seitz Mat Res Lab, Urbana, IL 61801 USA. [Wen, Jinsheng; Xu, Zhijun; Lin, Zhiwei; Li, Qiang; Gu, Genda] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Zuo, JM (reprint author), Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA. EM jianzuo@illinois.edu RI Wen, Jinsheng/F-4209-2010; xu, zhijun/A-3264-2013; Hu, Hefei/B-3482-2013 OI Wen, Jinsheng/0000-0001-5864-1466; xu, zhijun/0000-0001-7486-2015; Hu, Hefei/0000-0003-1216-2122 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC0298CH10886]; DOE [DE-FG02-07ER46453] FX This material is based upon work supported as part of the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under award number DE-AC0298CH10886. WKP is supported by the DOE (grant number DE-FG02-07ER46453). NR 24 TC 25 Z9 25 U1 3 U2 37 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD MAY 19 PY 2011 VL 13 AR 053031 DI 10.1088/1367-2630/13/5/053031 PG 11 WC Physics, Multidisciplinary SC Physics GA 782IQ UT WOS:000292002100001 ER PT J AU Zhao, S Ramakrishnan, G Su, D Rieger, R Koller, A Orlov, A AF Zhao, Shen Ramakrishnan, Girish Su, Dong Rieger, Robert Koller, Antonius Orlov, Alexander TI Novel photocatalytic applications of sub-nanometer gold particles for environmental liquid and gas phase reactions SO APPLIED CATALYSIS B-ENVIRONMENTAL LA English DT Article DE TiO(2); Photocatalysis; Gold nanoparticles; Phenol degradation; DRIFTS ID FERMI-LEVEL EQUILIBRATION; OPTICAL-PROPERTIES; METAL NANOCOMPOSITES; UNDECAGOLD CLUSTERS; CATALYTIC-ACTIVITY; PHOSPHINE-LIGANDS; TITANIUM-DIOXIDE; CO OXIDATION; NANOPARTICLES; SIZE AB Ultra small sub-1 nm gold nanoparticles were synthesized, characterized and deposited on TiO(2) Support. They exhibited a remarkable photocatalytic activity for both liquid and gas phase oxidation reactions, which have a significant potential for environmental applications. The NO(2) conversion on such catalysts was 6 times higher as compared to that of unmodified catalysts. This is the first ever application of such small clusters for environmental photocatalysis. The presence of sub-1 nm clusters was confirmed by TEM. MALDI-TOF MS and UV-vis spectroscopy. This work also included the novel use of modified DRIFT spectroscopy for photocatalytic testing as well improvement of known Au clusters synthesis procedures. (C) 2011 Elsevier B.V. All rights reserved. C1 [Zhao, Shen; Ramakrishnan, Girish; Orlov, Alexander] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. [Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Rieger, Robert; Koller, Antonius] SUNY Stony Brook, Univ Med Ctr, Dept Pathol, Stony Brook, NY 11794 USA. RP Orlov, A (reprint author), SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. EM aorlov@notes.cc.sunysb.edu RI Su, Dong/A-8233-2013 OI Su, Dong/0000-0002-1921-6683 FU U.S. Department of Energy, Office of Basic Energy Science [DE-AC02-98CH10886] FX The authors would like to acknowledge the assistance of Peichuan Shen in DRIFTS data analysis. Additionally, we appreciate the assistance of Bingyin Jiang in developing the Au synthesis procedures. The work of D. S. was supported by the U.S. Department of Energy, Office of Basic Energy Science, under contract number DE-AC02-98CH10886. NR 44 TC 15 Z9 15 U1 5 U2 31 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-3373 J9 APPL CATAL B-ENVIRON JI Appl. Catal. B-Environ. PD MAY 18 PY 2011 VL 104 IS 3-4 BP 239 EP 244 DI 10.1016/j.apcatb.2011.03.026 PG 6 WC Chemistry, Physical; Engineering, Environmental; Engineering, Chemical SC Chemistry; Engineering GA 771SX UT WOS:000291182100005 ER PT J AU Glaeser, RM Hall, RJ AF Glaeser, Robert M. Hall, Richard J. TI Reaching the Information Limit in Cryo-EM of Biological Macromolecules: Experimental Aspects SO BIOPHYSICAL JOURNAL LA English DT Article ID TRANSMISSION ELECTRON-MICROSCOPY; SINGLE-PARTICLE ANALYSIS; CRYOELECTRON MICROSCOPY; PHASE-CONTRAST; SENSITIVE SPECIMENS; REFINED STRUCTURE; RADIATION-DAMAGE; RESOLUTION; CRYOMICROSCOPY; RIBOSOME AB Although cryo-electron microscopy (cryo-EM) of biological macromolecules has made important advances in the past few years, the level of current technical performance is still well below what the physics of electron scattering would allow. It should be possible, for example, to use cryo-EM to solve protein structures at atomic resolution for particle sizes well below 80 kDa, but currently this has been achieved only for particles at least 10 times larger than that. In this review, we first examine some of the reasons for this large gap in performance. We then give an overview of work that is currently in progress to 1), improve the signal/noise ratio for area detectors; 2), improve the signal transfer between the scattered electrons and the corresponding images; and 3), reduce the extent to which beam-induced movement causes a steep fall-off of signal at high resolution. In each case, there is substantial reason to think that cryo-EM can indeed be made to approach the estimated physical limits. C1 [Glaeser, Robert M.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Life Sci, Berkeley, CA 94720 USA. [Hall, Richard J.] Univ Calif Berkeley, Inst QB3, Berkeley, CA 94720 USA. RP Glaeser, RM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Life Sci, Berkeley, CA 94720 USA. EM rmglaeser@lbl.gov FU ENIGMA; U.S. Department of Energy, Office of Science. Office of Biological and Environmental Research [DE-AC02-05CH11231]; Human Frontiers Science Program [RPG0039] FX This work was supported as part of ENIGMA, a Scientific Focus Area Program supported by the U.S. Department of Energy, Office of Science. Office of Biological and Environmental Research, Genomics:GTL Foundational Science through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U.S. Department of Energy, and by Grant RPG0039 from the Human Frontiers Science Program. NR 64 TC 25 Z9 25 U1 4 U2 25 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 J9 BIOPHYS J JI Biophys. J. PD MAY 18 PY 2011 VL 100 IS 10 BP 2331 EP 2337 DI 10.1016/j.bpj.2011.04.018 PG 7 WC Biophysics SC Biophysics GA 767BS UT WOS:000290830900003 PM 21575566 ER PT J AU Stanley, CB Perevozchikova, T Berthelier, V AF Stanley, Christopher B. Perevozchikova, Tatiana Berthelier, Valerie TI Structural Formation of Huntingtin Exon 1 Aggregates Probed by Small-Angle Neutron Scattering SO BIOPHYSICAL JOURNAL LA English DT Article ID MUTANT HUNTINGTIN; AMYLOID FIBRILS; IN-VITRO; POLYGLUTAMINE; DISEASE; NUCLEUS; TRANSITIONS; ASSEMBLIES; INCLUSIONS; FRAGMENTS AB In several neurodegenerative disorders, including Huntington's disease, aspects concerning the earliest of protein structures that form along the aggregation pathway have increasingly gained attention because these particular species are likely to be neurotoxic. We used time-resolved small-angle neutron scattering to probe in solution these transient structures formed by peptides having the N-terminal sequence context of mutant huntingtin exon 1. We obtained snapshots of the formed aggregates as the kinetic reaction ensued to yield quantitative information on their size and mass. At the early stage, small precursor species with an initial radius of gyration of 16.1 +/- 5.9 angstrom and average mass of a dimer to trimer were monitored. Structural growth was treated as two modes with a transition from three-dimensional early aggregate formation to two-dimensional fibril growth and association. Our small-angle neutron scattering results on the internal structure of the mature fibrils demonstrate loose packing with similar to 1 peptide per 4.75 angstrom beta-sheet repeat distance, which is shown to be quantitatively consistent with a beta-helix model. This research provides what we believe to be new insights into the structures forming along the pathway of huntingtin exon 1 aggregation and should assist in determining the role that precursors play in neuronal toxicity. C1 [Stanley, Christopher B.] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. [Perevozchikova, Tatiana; Berthelier, Valerie] Univ Tennessee, Hlth Sci Ctr, Grad Sch Med, Knoxville, TN USA. RP Stanley, CB (reprint author), Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. EM stanleycb@ornl.gov; vberthel@mc.utmck.edu OI Stanley, Christopher/0000-0002-4226-7710 FU U.S. Department of Energy [DE-AC05-00OR22725]; Oak Ridge National Laboratory; National Institutes of Health [1R21NS056325-01A1] FX This research at Oak Ridge National Laboratory's Center for Structural Molecular Biology was supported by the Office of Biological and Environmental Research, using facilities supported by the U.S. Department of Energy, managed by UT-Battelle, LLC under contract No. DE-AC05-00OR22725. This research was also supported by the Clifford Shull Fellowship Program at Oak Ridge National Laboratory (to C.B.S.) and by National Institutes of Health grant No. 1R21NS056325-01A1 (to V.B.). NR 37 TC 12 Z9 12 U1 1 U2 14 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 J9 BIOPHYS J JI Biophys. J. PD MAY 18 PY 2011 VL 100 IS 10 BP 2504 EP 2512 DI 10.1016/j.bpj.2011.04.022 PG 9 WC Biophysics SC Biophysics GA 767BS UT WOS:000290830900022 PM 21575585 ER PT J AU Kojima, T Antonio, MR Ozeki, T AF Kojima, Tatsuhiro Antonio, Mark R. Ozeki, Tomoji TI Solvent-Driven Association and Dissociation of the Hydrogen-Bonded Protonated Decavanadates SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID NUCLEAR MAGNETIC-RESONANCE; X-RAY SOLUTION; TETRAALKYLAMMONIUM SALTS; AQUEOUS-SOLUTION; ANIONS; ION; HYDROLYSIS; TRANSITION; POLYANIONS; SCATTERING AB Hydrogen-bond-assisted molecular aggregation of decavanadate anions, [HnV10O28]((6-n)-), in nonaqueous solutions was probed by systematic small-angle X-ray scattering and H-1 and V-51 NMR spectroscopic measurements in mixtures of acetone and 1,4-dioxane. Under acetone-rich conditions, the decavanadate anion prefers a self-associated hydrogen-bonded dimer of {[H3V10O28](2)}(6-), which dissociates into monomeric species as the proportion of 1,4-dioxane increases. The association/dissociation behaviors of the decavanadate anions were proven to be reversible and driven by the protophobic/protophilic nature of the solvent. C1 [Antonio, Mark R.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Kojima, Tatsuhiro; Ozeki, Tomoji] Tokyo Inst Technol, Dept Chem & Mat Sci, Meguro Ku, Tokyo 1528551, Japan. RP Antonio, MR (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM mantonio@anl.gov; tozeki@cms.titech.ac.jp FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences, and Geosciences [DE-AC02-06CH11357]; JSPS [22550056]; Ministry of Education, Culture, Sports, Science, and Technology of Japan FX We thank Dr. Soenke Seifert for assistance at the APS. Preliminary 1H NMR measurements were carried out by S. Nakamura. Thanks are also due to Dr. H. Takahashi for the measurement of a NOESY spectrum and Prof. T. Kusumi for helpful dicussions. This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences, and Geosciences, under Contract DE-AC02-06CH11357 (for the parts performed at Argonne National Laboratory) and by JSPS Grant-in-Aid for Scientific Research (C) 22550056 and the Chemistry Education New Program for Graduate Students from the Ministry of Education, Culture, Sports, Science, and Technology of Japan (for the parts performed at Tokyo Institute of Technology). NR 32 TC 25 Z9 25 U1 1 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 18 PY 2011 VL 133 IS 19 BP 7248 EP 7251 DI 10.1021/ja110781f PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 766KY UT WOS:000290782200004 PM 21524072 ER PT J AU Yuhas, BD Smeigh, AL Samuel, APS Shim, Y Bag, S Douvalis, AP Wasielewski, MR Kanatzidis, MG AF Yuhas, Benjamin D. Smeigh, Amanda L. Samuel, Amanda P. S. Shim, Yurina Bag, Santanu Douvalis, Alexios P. Wasielewski, Michael R. Kanatzidis, Mercouri G. TI Biomimetic Multifunctional Porous Chalcogels as Solar Fuel Catalysts SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID IRON-SULFUR CLUSTERS; MOLECULAR-STRUCTURE; HYDROGEN EVOLUTION; ACTIVE-SITES; ANALOGS; MOSSBAUER; PROTEINS; THIOLATE; SYSTEMS; CORE AB Biological systems that can capture and store solar energy are rich in a variety of chemical functionalities, incorporating light-harvesting components, electron-transfer cofactors, and redox-active catalysts into one supramolecule. Any artificial mimic of such systems designed for solar fuels production will require the integration of complex subunits into a larger architecture. We present porous chalcogenide frameworks that can contain both immobilized redox-active Fe4S4 clusters and light-harvesting photoredox dye molecules in close proximity. These multifunctional gels are shown to electrocatalytically reduce protons and carbon disulfide. In addition, incorporation of a photoredox agent into the chalcogels is shown to photochemically produce hydrogen. The gels have a high degree of synthetic flexibility, which should allow for a wide range of light-driven processes relevant to the production of solar fuels. C1 [Yuhas, Benjamin D.; Smeigh, Amanda L.; Samuel, Amanda P. S.; Shim, Yurina; Bag, Santanu; Wasielewski, Michael R.; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Yuhas, Benjamin D.; Smeigh, Amanda L.; Samuel, Amanda P. S.; Shim, Yurina; Bag, Santanu; Wasielewski, Michael R.; Kanatzidis, Mercouri G.] Northwestern Univ, Argonne NW Solar Energy Res ANSER Ctr, Evanston, IL 60208 USA. [Douvalis, Alexios P.] Univ Ioannina, Dept Phys, GR-45110 Ioannina, Greece. [Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Kanatzidis, MG (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM m-kanatzidis@northwestern.edu RI Smeigh, Amanda/C-5605-2014 OI Smeigh, Amanda/0000-0002-8071-071X FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001059] FX We thank Prof. Joseph Hupp for use of the potentiostat. Electron microscopy and elemental analysis were performed at the Electron Probe Instrumentation Center at Northwestern University. This work was supported as part of the ANSER Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award No. DE-SC0001059. NR 31 TC 41 Z9 41 U1 6 U2 77 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 18 PY 2011 VL 133 IS 19 BP 7252 EP 7255 DI 10.1021/ja111275t PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 766KY UT WOS:000290782200005 PM 21410264 ER PT J AU Frame, FA Townsend, TK Chamousis, RL Sabio, EM Dittrich, T Browning, ND Osterloh, FE AF Frame, F. Andrew Townsend, Troy K. Chamousis, Rachel L. Sabio, Erwin M. Dittrich, Th Browning, Nigel D. Osterloh, Frank E. TI Photocatalytic Water Oxidation with Nonsensitized IrO2 Nanocrystals under Visible and UV Light SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CATALYSTS; OXYGEN; IRRADIATION; REDUCTION; EVOLUTION; COLLOIDS; FILM AB Rutile IrO2 is known as being among the best electrocatalysts for water oxidation. Here we report on the unexpected photocatalytic water oxidation activity of 1.98 nm +/- 0.11 nm succinic acid-stabilized IrO2 nanocrystals. From aqueous persulfate and silver nitrate solution the nonsensitized particles evolve oxygen with initial rates up to 0.96 mu mol min(-1) and with a quantum efficiency of at least 0.19% (measured at 530 nm). The catalytic process is driven by visible excitations from the Ir-d(t(2g)) to the Ir-d(e(g)) band (1.5-2.75 eV) and by ultraviolet excitations from the O-p band to the Ir-d(e(g)) (>3.0 eV) band. The formation of the photogenerated charge carriers can be directly observed with surface photovoltage spectroscopy. The results shed new light on the role of IrO2 in dye- and semiconductor-sensitized water splitting systems. C1 [Frame, F. Andrew; Townsend, Troy K.; Chamousis, Rachel L.; Sabio, Erwin M.; Osterloh, Frank E.] Univ Calif Davis, Dept Chem, Davis, CA 95616 USA. [Dittrich, Th] Helmholtz Zentrum Berlin Mat & Energie, D-14109 Berlin, Germany. [Browning, Nigel D.] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Osterloh, FE (reprint author), Univ Calif Davis, Dept Chem, 1 Shields Ave, Davis, CA 95616 USA. EM fosterloh@ucdavis.edu RI Dom, Rekha/B-7113-2012; OI Browning, Nigel/0000-0003-0491-251X; Osterloh, Frank /0000-0002-9288-3407 FU National Science Foundation [0829142]; U.S. Department of Energy [FG02-03ER46057]; DAAD (German Academic Exchange Service) FX We thank Stephanie R Dungan (UC Davis) for use of their DLS instrument and the National Science Foundation (Grant 0829142) and the U.S. Department of Energy (Grant FG02-03ER46057) for financial support of this work. FEO thanks the DAAD (German Academic Exchange Service) for a Faculty Research Visit Grant. NR 28 TC 100 Z9 101 U1 13 U2 123 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 18 PY 2011 VL 133 IS 19 BP 7264 EP 7267 DI 10.1021/ja200144w PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 766KY UT WOS:000290782200008 PM 21524069 ER PT J AU Wang, ZJ Brown, CJ Bergman, RG Raymond, KN Toste, FD AF Wang, Z. Jane Brown, Casey J. Bergman, Robert G. Raymond, Kenneth N. Toste, F. Dean TI Hydroalkoxylation Catalyzed by a Gold(I) Complex Encapsulated in a Supramolecular Host SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID AZA-COPE REARRANGEMENT; INTERMOLECULAR HYDROALKOXYLATION; DIELS-ALDER; ALLENES; HYDROAMINATION; ISOMERIZATION; ALKENES AB Gold(I)-phosphine complexes are readily encapsulated by a tetrahedral supramolecular host (Ga(4)L(6)). We have investigated the catalytic activity of the resulting complexes for the intramolecular hydroalkoxylation of allenes. The catalytic activity of Me(3)PAuBr was increased 8-fold by encapsulation, as determined by initial rate kinetics, and we observed up to 67 catalytic turnovers by Me(3)PAu(+) encapsulated in Ga(4)L(6). C1 [Bergman, Robert G.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Chem Sci, Berkeley, CA 94720 USA. Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Bergman, RG (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM rbergman@berkeley.edu; raymond@socrates.berkeley.edu; fdtoste@berkeley.edu OI Toste, F. Dean/0000-0001-8018-2198 FU Office of Science, Office of Basic Energy Sciences; Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231] FX Research leading to this project was partially supported by the Director, Office of Science, Office of Basic Energy Sciences, and the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL (DE-AC02-05CH11231). We thank Dr. Anthony Iavarone at QB3/Chemistry Mass Spectrometry at UC Berkeley for help with mass spectrometry. Z.J.W. thanks the Hertz Foundation for a graduate fellowship. NR 35 TC 104 Z9 104 U1 4 U2 60 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 18 PY 2011 VL 133 IS 19 BP 7358 EP 7360 DI 10.1021/ja202055v PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 766KY UT WOS:000290782200032 PM 21517023 ER PT J AU Lybarger, WE Berengut, JC Chiaverini, J AF Lybarger, Warren E., Jr. Berengut, Julian C. Chiaverini, John TI Precision measurement of the 5 S-2(1/2)-4 D-2(5/2) quadrupole transition isotope shift between Sr-88(+) and Sr-86(+) SO PHYSICAL REVIEW A LA English DT Article ID CHARGE RADII; CLOCK TRANSITION; FREQUENCY; STRONTIUM; ION; SPECTROSCOPY AB We present a high-precision measurement of the isotope shift of the narrow quadrupole-allowed 5 S-2(1/2) -4 D-2(5/2) transition in Sr-86(+) relative to the most abundant isotope Sr-88(+). This was accomplished using high-resolution laser spectroscopy of individual trapped ions, and the measured shift is Delta nu(88,86)(meas) = 570.281( 4) MHz. We also tested a recently developed and successful method for ab initio calculation of isotope shifts in alkali-metal-like atomic systems against this measurement, and our initial result of Delta nu(88,86)(calc) = 457( 28) MHz is also presented. While the measurement and the calculation are in broad agreement, there is a clear discrepancy between them, and we believe that the specific mass shift was underestimated in our calculation. Our measurement provides a stringent test for further refinements of theoretical isotope shift calculation methods for atomic systems with a single valence electron. C1 [Lybarger, Warren E., Jr.; Chiaverini, John] Los Alamos Natl Lab, Appl Modern Phys Grp, Los Alamos, NM 87545 USA. [Lybarger, Warren E., Jr.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Berengut, Julian C.] Univ New S Wales, Sch Phys, Sydney, NSW 2052, Australia. RP Lybarger, WE (reprint author), Los Alamos Natl Lab, Appl Modern Phys Grp, MS D434, Los Alamos, NM 87545 USA. EM weljr@lanl.gov; jcb@phys.unsw.edu.au; john.chiaverini@ll.mit.edu RI Berengut, Julian/A-1764-2010 FU DOE FX We gratefully acknowledge Dana Berkeland's efforts in building the ion trap and the interrogation laser used in these determinations and Bob Scarlett for help in improving the long- term stability of that laser. We thank Malcolm Boshier for helpful comments during the manuscript preparation and Xinxin Zhao for the use of the electro-optic modulator for the measurement of the free spectral range of the interrogation laser reference cavity. This work was supported by DOE through the LANL Laboratory Directed Research and Development Program. NR 35 TC 4 Z9 4 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 J9 PHYS REV A JI Phys. Rev. A PD MAY 18 PY 2011 VL 83 IS 5 AR 052509 DI 10.1103/PhysRevA.83.052509 PG 7 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 765LH UT WOS:000290707000006 ER PT J AU Mauro, NA Wessels, V Bendert, JC Klein, S Gangopadhyay, AK Kramer, MJ Hao, SG Rustan, GE Kreyssig, A Goldman, AI Kelton, KF AF Mauro, N. A. Wessels, V. Bendert, J. C. Klein, S. Gangopadhyay, A. K. Kramer, M. J. Hao, S. G. Rustan, G. E. Kreyssig, A. Goldman, A. I. Kelton, K. F. TI Short- and medium-range order in Zr80Pt20 liquids SO PHYSICAL REVIEW B LA English DT Article ID QUASI-CRYSTALLINE PHASE; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; MOLECULAR-DYNAMICS; METALLIC-GLASS; ELECTROSTATIC LEVITATOR; BINARY-ALLOYS; ZR-PD; NI; CU AB The atomic structures in equilibrium and supercooled liquids of Zr80Pt20 were determined as a function of temperature by in situ high-energy synchrotron diffraction studies of the levitated liquids (containerless processing) using the beamline electrostatic levitation (BESL) technique. The presence of a pronounced pre-peak at q similar to 1.7 angstrom(-1) in the static structure factor indicates medium-range order (MRO) in the liquid. The position and intensity of the pre-peak remain constant with cooling, indicating that the MRO is already present in the liquid above its melting temperature. An analysis of the liquid atomic structures obtained using the Reverse Monte Carlo method utilizing both the structure factor S(q) from x-ray diffraction experiments and the partial pair-correlation functions from ab initio molecular dynamics simulations show that the pre-peak arises from a Pt-Pt correlation that can be identified with icosahedral short-range order around the Pt atoms. The local atomic ordering is dominated by icosahedral-like structures, raising the nucleation barrier between the liquid and these phases, thus assisting glass formation. C1 [Mauro, N. A.; Bendert, J. C.; Gangopadhyay, A. K.; Kelton, K. F.] Washington Univ, Dept Phys, Ctr Mat Innovat, St Louis, MO 63130 USA. [Wessels, V.] Swiss Fed Inst Technol, Dept Mat, Zurich, Switzerland. [Klein, S.] Deutsch Zentrum Luft & Raumfahrt DLR, Inst Mat Phys Weltraum, DE-51170 Cologne, Germany. [Klein, S.] Ruhr Univ Bochum, Inst Festkorperphys, DE-44780 Bochum, Germany. [Kramer, M. J.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Kramer, M. J.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Hao, S. G.; Rustan, G. E.; Kreyssig, A.; Goldman, A. I.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Mauro, NA (reprint author), Washington Univ, Dept Phys, Ctr Mat Innovat, St Louis, MO 63130 USA. FU National Science Foundation [DMR-06-06065, DMR-08-56199, DMR-08157157]; NASA [NNX07AK27G, NNX09AJ19H]; US Department of Energy (DOE), Basic Energy Sciences, Office of Science [DE-AC02-06CH11357] FX We acknowledge the valuable assistance of D. Robinson, A. Logan, A. Lyons, J. Mai, and C. Tackes. The research was partially supported by the National Science Foundation under Grants No. DMR-06-06065, No. DMR-08-56199, and No. DMR-08157157, and NASA under Grants No. NNX07AK27G and No. NNX09AJ19H. The synchrotron measurements were made on the MUCAT beamline at the Advanced Photon Source. Use of the Advanced Photon Source is supported by the US Department of Energy (DOE), Basic Energy Sciences, Office of Science, under Contract No. DE-AC02-06CH11357. NR 55 TC 32 Z9 32 U1 3 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 18 PY 2011 VL 83 IS 18 AR 184109 DI 10.1103/PhysRevB.83.184109 PG 8 WC Physics, Condensed Matter SC Physics GA 765MH UT WOS:000290710500003 ER PT J AU Phatak, C Petford-Long, AK Heinonen, O Tanase, M De Graef, M AF Phatak, C. Petford-Long, A. K. Heinonen, O. Tanase, M. De Graef, M. TI Nanoscale structure of the magnetic induction at monopole defects in artificial spin-ice lattices SO PHYSICAL REVIEW B LA English DT Article ID PHASE AB Artificially frustrated spin-ice systems are of considerable interest since they simulate the spin frustration and concomitant rich behavior exhibited by atoms on a crystal lattice in naturally occurring spin-ice systems such as pyrochlores. As a result of the magnetic frustration, these systems can exhibit "magnetic monopole" type defects, which are an example of an exotic emergent quasiparticle. The local magnetization structure of such monopole defects determines their stability and thus is critical to understanding their behavior. In this paper, we report on the direct observation at room temperature of the nanoscale magnetic structure of individual magnetic monopoles in an artificially frustrated two-dimensional square spin-ice lattice, using high-resolution aberration-corrected Lorentz transmission electron microscopy. By combining the high-resolution microscopy with micromagnetic simulation, we demonstrate how nucleation of defect strings, reminiscent of Dirac strings, connecting monopole defects controls the demagnetization process in these spin-ice lattices. C1 [Phatak, C.; Petford-Long, A. K.; Heinonen, O.; Tanase, M.] Argonne Natl Lab, Argonne, IL 60439 USA. [Petford-Long, A. K.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Heinonen, O.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [De Graef, M.] Carnegie Mellon Univ, Dept Mat Sci & Engn, Pittsburgh, PA 15213 USA. RP Phatak, C (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM cd@anl.gov RI Phatak, Charudatta/A-1874-2010; DeGraef, Marc/G-5827-2010; Petford-Long, Amanda/P-6026-2014; OI DeGraef, Marc/0000-0002-4721-6226; Petford-Long, Amanda/0000-0002-3154-8090; Heinonen, Olle/0000-0002-3618-6092 FU UChicago Argonne, LLC [DE-AC02-06CH11357]; MS&E Division of the U.S. DOE; DOE's Office of Basic Energy Sciences [DE-FG02-01ER45893] FX This work was carried out at Argonne National Laboratory, a U.S. DOE Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. The funding for the TEM was provided by the MS&E Division of the U.S. DOE. We also acknowledge use of the Center for Nanoscale Materials at Argonne National Laboratory. M. D. G. acknowledges the DOE's Office of Basic Energy Sciences for partial financial support (Contract No. DE-FG02-01ER45893). NR 21 TC 54 Z9 54 U1 3 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 18 PY 2011 VL 83 IS 17 AR 174431 DI 10.1103/PhysRevB.83.174431 PG 5 WC Physics, Condensed Matter SC Physics GA 765LS UT WOS:000290708400005 ER PT J AU Zaliznyak, IA Savici, AT Garlea, VO Hu, RW Petrovic, C AF Zaliznyak, I. A. Savici, A. T. Garlea, V. O. Hu, Rongwei Petrovic, C. TI Absence of localized-spin magnetism in the narrow-gap semiconductor FeSb2 SO PHYSICAL REVIEW B LA English DT Article ID INELASTIC-NEUTRON-SCATTERING; RESOLUTION FUNCTION; CRYSTAL-STRUCTURE; TRANSITION; MARCASITE; SUPERCONDUCTIVITY; MNSB AB We report on the inelastic neutron scattering measurements aimed at investigating the origin of temperature-induced paramagnetism in narrow-gap semiconductor FeSb2. We find that inelastic response for energies up to 60 meV and at temperatures approximate to 4.2, approximate to 300, and approximate to 550 K is essentially consistent with the scattering by lattice phonon excitations. We observe no evidence for a well-defined magnetic peak corresponding to the excitation from the nonmagnetic S = 0 singlet ground state to a state of magnetic multiplet in the localized-spin picture. Our data establish the quantitative limit of S-eff(2) less than or similar to 0.25 on the fluctuating local spin. However, a broad magnetic scattering continuum in the 15 to 35 meV energy range is not ruled out by our data. Our findings make description in terms of the localized Fe spins unlikely and suggest that paramagnetic susceptibility of itinerant electrons is at the origin of the temperature-induced magnetism in FeSb2. C1 [Zaliznyak, I. A.; Hu, Rongwei; Petrovic, C.] Brookhaven Natl Lab, CMPMSD, Upton, NY 11973 USA. [Savici, A. T.] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Savici, A. T.; Garlea, V. O.] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. RP Zaliznyak, IA (reprint author), Brookhaven Natl Lab, CMPMSD, Upton, NY 11973 USA. EM zaliznyak@bnl.gov RI Hu, Rongwei/E-7128-2012; Savici, Andrei/F-2790-2013; Zaliznyak, Igor/E-8532-2014; Petrovic, Cedomir/A-8789-2009; Garlea, Vasile/A-4994-2016 OI Savici, Andrei/0000-0001-5127-8967; Zaliznyak, Igor/0000-0002-9886-3255; Petrovic, Cedomir/0000-0001-6063-1881; Garlea, Vasile/0000-0002-5322-7271 FU Materials Sciences and Engineering Division, US Department of Energy [DE-AC02-98CH10886]; National Science Foundation [DMR-0603126]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; US DOE [DE-AC05-00OR22725] FX This work was performed under the Contract No. DE-AC02-98CH10886, Materials Sciences and Engineering Division, US Department of Energy. A.T.S. was funded by National Science Foundation through DMR-0603126. The Research at Oak Ridge National Laboratory's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. ORNL is operated by UT-Battelle, LLC for the US DOE under Contract No. DE-AC05-00OR22725. We thank M. Lumsden, M. Stone, J. Tranquada, and A. Frenkel for discussions and B. Winn for assistance at HFIR. NR 44 TC 8 Z9 8 U1 1 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 18 PY 2011 VL 83 IS 18 AR 184414 DI 10.1103/PhysRevB.83.184414 PG 9 WC Physics, Condensed Matter SC Physics GA 765MH UT WOS:000290710500006 ER PT J AU Oganessian, YT Abdullin, FS Bailey, PD Benker, DE Bennett, ME Dmitriev, SN Ezold, JG Hamilton, JH Henderson, RA Itkis, MG Lobanov, YV Mezentsev, AN Moody, KJ Nelson, SL Polyakov, AN Porter, CE Ramayya, AV Riley, FD Roberto, JB Ryabinin, MA Rykaczewski, KP Sagaidak, RN Shaughnessy, DA Shirokovsky, IV Stoyer, MA Subbotin, VG Sudowe, R Sukhov, AM Taylor, R Tsyganov, YS Utyonkov, VK Voinov, AA Vostokin, GK Wilk, PA AF Oganessian, Yu. Ts. Abdullin, F. Sh. Bailey, P. D. Benker, D. E. Bennett, M. E. Dmitriev, S. N. Ezold, J. G. Hamilton, J. H. Henderson, R. A. Itkis, M. G. Lobanov, Yu. V. Mezentsev, A. N. Moody, K. J. Nelson, S. L. Polyakov, A. N. Porter, C. E. Ramayya, A. V. Riley, F. D. Roberto, J. B. Ryabinin, M. A. Rykaczewski, K. P. Sagaidak, R. N. Shaughnessy, D. A. Shirokovsky, I. V. Stoyer, M. A. Subbotin, V. G. Sudowe, R. Sukhov, A. M. Taylor, R. Tsyganov, Yu. S. Utyonkov, V. K. Voinov, A. A. Vostokin, G. K. Wilk, P. A. TI Eleven new heaviest isotopes of elements Z=105 to Z=117 identified among the products of Bk-249+Ca-48 reactions SO PHYSICAL REVIEW C LA English DT Article ID SPONTANEOUS-FISSION; SUPERHEAVY NUCLEI; EXTRACTION; MASSES; TABLES; DECAY AB The heaviest isotopes of elements Z = 117 to Z = 105, (294)117, (293)117, (290)115, (289)115, (286)113, (285)113, (282)Rg, (281)Rg, (278)Mt, (274)Bh, and (270)Db, were identified by means of the Dubna gas-filled recoil separator among the products of the Bk-249 + Ca-48 reaction. The details of the observed six decay chains, indicating the production and decay of isotopes (293)117 and (294)117, are presented and discussed. The decay energies and resulting half-lives of these new nuclei show a strong rise of stability with increasing neutron number, validating the concept of the island of enhanced stability for superheavy nuclei [Oganessian et al., Phys. Rev. Lett. 104, 142502 (2010)]. C1 [Bailey, P. D.; Benker, D. E.; Ezold, J. G.; Porter, C. E.; Riley, F. D.; Roberto, J. B.; Rykaczewski, K. P.; Taylor, R.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Bennett, M. E.; Sudowe, R.] Univ Nevada, Las Vegas, NV 89154 USA. [Hamilton, J. H.; Ramayya, A. V.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Henderson, R. A.; Moody, K. J.; Nelson, S. L.; Shaughnessy, D. A.; Stoyer, M. A.; Wilk, P. A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Ryabinin, M. A.] Res Inst Atom Reactors, RU-433510 Dimitrovgrad, Russia. [Oganessian, Yu. Ts.; Abdullin, F. Sh.; Dmitriev, S. N.; Itkis, M. G.; Lobanov, Yu. V.; Mezentsev, A. N.; Polyakov, A. N.; Sagaidak, R. N.; Shirokovsky, I. V.; Subbotin, V. G.; Sukhov, A. M.; Tsyganov, Yu. S.; Utyonkov, V. K.; Voinov, A. A.; Vostokin, G. K.] Joint Inst Nucl Res, RU-141980 Dubna, Russia. RP Oganessian, YT (reprint author), Joint Inst Nucl Res, RU-141980 Dubna, Russia. EM oganessian@jinr.ru RI Wilk, Philip/B-5954-2008 FU Russian Federal Agency of Atomic Energy (RFBR) [07-02-00029, 09-02-12060, 09-03-12214]; DOE Office of Nuclear Physics, Office of Basic Energy Sciences; DOE [09-040, DE-AC05-00OR22725, 08-ERD-030, DE-AC52-07NA27344]; UT-Battelle, LLC.; Lawrence Livermore National Security, LLC.; US DOE [DE-FG-05-88ER40407, DE-FG07-01AL67358] FX We are grateful to the JINR Directorate and U-400 cyclotron and ion source crews for their continuous support of the experiment and to the ORNL Radiochemical Engineering Development Center and High Flux Isotope Reactor staff for production and chemical separation of the berkelium target material. We acknowledge the support of the Russian Federal Agency of Atomic Energy (RFBR) Grants No. 07-02-00029, No. 09-02-12060, and No. 09-03-12214. Research at ORNL was supported by the DOE Office of Nuclear Physics, Office of Basic Energy Sciences (for support of the High Flux Isotope Reactor), and Laboratory Directed Research and Development (LDRD) Program Project 09-040, under DOE Contract DE-AC05-00OR22725 with UT-Battelle, LLC. Research at Lawrence Livermore National Laboratory was supported by LDRD Program Project 08-ERD-030, under DOE Contract DE-AC52-07NA27344 with Lawrence Livermore National Security, LLC. This work was also supported by the US DOE through Grants No. DE-FG-05-88ER40407 (Vanderbilt University) and No. DE-FG07-01AL67358 (UNLV). These studies were performed in the framework of the Russian Federation/US Joint Coordinating Committee for Research on Fundamental Properties of Matter. NR 63 TC 59 Z9 59 U1 0 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAY 18 PY 2011 VL 83 IS 5 AR 054315 DI 10.1103/PhysRevC.83.054315 PG 14 WC Physics, Nuclear SC Physics GA 765OL UT WOS:000290717900003 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Friedl, M Fruhwirth, R Ghete, VM Hammer, J Haensel, S Hoch, M Hormann, N Hrubec, J Jeitler, M Kasieczka, G Kiesenhofer, W Krammer, M Liko, D Mikulec, I Pernicka, M Rohringer, H Schofbeck, R Strauss, J Taurok, A Teischinger, F Wagner, P Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Benucci, L Cerny, K De Wolf, EA Janssen, X Maes, T Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Beauceron, S Blekman, F Blyweert, S D'Hondt, J Devroede, O Suarez, RG Kalogeropoulos, A Maes, J Maes, M Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Charaf, O Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hammad, GH Hreus, T Marage, PE Thomas, L Velde, CV Vanlaer, P Wickens, J Adler, V Costantini, S Grunewald, M Klein, B Marinov, A Mccartin, J Ryckbosch, D Thyssen, F Tytgat, M Vanelderen, L Verwilligen, P Walsh, S Zaganidis, N Basegmez, S Bruno, G Caudron, J Ceard, L De Jeneret, JD Delaere, C Demin, P Favart, D Giammanco, A Gregoire, G Hollar, J Lemaitre, V Liao, J Militaru, O Ovyn, S Pagano, D Pin, A Piotrzkowski, K Schul, N Beliy, N Caebergs, T Daubie, E Alves, GA Damiao, DD Pol, ME Souza, MHG Carvalho, W Da Costa, EM Martins, CD De Souza, SF Mundim, L Nogima, H Oguri, V Da Silva, WLP Santoro, A Do Amaral, SMS Sznajder, A De Araujo, FTD Dias, FA Dias, MAF Tomei, TRFP Gregores, EM Marinho, F Novaes, SF Padula, SS Darmenov, N Dimitrov, L Genchev, V Iaydjiev, P Piperov, S Rodozov, M Stoykova, S Sultanov, G Tcholakov, V Trayanov, R Vankov, I Dyulendarova, M Hadjiiska, R Kozhuharov, V Litov, L Marinova, E Mateev, M Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Wang, J Wang, J Wang, X Wang, Z Xu, M Yang, M Zang, J Zhang, Z Ban, Y Guo, S Guo, Y Li, W Mao, Y Qian, SJ Teng, H Zhang, L Zhu, B Zou, W Cabrera, A Moreno, BG Rios, AAO Oliveros, AFO Sanabria, JC Godinovic, N Lelas, D Lelas, K Plestina, R Polic, D Puljak, I Antunovic, Z Dzelalija, M Brigljevic, V Duric, S Kadija, K Morovic, S Attikis, A Galanti, M Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Finger, M Finger, M Assran, Y Mahmoud, MA Hektor, A Kadastik, M Kannike, K Muntel, M Raidal, M Rebane, L Azzolini, V Eerola, P Czellar, S Harkonen, J Heikkinen, A Karimaki, V Kinnunen, R Klem, J Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Tuominen, E Tuominiemi, J Tuovinen, E Ungaro, D Wendland, L Banzuzi, K Korpela, A Tuuva, T Sillou, D Besancon, M Choudhury, S Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Gentit, FX Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Marionneau, M Millischer, L Rander, J Rosowsky, A Shreyber, I Titov, M Verrecchia, P Baffioni, S Beaudette, F Bianchini, L Bluj, M Broutin, C Busson, P Charlot, C Dahms, T Dobrzynski, L de Cassagnac, RG Haguenauer, M Mine, P Mironov, C Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Thiebaux, C Wyslouch, B Zabi, A Agram, JL Andrea, J Besson, A Bloch, D Bodin, D Brom, JM Cardaci, M Chabert, EC Collard, C Conte, E Drouhin, F Ferro, C Fontaine, JC Gele, D Goerlach, U Greder, S Juillot, P Karim, M Le Bihan, AC Mikami, Y Van Hove, P Fassi, F Mercier, D Baty, C Beaupere, N Bedjidian, M Bondu, O Boudoul, G Boumediene, D Brun, H Chanon, N Chierici, R Contardo, D Depasse, P El Mamouni, H Falkiewicz, A Fay, J Gascon, S Ille, B Kurca, T Le Grand, T Lethuillier, M Mirabito, L Perries, S Sordini, V Tosi, S Tschudi, Y Verdier, P Xiao, H Megrelidze, L Roinishvili, V Lomidze, D Anagnostou, G Edelhoff, M Feld, L Heracleous, N Hindrichs, O Jussen, R Klein, K Merz, J Mohr, N Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Weber, M Wittmer, B Ata, M Bender, W Erdmann, M Frangenheim, J Hebbeker, T Hinzmann, A Hoepfner, K Hof, C Klimkovich, T Klingebiel, D Kreuzer, P Lanske, D Magass, C Masetti, G Merschmeyer, M Meyer, A Papacz, P Pieta, H Reithler, H Schmitz, SA Sonnenschein, L Steggemann, J Teyssier, D Bontenackels, M Davids, M Duda, M Flugge, G Geenen, H Giffels, M Ahmad, WH Heydhausen, D Kress, T Kuessel, Y Linn, A Nowack, A Perchalla, L Pooth, O Rennefeld, J Sauerland, P Stahl, A Thomas, M Tornier, D Zoeller, MH Martin, MA Behrenhoff, W Behrens, U Bergholz, M Borras, K Cakir, A Campbell, A Castro, E Dammann, D Eckerlin, G Eckstein, D Flossdorf, A Flucke, G Geiser, A Glushkov, I Hauk, J Jung, H Kasemann, M Katkov, I Katsas, P Kleinwort, C Kluge, H Knutsson, A Krucker, D Kuznetsova, E Lange, W Lohmann, W Mankel, R Marienfeld, M Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Olzem, J Parenti, A Raspereza, A Raval, A Schmidt, R Schoerner-Sadenius, T Sen, N Stein, M Tomaszewska, J Volyanskyy, D Walsh, R Wissing, C Autermann, C Bobrovskyi, S Draeger, J Enderle, H Gebbert, U Kaschube, K Kaussen, G Klanner, R Lange, J Mura, B Naumann-Emme, S Nowak, F Pietsch, N Sander, C Schettler, H Schleper, P Schroder, M Schum, T Schwandt, J Srivastava, AK Stadie, H Steinbruck, G Thomsen, J Wolf, R Barth, C Bauer, J Buege, V Chwalek, T De Boer, W Dierlamm, A Dirkes, G Feindt, M Gruschke, J Hackstein, C Hartmann, F Heindl, SM Heinrich, M Held, H Hoffmann, KH Honc, S Kuhr, T Martschei, D Mueller, S Muller, T Niegel, M Oberst, O Oehler, A Ott, J Peiffer, T Piparo, D Quast, G Rabbertz, K Ratnikov, F Renz, M Saout, C Scheurer, A Schieferdecker, P Schilling, FP Schott, G Simonis, HJ Stober, FM Troendle, D Wagner-Kuhr, J Zeise, M Zhukov, V Ziebarth, EB Daskalakis, G Geralis, T Kesisoglou, S Kyriakis, A Loukas, D Manolakos, I Markou, A Markou, C Mavrommatis, C Ntomari, E Petrakou, E Gouskos, L Mertzimekis, TJ Panagiotou, A Evangelou, I Foudas, C Kokkas, P Manthos, N Papadopoulos, I Patras, V Triantis, FA Aranyi, A Bencze, G Boldizsar, L Debreczeni, G Hajdu, C Horvath, D Kapusi, A Krajczar, K Laszlo, A Sikler, F Vesztergombi, G Beni, N Molnar, J Palinkas, J Szillasi, Z Veszpremi, V Raics, P Trocsanyi, ZL Ujvari, B Bansal, S Beri, SB Bhatnagar, V Dhingra, N Gupta, R Jindal, M Kaur, M Kohli, JM Mehta, MZ Nishu, N Saini, LK Sharma, A Singh, AP Singh, JB Singh, SP Ahuja, S Bhattacharya, S Choudhary, BC Gupta, P Jain, S Jain, S Kumar, A Shivpuri, RK Choudhury, RK Dutta, D Kailas, S Kataria, SK Mohanty, AK Pant, LM Shukla, P Aziz, T Guchait, M Gurtu, A Maity, M Majumder, D Majumder, G Mazumdar, K Mohanty, GB Saha, A Sudhakar, K Wickramage, N Banerjee, S Dugad, S Mondal, NK Arfaei, H Bakhshiansohi, H Etesami, SM Fahim, A Hashemi, M Jafari, A Khakzad, M Mohammadi, A Najafabadi, MM Mehdiabadi, SP Safarzadeh, B Zeinali, M Abbrescia, M Barbone, L Calabria, C Colaleo, A Creanza, D De Filippis, N De Palma, M Dimitrov, A Fiore, L Iaselli, G Lusito, L Maggi, G Maggi, M Manna, N Marangelli, B My, S Nuzzo, S Pacifico, N Pierro, GA Pompili, A Pugliese, G Romano, F Roselli, G Selvaggi, G Silvestris, L Trentadue, R Tupputi, S Zito, G Abbiendi, G Benvenuti, AC Bonacorsi, D Braibant-Giacomelli, S Brigliadori, L Capiluppi, P Castro, A Cavallo, FR Cuffiani, M Dallavalle, GM Fabbri, F Fanfani, A Fasanella, D Giacomelli, P Giunta, M Grandi, C Marcellini, S Meneghelli, M Montanari, A Navarria, FL Odorici, F Perrotta, A Primavera, F Rossi, AM Rovelli, T Siroli, G Travaglini, R Albergo, S Cappello, G Chiorboli, M Costa, S Tricomi, A Tuve, C Barbagli, G Ciulli, V Civinini, C D'Alessandro, R Focardi, E Frosali, S Gallo, E Gonzi, S Lenzi, P Meschini, M Paoletti, S Sguazzoni, G Tropiano, A Benussi, L Bianco, S Colafranceschi, S Fabbri, F Piccolo, D Fabbricatore, P Musenich, R Benaglia, A De Guio, F Di Matteo, L Ghezzi, A Malberti, M Malvezzi, S Martelli, A Massironi, A Menasce, D Moroni, L Paganoni, M Pedrini, D Ragazzi, S Redaelli, N Sala, S de Fatis, TT Tancini, V Buontempo, S Montoya, CAC Cimmino, A De Cosa, A De Gruttola, M 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Barker, A. Duggan, D. Gershtein, Y. Gray, R. Halkiadakis, E. Hidas, D. Hits, D. Lath, A. Panwalkar, S. Patel, R. Richards, A. Rose, K. Schnetzer, S. Somalwar, S. Stone, R. Thomas, S. Cerizza, G. Hollingsworth, M. Spanier, S. Yang, Z. C. York, A. Asaadi, J. Eusebi, R. Gilmore, J. Gurrola, A. Kamon, T. Khotilovich, V. Montalvo, R. Nguyen, C. N. Osipenkov, I. Pivarski, J. Safonov, A. Sengupta, S. Tatarinov, A. Toback, D. Weinberger, M. Akchurin, N. Damgov, J. Jeong, C. Kovitanggoon, K. Lee, S. W. Roh, Y. Sill, A. Volobouev, I. Wigmans, R. Yazgan, E. Appelt, E. Brownson, E. Engh, D. Florez, C. Gabella, W. Johns, W. Kurt, P. Maguire, C. Melo, A. Sheldon, P. Tuo, S. Velkovska, J. Arenton, M. W. Balazs, M. Boutle, S. Buehler, M. Conetti, S. Cox, B. Francis, B. Hirosky, R. Ledovskoy, A. Lin, C. Neu, C. Yohay, R. Gollapinni, S. Harr, R. Karchin, P. E. Lamichhane, P. Mattson, M. Milstene, C. Sakharov, A. Anderson, M. Bachtis, M. Bellinger, J. N. Carlsmith, D. Dasu, S. Efron, J. Gray, L. Grogg, K. S. Grothe, M. Hall-Wilton, R. Herndon, M. Klabbers, P. Klukas, J. Lanaro, A. Lazaridis, C. Leonard, J. Loveless, R. Mohapatra, A. Reeder, D. Ross, I. Savin, A. Smith, W. H. Swanson, J. Weinberg, M. CA CMS Collaboration TI Measurement of Dijet Angular Distributions and Search for Quark Compositeness in pp Collisions at root s=7 TeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID COLLIDER; DETECTOR; PHYSICS; LIMIT AB Dijet angular distributions are measured over a wide range of dijet invariant masses in pp collisions at root s = 7 TeV, at the CERN LHC. The event sample, recorded with the CMS detector, corresponds to an integrated luminosity of 36 pb(-1). The data are found to be in good agreement with the predictions of perturbative QCD, and yield no evidence of quark compositeness. 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[Andrea, J.; Besson, A.; Bloch, D.; Bodin, D.; Brom, J. -M.; Cardaci, M.; Chabert, E. C.; Collard, C.; Conte, E.; Drouhin, F.; Ferro, C.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Greder, S.; Juillot, P.; Karim, M.; Le Bihan, A. -C.; Mikami, Y.; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, CNRS, Inst Pluridisciplinaire Hubert Curien,IN2P3, Strasbourg, France. [Fassi, F.; Mercier, D.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. [Baty, C.; Beaupere, N.; Bedjidian, M.; Bondu, O.; Boudoul, G.; Boumediene, D.; Brun, H.; Chanon, N.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Falkiewicz, A.; Fay, J.; Gascon, S.; Ille, B.; Kurca, T.; Le Grand, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Sordini, V.; Tosi, S.; Tschudi, Y.; Verdier, P.; Xiao, H.] Univ Lyon 1, Inst Nucl Phys, IN2P3, CNRS, Villeurbanne, France. [Megrelidze, L.; Roinishvili, V.] Acad Sci, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Lomidze, D.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Anagnostou, G.; Edelhoff, M.; Feld, L.; Heracleous, N.; Hindrichs, O.; Jussen, R.; Klein, K.; Merz, J.; Mohr, N.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Weber, M.; Wittmer, B.] RWTH Aachen Univ I, Physikal Inst, Aachen, Germany. [Ata, M.; Bender, W.; Erdmann, M.; Frangenheim, J.; Hebbeker, T.; Hinzmann, A.; Hoepfner, K.; Hof, C.; Klimkovich, T.; Klingebiel, D.; Kreuzer, P.; Lanske, D.; Magass, C.; Masetti, G.; Merschmeyer, M.; Meyer, A.; Papacz, P.; Pieta, H.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Steggemann, J.; Teyssier, D.; Bontenackels, M.] RWTH Aachen Univ III, Physikal Inst A, Aachen, Germany. [Davids, M.; Duda, M.; Fluegge, G.; Geenen, H.; Giffels, M.; Ahmad, W. Haj; Heydhausen, D.; Kress, T.; Kuessel, Y.; Linn, A.; Nowack, A.; Perchalla, L.; Pooth, O.; Rennefeld, J.; Sauerland, P.; Stahl, A.; Thomas, M.; Tornier, D.; Zoeller, M. H.] RWTH Aachen Univ III, Physikal Inst B, Aachen, Germany. [Martin, M. Aldaya; Behrenhoff, W.; Behrens, U.; Bergholz, M.; Borras, K.; Cakir, A.; Campbell, A.; Castro, E.; Dammann, D.; Eckerlin, G.; Eckstein, D.; Flossdorf, A.; Flucke, G.; Geiser, A.; Glushkov, I.; Hauk, J.; Jung, H.; Kasemann, M.; Katkov, I.; Katsas, P.; Kleinwort, C.; Kluge, H.; Knutsson, A.; Kruecker, D.; Kuznetsova, E.; Lange, W.; Lohmann, W.; Mankel, R.; Marienfeld, M.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Olzem, J.; Parenti, A.; Raspereza, A.; Raval, A.; Schmidt, R.; Schoerner-Sadenius, T.; Sen, N.; Stein, M.; Tomaszewska, J.; Volyanskyy, D.; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Autermann, C.; Bobrovskyi, S.; Draeger, J.; Enderle, H.; Gebbert, U.; Kaschube, K.; Kaussen, G.; Klanner, R.; Lange, J.; Mura, B.; Naumann-Emme, S.; Nowak, F.; Pietsch, N.; Sander, C.; Schettler, H.; Schleper, P.; Schroeder, M.; Schum, T.; Schwandt, J.; Srivastava, A. K.; Stadie, H.; Steinbrueck, G.; Thomsen, J.; Wolf, R.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Bauer, J.; Buege, V.; Chwalek, T.; De Boer, W.; Dierlamm, A.; Dirkes, G.; Feindt, M.; Gruschke, J.; Hackstein, C.; Hartmann, F.; Heindl, S. M.; Heinrich, M.; Held, H.; Hoffmann, K. H.; Honc, S.; Kuhr, T.; Martschei, D.; Mueller, S.; Mueller, Th.; Niegel, M.; Oberst, O.; Oehler, A.; Ott, J.; Peiffer, T.; Piparo, D.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Renz, M.; Saout, C.; Scheurer, A.; Schieferdecker, P.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Troendle, D.; Wagner-Kuhr, J.; Zeise, M.; Zhukov, V.; Ziebarth, E. B.] Univ Karlsruhe, Inst Expt Kernphys, D-7500 Karlsruhe, Germany. [Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Manolakos, I.; Markou, A.; Markou, C.; Mavrommatis, C.; Ntomari, E.; Petrakou, E.] Inst Nucl Phys Demokritos, Aghia Paraskevi, Greece. [Gouskos, L.; Mertzimekis, T. J.; Panagiotou, A.; Sphicas, P.] Univ Athens, Athens, Greece. [Evangelou, I.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Patras, V.; Triantis, F. A.] Univ Ioannina, GR-45110 Ioannina, Greece. [Aranyi, A.; Bencze, G.; Boldizsar, L.; Debreczeni, G.; Hajdu, C.; Horvath, D.; Kapusi, A.; Krajczar, K.; Laszlo, A.; Sikler, F.; Vesztergombi, G.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Molnar, J.; Palinkas, J.; Szillasi, Z.] ATOMKI, Inst Nucl Res, Debrecen, Hungary. [Veszpremi, V.; Raics, P.; Trocsanyi, Z. L.] Univ Debrecen, H-4012 Debrecen, Hungary. [Ujvari, B.; Bansal, S.; Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Jindal, M.; Kaur, M.; Kohli, J. M.; Mehta, M. Z.; Nishu, N.; Saini, L. K.; Sharma, A.; Singh, A. P.; Singh, J. B.; Singh, S. P.] Panjab Univ, Chandigarh 160014, India. [Ahuja, S.; Bhattacharya, S.; Choudhary, B. C.; Gupta, P.; Jain, S.; Kumar, A.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Choudhury, R. K.; Dutta, D.; Kailas, S.; Kataria, S. K.; Mohanty, A. K.; Pant, L. M.; Shukla, P.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Aziz, T.; Guchait, M.; Gurtu, A.; Maity, M.; Majumder, D.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Saha, A.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Mumbai, Maharashtra, India. [Guchait, M.; Banerjee, S.; Dugad, S.; Mondal, N. K.] Tata Inst Fundamental Res HECR, Mumbai, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Hashemi, M.; Jafari, A.; Khakzad, M.; Mohammadi, A.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res & Fundamental Sci IPM, Tehran, Iran. [Abbrescia, M.; Barbone, L.; Calabria, C.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Dimitrov, A.; Fiore, L.; Iaselli, G.; Lusito, L.; Maggi, G.; Maggi, M.; Manna, N.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pierro, G. A.; Pompili, A.; Pugliese, G.; Romano, F.; Roselli, G.; Selvaggi, G.; Silvestris, L.; Trentadue, R.; Tupputi, S.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; De Filippis, N.; De Palma, M.; Lusito, L.; Manna, N.; Marangelli, B.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Roselli, G.; Selvaggi, G.; Tupputi, S.; Zito, G.] Univ Bari, Bari, Italy. [Colaleo, A.; Creanza, D.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.; Romano, F.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Giunta, M.; Grandi, C.; Marcellini, S.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Braibant-Giacomelli, S.; Capiluppi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Meneghelli, M.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Tricomi, A.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Frosali, S.; Gonzi, S.; Lenzi, P.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Colafranceschi, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Ghezzi, A.; Malberti, M.; Malvezzi, S.; Martelli, A.; Massironi, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; Sala, S.; de Fatis, T. Tabarelli; Tancini, V.] Ist Nazl Fis Nucl, Sez Milano Biccoca, I-20133 Milan, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Ghezzi, A.; Malberti, M.; Martelli, A.; Massironi, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli; Tancini, V.] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Montoya, C. A. Carrillo; Cimmino, A.; De Cosa, A.; De Gruttola, M.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Merola, M.; Noli, P.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Cimmino, A.; De Cosa, A.; De Gruttola, M.; Lista, L.; Merola, M.; Noli, P.] Univ Naples Federico II, Naples, Italy. [Bellan, P.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Conti, E.; De Mattia, M.; Dorigo, T.; Dosselli, U.; Fanzago, F.; Gasparini, F.; Giubilato, P.; Gresele, A.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Mazzucato, M.; Meneguzzo, A. T.; Nespolo, M.; Perrozzi, L.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bellan, P.; Bisello, D.; Carlin, R.; Checchia, P.; Dorigo, T.; Gasparini, F.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Univ Padua, Padua, Italy. [Gresele, A.; Lazzizzera, I.] Univ Trent, Padua, Italy. [Berzano, U.; Riccardi, C.; Torre, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez pavia, I-27100 Pavia, Italy. [Berzano, U.; Riccardi, C.; Torre, P.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Pioppi, M.; Musienko, Y.] Univ Perugia, Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Caponeri, B.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Nappi, A.; Santocchia, A.; Taroni, S.; Valdata, M.; Volpe, R.] Univ Perugia, I-06100 Perugia, Italy. [Castro, A.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Palmonari, F.; Sarkar, S.; Segneri, G.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bernardini, J.; Fiori, F.; Messineo, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Azzurri, P.; Broccolo, G.; D'Agnolo, R. T.; Foa, L.; Ligabue, F.; Sarkar, S.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Di Marco, E.; Diemoz, M.; Franci, D.; Grassi, M.; Longo, E.; Nourbakhsh, S.; Organtini, G.; Palma, A.; Pandolfi, F.; Paramatti, R.; Rahatlou, S.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Di Marco, E.; Franci, D.; Longo, E.; Organtini, G.; Palma, A.; Pandolfi, F.; Rahatlou, S.] Univ Roma La Sapienza, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Botta, C.; Cartiglia, N.; Castello, R.; Costa, M.; Demaria, N.; Graziano, A.; Mariotti, C.; Marone, M.; Maselli, S.; Migliore, E.; Mila, G.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Romero, A.; Ruspa, M.; Sacchi, R.; Sola, V.; Solano, A.; Staiano, A.; Trocino, D.; Pereira, A. Vilela] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Botta, C.; Castello, R.; Costa, M.; Graziano, A.; Marone, M.; Migliore, E.; Mila, G.; Monaco, V.; Musich, M.; Pelliccioni, M.; Romero, A.; Sacchi, R.; Sola, V.; Solano, A.; Trocino, D.; Pereira, A. Vilela] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Montanino, D.; Penzo, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Della Ricca, G.; Montanino, D.] Univ Trieste, Trieste, Italy. [Heo, S. G.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Chung, J.; Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Park, H.; Son, D.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, Zero; Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Hong, B.; Jo, M.; Kim, H.; Kim, J. H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.; Rhee, H. B.; Seo, E.; Shin, S.; Sim, K. S.] Korea Univ, Seoul, South Korea. [Choi, M.; Kang, S.; Kim, H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Martisiute, D.; Petrov, P.; Sabonis, T.] Vilnius Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De la Cruz-Burelo, E.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Moreno, S. Carrillo; Valencia, F. Vazquez] Univ Iberoamer, Mexico City, DF, Mexico. [Ibarguen, H. A. Salazar] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Linares, E. Casimiro; Pineda, A. Morelos; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Allfrey, P.; Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ahmed, I.; Asghar, M. I.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Broutin, C.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Soltan Inst Nucl Studies, PL-00681 Warsaw, Poland. [Almeida, N.; David, A.; Faccioli, P.; Parracho, P. G. Ferreira; Gallinaro, M.; Martins, P.; Musella, P.; Nayak, A.; Ribeiro, P. Q.; Seixas, J.; Silva, P.; Varela, J.; Woehri, H. K.] Lab Instrumentac & Fis Expt Particuas, Lisbon, Portugal. [Belotelov, I.; Bunin, P.; Golutvin, I.; Kamenev, A.; Karjavin, V.; Kozlov, G.; Lanev, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Bondar, N.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, Gatchina, St Petersburg, Russia. [Andreev, Yu.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Toropin, A.; Troitsky, S.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Kaftanov, V.; Kossov, M.; Krokhotin, A.; Lychkovskaya, N.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Zhukov, V.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Sarycheva, L.; Savrin, V.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Snigirev, A.; Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Rusakov, S. V.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Vinogradov, A.; Azhgirey, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Slabospitsky, S.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Arce, P.; Battilana, C.; Calvo, E.; Cepeda, M.; Cerrada, M.; Colino, N.; De La Cruz, B.; Diez Pardos, C.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Redondo, I.; Romero, L.; Santaolalla, J.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chamizo Llatas, M.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Jorda, C.; Lobelle Pardo, P.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Ruiz-Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Darmenov, N.; Genchev, V.; Iaydjiev, P.; Hajdu, C.; Mohanty, A. K.; Lusito, L.; Tropiano, A.; De Guio, F.; Ghezzi, A.; Nespolo, M.; Perrozzi, L.; Lucaroni, A.; Boccali, T.; Tonelli, G.; Venturi, A.; Pandolfi, F.; Botta, C.; Graziano, A.; Pelliccioni, M.; Pereira, A. Vilela; Kossov, M.; Bitioukov, S.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Baillon, P.; Ball, A. H.; Barney, D.; Bell, A. J.; Benedetti, D.; Bernet, C.; Bialas, W.; Bloch, P.; Bocci, A.; Bolognesi, S.; Brona, G.; Bunkowski, K.; Camporesi, T.; Cano, E.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Cure, B.; D'Enterria, D.; De Roeck, A.; Di Guida, S.; Ramos, F. Duarte; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Gaddi, A.; Gennai, S.; Georgiou, G.; Gerwig, H.; Gigi, D.; Gill, K.; Giordano, D.; Glege, F.; Garrido, R. Gomez-Reino; Gouzevitch, M.; Govoni, P.; Gowdy, S.; Guiducci, L.; Hansen, M.; Harvey, J.; Hegeman, J.; Hegner, B.; Henderson, C.; Hesketh, G.; Hoffmann, H. F.; Honma, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Lecoq, P.; Lourenco, C.; Macpherson, A.; Maeki, T.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Nesvold, E.; Nguyen, M.; Orimoto, T.; Orsini, L.; Perez, E.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Polese, G.; Racz, A.; Antunes, J. Rodrigues; Rolandi, G.; Rommerskirchen, T.; Rovelli, C.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Segoni, I.; Sharma, A.; Siegrist, P.; Simon, M.; Sphicas, P.; Spiga, D.; Spiropulu, M.; Stoeckli, F.; Stoye, M.; Tropea, P.; Tsirou, A.; Tsyganov, A.; Veres, G. I.; Vichoudis, P.; Voutilainen, M.; Zeuner, W. D.; Hall-Wilton, R.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Starodumov, A.; Caminada, L.; Marchica, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bortignon, P.; Caminada, L.; Chen, Z.; Cittolin, S.; Dissertori, G.; Dittmar, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Herve, A.; Hintz, W.; Lecomte, P.; Lustermann, W.; Marchica, C.; del Arbol, P. Martinez Ruiz; Meridiani, P.; Milenovic, P.; Moortgat, F.; Nef, P.; Nessi-Tedaldi, F.; Pape, L.; Pauss, F.; Punz, T.; Rizzi, A.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Sawley, M. -C.; Stieger, B.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, M.; Wehrli, L.; Weng, J.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aguilo, E.; Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Regenfus, C.; Robmann, P.; Schmidt, A.; Snoek, H.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Chen, W. T.; Dutta, S.; Go, A.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, M. H.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Wu, J. H.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Demir, Z.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Topaksu, A. Kayis; Nart, A.; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Tali, B.; Topakli, H.; Uzun, D.; Vergili, L. N.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Deliomeroglu, M.; Demir, D.; Guelmez, E.; Halu, A.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Levchuk, L.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Bell, P.; Bostock, F.; Brooke, J. J.; Cheng, T. L.; Clement, E.; Cussans, D.; Frazier, R.; Goldstein, J.; Grimes, M.; Hansen, M.; Hartley, D.; Heath, G. P.; Heath, H. F.; Huckvale, B.; Jackson, J.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Ward, S.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Camanzi, B.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Ballin, J.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Davies, G.; Della Negra, M.; Fulcher, J.; Futyan, D.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Karapostoli, G.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rompotis, N.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Tourneur, S.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardrope, D.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Barrett, M.; Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Martin, W.; Reid, I. D.; Teodorescu, L.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.] Baylor Univ, Waco, TX 76706 USA. [Bose, T.; Jarrin, E. Carrera; Fantasia, C.; Heister, A.; John, J. St.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Avetisyan, A.; Bhattacharya, S.; Chou, J. P.; Cutts, D.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Landsberg, G.; Narain, M.; Nguyen, D.; Segala, M.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Borgia, M. A.; Breedon, R.; De la Barca Sanchez, M. Calderon; Cebra, D.; Chauhan, S.; Chertok, M.; Conway, J.; Cox, P. T.; Dolen, J.; Erbacher, R.; Friis, E.; Ko, W.; Kopecky, A.; Lander, R.; Liu, H.; Maruyama, S.; Miceli, T.; Nikolic, M.; Pellett, D.; Robles, J.; Salur, S.; Schwarz, T.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez; Veelken, C.; Gurrola, A.] Univ Calif Davis, Davis, CA 95616 USA. [Felcini, M.; Andreev, V.; Arisaka, K.; Cline, D.; Cousins, R.; Deisher, A.; Duris, J.; Erhan, S.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Tucker, J.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Kao, S. C.; Liu, F.; Liu, H.; Luthra, A.; Nguyen, H.; Shen, B. C.; Stringer, R.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Dusinberre, E.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Mangano, B.; Muelmenstaedt, J.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pi, H.; Pieri, M.; Ranieri, R.; Sani, M.; Sharma, V.; Simon, S.; Tu, Y.; Vartak, A.; Rthwein, F. Wu; Yagil, A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; Vlimant, J. R.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Spiropulu, M.; Bornheim, A.; Bunn, J.; Kcira, D.; Mott, A.; Newman, H. B.; Rogan, C.; Akgun, B.] CALTECH, Pasadena, CA 91125 USA. [Iiyama, Y.; Jang, D. W.; Jun, S. Y.; Liu, Y. F.; Paulini, M.; Russ, J.; Terentyev, N.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Dinardo, M. E.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Gaz, A.; Heyburn, B.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.; Zang, S. L.] Univ Colorado, Boulder, CO 80309 USA. [Agostino, L.; Alexander, J.; Chatterjee, A.; Das, S.; Eggert, N.; Fields, L. J.; Gibbons, L. K.; Heltsley, B.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Kuznetsov, V.; Kaufman, G. Nicolas; Patterson, J. R.; Puigh, D.; Riley, D.; Ryd, A.; Shi, X.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY 14853 USA. [Biselli, A.; Cirino, G.; Winn, D.] Fairfield Univ, Fairfield, CT 06824 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Atac, M.; Bakken, J. A.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Borcherding, F.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Demarteau, M.; Eartly, D. P.; Elvira, V. D.; Esen, S.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Green, D.; Gunthoti, K.; Gutsche, O.; Hahn, A.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; James, E.; Jensen, H.; Johnson, M.; Joshi, U.; Khatiwada, R.; Kilminster, B.; Klima, B.; Kousouris, K.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Limon, P.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Mason, D.; McBride, P.; McCauley, T.; Miao, T.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Popescu, S.; Pordes, R.; Prokofyev, O.; Saoulidou, N.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Tan, P.; Taylor, L.; Tkaczyk, S.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Piedra Gomez, J.; Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Goldberg, S.; Kim, B.; Klimenko, S.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Matchev, K.; Mitselmakher, G.; Muniz, L.; Pakhotin, Y.; Prescott, C.; Remington, R.; Schmitt, M.; Scurlock, B.; Sellers, P.; Skhirtladze, N.; Wang, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL 32611 USA. [Ceron, C.; Gaultney, V.; Kramer, L.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bandurin, D.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Quertenmont, L.; Sekmen, S.; Veeraraghavan, V.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Guragain, S.; Hohlmann, M.; Kalakhety, H.; Ralich, R.; Vodopiyanov, I.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Callner, J.; Cavanaugh, R.; Dragoiu, C.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; O'Brien, C.; Silvestre, C.; Varelas, N.] Univ Illinois, Chicago, IL 60607 USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Cankocak, K.; Clarida, W.; Duru, F.; Lae, C. K.; McCliment, E.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Olson, J.; Onel, Y.; Ozok, F.; Sen, S.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA 52242 USA. [Barnett, B. A.; Blumenfeld, B.; Bonato, A.; Eskew, C.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Guo, Z. J.; Hu, G.; Maksimovic, P.; Rappoccio, S.; Swartz, M.; Tran, N. V.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD 21218 USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Grachov, O.; Murray, M.; Noonan, D.; Radicci, V.; Sanders, S.; Wood, J. S.; Zhukova, V.] Univ Kansas, Lawrence, KS 66045 USA. [Bolton, T.; Chakaberia, I.; Ivanov, A.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.; Wan, Z.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA 94720 USA. [Baden, A.; Boutemeur, M.; Eno, S. C.; Ferencek, D.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kim, M.; Lu, Y.; Mignerey, A. C.; Rossato, K.; Rumerio, P.; Santanastasio, F.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.; Twedt, E.] Univ Maryland, College Pk, MD 20742 USA. [Wyslouch, B.; Alver, B.; Bauer, G.; Bendavid, J.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Everaerts, P.; Ceballos, G. Gomez; Goncharov, M.; Hahn, K. A.; Harris, P.; Kim, Y.; Klute, M.; Lee, Y. -J.; Li, W.; Loizides, C.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Rudolph, M.; Stephans, G. S. F.; Sumorok, K.; Sung, K.; Wenger, E. A.; Xie, S.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.] MIT, Cambridge, MA 02139 USA. [Cole, P.; Cooper, S. I.; Cushman, P.; Dahmes, B.; De Benedetti, A.; Dudero, P. R.; Franzoni, G.; Haupt, J.; Klapoetke, K.; Kubota, Y.; Mans, J.; Rekovic, V.; Rusack, R.; Sasseville, M.; Singovsky, A.; Cremaldi, L. M.] Univ Minnesota, Minneapolis, MN 55455 USA. [Godang, R.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, University, MS 38677 USA. [Bloom, K.; Bose, S.; Butt, J.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kelly, T.; Kravchenko, I.; Lazo-Flores, J.; Lundstedt, C.; Malbouisson, H.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE 68588 USA. [Baur, U.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Shipkowski, S. P.; Smith, K.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Boeriu, O.; Chasco, M.; Reucroft, S.; Swain, J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Kubik, A.; Odell, N.; Ofierzynski, R. A.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL 60208 USA. [Antonelli, L.; Berry, D.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Kolberg, T.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Warchol, J.; Wayne, M.; Ziegler, J.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Bylsma, B.; Durkin, L. S.; Gu, J.; Hill, C.; Killewald, P.; Kotov, K.; Ling, T. Y.; Rodenburg, M.; Williams, G.] Ohio State Univ, Columbus, OH 43210 USA. [Adam, N.; Berry, E.; Elmer, P.; Gerbaudo, D.; Halyo, V.; Hebda, P.; Hunt, A.; Jones, J.; Laird, E.; Pegna, D. Lopes; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Acosta, J. G.; Huang, X. T.; Lopez, A.; Mendez, H.; Oliveros, S.; Vargas, J. E. Ramirez; Zatserklyaniy, A.] Univ Puerto Rico, Mayaguez, PR 00680 USA. [Alagoz, E.; Barnes, V. E.; Bolla, G.; Borrello, L.; Bortoletto, D.; Everett, A.; Garfinkel, A. F.; Gecse, Z.; Gutay, L.; Hu, Z.; Jones, M.; Koybasi, O.; Kress, M.; Laasanen, A. T.; Leonardo, N.; Liu, C.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Jindal, P.; Parashar, N.] Purdue Univ Calumet, Hammond, IN 46323 USA. [Boulahouache, C.; Cuplov, V.; Ecklund, K. M.; Geurts, F. J. M.; Liu, J. H.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX 77251 USA. [Betchart, B.; Bodek, A.; Chung, Y. S.; Covarelli, R.; De Barbaro, P.; Demina, R.; Eshaq, Y.; Flacher, H.; Garcia-Bellido, A.; Goldenzweig, P.; Gotra, Y.; Han, J.; Harel, A.; Miner, D. C.; Orbaker, D.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.; Yan, M.] Rockefeller Univ, New York, NY 10021 USA. [Atramentov, O.; Barker, A.; Duggan, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hits, D.; Lath, A.; Panwalkar, S.; Patel, R.; Richards, A.; Rose, K.; Schnetzer, S.; Somalwar, S.; Stone, R.; Thomas, S.] Rutgers State Univ, Piscataway, NJ 08854 USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN 37996 USA. [Asaadi, J.; Eusebi, R.; Gilmore, J.; Gurrola, A.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Nguyen, C. N.; Osipenkov, I.; Pivarski, J.; Safonov, A.; Sengupta, S.; Tatarinov, A.; Toback, D.; Weinberger, M.] Texas A&M Univ, College Stn, TX 77843 USA. [Akchurin, N.; Damgov, J.; Jeong, C.; Kovitanggoon, K.; Lee, S. W.; Roh, Y.; Sill, A.; Volobouev, I.; Wigmans, R.; Yazgan, E.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Brownson, E.; Engh, D.; Florez, C.; Gabella, W.; Johns, W.; Kurt, P.; Maguire, C.; Melo, A.; Sheldon, P.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Balazs, M.; Boutle, S.; Buehler, M.; Conetti, S.; Cox, B.; Francis, B.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Yohay, R.] Univ Virginia, Charlottesville, VA 22901 USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Lamichhane, P.; Mattson, M.; Milstene, C.; Sakharov, A.] Wayne State Univ, Detroit, MI 48202 USA. [Anderson, M.; Bachtis, M.; Bellinger, J. N.; Carlsmith, D.; Dasu, S.; Efron, J.; Gray, L.; Grogg, K. S.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Leonard, J.; Loveless, R.; Mohapatra, A.; Reeder, D.; Ross, I.; Savin, A.; Smith, W. H.; Swanson, J.; Weinberg, M.] Univ Wisconsin, Madison, WI 53706 USA. Univ Fed ABC, Santo Andre, Brazil. Suez Canal Univ, Suez, Egypt. Fayoum Univ, Al Fayyum, Egypt. [Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.; Karim, M.] Univ Haute Alsace, Mulhouse, France. [Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Krajczar, K.; Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Rovelli, C.] Univ Roma La Sapienza, Sez Roma, Ist Nazl Fis Nucl, Rome, Italy. [Colafranceschi, S.] Univ Roma La Sapienza, Fac Ingn, Rome, Italy. [Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Martini, L.] Univ Siena, I-53100 Siena, Italy. [Benedetti, D.] Univ Geneva, Geneva, Switzerland. [Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale & Sez, Pisa, Italy. [Bakirci, M. N.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.] Adiyaman Univ, Adiyaman, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Demir, D.] Izmir Inst Technol, Izmir, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Ozkorucuklu, S.] Suleyman Demirel Univ, TR-32200 Isparta, Turkey. [Sonmez, N.] Ege Univ, Izmir, Turkey. [Basso, L.; Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Popescu, S.] Horia Hulubei Natl Inst Phys & Nucl Engn IFIN HIH, Bucharest, Romania. [Lacaprara, S.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Cankocak, K.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Varela, Joao/K-4829-2016; Menasce, Dario Livio/A-2168-2016; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Fassi, Farida/F-3571-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Gerbaudo, Davide/J-4536-2012; Flix, Josep/G-5414-2012; Ozdemir, Kadri/P-8058-2014; Azarkin, Maxim/N-2578-2015; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Haj Ahmad, Wael/E-6738-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Govoni, Pietro/K-9619-2016; Bedoya, Cristina/K-8066-2014; Matorras, Francisco/I-4983-2015; My, Salvatore/I-5160-2015; Muelmenstaedt, Johannes/K-2432-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Arce, Pedro/L-1268-2014; Benussi, Luigi/O-9684-2014; Russ, James/P-3092-2014; Dahms, Torsten/A-8453-2015; Grandi, Claudio/B-5654-2015; Ahmed, Ijaz/E-9144-2015; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; Santoro, Alberto/E-7932-2014; Codispoti, Giuseppe/F-6574-2014; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Calderon, Alicia/K-3658-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; Vogel, Helmut/N-8882-2014; Marinho, Franciole/N-8101-2014; Ragazzi, Stefano/D-2463-2009; Tinoco Mendes, Andre David/D-4314-2011; Mignerey, Alice/D-6623-2011; Ganjour, Serguei/D-8853-2011; Ruiz, Alberto/E-4473-2011; Dudko, Lev/D-7127-2012; Stahl, Achim/E-8846-2011; Hektor, Andi/G-1804-2011; Wulz, Claudia-Elisabeth/H-5657-2011; Chen, Jie/H-6210-2011; Bolton, Tim/A-7951-2012; Yang, Fan/B-2755-2012; Krammer, Manfred/A-6508-2010; Lokhtin, Igor/D-7004-2012; Kodolova, Olga/D-7158-2012; Katkov, Igor/E-2627-2012; Boos, Eduard/D-9748-2012; Snigirev, Alexander/D-8912-2012; Servoli, Leonello/E-6766-2012; Tomei, Thiago/E-7091-2012; Novaes, Sergio/D-3532-2012; Padula, Sandra /G-3560-2012; Fruhwirth, Rudolf/H-2529-2012; Azzi, Patrizia/H-5404-2012; Torassa, Ezio/I-1788-2012; Giacomelli, Paolo/B-8076-2009; Jeitler, Manfred/H-3106-2012; Venturi, Andrea/J-1877-2012; de Jesus Damiao, Dilson/G-6218-2012; Montanari, Alessandro/J-2420-2012; Amapane, Nicola/J-3683-2012; tosi, mia/J-5777-2012; Petrushanko, Sergey/D-6880-2012; Raidal, Martti/F-4436-2012; Della Ricca, Giuseppe/B-6826-2013; Kadastik, Mario/B-7559-2008; Mundim, Luiz/A-1291-2012; Santaolalla, Javier/C-3094-2013; Alves, Gilvan/C-4007-2013; Rolandi, Luigi (Gigi)/E-8563-2013; Zalewski, Piotr/H-7335-2013; Ivanov, Andrew/A-7982-2013; Hill, Christopher/B-5371-2012; Troitsky, Sergey/C-1377-2014; Marlow, Daniel/C-9132-2014; Oguri, Vitor/B-5403-2013; Janssen, Xavier/E-1915-2013 OI Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Varela, Joao/0000-0003-2613-3146; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Lloret Iglesias, Lara/0000-0002-0157-4765; Carrera, Edgar/0000-0002-0857-8507; Sguazzoni, Giacomo/0000-0002-0791-3350; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Fassi, Farida/0000-0002-6423-7213; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Gerbaudo, Davide/0000-0002-4463-0878; Vieira de Castro Ferreira da Silva, Pedro Manuel/0000-0002-5725-041X; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Flix, Josep/0000-0003-2688-8047; Ozdemir, Kadri/0000-0002-0103-1488; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Haj Ahmad, Wael/0000-0003-1491-0446; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Govoni, Pietro/0000-0002-0227-1301; Bedoya, Cristina/0000-0001-8057-9152; Matorras, Francisco/0000-0003-4295-5668; My, Salvatore/0000-0002-9938-2680; Muelmenstaedt, Johannes/0000-0003-1105-6678; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Arce, Pedro/0000-0003-3009-0484; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Codispoti, Giuseppe/0000-0003-0217-7021; Cerrada, Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Vogel, Helmut/0000-0002-6109-3023; Marinho, Franciole/0000-0002-7327-0349; Ragazzi, Stefano/0000-0001-8219-2074; Tinoco Mendes, Andre David/0000-0001-5854-7699; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Stahl, Achim/0000-0002-8369-7506; Hektor, Andi/0000-0001-7873-8118; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Krammer, Manfred/0000-0003-2257-7751; Katkov, Igor/0000-0003-3064-0466; Servoli, Leonello/0000-0003-1725-9185; Tomei, Thiago/0000-0002-1809-5226; Novaes, Sergio/0000-0003-0471-8549; Azzi, Patrizia/0000-0002-3129-828X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Montanari, Alessandro/0000-0003-2748-6373; Amapane, Nicola/0000-0001-9449-2509; Della Ricca, Giuseppe/0000-0003-2831-6982; Mundim, Luiz/0000-0001-9964-7805; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Ivanov, Andrew/0000-0002-9270-5643; Hill, Christopher/0000-0003-0059-0779; Troitsky, Sergey/0000-0001-6917-6600; FU FMSR (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences (Estonia); NICPB (Estonia); Academy of Finland (Finland); ME (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Korea); WCU (Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MST (Russia); MAE (Russia); MSTD (Serbia); MICINN (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK (Turkey); TAEK (Turkey); STFC (United Kingdom); DOE (U.S.); NSF (U.S.) FX We wish to congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine. We thank the technical and administrative staff at CERN and other CMS institutes, and acknowledge support from: FMSR (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences and NICPB (Estonia); Academy of Finland, ME, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MST and MAE (Russia); MSTD (Serbia); MICINN and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK and TAEK (Turkey); STFC (United Kingdom); DOE and NSF (U.S.). NR 28 TC 44 Z9 44 U1 3 U2 48 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 18 PY 2011 VL 106 IS 20 AR 201804 DI 10.1103/PhysRevLett.106.201804 PG 14 WC Physics, Multidisciplinary SC Physics GA 765SV UT WOS:000290729800003 PM 21668222 ER PT J AU Pan, W Masuhara, N Sullivan, NS Baldwin, KW West, KW Pfeiffer, LN Tsui, DC AF Pan, W. Masuhara, N. Sullivan, N. S. Baldwin, K. W. West, K. W. Pfeiffer, L. N. Tsui, D. C. TI Impact of Disorder on the 5/2 Fractional Quantum Hall State SO PHYSICAL REVIEW LETTERS LA English DT Article ID FILLED LANDAU-LEVEL; 2-DIMENSIONAL ELECTRON; GROUND-STATE; LOCALIZATION; LIMIT AB We compare the energy gap of the nu = 5/2 fractional quantum Hall effect state obtained in conventional high mobility modulation-doped quantum-well samples with those obtained in high quality GaAs transistors (heterojunction insulated gate field-effect transistors). We are able to identify the different roles that long-range and short-range disorders play in the 5/2 state and observe that the long-range potential fluctuations are more detrimental to the strength of the 5/2 state than short-range potential disorder. C1 [Pan, W.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Masuhara, N.; Sullivan, N. S.] Univ Florida, Gainesville, FL 32611 USA. [Masuhara, N.; Sullivan, N. S.] Natl High Magnet Field Lab, Gainesville, FL 32611 USA. [Baldwin, K. W.; West, K. W.; Pfeiffer, L. N.; Tsui, D. C.] Princeton Univ, Princeton, NJ 08544 USA. RP Pan, W (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. FU Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, U.S. Department of Energy; Laboratory Directed Research and Development fund at Sandia; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; DOE [DE-FG-02- 98ER45683]; NSF [DMR-0084173]; State of Florida FX We thank Dr. Z. G. Ge for his assistance at the beginning stage of this project. We would like to thank Dr. Muraki and Dr. Gamez for discussions. This work was supported by Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, U.S. Department of Energy and by a Laboratory Directed Research and Development fund at Sandia. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. Work at Princeton was supported on the DOE Grant No. DE-FG-02- 98ER45683. A portion of this work was carried out at the high B/T facility of the National High Magnetic Field Laboratory, which is supported by NSF Cooperative Agreement No. DMR-0084173, by the State of Florida, and by the DOE. NR 37 TC 33 Z9 33 U1 2 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 18 PY 2011 VL 106 IS 20 AR 206806 DI 10.1103/PhysRevLett.106.206806 PG 4 WC Physics, Multidisciplinary SC Physics GA 765SV UT WOS:000290729800004 ER PT J AU Gutenkunst, RN Coombs, D Starr, T Dustin, ML Goldstein, B AF Gutenkunst, Ryan N. Coombs, Daniel Starr, Toby Dustin, Michael L. Goldstein, Byron TI A Biophysical Model of Cell Adhesion Mediated by Immunoadhesin Drugs and Antibodies SO PLOS ONE LA English DT Article ID 2-DIMENSIONAL DISSOCIATION-CONSTANT; FC-GAMMA-RIII; T-CELLS; MONOCLONAL-ANTIBODIES; IMMUNOGLOBULIN-G; SHEAR-FLOW; RECEPTORS; CD2; AFFINITY; CYTOTOXICITY AB A promising direction in drug development is to exploit the ability of natural killer cells to kill antibody-labeled target cells. Monoclonal antibodies and drugs designed to elicit this effect typically bind cell-surface epitopes that are overexpressed on target cells but also present on other cells. Thus it is important to understand adhesion of cells by antibodies and similar molecules. We present an equilibrium model of such adhesion, incorporating heterogeneity in target cell epitope density, nonspecific adhesion forces, and epitope immobility. We compare with experiments on the adhesion of Jurkat T cells to bilayers containing the relevant natural killer cell receptor, with adhesion mediated by the drug alefacept. We show that a model in which all target cell epitopes are mobile and available is inconsistent with the data, suggesting that more complex mechanisms are at work. We hypothesize that the immobile epitope fraction may change with cell adhesion, and we find that such a model is more consistent with the data, although discrepancies remain. We also quantitatively describe the parameter space in which binding occurs. Our model elaborates substantially on previous work, and our results offer guidance for the refinement of therapeutic immunoadhesins. Furthermore, our comparison with data from Jurkat T cells also points toward mechanisms relating epitope immobility to cell adhesion. C1 [Gutenkunst, Ryan N.] Univ Arizona, Dept Mol & Cellular Biol, Tucson, AZ 85721 USA. [Coombs, Daniel] Univ British Columbia, Dept Math, Vancouver, BC, Canada. [Coombs, Daniel] Univ British Columbia, Inst Appl Math, Vancouver, BC V5Z 1M9, Canada. [Starr, Toby; Dustin, Michael L.] NYU, Sch Med, Dept Pathol, New York, NY USA. [Starr, Toby; Dustin, Michael L.] Skirball Inst Biomol Med, Program Mol Pathogenesis, New York, NY USA. [Goldstein, Byron] Los Alamos Natl Lab, Div Theoret, Theoret Biol & Biophys Grp, Los Alamos, NM USA. RP Gutenkunst, RN (reprint author), Univ Arizona, Dept Mol & Cellular Biol, Tucson, AZ 85721 USA. EM ryan.gutenkunst@arizona.edu OI Coombs, Daniel/0000-0002-8038-6278; Dustin, Michael/0000-0003-4983-6389 FU Department of Energy [W-7405-ENG-36]; National Institutes of Health [R37-GM035556, R56-AI44931, P30-6M092391]; National Science and Engineering Research Council; Mathematics of Information Technology and Complex Systems National Centre of Excellence FX This work was supported by the Department of Energy through contract W-7405-ENG-36 and the National Institutes of Health through grants R37-GM035556 and R56-AI44931 and P30-6M092391. Further support was provided by the National Science and Engineering Research Council and the Mathematics of Information Technology and Complex Systems National Centre of Excellence. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 40 TC 1 Z9 1 U1 0 U2 2 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 18 PY 2011 VL 6 IS 5 AR e19701 DI 10.1371/journal.pone.0019701 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 765PE UT WOS:000290720200027 PM 21629715 ER PT J AU Skennerton, CT Angly, FE Breitbart, M Bragg, L He, SM McMahon, KD Hugenholtz, P Tyson, GW AF Skennerton, Connor T. Angly, Florent E. Breitbart, Mya Bragg, Lauren He, Shaomei McMahon, Katherine D. Hugenholtz, Philip Tyson, Gene W. TI Phage Encoded H-NS: A Potential Achilles Heel in the Bacterial Defence System SO PLOS ONE LA English DT Article ID BIOLOGICAL PHOSPHORUS REMOVAL; STREPTOCOCCUS-THERMOPHILUS BACTERIOPHAGES; NUCLEOID-ASSOCIATED PROTEIN; ESCHERICHIA-COLI; GENE-EXPRESSION; DNA; GENOME; VIRUSES; TRANSCRIPTION; COMMUNITY AB The relationship between phage and their microbial hosts is difficult to elucidate in complex natural ecosystems. Engineered systems performing enhanced biological phosphorus removal (EBPR), offer stable, lower complexity communities for studying phage-host interactions. Here, metagenomic data from an EBPR reactor dominated by Candidatus Accumulibacter phosphatis (CAP), led to the recovery of three complete and six partial phage genomes. Heat-stable nucleoid structuring (H-NS) protein, a global transcriptional repressor in bacteria, was identified in one of the complete phage genomes (EPV1), and was most similar to a homolog in CAP. We infer that EPV1 is a CAP-specific phage and has the potential to repress up to 6% of host genes based on the presence of putative H-NS binding sites in the CAP genome. These genes include CRISPR associated proteins and a Type III restriction-modification system, which are key host defense mechanisms against phage infection. Further, EPV1 was the only member of the phage community found in an EBPR microbial metagenome collected seven months prior. We propose that EPV1 laterally acquired H-NS from CAP providing it with a means to reduce bacterial defenses, a selective advantage over other phage in the EBPR system. Phage encoded H-NS could constitute a previously unrecognized weapon in the phage-host arms race. C1 [Skennerton, Connor T.; Angly, Florent E.; Bragg, Lauren; Tyson, Gene W.] Univ Queensland, Adv Water Management Ctr, St Lucia, Qld, Australia. [Skennerton, Connor T.; Angly, Florent E.; Bragg, Lauren; Hugenholtz, Philip; Tyson, Gene W.] Univ Queensland, Australian Ctr Ecogenom, Sch Chem & Mol Biosci, St Lucia, Qld, Australia. [Skennerton, Connor T.; Angly, Florent E.; Bragg, Lauren; Hugenholtz, Philip; Tyson, Gene W.] Univ Queensland, Inst Mol Biosci, St Lucia, Qld, Australia. [Breitbart, Mya] Univ S Florida, Coll Marine Sci, St Petersburg, FL 33701 USA. [Bragg, Lauren] CSIRO Math Informat & Stat, St Lucia, Qld, Australia. [He, Shaomei] Joint Genome Inst, Dept Energy, Walnut Creek, CA USA. [He, Shaomei] Univ Calif Berkeley, Energy Biosci Inst, Berkeley, CA 94720 USA. [McMahon, Katherine D.] Univ Wisconsin, Dept Civil & Environm Engn, Madison, WI 53706 USA. RP Skennerton, CT (reprint author), Univ Queensland, Adv Water Management Ctr, St Lucia, Qld, Australia. EM g.tyson@uq.edu.au RI Angly, Florent/A-7717-2011; Hugenholtz, Philip/G-9608-2011; Bragg, Lauren/B-8554-2009; Breitbart, Mya/B-1366-2009; McMahon, Katherine/I-3651-2012; Tyson, Gene/C-6558-2013; OI Angly, Florent/0000-0002-8999-0738; Breitbart, Mya/0000-0003-3210-2899; Skennerton, Connor/0000-0003-1320-4873; McMahon, Katherine D./0000-0002-7038-026X FU Australian Research Council [DP1093175]; US National Science Foundation [BES-0332136] FX This work was supported by the Australian Research Council (www.arc.gov.au/), 265 grant DP1093175, and US National Science Foundation (www.nsf.gov/) grant BES-0332136. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 56 TC 17 Z9 17 U1 2 U2 16 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 18 PY 2011 VL 6 IS 5 AR e20095 DI 10.1371/journal.pone.0020095 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 765PE UT WOS:000290720200063 PM 21625595 ER PT J AU Maiti, A AF Maiti, A. TI Energetic stability of hydrogen-chemisorbed carbon nanotube structures SO CHEMICAL PHYSICS LETTERS LA English DT Article ID STORAGE; SPILLOVER; SURFACE AB To optimize the performance of carbon nanotubes in the area of hydrogen storage we explore stable structures that can form upon hydrogenation. Through free energy calculations using first-principles DFT we find that at room temperature the trans-hydride structure, i.e., one in which H-atoms chemisorbed on nearest-neighbor sites alternate between outside and inside of the nanotube is the most stable structure under moderate hydrogen dosage for tubes with diameter > 1.2 nm. Such structures are energetically stable with respect to recombination into H(2) or decomposition into hydrocarbons like benzene or ethylene. We also find that the IR spectrum of the trans-hydrides display striking dependence on nanotube chirality. (C) 2011 Elsevier B. V. All rights reserved. C1 Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Maiti, A (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM amaiti@llnl.gov FU US DOE, Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the US DOE by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 22 TC 9 Z9 9 U1 1 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD MAY 18 PY 2011 VL 508 IS 1-3 BP 107 EP 110 DI 10.1016/j.cplett.2011.04.020 PG 4 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 760CA UT WOS:000290298200022 ER PT J AU Alaboson, JMP Wang, QH Kellar, JA Park, J Elam, JW Pellin, MJ Hersam, MC AF Alaboson, Justice M. P. Wang, Qing Hua Kellar, Joshua A. Park, Joohee Elam, Jeffrey W. Pellin, Michael J. Hersam, Mark C. TI Conductive Atomic Force Microscope Nanopatterning of Epitaxial Graphene on SiC(0001) in Ambient Conditions SO ADVANCED MATERIALS LA English DT Article ID SCANNED PROBE OXIDATION; HYDROGEN-PASSIVATED SILICON; FIELD-INDUCED OXIDATION; INDUCED LOCAL OXIDATION; INERT ORGANIC-SOLVENTS; GRAPHITE OXIDE; SPACE-CHARGE; KINETICS; MECHANISM; MODEL AB Conductive atomic force microscope (cAFM) nanopatterning is demonstrated on epitaxial graphene on SiC (0001) under ambient conditions. Nanopatterning kinetics and chemistry suggest that ambient cAFM nanopatterning induces local oxidization with the surface, interface, and bulk layers of epitaxial graphene on SiC (0001) playing distinct roles in the depth profile of the final nanopatterned structure. C1 [Alaboson, Justice M. P.; Wang, Qing Hua; Kellar, Joshua A.; Park, Joohee; Hersam, Mark C.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Alaboson, Justice M. P.; Pellin, Michael J.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Elam, Jeffrey W.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. RP Hersam, MC (reprint author), Northwestern Univ, Dept Mat Sci & Engn, 2220 Campus Dr, Evanston, IL 60208 USA. EM m-hersam@northwestern.edu RI Pellin, Michael/B-5897-2008; Hersam, Mark/B-6739-2009; Wang, Qing Hua/G-1596-2016 OI Pellin, Michael/0000-0002-8149-9768; Wang, Qing Hua/0000-0002-7982-7275 FU National Science Foundation [EEC-0647560, DMR-0520513]; Army Research Office [ARO W911NF-05-1-0177]; Argonne National Laboratory (ANL); U.S. Department of Energy Office of Science Laboratory [DE-AC02-06CH11357] FX This work was supported by the National Science Foundation (Award Numbers EEC-0647560 and DMR-0520513), the Army Research Office (Award Number ARO W911NF-05-1-0177), and Argonne National Laboratory (ANL). ANL is a U.S. Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. The authors also thank Joseph Lyding for use of his STM control software. NR 45 TC 22 Z9 22 U1 4 U2 90 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA PO BOX 10 11 61, D-69451 WEINHEIM, GERMANY SN 0935-9648 J9 ADV MATER JI Adv. Mater. PD MAY 17 PY 2011 VL 23 IS 19 BP 2181 EP + DI 10.1002/adma.201100367 PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 773GR UT WOS:000291295500003 PM 21381135 ER PT J AU Shao, M Yan, L Pan, HP Ivanov, I Hu, B AF Shao, Ming Yan, Liang Pan, Haiping Ivanov, Ilia Hu, Bin TI Giant Magnetic Field Effects on Electroluminescence in Electrochemical Cells SO ADVANCED MATERIALS LA English DT Article ID ELECTROGENERATED CHEMILUMINESCENCE; ANTHRACENE; ECL; ANNIHILATION; GENERATION; REDUCTION; CRYSTALS; DEVICES; CATION AB Giant magnetic field effects on the electroluminescence intensity with a magnitude of 400% are demonstrated by using Lorentz force effects in an electrochemical co-reaction with planar electrodes. A magnetic field increases the ion penetration in the diffusion layer in the electrochemical reaction through Lorentz force effects and greatly enhances the electro-generated chemiluminescence intensity (ECL), leading to giant magnetic field effects in liquid states. C1 [Shao, Ming; Yan, Liang; Hu, Bin] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Pan, Haiping] Huazhong Univ Sci & Technol, Wuhan 430074, Peoples R China. [Ivanov, Ilia] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Hu, B (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM bhu@utk.edu RI Yan, Liang/H-6471-2011; Shao, Ming/A-6240-2013; Hu, Bin/A-2954-2015; ivanov, ilia/D-3402-2015 OI Yan, Liang/0000-0003-4122-7466; Hu, Bin/0000-0002-1573-7625; ivanov, ilia/0000-0002-6726-2502 FU National Science Foundation [ECCS-0644945]; Center for Materials Processing at the University of Tennessee; Division of Scientific User Facilities, U.S. Department of Energy [CNMS2009-055] FX This research was supported by the National Science Foundation (ECCS-0644945) and Center for Materials Processing at the University of Tennessee. This research was partially conducted at the Center for Nanophase Materials Sciences based on user project (CNMS2009-055), which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, U.S. Department of Energy. NR 30 TC 16 Z9 16 U1 4 U2 50 PU WILEY-BLACKWELL PI MALDEN PA COMMERCE PLACE, 350 MAIN ST, MALDEN 02148, MA USA SN 0935-9648 J9 ADV MATER JI Adv. Mater. PD MAY 17 PY 2011 VL 23 IS 19 BP 2216 EP + DI 10.1002/adma.201100193 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 773GR UT WOS:000291295500010 PM 21462373 ER PT J AU Campisi, J AF Campisi, Judith TI Parsing p53 Transactivation SO DEVELOPMENTAL CELL LA English DT Editorial Material ID TUMOR SUPPRESSION; DNA-DAMAGE; MICE AB Two functions of p53 are undisputed. Biologically, p53 is a potent tumor suppressor, whereas biochemically, it is a robust transcriptional activator of numerous target genes. Are these biological and biochemical functions of p53 related? The surprising answer, recently reported by Brady et al. (2011) in Cell, is minimally. C1 [Campisi, Judith] Buck Inst Res Aging, Novato, CA 94945 USA. [Campisi, Judith] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Campisi, J (reprint author), Buck Inst Res Aging, 8001 Redwood Blvd, Novato, CA 94945 USA. EM jcampisi@buckinstitute.org NR 8 TC 1 Z9 1 U1 0 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1534-5807 J9 DEV CELL JI Dev. Cell PD MAY 17 PY 2011 VL 20 IS 5 BP 573 EP 574 DI 10.1016/j.devcel.2011.04.015 PG 2 WC Cell Biology; Developmental Biology SC Cell Biology; Developmental Biology GA 771FC UT WOS:000291141600001 PM 21571212 ER PT J AU Anderson, NL Vedula, RP Schultz, PA Van Ginhoven, RM Strachan, A AF Anderson, Nathan L. Vedula, Ravi Pramod Schultz, Peter A. Van Ginhoven, R. M. Strachan, Alejandro TI First-Principles Investigation of Low Energy E ' Center Precursors in Amorphous Silica SO PHYSICAL REVIEW LETTERS LA English DT Article ID OXYGEN; OXIDE; DEFECTS; GLASSES AB We show that oxygen vacancies are not necessary for the formation of E' centers in amorphous SiO(2) and that a single O deficiency can lead to two charge traps. Employing molecular dynamics with a reactive potential and density functional theory, we generate an ensemble of stoichiometric and oxygen-deficient amorphous SiO(2) atomic structures and identify low-energy network defects. Three-coordinated Si atoms appear in several low-energy defects both in stoichiometric and O-deficient samples where, in addition to the neutral oxygen vacancy, they appear as isolated defects. C1 [Anderson, Nathan L.; Strachan, Alejandro] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. [Vedula, Ravi Pramod] Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47907 USA. [Schultz, Peter A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Van Ginhoven, R. M.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Anderson, NL (reprint author), Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. FU U.S. DOE's National Nuclear Security Administration [DE-FC52-08NA28617, DE-AC04-94AL85000] FX We thank H. P. Hjalmarson and A. H. Edwards for useful discussions. This work was partly supported by Purdue's PRISM Center funded by the U.S. DOE's National Nuclear Security Administration under Contract No. DE-FC52-08NA28617. Computational resources of nanoHUB.org are gratefully acknowledged. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin company, for the U.S. DOE's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 21 TC 22 Z9 22 U1 1 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 17 PY 2011 VL 106 IS 20 AR 206402 DI 10.1103/PhysRevLett.106.206402 PG 4 WC Physics, Multidisciplinary SC Physics GA 765SR UT WOS:000290729400009 PM 21668246 ER PT J AU Berger, EL Cao, QH Chen, CR Li, CS Zhang, H AF Berger, Edmond L. Cao, Qing-Hong Chen, Chuan-Ren Li, Chong Sheng Zhang, Hao TI Top Quark Forward-Backward Asymmetry and Same-Sign Top Quark Pairs SO PHYSICAL REVIEW LETTERS LA English DT Article ID CHIRAL COLOR SYMMETRY; HADRON COLLIDERS; G'-BOSON; LHC; TEVATRON; PHYSICS AB The top quark forward-backward asymmetry measured at the Tevatron collider shows a large deviation from standard model expectations. Among possible interpretations, a nonuniversal Z' model is of particular interest as it naturally predicts a top quark in the forward region of large rapidity. To reproduce the size of the asymmetry, the couplings of the Z' to standard model quarks must be large, inevitably leading to copious production of same-sign top quark pairs at the energies of the Large Hadron Collider (LHC). We explore the discovery potential for tt and ttj production in early LHC experiments at 7-8 TeV and conclude that if no tt signal is observed with 1 fb(-1) of integrated luminosity, then a nonuniversal Z' alone cannot explain the Tevatron forward-backward asymmetry. C1 [Berger, Edmond L.; Cao, Qing-Hong] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Cao, Qing-Hong] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Chen, Chuan-Ren] Univ Tokyo, Inst Phys & Math Universe, Chiba 2778568, Japan. [Cao, Qing-Hong; Li, Chong Sheng; Zhang, Hao] Peking Univ, Dept Phys, Beijing 100871, Peoples R China. [Cao, Qing-Hong; Li, Chong Sheng; Zhang, Hao] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. RP Berger, EL (reprint author), Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. EM berger@anl.gov; caoq@hep.anl.gov; chuan-ren.chen@ipmu.jp; csli@pku.edu.cn; haozhang.pku@pku.edu.cn RI ZHANG, Hao/G-6430-2015 FU U.S. DOE [DE-AC02-06CH11357]; Argonne National Laboratory; University of Chicago Joint Theory Institute [03921-07-137]; World Premier International Center Initiative, MEXT, Japan; National Natural Science Foundation of China [11021092, 10975004] FX The work by E. L. B. and Q. H. C. is supported in part by the U.S. DOE under Contract No. DE-AC02-06CH11357. Q. H. C. is also supported in part by the Argonne National Laboratory and University of Chicago Joint Theory Institute Grant 03921-07-137. C. R. C. is supported by World Premier International Center Initiative (WPI Program), MEXT, Japan. C. S. L. and H. Z. are supported in part by the National Natural Science Foundation of China, under Grants No. 11021092 and No. 10975004. Q. H. C. thanks Shanghai Jiaotong University for hospitality where part of this work was done. E. L. B. and C. R. C. also thank NCTS in Taiwan for hospitality where part of this work was done. NR 55 TC 78 Z9 78 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 17 PY 2011 VL 106 IS 20 AR 201801 DI 10.1103/PhysRevLett.106.201801 PG 4 WC Physics, Multidisciplinary SC Physics GA 765SR UT WOS:000290729400003 PM 21668219 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hammer, J Hansel, S Hartl, C Hoch, M Hormann, N Hrubec, J Jeitler, M Kasieczka, G Kiesenhofer, W Krammer, M Liko, D Mikulec, I Pernicka, M Rohringer, H Schofbeck, R Strauss, J Taurok, A Teischinger, F Wagner, P Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Benucci, L Cerny, K DeWolf, EA Janssen, X Maes, T Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Beauceron, S Blekman, F Blyweert, S D'Hondt, J Devroede, O Suarez, RG Kalogeropoulos, A Maes, J Maes, M Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Charaf, O Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hammad, GH Hreus, T Marage, PE Thomas, L Velde, CV Vanlaer, P Wickens, J Adler, V Costantini, S Grunewald, M Klein, B Marinov, A Mccartin, J Ryckbosch, D Thyssen, F Tytgat, M Vanelderen, L Verwilligen, P Walsh, S Zaganidis, N Basegmez, S Bruno, G Caudron, J Ceard, L De Jeneret, JD Delaere, C Demin, P Favart, D Giammanco, A Gregoire, G Hollar, J Lemaitre, V Liao, J Militaru, O Ovyn, S Pagano, D Pin, A Piotrzkowski, K Schul, N Beliy, N Caebergs, T Daubie, E Alves, GA Damiao, DJ Pol, ME Souza, MHG Carvalho, W Da Costa, EM Martins, CD De Souza, SF Mundim, L Nogima, H Oguri, V Da Silva, WLP Santoro, A Do Amaral, SMS Sznajder, A De Araujo, FTD Dias, FA Dias, MAF Tomei, TRFP Gregores, EM Marinho, F Novaes, SF Padula, SS Darmenov, N Dimitrov, L Genchev, V Iaydjiev, P Piperov, S Rodozov, M Stoykova, S Sultanov, G Tcholakov, V Trayanov, R Vankov, I Dyulendarova, M Hadjiiska, R Kozhuharov, V Litov, L Marinova, E Mateev, M Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Wang, J Wang, J Wang, X Wang, Z Xu, M Yang, M Zang, J Zhang, Z Ban, Y Guo, S Guo, Y Li, W Mao, Y Qian, SJ Teng, H Zhang, L Zhu, B Zou, W Cabrera, A Moreno, BG Rios, AAO Oliveros, AFO Sanabria, JC Godinovic, N Lelas, D Lelas, K Plestina, R Polic, D Puljak, I Antunovic, Z Dzelalija, M Brigljevic, V Duric, S Kadija, K Morovic, S Attikis, A Galanti, M Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Assran, Y Mahmoud, MA Hektor, A Kadastik, M Kannike, K Ntel, MM Raidal, M Rebane, L Azzolini, V Eerola, P Czellar, S Harkonen, J Heikkinen, A Karimaki, V Kinnunen, R Klem, J Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Tuominen, E Tuominiemi, J Tuovinen, E Ungaro, D Wendland, L Banzuzi, K Korpela, A Tuuva, T Sillou, D Besancon, M Choudhury, S Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Gentit, FX Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Marionneau, M Millischer, L Rander, J Rosowsky, A Shreyber, I Titov, M Verrecchia, P Baffioni, S Beaudette, F Bianchini, L Bluj, M Broutin, C Busson, P Charlot, C Dahms, T Dobrzynski, L de Cassagnac, RG Haguenauer, M Mine, P Mironov, C Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Thiebaux, C Wyslouch, B Zabi, A Agram, JL Andrea, J Besson, A Bloch, D Bodin, D Brom, JM Cardaci, M Chabert, EC Collard, C Conte, E Drouhin, F Ferro, C Fontaine, JC Gele, D Goerlach, U Greder, S Juillot, P Karim, M Le Bihan, AC Mikami, Y Van Hove, P Fassi, F Mercier, D Baty, C Beaupere, N Bedjidian, M Bondu, O Boudoul, G Boumediene, D Brun, H Chanon, N Chierici, R Contardo, D Depasse, P El Mamouni, H Falkiewicz, A Fay, J Gascon, S Ille, B Kurca, T Le Grand, T Lethuillier, M Mirabito, L Perries, S Sordini, V Tosi, S Tschudi, Y Verdier, P Xiao, H Megrelidze, L Roinishvili, V Lomidze, D Anagnostou, G Edelhoff, M Feld, L Heracleous, N Hindrichs, O Jussen, R Klein, K Merz, J Mohr, N Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Weber, M Wittmer, B Ata, M Bender, W Erdmann, M Frangenheim, J Hebbeker, T Hinzmann, A Hoepfner, K Hof, C Klimkovich, T Klingebiel, D Kreuzer, P Lanske, D Magass, C Masetti, G Merschmeyer, M Meyer, A Papacz, P Pieta, H Reithler, H Schmitz, SA Sonnenschein, L Steggemann, J Teyssier, D Bontenackels, M Davids, M Duda, M Flugge, G Geenen, H Giffels, M Ahmad, WH Heydhausen, D Kress, T Kuessel, Y Linn, A Nowack, A Perchalla, L Pooth, O Rennefeld, J Sauerland, P Stahl, A Thomas, M Tornier, D Zoeller, MH Martin, MA Behrenhoff, W Behrens, U Bergholz, M Borras, K Cakir, A Campbell, A Castro, E Dammann, D Eckerlin, G Eckstein, D Flossdorf, A Flucke, G Geiser, A Glushkov, I Hauk, J Jung, H Kasemann, M Katkov, I Katsas, P Kleinwort, C Kluge, H Knutsson, A Krucker, D Kuznetsova, E Lange, W Lohmann, W Mankel, R Marienfeld, M Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Olzem, J Parenti, A Raspereza, A Raval, A Schmidt, R Schoerner-Sadenius, T Sen, N Stein, M Tomaszewska, J Volyanskyy, D Walsh, R Wissing, C Autermann, C Bobrovskyi, S Draeger, J Enderle, H Gebbert, U Kaschube, K Kaussen, G Klanner, R Lange, J Mura, B Naumann-Emme, S Nowak, F Pietsch, N Sander, C Schettler, H Schleper, P Schroder, M Schum, T Schwandt, J Srivastava, AK Stadie, H Steinbruck, G Thomsen, J Wolf, R Barth, C Bauer, J Buege, V Chwalek, T De Boer, W Dierlamm, A Dirkes, G Feindt, M Gruschke, J Hackstein, C Hartmann, F Heindl, SM Heinrich, M Held, H Hoffmann, KH Honc, S Kuhr, T Martschei, D Mueller, S Muller, T Niegel, M Oberst, O Oehler, A Ott, J Peiffer, T Piparo, D Quast, G Rabbertz, K Ratnikov, F Renz, M Saout, C Scheurer, A Schieferdecker, P Schilling, FP Schott, G Simonis, HJ Stober, FM Troendle, D Wagner-Kuhr, J Zeise, M Zhukov, V Ziebarth, EB Daskalakis, G Geralis, T Kesisoglou, S Kyriakis, A Loukas, D Manolakos, I Markou, A Markou, C Mavrommatis, C Ntomari, E Petrakou, E Gouskos, L Mertzimekis, TJ Panagiotou, A Evangelou, I Foudas, C Kokkas, P Manthos, N Papadopoulos, I Patras, V Triantis, FA Aranyi, A Bencze, G Boldizsar, L Debreczeni, G Hajdu, C Horvath, D Kapusi, A Krajczar, K Laszlo, A Sikler, F Vesztergombi, G Beni, N Molnar, J Palinkas, J Szillasi, Z Veszpremi, V Raics, P Trocsanyi, ZL Ujvari, B Bansal, S Beri, SB Bhatnagar, V Dhingra, N Gupta, R Jindal, M Kaur, M Kohli, JM Mehta, MZ Nishu, N Saini, LK Sharma, A Singh, AP Singh, JB Singh, SP Ahuja, S Bhattacharya, S Choudhary, BC Gupta, P Jain, S Jain, S Kumar, A Shivpuri, RK Choudhury, RK Dutta, D Kailas, S Kataria, SK Mohanty, AK Pant, LM Shukla, P Aziz, T Guchait, M Gurtu, A Maity, M Majumder, D Majumder, G Mazumdar, K Mohanty, GB Saha, A Sudhakar, K Wickramage, N Banerjee, S Dugad, S Mondal, NK Arfaei, H Bakhshiansohi, H Etesami, SM Fahim, A Hashemi, M Jafari, A Khakzad, M Mohammadi, A Najafabadi, MM Mehdiabadi, SP Safarzadeh, B Zeinali, M Abbrescia, M Barbone, L Calabria, C Colaleo, A Creanza, D De Filippis, N De Palma, M Dimitrov, A Fiore, L Iaselli, G Lusito, L Maggi, G Maggi, M Manna, N Marangelli, B My, S Nuzzo, S Pacifico, N 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Ciesielski, R. Demortier, L. Goulianos, K. Lungu, G. Mesropian, C. Yan, M. Atramentov, O. Barker, A. Duggan, D. Gershtein, Y. Gray, R. Halkiadakis, E. Hidas, D. Hits, D. Lath, A. Panwalkar, S. Patel, R. Richards, A. Rose, K. Schnetzer, S. Somalwar, S. Stone, R. Thomas, S. Cerizza, G. Hollingsworth, M. Spanier, S. Yang, Z. C. York, A. Asaadi, J. Eusebi, R. Gilmore, J. Gurrola, A. Kamon, T. Khotilovich, V. Montalvo, R. Nguyen, C. N. Osipenkov, I. Pivarski, J. Safonov, A. Sengupta, S. Tatarinov, A. Toback, D. Weinberger, M. Akchurin, N. Bardak, C. Damgov, J. Jeong, C. Kovitanggoon, K. Lee, S. W. Mane, P. Roh, Y. Sill, A. Volobouev, I. Wigmans, R. Yazgan, E. Appelt, E. Brownson, E. Engh, D. Florez, C. Gabella, W. Johns, W. Kurt, P. Maguire, C. Melo, A. Sheldon, P. Tuo, S. Velkovska, J. Arenton, M. W. Balazs, M. Boutle, S. Buehler, M. Conetti, S. Cox, B. Francis, B. Hirosky, R. Ledovskoy, A. Lin, C. Neu, C. Yohay, R. Gollapinni, S. Harr, R. Karchin, P. E. Lamichhane, P. Mattson, M. Ne, C. Milste Sakharov, A. Anderson, M. Bachtis, M. Bellinger, J. N. Carlsmith, D. Dasu, S. Efron, J. Gray, L. Grogg, K. S. Grothe, M. Hall-Wilton, R. Herndon, M. Klabbers, P. Klukas, J. Lanaro, A. Lazaridis, C. Leonard, J. Loveless, R. Mohapatra, A. Reeder, D. Ross, I. Savin, A. Smith, W. H. Swanson, J. Weinberg, M. CA CMS Collaboration TI Search for Pair Production of First-Generation Scalar Leptoquarks in pp Collisions at root s=7 TeV SO PHYSICAL REVIEW LETTERS LA English DT Article AB A search for pair production of first-generation scalar leptoquarks is performed in the final state containing two electrons and two jets using proton-proton collision data at root s = 7 TeV. The data sample used corresponds to an integrated luminosity of 33 pb(-1) collected with the CMS detector at the CERN LHC. The number of observed events is in good agreement with the predictions for the standard model background processes, and an upper limit is set on the leptoquark pair production cross section times beta(2) as a function of the leptoquark mass, where beta is the branching fraction of the leptoquark decay to an electron and a quark. A 95% confidence level lower limit is set on the mass of a first-generation scalar leptoquark at 384 GeV for beta = 1, which is the most stringent direct limit to date. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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[Czellar, S.; Harkonen, J.; Heikkinen, A.; Karimaki, V.; Kinnunen, R.; Klem, J.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Ungaro, D.; Wendland, L.; Drozdetskiy, A.] Helsinki Inst Phys, Helsinki, Finland. [Banzuzi, K.; Korpela, A.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Sillou, D.] CNRS, IN2P3, Lab Annecy Le Vieux Phys Particules, Annecy Le Vieux, France. [Besancon, M.; Choudhury, S.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Ferri, F.; Ganjour, S.; Gentit, F. X.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Marionneau, M.; Millischer, L.; Rander, J.; Rosowsky, A.; Shreyber, I.; Titov, M.; Verrecchia, P.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Plestina, R.; Baffioni, S.; Beaudette, F.; Bianchini, L.; Bluj, M.; Broutin, C.; Busson, P.; Charlot, C.; Dahms, T.; Dobrzynski, L.; de Cassagnac, R. 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[Baty, C.; Beaupere, N.; Bedjidian, M.; Bondu, O.; Boudoul, G.; Boumediene, D.; Brun, H.; Chanon, N.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Falkiewicz, A.; Fay, J.; Gascon, S.; Ille, B.; Kurca, T.; Le Grand, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Sordini, V.; Tosi, S.; Tschudi, Y.; Verdier, P.; Xiao, H.] Univ Lyon 1, CNRS, IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Megrelidze, L.; Roinishvili, V.] Georgian Acad Sci, E Andronikashvili Inst Phys, GE-380060 Tbilisi, Rep of Georgia. [Lomidze, D.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Anagnostou, G.; Edelhoff, M.; Feld, L.; Heracleous, N.; Hindrichs, O.; Jussen, R.; Klein, K.; Merz, J.; Mohr, N.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Weber, M.; Wittmer, B.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Bender, W.; Erdmann, M.; Frangenheim, J.; Hebbeker, T.; Hinzmann, A.; Hoepfner, K.; Hof, C.; Klimkovich, T.; Klingebiel, D.; Kreuzer, P.; Lanske, D.; Magass, C.; Masetti, G.; Merschmeyer, M.; Meyer, A.; Papacz, P.; Pieta, H.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Steggemann, J.; Teyssier, D.] Rhein Westfal TH Aachen, Inst Phys A 3, Aachen, Germany. [Bontenackels, M.; Davids, M.; Duda, M.; Fluegge, G.; Geenen, H.; Giffels, M.; Ahmad, W. Haj; Heydhausen, D.; Kress, T.; Kuessel, Y.; Linn, A.; Nowack, A.; Perchalla, L.; Pooth, O.; Rennefeld, J.; Sauerland, P.; Stahl, A.; Thomas, M.; Tornier, D.; Zoeller, M. H.] Rhein Westfal TH Aachen, Inst Phys B 3, Aachen, Germany. [Martin, M. Aldaya; Behrenhoff, W.; Behrens, U.; Bergholz, M.; Borras, K.; Cakir, A.; Campbell, A.; Castro, E.; Dammann, D.; Eckerlin, G.; Eckstein, D.; Flossdorf, A.; Flucke, G.; Geiser, A.; Glushkov, I.; Hauk, J.; Jung, H.; Kasemann, M.; Katkov, I.; Katsas, P.; Kleinwort, C.; Kluge, H.; Knutsson, A.; Kruecker, D.; Kuznetsova, E.; Lange, W.; Lohmann, W.; Mankel, R.; Marienfeld, M.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Olzem, J.; Parenti, A.; Raspereza, A.; Raval, A.; Schmidt, R.; Schoerner-Sadenius, T.; Sen, N.; Stein, M.; Tomaszewska, J.; Volyanskyy, D.; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Autermann, C.; Bobrovskyi, S.; Draeger, J.; Enderle, H.; Gebbert, U.; Kaschube, K.; Kaussen, G.; Klanner, R.; Lange, J.; Mura, B.; Naumann-Emme, S.; Nowak, F.; Pietsch, N.; Sander, C.; Schettler, H.; Schleper, P.; Schroeder, M.; Schum, T.; Schwandt, J.; Srivastava, A. K.; Stadie, H.; Steinbrueck, G.; Thomsen, J.; Wolf, R.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Bauer, J.; Buege, V.; Chwalek, T.; De Boer, W.; Dierlamm, A.; Dirkes, G.; Feindt, M.; Gruschke, J.; Hackstein, C.; Hartmann, F.; Heindl, S. M.; Heinrich, M.; Held, H.; Hoffmann, K. H.; Honc, S.; Kuhr, T.; Martschei, D.; Mueller, S.; Mueller, Th.; Niegel, M.; Oberst, O.; Oehler, A.; Ott, J.; Peiffer, T.; Piparo, D.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Renz, M.; Saout, C.; Scheurer, A.; Schieferdecker, P.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Troendle, D.; Wagner-Kuhr, J.; Zeise, M.; Zhukov, V.; Ziebarth, E. B.] Univ Karlsruhe, Inst Expt Kernphys, D-7500 Karlsruhe, Germany. [Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Manolakos, I.; Markou, A.; Markou, C.; Mavrommatis, C.; Ntomari, E.; Petrakou, E.] Inst Nucl Phys Demokritos, Aghia Paraskevi, Greece. [Gouskos, L.; Mertzimekis, T. J.; Panagiotou, A.; Sphicas, P.] Univ Athens, Athens, Greece. [Evangelou, I.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Patras, V.; Triantis, F. A.] Univ Ioannina, GR-45110 Ioannina, Greece. [Aranyi, A.; Bencze, G.; Boldizsar, L.; Debreczeni, G.; Hajdu, C.; Horvath, D.; Kapusi, A.; Krajczar, K.; Laszlo, A.; Sikler, F.; Vesztergombi, G.; Pasztor, G.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Molnar, J.; Palinkas, J.; Szillasi, Z.; Veszpremi, V.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Jindal, M.; Kaur, M.; Kohli, J. M.; Mehta, M. Z.; Nishu, N.; Saini, L. K.; Sharma, A.; Singh, A. P.; Singh, J. B.; Singh, S. P.] Panjab Univ, Chandigarh 160014, India. [Ahuja, S.; Bhattacharya, S.; Choudhary, B. C.; Gupta, P.; Jain, S.; Jain, S.; Kumar, A.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Choudhury, R. K.; Dutta, D.; Kailas, S.; Kataria, S. K.; Mohanty, A. K.; Pant, L. M.; Shukla, P.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Aziz, T.; Guchait, M.; Gurtu, A.; Maity, M.; Majumder, D.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Saha, A.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Mumbai, Maharashtra, India. [Guchait, M.; Banerjee, S.; Dugad, S.; Mondal, N. K.] Tata Inst Fundamental Res HECR, Mumbai, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Hashemi, M.; Jafari, A.; Khakzad, M.; Mohammadi, A.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res & Fundamental Sci IPM, Tehran, Iran. [Abbrescia, M.; Barbone, L.; Calabria, C.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Dimitrov, A.; Fiore, L.; Iaselli, G.; Lusito, L.; Maggi, G.; Maggi, M.; Manna, N.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pierro, G. A.; Pompili, A.; Pugliese, G.; Romano, F.; Roselli, G.; Selvaggi, G.; Silvestris, L.; Trentadue, R.; Tupputi, S.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; De Palma, M.; Lusito, L.; Manna, N.; Marangelli, B.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Roselli, G.; Selvaggi, G.; Tupputi, S.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.; Romano, F.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Giunta, M.; Marcellini, S.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Braibant-Giacomelli, S.; Capiluppi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Meneghelli, M.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Tricomi, A.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Genta, C.; Gonzi, S.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Lenzi, P.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Colafranceschi, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Ghezzi, A.; Malberti, M.; Malvezzi, S.; Martelli, A.; Massironi, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; Sala, S.; de Fatis, T. Tabarelli; Tancini, V.] Ist Nazl Fis Nucl, Sez Milano Biccoca, I-20133 Milan, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Ghezzi, A.; Malberti, M.; Martelli, A.; Massironi, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli; Tancini, V.] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Montoy, C. A. Carrillo; Cimmino, A.; De Cosa, A.; De Gruttola, M.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Merola, M.; Noli, P.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Cimmino, A.; De Cosa, A.; De Gruttola, M.; Merola, M.; Noli, P.] Univ Naples Federico II, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bellan, P.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Conti, E.; De Mattia, M.; Dorigo, T.; Dosselli, U.; Fanzago, F.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gresele, A.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Mazzucato, M.; Meneguzzo, A. T.; Perrozzi, L.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, I-35100 Padua, Italy. [Bellan, P.; Bisello, D.; Carlin, R.; De Mattia, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Univ Padua, Padua, Italy. [Gresele, A.; Lazzizzera, I.] Univ Trent, Trento, Italy. [Baesso, P.; Berzano, U.; Riccardi, C.; Torre, P.; Vitulo, P.; Viviani, C.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Baesso, P.; Riccardi, C.; Torre, P.; Vitulo, P.; Viviani, C.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Caponeri, B.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Menichelli, M.; Nappi, A.; Santocchia, A.; Servoli, L.; Taroni, S.; Valdata, M.; Volpe, R.; Pioppi, M.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Caponeri, B.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Nappi, A.; Santocchia, A.; Taroni, S.; Valdata, M.; Volpe, R.; Pioppi, M.] Univ Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Palmonari, F.; Sarkar, S.; Segneri, G.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Rolandi, G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bernardini, J.; Fiori, F.; Messineo, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Azzurri, P.; Broccolo, G.; D'Agnolo, R. T.; Foa, L.; Ligabue, F.; Sarkar, S.; Rolandi, G.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Di Marco, E.; Diemoz, M.; Franci, D.; Grassi, M.; Longo, E.; Organtini, G.; Palma, A.; Pandolfi, F.; Paramatti, R.; Rahatlou, S.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Di Marco, E.; Franci, D.; Longo, E.; Organtini, G.; Palma, A.; Pandolfi, F.; Rahatlou, S.] Univ Roma La Sapienza, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Botta, C.; Cartiglia, N.; Castello, R.; Costa, M.; Demaria, N.; Graziano, A.; Mariotti, C.; Marone, M.; Maselli, S.; Migliore, E.; Mila, G.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Romero, A.; Ruspa, M.; Sacchi, R.; Sola, V.; Solano, A.; Staiano, A.; Trocino, D.; Pereira, A. Vilela] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Botta, C.; Castello, R.; Costa, M.; Graziano, A.; Marone, M.; Migliore, E.; Mila, G.; Monaco, V.; Musich, M.; Pelliccioni, M.; Romero, A.; Sacchi, R.; Sola, V.; Solano, A.; Trocino, D.; Pereira, A. Vilela] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Montanino, D.; Penzo, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Della Ricca, G.; Montanino, D.] Univ Trieste, Trieste, Italy. [Heo, S. G.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Chung, J.; Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Park, H.; Son, D.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, Zero; Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Hong, B.; Jo, M.; Kim, H.; Kim, J. H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.; Rhee, H. B.; Seo, E.; Shin, S.; Sim, K. S.] Korea Univ, Seoul, South Korea. [Choi, M.; Kang, S.; Kim, H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Martisiute, D.; Petrov, P.; Sabonis, T.] Vilnius Univ, Vilnius, Lithuania. [Castilla Valdez, H.; De La Cruz Burelo, E.; Lopez-Fernandez, R.; Sanchez Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Allfrey, P.; Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.] Univ Canterbury, Christchurch 1, New Zealand. [Silverwood, H.; Ahmad, M.; Ahmed, I.; Asghar, M. I.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bluj, M.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Soltan Inst Nucl Studies, PL-00681 Warsaw, Poland. [Almeida, N.; David, A.; Faccioli, P.; Parracho, P. G. Ferreira; Gallinaro, M.; Martins, P.; Musella, P.; Nayak, A.; Ribeiro, P. Q.; Seixas, J.; Silva, P.; Varela, J.; Woehri, H. K.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Belotelov, I.; Bunin, P.; Finger, M.; Finger, M., Jr.; Golutvin, I.; Kamenev, A.; Karjavin, V.; Kozlov, G.; Lanev, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Bondar, N.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Toropin, A.; Troitsky, S.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Kaftanov, V.; Kossov, M.; Krokhotin, A.; Lychkovskaya, N.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Sarycheva, L.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Azhgirey, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Slabospitsky, S.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Arce, P.; Battilana, C.; Calvo, E.; Cepeda, M.; Cerrada, M.; Colino, N.; De La Cruz, B.; Diez Pardos, C.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Redondo, I.; Romero, L.; Santaolalla, J.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chamizo Llatas, M.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Jorda, C.; Lobelle Pardo, P.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Ruiz Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, IFCA, E-39005 Santander, Spain. [Hammer, J.; Darmenov, N.; Genchev, V.; Iaydjiev, P.; Hajdu, C.; Mohanty, A. K.; Lusito, L.; Chiorboli, M.; Tropiano, A.; De Guio, F.; Ghezzi, A.; Perrozzi, L.; Lucaroni, A.; Volpe, R.; Boccali, T.; Tonelli, G.; Venturi, A.; Botta, C.; Graziano, A.; Pelliccioni, M.; Kossov, M.; Grishin, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Baillon, P.; Ball, A. H.; Barney, D.; Bell, A. J.; Benedetti, D.; Bernet, C.; Bialas, W.; Bloch, P.; Bocci, A.; Bolognesi, S.; Breuker, H.; Brona, G.; Bunkowski, K.; Camporesi, T.; Cano, E.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Cure, B.; D'Enterria, D.; De Roeck, A.; Di Guida, S.; Ramos, F. Duarte; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Gaddi, A.; Gennai, S.; Georgiou, G.; Gerwig, H.; Gigi, D.; Gill, K.; Giordano, D.; Glege, F.; Garrido, R. Gomez-Reino; Gouzevitch, M.; Govoni, P.; Gowdy, S.; Guiducci, L.; Hansen, M.; Harvey, J.; Hegeman, J.; Hegner, B.; Henderson, C.; Hesketh, G.; Hoffmann, H. F.; Honma, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Lecoq, P.; Lourenco, C.; Macpherson, A.; Maeki, T.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Nesvold, E.; Nguyen, M.; Orimoto, T.; Orsini, L.; Perez, E.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Polese, G.; Racz, A.; Antunes, J. Rodrigues; Rolandi, G.; Rommerskirchen, T.; Rovelli, C.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Segoni, I.; Sharma, A.; Siegrist, P.; Simon, M.; Sphicas, P.; Spiga, D.; Spiropulu, M.; Stoeckli, F.; Stoye, M.; Tropea, P.; Tsirou, A.; Tsyganov, A.; Veres, G. I.; Vichoudis, P.; Voutilainen, M.; Zeuner, W. D.; Caminada, L.; Marchica, C.; Sharma, V.; Hall-Wilton, R.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Nig, S. Ko; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Starodumov, A.; Caminada, L.; Marchica, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bortignon, P.; Caminada, L.; Chen, Z.; Cittolin, S.; Dissertori, G.; Dittmar, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Herve, A.; Hintz, W.; Lecomte, P.; Lustermann, W.; Marchica, C.; del Arbol, P. Martinez Ruiz; Meridiani, P.; Milenovic, P.; Moortgat, F.; Nef, P.; Nessi-Tedaldi, F.; Pape, L.; Pauss, F.; Punz, T.; Rizzi, A.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Sawley, M. -C.; Stieger, B.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, M.; Wehrli, L.; Weng, J.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Aguilo, E.; Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Regenfus, C.; Robmann, P.; Schmidt, A.; Snoek, H.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Chen, W. T.; Dutta, S.; Go, A.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, M. H.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Wu, J. H.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Demir, Z.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Topaksu, A. Kayis; Nart, A.; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Tali, B.; Topakli, H.; Uzun, D.; Vergili, L. N.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Deliomeroglu, M.; Demir, D.; Guelmez, E.; Halu, A.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Levchuk, L.] Natl Sci Ctr, Kharkov Inst Phys & Technol, Kharkov, Ukraine. [Bell, P.; Bostock, F.; Brooke, J. J.; Cheng, T. L.; Clement, E.; Cussans, D.; Frazier, R.; Goldstein, J.; Grimes, M.; Hansen, M.; Hartley, D.; Heath, G. P.; Heath, H. F.; Huckvale, B.; Jackson, J.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Ward, S.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Camanzi, B.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Ballin, J.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Davies, G.; Della Negra, M.; Fulcher, J.; Futyan, D.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Karapostoli, G.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rompotis, N.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Tourneur, S.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardrope, D.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Barrett, M.; Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Martin, W.; Reid, I. D.; Teodorescu, L.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.] Baylor Univ, Waco, TX 76798 USA. [Bose, T.; Jarrin, E. Carrera; Fantasia, C.; Heister, A.; John, J. St.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Avetisyan, A.; Bhattacharya, S.; Chou, J. P.; Cutts, D.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Landsberg, G.; Narain, M.; Nguyen, D.; Segala, M.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Borgia, M. A.; Breedon, R.; Sanchez, M. Calderon De La Barca; Cebra, D.; Chauhan, S.; Chertok, M.; Conway, J.; Cox, P. T.; Dolen, J.; Erbacher, R.; Friis, E.; Ko, W.; Kopecky, A.; Lander, R.; Liu, H.; Maruyama, S.; Miceli, T.; Nikolic, M.; Pellett, D.; Robles, J.; Salur, S.; Schwarz, T.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez; Veelken, C.] Univ Calif Davis, Davis, CA 95616 USA. [Felcini, M.; Andreev, V.; Arisaka, K.; Cline, D.; Cousins, R.; Deisher, A.; Duris, J.; Erhan, S.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Tucker, J.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Kao, S. C.; Liu, F.; Liu, H.; Luthra, A.; Nguyen, H.; Pasztor, G.; Satpathy, A.; Shen, B. C.; Stringer, R.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Dusinberre, E.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Mangano, B.; Muelmenstaedt, J.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pi, H.; Pieri, M.; Ranieri, R.; Sani, M.; Sharma, V.; Simon, S.; Tu, Y.; Vartak, A.; Wuerthwein, F.; Yagil, A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; Vlimant, J. R.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Spiropulu, M.; Bornheim, A.; Bunn, J.; Chen, Y.; Gataullin, M.; Kcira, D.; Litvine, V.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Timciuc, V.; Traczyk, P.; Veverka, J.; Wilkinson, R.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Akgun, B.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Jun, S. Y.; Liu, Y. F.; Paulini, M.; Russ, J.; Terentyev, N.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Dinardo, M. E.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Gaz, A.; Heyburn, B.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.; Zang, S. L.] Univ Colorado, Boulder, CO 80309 USA. [Agostino, L.; Alexander, J.; Chatterjee, A.; Das, S.; Eggert, N.; Fields, L. J.; Gibbons, L. K.; Heltsley, B.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Kuznetsov, V.; Kaufman, G. Nicolas; Patterson, J. R.; Puigh, D.; Riley, D.; Ryd, A.; Shi, X.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Biselli, A.; Cirino, G.; Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Atac, M.; Bakken, J. A.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Borcherding, F.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Demarteau, M.; Eartly, D. P.; Elvira, V. D.; Esen, S.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Green, D.; Gunthoti, K.; Gutsche, O.; Hahn, A.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; James, E.; Jensen, H.; Johnson, M.; Joshi, U.; Khatiwada, R.; Kilminster, B.; Klima, B.; Kousouris, K.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Limon, P.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Mason, D.; McBride, P.; McCauley, T.; Miao, T.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Popescu, S.; Pordes, R.; Prokofyev, O.; Saoulidou, N.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Tan, P.; Taylor, L.; Tkaczyk, S.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Piedra Gomez, J.; Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Goldberg, S.; Kim, B.; Klimenko, S.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Matchev, K.; Mitselmakher, G.; Muniz, L.; Pakhotin, Y.; Prescott, C.; Remington, R.; Schmitt, M.; Scurlock, B.; Sellers, P.; Skhirtladze, N.; Wang, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Ceron, C.; Gaultney, V.; Kramer, L.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bandurin, D.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Quertenmont, L.; Sekmen, S.; Veeraraghavan, V.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Guragain, S.; Hohlmann, M.; Kalakhety, H.; Ralich, R.; Vodopiyanov, I.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Callner, J.; Cavanaugh, R.; Dragoiu, C.; Garcia-Solis, E. J.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Lacroix, F.; Malek, M.; O'Brien, C.; Silvestre, C.; Smoron, A.; Strom, D.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Cankocak, K.; Clarida, W.; Duru, F.; Lae, C. K.; McCliment, E.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Olson, J.; Onel, Y.; Ozok, F.; Sen, S.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bonato, A.; Eskew, C.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Guo, Z. J.; Hu, G.; Maksimovic, P.; Rappoccio, S.; Swartz, M.; Tran, N. V.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Grachov, O.; Murray, M.; Noonan, D.; Radicci, V.; Sanders, S.; Wood, J. S.; Zhukova, V.] Univ Kansas, Lawrence, KS 66045 USA. [Bolton, T.; Chakaberia, I.; Ivanov, A.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.; Wan, Z.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Boutemeur, M.; Eno, S. C.; Ferencek, D.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kirn, M.; Lu, Y.; Mignerey, A. C.; Rossato, K.; Rumerio, P.; Santanastasio, F.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.; Twedt, E.] Univ Maryland, College Pk, MD 20742 USA. [Alver, B.; Bauer, G.; Bendavid, J.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Everaerts, P.; Ceballos, G. Gomez; Goncharov, M.; Hahn, K. A.; Harris, P.; Kim, Y.; Klute, M.; Lee, Y. -J.; Li, W.; Loizides, C.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Rudolph, M.; Stephans, G. S. F.; Sumorok, K.; Sung, K.; Wenger, E. A.; Xie, S.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.] MIT, Cambridge, MA 02139 USA. [Cole, P.; Cooper, S. I.; Cushman, P.; Dahmes, B.; De Benedetti, A.; Dudero, P. R.; Franzoni, G.; Haupt, J.; Klapoetke, K.; Kubota, Y.; Mans, J.; Rekovic, V.; Rusack, R.; Sasseville, M.; Singovsky, A.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Godang, R.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, University, MS 38677 USA. [Bloom, K.; Bose, S.; Butt, J.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kelly, T.; Kravchenko, I.; Lazo-Flores, J.; Lundstedt, C.; Malbouisson, H.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Baur, U.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Shipkowski, S. P.; Smith, K.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Boeriu, O.; Chasco, M.; Reucroft, S.; Swain, J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Kubik, A.; Odell, N.; Ofierzynski, R. A.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Antonelli, L.; Berry, D.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Kolberg, T.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Warchol, J.; Wayne, M.; Ziegler, J.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Bylsma, B.; Durkin, L. S.; Gu, J.; Hill, C.; Killewald, P.; Kotov, K.; Ling, T. Y.; Rodenburg, M.; Williams, G.] Ohio State Univ, Columbus, OH 43210 USA. [Adam, N.; Berry, E.; Elmer, P.; Gerbaudo, D.; Halyo, V.; Hebda, P.; Hunt, A.; Jones, J.; Laird, E.; Pegna, D. Lopes; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Acosta, J. G.; Huang, X. T.; Lopez, A.; Mendez, H.; Oliveros, S.; Vargas, J. E. Ramirez; Zatserklyaniy, A.] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Barnes, V. E.; Bolla, G.; Borrello, L.; Bortoletto, D.; Everett, A.; Garfinkel, A. F.; Gecse, Z.; Gutay, L.; Hu, Z.; Jones, M.; Koybasi, O.; Kress, M.; Laasanen, A. T.; Leonardo, N.; Liu, C.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Jindal, P.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Boulahouache, C.; Cuplov, V.; Ecklund, K. M.; Geurts, F. J. M.; Liu, J. H.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Chung, Y. S.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Flacher, H.; Garcia-Bellido, A.; Goldenzweig, P.; Gotra, Y.; Han, J.; Harel, A.; Miner, D. C.; Orbaker, D.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.; Yan, M.] Rockefeller Univ, New York, NY 10021 USA. [Atramentov, O.; Barker, A.; Duggan, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hits, D.; Lath, A.; Panwalkar, S.; Patel, R.; Richards, A.; Rose, K.; Schnetzer, S.; Somalwar, S.; Stone, R.; Thomas, S.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Asaadi, J.; Eusebi, R.; Gilmore, J.; Gurrola, A.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Nguyen, C. N.; Osipenkov, I.; Pivarski, J.; Safonov, A.; Sengupta, S.; Tatarinov, A.; Toback, D.; Weinberger, M.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Bardak, C.; Damgov, J.; Jeong, C.; Kovitanggoon, K.; Lee, S. W.; Mane, P.; Roh, Y.; Sill, A.; Volobouev, I.; Wigmans, R.; Yazgan, E.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Brownson, E.; Engh, D.; Florez, C.; Gabella, W.; Johns, W.; Kurt, P.; Maguire, C.; Melo, A.; Sheldon, P.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN USA. [Arenton, M. W.; Balazs, M.; Boutle, S.; Buehler, M.; Conetti, S.; Cox, B.; Francis, B.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Yohay, R.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Lamichhane, P.; Mattson, M.; Ne, C. Milste; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Anderson, M.; Bachtis, M.; Bellinger, J. N.; Carlsmith, D.; Dasu, S.; Efron, J.; Gray, L.; Grogg, K. S.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Leonard, J.; Loveless, R.; Mohapatra, A.; Reeder, D.; Ross, I.; Savin, A.; Smith, W. H.; Swanson, J.; Weinberg, M.] Univ Wisconsin, Madison, WI USA. Univ Fed ABC, Santo Andre, Brazil. [Assran, Y.] Suez Canal Univ, Suez, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Krajczar, K.; Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Colafranceschi, S.] Univ Roma La Sapienza, Fac Ingn, Rome, Italy. [Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Bell, A. J.] Univ Geneva, Geneva, Switzerland. [Bakirci, M. N.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.] Adiyaman Univ, Adiyaman, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Demir, D.] Izmir Inst Technol, Izmir, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Ozkorucuklu, S.] Suleyman Demirel Univ, TR-32200 Isparta, Turkey. [Sonmez, N.] Ege Univ, Izmir, Turkey. [Basso, L.; Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Popescu, S.] Horia Hulubei Natl Inst Phys & Nucl Engn IFIN HH, Bucharest, Romania. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Wulz, Claudia-Elisabeth/H-5657-2011; Chen, Jie/H-6210-2011; Tinoco Mendes, Andre David/D-4314-2011; Mignerey, Alice/D-6623-2011; Ganjour, Serguei/D-8853-2011; Ruiz, Alberto/E-4473-2011; Stahl, Achim/E-8846-2011; Hektor, Andi/G-1804-2011; Bolton, Tim/A-7951-2012; Yang, Fan/B-2755-2012; Krammer, Manfred/A-6508-2010; Lokhtin, Igor/D-7004-2012; Kodolova, Olga/D-7158-2012; Dudko, Lev/D-7127-2012; Katkov, Igor/E-2627-2012; Boos, Eduard/D-9748-2012; Snigirev, Alexander/D-8912-2012; Servoli, Leonello/E-6766-2012; Tomei, Thiago/E-7091-2012; Novaes, Sergio/D-3532-2012; Padula, Sandra /G-3560-2012; Fruhwirth, Rudolf/H-2529-2012; Azzi, Patrizia/H-5404-2012; Torassa, Ezio/I-1788-2012; Giacomelli, Paolo/B-8076-2009; Jeitler, Manfred/H-3106-2012; Venturi, Andrea/J-1877-2012; Varela, Joao/K-4829-2016; Menasce, Dario Livio/A-2168-2016; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Fassi, Farida/F-3571-2016; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Gerbaudo, Davide/J-4536-2012; Ozdemir, Kadri/P-8058-2014; Azarkin, Maxim/N-2578-2015; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Sznajder, Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Haj Ahmad, Wael/E-6738-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Matorras, Francisco/I-4983-2015; My, Salvatore/I-5160-2015; Muelmenstaedt, Johannes/K-2432-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Arce, Pedro/L-1268-2014; Flix, Josep/G-5414-2012; Benussi, Luigi/O-9684-2014; Russ, James/P-3092-2014; Dahms, Torsten/A-8453-2015; Ahmed, Ijaz/E-9144-2015; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; Bedoya, Cristina/K-8066-2014; Janssen, Xavier/E-1915-2013; Codispoti, Giuseppe/F-6574-2014; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Calderon, Alicia/K-3658-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; Vogel, Helmut/N-8882-2014; Marinho, Franciole/N-8101-2014; Ragazzi, Stefano/D-2463-2009; Zalewski, Piotr/H-7335-2013; Ivanov, Andrew/A-7982-2013; Raidal, Martti/F-4436-2012; Kadastik, Mario/B-7559-2008; Hill, Christopher/B-5371-2012; Troitsky, Sergey/C-1377-2014; Marlow, Daniel/C-9132-2014; Oguri, Vitor/B-5403-2013; de Jesus Damiao, Dilson/G-6218-2012; Montanari, Alessandro/J-2420-2012; Amapane, Nicola/J-3683-2012; tosi, mia/J-5777-2012; Petrushanko, Sergey/D-6880-2012; Della Ricca, Giuseppe/B-6826-2013; Mundim, Luiz/A-1291-2012; Santaolalla, Javier/C-3094-2013; Alves, Gilvan/C-4007-2013; Rolandi, Luigi (Gigi)/E-8563-2013 OI Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Tinoco Mendes, Andre David/0000-0001-5854-7699; Ruiz, Alberto/0000-0002-3639-0368; Stahl, Achim/0000-0002-8369-7506; Hektor, Andi/0000-0001-7873-8118; Krammer, Manfred/0000-0003-2257-7751; Dudko, Lev/0000-0002-4462-3192; Katkov, Igor/0000-0003-3064-0466; Servoli, Leonello/0000-0003-1725-9185; Tomei, Thiago/0000-0002-1809-5226; Novaes, Sergio/0000-0003-0471-8549; Azzi, Patrizia/0000-0002-3129-828X; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Varela, Joao/0000-0003-2613-3146; Heath, Helen/0000-0001-6576-9740; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Lloret Iglesias, Lara/0000-0002-0157-4765; Carrera, Edgar/0000-0002-0857-8507; Sguazzoni, Giacomo/0000-0002-0791-3350; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Fassi, Farida/0000-0002-6423-7213; Ghezzi, Alessio/0000-0002-8184-7953; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Gerbaudo, Davide/0000-0002-4463-0878; Vieira de Castro Ferreira da Silva, Pedro Manuel/0000-0002-5725-041X; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Ozdemir, Kadri/0000-0002-0103-1488; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Haj Ahmad, Wael/0000-0003-1491-0446; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Matorras, Francisco/0000-0003-4295-5668; My, Salvatore/0000-0002-9938-2680; Muelmenstaedt, Johannes/0000-0003-1105-6678; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Arce, Pedro/0000-0003-3009-0484; Flix, Josep/0000-0003-2688-8047; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Dahms, Torsten/0000-0003-4274-5476; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bedoya, Cristina/0000-0001-8057-9152; Codispoti, Giuseppe/0000-0003-0217-7021; Cerrada, Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Vogel, Helmut/0000-0002-6109-3023; Marinho, Franciole/0000-0002-7327-0349; Ragazzi, Stefano/0000-0001-8219-2074; Ivanov, Andrew/0000-0002-9270-5643; Hill, Christopher/0000-0003-0059-0779; Troitsky, Sergey/0000-0001-6917-6600; de Jesus Damiao, Dilson/0000-0002-3769-1680; Montanari, Alessandro/0000-0003-2748-6373; Amapane, Nicola/0000-0001-9449-2509; Della Ricca, Giuseppe/0000-0003-2831-6982; Mundim, Luiz/0000-0001-9964-7805; Rolandi, Luigi (Gigi)/0000-0002-0635-274X FU FMSR (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences (Estonia); NICPB (Estonia); Academy of Finland (Finland); ME (Finland); HIP (Finland); CEA (France); CNRS (France) [IN2P3]; BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Korea); WCU (Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MST (Russia); MAE (Russia); MSTD (Serbia); MICINN (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK (Turkey); TAEK (Turkey); STFC (United Kingdom); DOE (USA); NSF (USA) FX We wish to thank Michael Kramer for providing the NLO LQ pair production cross sections at root s = 7 TeV. We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine. We thank the technical and administrative staff at CERN and other CMS institutes, and acknowledge support from: FMSR (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences and NICPB (Estonia); Academy of Finland, ME, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MST and MAE (Russia); MSTD (Serbia); MICINN and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK and TAEK (Turkey); STFC (United Kingdom); DOE and NSF (USA). NR 30 TC 20 Z9 20 U1 2 U2 42 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 17 PY 2011 VL 106 IS 20 AR 201802 DI 10.1103/PhysRevLett.106.201802 PG 15 WC Physics, Multidisciplinary SC Physics GA 765SR UT WOS:000290729400004 PM 21668220 ER PT J AU Nguyen, DH Oketch-Rabah, HA Illa-Bochaca, I Geyer, FC Reis-Filho, JS Mao, JH Ravani, SA Zavadi, J Borowsky, AD Jerry, DJ Dunphy, KA Seo, JH Haslam, S Medina, D Barcellos-Hoff, MH AF Nguyen, David H. Oketch-Rabah, Hellen A. Illa-Bochaca, Irineu Geyer, Felipe C. Reis-Filho, Jorge S. Mao, Jian-Hua Ravani, Shraddha A. Zavadi, Jiri Borowsky, Alexander D. Jerry, D. Joseph Dunphy, Karen A. Seo, Jae Hong Haslam, Sandra Medina, Daniel Barcellos-Hoff, Mary Helen TI Radiation Acts on the Microenvironment to Affect Breast Carcinogenesis by Distinct Mechanisms that Decrease Cancer Latency and Affect Tumor Type SO CANCER CELL LA English DT Article ID GROWTH-FACTOR-BETA; MAMMARY STEM-CELL; IN-SITU; IONIZING-RADIATION; ESTROGEN-RECEPTOR; GLAND; MOUSE; P53; EXPRESSION; ORIGIN AB Tissue microenvironment is an important determinant of carcinogenesis. We demonstrate that ionizing radiation, a known carcinogen, affects cancer frequency and characteristics by acting on the microenvironment. Using a mammary chimera model in which an irradiated host is transplanted with oncogenic Trp53 null epithelium, we show accelerated development of aggressive tumors whose molecular signatures were distinct from tumors arising in nonirradiated hosts. Molecular and genetic approaches show that TGF beta mediated tumor acceleration. Tumor molecular signatures implicated TGF beta, and genetically reducing TGF beta abrogated the effect on latency. Surprisingly, tumors from irradiated hosts were predominantly estrogen receptor negative. This effect was TGF beta independent and linked to mammary stem cell activity. Thus, the irradiated microenvironment affects latency and clinically relevant features of cancer through distinct and unexpected mechanisms. C1 [Nguyen, David H.; Illa-Bochaca, Irineu; Barcellos-Hoff, Mary Helen] NYU, Sch Med, Dept Radiat Oncol, New York, NY 10016 USA. [Nguyen, David H.; Oketch-Rabah, Hellen A.; Mao, Jian-Hua; Ravani, Shraddha A.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Life Sci, Berkeley, CA 94720 USA. [Geyer, Felipe C.; Reis-Filho, Jorge S.] Inst Canc Res, Breakthrough Breast Canc Res Ctr, Mol Pathol Lab, London SW3 6JB, England. [Zavadi, Jiri] NYU Langone Med Ctr, NYU Canc Inst, Dept Pathol, New York, NY 10016 USA. [Zavadi, Jiri] NYU Langone Med Ctr, Ctr Hlth Informat & Bioinformat, New York, NY 10016 USA. [Borowsky, Alexander D.] Univ Calif Davis, Dept Med Pathol, Ctr Comparat Med, Davis, CA 95616 USA. [Jerry, D. Joseph; Dunphy, Karen A.] Pioneer Valley Life Sci Inst, Springfield, MA 01199 USA. [Haslam, Sandra] Michigan State Univ, Dept Physiol, E Lansing, MI USA. [Medina, Daniel] Baylor Coll Med, Houston, TX 77030 USA. [Seo, Jae Hong] Korea Univ, Dept Internal Med, Sect Med Oncol, Seoul 136701, South Korea. RP Barcellos-Hoff, MH (reprint author), NYU, Sch Med, Dept Radiat Oncol, 566 1st Ave, New York, NY 10016 USA. EM mhbarcellos-hoff@nyumc.org RI Illa-Bochaca, Irineu/K-3191-2013; OI Illa-Bochaca, Irineu/0000-0002-8039-565X; Zavadil, Jiri/0000-0003-0640-5562 FU DOD-BCRP; Breakthrough Breast Cancer; Department of Energy, Office of Biological and Environment Research; National Institute of Environmental Health Sciences [U01 ES/CA 012801, 012800]; National Cancer Institute of the National Institutes of Health FX The authors thank Drs. P. Cowin, C. Allred, and P. Williams for helpful discussion, Dr. J. Paupert and Y. Huang for assistance with slide scoring, W. Chou, B. Chu, R. Chou, and B. Yang for technical assistance, and Y. Zhang of the NYU Cancer Institute Genomics Facility for generating the microarray data. This research was supported by a DOD-BCRP predoctoral fellowship to D.H.N., funds from Breakthrough Breast Cancer to F.C.G. and J.S.R.-F.; and grants to M.H.B.-H. from California Breast Cancer Research Program, the Department of Energy, Office of Biological and Environment Research Low Dose program, and the Breast Cancer and the Environment Research Centers grant number U01 ES/CA 012801 (M.H.B.-H.) and 012800 (S.H.) from the National Institute of Environmental Health Sciences and the National Cancer Institute of the National Institutes of Health. M.H.B.-H. designed research. H.A.O.-R., I.I.-B., S.A.R., S. H., F.C.G., J.S.R.-F., A.D.B., and D.H.N. performed research. D.J.J. and D.M. contributed reagents. D.H.N., I.I.-B., J.Z., J-H.M., and M.H.B.-H. analyzed data. D.H.N., D.M., and M.H.B.-H wrote the paper. NR 53 TC 75 Z9 77 U1 0 U2 10 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1535-6108 J9 CANCER CELL JI Cancer Cell PD MAY 17 PY 2011 VL 19 IS 5 BP 640 EP 651 DI 10.1016/j.ccr.2011.03.011 PG 12 WC Oncology; Cell Biology SC Oncology; Cell Biology GA 768KD UT WOS:000290932400009 PM 21575864 ER PT J AU Daub, EG Shelly, DR Guyer, RA Johnson, PA AF Daub, Eric G. Shelly, David R. Guyer, Robert A. Johnson, Paul A. TI Brittle and ductile friction and the physics of tectonic tremor SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID SAN-ANDREAS FAULT; SOUTHWEST JAPAN; EPISODIC TREMOR; SILENT SLIP; EARTHQUAKES; SUBDUCTION; CALIFORNIA; PARKFIELD; CONTACTS; BENEATH AB Observations of nonvolcanic tremor provide a unique window into the mechanisms of deformation and failure in the lower crust. At increasing depths, rock deformation gradually transitions from brittle, where earthquakes occur, to ductile, with tremor occurring in the transitional region. The physics of deformation in the transition region remain poorly constrained, limiting our basic understanding of tremor and its relation to earthquakes. We combine field and laboratory observations with a physical friction model comprised of brittle and ductile components, and use the model to provide constraints on the friction and stress state in the lower crust. A phase diagram is constructed that characterizes under what conditions all faulting behaviors occur, including earthquakes, tremor, silent transient slip, and steady sliding. Our results show that tremor occurs over a range of ductile and brittle frictional strengths, and advances our understanding of the physical conditions at which tremor and earthquakes take place. Citation: Daub, E. G., D. R. Shelly, R. A. Guyer, and P. A. Johnson (2011), Brittle and ductile friction and the physics of tectonic tremor, Geophys. Res. Lett., 38, L10301, doi:10.1029/2011GL046866. C1 [Daub, Eric G.; Guyer, Robert A.; Johnson, Paul A.] Los Alamos Natl Lab, Geophys Grp, Los Alamos, NM 87545 USA. [Shelly, David R.] US Geol Survey, Menlo Pk, CA 94025 USA. [Daub, Eric G.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Guyer, Robert A.] Univ Nevada, Dept Phys, Reno, NV 89557 USA. RP Daub, EG (reprint author), Los Alamos Natl Lab, Geophys Grp, MS D443, Los Alamos, NM 87545 USA. EM edaub@lanl.gov OI Johnson, Paul/0000-0002-0927-4003 NR 26 TC 13 Z9 13 U1 0 U2 9 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAY 17 PY 2011 VL 38 AR L10301 DI 10.1029/2011GL046866 PG 4 WC Geosciences, Multidisciplinary SC Geology GA 767QT UT WOS:000290871800002 ER PT J AU Ouchi, T Sakai, K Fukuzawa, H Higuchi, I Demekhin, PV Chiang, YC Stoychev, SD Kuleff, AI Mazza, T Schoffler, M Nagaya, K Yao, M Tamenori, Y Saito, N Ueda, K AF Ouchi, T. Sakai, K. Fukuzawa, H. Higuchi, I. Demekhin, Ph. V. Chiang, Y. -C. Stoychev, S. D. Kuleff, A. I. Mazza, T. Schoeffler, M. Nagaya, K. Yao, M. Tamenori, Y. Saito, N. Ueda, K. TI Interatomic Coulombic decay following Ne 1s Auger decay in NeAr SO PHYSICAL REVIEW A LA English DT Article ID PHOTOCHEMISTRY BEAMLINE BL27SU; MOMENTUM SPECTROSCOPY; CLUSTERS; SPECTRUM; SPRING-8; ION; AR AB Using momentum-resolved electron-ion multicoincidence spectroscopy, we have investigated interatomic Coulombic decay (ICD) in the heteronuclear NeAr dimer following Ne 1s Auger decay. The measured intensity ratio for the three ICD transitions Ne2+(2s(-1)2p(-1) P-1)Ar to Ne2+(2p(-2 1)S)-Ar+(3p(-1)), Ne2+(2s(-1)2p(-1 1)P) Ar to Ne2+(2p(-2 1)D)-Ar+(3p(-1)), and Ne2+(2s(-1)2p(-1 3)P)Ar to Ne2+(2p-P-2 3)-Ar+(3p(-1)) reasonably agree with predictions. The kinetic energy release distribution for the fragmentation to Ne2+(2p(-2 1)D)-Ar+(3p(-1)) after the ICD transition from singlet Ne2+(2s(-1)2p(-1 1)P) Ar state, which is amirror image of the kinetic energy distribution of the emitted ICD electrons, suggests that the corresponding ICD rate is roughly two times lower than predicted by ab initio calculations. C1 [Ouchi, T.; Sakai, K.; Fukuzawa, H.; Mazza, T.; Ueda, K.] Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan. [Higuchi, I.; Tamenori, Y.] Japan Synchrotron Radiat Res Inst, Sayo, Hyogo 6795198, Japan. [Demekhin, Ph. V.; Chiang, Y. -C.; Stoychev, S. D.; Kuleff, A. I.] Heidelberg Univ, D-69120 Heidelberg, Germany. [Mazza, T.] Univ Milan, Dipartimento Fis, I-20133 Milan, Italy. [Schoeffler, M.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Nagaya, K.; Yao, M.] Kyoto Univ, Dept Phys, Kyoto 6068502, Japan. [Saito, N.] Natl Meteorol Inst Japan, Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058568, Japan. RP Ouchi, T (reprint author), Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan. EM ueda@tagen.tohoku.ac.jp RI Schoeffler, Markus/B-6261-2008; Tamenori, Yusuke/F-8867-2014; Saito, Norio/E-2890-2014; Demekhin, Philipp/K-9375-2016 OI Schoeffler, Markus/0000-0001-9214-6848; Tamenori, Yusuke/0000-0001-8004-895X; FU Japan Society for the Promotion of Science [21244062]; Ministry of Education, Culture, Sports, Science and Technology; Institute of Multidisciplinary Research for Advanced Materials; Alexander-vonHumboldt foundation; European Union [227597]; Max Planck Research School for Quantum Dynamics in Physics, Chemistry and Biology FX We are grateful to L. S. Cederbaum and P. Kolorenc for many fruitful discussions. The experiments were performed at SPring-8 with the approval of the Japan Synchrotron Radiation Research Institute. The work was supported by Grant-in-Aid (Grant No. 21244062) from the Japan Society for the Promotion of Science, the Management Expenses Grants for National Universities Corporations from the Ministry of Education, Culture, Sports, Science and Technology, and by the Institute of Multidisciplinary Research for Advanced Materials. M. S. acknowledges support from the Alexander-vonHumboldt foundation. A.I.K and Ph.V.D. acknowledge the financial support of the European Union's Seventh Framework Program European Research Council Advanced Investigator Grant No. 227597. Y.-C.C. acknowledges the International Max Planck Research School for Quantum Dynamics in Physics, Chemistry and Biology for financial support. NR 40 TC 19 Z9 19 U1 0 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD MAY 17 PY 2011 VL 83 IS 5 AR 053415 DI 10.1103/PhysRevA.83.053415 PG 6 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 765LG UT WOS:000290706800009 ER PT J AU Chua, V Yao, H Fiete, GA AF Chua, Victor Yao, Hong Fiete, Gregory A. TI Exact chiral spin liquid with stable spin Fermi surface on the kagome lattice SO PHYSICAL REVIEW B LA English DT Article ID RESONATING-VALENCE-BOND; SUPERCONDUCTIVITY; INSULATOR; PHYSICS; STATES; PHASE; MODEL AB We study an exactly solvable quantum spin model of Kitaev type on the kagome lattice. We find a rich phase diagram which includes a topological (gapped) chiral spin liquid with gapless chiral edge states, and a gapless chiral spin liquid phase with a spin Fermi surface. The ground state of the current model contains an odd number of electrons per unit cell, which qualitatively distinguishes it from previously studied exactly solvable models with a spin Fermi surface. Moreover, we show that the spin Fermi surface is stable against weak perturbations. C1 [Chua, Victor; Fiete, Gregory A.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Yao, Hong] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Yao, Hong] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Chua, V (reprint author), Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. RI Yao, Hong/D-3202-2011 OI Yao, Hong/0000-0003-2867-6144 FU NSF at Austin [DMR-0955778]; DOE at Berkeley [DE-AC02-05CH11231] FX We thank M. Kargarian, D.-H. Lee, A. Ruegg, and J. Wen for helpful discussions. We are grateful to Steve Kivelson for importantly inspiring this work. This work is supported in part by NSF Grant No. DMR-0955778 (V.C. and G.A.F.) at Austin and DOE Grant No. DE-AC02-05CH11231 (HY) at Berkeley. NR 40 TC 20 Z9 20 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 17 PY 2011 VL 83 IS 18 AR 180412 DI 10.1103/PhysRevB.83.180412 PG 4 WC Physics, Condensed Matter SC Physics GA 765MA UT WOS:000290709800001 ER PT J AU Lu, X Venugopalan, S Kim, H Grimsditch, M Rodriguez, S Ramdas, AK AF Lu, X. Venugopalan, S. Kim, Hyunjung Grimsditch, M. Rodriguez, S. Ramdas, A. K. TI Level mixing and anisotropy effect in resonant Raman electron paramagnetic transitions in ruby for B perpendicular to c SO PHYSICAL REVIEW B LA English DT Article ID ABSORPTION SPECTRA; OPTICAL-DETECTION; LINE SPECTRA; SCATTERING; CRYSTALS; AL2O3; CR-3; IONS AB Doubly resonant Raman electron paramagnetic transitions in ruby (Al(2)O(3):Cr(3+)) have been investigated using dye laser excitation tuned across the range of the Zeeman components of its well-known R(1) emission line. With magnetic field B normal to c, the optic axis of ruby, it is seen that the Raman electron paramagnetic resonance (EPR) lines exhibit significant intensity enhancements due to the simultaneous occurrence of "in resonance" and "out resonance," as visualized in the Kramers-Heisenberg formalism of inelastic light scattering. The specific Raman EPR features observed in the present study, together with their resonances, however, differ markedly from those observed in our previous investigation with B parallel to c. These differences can be traced to level mixing effects within the Zeeman multiplet of the (4)A(2) (ground) state on the one hand, and the negligible value of g perpendicular to for the (E) over bar (excited) state of the R(1) emission line on the other. Furthermore, we note that with B perpendicular to c and under resonant conditions, the experimentally observed Lambda m = +/- 1 pair of Stokes and anti-Stokes Raman lines are not connected by time-reversal symmetry. C1 [Lu, X.; Rodriguez, S.; Ramdas, A. K.] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. [Venugopalan, S.] SUNY Binghamton, Dept Phys, Binghamton, NY 13902 USA. [Kim, Hyunjung] Sogang Univ, Dept Phys, Seoul 121742, South Korea. [Grimsditch, M.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Lu, X (reprint author), Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. FU US National Science Foundation [DMR-0405082, DMR-0705793]; US Department of Energy, BES Material Sciences [W-31-109-ENG-38]; Sogang University FX X.L., S. R. and A. K. R acknowledge support from the US National Science Foundation (DMR-0405082 and DMR-0705793), M. G. from the US Department of Energy, BES Material Sciences (Grant No. W-31-109-ENG-38), and H. K. from Sogang University Special Research Grant (2009). NR 22 TC 3 Z9 3 U1 1 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 17 PY 2011 VL 83 IS 19 AR 195126 DI 10.1103/PhysRevB.83.195126 PG 6 WC Physics, Condensed Matter SC Physics GA 765MU UT WOS:000290712300001 ER PT J AU Luo, QL Yao, DX Moreo, A Dagotto, E AF Luo, Qinlong Yao, Dao-Xin Moreo, Adriana Dagotto, Elbio TI Charge stripes in the two-orbital Hubbard model for iron pnictides SO PHYSICAL REVIEW B LA English DT Article ID KEY ROLE; MAGNETISM; STATE AB The two-orbital Hubbard model for the pnictides is studied numerically using the real-space Hartree-Fock approximation on finite clusters. Upon electron doping, states with a nonuniform distribution of charge are stabilized. The observed patterns correspond to charge stripes oriented perpendicular to the direction of the spin stripes of the undoped magnetic ground state. While these charge-striped states are robust when the undoped state has a Hubbard gap, their existence when the intermediate-coupling magnetic metallic state of pnictides is doped was also observed for particular model parameters. Results for hole doping and implications for recent experiments that reported electronic nematic states and spin incommensurability are also briefly discussed. C1 [Luo, Qinlong; Moreo, Adriana; Dagotto, Elbio] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Luo, Qinlong; Moreo, Adriana; Dagotto, Elbio] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Yao, Dao-Xin] Sun Yat Sen Univ, Sch Phys & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R China. RP Luo, QL (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. FU US Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; Fundamental Research Funds for the Central Universities [NSFC-11074310] FX This work was supported by the US Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division (Q. L., A. M., E. D.), and the Fundamental Research Funds for the Central Universities and NSFC-11074310 (D.X.Y). The computational studies were performed using the Kraken supercomputer of the National Institute for Computational Sciences and the Newton HPC Cluster at the University of Tennessee. The help of G. Alvarez and R. Yu for the programming of the spin-fermion and HF models is acknowledged. NR 28 TC 12 Z9 12 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 17 PY 2011 VL 83 IS 17 AR 174513 DI 10.1103/PhysRevB.83.174513 PG 5 WC Physics, Condensed Matter SC Physics GA 765LQ UT WOS:000290708100004 ER PT J AU Mendelsberg, RJ Allen, MW Durbin, SM Reeves, RJ AF Mendelsberg, R. J. Allen, M. W. Durbin, S. M. Reeves, R. J. TI Photoluminescence and the exciton-phonon coupling in hydrothermally grown ZnO SO PHYSICAL REVIEW B LA English DT Article ID BOUND-EXCITON; TEMPERATURE-DEPENDENCE; SINGLE-CRYSTALS; BAND-GAP; POLARITON; GERMANIUM; EMISSION; SILICON; ENERGY; STATES AB Near band-edge photoluminescence (PL) from hydrothermally grown bulk ZnO was studied as a function of temperature along with the effects of simultaneous excitation with below-gap photons, allowing for accurate assignment of the emission features not possible from low-temperature data alone. Free exciton emission was clearly observed at low temperatures and dominated the PL spectrum above 100 K. Emission from A excitons bound to three neutral donors dominated the low-temperature PL spectrum. Recombination of B excitons bound to these same neutral donors were also identified along with A excitons bound to the donors in their ionized state. A clear difference in the redshift of free and bound excitons with increasing temperature was observed and attributed to reduced exciton-phonon coupling for the bound excitons. Additionally, Fano resonance of the 1-LO replica of the dominant bound A exciton was observed to reduce its PL intensity which can lead to the misidentification of the 2-LO replica as a donor-acceptor-pair transition. C1 [Mendelsberg, R. J.; Reeves, R. J.] Univ Canterbury, Dept Phys & Astron, Christchurch 1, New Zealand. [Allen, M. W.; Durbin, S. M.] Univ Canterbury, Dept Elect & Comp Engn, Christchurch 1, New Zealand. RP Mendelsberg, RJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM roger.reeves@canterbury.ac.nz OI Allen, Martin/0000-0001-8786-6429 FU Marsden Fund [UOC0604]; MacDiarmid Institute for Advanced Materials and Nanotechnology FX The authors would like to acknowledge Paul Miller, Russel Gillard, Geoff Graham, and Bob Flygenring for their assistance. This work was supported in part by Marsden Fund Grant No. UOC0604 and the MacDiarmid Institute for Advanced Materials and Nanotechnology. NR 42 TC 16 Z9 16 U1 4 U2 40 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 17 PY 2011 VL 83 IS 20 AR 205202 DI 10.1103/PhysRevB.83.205202 PG 8 WC Physics, Condensed Matter SC Physics GA 765NK UT WOS:000290714800008 ER PT J AU Muduli, PK Heinonen, OG Akerman, J AF Muduli, P. K. Heinonen, O. G. Akerman, Johan TI Bias dependence of perpendicular spin torque and of free- and fixed-layer eigenmodes in MgO-based nanopillars SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC TUNNEL-JUNCTIONS; TRANSFER SWITCHING CURRENT; VOLTAGE-DEPENDENCE; MICROWAVE EMISSION; DRIVEN; MAGNETORESISTANCE; OSCILLATORS; MULTILAYERS; CRITERIA; DEVICES AB We have measured the bias voltage and field dependence of eigenmode frequencies in a magnetic tunnel junction with MgO barrier. We show that both free layer (FL) and reference layer (RL) modes are excited, and that a crossover between these modes is observed by varying external field and bias voltage. The bias voltage dependence of the FL and RL modes are shown to be dramatically different. The bias dependence of the FL modes is linear in bias voltage, whereas that of the RL mode is strongly quadratic. Using modeling and micromagnetic simulations, we show that the linear bias dependence of FL frequencies is primarily due to a linear dependence of the perpendicular spin torque on bias voltage, whereas the quadratic dependence of the RL on bias voltage is dominated by the reduction of exchange bias due to Joule heating, and is not attributable to a quadratic dependence of the perpendicular spin torque on bias voltage. C1 [Muduli, P. K.; Akerman, Johan] Univ Gothenburg, Dept Phys, S-41296 Gothenburg, Sweden. [Heinonen, O. G.] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. RP Muduli, PK (reprint author), Univ Gothenburg, Dept Phys, S-41296 Gothenburg, Sweden. EM pranaba.muduli@physics.gu.se RI Akerman, Johan/B-5726-2008; Muduli, Pranaba/B-9334-2008; OI Akerman, Johan/0000-0002-3513-6608; Muduli, Pranaba/0000-0002-0061-8455; Heinonen, Olle/0000-0002-3618-6092 FU Swedish Foundation for Strategic Research (SSF); Swedish Research Council (VR); Goran Gustafsson Foundation; Knut and Alice Wallenberg Foundation; Argonne National Laboratory; UChicago Argonne, LLC [DE-AC02-06CH11357] FX Support from the Swedish Foundation for Strategic Research (SSF), the Swedish Research Council (VR), the Goran Gustafsson Foundation, and the Knut and Alice Wallenberg Foundation are gratefully acknowledged. J.A. is a Royal Swedish Academy of Sciences Research Fellow supported by a grant from the Knut and Alice Wallenberg Foundation. O.H. thanks K. Rivkin for help in setting up the micromagnetic eigenmode calculations, and also acknowledges support from Argonne National Laboratory. Argonne National Laboratory is operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. NR 51 TC 24 Z9 24 U1 1 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 17 PY 2011 VL 83 IS 18 AR 184410 DI 10.1103/PhysRevB.83.184410 PG 8 WC Physics, Condensed Matter SC Physics GA 765MA UT WOS:000290709800006 ER PT J AU Yu, YS Lee, KS Jung, H Choi, YS Yoo, MW Han, DS Im, MY Fischer, P Kim, SK AF Yu, Young-Sang Lee, Ki-Suk Jung, Hyunsung Choi, Youn-Seok Yoo, Myoung-Woo Han, Dong-Soo Im, Mi-Young Fischer, Peter Kim, Sang-Koog TI Polarization-selective vortex-core switching by tailored orthogonal Gaussian-pulse currents SO PHYSICAL REVIEW B LA English DT Article ID SPINTRONICS; FIELD AB We experimentally demonstrate low-power-consumption vortex-core switching in magnetic nanodisks using tailored rotating magnetic fields produced with orthogonal and unipolar Gaussian-pulse currents. The optimal width of the orthogonal pulses and their time delay are found, from analytical and micromagnetic numerical calculations, to be determined only by the angular eigenfrequency omega(D) for a given vortex-state disk of polarization p, such that sigma = 1/omega(D) and Delta t = pi/2p/omega(D). The estimated optimal pulse parameters are in good agreement with the experimental results. This work lays a foundation for energy-efficient information recording in vortex-core cross-point architecture. C1 [Yu, Young-Sang; Lee, Ki-Suk; Jung, Hyunsung; Choi, Youn-Seok; Yoo, Myoung-Woo; Han, Dong-Soo; Kim, Sang-Koog] Seoul Natl Univ, Natl Creat Res Initiat, Ctr Spin Dynam & Spin Wave Devices, Seoul 151744, South Korea. [Yu, Young-Sang; Lee, Ki-Suk; Jung, Hyunsung; Choi, Youn-Seok; Yoo, Myoung-Woo; Han, Dong-Soo; Kim, Sang-Koog] Seoul Natl Univ, Dept Mat Sci & Engn, Res Inst Adv Mat, Nanospin Lab, Seoul 151744, South Korea. [Im, Mi-Young; Fischer, Peter; Kim, Sang-Koog] Univ Calif Berkeley, Lawrence Berkeley Lab, Ctr Xray Opt, Berkeley, CA 94720 USA. RP Kim, SK (reprint author), Seoul Natl Univ, Natl Creat Res Initiat, Ctr Spin Dynam & Spin Wave Devices, Seoul 151744, South Korea. EM sangkoog@snu.ac.kr RI Fischer, Peter/A-3020-2010; MSD, Nanomag/F-6438-2012; Kim, Sang-Koog/J-4638-2014 OI Fischer, Peter/0000-0002-9824-9343; FU Ministry of Education, Science, and Technology [20110000441]; LG YONAM foundation FX This research was supported by the Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science, and Technology (Grant No. 20110000441). S.-K. K. was supported by the LG YONAM foundation under the Professors' Overseas Research Program. Use of the soft x-ray microscope was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy. NR 31 TC 10 Z9 10 U1 0 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 17 PY 2011 VL 83 IS 17 AR 174429 DI 10.1103/PhysRevB.83.174429 PG 7 WC Physics, Condensed Matter SC Physics GA 765LQ UT WOS:000290708100002 ER PT J AU Daugas, JM Matea, I Delaroche, JP Pfutzner, M Sawicka, M Becker, F Belier, G Bingham, CR Borcea, R Bouchez, E Buta, A Dragulescu, E Georgiev, G Giovinazzo, J Girod, M Grawe, H Grzywacz, R Hammache, F Ibrahim, F Lewitowicz, M Libert, J Mayet, P Meot, V Negoita, F Santos, FD Perru, O Roig, O Rykaczewski, K Saint-Laurent, MG Sauvestre, JE Sorlin, O Stanoiu, M Stefan, I Stodel, C Theisen, C Verney, D Zylicz, J AF Daugas, J. M. Matea, I. Delaroche, J-P Pfuetzner, M. Sawicka, M. Becker, F. Belier, G. Bingham, C. R. Borcea, R. Bouchez, E. Buta, A. Dragulescu, E. Georgiev, G. Giovinazzo, J. Girod, M. Grawe, H. Grzywacz, R. Hammache, F. Ibrahim, F. Lewitowicz, M. Libert, J. Mayet, P. Meot, V. Negoita, F. Santos, F. de Oliveira Perru, O. Roig, O. Rykaczewski, K. Saint-Laurent, M. G. Sauvestre, J. E. Sorlin, O. Stanoiu, M. Stefan, I. Stodel, Ch. Theisen, Ch. Verney, D. Zylicz, J. TI beta-decay measurements for N > 40 Mn nuclei and inference of collectivity for neutron-rich Fe isotopes SO PHYSICAL REVIEW C LA English DT Article ID SUBSHELL CLOSURE; HALF-LIVES; DEFORMATION; NI-68; N=40; STATES; ISLAND; MODEL AB A decay spectroscopic study of the neutron-rich isotopes has been performed using fragmentation of a Kr-86 primary beam. Fragments from this reaction have been selected by the LISE2000 spectrometer at the Grand Accelerateur National d'Ions Lourds (GANIL). Half-lives of 29 isotopes, including the first ones identified for Ti-61 (15 +/- 4 ms), V-64 (19 +/- 8 ms), and Fe-71 (28 +/- 5 ms), have been determined and compared with model predictions. Mn-67,Mn-68 beta-delayed gamma rays were observed for the first time. The branching for the beta-delayed neutron emission was measured to be greater than 10(5)% in the Mn-67 decay. The Fe-67 isomeric level is firmly determined at higher energy than assigned in previous works. The excitation energies of the first (2(+)) and (4(+)) states of Fe-68 are suggested to lie at 522(1) and 1389(1) keV, respectively, thus bringing confirmation of assignments based on in-beam gamma-ray spectroscopy. Beyond-mean-field calculations with the Gogny D1S force have been performed for even-mass nuclei through the Fe isotopic chain. Not only Fe-68 but most of the neutron-rich Fe isotopes with neutron numbers below N = 50 are interpreted as soft rotors. The calculated mean occupancy of the neutron g(9/2) and d(5/2) orbitals in correlated ground states is steadily growing with increasing neutron number throughout the isotopic chain. Interpretation of Fe-67 data is based upon the present calculations for the Fe-66 and Fe-68 even cores. C1 [Daugas, J. M.; Delaroche, J-P; Belier, G.; Girod, M.; Meot, V.; Perru, O.; Roig, O.; Sauvestre, J. E.] CEA, DAM, DIF, F-91297 Arpajon, France. [Pfuetzner, M.; Sawicka, M.; Zylicz, J.] Warsaw Univ, Inst Expt Phys, PL-00681 Warsaw, Poland. [Matea, I.; Hammache, F.; Ibrahim, F.; Libert, J.; Stefan, I.; Verney, D.] CNRS, Inst Phys Nucl, IN2P3, F-91406 Orsay, France. [Matea, I.; Hammache, F.; Ibrahim, F.; Libert, J.; Stefan, I.; Verney, D.] Univ Paris 11, F-91406 Orsay, France. [Becker, F.; Grawe, H.; Mayet, P.; Stanoiu, M.] Gesell Schwerionenforsch mbH, D-64291 Darmstadt, Germany. [Bingham, C. R.; Grzywacz, R.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Borcea, R.; Buta, A.; Dragulescu, E.; Negoita, F.; Stanoiu, M.] Horia Hulubei Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Bouchez, E.; Theisen, Ch.] CEA, Ctr Saclay, IRFU, Serv Phys Nucl, F-91191 Gif Sur Yvette, France. [Georgiev, G.] Univ Paris 11, CNRS, IN2P3, CSNSM,UMR 8609, F-91405 Orsay, France. [Giovinazzo, J.] Univ Bordeaux 1, CNRS, IN2P3, Ctr Etud Nucl Bordeaux Gradignan,UMR5797, F-33175 Gradignan, France. [Grzywacz, R.; Rykaczewski, K.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Lewitowicz, M.; Santos, F. de Oliveira; Saint-Laurent, M. G.; Sorlin, O.; Stodel, Ch.] CNRS, IN2P3, CEA, DSM,GANIL, F-14076 Caen 5, France. RP Daugas, JM (reprint author), CEA, DAM, DIF, F-91297 Arpajon, France. RI THEISEN, Christophe/A-9343-2015; Georgiev, Georgi/C-5110-2008; Hammache, Fairouz/K-6132-2016 OI THEISEN, Christophe/0000-0002-8509-1022; Georgiev, Georgi/0000-0003-1467-1764; FU EU; U.S. Department of Energy [DE-AC05-00OR22725]; CNCSIS, Romania [294/2007] FX We are grateful for the technical support provided by the staff of the GANIL facility. This work has been partially supported by the EU Access to Large Scale Facilities Program. The germanium detectors used in this experiment were provided by the EXOGAM collaboration. ORNL is managed by UT-Battelle, LLC, for the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. One of us (A.B.) acknowledges the partial financial support from CNCSIS, Romania, under Grant IDEI No. 294/2007. NR 63 TC 29 Z9 29 U1 0 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 17 PY 2011 VL 83 IS 5 AR 054312 DI 10.1103/PhysRevC.83.054312 PG 12 WC Physics, Nuclear SC Physics GA 765OJ UT WOS:000290717600002 ER PT J AU Andersen, KK Klein, SR AF Andersen, Kristoffer K. Klein, Spencer R. TI High energy cosmic-ray interactions with particles from the Sun SO PHYSICAL REVIEW D LA English DT Article ID BARYON SPECTROSCOPY; CROSS-SECTION; PHOTOPRODUCTION; PROSPECTS; DEUTERON; SPECTRUM; ARIANNA; SURFACE; REGION; RANGE AB Cosmic-ray protons with energies above 10(16) eV passing near the Sun may interact with photons emitted by the Sun and be excited to a Delta(+) resonance. When the Delta(+) decays, it produces pions which further decay to muons and photons which may be detected with terrestrial detectors. A flux of muons, photon pairs (from pi(0) decay), or individual high energy photons coming from near the Sun would be a rather striking signature, and the flux of these particles is a fairly direct measure of the flux of cosmic-ray nucleons, independent of the cosmic-ray composition. In a solid angle within 15 degrees around the Sun, the flux of photon pairs is about 1.3 x 10(-3) particles/(km(2) . yr), while the flux of muons is about 0.33 x 10(-3) particles/(km(2) . yr). This is beyond the reach of current detectors like the Telescope Array, Auger, KASCADE-Grande, or IceCube. However, the muon flux might be detectable by next-generation air-shower arrays or neutrino detectors such as ARIANNA or ARA. We discuss the experimental prospects in some detail. Other cosmic-ray interactions occurring close to the Sun are also briefly discussed. C1 [Andersen, Kristoffer K.] Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus C, Denmark. [Andersen, Kristoffer K.; Klein, Spencer R.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Klein, Spencer R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Andersen, KK (reprint author), Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus C, Denmark. RI Andersen, Kristoffer/A-2160-2015 OI Andersen, Kristoffer/0000-0001-6204-3522 NR 38 TC 1 Z9 1 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 17 PY 2011 VL 83 IS 10 AR 103519 DI 10.1103/PhysRevD.83.103519 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 765PM UT WOS:000290721000003 ER PT J AU Sims, GE Kim, SH AF Sims, Gregory E. Kim, Sung-Hou TI Whole-genome phylogeny of Escherichia coli/Shigella group by feature frequency profiles (FFPs) SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE prokaryotic phylogeny; commensal minimalism; Jensen-Shannon Divergence; phylotyping ID PATHOGENICITY ISLAND; EVOLUTIONARY HISTORY; SHIGELLA-FLEXNERI; COLI STRAINS; SEQUENCE; VIRULENCE; GENE; DIVERGENCE; MAMMALS; DISEASE AB A whole-genome phylogeny of the Escherichia coli/Shigella group was constructed by using the feature frequency profile (FFP) method. This alignment-free approach uses the frequencies of l-mer features of whole genomes to infer phylogenic distances. We present two phylogenies that accentuate different aspects of E. coli/Shigella genomic evolution: (i) one based on the compositions of all possible features of length l = 24 (similar to 8.4 million features), which are likely to reveal the phenetic grouping and relationship among the organisms and (ii) the other based on the compositions of core features with low frequency and low variability (similar to 0.56 million features), which account for similar to 69% of all commonly shared features among 38 taxa examined and are likely to have genome-wide lineal evolutionary signal. Shigella appears as a single clade when all possible features are used without filtering of noncore features. However, results using core features show that Shigella consists of at least two distantly related subclades, implying that the subclades evolved into a single clade because of a high degree of convergence influenced by mobile genetic elements and niche adaptation. In both FFP trees, the basal group of the E. coli/Shigella phylogeny is the B2 phylogroup, which contains primarily uropathogenic strains, suggesting that the E. coli/Shigella ancestor was likely a facultative or opportunistic pathogen. The extant commensal strains diverged relatively late and appear to be the result of reductive evolution of genomes. We also identify clade distinguishing features and their associated genomic regions within each phylogroup. Such features may provide useful information for understanding evolution of the groups and for quick diagnostic identification of each phylogroup. C1 [Sims, Gregory E.; Kim, Sung-Hou] Univ Calif Berkeley, Lawrence Berkeley Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Sims, Gregory E.] J Craig Venter Inst, Dept Informat, Rockville, MD 20850 USA. [Kim, Sung-Hou] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Kim, Sung-Hou] Yonsei Univ, Grad Sch, Dept Integrated OMICS Biomed Sci, Seoul 120749, South Korea. RP Kim, SH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Phys Biosci Div, Berkeley, CA 94720 USA. EM shkim@cchem.berkeley.edu FU Korean Ministry of Science [R31-2008-000-10086-0] FX We thank Dr. Se-Ran Jun for discussion on her similar studies using proteome sequences, and Seong-Yong You for his help with data classification. This work was supported by World Class University Project Grant R31-2008-000-10086-0 from the Korean Ministry of Science. NR 33 TC 52 Z9 55 U1 0 U2 10 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 17 PY 2011 VL 108 IS 20 BP 8329 EP 8334 DI 10.1073/pnas.1105168108 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 765OZ UT WOS:000290719600052 PM 21536867 ER PT J AU Li, H Wang, S Chuang, AY Cohen, BE Chuang, HH AF Li, Hui Wang, Shu Chuang, Alexander Y. Cohen, Bruce E. Chuang, Huai-hu TI Activity-dependent targeting of TRPV1 with a pore-permeating capsaicin analog SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE activity-dependent capsaicinoids; hyperalgesia; ion permeation; selective analgesia ID PROTEIN-KINASE-C; VANILLOID RECEPTOR TRPV1; ACTIVATED ION-CHANNEL; ANALGESIC AGENTS; AGONIST ACTIVITY; NOCICEPTIVE NEURONS; MOLECULAR-BASIS; SELECTIVITY; HEAT; CYSTEINE AB The capsaicin receptor TRPV1 is the principal transduction channel for nociception. Excessive TRPV1 activation causes pathological pain. Ideal pain mangement requires selective inhibition of hyperactive pain-sensing neurons, but sparing normal nociception. We sought to determine whether it is possible to use activity-dependent TRPV1 agonists to identify nerves with excessive TRPV1 activity, as well as exploit the TRPV1 pore to deliver charged anesthetics for neuronal silencing. We synthesized a series of permanently charged capsaicinoids and found that one, cap-ET, efficaciously evoked TRPV1-dependent entry of Ca(2+) or the large cationic dye YO-PRO-1 comparably to capsaicin, but far smaller electrical currents. Cap-ET-induced YO-PRO-1 transport required permeation of both the agonist and the dye through the TRPV1 pore and could be enhanced by kinase activation or oxidative covalent modification. Moreover, cap-ET reduced capsaicin-induced currents by a voltage-dependent block of the pore. A low dose of cap-ET elicited entry of permanently charged Na(+) channel blockers to effectively suppress Na(+) currents in sensory neurons presensitized with oxidative chemicals. These results implicate therapeutic potential of these unique TRPV1 agonists exhibiting activity-dependent ion transport but of minimal pain-producing risks. C1 [Li, Hui; Wang, Shu; Chuang, Huai-hu] Cornell Univ, Dept Biomed Sci, Ithaca, NY 14853 USA. [Chuang, Alexander Y.] Lowell High Sch, San Francisco, CA 94132 USA. [Cohen, Bruce E.] Univ Calif Berkeley, Lawrence Berkeley Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Chuang, HH (reprint author), Cornell Univ, Dept Biomed Sci, Ithaca, NY 14853 USA. EM huai-hu.chuang@cornell.edu RI Wang, Shu/F-2976-2011 FU American Heart Association; Cornell University college FX The authors thank Drs. Robert Oswald, Linda Nowak, Robert Gilmour, and Benjamin R. Myers for critical comments on the manuscript. This work was supported by a Scientist Development Grant from the American Heart Association (to H.-h.C.) and Cornell University college funds. NR 47 TC 10 Z9 11 U1 0 U2 5 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 17 PY 2011 VL 108 IS 20 BP 8497 EP 8502 DI 10.1073/pnas.1018550108 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 765OZ UT WOS:000290719600081 PM 21536874 ER PT J AU Zheng, Y Patel, AB Narayanaswami, V Hura, GL Hang, B Bielicki, JK AF Zheng, Ying Patel, Arti B. Narayanaswami, Vasanthy Hura, Gregory L. Hang, Bo Bielicki, John K. TI HDL Mimetic Peptide ATI-5261 Forms an Oligomeric Assembly in Solution That Dissociates to Monomers upon Dilution SO BIOCHEMISTRY LA English DT Article ID APOLIPOPROTEIN-A-I; HIGH-DENSITY-LIPOPROTEIN; REVERSE CHOLESTEROL TRANSPORT; RANDOMIZED CONTROLLED-TRIAL; CELLULAR CHOLESTEROL; CORONARY ATHEROSCLEROSIS; ALZHEIMERS-DISEASE; INFUSION THERAPY; BINDING DOMAIN; LIPID-BINDING AB ATI-5261 is a 26-mer peptide that stimulates cellular cholesterol efflux with high potency. This peptide displays high aqueous solubility, despite having amphipathic a-helix structure and a broad nonpolar surface. These features suggested to us that ATI-5261 may adopt a specific form in solution, having favorable structural characteristics and dynamics. To test this, we subjected ATI-5261 to a series of biophysical studies and correlated self-association with secondary structure and activity. Gel-filtration chromatography and native gel electrophoresis indicated ATI-5261 adopted a discrete self-associated form of low molecular weight at concentrations >1 mg/ml. Formation of a discrete molecular species was verified by small-angle X-ray scattering (SAXS), which further revealed the peptide formed a tetrameric assembly having an elongated shape and hollow central core. This assembly dissociated to individual peptide strands upon dilution to concentrations required for promoting high-affinity cholesterol efflux from cells, Moreover, the alpha-helical content of ATI-5261 was exceptionally high (74.1 +/- 6.8%) regardless of physical form and concentration. Collectively, these results indicate ATI-5261 displays oligomeric behavior generally similar to native apolipoproteins and dissociates to monomers of high a-helical content upon dilution. Optimizing self-association behavior and secondary structure may prove useful for improving the translatability and efficacy of apolipoprotein mimetic peptides. C1 [Zheng, Ying; Hang, Bo; Bielicki, John K.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Life Sci, Donner Lab, Berkeley, CA 94720 USA. [Patel, Arti B.; Narayanaswami, Vasanthy] Calif State Univ Long Beach, Dept Chem & Biochem, Long Beach, CA 90840 USA. [Narayanaswami, Vasanthy] Childrens Hosp, Oakland Res Inst, Oakland, CA 94609 USA. [Hura, Gregory L.] Univ Calif Berkeley, Lawrence Berkeley Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Bielicki, JK (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Life Sci, Donner Lab, Berkeley, CA 94720 USA. EM jkbielicki@lbl.gov FU Tobacco-Related Disease Research Program (TRDRP) of the state of California [17RT-0082, 17RT-0165]; NIH [R21-HL085791]; United States Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231] FX The work was supported by funds from the Tobacco-Related Disease Research Program (TRDRP) of the state of California grant 17RT-0082 (J.K.B.) and 17RT-0165 (V.N.) and NIH grant R21-HL085791 (J.K.B.). The work was conducted, in part, at Lawrence Berkeley National Laboratory through the United States Department of Energy, Office of Science, Office of Biological and Environmental Research, under contract DE-AC02-05CH11231. Dr. Gregory Hura's contribution was supported by this contract. NR 53 TC 7 Z9 7 U1 0 U2 6 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD MAY 17 PY 2011 VL 50 IS 19 BP 4068 EP 4076 DI 10.1021/bi2002955 PG 9 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 760AP UT WOS:000290293300024 PM 21476522 ER PT J AU Yao, JZ Nellas, RB Glover, MM Shen, TY AF Yao, Jianzhuang Nellas, Ricky B. Glover, Mary M. Shen, Tongye TI Stability and Sugar Recognition Ability of Ricin-like Carbohydrate Binding Domains SO BIOCHEMISTRY LA English DT Article ID RIBOSOME-INACTIVATING PROTEIN; B-CHAIN; COMMUNIS AGGLUTININ; CRYSTAL-STRUCTURE; A-CHAIN; LECTIN; CELLS; GALACTOSE; TOXINS; 2.5-A AB Lectins are a class of proteins known for their novel binding to saccharides. Understanding this sugar recognition process can be crucial in creating structure-based designs of proteins with various biological roles. We focus on the sugar binding of a particular lectin, ricin, which has two a-trefoil carbohydrate-binding domains (CRDs) found in several plant protein toxins. The binding ability of possible sites of ricin-like CRD has been puzzling. The apo and various (multiple) ligand-bound forms of the sugar-binding domains of ricin were studied by molecular dynamics simulations. By evaluating structural stability, hydrogen bond dynamics, flexibility, and binding energy, we obtained a detailed picture of the sugar recognition of the ricin-like CRD. Unlike what was previously believed, we found that the binding abilities of the two known sites are not independent of each other. The binding ability of one site is positively affected by the other site. While the mean positions of different binding scenarios are not altered significantly, the flexibility of the binding pockets visibly decreases upon multiple ligand binding. This change in flexibility seems to be the origin of the binding cooperativity. All the hydrogen bonds that are strong in the monoligand state are also strong in the double-ligand complex, although the stability is much higher in the latter form due to cooperativity. These strong hydrogen bonds in a monoligand state are deemed to be the essential hydrogen bonds. Furthermore, by examining the structural correlation matrix, the two domains are structurally one entity. Galactose hydroxyl groups, OH4 and OH3, are the most critical parts in both site l alpha and site 2 gamma recognition. C1 [Yao, Jianzhuang; Nellas, Ricky B.; Shen, Tongye] Univ Tennessee, Dept Biochem Cellular & Mol Biol, Knoxville, TN 37996 USA. [Yao, Jianzhuang; Nellas, Ricky B.; Glover, Mary M.; Shen, Tongye] Oak Ridge Natl Lab, Ctr Biophys Mol, Oak Ridge, TN 37830 USA. RP Shen, TY (reprint author), Univ Tennessee, Dept Biochem Cellular & Mol Biol, Knoxville, TN 37996 USA. EM tshen@utk.edu RI Shen, Tongye/A-9718-2008 OI Shen, Tongye/0000-0003-1495-3104 NR 39 TC 7 Z9 7 U1 0 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD MAY 17 PY 2011 VL 50 IS 19 BP 4097 EP 4104 DI 10.1021/bi102021p PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 760AP UT WOS:000290293300027 PM 21510689 ER PT J AU Patete, JM Peng, XH Serafin, JM Wong, SS AF Patete, Jonathan M. Peng, Xiaohui Serafin, Joseph M. Wong, Stanislaus S. TI Quantitatively Probing the Means of Controlling Nanoparticle Assembly on Surfaces SO LANGMUIR LA English DT Article ID ENHANCED RAMAN-SCATTERING; GOLD NANOPARTICLES; MARANGONI FLOW; DRYING DROPS; LATEX FILMS; NANOCRYSTALS; SILVER; SPECTROSCOPY; MORPHOLOGY; SUBSTRATE AB As a means of developing a simple, cost-effective, and reliable method for probing nanoparticle behavior, we have used atomic force microscopy to gain a quantitative 3D visual representation of the deposition patterns of citrate-capped Au nanoparticles on a substrate as a function of (a) sample preparation, (b) the choice of substrate, (c) the dispersion solvent, and (d) the number of loading steps. Specifically, we have found that all four parameters can be independently controlled and manipulated in order to alter the resulting pattern and quantity of as-deposited nanoparticles. From these data, the sample preparation technique appears to influence deposition patterns most broadly, and the dispersion solvent is the most convenient parameter to use in tuning the quantity of nanoparticles deposited onto the surface under spin-coating conditions. Indeed, we have quantitatively measured the effect of surface coverage for both mica and silicon substrates under preparation techniques associated with (i) evaporation under ambient air, (ii) heat treatment, and (iii) spin-coating preparation conditions. In addition, we have observed a decrease in nanoparticle adhesion to a substrate when the ethylene glycol content of the colloidal dispersion solvent is increased, which had the effect of decreasing interparticle-substrate interactions. Finally, we have shown that substrates prepared by these diverse techniques have potential applicability in surface-enhanced Raman spectroscopy. C1 [Patete, Jonathan M.; Peng, Xiaohui; Wong, Stanislaus S.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Serafin, Joseph M.] St Johns Univ, Dept Chem, Queens, NY 11439 USA. [Wong, Stanislaus S.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Wong, SS (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM sswong@notes.cc.sunysb.edu FU U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX We acknowledge the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division for facility and personnel (including PI) support. S.S.W. thanks the Alfred P. Sloan Foundation for experimental supplies necessary for the synthesis reactions. Dr. James Quinn is also acknowledged for assistance with the scanning electron microscopy data. In addition, we thank Christopher Koenigsmann, Alexander Santulli, and Amanda Tiano for engaging in valuable discussions and making helpful comments. NR 62 TC 2 Z9 2 U1 1 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAY 17 PY 2011 VL 27 IS 10 BP 5792 EP 5805 DI 10.1021/la105082a PG 14 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 760AL UT WOS:000290292900010 PM 21491942 ER PT J AU Soto-Cantu, E Lokitz, BS Hinestrosa, JP Deodhar, C Messman, JM Ankner, JF Kilbey, SM AF Soto-Cantu, Erick Lokitz, Bradley S. Hinestrosa, Juan Pablo Deodhar, Chaitra Messman, Jamie M. Ankner, John F. Kilbey, S. Michael, II TI Versatility of Alkyne-Modified Poly(Glycidyl Methacrylate) Layers for Click Reactions SO LANGMUIR LA English DT Article ID TRANSFER RADICAL POLYMERIZATION; RAFT POLYMERIZATION; SURFACE MODIFICATION; CHEMISTRY; BRUSHES; COPOLYMERS; ACID; POLYMERS; FUNCTIONALITY; NANOPARTICLES AB Functional soft interfaces are of interest for a variety of technologies. We describe three methods for preparing substrates with alkyne groups, which show versatility for "click" chemistry reactions. Two of the methods have the same root: formation of thin, covalently attached, reactive interfacial layers of poly(glycidyl methacrylate) (PGMA) via spin coating onto silicon wafers followed by reactive modification with either propargylamine or 5-heicynoic acid. The amine or the carboxylic acid moieties react with the epoxy groups of PGMA, creating interfacial polymer layers decorated with alkyne groups. The third method consists of using copolymers comprising glycidyl methacrylate and propargyl methacrylate (pGP). The pGP copolymers are spin coated and covalently attached on silicon wafers. For each method, we investigate the factors that control film thickness and content of alkyne groups using ellipsometry, and study the nanophase structure of the films using neutron reflectometry. Azide-terminated polymers of methacrylic acid and 2-vinyl-4, 4-dimethylazlactone synthesized via reversible addition - fragmentation chain transfer polymerization were attached to the alkyne-modified substrates using "click" chemistry, and grafting densities in the range of 0.007-0.95 chains nm(-2) were attained. The maximum density of alkyne groups attained by functionalization of PGMA with propargylamine or 5-hexynoic acid was approximately 2 allcynes nm(-3). The allcyne content obtained by the three decorating approaches was sufficiently high that it was not the limiting factor for the click reaction of azide-capped polymers. C1 [Soto-Cantu, Erick; Deodhar, Chaitra; Kilbey, S. Michael, II] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Ankner, John F.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Hinestrosa, Juan Pablo] Clemson Univ, Dept Chem & Biomol Engn, Clemson, SC 29634 USA. [Lokitz, Bradley S.; Messman, Jamie M.; Kilbey, S. Michael, II] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Kilbey, SM (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM mkilbey@utk.edu RI Lokitz, Bradley/Q-2430-2015; OI Lokitz, Bradley/0000-0002-1229-6078; Ankner, John/0000-0002-6737-5718 FU National Science Foundation; Transport program [0840249]; Center for Nanophase Materials Sciences [2005-024, 2008-297]; Spallation Neutron Source [IPTS-2606, IPTS-1823]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX E S.-C., C.D., and S.M.K II gratefully acknowledge support from the National Science Foundation through the Chemical, Bioengineering, Environmental. and Transport program (Award No. 0840249). A portion of this research was conducted at the Center for Nanophase Materials Sciences (User Proposal Nos. 2005-024 and 2008-297) and Spallation Neutron Source (User Proposals IPTS-2606 and IPTS-1823), which are both located at Oak Ridge National Laboratory and sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 54 TC 29 Z9 29 U1 4 U2 73 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAY 17 PY 2011 VL 27 IS 10 BP 5986 EP 5996 DI 10.1021/la2000798 PG 11 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 760AL UT WOS:000290292900031 PM 21506527 ER PT J AU Cordeiro, PJ Tilley, TD AF Cordeiro, Paul J. Tilley, T. Don TI Enhancement of Epoxidation Efficiencies for Ta-SBA15 Catalysts. The Influence of Modification with -EMe3 (E = Si, Ge, Sn) Groups SO LANGMUIR LA English DT Article ID AQUEOUS HYDROGEN-PEROXIDE; LIQUID-PHASE OXIDATION; SUPPORTED TANTALUM CATALYSTS; MOLECULAR PRECURSOR APPROACH; BAEYER-VILLIGER OXIDATIONS; OLEFIN EPOXIDATION; MESOPOROUS SILICA; SELECTIVE OXIDATION; ACTIVE-SITES; STRUCTURAL-CHARACTERIZATION AB Site-isolated Ta(V) centers were introduced onto the surface of a mesoporous SBA-15 support via the thermolytic molecular precursor method. After thermal treatment under oxygen, the resulting Si OH and Ta OH sites of TaSBA15-O-2 were modified with a series of trimethyl group 14 species, Me3E-, by treatment with Me3E-NMe2 (E = Si, Ge, Sn) reagents. The resulting surface-modified catalysts (Me3E)(cap)TaSBA15 exhibit a significantly increased rate of cyclohexene epoxidation with H2O2 as an oxidant, and provided a decreased amount of allylic oxidation products with respect to the unmodified material, TaSBA15-O-2. The rate of nonproductive H2O2 decomposition, as monitored via H-1-NMR spectroscopy, significantly decreased after the surface modification. The structure of the TaSBA15 catalysts and potential Ta(V) epoxidation intermediates (formed upon treatment of Ta(V) materials with H2O2) were probed using UV-visible absorbance and diffuse-reflectance UV visible spectroscopy. A Ta(V)(eta(2)-O-2) intermediate species is proposed for the TaSBA15-O-2, (Me3Si)(cap)TaSBA15, and (Me3Ge)(cap)TaSBA15 catalysts, while intermediate species for the (Me3Sn)(cap)TaSBA15 catalysts could not be characterized. C1 [Tilley, T. Don] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Cordeiro, Paul J.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Cordeiro, Paul J.; Tilley, T. Don] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Tilley, TD (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM tdtilley@berkeley.edu FU Office of Energy Research, Office of Baisc Energy Sciences, Chemical Sciences division, of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors gratefully acknowledge the support of the Director, Office of Energy Research, Office of Baisc Energy Sciences, Chemical Sciences division, of the U.S. Department of Energy under contract DE-AC02-05CH11231. We thank Professor A. P. Alivisatos of the University of California, Berkeley for the use of instrumentation (TEM, SAXS, PXRD). NR 90 TC 15 Z9 15 U1 3 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAY 17 PY 2011 VL 27 IS 10 BP 6295 EP 6304 DI 10.1021/la200090u PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 760AL UT WOS:000290292900067 PM 21517024 ER PT J AU Coppe, JP Xu, ZD Chen, Y Liu, GL AF Coppe, Jean-Philippe Xu, Zhida Chen, Yi Liu, G. Logan TI Metallic nanocone array photonic substrate for high-uniformity surface deposition and optical detection of small molecules SO NANOTECHNOLOGY LA English DT Article ID MICROARRAYS AB Molecular probe arrays printed on solid surfaces such as DNA, peptide, and protein microarrays are widely used in chemical and biomedical applications especially genomic and proteomic studies (Pollack et al 1999 Nat. Genet. 23 41-6, Houseman et al 2002 Nat. Biotechnol. 20 270-4, Sauer et al 2005 Nat. Rev. Genet. 6 465-76) as well as surface imaging and spectroscopy (Mori et al 2008 Anal. Biochem. 375 223-31, Liu et al 2006 Nat. Nanotechnol. 1 47-52, Liu 2010 IEEE J. Sel. Top. Quantum Electron. 16 662-71). Unfortunately the printed molecular spots on solid surfaces often suffer low distribution uniformity due to the lingering 'coffee stain' (Deegan et al 1997 Nature 389 827-9) problem of molecular accumulations and blotches, especially around the edge of deposition spots caused by solvent evaporation and convection processes. Here we present, without any surface chemistry modification, a unique solid surface of high-aspect-ratio silver-coated silicon nanocone arrays that allows highly uniform molecular deposition and thus subsequent uniform optical imaging and spectroscopic molecular detection. Both fluorescent Rhodamine dye molecules and unlabeled oligopeptides are printed on the metallic nanocone photonic substrate surface as circular spot arrays. In comparison with the printed results on ordinary glass slides and silver-coated glass slides, not only high printing density but uniform molecular distribution in every deposited spot is achieved. The high-uniformity and repeatability of molecular depositions on the 'coffee stain'-free nanocone surface is confirmed by laser scanning fluorescence imaging and surface enhanced Raman imaging experiments. The physical mechanism for the uniform molecular deposition is attributed to the superhydrophobicity and localized pinned liquid-solid-air interface on the silver-coated silicon nanocone surface. The unique surface properties of the presented nanocone surface enabled high-density, high-uniformity probe spotting beneficial for genomic and proteomic microarrays and surface molecular imaging. C1 [Xu, Zhida; Chen, Yi; Liu, G. Logan] Univ Illinois, Dept Elect & Comp Engn, Micro & Nanotechnol Lab, Urbana, IL 61801 USA. [Coppe, Jean-Philippe] Kinogea Inc, Berkeley, CA 94704 USA. [Coppe, Jean-Philippe] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Life Sci, Berkeley, CA 94720 USA. [Liu, G. Logan] Univ Illinois, Dept Bioengn, Urbana, IL 61801 USA. RP Liu, GL (reprint author), Univ Illinois, Dept Elect & Comp Engn, Micro & Nanotechnol Lab, 1406 W Green St, Urbana, IL 61801 USA. EM loganliu@illinois.edu RI Chen, Yi/E-9781-2010 OI Chen, Yi/0000-0002-2047-724X FU Illinois ECE; NIH/NCI; NIH FX We thank Illinois ECE startup funding and an NIH/NCI SCCNE Nanotechnology grant for support and Kinogea Inc. for providing the laser scanning Raman microspectroscopic system. This work was supported in part by grants from NIH. NR 25 TC 11 Z9 11 U1 2 U2 24 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 J9 NANOTECHNOLOGY JI Nanotechnology PD MAY 17 PY 2011 VL 22 IS 24 AR 245710 DI 10.1088/0957-4484/22/24/245710 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 759AZ UT WOS:000290213500040 PM 21543836 ER PT J AU Guan, WH Park, JH Krstic, PS Reed, MA AF Guan, Weihua Park, Jae Hyun Krstic, Predrag S. Reed, Mark A. TI Non-vanishing ponderomotive AC electrophoretic effect for particle trapping SO NANOTECHNOLOGY LA English DT Article ID SUBMICROMETER LATEX SPHERES; COLLOIDAL PARTICLES; DIELECTROPHORESIS; SEPARATION; FORCES; MOTION; FIELDS; TRAPS; CELLS AB We present here a study on overlooked aspects of alternating current (AC) electrokinetics-AC electrophoretic (ACEP) phenomena. The dynamics of a particle with both polarizability and net charges in a non-uniform AC electric trapping field is investigated. It is found that either electrophoretic (EP) or dielectrophoretic (DEP) effects can dominate the trapping dynamics, depending on experimental conditions. A dimensionless parameter gamma is developed to predict the relative strength of EP and DEP effects in a quadrupole AC field. An ACEP trap is feasible for charged particles in 'salt-free' or low salt concentration solutions. In contrast to DEP traps, an ACEP trap favors the downscaling of the particle size. C1 [Guan, Weihua; Reed, Mark A.] Yale Univ, Dept Elect Engn, New Haven, CT 06520 USA. [Park, Jae Hyun; Krstic, Predrag S.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RP Guan, WH (reprint author), Yale Univ, Dept Elect Engn, New Haven, CT 06520 USA. EM mark.reed@yale.edu RI Guan, Weihua/C-5030-2008 OI Guan, Weihua/0000-0002-8435-9672 FU US National Human Genome Research Institute of the National Institutes of Health [1R21HG004764-01] FX This research is supported by the US National Human Genome Research Institute of the National Institutes of Health under grant no. 1R21HG004764-01. NR 33 TC 5 Z9 5 U1 0 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 J9 NANOTECHNOLOGY JI Nanotechnology PD MAY 17 PY 2011 VL 22 IS 24 AR 245103 DI 10.1088/0957-4484/22/24/245103 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 759AZ UT WOS:000290213500003 PM 21508497 ER PT J AU Kim, DH Kim, YK Hong, S Kim, Y Baik, S AF Kim, Dae Hong Kim, Yong Kwan Hong, Seungbum Kim, Yunseok Baik, Sunggi TI Nanoscale bit formation in highly (111)-oriented ferroelectric thin films deposited on glass substrates for high-density storage media SO NANOTECHNOLOGY LA English DT Article ID ATOMIC-FORCE MICROSCOPY; ADHESION LAYERS; PBTIO3; PT(001)/MGO(001); POLARIZATION; TECHNOLOGY; ELECTRODES; DEPENDENCE; MEMORIES; SCALE AB PbTiO3 ( PTO) ferroelectric films on Pt(111) bottom electrode layers covering Ta/glass were prepared using pulsed laser deposition. X-ray diffraction patterns revealed that the PTO films were preferentially (111)-oriented. The films were highly crystalline and had a smooth surface with root mean square (RMS) roughness of 1.5 nm. Ferroelectric properties of the PTO films were characterized using piezoresponse force microscopy (PFM). PFM techniques achieved ferroelectric polarization bits with a minimum width of 22 nm, which corresponds to a potential recording density of 1.3 Tbit/in(2) in ferroelectric storage devices. C1 [Kim, Dae Hong; Baik, Sunggi] Pohang Univ Sci & Technol POSTECH, Dept Mat Sci & Engn, Pohang 790784, South Korea. [Kim, Yong Kwan] Samsung Elect Co Ltd, Semicond R&D Ctr, Hwasung 445701, South Korea. [Hong, Seungbum] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Kim, Yunseok] Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Taejon 305701, South Korea. RP Kim, DH (reprint author), Pohang Univ Sci & Technol POSTECH, Dept Mat Sci & Engn, Pohang 790784, South Korea. EM sgbaik@postech.ac.kr RI Hong, Seungbum/B-7708-2009 OI Hong, Seungbum/0000-0002-2667-1983 FU Samsung Electronics; US DOE Office of Science Laboratory [DE-AC02-06CH11357] FX The authors gratefully acknowledge the financial support of Samsung Electronics. The submitted manuscript has been in part created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ('Argonne'). Argonne, a US DOE Office of Science Laboratory, operated under contract No. DE-AC02-06CH11357. NR 44 TC 6 Z9 6 U1 1 U2 15 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD MAY 17 PY 2011 VL 22 IS 24 AR 245705 DI 10.1088/0957-4484/22/24/245705 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 759AZ UT WOS:000290213500035 PM 21508503 ER PT J AU Santulli, AC Koenigsmann, C Tiano, AL DeRosa, D Wong, SS AF Santulli, Alexander C. Koenigsmann, Christopher Tiano, Amanda L. DeRosa, Donald Wong, Stanislaus S. TI Correlating titania morphology and chemical composition with dye-sensitized solar cell performance SO NANOTECHNOLOGY LA English DT Article ID NANOCRYSTALLINE TIO2 FILMS; CONVERSION EFFICIENCY; ZINC PHTHALOCYANINE; ELECTRON LIFETIME; NANOTUBE ARRAYS; HOLE COLLECTOR; ANATASE; NANOSTRUCTURES; DIOXIDE; LAYER AB We have investigated the use of various morphologies, including nanoparticles, nanowires, and sea-urchins of TiO(2) as the semiconducting material used as components of dye-sensitized solar cells (DSSCs). Analysis of the solar cells under AM 1.5 solar irradiation reveals the superior performance of hydrothermally derived nanoparticles, by comparison with two readily available commercial nanoparticle materials, within the DSSC architecture. The sub-structural morphology of films of these nanostructured materials has been directly characterized using SEM and indirectly probed using dye desorption. Furthermore, the surfaces of these nanomaterials were studied using TEM in order to visualize their structure, prior to their application within DSSCs. Surface areas of the materials have been quantitatively analyzed by collecting BET adsorption and dye desorption data. Additional investigation using open circuit voltage decay measurements reveals the efficiency of electron conduction through each TiO(2) material. Moreover, the utilization of various chemically distinctive titanate materials within the DSSCs has also been investigated, demonstrating the deficiencies of using these particular chemical compositions within traditional DSSCs. C1 [Santulli, Alexander C.; Koenigsmann, Christopher; Tiano, Amanda L.; Wong, Stanislaus S.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [DeRosa, Donald] SUNY Albany, Coll Nanoscale Sci & Engn, Albany, NY 12203 USA. [Wong, Stanislaus S.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Wong, SS (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM sswong@notes.cc.sunysb.edu FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX We acknowledge the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division for PI and student support as well as for experimental supplies. This work was also conducted with the use of facilities at the Center for Functional Nanomaterials (CFN) at Brookhaven National Laboratory. We also acknowledge assistance from Dr Martin Schoonen for his help with the BET experiments. NR 82 TC 13 Z9 13 U1 1 U2 25 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 J9 NANOTECHNOLOGY JI Nanotechnology PD MAY 17 PY 2011 VL 22 IS 24 AR 245402 DI 10.1088/0957-4484/22/24/245402 PG 13 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 759AZ UT WOS:000290213500017 PM 21508451 ER PT J AU Huang, SW Lin, YY You, EM Liu, TT Shu, HY Wu, KM Tsai, SF Lo, CF Kou, GH Ma, GC Chen, M Wu, DY Aoki, T Hirono, I Yu, HT AF Huang, Shiao-Wei Lin, You-Yu You, En-Min Liu, Tze-Tze Shu, Hung-Yu Wu, Keh-Ming Tsai, Shih-Feng Lo, Chu-Fang Kou, Guang-Hsiung Ma, Gwo-Chin Chen, Ming Wu, Dongying Aoki, Takashi Hirono, Ikuo Yu, Hon-Tsen TI Fosmid library end sequencing reveals a rarely known genome structure of marine shrimp Penaeus monodon SO BMC GENOMICS LA English DT Article ID SPOT SYNDROME VIRUS; NON-LTR RETROTRANSPOSONS; PENELOPE-LIKE ELEMENTS; IMMUNE-RELATED GENES; LITOPENAEUS-VANNAMEI; MICROSATELLITE REPEATS; TRANSPOSABLE ELEMENTS; ANOPHELES-GAMBIAE; MOLECULAR-CLONING; MALARIA MOSQUITO AB Background: The black tiger shrimp (Penaeus monodon) is one of the most important aquaculture species in the world, representing the crustacean lineage which possesses the greatest species diversity among marine invertebrates. Yet, we barely know anything about their genomic structure. To understand the organization and evolution of the P. monodon genome, a fosmid library consisting of 288,000 colonies and was constructed, equivalent to 5.3-fold coverage of the 2.17 Gb genome. Approximately 11.1 Mb of fosmid end sequences (FESs) from 20,926 non-redundant reads representing 0.45% of the P. monodon genome were obtained for repetitive and protein-coding sequence analyses. Results: We found that microsatellite sequences were highly abundant in the P. monodon genome, comprising 8.3% of the total length. The density and the average length of microsatellites were evidently higher in comparison to those of other taxa. AT-rich microsatellite motifs, especially poly (AT) and poly (AAT), were the most abundant. High abundance of microsatellite sequences were also found in the transcribed regions. Furthermore, via self-BlastN analysis we identified 103 novel repetitive element families which were categorized into four groups, i.e., 33 WSSV-like repeats, 14 retrotransposons, 5 gene-like repeats, and 51 unannotated repeats. Overall, various types of repeats comprise 51.18% of the P. monodon genome in length. Approximately 7.4% of the FESs contained protein-coding sequences, and the Inhibitor of Apoptosis Protein (IAP) gene and the Innexin 3 gene homologues appear to be present in high abundance in the P. monodon genome. Conclusions: The redundancy of various repeat types in the P. monodon genome illustrates its highly repetitive nature. In particular, long and dense microsatellite sequences as well as abundant WSSV-like sequences highlight the uniqueness of genome organization of penaeid shrimp from those of other taxa. These results provide substantial improvement to our current knowledge not only for shrimp but also for marine crustaceans of large genome size. C1 [Huang, Shiao-Wei; Lin, You-Yu; You, En-Min; Lo, Chu-Fang; Kou, Guang-Hsiung; Chen, Ming; Yu, Hon-Tsen] Natl Taiwan Univ, Inst Zool, Taipei 10617, Taiwan. [Huang, Shiao-Wei; Lin, You-Yu; You, En-Min; Lo, Chu-Fang; Kou, Guang-Hsiung; Chen, Ming; Yu, Hon-Tsen] Natl Taiwan Univ, Dept Life Sci, Taipei 10617, Taiwan. [Liu, Tze-Tze; Shu, Hung-Yu] Natl Yang Ming Univ, Genome Res Ctr, Taipei 112, Taiwan. [Wu, Keh-Ming; Tsai, Shih-Feng] Natl Hlth Res Inst, Div Mol & Genom Med, Kawagoe, Saitama 350, Japan. [Ma, Gwo-Chin; Chen, Ming] Changhua Christian Hosp, Ctr Med Genet, Changhua 500, Taiwan. [Ma, Gwo-Chin; Chen, Ming] Changhua Christian Hosp, Genet Lab, Dept Med Res, Changhua 500, Taiwan. [Chen, Ming] Natl Taiwan Univ, Coll Med, Dept Obstet & Gynecol, Taipei 106, Taiwan. [Wu, Dongying] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. [Wu, Dongying] Univ Calif Davis, Dept Ecol & Evolut, Genome Ctr, Davis, CA 95616 USA. [Aoki, Takashi; Hirono, Ikuo] Tokyo Univ Marine Sci & Technol, Lab Genome Sci, Minato Ku, Tokyo 1088477, Japan. RP Yu, HT (reprint author), Natl Taiwan Univ, Inst Zool, Taipei 10617, Taiwan. EM ayu@ntu.edu.tw RI Tsai, Shih-Feng/E-3997-2010; Lo, Chu-Fang/G-3088-2014; HIRONO, Ikuo/O-1940-2014; OI Lo, Chu-Fang/0000-0001-5136-8129; Chen, Ming/0000-0001-5076-2917 FU National Science Council of Taiwan, ROC [952317B002008, 962317B002012]; National Taiwan University, ROC [97R006628, 98R006628] FX We thank Wen-Hsiung Li, Manyuan Long, Kevin Bullaughey and two anonymous reviewers for their helpful comments. We also thank Chung-Yen Lin and his lab for technical support in bioinformatic analysis. Financial support was granted to Hon-Tsen Yu by the National Science Council of Taiwan, ROC (952317B002008 and 962317B002012), and the National Taiwan University, ROC (97R006628 and 98R006628). NR 67 TC 12 Z9 12 U1 1 U2 13 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD MAY 17 PY 2011 VL 12 AR 242 DI 10.1186/1471-2164-12-242 PG 19 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA 784FU UT WOS:000292142500001 PM 21575266 ER PT J AU Anglani, R Mannarelli, M Ruggieri, M AF Anglani, Roberto Mannarelli, Massimo Ruggieri, Marco TI Collective modes in the color flavor-locked phase SO NEW JOURNAL OF PHYSICS LA English DT Article ID DENSE QUARK MATTER; BLACK-HOLE EVAPORATION; DYNAMICAL MODEL; CFL PHASE; QCD; SUPERCONDUCTIVITY; EVOLUTION; LOCKING; ANALOGY AB We study the low-energy effective action for some collective modes of the color flavor-locked (CFL) phase of QCD. This phase of matter has long been known to be a superfluid because by picking a phase its order parameter breaks the quark-number U(1)(B) symmetry spontaneously. We consider the modes describing fluctuations in the magnitude of the condensate, namely the Higgs mode, and in the phase of the condensate, namely the Nambu-Goldstone (NG) (or Anderson-Bogoliubov) mode associated with the breaking of U(1)(B). By employing as microscopic theory the Nambu-Jona-Lasinio model, we reproduce known results for the Lagrangian of the NG field to the leading order in the chemical potential and extend such results evaluating corrections due to the gap parameter. Moreover, we determine the interaction terms between the Higgs and the NG field. This study paves the way for a more reliable study of various dissipative processes in rotating compact stars with a quark matter core in the CFL phase. C1 [Mannarelli, Massimo] Univ Barcelona, Dept Estruct & Constituents Mat, E-08028 Barcelona, Spain. [Mannarelli, Massimo] Univ Barcelona, Inst Ciencies Cosmos, E-08028 Barcelona, Spain. [Anglani, Roberto] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Anglani, Roberto] CNR, Inst Intelligent Syst Automat, I-70126 Bari, Italy. [Mannarelli, Massimo] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, Assergi, AQ, Italy. [Ruggieri, Marco] Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan. RP Mannarelli, M (reprint author), Univ Barcelona, Dept Estruct & Constituents Mat, Marti i Franques 1, E-08028 Barcelona, Spain. EM massimo.mannarelli@lngs.infn.it FU INFN-MICINN [FPA2008-03918E]; US Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357]; Centro Nacional de Fisica de Particulas, Astroparticulas y Nuclear (CPAN); Ministerio de Educacion y Ciencia (MEC) [FPA2007-66665, 2009SGR502]; JSPS [P09028] FX We thank H Abuki, M Alford, C Manuel and M Nitta for comments and suggestions. This work has been supported in part by the INFN-MICINN grant with reference number FPA2008-03918E. The work of RA was supported in part by the US Department of Energy, Office of Nuclear Physics, contract no. DE-AC02-06CH11357. The work of MM was supported by the Centro Nacional de Fisica de Particulas, Astroparticulas y Nuclear (CPAN) and by the Ministerio de Educacion y Ciencia (MEC) under grant nos FPA2007-66665 and 2009SGR502. The work of MR was supported by JSPS under contract number P09028. NR 49 TC 9 Z9 9 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD MAY 17 PY 2011 VL 13 AR 055002 DI 10.1088/1367-2630/13/5/055002 PG 21 WC Physics, Multidisciplinary SC Physics GA 782IO UT WOS:000292001900002 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruuhwirth, R Ghete, VM Hammer, J Nsel, SH Hartl, C Hoch, M Hormann, N Hrubec, J Jeitler, M Kasieczka, G Kiesenhofer, W Krammer, M Liko, D Mikulec, I Pernicka, M Rohringer, H Schofbeck, R Strauss, J Taurok, A Teischinger, F Wagner, P Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Benucci, L Cerny, K DeWolf, EA Janssen, X Maes, T Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Beauceron, S Blekman, F Blyweert, S D'Hondt, J Devroede, O Suarez, RG Kalogeropoulos, A Maes, J Maes, M Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Charaf, O Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hammad, GH Hreus, T Marage, PE Thomas, L Velde, CV Vanlaer, P Wickens, J Adler, V Costantini, S Grunewald, M Klein, B Marinov, A Mccartin, J Ryckbosch, D Thyssen, F Tytgat, M Vanelderen, L Verwilligen, P Walsh, S Zaganidis, N Basegmez, S Bruno, G Caudron, J Ceard, L De Jeneret, JD Delaere, C Demin, P Favart, D Giammanco, A Gregoire, G Hollar, J Lemaitre, V Liao, J Militaru, O Ovyn, S Pagano, D Pin, A Piotrzkowski, K Schul, N Beliy, N Caebergs, T Daubie, E Alves, GA Damiao, DD Pol, ME Souza, MHG Carvalho, W Da Costa, EM Martins, CD De Souza, SF Mundim, L Nogima, H Oguri, V Da Silva, WLP Santoro, A Do Amaral, SMS Sznajder, A De Araujo, FTD Dias, FA Dias, MAF Tomei, TRFP Gregores, EM Marinho, F Novaes, SF Padula, SS Darmenov, N Dimitrov, L Genchev, V Iaydjiev, P Piperov, S Rodozov, M Stoykova, S Sultanov, G Tcholakov, V Trayanov, R Vankov, I Dyulendarova, M Hadjiiska, R Kozhuharov, V Litov, L Marinova, E Mateev, M Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Wang, J Wang, J Wang, X Wang, Z Xu, M Yang, M Zang, J Zhang, Z Ban, Y Guo, S Guo, Y Li, W Mao, Y Qian, SJ Teng, H Zhang, L Zhu, B Zou, W Cabrera, A Moreno, BG Rios, AAO Oliveros, AFO Sanabria, JC Godinovic, N Lelas, D Lelas, K Plestina, R Polic, D Puljak, I Antunovic, Z Dzelalija, M Brigljevic, V Duric, S Kadija, K Morovic, S Attikis, A Galanti, M Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Assran, Y Mahmoud, MA Hektor, A Kadastik, M Kannike, K Muntel, M Raidal, M Rebane, L Azzolini, V Eerola, P Czellar, S Harkonen, J Heikkinen, A Karimaki, V Kinnunen, R Klem, J Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Tuominen, E Tuominiemi, J Tuovinen, E Ungaro, D Wendland, L Banzuzi, K Korpela, A Tuuva, T Sillou, D Besancon, M Choudhury, S Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Gentit, FX Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Marionneau, M Millischer, L Rander, J Rosowsky, A Shreyber, I Titov, M Verrecchia, P Baffioni, S Beaudette, F Bianchini, L Bluj, M Broutin, C Busson, P Charlot, C Dahms, T Dobrzynski, L de Cassagnac, RG Haguenauer, M Mine, P Mironov, C Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Thiebaux, C Wyslouch, B Zabi, A Agram, JL Andrea, J Besson, A Bloch, D Bodin, D Brom, JM Cardaci, M Chabert, EC Collard, C Conte, E Drouhin, F Ferro, C Fontaine, JC Gele, D Goerlach, U Greder, S Juillot, P Karim, M Le Bihan, AC Mikami, Y Van Hove, P Fassi, F Mercier, D Baty, C Beaupere, N Bedjidian, M Bondu, O Boudoul, G Boumediene, D Brun, H Chanon, N Chierici, R Contardo, D Depasse, P El Mamouni, H Falkiewicz, A Fay, J Gascon, S Ille, B Kurca, T Le Grand, T Lethuillier, M Mirabito, L Perries, S Sordini, V Tosi, S Tschudi, Y Verdier, P Xiao, H Megrelidze, L Roinishvili, V Lomidze, D Anagnostou, G Edelhoff, M Feld, L Heracleous, N Hindrichs, O Jussen, R Klein, K Merz, J Mohr, N Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Weber, M Wittmer, B Ata, M Bender, W Erdmann, M Frangenheim, J Hebbeker, T Hinzmann, A Hoepfner, K Hof, C Klimkovich, T Klingebiel, D Kreuzer, P Lanske, D Magass, C Masetti, G Merschmeyer, M Meyer, A Papacz, P Pieta, H Reithler, H Schmitz, SA Sonnenschein, L Steggemann, J Teyssier, D Bontenackels, M Davids, M Duda, M Flugge, G Geenen, H Giffels, M Ahmad, WH Heydhausen, D Kress, T Kuessel, Y Linn, A Nowack, A Perchalla, L Pooth, O Rennefeld, J Sauerland, P Stahl, A Thomas, M Tornier, D Zoeller, MH Martin, MA Behrenhoff, W Behrens, U Bergholz, M Borras, K Cakir, A Campbell, A Castro, E Dammann, D Eckerlin, G Eckstein, D Flossdorf, A Flucke, G Geiser, A Glushkov, I Hauk, J Jung, H Kasemann, M Katkov, I Katsas, P Kleinwort, C Kluge, H Knutsson, A Kruucker, D Kuznetsova, E Lange, W Lohmann, W Mankel, R Marienfeld, M Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Olzem, J Parenti, A Raspereza, A Raval, A Schmidt, R Schoerner-Sadenius, T Sen, N Stein, M Tomaszewska, J Volyanskyy, D Walsh, R Wissing, C Autermann, C Bobrovskyi, S Draeger, J Enderle, H Gebbert, U Kaschube, K Kaussen, G Klanner, R Lange, J Mura, B Naumann-Emme, S Nowak, F Pietsch, N Sander, C Schettler, H Schleper, P Schroder, M Schum, T Schwandt, J Srivastava, AK Stadie, H Steinbruck, G Thomsen, J Wolf, R Barth, C Bauer, J Buege, V Chwalek, T De Boer, W Dierlamm, A Dirkes, G Feindt, M Gruschke, J Hackstein, C Hartmann, F Heindl, SM Heinrich, M Held, H Hoffmann, KH Honc, S Kuhr, T Martschei, D Mueller, S Muller, T Niegel, M Oberst, O Oehler, A Ott, J Peiffer, T Piparo, D Quast, G Rabbertz, K Ratnikov, F Renz, M Saout, C Scheurer, A Schieferdecker, P Schilling, FP Schott, G Simonis, HJ Stober, FM Troendle, D Wagner-Kuhr, J Zeise, M Zhukov, V Ziebarth, EB Daskalakis, G Geralis, T Kesisoglou, S Kyriakis, A Loukas, D Manolakos, I Markou, A Markou, C Mavrommatis, C Ntomari, E Petrakou, E Gouskos, L Mertzimekis, TJ Panagiotou, A Evangelou, I Foudas, C Kokkas, P Manthos, N Papadopoulos, I Patras, V Triantis, FA Aranyi, A Bencze, G Boldizsar, L Debreczeni, G Hajdu, C Horvath, D Kapusi, A Krajczar, K Laszlo, A Sikler, F Vesztergombi, G Beni, N Molnar, J Palinkas, J Szillasi, Z Veszpremi, V Raics, P Trocsanyi, ZL Ujvari, B Bansal, S Beri, SB Bhatnagar, V Dhingra, N Gupta, R Jindal, M Kaur, M Kohli, JM Mehta, MZ Nishu, N Saini, LK Sharma, A Singh, AP Singh, JB Singh, SP Ahuja, S Bhattacharya, S Choudhary, BC Gupta, P Jain, S Jain, S Kumar, A Shivpuri, RK Choudhury, RK Dutta, D Kailas, S Kataria, SK Mohanty, AK Pant, LM Shukla, P Aziz, T Guchait, M Gurtu, A Maity, M Majumder, D Majumder, G Mazumdar, K Mohanty, GB Saha, A Sudhakar, K Wickramage, N Banerjee, S Dugad, S Mondal, NK Arfaei, H Bakhshiansohi, H Etesami, SM Fahim, A Hashemi, M Jafari, A Khakzad, M Mohammadi, A Najafabadi, MM Mehdiabadi, SP Safarzadeh, B Zeinali, M Abbrescia, M Barbone, L Calabria, C Colaleo, A Creanza, D De Filippis, N De Palma, M Dimitrov, A Fiore, L Iaselli, G Lusito, L Maggi, G Maggi, M Manna, N Marangelli, B My, S Nuzzo, S Pacifico, N Pierro, GA Pompili, A Pugliese, G Romano, F Roselli, G Selvaggi, G Silvestris, L Trentadue, R Tupputi, S Zito, G Abbiendi, G Benvenuti, AC Bonacorsi, D Braibant-Giacomelli, S Brigliadori, L Capiluppi, P Castro, A Cavallo, FR Cuffiani, M Dallavalle, GM Fabbri, F Fanfani, A Fasanella, D Giacomelli, P Giunta, M Marcellini, S Meneghelli, M Montanari, A Navarria, FL Odorici, F Perrotta, A Primavera, F Rossi, AM Rovelli, T Siroli, G Travaglini, R Albergo, S Cappello, G Chiorboli, M Costa, S Tricomi, A Tuve, C Barbagli, G Ciulli, V Civinini, C D'Alessandro, R Focardi, E Frosali, S Gallo, E Genta, C Gonzi, S Lenzi, P Meschini, M Paoletti, S Sguazzoni, G Tropiano, A Benussi, L Bianco, S Colafranceschi, S Fabbri, F Piccolo, D Fabbricatore, P Musenich, R Benaglia, A De Guio, F Di Matteo, L Ghezzi, A Malberti, M Malvezzi, S Martelli, A Massironi, A Menasce, D Moroni, L Paganoni, M Pedrini, D Ragazzi, S Redaelli, N Sala, S de Fatis, TT Tancini, V Buontempo, S Montoya, CAC Cimmino, A De Cosa, A De Gruttola, M Fabozzi, F Iorio, AOM Lista, L Merola, M Noli, P Paolucci, P Azzi, P Bacchetta, N Bellan, P Bisello, D Branca, A Carlin, R Checchia, P Conti, E De Mattia, M Dorigo, T Dosselli, U Fanzago, F Gasparini, F Gasparini, U Giubilato, P Gresele, A Lacaprara, S Lazzizzera, I Margoni, M Mazzucato, M Meneguzzo, AT Perrozzi, L Pozzobon, N Ronchese, P Simonetto, F Torassa, E Tosi, M Vanini, S Zotto, P Zumerle, G Baesso, P Berzano, U Riccardi, C Torre, P Vitulo, P Viviani, C Biasini, M Bilei, GM Caponeri, B Fano, L Lariccia, P Lucaroni, A Mantovani, G Menichelli, M Nappi, A Santocchia, A Servoli, L Taroni, S Valdata, M Volpe, R Azzurri, P Bagliesi, G Bernardini, J Boccali, T Broccolo, G Castaldi, R D'Agnolo, RT Dell'Orso, R Fiori, F Foa, L Giassi, A Kraan, A Ligabue, F Lomtadze, T Martini, L Messineo, A Palla, F Palmonari, F Sarkar, S Segneri, G Serban, AT Spagnolo, P Tenchini, R Tonelli, G Venturi, A Verdini, PG Barone, L Cavallari, F Del Re, D Di Marco, E Diemoz, M Franci, D Grassi, M 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Ciesielski, R. Demortier, L. Goulianos, K. Lungu, G. Mesropian, C. Yan, M. Atramentov, O. Barker, A. Duggan, D. Gershtein, Y. Gray, R. Halkiadakis, E. Hidas, D. Hits, D. Lath, A. Panwalkar, S. Patel, R. Richards, A. Rose, K. Schnetzer, S. Somalwar, S. Stone, R. Thomas, S. Cerizza, G. Hollingsworth, M. Spanier, S. Yang, Z. C. York, A. Asaadi, J. Eusebi, R. Gilmore, J. Gurrola, A. Kamon, T. Khotilovich, V. Montalvo, R. Nguyen, C. N. Osipenkov, I. Pivarski, J. Safonov, A. Sengupta, S. Tatarinov, A. Toback, D. Weinberger, M. Akchurin, N. Bardak, C. Damgov, J. Jeong, C. Kovitanggoon, K. Lee, S. W. Mane, P. Roh, Y. Sill, A. Volobouev, I. Wigmans, R. Yazgan, E. Appelt, E. Brownson, E. Engh, D. Florez, C. Gabella, W. Johns, W. Kurt, P. Maguire, C. Melo, A. Sheldon, P. Tuo, S. Velkovska, J. Arenton, M. W. Balazs, M. Boutle, S. Buehler, M. Conetti, S. Cox, B. Francis, B. Hirosky, R. Ledovskoy, A. Lin, C. Neu, C. Yohay, R. Gollapinni, S. Harr, R. Karchin, P. E. Lamichhane, P. Mattson, M. Milstene, C. Sakharov, A. Anderson, M. Bachtis, M. Bellinger, J. N. Carlsmith, D. Dasu, S. Efron, J. Gray, L. Grogg, K. S. Grothe, M. Hall-Wilton, R. Herndon, M. Klabbers, P. Klukas, J. Lanaro, A. Lazaridis, C. Leonard, J. Loveless, R. Mohapatra, A. Reeder, D. Ross, I. Savin, A. Smith, W. H. Swanson, J. Weinberg, M. CA CMS Collaboration TI Search for Pair Production of Second-Generation Scalar Leptoquarks in pp Collisions at root s=7 TeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID CONSTRAINTS; PARTICLES AB A search for pair production of second-generation scalar leptoquarks in the final state with two muons and two jets is performed using proton-proton collision data at root s = 7 TeV collected by the CMS detector at the LHC. The data sample used corresponds to an integrated luminosity of 34 pb(-1). The number of observed events is in good agreement with the predictions from the standard model processes. An upper limit is set on the second-generation leptoquark cross section times beta(2) as a function of the leptoquark mass, and leptoquarks with masses below 394 GeV are excluded at a 95% confidence level for beta = 1, where beta is the leptoquark branching fraction into a muon and a quark. These limits are the most stringent to date. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Ero, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hammer, J.; Nsel, S. Ha; Hartl, C.; Hoch, M.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kasieczka, G.; Kiesenhofer, W.; Krammer, M.; Liko, D.; Mikulec, I.; Pernicka, M.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Taurok, A.; Teischinger, F.; Wagner, P.; Waltenberger, W.; Walzel, G.; Widl, E.; Wulz, C. -E.] OeAW, Inst Hochenergiephys, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. 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J.; Panagiotou, A.; Sphicas, P.] Univ Athens, Athens, Greece. [Evangelou, I.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Patras, V.; Triantis, F. A.] Univ Ioannina, GR-45110 Ioannina, Greece. [Aranyi, A.; Bencze, G.; Boldizsar, L.; Debreczeni, G.; Hajdu, C.; Horvath, D.; Kapusi, A.; Krajczar, K.; Laszlo, A.; Sikler, F.; Vesztergombi, G.; Pasztor, G.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Molnar, J.; Palinkas, J.; Szillasi, Z.; Veszpremi, V.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Jindal, M.; Kaur, M.; Kohli, J. M.; Mehta, M. Z.; Nishu, N.; Saini, L. K.; Sharma, A.; Singh, A. P.; Singh, J. B.; Singh, S. P.] Panjab Univ, Chandigarh 160014, India. [Ahuja, S.; Bhattacharya, S.; Choudhary, B. C.; Gupta, P.; Jain, S.; Kumar, A.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Choudhury, R. 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[Braibant-Giacomelli, S.; Capiluppi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Meneghelli, M.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Tricomi, A.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Genta, C.; Gonzi, S.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Lenzi, P.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Colafranceschi, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. 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[Biasini, M.; Caponeri, B.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Nappi, A.; Santocchia, A.; Taroni, S.; Valdata, M.; Volpe, R.] Univ Perugia, I-06100 Perugia, Italy. [Biasini, M.; Bilei, G. M.; Caponeri, B.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Menichelli, M.; Nappi, A.; Santocchia, A.; Servoli, L.; Taroni, S.; Valdata, M.; Volpe, R.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Palmonari, F.; Sarkar, S.; Segneri, G.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, I-56010 Pisa, Italy. [Bernardini, J.; Fiori, F.; Messineo, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Azzurri, P.; Broccolo, G.; D'Agnolo, R. 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[Amapane, N.; Argiro, S.; Botta, C.; Castello, R.; Costa, M.; Graziano, A.; Marone, M.; Migliore, E.; Mila, G.; Monaco, V.; Musich, M.; Pelliccioni, M.; Romero, A.; Sacchi, R.; Sola, V.; Solano, A.; Trocino, D.; Pereira, A. Vilela] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Della Ricca, G.] Univ Trieste, Trieste, Italy. [Belforte, S.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Montanino, D.; Penzo, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Heo, S. G.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Chung, J.; Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Park, H.; Son, D.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, Zero; Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Hong, B.; Jo, M.; Kim, H.; Kim, J. H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.; Rhee, H. B.; Seo, E.; Shin, S.; Sim, K. S.] Korea Univ, Seoul, South Korea. [Choi, M.; Kang, S.; Kim, H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Martisiute, D.; Petrov, P.; Sabonis, T.] Vilnius State Univ, Vilnius, Lithuania. [Castilla Valdez, H.; Burelo, E. De la Cruz; Lopez-Fernandez, R.; Sanchez Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Allfrey, P.; Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ahmed, I.; Asghar, M. I.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bluj, M.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Soltan Inst Nucl Studies, PL-00681 Warsaw, Poland. [Almeida, N.; David, A.; Faccioli, P.; Parracho, P. G. Ferreira; Gallinaro, M.; Martins, P.; Musella, P.; Nayak, A.; Ribeiro, P. Q.; Seixas, J.; Silva, P.; Varela, J.; Woehri, H. K.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. 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[Zhukov, V.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Sarycheva, L.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Rusakov, S. V.; Vinogradov, A.; Nef, P.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Azhgirey, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Slabospitsky, S.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Maestre, J. 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J.; Piedra Gomez, J.; Rodrigo, T.; Ruiz Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, IFCA, E-39005 Santander, Spain. [Hammer, J.; Darmenov, N.; Genchev, V.; Iaydjiev, P.; Hajdu, C.; Mohanty, A. K.; Lusito, L.; Chiorboli, M.; Tropiano, A.; De Guio, F.; Ghezzi, A.; Perrozzi, L.; Lucaroni, A.; Volpe, R.; Boccali, T.; Tonelli, G.; Venturi, A.; Botta, C.; Graziano, A.; Pelliccioni, M.; Pereira, A. Vilela; Kossov, M.; Grishin, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Baillon, P.; Ball, A. H.; Barney, D.; Bell, A. J.; Benedetti, D.; Bernet, C.; Bialas, W.; Bloch, P.; Bocci, A.; Bolognesi, S.; Breuker, H.; Brona, G.; Bunkowski, K.; Camporesi, T.; Cano, E.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Cure, B.; D'Enterria, D.; De Roeck, A.; Di Guida, S.; Ramos, F. Duarte; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Gaddi, A.; Gennai, S.; Georgiou, G.; Gerwig, H.; Gigi, D.; Gill, K.; Giordano, D.; Glege, F.; Garrido, R. Gomez-Reino; Gouzevitch, M.; Govoni, P.; Gowdy, S.; Guiducci, L.; Hansen, M.; Harvey, J.; Hegeman, J.; Hegner, B.; Henderson, C.; Hesketh, G.; Hoffmann, H. F.; Honma, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Lecoq, P.; Lourenco, C.; Macpherson, A.; Maeki, T.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Nesvold, E.; Nguyen, M.; Orimoto, T.; Orsini, L.; Perez, E.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Polese, G.; Racz, A.; Rodrigues Antunes, J.; Rolandi, G.; Rommerskirchen, T.; Rovelli, C.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Segoni, I.; Sharma, A.; Siegrist, P.; Simon, M.; Sphicas, P.; Spiga, D.; Spiropulu, M.; Stoeckli, F.; Stoye, M.; Tropea, P.; Tsirou, A.; Tsyganov, A.; Veres, G. I.; Vichoudis, P.; Voutilainen, M.; Zeuner, W. D.; Caminada, L.; Marchica, C.; Sharma, V.; Hall-Wilton, R.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Starodumov, A.; Caminada, L.; Marchica, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bortignon, P.; Caminada, L.; Chen, Z.; Cittolin, S.; Dissertori, G.; Dittmar, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Herve, A.; Hintz, W.; Lecomte, P.; Lustermann, W.; Marchica, C.; Martinez Ruiz del Arbol, P.; Meridiani, P.; Milenovic, P.; Moortgat, F.; Nef, P.; Nessi-Tedaldi, F.; Pape, L.; Pauss, F.; Punz, T.; Rizzi, A.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Sawley, M. -C.; Stieger, B.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, M.; Wehrli, L.; Weng, J.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Aguilo, E.; Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Regenfus, C.; Robmann, P.; Schmidt, A.; Snoek, H.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Chen, W. T.; Dutta, S.; Go, A.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, M. H.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Wu, J. H.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R-S.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Demir, Z.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Topaksu, A. Kayis; Nart, A.; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Tali, B.; Topakli, H.; Uzun, D.; Vergili, L. N.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Deliomeroglu, M.; Demir, D.; Guelmez, E.; Halu, A.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Levchuk, L.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Bell, P.; Bostock, F.; Brooke, J. J.; Cheng, T. L.; Clement, E.; Cussans, D.; Frazier, R.; Goldstein, J.; Grimes, M.; Hansen, M.; Hartley, D.; Heath, G. P.; Heath, H. F.; Jackson, J.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Ward, S.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Camanzi, B.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Ballin, J.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Davies, G.; Della Negra, M.; Fulcher, J.; Futyan, D.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Karapostoli, G.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rompotis, N.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Tourneur, S.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardrope, D.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Barrett, M.; Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Reid, I. D.; Teodorescu, L.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.] Baylor Univ, Waco, TX 76798 USA. [Bose, T.; Jarrin, E. Carrera; Fantasia, C.; Heister, A.; John, J. St.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Avetisyan, A.; Bhattacharya, S.; Chou, J. P.; Cutts, D.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Landsberg, G.; Narain, M.; Nguyen, D.; Segala, M.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Borgia, M. A.; Breedon, R.; De la Barca Sanchez, M. Calderon; Cebra, D.; Chauhan, S.; Chertok, M.; Conway, J.; Cox, P. T.; Dolen, J.; Erbacher, R.; Friis, E.; Ko, W.; Kopecky, A.; Lander, R.; Liu, H.; Maruyama, S.; Miceli, T.; Nikolic, M.; Pellett, D.; Robles, J.; Salur, S.; Schwarz, T.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez; Veelken, C.] Univ Calif Davis, Davis, CA 95616 USA. [Felcini, M.; Andreev, V.; Arisaka, K.; Cline, D.; Cousins, R.; Deisher, A.; Duris, J.; Erhan, S.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Tucker, J.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Kao, S. C.; Liu, F.; Liu, H.; Luthra, A.; Nguyen, H.; Pasztor, G.; Satpathy, A.; Shen, B. C.; Stringer, R.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Dusinberre, E.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Mangano, B.; Muelmenstaedt, J.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pi, H.; Pieri, M.; Ranieri, R.; Sani, M.; Sharma, V.; Simon, S.; Tu, Y.; Vartak, A.; Wuerthwein, F.; Yagil, A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; Vlimant, J. R.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Spiropulu, M.; Bornheim, A.; Bunn, J.; Chen, Y.; Gataullin, M.; Kcira, D.; Litvine, V.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Timciuc, V.; Traczyk, P.; Veverka, J.; Wilkinson, R.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Akgun, B.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Jun, S. Y.; Liu, Y. F.; Paulini, M.; Russ, J.; Terentyev, N.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Dinardo, M. E.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Gaz, A.; Heyburn, B.; Luiggi Lopez, E.; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.; Zang, S. L.] Univ Colorado, Boulder, CO 80309 USA. [Agostino, L.; Alexander, J.; Chatterjee, A.; Das, S.; Eggert, N.; Fields, L. J.; Gibbons, L. K.; Heltsley, B.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Kuznetsov, V.; Kaufman, G. Nicolas; Patterson, J. R.; Puigh, D.; Riley, D.; Ryd, A.; Shi, X.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Vaughan, J.; Weng, Y.; Winstrom, L.] Cornell Univ, Ithaca, NY USA. [Wittich, P.; Biselli, A.; Cirino, G.; Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Atac, M.; Bakken, J. A.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Borcherding, F.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Demarteau, M.; Eartly, D. P.; Elvira, V. D.; Esen, S.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Green, D.; Gunthoti, K.; Gutsche, O.; Hahn, A.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; James, E.; Jensen, H.; Johnson, M.; Joshi, U.; Khatiwada, R.; Kilminster, B.; Klima, B.; Kousouris, K.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Limon, P.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Mason, D.; McBride, P.; McCauley, T.; Miao, T.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Popescu, S.; Pordes, R.; Prokofyev, O.; Saoulidou, N.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Tan, P.; Taylor, L.; Tkaczyk, S.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Piedra Gomez, J.; Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Goldberg, S.; Kim, B.; Klimenko, S.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Matchev, K.; Mitselmakher, G.; Muniz, L.; Pakhotin, Y.; Prescott, C.; Remington, R.; Schmitt, M.; Scurlock, B.; Sellers, P.; Skhirtladze, N.; Wang, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Ceron, C.; Gaultney, V.; Kramer, L.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bandurin, D.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Quertenmont, L.; Sekmen, S.; Veeraraghavan, V.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Guragain, S.; Hohlmann, M.; Kalakhety, H.; Ralich, R.; Vodopiyanov, I.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Callner, J.; Cavanaugh, R.; Dragoiu, C.; Garcia-Solis, E. J.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Lacroix, F.; Malek, M.; O'Brien, C.; Silvestre, C.; Smoron, A.; Strom, D.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Cankocak, K.; Clarida, W.; Duru, F.; Lae, C. K.; McCliment, E.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Olson, J.; Onel, Y.; Ozok, F.; Sen, S.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bonato, A.; Eskew, C.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Guo, Z. J.; Hu, G.; Maksimovic, P.; Rappoccio, S.; Swartz, M.; Tran, N. V.; Whitbeck, A.; Bean, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Benelli, G.; Grachov, O.; Murray, M.; Noonan, D.; Radicci, V.; Sanders, S.; Wood, J. S.; Zhukova, V.] Univ Kansas, Lawrence, KS 66045 USA. [Bolton, T.; Chakaberia, I.; Ivanov, A.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.; Wan, Z.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Boutemeur, M.; Eno, S. C.; Ferencek, D.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kirn, M.; Lu, Y.; Mignerey, A. C.; Rossato, K.; Rumerio, P.; Santanastasio, F.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.; Twedt, E.] Univ Maryland, College Pk, MD 20742 USA. [Wyslouch, B.; Pandolfi, F.; Alver, B.; Bauer, G.; Bendavid, J.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Everaerts, P.; Gomez Ceballos, G.; Goncharov, M.; Hahn, K. A.; Harris, P.; Kim, Y.; Klute, M.; Lee, Y. -J.; Li, W.; Loizides, C.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Rudolph, M.; Stephans, G. S. F.; Sumorok, K.; Sung, K.; Wenger, E. A.; Xie, S.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.] MIT, Cambridge, MA 02139 USA. [Cole, P.; Cooper, S. I.; Cushman, P.; Dahmes, B.; De Benedetti, A.; Dudero, P. R.; Franzoni, G.; Haupt, J.; Klapoetke, K.; Kubota, Y.; Mans, J.; Rekovic, V.; Rusack, R.; Sasseville, M.; Singovsky, A.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Godang, R.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, University, MS 38677 USA. [Bloom, K.; Bose, S.; Butt, J.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kelly, T.; Kravchenko, I.; Lazo-Flores, J.; Lundstedt, C.; Malbouisson, H.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Baur, U.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Shipkowski, S. P.; Smith, K.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Boeriu, O.; Chasco, M.; Reucroft, S.; Swain, J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Kubik, A.; Odell, N.; Ofierzynski, R. A.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Antonelli, L.; Berry, D.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Kolberg, T.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Warchol, J.; Wayne, M.; Ziegler, J.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Bylsma, B.; Durkin, L. S.; Gu, J.; Hill, C.; Killewald, P.; Kotov, K.; Ling, T. Y.; Rodenburg, M.; Williams, G.] Ohio State Univ, Columbus, OH 43210 USA. [Adam, N.; Berry, E.; Elmer, P.; Gerbaudo, D.; Halyo, V.; Hebda, P.; Hunt, A.; Jones, J.; Laird, E.; Pegna, D. Lopes; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Acosta, J. G.; Huang, X. T.; Lopez, A.; Mendez, H.; Oliveros, S.; Ramirez Vargas, J. E.; Zatserklyaniy, A.] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Barnes, V. E.; Bolla, G.; Borrello, L.; Bortoletto, D.; Everett, A.; Garfinkel, A. F.; Gecse, Z.; Gutay, L.; Hu, Z.; Jones, M.; Koybasi, O.; Kress, M.; Laasanen, A. T.; Leonardo, N.; Liu, C.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Jindal, P.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Boulahouache, C.; Cuplov, V.; Ecklund, K. M.; Geurts, F. J. M.; Liu, J. H.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Chung, Y. S.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Flacher, H.; Garcia-Bellido, A.; Goldenzweig, P.; Gotra, Y.; Han, J.; Harel, A.; Miner, D. C.; Orbaker, D.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.; Yan, M.] Rockefeller Univ, New York, NY 10021 USA. [Atramentov, O.; Barker, A.; Duggan, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hits, D.; Lath, A.; Panwalkar, S.; Patel, R.; Richards, A.; Rose, K.; Schnetzer, S.; Somalwar, S.; Stone, R.; Thomas, S.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Asaadi, J.; Eusebi, R.; Gilmore, J.; Gurrola, A.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Nguyen, C. N.; Osipenkov, I.; Pivarski, J.; Safonov, A.; Sengupta, S.; Tatarinov, A.; Toback, D.; Weinberger, M.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Bardak, C.; Damgov, J.; Jeong, C.; Kovitanggoon, K.; Lee, S. W.; Mane, P.; Roh, Y.; Sill, A.; Volobouev, I.; Wigmans, R.; Yazgan, E.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Brownson, E.; Engh, D.; Florez, C.; Gabella, W.; Johns, W.; Kurt, P.; Maguire, C.; Melo, A.; Sheldon, P.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN USA. [Arenton, M. W.; Balazs, M.; Boutle, S.; Buehler, M.; Conetti, S.; Cox, B.; Francis, B.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Yohay, R.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Lamichhane, P.; Mattson, M.; Milstene, C.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Anderson, M.; Bachtis, M.; Bellinger, J. N.; Carlsmith, D.; Dasu, S.; Efron, J.; Gray, L.; Grogg, K. S.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Leonard, J.; Loveless, R.; Mohapatra, A.; Reeder, D.; Ross, I.; Savin, A.; Smith, W. H.; Swanson, J.; Weinberg, M.] Univ Wisconsin, Madison, WI 53706 USA. [Gregores, E. M.; Milenovic, P.] Univ Fed ABC, Santo Andre, Brazil. [Assran, Y.] Suez Canal Univ, Suez, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.; Karim, M.] Univ Haute Alsace, Mulhouse, France. [Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Krajczar, K.; Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Colafranceschi, S.] Univ Roma La Sapienza, Fac Ingn, Rome, Italy. [Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Bell, A. J.] Univ Geneva, Geneva, Switzerland. [Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale Sez, Pisa, Italy. Ist Nazl Fis Nucl, Pisa, Italy. [Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Bakirci, M. N.; Cerci, S.] Adiyaman Univ, Adiyaman, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Demir, D.] Izmir Inst Technol, Izmir, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Ozkorucuklu, S.] Suleyman Demirel Univ, TR-32200 Isparta, Turkey. [Sonmez, N.] Ege Univ, Izmir, Turkey. [Basso, L.; Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Popescu, S.] Horia Hulubei Natl Inst Phys & Nucl Engn IFIN HH, Bucharest, Romania. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. 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Hektor, Andi/0000-0001-7873-8118; Cerrada, Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Gonzalez Suarez, Rebeca/0000-0002-6126-7230; Calvo Alamillo, Enrique/0000-0002-1100-2963; Amapane, Nicola/0000-0001-9449-2509; Montanari, Alessandro/0000-0003-2748-6373; Novaes, Sergio/0000-0003-0471-8549; de Jesus Damiao, Dilson/0000-0002-3769-1680; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Codispoti, Giuseppe/0000-0003-0217-7021; Dudko, Lev/0000-0002-4462-3192; Tinoco Mendes, Andre David/0000-0001-5854-7699; Stahl, Achim/0000-0002-8369-7506; Krammer, Manfred/0000-0003-2257-7751; Ruiz, Alberto/0000-0002-3639-0368; Azzi, Patrizia/0000-0002-3129-828X; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Troitsky, Sergey/0000-0001-6917-6600; Servoli, Leonello/0000-0003-1725-9185; Della Ricca, Giuseppe/0000-0003-2831-6982; Hill, Christopher/0000-0003-0059-0779; Ivanov, Andrew/0000-0002-9270-5643; Gulmez, Erhan/0000-0002-6353-518X; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Haj Ahmad, Wael/0000-0003-1491-0446; Katkov, Igor/0000-0003-3064-0466; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Tomei, Thiago/0000-0002-1809-5226; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Arce, Pedro/0000-0003-3009-0484; Flix, Josep/0000-0003-2688-8047; Ozdemir, Kadri/0000-0002-0103-1488; Paganoni, Marco/0000-0003-2461-275X; Belyaev, Alexander/0000-0002-1733-4408; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Ragazzi, Stefano/0000-0001-8219-2074; Muelmenstaedt, Johannes/0000-0003-1105-6678; Rovelli, Tiziano/0000-0002-9746-4842; Paulini, Manfred/0000-0002-6714-5787; Gerbaudo, Davide/0000-0002-4463-0878; Vieira de Castro Ferreira da Silva, Pedro Manuel/0000-0002-5725-041X; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686 FU FMSR (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences (Estonia); NICPB (Estonia); Academy of Finland (Finland); ME (Finland); HIP (Finland); CEA (France); CNRS (France) [IN2P3]; BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Korea); WCU (Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MST (Russia); MAE (Russia); MSTD (Serbia); MICINN (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK (Turkey); TAEK (Turkey); STFC (United Kingdom); DOE (USA); NSF (USA) FX We extend our thanks to Michael Kramer for providing the tools for calculation of the leptoquark theoretical cross section and PDF uncertainty. We wish to congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine. We thank the technical and administrative staff at CERN and other CMS institutes, and acknowledge support from: FMSR (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences and NICPB (Estonia); Academy of Finland, ME, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MST and MAE (Russia); MSTD (Serbia); MICINN and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK and TAEK (Turkey); STFC (United Kingdom); DOE and NSF (USA). NR 25 TC 13 Z9 13 U1 1 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 17 PY 2011 VL 106 IS 20 AR 201803 DI 10.1103/PhysRevLett.106.201803 PG 15 WC Physics, Multidisciplinary SC Physics GA 765SR UT WOS:000290729400005 PM 21668221 ER PT J AU Ezekoye, OK Drews, AR Jen, HW Kudla, RJ McCabe, RW Sharma, M Howe, JY Allard, LF Graham, GW Pan, XQ AF Ezekoye, O. K. Drews, A. R. Jen, H. -W. Kudla, R. J. McCabe, R. W. Sharma, M. Howe, J. Y. Allard, L. F. Graham, G. W. Pan, X. Q. TI Characterization of alumina-supported Pt and Pt-Pd NO oxidation catalysts with advanced electron microscopy SO JOURNAL OF CATALYSIS LA English DT Article DE NO oxidation catalysts; Pt; Pt-Pd alloys; Aberration-corrected TEM ID BIMETALLIC CLUSTERS; SIZE DISTRIBUTIONS; NANOPARTICLES; DEACTIVATION; SPECTROSCOPY; DISPERSION; PLATINUM; SITES; MODEL AB Alumina-supported Pt and Pt-Pd catalysts for NO oxidation were fabricated from two different precursors, acetylacetonate and nitrate. A variety of electron microscopy techniques, notably aberration-corrected scanning transmission electron microscopy, were used to investigate both sets of catalysts in the fresh state (air calcined at 300 degrees C, then reduced in 1% H-2 at 300 or 500 degrees C) and after oxygen-rich hydrothermal aging at 500 degrees C and 900 degrees C. Aberration-corrected microscopy and spectroscopic analysis revealed a significant difference in particle size and composition between the two fresh bimetallic catalysts, with the catalyst made from nitrate precursors containing relatively large (3-10 nm) Pd-rich particles in addition to smaller (1-2 nm) Pt-rich particles that were typical of the acetylacetonate precursors. Regardless of initial state, however, bimetallic particles underwent similar degrees of growth and homogenization (alloying) with aging. In particular, particle growth in the bimetallic catalysis from both precursors was limited relative to that in the pure Pt catalysts, where anomalously large (similar to 500 nm) particles formed at 900 degrees C, and the bimetallic catalysts from both precursors thus showed similar improvements in thermal stability, with little effect on measured NO reaction rates. (C) 2011 Elsevier Inc. All rights reserved. C1 [Ezekoye, O. K.; Graham, G. W.; Pan, X. Q.] Univ Michigan, Dept Mat Sci & Engn, Ann Arbor, MI 48109 USA. [Drews, A. R.; Jen, H. -W.; Kudla, R. J.; McCabe, R. W.; Sharma, M.] Ford Motor Co, Res & Innovat Ctr, Dept Chem Engn, Dearborn, MI 48121 USA. [Howe, J. Y.; Allard, L. F.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Graham, GW (reprint author), Univ Michigan, Dept Mat Sci & Engn, Ann Arbor, MI 48109 USA. EM gwgraham@umich.edu RI Howe, Jane/G-2890-2011 FU National Science Foundation [DMR-0907191, CBET-0933239, DMR-0723032]; US Department of Energy, Office of Energy Efficiency and Renewable Energy FX The work at the University of Michigan was supported by the National Science Foundation under Grants DMR-0907191, CBET-0933239, and DMR-0723032. The research at the Oak Ridge National Laboratory's High Temperature Materials Laboratory was sponsored by the US Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Program. NR 38 TC 19 Z9 20 U1 4 U2 52 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9517 J9 J CATAL JI J. Catal. PD MAY 16 PY 2011 VL 280 IS 1 BP 125 EP 136 DI 10.1016/j.jcat.2011.03.011 PG 12 WC Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA 776GV UT WOS:000291523400014 ER PT J AU Andonian, G Williams, O Wei, X Niknejadi, P Hemsing, E Rosenzweig, JB Muggli, P Babzien, M Fedurin, M Kusche, K Malone, R Yakimenko, V AF Andonian, G. Williams, O. Wei, X. Niknejadi, P. Hemsing, E. Rosenzweig, J. B. Muggli, P. Babzien, M. Fedurin, M. Kusche, K. Malone, R. Yakimenko, V. TI Resonant excitation of coherent Cerenkov radiation in dielectric lined waveguides SO APPLIED PHYSICS LETTERS LA English DT Article ID WAKE-FIELD AB We report the observation of coherent Cerenkov radiation in the terahertz regime emitted by a relativistic electron pulse train passing through a dielectric lined cylindrical waveguide. We describe the beam manipulations and measurements involved in repetitive pulse train creation including comb collimation and nonlinear optics corrections. With this technique, modes beyond the fundamental are selectively excited by use of the appropriate frequency train. The spectral characterization of the structure shows preferential excitation of the fundamental and of a higher longitudinal mode. (C) 2011 American Institute of Physics. [doi:10.1063/1.3592579] C1 [Andonian, G.; Williams, O.; Wei, X.; Niknejadi, P.; Hemsing, E.; Rosenzweig, J. B.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Muggli, P.] Univ So Calif, Los Angeles, CA 90089 USA. [Babzien, M.; Fedurin, M.; Kusche, K.; Malone, R.; Yakimenko, V.] Brookhaven Natl Lab, Accelerator Test Facil, Upton, NY 11973 USA. RP Andonian, G (reprint author), Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. EM gerard@physics.ucla.edu FU U.S. Department of Energy [DE-FG02-04ER41294, DE-AC02-98CH10886, DE-FG03-92ER40695, DE-FG02-92ER40745] FX Work supported by U.S. Department of Energy under Grant Nos. DE-FG02-04ER41294, DE-AC02-98CH10886, DE-FG03-92ER40695, and DE-FG02-92ER40745. NR 9 TC 29 Z9 29 U1 0 U2 9 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 16 PY 2011 VL 98 IS 20 AR 202901 DI 10.1063/1.3592579 PG 3 WC Physics, Applied SC Physics GA 766UN UT WOS:000290812100045 ER PT J AU Bobela, DC Branz, HM Stradins, P AF Bobela, David C. Branz, Howard M. Stradins, Paul TI Anneal treatment to reduce the creation rate of light-induced metastable defects in device-quality hydrogenated amorphous silicon SO APPLIED PHYSICS LETTERS LA English DT Article ID A-SI-H; ABSORPTION; FILMS AB We observe a dramatic reduction in the Staebler-Wronski metastable defect creation efficiency in device-quality films of hydrogenated amorphous silicon after they undergo a 20 min anneal treatment at 350 to 400 degrees C. After several hours of rapid degradation with a high intensity pulsed laser, there are about half as many total dangling bond defects in the annealed samples as in unannealed control samples. This reduction is observed in both 1.02-mu m- and 0.22-mu m-thick films, indicating it is not a surface-related artifact. The improved stability is likely caused by H motion, which restructures the Si-Si network and H-related nanovoids. (C) 2011 American Institute of Physics. [doi:10.1063/1.3592264] C1 [Bobela, David C.; Branz, Howard M.; Stradins, Paul] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Bobela, DC (reprint author), Natl Renewable Energy Lab, 1617 Cole Blvd, Golden, CO 80401 USA. EM David_Bobela@nrel.gov FU U.S. DOE [DE-AC36-08GO28308]; U.S. DOE under the Solar America Initiative [DE-FC36-07GO17053] FX This work is supported by the U.S. DOE under Contract No. DE-AC36-08GO28308 and by subcontract to United Solar Ovonic under the Solar America Initiative Contract No. DE-FC36-07GO17053. We are grateful to our late colleague Yueqin Xu for assistance with the film depositions. We also thank Dr. Chris Deyer for his support with the pulsed laser light soaking, Robert Reedy for secondary ion mass spectrometry profiling on the H content, and Lynn Gedvilas for the FTIR measurements. We acknowledge Dr. Don Williamson for helpful discussions. NR 19 TC 5 Z9 5 U1 1 U2 9 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 16 PY 2011 VL 98 IS 20 AR 201908 DI 10.1063/1.3592264 PG 3 WC Physics, Applied SC Physics GA 766UN UT WOS:000290812100025 ER PT J AU Cho, K Ruebusch, DJ Lee, MH Moon, JH Ford, AC Kapadia, R Takei, K Ergen, O Javey, A AF Cho, Kee Ruebusch, Daniel J. Lee, Min Hyung Moon, Jae Hyun Ford, Alexandra C. Kapadia, Rehan Takei, Kuniharu Ergen, Onur Javey, Ali TI Molecular monolayers for conformal, nanoscale doping of InP nanopillar photovoltaics SO APPLIED PHYSICS LETTERS LA English DT Article ID SURFACE RECOMBINATION VELOCITY; SOLAR-CELLS; SEMICONDUCTORS; STABILITY AB Semiconductor nanopillar arrays with radially doped junctions have been widely proposed as an attractive device architecture for cost effective and high efficiency solar cells. A challenge in the fabrication of three-dimensional nanopillar devices is the need for highly abrupt and conformal junctions along the radial axes. Here, a sulfur monolayer doping scheme is implemented to achieve conformal ultrashallow junctions with sub-10 nm depths and a high electrically active dopant concentration of 10(19)-10(20) cm(-3) in arrays of InP nanopillars. The enabled solar cells exhibit a respectable conversion efficiency of 8.1% and a short circuit current density of 25 mA/cm(3). The work demonstrates the utility of well-established surface chemistry for fabrication of nonplanar junctions for complex devices. (C) 2011 American Institute of Physics. [doi:10.1063/1.3585138] C1 [Javey, Ali] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. Univ Calif Berkeley, Berkeley Sensor & Actuator Ctr, Berkeley, CA 94720 USA. RP Cho, K (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM ajavey@berkeley.edu RI Lee, Min Hyung/H-6777-2012; Kapadia, Rehan/B-4100-2013; Javey, Ali/B-4818-2013 OI Kapadia, Rehan/0000-0002-7611-0551; FU Mohr Davidow Ventures; NSF [0826145]; LBNL; Sloan research fellowship; Sunchon National University; Korea Institute for Advancement of Technology (KIAT) FX This work was supported by Mohr Davidow Ventures and NSF (Grant No. 0826145). The S-MLD process development was supported by a LDRD from LBNL. A.J. acknowledges a Sloan research fellowship and support from the World Class University program at Sunchon National University. J.M. acknowledges financial support from Korea Institute for Advancement of Technology (KIAT). R.K. acknowledges an NSF Graduate Fellowship. NR 17 TC 25 Z9 26 U1 1 U2 15 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 16 PY 2011 VL 98 IS 20 AR 203101 DI 10.1063/1.3585138 PG 3 WC Physics, Applied SC Physics GA 766UN UT WOS:000290812100049 ER PT J AU Gabbay, A Reno, J Wendt, JR Gin, A Wanke, MC Sinclair, MB Shaner, E Brener, I AF Gabbay, Alon Reno, John Wendt, Joel R. Gin, Aaron Wanke, Michael C. Sinclair, Michael B. Shaner, Eric Brener, Igal TI Interaction between metamaterial resonators and intersubband transitions in semiconductor quantum wells SO APPLIED PHYSICS LETTERS LA English DT Article ID MAGNETIC RESPONSE; TERAHERTZ AB We report on the coupling and interaction between the fundamental resonances of planar metamaterials (split ring resonators) and intersubband transitions in GaAs/AlGaAs quantum wells structures in the mid-infrared. An incident field polarized parallel to the sample surface is converted by the metamaterial resonators into a field with a finite component polarized normal to the surface and interacts strongly with the large dipole moment associated with quantum well intersubband transitions. (C) 2011 American Institute of Physics. [doi: 10.1063/1.3592266] C1 [Gabbay, Alon; Reno, John; Gin, Aaron; Shaner, Eric; Brener, Igal] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. RP Gabbay, A (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. EM angabba@sandia.gov RI Brener, Igal/G-1070-2010 OI Brener, Igal/0000-0002-2139-5182 FU Energy Frontier Research Center for Solid State Lighting Science; DARPA/MTO's CEE program under DOE/NNSA [DE-AC52-06NA25396] FX We thank James Ginn and Dale Huber for technical assistance. The simulation portion was funded by the Energy Frontier Research Center for Solid State Lighting Science. Other parts were funded by DARPA/MTO's CEE program under DOE/NNSA (Contract No. DE-AC52-06NA25396). This work was performed, in part, at the Center for Integrated Nanotechnologies, a U. S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a Lockheed-Martin Co., for the U. S. Department of Energy under Contract No. DE-AC04-94AL85000. NR 13 TC 21 Z9 21 U1 1 U2 17 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 16 PY 2011 VL 98 IS 20 AR 203103 DI 10.1063/1.3592266 PG 3 WC Physics, Applied SC Physics GA 766UN UT WOS:000290812100051 ER PT J AU Han, WQ Yu, HG Liu, ZX AF Han, Wei-Qiang Yu, Hua-Gen Liu, Zhenxian TI Convert graphene sheets to boron nitride and boron nitride-carbon sheets via a carbon-substitution reaction SO APPLIED PHYSICS LETTERS LA English DT Article ID BN NANOTUBES; SEMICONDUCTORS; NANOPARTICLES; TEMPLATES; DENSITY; LAYERS AB Here we discuss our synthesis of highly crystalline pure boron nitride (BN) and BN-carbon (BN-C) sheets by using graphene sheets as templates via a carbon-substitution reaction. Typically, these sheets are several micrometers wide and have a few layers. The composition ratios of BN-C sheets can be controlled by the post-treatment (remove carbon by oxidation) temperature. We also observed pure BN and BN-C nanoribbons. We characterized the BN-C sheets via Raman spectroscopy and density functional theory calculations. The results reveal that BN-C sheets with an armchair C-BN chain, and embedded C(2) or C(6) units in BN-dominated regions energetically are the most favorable. (C) 2011 American Institute of Physics. [doi: 10.1063/1.3593492] C1 [Han, Wei-Qiang] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Yu, Hua-Gen] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Liu, Zhenxian] Carnegie Inst Washington, Geophys Lab, Washington, DC 20015 USA. RP Han, WQ (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM whan@bnl.gov RI Han, WQ/E-2818-2013; Yu, Hua-Gen/N-7339-2015 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This research was carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory (BNL), which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. Calculations were performed at NERSC. The use of the U2A beamline for the Raman experiments is supported by COMPRES, the Consortium for Materials Properties Research in Earth Sciences under NSF Cooperative Agreement No. EAR 06-49658. NR 24 TC 27 Z9 27 U1 4 U2 56 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 16 PY 2011 VL 98 IS 20 AR 203112 DI 10.1063/1.3593492 PG 3 WC Physics, Applied SC Physics GA 766UN UT WOS:000290812100060 ER PT J AU Kinion, D Clarke, J AF Kinion, D. Clarke, John TI Superconducting quantum interference device as a near-quantum-limited amplifier for the axion dark-matter experiment SO APPLIED PHYSICS LETTERS LA English DT Article ID JOSEPHSON RING MODULATOR; LOW-NOISE; DC SQUID; AMPLIFICATION AB We characterized a microstrip superconducting quantum interference device amplifier (MSA) as a function of frequency and temperature. At 40 mK, with optimal current and flux biases, the maximum gain of 20.4 dB was at 620 MHz; the bandwidth was 21 MHz. The minimum noise temperature T(N)=48 +/- 5 mK occurred at 612 MHz, slightly below the frequency of maximum gain. This value of T(N) is within a factor of 1.6 of the quantum limit T(Q)=hf/k(B) (f is frequency) for a linear, phase-preserving amplifier. Incorporating the MSA into the axion detector at the University of Washington will increase the scan rate by two to three orders of magnitude. (C) 2011 American Institute of Physics. [doi:10.1063/1.3583380] C1 [Kinion, D.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Kinion, D.; Clarke, John] Univ Calif Berkeley, Lawrence Berkeley Lab, Dept Phys, Div Mat Sci, Berkeley, CA 94720 USA. RP Kinion, D (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM kinion1@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05CH11231] FX A portion of this work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344 (D.K.). This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 20 TC 18 Z9 18 U1 1 U2 9 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 16 PY 2011 VL 98 IS 20 AR 202503 DI 10.1063/1.3583380 PG 3 WC Physics, Applied SC Physics GA 766UN UT WOS:000290812100041 ER PT J AU Kumar, A Ovchinnikov, OS Funakubo, H Jesse, S Kalinin, SV AF Kumar, A. Ovchinnikov, O. S. Funakubo, H. Jesse, S. Kalinin, S. V. TI Real-space mapping of dynamic phenomena during hysteresis loop measurements: Dynamic switching spectroscopy piezoresponse force microscopy SO APPLIED PHYSICS LETTERS LA English DT Article AB Dynamic switching spectroscopy piezoresponse force microscopy is developed to separate thermodynamic and kinetic effects in local bias-induced phase transitions. The approaches for visualization and analysis of five-dimensional data are discussed. The spatial and voltage variability of relaxation behavior of the a-c domain lead zirconate-titanate surface suggest the interpretation in terms of surface charge dynamics. This approach is applicable to local studies of dynamic behavior in any system with reversible bias-induced phase transitions ranging from ferroelectrics and multiferroics to ionic systems such as batteries, fuel cells, and electroresistive materials. (C) 2011 American Institute of Physics. [doi:10.1063/1.3590919] C1 [Kumar, A.; Ovchinnikov, O. S.; Jesse, S.; Kalinin, S. V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Funakubo, H.] Tokyo Inst Technol, Dept Innovat & Engn Mat, Midori Ku, Yokohama, Kanagawa 2268502, Japan. RP Kumar, A (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM ka7@ornl.gov; sjesse@ornl.gov; sergei2@ornl.gov RI Kumar, Amit/C-9662-2012; Kalinin, Sergei/I-9096-2012; Jesse, Stephen/D-3975-2016 OI Kumar, Amit/0000-0002-1194-5531; Kalinin, Sergei/0000-0001-5354-6152; Jesse, Stephen/0000-0002-1168-8483 FU Scientific User Facilities Divison, U.S. Department of Energy FX This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge national Laboratory by the Scientific User Facilities Divison, U.S. Department of Energy. NR 21 TC 15 Z9 15 U1 2 U2 26 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 16 PY 2011 VL 98 IS 20 AR 202903 DI 10.1063/1.3590919 PG 3 WC Physics, Applied SC Physics GA 766UN UT WOS:000290812100047 ER PT J AU Meulenberg, RW Willey, TM Lee, JRI Terminello, LJ van Buuren, T AF Meulenberg, Robert W. Willey, Trevor M. Lee, Jonathan R. I. Terminello, Louis J. van Buuren, Tony TI Erbium doping effects on the conduction band edge in germanium nanocrystals SO APPLIED PHYSICS LETTERS LA English DT Article ID CDSE QUANTUM DOTS; SI NANOCRYSTALS; SILICON; NANOPARTICLES; LUMINESCENCE; ENERGY AB We have produced erbium doped germanium nanocrystals (NCs) using a two cell physical vapor deposition system. Using element specific x-ray techniques, we are able to probe the chemical environment of Er in the Ge NCs. Evidence for the optically active Er(3+) state is seen at low Er concentrations, with a disruption of NC formation at high Er concentrations. The x-ray absorption measurements suggest that the Er occupies lattice sites near the surface of the NC. Analysis of the quantum confinement effect with Er doping suggests that the native quantum properties of the Ge NC are maintained at low Er concentrations. (C) 2011 American Institute of Physics. [doi: 10.1063/1.3592999] C1 [Meulenberg, Robert W.] Univ Maine, Dept Phys & Astron, Orono, ME 04469 USA. [Meulenberg, Robert W.] Univ Maine, Lab Surface Sci & Technol, Orono, ME 04469 USA. [Willey, Trevor M.; Lee, Jonathan R. I.; van Buuren, Tony] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Terminello, Louis J.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Meulenberg, RW (reprint author), Univ Maine, Dept Phys & Astron, Orono, ME 04469 USA. EM robert.meulenberg@maine.edu RI Willey, Trevor/A-8778-2011; OI Willey, Trevor/0000-0002-9667-8830; Meulenberg, Robert/0000-0003-2696-8792 FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences (OBES), Division of Materials Sciences and Engineering FX T.v.B. was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences (OBES), Division of Materials Sciences and Engineering. This work was performed under the auspices of the U.S. DOE by LLNL under Contract Nos. W-7405-Eng-48 and DE-AC52-07NA27344. The ALS is supported by the Director, Office of Science, OBES, of the U.S. DOE under Contract No. DE-AC02-05CH11231. NR 21 TC 1 Z9 1 U1 0 U2 10 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 16 PY 2011 VL 98 IS 20 AR 203107 DI 10.1063/1.3592999 PG 3 WC Physics, Applied SC Physics GA 766UN UT WOS:000290812100055 ER PT J AU Polyakov, A Cabrini, S Dhuey, S Harteneck, B Schuck, PJ Padmore, HA AF Polyakov, A. Cabrini, S. Dhuey, S. Harteneck, B. Schuck, P. J. Padmore, H. A. TI Plasmonic light trapping in nanostructured metal surfaces SO APPLIED PHYSICS LETTERS LA English DT Article ID ENHANCEMENT AB We demonstrate the plasmonic trapping of light in nanometer sized trenches etched into in a planar metal surface. The subwavelength grating structure is shown to efficiently couple to p-polarized light and can be designed to achieve complete absorption at any desired wavelength from the UV to the IR. These structures have a number of useful practical features such as high polarization sensitivity, omnidirectional absorption and extreme field concentration. (C) 2011 American Institute of Physics. [doi: 10.1063/1.3592567] C1 [Polyakov, A.; Cabrini, S.; Dhuey, S.; Harteneck, B.; Schuck, P. J.; Padmore, H. A.] LBNL, Berkeley, CA 94720 USA. RP Polyakov, A (reprint author), Univ Calif Berkeley, AS&T Grad Grp, Berkeley, CA 94720 USA. EM apolyakov@berkeley.edu FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC0205CH11231] FX Portions of this work were performed as a User project at the Molecular Foundry, Lawrence Berkeley National Laboratory, which is supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC0205CH11231. NR 8 TC 31 Z9 32 U1 0 U2 18 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 16 PY 2011 VL 98 IS 20 AR 203104 DI 10.1063/1.3592567 PG 3 WC Physics, Applied SC Physics GA 766UN UT WOS:000290812100052 ER PT J AU Vogel, A Wintz, S Gerhardt, T Bocklage, L Strache, T Im, MY Fischer, P Fassbender, J McCord, J Meier, G AF Vogel, Andreas Wintz, Sebastian Gerhardt, Theo Bocklage, Lars Strache, Thomas Im, Mi-Young Fischer, Peter Fassbender, Juergen McCord, Jeffrey Meier, Guido TI Field- and current-induced domain-wall motion in permalloy nanowires with magnetic soft spots SO APPLIED PHYSICS LETTERS LA English DT Article ID IMPLANTATION AB We study field- and current-induced domain-wall motion in permalloy nanowires containing a square-shaped magnetically softened region. Implantation of chromium ions is used to induce pinning sites via a local reduction in the saturation magnetization. Micromagnetic simulations, magnetic transmission soft x-ray microscopy, and electrical measurements are employed to characterize the pinning potential which significantly differs for transverse and vortex walls. Reliable domain-wall depinning from a so-called magnetic soft spot by single current pulses is observed. This demonstrates the suitability of these pinning sites for applications. (C) 2011 American Institute of Physics. [doi:10.1063/1.3590267] C1 [Vogel, Andreas; Gerhardt, Theo; Bocklage, Lars; Meier, Guido] Univ Hamburg, Inst Angew Phys, D-20355 Hamburg, Germany. [Vogel, Andreas; Gerhardt, Theo; Bocklage, Lars; Meier, Guido] Univ Hamburg, Zentrum Mikrostrukturforsch, D-20355 Hamburg, Germany. [Wintz, Sebastian; Strache, Thomas; Fassbender, Juergen; McCord, Jeffrey] Helmholtz Zentrum Dresden Rossendorf, Inst Ionenstrahlphys & Mat Forsch, D-01314 Dresden, Germany. [Im, Mi-Young; Fischer, Peter] Univ Calif Berkeley, Lawrence Berkeley Lab, Ctr Xray Opt, Berkeley, CA 94720 USA. RP Vogel, A (reprint author), Univ Hamburg, Inst Angew Phys, D-20355 Hamburg, Germany. EM andreas.vogel@physnet.uni-hamburg.de RI McCord, Jeffrey/B-3234-2010; Wintz, Sebastian/E-3456-2012; MSD, Nanomag/F-6438-2012; Fischer, Peter/A-3020-2010; Fassbender, Juergen/A-8664-2008 OI Wintz, Sebastian/0000-0001-6138-8078; Fischer, Peter/0000-0002-9824-9343; Bocklage, Lars/0000-0001-9769-4173; Fassbender, Juergen/0000-0003-3893-9630 FU Deutsche Forschungsgemeinschaft [FA314/3-2, MC9/7-2]; Sonderforschungsbereich [668]; Graduiertenkolleg [1286]; Forschungsund Wissenschaftsstiftung Hamburg via the Exzellenzcluster "Nano-Spintronik"; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05-CH11231] FX We thank Ulrich Merkt for fruitful discussions and continuous support as well as Michael Volkmann and Ingolf Winkler for superb technical assistance. Financial support of the Deutsche Forschungsgemeinschaft via Grant Nos. FA314/3-2 and MC9/7-2, the Sonderforschungsbereich 668 and the Graduiertenkolleg 1286 as well as of the Forschungsund Wissenschaftsstiftung Hamburg via the Exzellenzcluster "Nano-Spintronik" is gratefully acknowledged. Operation of the x-ray microscope is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05-CH11231. NR 22 TC 18 Z9 18 U1 0 U2 22 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 16 PY 2011 VL 98 IS 20 AR 202501 DI 10.1063/1.3590267 PG 3 WC Physics, Applied SC Physics GA 766UN UT WOS:000290812100039 ER PT J AU Jilek, RE Spencer, LP Kuiper, DL Scott, BL Williams, UJ Kikkawa, JM Schelter, EJ Boncella, JM AF Jilek, Robert. E. Spencer, Liam P. Kuiper, David L. Scott, Brian L. Williams, Ursula J. Kikkawa, James M. Schelter, Eric J. Boncella, James M. TI A General and Modular Synthesis of Monoimidouranium(IV) Dihalides SO INORGANIC CHEMISTRY LA English DT Article ID VALENT ORGANOURANIUM COMPLEXES; ACTINIDE COMPLEXES; CRYSTAL-STRUCTURES; FUNCTIONAL-GROUPS; COMMUNICATION; ORGANOIMIDO; LIGAND AB The conproportionation reaction between the dimeric diimidouranium(V) species [U(N(t)Bu)(2)(I)((t)Bu(2)-bpy)](2) ((t)Bu(2)bpy = 4,4'-di-tert-butyl-2,2'-bipyridyl) and UI(3)(THF)(4) in the presence of additional (t)Bu(2)bpy yields U(N(t)Bu)(I)(2)((t)Bu(2)bPy)(THF)(2) (2), an unprecedented example of a monoimidouranium(IV) dihalide complex. The general synthesis of this family of uranium(IV) derivatives can be achieved more readily by adding 2 equiv of MN(H)R (M = Li, K; R = (t)Bu, 2,6-(i)PrC(6)H(3), 2-(t)BuC(6)H(4)) to UX(4) in the presence of coordinating Lewis bases to give complexes with the general formula U(NR)(X)(2)(L)(n) (X = Cl, I; L = (t)Bu(2)bpy, n = 1; L = THF, n = 2). The complexes were characterized by (1)H NMR spectroscopy and single-crystal X-ray diffraction analysis of compounds 2 and {U[N(2,6-(i)PrC(6)H(3))] (Cl)(2)-(THF)(2)}2 (4). (The X-ray structures of 5 and 6 are reported in the Supporting Information.) C1 [Jilek, Robert. E.; Spencer, Liam P.; Kuiper, David L.; Scott, Brian L.; Boncella, James M.] Los Alamos Natl Lab, MPA Div, Los Alamos, NM 87545 USA. [Williams, Ursula J.; Schelter, Eric J.] Univ Penn, P Roy & Diana T Vagelos Labs, Dept Chem, Philadelphia, PA 19104 USA. [Kikkawa, James M.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. RP Boncella, JM (reprint author), Los Alamos Natl Lab, MPA Div, MS J514, Los Alamos, NM 87545 USA. EM boncella@lanl.gov RI Schelter, Eric/E-2962-2013; Scott, Brian/D-8995-2017; OI Scott, Brian/0000-0003-0468-5396; Boncella, James/0000-0001-8393-392X FU University of Pennsylvania; NSF MRSEC [DMR-0520020]; Seaborg Institute (Los Alamos National Laboratory); LANL LDRD FX R.E.J. and L.P.S. thank the Seaborg Institute (Los Alamos National Laboratory) and the LANL LDRD program for partial support of this work E.J.S. acknowledges financial support from the University of Pennsylvania. E.J.S. and J.M.K. are grateful for partial support from the NSF MRSEC program under Award DMR-0520020. NR 21 TC 31 Z9 31 U1 0 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 J9 INORG CHEM JI Inorg. Chem. PD MAY 16 PY 2011 VL 50 IS 10 BP 4235 EP 4237 DI 10.1021/ic200377b PG 3 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 759LQ UT WOS:000290246600005 PM 21476537 ER PT J AU Gaunt, AJ May, I Neu, MP Reilly, SD Scott, BL AF Gaunt, Andrew J. May, Iain Neu, Mary P. Reilly, Sean D. Scott, Brian L. TI Structural and Spectroscopic Characterization of Plutonyl(VI) Nitrate under Acidic Conditions SO INORGANIC CHEMISTRY LA English DT Article ID PLUTONIUM(VI) CARBONATE; COMPLEXES; URANYL; EQUILIBRIA; SPECIATION; CHEMISTRY; COMPOUND; SPECTRA; PU(VI); IONS AB The plutonyl(VI) dinitrate complex [PuO(2)-(NO(3))(2)(H(2)O)(2)]center dot H(2)O (1) has been structurally characterized by single-crystal X-ray diffraction and spectroscopically characterized by solid-state vis-NIR and Raman spectroscopies. Aqueous solution spectroscopic studies indicate only weak plutonyl(VI) nitrate complexation, with the mononitrate complex dominating and negligible dinitrate formation, even in concentrated nitric acid. C1 [Gaunt, Andrew J.; May, Iain; Reilly, Sean D.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Neu, Mary P.] Los Alamos Natl Lab, USDA, Environm Management Off, Los Alamos, NM 87545 USA. [Scott, Brian L.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Reilly, SD (reprint author), Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. EM sreilly@lanl.gov RI Scott, Brian/D-8995-2017; OI Scott, Brian/0000-0003-0468-5396; Gaunt, Andrew/0000-0001-9679-6020 FU U.S. Department of Energy (D.O.E.), Basic Energy Sciences; ARRA [DE-AC52-06NA25396]; Heavy Element Chemistry Program; Chemical Sciences Division of the Office of Basic Energy Sciences; U.S. D.O.E. FX We are thankful for an Early Career Research Program award (U.S. Department of Energy (D.O.E.), Basic Energy Sciences, ARRA funding, Contract DE-AC52-06NA25396) and the Heavy Element Chemistry Program, Chemical Sciences Division of the Office of Basic Energy Sciences, U.S. D.O.E., for funding. NR 37 TC 17 Z9 17 U1 2 U2 43 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 J9 INORG CHEM JI Inorg. Chem. PD MAY 16 PY 2011 VL 50 IS 10 BP 4244 EP 4246 DI 10.1021/ic200525u PG 3 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 759LQ UT WOS:000290246600008 PM 21510662 ER PT J AU Vasudeyan, KV Smith, NA Scott, BL McKigney, EA Blair, MW Gordon, JC Muenchausen, RE AF Vasudeyan, Kalyan V. Smith, Nickolaus A. Scott, Brian L. McKigney, Edward A. Blair, Michael W. Gordon, John C. Muenchausen, Ross E. TI An Ionic Liquid-Mediated Route to Cerium(III) Bromide Solvates SO INORGANIC CHEMISTRY LA English DT Article ID RAY CRYSTAL-STRUCTURES; ORGANOLANTHANIDE CHEMISTRY; SCINTILLATION PROPERTIES; HALIDE-COMPLEXES; LANTHANIDE; CE; ND AB A novel synthetic route to a series of cerium bromide solvates is reported. The combination of bulk cerium bromide and the ionic liquid (IL) 1-butyl-1-methylpyrrolidinium bis(trifluoromethylsulfonyl)imide results in a precursor paste that enhances the solubility of the cerium(III)bromide moiety in a number of donor solvents. Crystallization from these solvents has resulted in the isolation and characterization of CeBr(3)(THF)(4) (2), CeBr(3)(2-Me-THF)(4) (3), and CeBr(3)- (MeCN)(5) center dot MeCN (4). Additionally, 2 is shown to be an efficient precursor for the new species CeBr(3)(py)(4) (5) and CeBr(3)(bipy)(py)(3) (6). C1 [Vasudeyan, Kalyan V.; Gordon, John C.] Los Alamos Natl Lab, Chem Div, Los Alamos, NM 87545 USA. [Smith, Nickolaus A.; Muenchausen, Ross E.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Scott, Brian L.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. [McKigney, Edward A.] Los Alamos Natl Lab, Nucl Nonproliferat Div, Los Alamos, NM 87545 USA. [Blair, Michael W.] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. RP Gordon, JC (reprint author), Los Alamos Natl Lab, Chem Div, MS J582, Los Alamos, NM 87545 USA. EM jgordon@lanl.gov RI Scott, Brian/D-8995-2017 OI Scott, Brian/0000-0003-0468-5396 FU Department of Energy (Office of Basic Energy Sciences); G. T. Seaborg Institute at LANL FX We gratefully acknowledge the Department of Energy (Office of Basic Energy Sciences) and the G. T. Seaborg Institute at LANL (Fellowship to K.V.V.) for their funding and support of this research. NR 22 TC 7 Z9 7 U1 0 U2 9 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 J9 INORG CHEM JI Inorg. Chem. PD MAY 16 PY 2011 VL 50 IS 10 BP 4627 EP 4631 DI 10.1021/ic200353s PG 5 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 759LQ UT WOS:000290246600055 PM 21476538 ER PT J AU Fluegel, B Alberi, K Bhusal, L Mascarenhas, A Snoke, DW Karunasiri, G Pfeiffer, LN West, K AF Fluegel, B. Alberi, K. Bhusal, L. Mascarenhas, A. Snoke, D. W. Karunasiri, G. Pfeiffer, L. N. West, K. TI Exciton pattern generation in GaAs/AlxGa1-xAs multiple quantum wells SO PHYSICAL REVIEW B LA English DT Article AB Exciton photoluminescence pattern generation is investigated in multiple quantum wells. High-contrast outer rings and localized bright spots are generated using efficient field-assisted upconversion of laser light whose photon energy lies below the energy of the luminescing quantum well transition. Time-resolved images of the bright spots reveal unexpected dynamics that are not explained by two-dimensional rate equations for generation and diffusion. This behavior can be understood as a result of three-dimensional transport in the vertically extended samples. C1 [Fluegel, B.; Alberi, K.; Bhusal, L.; Mascarenhas, A.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Snoke, D. W.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Karunasiri, G.] USN, Dept Phys, Postgrad Sch, Monterey, CA 93943 USA. [Pfeiffer, L. N.; West, K.] Bell Labs, Lucent Technol, Murray Hill, NJ 07974 USA. RP Fluegel, B (reprint author), Natl Renewable Energy Lab, 1617 Cole Blvd, Golden, CO 80401 USA. FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC36-08GO28308] FX Research at NREL was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award DE-AC36-08GO28308. NR 13 TC 4 Z9 4 U1 3 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 16 PY 2011 VL 83 IS 19 AR 195320 DI 10.1103/PhysRevB.83.195320 PG 6 WC Physics, Condensed Matter SC Physics GA 765MQ UT WOS:000290711800007 ER PT J AU Huang, L Wang, CZ Ho, KM AF Huang, Li Wang, C. Z. Ho, K. M. TI Structure and dynamics of liquid Ni36Zr64 by ab initio molecular dynamics SO PHYSICAL REVIEW B LA English DT Article ID BOND-ORIENTATIONAL ORDER; AUGMENTED-WAVE METHOD; SUPERCOOLED LIQUIDS; BINARY-ALLOYS; GLASSES; METALS; RESISTIVITY AB First-principles molecular dynamics simulations are performed to investigate the interplay between the local structure and atomic dynamics of liquid Ni36Zr64 eutectic alloy in the equilibrium and undercooled states. The topological and chemical short-range orders (SROs) as characterized by the partial pair-correlation functions show good agreement with recent neutron-scattering experiments. Three-dimensional structural analysis shows that the local environment around both Ni and Zr atoms is more complex than the icosahedral SRO due to the frustration of icosahedra driven by the strong directional interaction and large size difference between Ni and Zr. The atomic dynamics analysis shows that the Ni-centered < 0,2,8,1,0 > and Zr-centered < 0,1,10,4,0 > Voronoi polyhedra with relatively longer lifetime play a key role in slowing down the dynamics. The fraction of these clusters increases significantly as the liquid is cooled down and thus facilitates glass formation in the rapidly quenched alloys. C1 [Huang, Li; Wang, C. Z.; Ho, K. M.] US DOE, Ames Lab, Ames, IA 50011 USA. [Wang, C. Z.; Ho, K. M.] Iowa State Univ, Dept Phys, Ames, IA 50011 USA. RP Huang, L (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. FU U.S. Department of Energy, Basic Energy Sciences [DE-AC02-07CH11358] FX Work at Ames Laboratory was supported by the U.S. Department of Energy, Basic Energy Sciences, including a grant of computer time at the National Energy Research Supercomputing Center (NERSC) in Berkeley, under Contract No. DE-AC02-07CH11358. NR 37 TC 21 Z9 21 U1 5 U2 29 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 16 PY 2011 VL 83 IS 18 AR 184103 DI 10.1103/PhysRevB.83.184103 PG 8 WC Physics, Condensed Matter SC Physics GA 765LY UT WOS:000290709300003 ER PT J AU Lei, HC Abeykoon, M Bozin, ES Petrovic, C AF Lei, Hechang Abeykoon, Milinda Bozin, Emil S. Petrovic, C. TI Spin-glass behavior of semiconducting KxFe2-yS2 SO PHYSICAL REVIEW B LA English DT Article ID SUPERCONDUCTIVITY; HEAT; CUMN AB We report the discovery of KxFe2-yS2 single crystals, isostructural to KxFe2-ySe2 superconductors. The sulfide compound is a small gap semiconductor and shows spin-glass behavior below 32 K. Our results indicate that stoichiometry, defects, and the local environment of FeCh (Ch = S, Se) tetrahedra have important effects on the physical properties of isostructural and isoelectronic K(x)Fe(2-y)Ch(2) compounds. C1 [Lei, Hechang; Abeykoon, Milinda; Bozin, Emil S.; Petrovic, C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Lei, HC (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RI Bozin, Emil/E-4679-2011; Petrovic, Cedomir/A-8789-2009; LEI, Hechang/H-3278-2016 OI Petrovic, Cedomir/0000-0001-6063-1881; FU US Department of Energy (DOE) [DE-AC02-98CH10886]; DOE Office for Basic Energy Science FX We thank S. L. Bud'ko for discussions, John Warren for help with scanning electron microscopy measurements, and John Hanson for help in facilitating the X7B experiment. The work at Brookhaven is supported by the US Department of Energy (DOE) under Contract No. DE-AC02-98CH10886 and in part by the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the DOE Office for Basic Energy Science. NR 28 TC 30 Z9 30 U1 1 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 16 PY 2011 VL 83 IS 18 AR 180503 DI 10.1103/PhysRevB.83.180503 PG 4 WC Physics, Condensed Matter SC Physics GA 765LY UT WOS:000290709300001 ER PT J AU Macutkevic, J Banys, J Bussmann-Holder, A Bishop, AR AF Macutkevic, J. Banys, J. Bussmann-Holder, A. Bishop, A. R. TI Origin of polar nanoregions in relaxor ferroelectrics: Nonlinearity, discrete breather formation, ge transfer SO PHYSICAL REVIEW B LA English DT Article ID SCATTERING; POLARIZATION; PEROVSKITES; MODEL AB A central issue in the physics of relaxor ferroelectrics is the origin of the formation of polar nanoregions below some characteristic temperature scale. While it is often attributed to chemical disorder, random bond-random field appearance, or local symmetry lowering, it is shown here that the huge intrinsic nonlinearity of ferroelectrics gives rise to spatially limited excitations of discrete breather (DB) type, which interact strongly and self-consistently with the remaining lattice. This scenario corresponds to a two-component approach to relaxor physics with distinctive signatures in the dielectric spectra and strong charge-transfer effects. The theoretical results are compared to broadband dielectric spectroscopy on 0.2PSN-0.4PMN-0.4PZN ceramics, which provides clear evidence for the two-component scenario and the emergence of DB-like dynamics with decreasing temperature. C1 [Macutkevic, J.; Banys, J.] Vilnius Univ, Fac Phys, LT-10222 Vilnius, Lithuania. [Bussmann-Holder, A.] Max Planck Inst Solid State Res, D-70569 Stuttgart, Germany. [Bishop, A. R.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Macutkevic, J (reprint author), Vilnius Univ, Fac Phys, Sauletekio 9, LT-10222 Vilnius, Lithuania. OI Macutkevic, Jan/0000-0003-2602-1953 NR 48 TC 21 Z9 23 U1 3 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 16 PY 2011 VL 83 IS 18 AR 184301 DI 10.1103/PhysRevB.83.184301 PG 6 WC Physics, Condensed Matter SC Physics GA 765LY UT WOS:000290709300004 ER PT J AU Wu, SQ Umemoto, K Ji, M Wang, CZ Ho, KM Wentzcovitch, RM AF Wu, Shunqing Umemoto, Koichiro Ji, Min Wang, Cai-Zhuang Ho, Kai-Ming Wentzcovitch, Renata M. TI Identification of post-pyrite phase transitions in SiO2 by a genetic algorithm SO PHYSICAL REVIEW B LA English DT Article ID MOLECULAR-DYNAMICS; CRYSTAL-STRUCTURE; PEROVSKITE PHASE; LOWER MANTLE; MGSIO3; PLANETS; PRINCIPLES; NAMGF3; GAS AB Using a first-principles genetic algorithm we predict an Fe2P phase is the first post-pyrite phase of SiO2 at low temperatures. This contrasts with a recently predicted cotunnite phase. Static enthalpy differences between these two phases are small near the transition pressure (0.69 TPa). While quasiharmonic free energy calculations predict an Fe2P--> cotunnite-type transition with increasing temperature, another phase, NbCoB type, is identified as being structurally and energetically intermediate between Fe2P and cotunnite phases. This structure suggests a possible temperature-induced gradual transformation between Fe2P and cotunnite phases. This finding would change our understanding of how planet-forming silicates, for example, MgSiO3 post-perovskite and its solid solutions, dissociate into elementary oxides at thermodynamic conditions expected in the interior of solar giants and exoplanets. C1 [Wu, Shunqing; Ji, Min; Wang, Cai-Zhuang; Ho, Kai-Ming] US DOE, Ames Lab, Ames, IA 50011 USA. [Wu, Shunqing; Ji, Min; Wang, Cai-Zhuang; Ho, Kai-Ming] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Wu, Shunqing] Xiamen Univ, Dept Phys, Xiamen 361005, Peoples R China. [Umemoto, Koichiro] Univ Minnesota, Dept Geol & Geophys, Minneapolis, MN 55455 USA. [Wentzcovitch, Renata M.] Univ Minnesota, Minnesota Supercomp Inst, Minneapolis, MN 55455 USA. [Wentzcovitch, Renata M.] Univ Minnesota, Dept Chem Engn & Mat Sci, Minneapolis, MN 55455 USA. RP Wu, SQ (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. RI Wu, S.Q./G-3992-2010; Ji, Min/F-3503-2011; Wentzcovitch, Renata/J-8768-2015 OI Wu, S.Q./0000-0002-2545-0054; FU US Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-07CH11358]; NSF [EAR-0757903, EAR-0810272, EAR-1047629, ATM-0426757] FX Work at Ames Laboratory was supported by the US Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering, under Contract No. DE-AC02-07CH11358, including a grant of computer time at the National Energy Research Supercomputing Center (NERSC) in Berkeley, CA. K. U. and R.M.W.'s work were supported by NSF Grants No. EAR-0757903, No. EAR-0810272, No. EAR-1047629, and No. ATM-0426757 (VLab). Computations at the University of Minnesota were performed at the Minnesota Supercomputing Institute and at the Laboratory for Computational Science and Engineering. During the review process, a paper reporting the Fe2P-type phase of SiO2 by Tsuchiya and Tsuchiya was published.37 NR 37 TC 12 Z9 12 U1 1 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 16 PY 2011 VL 83 IS 18 AR 184102 DI 10.1103/PhysRevB.83.184102 PG 4 WC Physics, Condensed Matter SC Physics GA 765LY UT WOS:000290709300002 ER PT J AU Ryan, SD Haines, BM Berlyand, L Ziebert, F Aranson, IS AF Ryan, Shawn D. Haines, Brian M. Berlyand, Leonid Ziebert, Falko Aranson, Igor S. TI Viscosity of bacterial suspensions: Hydrodynamic interactions and self-induced noise SO PHYSICAL REVIEW E LA English DT Article AB The viscosity of a suspension of swimming bacteria is investigated analytically and numerically. We propose a simple model that allows for efficient computation for a large number of bacteria. Our calculations show that long-range hydrodynamic interactions, intrinsic to self-locomoting objects in a viscous fluid, result in a dramatic reduction of the effective viscosity. In agreement with experiments on suspensions of Bacillus subtilis, we show that the viscosity reduction is related to the onset of large-scale collective motion due to interactions between the swimmers. The simulations reveal that the viscosity reduction occurs only for relatively low concentrations of swimmers: Further increases of the concentration yield an increase of the viscosity. We derive an explicit asymptotic formula for the effective viscosity in terms of known physical parameters and show that hydrodynamic interactions are manifested as self-induced noise in the absence of any explicit stochasticity in the system. C1 [Ryan, Shawn D.; Haines, Brian M.; Berlyand, Leonid] Penn State Univ, Dept Math, University Pk, PA 16802 USA. [Ryan, Shawn D.; Haines, Brian M.; Aranson, Igor S.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Ziebert, Falko] ESPCI, CNRS, UMR Gulliver 7083, Lab Physicochim Theor, F-75231 Paris, France. RP Ryan, SD (reprint author), Penn State Univ, Dept Math, University Pk, PA 16802 USA. RI Aranson, Igor/I-4060-2013 FU US DOE BES, Division of Materials Science and Engineering [DE AC02-06CH11357]; DOE [DE-FG02-08ER25862]; NSF [DMS-0708324] FX I. A. was supported by the US DOE BES, Division of Materials Science and Engineering, under contract no. DE AC02-06CH11357. S. D. R., B. M. H., and L. B. were supported by the DOE Grant No. DE-FG02-08ER25862 and NSF Grant No. DMS-0708324. NR 25 TC 31 Z9 31 U1 3 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 J9 PHYS REV E JI Phys. Rev. E PD MAY 16 PY 2011 VL 83 IS 5 AR 050904 DI 10.1103/PhysRevE.83.050904 PN 1 PG 4 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 765PY UT WOS:000290722200002 PM 21728480 ER PT J AU Donev, A Bell, JB de la Fuente, A Garcia, AL AF Donev, Aleksandar Bell, John B. de la Fuente, Anton Garcia, Alejandro L. TI Diffusive Transport by Thermal Velocity Fluctuations SO PHYSICAL REVIEW LETTERS LA English DT Article AB We study the contribution of advection by thermal velocity fluctuations to the effective diffusion coefficient in a mixture of two identical fluids. We find good agreement between a simple fluctuating hydrodynamics theory and particle and finite-volume simulations. The enhancement of the diffusive transport depends on the system size L and grows as ln(L/L-0) in quasi-two-dimensional systems, while in three dimensions it scales as L-0(-1)-L-1, where L-0 is a reference length. Our results demonstrate that fluctuations play an important role in the hydrodynamics of small-scale systems. C1 [Donev, Aleksandar] NYU, Courant Inst Math Sci, New York, NY 10012 USA. [Bell, John B.] Univ Calif Berkeley, Lawrence Berkeley Lab, Ctr Computat Sci & Engn, Berkeley, CA 94720 USA. [de la Fuente, Anton; Garcia, Alejandro L.] San Jose State Univ, Dept Phys & Astron, San Jose, CA 95192 USA. RP Donev, A (reprint author), NYU, Courant Inst Math Sci, 251 Mercer St, New York, NY 10012 USA. EM donev@courant.nyu.edu FU DOE [DE-AC02-05CH11231] FX We thank B. Alder, D. Brogioli, J. Goodman, and E. Vanden-Eijnden for informative discussions. This work was supported by the DOE Applied Mathematics Program (DE-AC02-05CH11231). NR 17 TC 31 Z9 31 U1 0 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 16 PY 2011 VL 106 IS 20 AR 204501 DI 10.1103/PhysRevLett.106.204501 PG 4 WC Physics, Multidisciplinary SC Physics GA 765RZ UT WOS:000290727600004 PM 21668233 ER PT J AU Sumikama, T Yoshinaga, K Watanabe, H Nishimura, S Miyashita, Y Yamaguchi, K Sugimoto, K Chiba, J Li, Z Baba, H Berryman, JS Blasi, N Bracco, A Camera, F Doornenbal, P Go, S Hashimoto, T Hayakawa, S Hinke, C Ideguchi, E Isobe, T Ito, Y Jenkins, DG Kawada, Y Kobayashi, N Kondo, Y Krucken, R Kubono, S Lorusso, G Nakano, T Kurata-Nishimura, M Odahara, A Ong, HJ Ota, S Podolyak, Z Sakurai, H Scheit, H Steiger, K Steppenbeck, D Takano, S Takashima, A Tajiri, K Teranishi, T Wakabayashi, Y Walker, PM Wieland, O Yamaguchi, H AF Sumikama, T. Yoshinaga, K. Watanabe, H. Nishimura, S. Miyashita, Y. Yamaguchi, K. Sugimoto, K. Chiba, J. Li, Z. Baba, H. Berryman, J. S. Blasi, N. Bracco, A. Camera, F. Doornenbal, P. Go, S. Hashimoto, T. Hayakawa, S. Hinke, C. Ideguchi, E. Isobe, T. Ito, Y. Jenkins, D. G. Kawada, Y. Kobayashi, N. Kondo, Y. Kruecken, R. Kubono, S. Lorusso, G. Nakano, T. Kurata-Nishimura, M. Odahara, A. Ong, H. J. Ota, S. Podolyak, Zs. Sakurai, H. Scheit, H. Steiger, K. Steppenbeck, D. Takano, S. Takashima, A. Tajiri, K. Teranishi, T. Wakabayashi, Y. Walker, P. M. Wieland, O. Yamaguchi, H. TI Structural Evolution in the Neutron-Rich Nuclei Zr-106 and Zr-108 SO PHYSICAL REVIEW LETTERS LA English DT Article ID TRANSITION; REGION; DECAY AB The low-lying states in Zr-106 and Zr-108 have been investigated by means of beta-gamma and isomer spectroscopy at the radioactive isotope beam factory (RIBF), respectively. A new isomer with a half-life of 620 +/- 150 ns has been identified in Zr-108. For the sequence of even-even Zr isotopes, the excitation energies of the first 2(+) states reach a minimum at N = 64 and gradually increase as the neutron number increases up to N = 68, suggesting a deformed subshell closure at N = 64. The deformed ground state of Zr-108 indicates that a spherical subshell gap predicted at N = 70 is not large enough to change the ground state of Zr-108 to the spherical shape. The possibility of a tetrahedral shape isomer in Zr-108 is also discussed. C1 [Sumikama, T.; Yoshinaga, K.; Miyashita, Y.; Sugimoto, K.; Chiba, J.; Nakano, T.; Takano, S.] Tokyo Univ Sci, Dept Phys, Chiba 2788510, Japan. [Watanabe, H.; Nishimura, S.; Li, Z.; Baba, H.; Doornenbal, P.; Isobe, T.; Lorusso, G.; Kurata-Nishimura, M.; Sakurai, H.; Scheit, H.; Steppenbeck, D.] RIKEN, Nishina Ctr, Wako, Saitama 3510198, Japan. [Yamaguchi, K.; Ito, Y.; Odahara, A.; Takashima, A.; Tajiri, K.] Osaka Univ, Dept Phys, Osaka 5600043, Japan. [Berryman, J. S.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Berryman, J. S.; Lorusso, G.] Michigan State Univ, NSCL, E Lansing, MI 48824 USA. [Blasi, N.; Bracco, A.; Camera, F.; Wieland, O.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Bracco, A.; Camera, F.] Univ Milan, Dipartimento Fis, I-20133 Milan, Italy. [Go, S.; Hashimoto, T.; Hayakawa, S.; Ideguchi, E.; Kubono, S.; Ota, S.; Yamaguchi, H.] Univ Tokyo, CNS, Wako, Saitama 3510198, Japan. [Hinke, C.; Kruecken, R.; Steiger, K.] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany. [Jenkins, D. G.] Univ York, Dept Phys, York YO10 5DD, N Yorkshire, England. [Kawada, Y.; Kobayashi, N.; Kondo, Y.] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan. [Ong, H. J.] Osaka Univ, RCNP, Osaka 5670047, Japan. [Podolyak, Zs.; Walker, P. M.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. [Teranishi, T.] Kyushu Univ, Dept Phys, Fukuoka 8128581, Japan. [Wakabayashi, Y.] Japan Atom Energy Agcy, Tokai, Ibaraki 3191195, Japan. RP Sumikama, T (reprint author), Tokyo Univ Sci, Dept Phys, 2641 Yamazaki, Chiba 2788510, Japan. EM sumikama@ph.noda.tus.ac.jp RI Wieland, Oliver/G-1784-2011; Teranishi, Takashi/D-2166-2012; SAKURAI, HIROYOSHI/G-5085-2014; Scheit, Heiko/B-4779-2008; Kruecken, Reiner/A-1640-2013 OI Scheit, Heiko/0000-0002-8937-1101; Kruecken, Reiner/0000-0002-2755-8042 FU KAKENHI [50126124, 19340074]; RIKEN; DFG [EXC 153, KR 2326/2]; UK STFC; AWE plc FX The authors acknowledge the accelerator staff and the members of the BigRIPS team for their efforts in delivering the 238U and RI beams. This work was supported by KAKENHI (50126124 and 19340074), RIKEN President Fund 2005, the DFG (EXC 153, KR 2326/2), UK STFC, and AWE plc. NR 26 TC 41 Z9 41 U1 2 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 16 PY 2011 VL 106 IS 20 AR 202501 DI 10.1103/PhysRevLett.106.202501 PG 4 WC Physics, Multidisciplinary SC Physics GA 765RZ UT WOS:000290727600002 PM 21668223 ER PT J AU Loire, M Simonet, V Petit, S Marty, K Bordet, P Lejay, P Ollivier, J Enderle, M Steffens, P Ressouche, E Zorko, A Ballou, R AF Loire, M. Simonet, V. Petit, S. Marty, K. Bordet, P. Lejay, P. Ollivier, J. Enderle, M. Steffens, P. Ressouche, E. Zorko, A. Ballou, R. TI Parity-Broken Chiral Spin Dynamics in Ba3NbFe3Si2O14 SO PHYSICAL REVIEW LETTERS LA English DT Article ID NEUTRON-SCATTERING; POLARIZED NEUTRONS AB The spin-wave excitations emerging from the chiral helically modulated 120 degrees magnetic order in a langasite Ba3NbFe3Si2O14 enantiopure crystal were investigated by unpolarized and polarized inelastic neutron scattering. A dynamical fingerprint of the chiral ground state is obtained, singularized by (i) spectral weight asymmetries answerable to the structural chirality and (ii) a full chirality of the spin correlations observed over the whole energy spectrum. The intrinsic chiral nature of the spin waves' elementary excitations is shown in the absence of macroscopic time-reversal symmetry breaking. C1 [Loire, M.; Simonet, V.; Marty, K.; Bordet, P.; Lejay, P.; Ballou, R.] CNRS, Inst Neel, BP166, F-38042 Grenoble 9, France. [Loire, M.; Simonet, V.; Marty, K.; Bordet, P.; Lejay, P.; Ballou, R.] Univ Grenoble 1, BP166, F-38042 Grenoble 9, France. [Petit, S.] CE Saclay, CEA CNRS, Lab Leon Brillouin, F-91191 Gif Sur Yvette, France. [Marty, K.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Ollivier, J.; Enderle, M.; Steffens, P.] Inst Laue Langevin, BP156, F-38042 Grenoble 9, France. [Ressouche, E.] CEA Grenoble, SPSMS MDN, Inst Nanosci & Cryogenie, F-38054 Grenoble 9, France. [Zorko, A.] Jozef Stefan Inst, Ljubljana 1000, Slovenia. [Zorko, A.] EN FIST Ctr Excellence, SI-1000 Ljubljana, Slovenia. RP Loire, M (reprint author), CNRS, Inst Neel, BP166, F-38042 Grenoble 9, France. EM rafik.ballou@grenoble.cnrs.fr RI Enderle, Mechthild/E-8832-2014 OI Enderle, Mechthild/0000-0001-7304-2162 FU ANR [06-BLAN-01871] FX This work was financially supported by the ANR 06-BLAN-01871. We would like to thank B. Canals and A. Ralko for fruitful discussions, and A. Hadj-Azzem, J. Balay, and J. Debray for the sample preparation. NR 24 TC 24 Z9 24 U1 4 U2 29 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 16 PY 2011 VL 106 IS 20 AR 207201 DI 10.1103/PhysRevLett.106.207201 PG 4 WC Physics, Multidisciplinary SC Physics GA 031LE UT WOS:000310640700001 PM 21668258 ER PT J AU Ling, SL Mei, DH Gutowski, M AF Ling, Sanliang Mei, Donghai Gutowski, Maciej TI Reactivity of hydrogen and methanol on (0 0 1) surfaces of WO3, ReO3, WO3/ReO3 and ReO3/WO3 SO CATALYSIS TODAY LA English DT Article DE Tungsten trioxide; Rhenium trioxide; Heterostructure; Epitaxy; Methanol; Hydrogen; Density functional theory ID AUGMENTED-WAVE METHOD; TUNGSTEN TRIOXIDE; SELECTIVE OXIDATION; WO3(001) SURFACES; TRANSITION; METHYLAL; POINTS; METALS AB Bulk tungsten trioxide (WO3) and rhenium trioxide (ReO3) share very similar structures but display different electronic properties. WO3 is a wide bandgap semiconductor while ReO3 is an electronic conductor. With the advanced molecular beam epitaxy techniques, it is possible to make heterostructures comprised of layers of WO3 and ReO3. These heterostructures might display reactivity different than pure WO3 and ReO3. The interactions of two probe molecules (hydrogen and methanol) with the (0 0 1) surfaces of WO3, ReO3, and two heterostructures ReO3/WO3 and WO3/ReO3 were investigated at the density functional theory level. Atomic hydrogen prefers to adsorb at the mono-coordinated O (O-1C) sites forming a surface hydroxyl on four surfaces. Dissociative adsorption of a hydrogen molecule at the O-1C site leads to formation of a water molecule adsorbed at the penta-coordinated metal (M-5C) site. This is thermodynamically the most stable state. A thermodynamically less stable dissociative state involves two surface hydroxyl groups O1CH and O2CH. The interaction of molecular hydrogen and methanol with pure ReO3 is stronger than with pure WO3 and the strength of the interaction substantially changes on the WO3/ReO3 and ReO3/WO3 heterostructures. The reaction barriers for decomposition and recombination reactions are sensitive to the nature of heterostructure. The calculated adsorption energy of methanol on WO3(001) of -65.6 kJ/mol is consistent with the previous experimental estimation of -67 kJ/mol. (c) 2011 Elsevier B.V. All rights reserved. C1 [Ling, Sanliang; Gutowski, Maciej] Heriot Watt Univ, Chem Sch Engn & Phys Sci, Edinburgh EH14 4AS, Midlothian, Scotland. [Mei, Donghai] Pacific NW Natl Lab, Inst Interfacial Catalysis, Richland, WA 99352 USA. RP Ling, SL (reprint author), Heriot Watt Univ, Chem Sch Engn & Phys Sci, Edinburgh EH14 4AS, Midlothian, Scotland. EM s.ling@hw.ac.uk; donghai.mei@pnl.gov; m.gutowski@hw.ac.uk RI Mei, Donghai/D-3251-2011; Mei, Donghai/A-2115-2012; OI Mei, Donghai/0000-0002-0286-4182; Ling, Sanliang/0000-0003-1574-7476 FU PNNL; Catalysis Initiative at PNNL; National Energy Research Scientific Computing (NERSC) Center at Lawrence Berkeley National Laboratory; William R. Wiley Environmental Molecular Sciences Laboratory (EMSL) [gc34000] FX We thank Prof. Q. Ge (Southern Illinois University) for helpful discussions. We thank Prof. B. Frederick (University of Maine) for providing updated experimental estimation of the adsorption energy of methanol on the oxidized WO3(0 0 1) surface. S.L. and M.G. thank PNNL for providing a fellowship through the Summer Research Institute program. D.M. is supported by a LDRD project from Catalysis Initiative at PNNL. The computing time was granted by the National Energy Research Scientific Computing (NERSC) Center at Lawrence Berkeley National Laboratory and the computational catalyst design project (gc34000) at the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL). EMSL is a DOE national scientific user facility located at PNNL. NR 30 TC 16 Z9 16 U1 3 U2 33 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 J9 CATAL TODAY JI Catal. Today PD MAY 16 PY 2011 VL 165 IS 1 BP 41 EP 48 DI 10.1016/j.cattod.2011.01.017 PG 8 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA 753OT UT WOS:000289789800007 ER PT J AU Mei, DH Lin, G AF Mei, Donghai Lin, Guang TI Effects of heat and mass transfer on the kinetics of CO oxidation over RuO2(1 1 0) catalyst SO CATALYSIS TODAY LA English DT Article DE Multiscale model; Heat and mass transfer; CO oxidation; First-principles kinetic Monte Carlo ID MONTE-CARLO-SIMULATION; METHANE PARTIAL OXIDATION; MECHANISM DEVELOPMENT; MULTISCALE MODEL; PRESSURE GAP; NITRIC-OXIDE; DECOMPOSITION; REACTORS; HYDROGENATION; RUTHENIUM AB Combining first-principles kinetic Monte Carlo (KMC) simulation with a finite difference continuum model, a hybrid computational model was developed to study the effects of heat and mass transfer on the heterogeneous reaction kinetics. The integrated computational framework consists of a surface phase where catalytic surface reactions occur and a gas-phase boundary layer imposed on the catalyst surface where the fluctuating temperature and pressure gradients exist. The surface phase domain is modeled by the site-explicit first-principles KMC simulation. The gas-phase boundary layer domain is described using the second-order grid-based Crank-Nicolson method. To simplify the model, the flow and gas-phase reactions are excluded. The temperature and pressure gradients in the gas-phase boundary layer are the consequence of thermal and molecular diffusions of reactants and products under nominal reaction conditions. Different from previous hybrid multiscale models, the heat and mass fluxes between two domains are directly coupled by the varying boundary conditions at each simulation timestep from the unsteady state reaction regime to the steady state reaction regime in the present model. At the steady-state reaction regime, the activity, the surface coverages of reaction intermediates, along with the temperature and pressure gradient profiles in the gas-phase boundary layer are statistically constant with very small fluctuations. As an illustration example, we studied the effects of heat and mass transfer on the reaction kinetics of CO oxidation over the RuO2(1 1 0) catalysts. We assume the heat from CO oxidation is exclusively dissipated into the gas-phase via thermal diffusion. By varying the thickness of RuO2( 1 1 0) catalysts, the surface temperature changes correspondingly with the heat produced by occurring surface reactions, resulting in the pronounced temperature and pressure gradients in the gas-phase boundary layer. Our simulation results indicate that the limitation of heat and mass transfer in the surrounding environment over the catalyst could dramatically affect the observed macroscopic reaction kinetics under presumed operating reaction conditions. To fully elucidate the complex heterogeneous catalytic system, proper physical description of fluid phase that imposed on the catalyst and its effect on the surface kinetics should be integrated with current surface computational models. (c) 2010 Elsevier B.V. All rights reserved. C1 [Mei, Donghai] Pacific NW Natl Lab, Inst Interfacial Catalysis, Richland, WA 99352 USA. [Lin, Guang] Pacific NW Natl Lab, Computat Sci & Math Div, Richland, WA 99352 USA. RP Mei, DH (reprint author), Pacific NW Natl Lab, Inst Interfacial Catalysis, POB 999, Richland, WA 99352 USA. EM donghai.mei@pnl.gov RI Lin, Guang/D-1376-2011; Mei, Donghai/D-3251-2011; Mei, Donghai/A-2115-2012 OI Mei, Donghai/0000-0002-0286-4182 FU Pacific Northwest National Laboratory (PNNL); US DOE Office of Advanced Scientific Computing Research; National Energy Research Scientific Computing Center at Lawrence Berkeley National Laboratory; William R. Wiley Environmental Molecular Sciences Laboratory (EMSL); U.S. Department of Energy [DE-AC05-76RL01830] FX This work was financially supported by the Laboratory Directed Research and Development (LDRD) project at Pacific Northwest National Laboratory (PNNL) and Applied Mathematics program of the US DOE Office of Advanced Scientific Computing Research. The computing time was granted by the National Energy Research Scientific Computing Center at Lawrence Berkeley National Laboratory and the computational catalyst design project at the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL). EMSL is a DOE national scientific user facility located at PNNL. D. Mei also acknowledged Prof. Karsten Reuter and Sebastian Matera for valuable discussions on the coupling issue, and for providing DFT parameters of CO oxidation on RuO2(1 1 0) used in this work. PNNL is operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830. NR 29 TC 9 Z9 9 U1 0 U2 26 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 J9 CATAL TODAY JI Catal. Today PD MAY 16 PY 2011 VL 165 IS 1 BP 56 EP 63 DI 10.1016/j.cattod.2010.11.041 PG 8 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA 753OT UT WOS:000289789800009 ER PT J AU Choi, YM Liu, P AF Choi, YongMan Liu, Ping TI Understanding of ethanol decomposition on Rh(1 1 1) from density functional theory and kinetic Monte Carlo simulations SO CATALYSIS TODAY LA English DT Article DE Ethanol decomposition; Rhodium; Alloy; Density functional theory; Kinetic Monte Carlo ID STRUCTURE-SENSITIVITY; HYDROGEN-PRODUCTION; FUEL-CELL; C-C; SURFACE; OXIDATION; CATALYSTS; MECHANISM; BOND; ELECTROCATALYSTS AB Reaction mechanisms of ethanol decomposition on Rh(1 1 1) were elucidated by means of periodic density functional theory (DFT) calculations and kinetic Monte Carlo (KMC) simulations. We propose that the most probable reaction pathway is via CH3CH2O* on the basis of our mechanistic study: CH3CH2OH* -> CH3CH2O* -> CH2CH2O* -> CH2CHO* -> CH2CO* -> CHCO* -> CH* + CO* -> C* + CO*. In contrast, the contribution from the pathway via CH3CHOH* is relatively small, CH3CH2OH* -> CH3CHOH* -> CH3CHO* -> CH3CO* -> CH2CO* -> CHCO* -> CH* + CO* -> C* + CO*. According to our calculations, one of the slow steps is the formation of the oxametallacycle CH2CH2O* species, which leads to the production of CHCO*, the precursor for C-C bond breaking. Finally, the decomposition of ethanol leads to the production of C and CO. Our calculations, for ethanol combustion on Rh, the major obstacle is not C-C bond cleavage, but the C contamination on Rh(1 1 1). The strong C-Rh interaction may deactivate the Rh catalyst. The formation of Rh alloys with Pt and Pd weakens the C-Rh interaction, easing the removal of C, and, as expected, in accordance with the experimental findings, facilitating ethanol combustion. (c) 2010 Elsevier B. V. All rights reserved. C1 [Choi, YongMan; Liu, Ping] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Liu, P (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM pingliu3@bnl.gov RI Choi, YongMan/N-3559-2014 OI Choi, YongMan/0000-0003-4276-1599 FU U.S. Department of Energy (Division of Chemical Sciences) [DE-AC02-98CH10886] FX This research was carried out at Brookhaven National Laboratory under Contract DE-AC02-98CH10886 with the U.S. Department of Energy (Division of Chemical Sciences). Y.C. thanks Drs. Laura Barrio-Pliego, Joon Bum Park, Sanjaya Senanayake, Dario Stacchiola, and Fan Yang for fruitful discussions of characterization methods for surface reactions, Drs. Altaf Karim and Victor Milman for kind instructions related to KMC simulations, and Dr. Weiping Zhou for continuous discussions of electro-oxidation of ethanol on electrocatalysts. Also, Y.C. also appreciates Prof. Jeng-Han Wang for fruitful discussions about ethanol decomposition on Rh(1 1 1). We acknowledge valuable experimental information from Prof. Hicham Idriss. DFT calculations were performed at the Center for Functional Nanomaterials at Brookhaven National Laboratory and the National Energy Research Scientific Computing (NERSC) Center. Y.C. is pleased to acknowledge Prof. M.C. Lin for CPU time and helpful discussions on ethanol utilization in high temperature fuel cells. NR 42 TC 36 Z9 37 U1 6 U2 61 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 EI 1873-4308 J9 CATAL TODAY JI Catal. Today PD MAY 16 PY 2011 VL 165 IS 1 BP 64 EP 70 DI 10.1016/j.cattod.2010.12.017 PG 7 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA 753OT UT WOS:000289789800010 ER PT J AU Xu, LJ Xu, Y AF Xu, Lijun Xu, Ye TI Effect of Pd surface structure on the activation of methyl acetate SO CATALYSIS TODAY LA English DT Article DE Ester; Methyl acetate; Palladium; Selectivity; Step/kink; DFT ID DENSITY-FUNCTIONAL THEORY; FINDING SADDLE-POINTS; NITRIC-OXIDE DECOMPOSITION; TRANSITION-METAL CATALYSTS; INITIO MOLECULAR-DYNAMICS; SINGLE-CRYSTAL SURFACES; COPPER-BASED CATALYSTS; MINIMUM ENERGY PATHS; ELASTIC BAND METHOD; ACETIC-ACID AB The activation of methyl acetate (CH(3)COOCH(3)) has been studied using periodic density functional theory calculations to probe the effect of Pd surface structure on this reaction. The adsorption of methyl acetate, dehydrogenated derivatives including enolate (CH(2)COOCH(3)) and methylene acetate (CH(3)COOCH(2)), and dissociation products including acetate, acetyl, ketene, methoxy, formaldehyde, CO, C, O, and H; and the C-H and RCO-OR'C-O bond dissociation in methyl acetate, enolate, and methylene acetate, are calculated on Pd(1 1 1) terrace, step edge, and kink; and on Pd(1 0 0) terrace and step edge. The adsorption of most species is not strongly affected from (1 1 1)- to (1 0 0)- type surfaces, but is clearly enhanced by step/kink compared to the corresponding terrace. For a given reactant, going both from terrace to step edge and from (1 1 1)- to (1 0 0)- type surfaces stabilizes the transition states of C-O bond dissociation steps. Going from terrace to step edge also stabilizes the transition states of C-H bond dissociation steps, but going from (1 1 1)- to (1 0 0)- type surfaces does not clearly do so. Our results suggest that compared to the Pd(1 1 1) terrace, the Pd(1 0 0) terrace is more selective for the C-O bond dissociation that is desirable for alcohol formation, whereas step edges are more selective for C-H bond dissociation. (c) 2010 Elsevier B.V. All rights reserved. C1 [Xu, Lijun; Xu, Ye] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Xu, Y (reprint author), 1 Bethel Valley Rd,POB 2008,MS-6493, Oak Ridge, TN 37831 USA. EM xuy2@ornl.gov RI Xu, Ye/B-5447-2009 OI Xu, Ye/0000-0002-6406-7832 FU Eastman Chemical Company; Division of Scientific User Facilities, U.S. Department of Energy FX This work was financially supported by Eastman Chemical Company and performed at the Center for Nanophase Materials Science, which is sponsored at Oak Ridge National Laboratory (ORNL) by the Division of Scientific User Facilities, U.S. Department of Energy. Computing resources provided by the Texas Advanced Computing Center (TACC), the National Center for Computing Sciences (NCCS), and ORNL were used and are gratefully acknowledged. NR 86 TC 13 Z9 13 U1 2 U2 26 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 J9 CATAL TODAY JI Catal. Today PD MAY 16 PY 2011 VL 165 IS 1 BP 96 EP 105 DI 10.1016/j.cattod.2010.12.021 PG 10 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA 753OT UT WOS:000289789800014 ER PT J AU Ray, AE Bargar, JR Sivaswamy, V Dohnalkova, AC Fujita, Y Peyton, BM Magnuson, TS AF Ray, Allison E. Bargar, John R. Sivaswamy, Vaideeswaran Dohnalkova, Alice C. Fujita, Yoshiko Peyton, Brent M. Magnuson, Timothy S. TI Evidence for multiple modes of uranium immobilization by an anaerobic bacterium SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID ABSORPTION FINE-STRUCTURE; DISSIMILATORY METAL REDUCTION; MICROBIAL U(VI) REDUCTION; IN-SITU BIOSTIMULATION; CONTAMINATED AQUIFER; REDUCING CONDITIONS; HEXAVALENT URANIUM; CRYSTAL-CHEMISTRY; URANYL ADSORPTION; CITROBACTER SP AB Microbial reduction of hexavalent uranium has been studied widely for its potential role in bioremediation and immobilization of soluble U(VI) in contaminated groundwater. More recently, some microorganisms have been examined for their role in immobilization of U(VI) via precipitation of uranyl phosphate minerals mediated by microbial phosphate release, alleviating the requirement for long-term redox control. Here, we investigated the mechanism of U(VI) removal mediated by an environmental isolate, strain UFO1, that is indigenous to the Field Research Center (FRC) in Oak Ridge, TN and has been detected in U(VI)contaminated sediments. Changes in U(VI) speciation were examined in the presence and absence of the electron-shuttling moiety, anthraquinone-2,6-disulfonate (AQDS). Cell suspensions were capable of nearly complete removal of 100 mu MU(VI) from solution within 48 h; U(VI) removal was not dependent on the presence of an exogenous electron donor or AQDS, although AQDS increased the rate of U(VI) removal. X-ray Absorption Near Edge Structure (XANES) and Extended X-ray Absorption Fine Structure (EXAFS) spectroscopic measurements indicated that U(IV) was the predominant oxidation state of uranium in cell suspensions in both the absence and presence of 100 mu M AQDS. Interestingly, 17% of the cell-associated precipitates in a U(VI)-treated suspension that lacked AQDS had spectral characteristics consistent with a uranyl phosphate solid phase. The potential involvement of phosphate was consistent with observed increases in soluble phosphate concentrations over time in UFO1 cell suspensions, which suggested phosphate liberation from the cells. TEM-EDS confirmed the presence of uranyl phosphate with a U:P ratio consistent with autunite (1:1). EXAFS analyses further suggested that U(IV) was bound to low-Z neighbors such as C or P, inferred to be present as functional groups on biomass. These results suggest that strain UFO1 has the ability to facilitate U(VI) removal from solution via reductive and phosphate precipitation mechanisms. Both mechanisms offer potential for the remediation of U-contaminated sediments at the FRC or elsewhere. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Ray, Allison E.; Fujita, Yoshiko] Idaho Natl Lab, Biol Syst Dept, Idaho Falls, ID 83415 USA. [Ray, Allison E.; Magnuson, Timothy S.] Idaho State Univ, Dept Biol Sci, Pocatello, ID 83209 USA. [Bargar, John R.] Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Sivaswamy, Vaideeswaran; Peyton, Brent M.] Washington State Univ, Ctr Multiphase Environm Res, Pullman, WA 99164 USA. [Sivaswamy, Vaideeswaran; Peyton, Brent M.] Washington State Univ, Dept Chem Engn, Pullman, WA 99164 USA. [Dohnalkova, Alice C.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Ray, AE (reprint author), Idaho Natl Lab, Biol Syst Dept, POB 1625, Idaho Falls, ID 83415 USA. EM alikona.ray@gmail.com RI Peyton, Brent/G-5247-2015; Fujita, Yoshiko/S-2007-2016 OI Peyton, Brent/0000-0003-0033-0651; Fujita, Yoshiko/0000-0002-4472-4102 FU Idaho National Laboratory (INL); Inland Northwest Research Alliance (INRA); DOE; Stanford Synchrotron Radiation Lightsource; Department of Energy's Office of Biological and Environmental Research FX This work was supported by the Idaho National Laboratory (INL) and Inland Northwest Research Alliance (INRA); AER was supported by an INRA Subsurface Science Graduate Fellowship, and an INL Graduate Scholarship. Peyton and Sivaswamy were supported by the DOE Environmental Remediation Sciences Program. Support from the Stanford Synchrotron Radiation Lightsource, a national scientific user facility supported by the Department of Energy's Offices of Basic Energy Sciences and Biological and Environmental Research, provided significant contributions to this research. We thank Chris Fuller (US Geological Survey) for providing the spectrum of autunite and David Clark (Los Alamos National Laboratory) for providing the sample of UO2.00. A portion of the research was also performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. We also thank George Redden for reviewing this manuscript and providing helpful comments. We thank Susan Glasauer and three anonymous reviewers for their help in improving the manuscript. NR 74 TC 30 Z9 31 U1 7 U2 48 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD MAY 15 PY 2011 VL 75 IS 10 BP 2684 EP 2695 DI 10.1016/j.gca.2011.02.040 PG 12 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 796XT UT WOS:000293087500007 ER PT J AU Santelli, CM Webb, SM Dohnalkova, AC Hansel, CM AF Santelli, Cara M. Webb, Samuel M. Dohnalkova, Alice C. Hansel, Colleen M. TI Diversity of Mn oxides produced by Mn(II)-oxidizing fungi SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; BIOGENIC MANGANESE OXIDES; MARINE BACILLUS SP.; SP STRAIN KR21-2; LEPTOTHRIX-DISCOPHORA; HEXAGONAL-BIRNESSITE; PSEUDOMONAS-PUTIDA; MN(II) OXIDATION; BACTERIAL BIOFILM; SORPTION AB Manganese (Mn) oxides are environmentally abundant, highly reactive mineral phases that mediate the biogeochemical cycling of nutrients, contaminants, carbon, and numerous other elements. Despite the belief that microorganisms (specifically bacteria and fungi) are responsible for the majority of Mn oxide formation in the environment, the impact of microbial species, physiology, and growth stage on Mn oxide formation is largely unresolved. Here, we couple microscopic and spectroscopic techniques to characterize the Mn oxides produced by four different species of Mn(II)-oxidizing Ascomycete fungi (Plectosphaerella cucumerina strain DS2psM2a2, Pyrenochaeta sp. DS3sAY3a, Stagonospora sp. SRC1lsM3a, and Acremonium strictum strain DS1bioAY4a) isolated from acid mine drainage treatment systems in central Pennsylvania. The site of Mn oxide formation varies greatly among the fungi, including deposition on hyphal surfaces, at the base of reproductive structures (e. g., fruiting bodies), and on envisaged extracellular polymers adjacent to the cell. The primary product of Mn(II) oxidation for all species growing under the same chemical and physical conditions is a nanoparticulate, poorly-crystalline hexagonal birnessite-like phase resembling synthetic delta-MnO(2). The phylogeny and growth conditions (planktonic versus surface-attached) of the fungi, however, impact the conversion of the initial phyllomanganate to more ordered phases, such as todorokite (A. strictum strain DS1bioAY4a) and triclinic birnessite (Stagonospora sp. SRC1lsM3a). Our findings reveal that the species of Mn(II)-oxidizing fungi impacts the size, morphology, and structure of Mn biooxides, which will likely translate to large differences in the reactivity of the Mn oxide phases. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Santelli, Cara M.; Hansel, Colleen M.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Webb, Samuel M.] Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA USA. [Dohnalkova, Alice C.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Hansel, CM (reprint author), Harvard Univ, Sch Engn & Appl Sci, 29 Oxford St, Cambridge, MA 02138 USA. EM hansel@seas.harvard.edu RI Webb, Samuel/D-4778-2009; OI Webb, Samuel/0000-0003-1188-0464; Santelli, Cara/0000-0001-8617-0008 FU Department of Energy, Office of Biological and Environmental Research; National Institutes of Health, National Center for Research Resources; National Science Foundation [ECS-0335765, EAR-0846715]; Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory FX The authors thank Lu Sun for assistance with fungal sample preparations and Christopher Lentini, Deric Learman, and Adiari Vazquez-Rodriguez for XAS and XRD data collection. We also thank two anonymous reviewers for their helpful comments and contributions. Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a national user facility operated by Stanford University on behalf of the US Department of Energy, Office of Basic Energy Sciences. The SSRL Structural Molecular Biology Program is supported by the Department of Energy, Office of Biological and Environmental Research, and by the National Institutes of Health, National Center for Research Resources, Biomedical Technology Program. SEM was performed at the Center for Nanoscale Systems (CNS), a member of the National Nanotechnology Infrastructure Network (NNIN), which is supported by the National Science Foundation under NSF Award No. ECS-0335765. CNS is part of the Faculty of Arts and Sciences at Harvard University. A portion of this research was also performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. This project was funded by the National Science Foundation, Grant Number EAR-0846715, awarded to C.M.H. NR 73 TC 52 Z9 56 U1 9 U2 69 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD MAY 15 PY 2011 VL 75 IS 10 BP 2762 EP 2776 DI 10.1016/j.gca.2011.02.022 PG 15 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 796XT UT WOS:000293087500013 ER PT J AU Wang, ZM Zachara, JM Boily, JF Xia, YX Resch, TC Moore, DA Liu, C AF Wang, Zheming Zachara, John M. Boily, Jean-Francois Xia, Yuanxian Resch, Tom C. Moore, Dean A. Liu, C. TI Determining individual mineral contributions to U(VI) adsorption in a contaminated aquifer sediment: A fluorescence spectroscopy study SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID SURFACE COMPLEXATION MODEL; TRANSMISSION ELECTRON-MICROSCOPY; 2-AND 6-LINE FERRIHYDRITE; HANFORD VADOSE ZONE; SORPTION COMPLEXES; X-RAY; URANIUM(VI) SORPTION; URANYL ADSORPTION; WATER INTERFACE; BINDING-SITES AB The adsorption and speciation of U(VI) was investigated on contaminated, fine grained sediment materials from the Hanford 300 area (SPP1 GWF) in simulated groundwater using cryogenic laser-induced U(VI) fluorescence spectroscopy combined with chemometric analysis. A series of reference minerals (montmorillonite, illite, Michigan chlorite, North Carolina chlorite, California clinochlore, quartz and synthetic 6-line ferrihydrite) was used for comparison that represents the mineralogical constituents of SPP1 GWF. Surface area-normalized K(d) values were measured at U(VI) concentrations of 5 x 10(-7) and 5 x 10(-6) mol L(-1) that displayed the following affinity series: 6-line-ferrihydrite > North Carolina chlorite approximate to California clinochlore > quartz approximate to Michigan chlorite > illite > montmorillonite. Both time-resolved spectra and asynchronous two-dimensional (2D) correlation analysis of SPP1 GWF at different delay times indicated that two major adsorbed U(VI) species were present in the sediment that resembled U(VI) adsorbed on quartz and phyllosilicates. Simulations of the normalized fluorescence spectra confirmed that the speciation of SPP1 GWF was best represented by a linear combination of U(VI) adsorbed on quartz (90%) and phyllosilicates (10%). However, the fluorescence quantum yield for U(VI) adsorbed on phyllosilicates was lower than quartz and, consequently, its fractional contribution to speciation may be underestimated. Spectral comparison with literature data suggested that U(VI) exist primarily as inner-sphere complexes with surface silanol groups on quartz and as surface U(VI) tricarbonate complexes on phyllosilicates. Published by Elsevier Ltd. C1 [Wang, Zheming; Zachara, John M.; Boily, Jean-Francois; Xia, Yuanxian; Resch, Tom C.; Moore, Dean A.; Liu, C.] Pacific NW Natl Lab, Richland, WA 99354 USA. RP Wang, ZM (reprint author), Pacific NW Natl Lab, POB 999,MS K8-96, Richland, WA 99354 USA. EM Zheming.Wang@pnl.gov; jean-francois.boily@chem.umu.se RI Wang, Zheming/E-8244-2010; Liu, Chongxuan/C-5580-2009 OI Wang, Zheming/0000-0002-1986-4357; FU Subsurface Biogeochemistry Research Program (SBR); US Department of Energy by Battelle [DE-AC06-76RLO 1830] FX The authors thank Drs. Ponnusamy Nachimuthu and Mark Bowden at the W. R. Wiley Environmental Molecular Sciences Laboratory (EMSL), Mr. Todd Schaef, Dr. Igor Kutnyakov and Ms. Colleen Russell for XRD analysis of the solids, and Mr. Bruce Arey (EMSL) for SEM and EDAX analysis. We also thank Dr. Eugene Ilton for helpful discussions and reviewing the manuscript. This project was supported by the Subsurface Biogeochemistry Research Program (SBR) managed by the U.S. DOE Office of Biological and Environmental Research (OBER) through the Pacific Northwest National Laboratory (PNNL) Scientific Focus Area (SFA). Part of this research was performed at EMSL, a national scientific user facility at PNNL managed by the Department of Energy's Office of Biological and Environmental Research. Pacific Northwest National Laboratory is operated for the US Department of Energy by Battelle under Contract DE-AC06-76RLO 1830. NR 93 TC 19 Z9 19 U1 5 U2 39 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD MAY 15 PY 2011 VL 75 IS 10 BP 2965 EP 2979 DI 10.1016/j.gca.2011.03.008 PG 15 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 796XT UT WOS:000293087500024 ER PT J AU Orme, CJ Stewart, FF AF Orme, Christopher J. Stewart, Frederick F. TI Separation of dimethyl ether from syn-gas components by poly(dimethylsiloxane) and poly(4-methyl-1-pentene) membranes SO CHEMICAL ENGINEERING JOURNAL LA English DT Article DE PDMS; TPX; Dimethyl ether; CO; CO(2); Mixed gas ID METHANOL DEHYDRATION; FUEL-CELL; CATALYSTS; PERMEABILITY; REACTOR; PERMEATION; SORPTION; SPINEL AB Dimethyl ether (DME) has been discussed as a potential fuel for both combustion and fuel cell applications. This paper evaluates the ability for membranes to separate DME from syn-gas components, such as H(2) and CO. Separations from CO(2) and CH(4) also are discussed. Experiments performed include permeability and selectivity of these gases through poly(4-methyl-1-pentene) (TPX) and poly(dimethylsiloxane) (PDMS) using variable temperature mixed gas experiments. The DME data is the first to be reported through these membranes. In this paper, the chosen polymers reflect both rubbery and semicrystalline materials. Rubbery polymers tend to be weakly size sieving, which, in this work, has resulted in larger permeabilities, lower separation factors, and lower activation energies of permeation (En). Conversely, the semicrystalline TPX membranes showed much greater sensitivity to penetrant size; although the gas condensability also played a role in transport. (C) 2011 Elsevier B.V. All rights reserved. C1 [Orme, Christopher J.; Stewart, Frederick F.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Stewart, FF (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM Frederick.Stewart@inl.gov FU Battelle Energy Alliance, LLC [DE-AC07-05ID14517]; U.S. Department of Energy [DE-AC07-05ID14517] FX This manuscript has been authored by Battelle Energy Alliance, LLC under contract no. DE-AC07-05ID14517 with the U.S. Department of Energy. The United States government retains and the publisher, by accepting the article for publication, acknowledges that the United States government retains a nonexclusive, paid-up, irrevocable, world wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States government purposes. NR 29 TC 2 Z9 2 U1 2 U2 17 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 1385-8947 J9 CHEM ENG J JI Chem. Eng. J. PD MAY 15 PY 2011 VL 170 IS 1 BP 178 EP 183 DI 10.1016/j.cej.2011.03.051 PG 6 WC Engineering, Environmental; Engineering, Chemical SC Engineering GA 775JC UT WOS:000291454600023 ER PT J AU Du, D Chen, AQ Xie, YY Zhang, AD Lin, YH AF Du, Dan Chen, Aiqiong Xie, Yunying Zhang, Aidong Lin, Yuehe TI Nanoparticle-based immunosensor with apoferritin templated metallic phosphate label for quantification of phosphorylated acetylcholinesterase SO BIOSENSORS & BIOELECTRONICS LA English DT Article DE Acetylcholinesterase; Organophosphate pesticides; Biomarker; Immunosensor; Apoferritin; Amplification ID MASS-SPECTROMETRIC ANALYSIS; ORGANOPHOSPHATE PESTICIDES; ELECTROCHEMICAL BIOSENSOR; CHOLINESTERASE ACTIVITY; ZIRCONIA NANOPARTICLES; NERVE AGENTS; EXPOSURE; BIOMARKER; AMPLIFICATION; STRATEGY AB A new sandwich-like electrochemical immunosensor has been developed for quantification of organophosphorylated acetylcholinesterase (OP-AChE), an exposure biomarker of organophosphate pesticides and nerve agents. Zirconia nanoparticles (ZrO2 NPs) were anchored on a screen printed electrode (SPE) to preferably capture OP-AChE adducts by metal chelation with phospho-moieties, which was selectively recognized by lead phosphate-apoferritin labeled anti-AChE antibody (LPA-anti-AChE). The sandwich-like immunoreactions were performed among ZrO2 NPs, OP-AChE and LPA-anti-AChE to form ZrO2/OP-AChE/LPA-anti-AChE complex and the released lead ions were detected on a disposable SPE. The binding affinity was investigated by both square wave voltammetry (SWV) and quartz crystal microbalance (QCM) measurements. The proposed immunosensor yielded a linear response current over a broad OP-AChE concentrations range from 0.05 nM to 10 nM, with detection limit of 0.02 nM, which has enough sensitivity for monitoring of low-dose exposure to OPs. This method avoids the drawback of unavailability of commercial OP-specific antibody as well as amplifies detection signal by using apoferritin encoded metallic phosphate nanoparticle tags. This nanoparticle-based immunosensor offers a new method for rapid, sensitive, selective and inexpensive quantification of phosphorylated adducts for monitoring of OP pesticides and nerve agents exposures. (C) 2011 Elsevier B.V. All rights reserved. C1 [Du, Dan; Chen, Aiqiong; Xie, Yunying; Zhang, Aidong] Cent China Normal Univ, Key Lab Pesticide & Chem Biol, Minist Educ, Coll Chem, Wuhan 430079, Peoples R China. [Lin, Yuehe] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Du, D (reprint author), Cent China Normal Univ, Key Lab Pesticide & Chem Biol, Minist Educ, Coll Chem, Wuhan 430079, Peoples R China. EM dudan@mail.ccnu.edu.cn RI Lin, Yuehe/D-9762-2011; Du, Dan (Annie)/G-3821-2012 OI Lin, Yuehe/0000-0003-3791-7587; FU National Natural Science Foundation of China [21075047, 20972056]; Program for Chenguang Young Scientist for Wuhan [200950431184]; Special Fund for Basic Scientific Research of Central Colleges [CCNU10A02005]; NIH [U01 NS058161-01]; DOE [DE-AC05-76L01830] FX This work was supported by the National Natural Science Foundation of China (21075047, 20972056) and Program for Chenguang Young Scientist for Wuhan (200950431184) and the Special Fund for Basic Scientific Research of Central Colleges (CCNU10A02005). Y. Lin acknowledges the financial support by Grant U01 NS058161-01 from the NIH's CounterACT Program through the National Institute of Neurological Disorders and Stroke, NIH. The contents of this publication are solely the responsibility of the authors and do not necessarily represent the official views of the federal government. Pacific Northwest National Laboratory is operated for DOE by Battelle under Contract DE-AC05-76L01830. NR 32 TC 26 Z9 27 U1 6 U2 52 PU ELSEVIER ADVANCED TECHNOLOGY PI OXFORD PA OXFORD FULFILLMENT CENTRE THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0956-5663 J9 BIOSENS BIOELECTRON JI Biosens. Bioelectron. PD MAY 15 PY 2011 VL 26 IS 9 BP 3857 EP 3863 DI 10.1016/j.bios.2011.02.047 PG 7 WC Biophysics; Biotechnology & Applied Microbiology; Chemistry, Analytical; Electrochemistry; Nanoscience & Nanotechnology SC Biophysics; Biotechnology & Applied Microbiology; Chemistry; Electrochemistry; Science & Technology - Other Topics GA 771RK UT WOS:000291178200021 PM 21481580 ER PT J AU Wang, W Kravchenko, AN Smucker, AJM Rivers, ML AF Wang, W. Kravchenko, A. N. Smucker, A. J. M. Rivers, M. L. TI Comparison of image segmentation methods in simulated 2D and 3D microtomographic images of soil aggregates SO GEODERMA LA English DT Article DE Simulated image; Indicator kriging method; Region non-uniformity measure; Misclassification error ID THRESHOLDING TECHNIQUES; QUANTITATIVE-ANALYSIS; SELECTION METHOD; PORE-SPACE; QUANTIFICATION; CT AB Advances in X-ray microtomography (mu CT) are opening new opportunities for examining soil pore structures. However, usefulness of mu CT data for pore structure characterization depends on how accurately the grayscale images are segmented into pore and solid components. Multiple segmentation algorithms have been developed; however, one of the difficulties in comparing the accuracy of segmentation algorithms is the lack of ground-truth information in the soil samples subjected to mu CT. This means that only the criteria that do not depend on the availability of the ground-truth data can be used in assessing accuracy of the segmentation methods, yet the reliability of such criteria in soil images is unclear. In this study, we simulated 2D and 3D soil images to resolve the problem of the lack of ground-truth information. The objectives of the study were (i) to explore optimal parameter selection for indicator kriging (IK) segmentation; (ii) to compare the accuracy of several commonly used segmentation methods, namely, entropy based method, iterative method, Otsu's method, and IK method; and (iii) to evaluate performance of the region non-uniformity measure (NU), the criterion that does not depend on presence of the ground-truth image, in segmentation method selection for soil images. We found that though there was no single segmentation method that preserved pore characteristics in all the cases, IK method yielded segmented images most similar to the ground-truth in most of the cases when the histogram of image grayscale values had clearly distinguishable peaks. For the image with poorly distinguishable histogram peaks. IK did not perform well, while Otsu's method produced acceptable segmentation results. The results indicated that selecting the segmentation method based on NU did not always produce optimal representation of pore characteristics. However, overall, the NU was found to be an acceptable criterion for segmentation method selection in mu CT soil images. Published by Elsevier B.V. C1 [Wang, W.; Kravchenko, A. N.; Smucker, A. J. M.] Michigan State Univ, Dept Crop & Soil Sci, E Lansing, MI 48824 USA. [Rivers, M. L.] Univ Chicago, Argonne Natl Lab, APS CARS CAT, Argonne, IL 60439 USA. RP Kravchenko, AN (reprint author), Michigan State Univ, Dept Crop & Soil Sci, E Lansing, MI 48824 USA. EM kravche1@msu.edu RI Wang, Wei/F-6555-2011 FU NSF; Michigan Agricultural Experiment Station; USDA-CSREES National Research Initiative [2008, 35102-04567] FX This research was funded in part by the NSF LTER Program at KBS, Michigan Agricultural Experiment Station, and USDA-CSREES National Research Initiative: Water and Watersheds Program (Project 2008, 35102-04567). The authors are grateful for two anonymous reviewers and Editor Dr. Edith Perrier's comments in clarifying several aspects of the manuscript. NR 48 TC 38 Z9 38 U1 2 U2 48 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0016-7061 J9 GEODERMA JI Geoderma PD MAY 15 PY 2011 VL 162 IS 3-4 BP 231 EP 241 DI 10.1016/j.geoderma.2011.01.006 PG 11 WC Soil Science SC Agriculture GA 771EL UT WOS:000291139900002 ER PT J AU Watrous, MG Delmore, JE AF Watrous, Matthew G. Delmore, James E. TI Measurement of trace uranium isotopes using a porous ion emitter SO INTERNATIONAL JOURNAL OF MASS SPECTROMETRY LA English DT Article DE Thermal ionization mass spectrometry (TIMS); Porous ion emitter (PIE); Uranium ID IONIZATION MASS-SPECTROMETRY; RESIN BEAD; SOIL SAMPLES; PLUTONIUM; RATIO; EFFICIENCY AB The extent to which thermal ionization mass spectrometry (TIMS) can measure trace quantities of (233)U and (236)U in the presence of a huge excess of natural uranium is evaluated. This is an important nuclear nonproliferation measurement. Four ion production methods were evaluated with three mass spectrometer combinations. The most favorable combinations are not limited by abundance sensitivity: rather, the limitations are the ability to generate a uranium ion beam of sufficient intensity to obtain the required number of counts on the minor isotopes in relationship to detector background. The most favorable situations can measure isotope ratios in the range of 1 x 10(-10) if sufficient sample intensity is available. These are the triple sector mass spectrometer with porous ion emitters (PIE) and the single sector mass spectrometer with energy filtering. (C) 2010 Elsevier B.V. All rights reserved. C1 [Watrous, Matthew G.; Delmore, James E.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Watrous, MG (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM matthew.watrous@inl.gov FU U.S. Department of Energy, under DOE Idaho Operations Office [DE-AC07-05ID14517]; U.S.Government FX This work is supported by the U.S. Department of Energy, under DOE Idaho Operations Office Contract DE-AC07-05ID14517.; This information was prepared as an account of work sponsored by an agency of the U.S.Government. Neither the U.S. Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. References herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise, does not necessarily constitute or imply its endorsement, recommendation, or favoring by the U.S. Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the U.S.Government or any agency thereof. NR 25 TC 2 Z9 2 U1 1 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-3806 J9 INT J MASS SPECTROM JI Int. J. Mass Spectrom. PD MAY 15 PY 2011 VL 303 IS 1 BP 1 EP 5 DI 10.1016/j.ijms.2010.11.016 PG 5 WC Physics, Atomic, Molecular & Chemical; Spectroscopy SC Physics; Spectroscopy GA 771DS UT WOS:000291138000001 ER PT J AU Kim, YS Kim, DS Guiver, MD Pivovar, BS AF Kim, Yu Seung Kim, Dae Sik Guiver, Michael D. Pivovar, Bryan S. TI Interpretation of direct methanol fuel cell electrolyte properties using non-traditional length-scale parameters SO JOURNAL OF MEMBRANE SCIENCE LA English DT Article DE Direct methanol fuel cell; Conductivity; Methanol permeability; Selectivity; Nafion (R); Polymer electrolyte membrane ID PROTON-EXCHANGE MEMBRANES; POLY(ARYLENE ETHER SULFONE); POLYMER ELECTROLYTE; BLEND MEMBRANES; BENZIMIDAZOLE GROUPS; TRANSPORT-PROPERTIES; POLYIMIDE MEMBRANES; COMPOSITE MEMBRANE; CROSS-LINKING; COPOLYMERS AB Numerous sulfonated polymer electrolyte membranes (PEMs) have been developed for direct methanol fuel cells (DMFCs) during the last decade. An analysis for DMFC PEMs obtained from the literature data and structural information is presented based on non-traditional length scale parameters. The analysis presented highlights specific differences in chemical composition between PEMs including perfluorinated sulfonic acids, hydrocarbon-based and polymers having specific interactions. Differences in cross-linked, homopolymer-like, random and multi-block polymer architectures are also discussed. The analysis presented gives important insight into molecular design aspects of sulfonated PEMs for DMFCs. (C) 2011 Elsevier B.V. All rights reserved. C1 [Kim, Yu Seung; Kim, Dae Sik] Los Alamos Natl Lab, Sensors & Electrochem Devices Grp, Los Alamos, NM 87545 USA. [Guiver, Michael D.] CNR, Inst Chem Proc & Environm Technol, Ottawa, ON K1A 0R6, Canada. [Guiver, Michael D.] Hanyang Univ, WCU Dept Energy Engn, Seoul 133791, South Korea. [Pivovar, Bryan S.] Natl Renewable Energy Lab, Hydrogen Technol & Syst Ctr, Golden, CO 80401 USA. RP Kim, YS (reprint author), Los Alamos Natl Lab, Sensors & Electrochem Devices Grp, POB 1663, Los Alamos, NM 87545 USA. EM yskim@lanl.gov RI Guiver, Michael/I-3248-2016 OI Guiver, Michael/0000-0003-2619-6809 FU US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; US DOE; Ministry of Education, Science and Technology [R31-2008-000-10092] FX Authors thank Professor Jim McGrath (Virginia Tech) for useful discussion. This work was supported by the US Department of Energy at Los Alamos National Laboratory operated by Los Alamos National Security LLC under Contract DE-AC52-06NA25396. The authors thank US DOE Fuel Cell Technologies Program, Technology Development Manager Dr. Nancy Garland, for financial support. M.D. Guiver acknowledges partial support from the WCU (World Class University) program through the National Research Foundation of Korea funded by the Ministry of Education, Science and Technology (No. R31-2008-000-10092). NR 62 TC 4 Z9 4 U1 3 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0376-7388 J9 J MEMBRANE SCI JI J. Membr. Sci. PD MAY 15 PY 2011 VL 374 IS 1-2 BP 49 EP 58 DI 10.1016/j.memsci.2011.03.004 PG 10 WC Engineering, Chemical; Polymer Science SC Engineering; Polymer Science GA 771BD UT WOS:000291131300006 ER PT J AU Quiter, BJ Ludewigt, BA Mozin, VV Wilson, C Korbly, S AF Quiter, B. J. Ludewigt, B. A. Mozin, V. V. Wilson, C. Korbly, S. TI Transmission nuclear resonance fluorescence measurements of U-238 in thick targets SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article DE Nuclear resonance fluorescence; Transmission; U-238; Non-destructive assay; Notch refill AB Transmission nuclear resonance fluorescence measurements were made on targets consisting of Pb and depleted U with total areal densities near 86 g/cm(2). The U-238 content in the targets varied from 0% to 8.5% (atom fraction). The experiment demonstrates the capability of using transmission measurements as a non-destructive technique to identify and quantify the presence of an isotope in samples with thicknesses comparable to the average thickness of a nuclear fuel assembly. The experimental data also appear to demonstrate the process of notch refilling with a predictable intensity. Comparison of measured spectra to previous backscatter U-238 measurements indicates general agreement in observed excited states. Evidence of two new U-238 excited states and possibly a third state have also been observed. Published by Elsevier B.V. C1 [Quiter, B. J.; Ludewigt, B. A.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Quiter, B. J.; Mozin, V. V.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Mozin, V. V.] Los Alamos Natl Lab, Los Alamos, NM USA. [Wilson, C.; Korbly, S.] Passport Syst Inc, Billerica, MA USA. RP Quiter, BJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, 1 Cyclotron Rd,MS 5R0121, Berkeley, CA 94720 USA. EM bjquiter@lbl.gov FU Office of Nuclear Energy; Office of Proliferation Detection, National Nuclear Security Administration, US Department of Energy [DE-AC02-05CH11231] FX The authors would like to thank Chatham Cooke for his operation of the Van de Graaff accelerator at the High Voltage Research Laboratory (HVRL) at MIT. This work was supported by the MPACT campaign of the FCR&D program of the Office of Nuclear Energy and by the Office of Proliferation Detection, National Nuclear Security Administration, US Department of Energy under Contract No. DE-AC02-05CH11231. NR 21 TC 17 Z9 17 U1 0 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD MAY 15 PY 2011 VL 269 IS 10 BP 1130 EP 1139 DI 10.1016/j.nimb.2011.02.081 PG 10 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 771SP UT WOS:000291181300017 ER PT J AU Deng, LP Wv, XQ AF Deng, Liping Wv, Xiaoqing TI Physical Mechanisms for the Maintenance of GCM-Simulated Madden-Julian Oscillation over the Indian Ocean and Pacific SO JOURNAL OF CLIMATE LA English DT Article ID CONVECTIVE MOMENTUM TRANSPORT; TOGA COARE IOP; COMMUNITY CLIMATE MODEL; CLOUD-RESOLVING MODEL; VERTICAL TRANSPORT; NATIONAL CENTER; CUMULUS CLOUDS; PART I; PARAMETERIZATION; SCHEME AB The kinetic energy budget is conducted to analyze the physical processes responsible for the improved Madden-Julian oscillation (MJO) simulated by the Iowa State University general circulation models (ISUGCMs). The modified deep convection scheme that includes the revised convection closure, convection trigger condition, and convective momentum transport (CMT) enhances the equatorial (10 degrees S-10 degrees N) MJO-related perturbation kinetic energy (PKE) in the upper troposphere and leads to a more robust and coherent eastward-propagating MJO signal. In the MJO source region, the Indian Ocean (45 degrees-120 degrees E), the upper-tropospheric MJO PKE is maintained by the vertical convergence of wave energy flux and the barotropic conversion through the horizontal shear of mean flow. In the convectively active region, the western Pacific (120 degrees E-180 degrees), the upper-tropospheric MJO PKE is supported by the convergence of horizontal and vertical wave energy fluxes. Over the central-eastern Pacific (180 degrees-120 degrees W), where convection is suppressed, the upper-tropospheric MJO PKE is mainly due to the horizontal convergence of wave energy flux. The deep convection trigger condition produces stronger convective heating that enhances the perturbation available potential energy (PAPE) production and the upward wave energy fluxes and leads to the increased MJO PKE over the Indian Ocean and western Pacific. The trigger condition also enhances the MJO PKE over the central-eastern Pacific through the increased convergence of meridional wave energy flux from the subtropical latitudes of both hemispheres. The revised convection closure affects the response of mean zonal wind shear to the convective heating over the Indian Ocean and leads to the enhanced upper-tropospheric MJO PKE through the barotropic conversion. The stronger eastward wave energy flux due to the increase of convective heating over the Indian Ocean and western Pacific by the revised closure is favorable to the eastward propagation of MJO and the convergence of horizontal wave energy flux over the central-eastern Pacific. The convection-induced momentum tendency tends to decelerate the upper-tropospheric wind, which results in a negative work to the PKE budget in the upper troposphere. However, the convection momentum tendency accelerates the westerly wind below 800 hPa over the western Pacific, which is partially responsible for the improved MJO simulation. C1 [Deng, Liping] Pacific NW Natl Lab, Richland, WA 99352 USA. [Deng, Liping; Wv, Xiaoqing] Iowa State Univ, Dept Geol & Atmospher Sci, Ames, IA USA. RP Deng, LP (reprint author), Pacific NW Natl Lab, POB 999,MSIN K9-24, Richland, WA 99352 USA. EM liping.deng@pnl.gov FU U.S. Department of Energy [DE-FG02-08ER64559]; National Science Foundation [ATM-0935263]; Department of Energy FX Computing support by Daryl Herzmann is greatly appreciated. This research was partly supported by the Biological and Environmental Research Program (BER), U.S. Department of Energy under Grant DE-FG02-08ER64559 and by the National Science Foundation under Grant ATM-0935263. Work performed while the first author was at PNNL was funded by the Department of Energy's Atmospheric System Research program. NR 35 TC 4 Z9 5 U1 0 U2 1 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0894-8755 J9 J CLIMATE JI J. Clim. PD MAY 15 PY 2011 VL 24 IS 10 BP 2469 EP 2482 DI 10.1175/2010JCLI3759.1 PG 14 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 768WM UT WOS:000290969400004 ER PT J AU Chang, CY Chiang, JCH Wehner, MF Friedman, AR Ruedy, R AF Chang, C. -Y. Chiang, J. C. H. Wehner, M. F. Friedman, A. R. Ruedy, R. TI Sulfate Aerosol Control of Tropical Atlantic Climate over the Twentieth Century SO JOURNAL OF CLIMATE LA English DT Article ID SEA-SURFACE TEMPERATURE; INTERTROPICAL CONVERGENCE ZONE; NORTH-ATLANTIC; BLACK CARBON; VARIABILITY; ANOMALIES; RAINFALL; PACIFIC; SYSTEM; OCEAN AB The tropical Atlantic interhemispheric gradient in sea surface temperature significantly influences the rainfall climate of the tropical Atlantic sector, including droughts over West Africa and Northeast Brazil. This gradient exhibits a secular trend from the beginning of the twentieth century until the 1980s, with stronger warming in the south relative to the north. This trend behavior is on top of a multidecadal variation associated with the Atlantic multidecadal oscillation. A similar long-term forced trend is found in a multimodel ensemble of forced twentieth-century climate simulations. Through examining the distribution of the trend slopes in the multimodel twentieth-century and preindustrial models, the authors conclude that the observed trend in the gradient is unlikely to arise purely from natural variations; this study suggests that at least half the observed trend is a forced response to twentieth-century climate forcings. Further analysis using twentieth-century single-forcing runs indicates that sulfate aerosol forcing is the predominant cause of the multimodel trend. The authors conclude that anthropogenic sulfate aerosol emissions, originating predominantly from the Northern Hemisphere, may have significantly altered the tropical Atlantic rainfall climate over the twentieth century. C1 [Chang, C. -Y.; Chiang, J. C. H.; Friedman, A. R.] Univ Calif Berkeley, Dept Geog, Berkeley, CA 94720 USA. [Chang, C. -Y.; Chiang, J. C. H.; Friedman, A. R.] Univ Calif Berkeley, Ctr Atmopsher Sci, Berkeley, CA 94720 USA. [Wehner, M. F.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Ruedy, R.] NASA, Goddard Inst Space Studies, New York, NY 10025 USA. RP Chang, CY (reprint author), Univ Calif Berkeley, Dept Geog, 595 McCone, Berkeley, CA 94720 USA. EM chingyee.chang@berkeley.edu RI Chiang, John/A-9421-2010; OI Friedman, Andrew/0000-0001-6994-2037 FU Office of Science, U.S. Department of Energy; Office of Science (BER), U.S. Department of Energy [DE-FG02-08ER64588] FX We acknowledge the modeling groups, the Program for Climate Model Diagnosis and Intercomparison (PCMDI) and the WCRP's Working Group on Coupled Modelling (WGCM) for their roles in making available the WCRP CMIP3 multimodel dataset. Support of this dataset is provided by the Office of Science, U.S. Department of Energy. We thank Yochanan Kushnir, Ping Chang, Alessandra Giannini, Michela Biasutti, and Mike Wallace for useful comments and suggestions on a previous version of this manuscript. We thank Zhaohua Wu for providing the code of EEMD analysis, and Ken Lo for help accessing the GISS ModelE single forcing runs, and Mingfang Ting for the use of her AMO index. This research is supported by the Office of Science (BER), U.S. Department of Energy (Award No. DE-FG02-08ER64588 to J. Chiang). NR 46 TC 54 Z9 55 U1 3 U2 12 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0894-8755 EI 1520-0442 J9 J CLIMATE JI J. Clim. PD MAY 15 PY 2011 VL 24 IS 10 BP 2540 EP 2555 DI 10.1175/2010JCLI4065.1 PG 16 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 768WM UT WOS:000290969400009 ER PT J AU Nasreen, F Torikachvili, MS Kothapalli, K Zapf, VS Jardim, RF Nakotte, H AF Nasreen, F. Torikachvili, M. S. Kothapalli, K. Zapf, V. S. Jardim, R. F. Nakotte, H. TI Non-Fermi-liquid behavior in UCu4+xAl8-x compounds SO PHYSICA B-CONDENSED MATTER LA English DT Article DE Non-Fermi-liquid scaling; Antiferromagnetic correlations; Quantum critical point ID INTERMETALLIC COMPOUNDS; THERMOELECTRIC-POWER; HEAVY FERMIONS; TEMPERATURE; URANIUM; ALLOY; PHASE AB We report on experimental studies of the Kondo physics and the development of non-Fermi-liquid scaling in UCu4+xAl8-x family. We studied 7 different compounds with compositions between x = 0 and 2. We measured electrical transport (down to 65 mK) and thermoelectric power (down to 1.8 K) as a function of temperature, hydrostatic pressure, and/or magnetic field. Compounds with Cu content below x = 1.25 exhibit long-range antiferromagnetic order at low temperatures. Magnetic order is suppressed with increasing Cu content and our data indicate a possible quantum critical point at x(cr) approximate to 1.15. For compounds with higher Cu content, non-Fermi-liquid behavior is observed. Non-Fermi-liquid scaling is inferred from electrical resistivity results for the x = 1.25 and 1.5 compounds. For compounds with even higher Cu content, a sharp kink occurs in the resistivity data at low temperatures, and this may be indicative of another quantum critical point that occurs at higher Cu compositions. For the magnetically ordered compounds, hydrostatic pressure is found to increase the Neel temperature, which can be understood in terms of the Kondo physics. For the non-magnetic compounds, application of a magnetic field promotes a tendency toward Fermi-liquid behavior. Thermoelectric power was analyzed using a two-band Lorentzian model, and the results indicate one fairly narrow band (10 meV and below) and a second broad band (around hundred meV). The results imply that there are two relevant energy scales that need to be considered for the physics in this family of compounds. (C) 2011 Elsevier B.V. All rights reserved. C1 [Nasreen, F.; Kothapalli, K.; Nakotte, H.] New Mexico State Univ, Dept Phys, Las Cruces, NM 88003 USA. [Torikachvili, M. S.] San Diego State Univ, Dept Phys, San Diego, CA 92182 USA. [Zapf, V. S.] Los Alamos Natl Lab, Natl High Magnet Field Lab, Pulse Field Facil, Los Alamos, NM 87545 USA. [Jardim, R. F.] Univ Sao Paulo, Inst Fis, BR-05315970 Sao Paulo, Brazil. RP Nakotte, H (reprint author), New Mexico State Univ, Dept Phys, MSC 3D,POB 30001, Las Cruces, NM 88003 USA. EM hnakotte@nmsu.edu RI Zapf, Vivien/K-5645-2013; Nanotecnologias, Inct/I-2407-2013; Jardim, Renato/J-8068-2014 OI Zapf, Vivien/0000-0002-8375-4515; Jardim, Renato/0000-0002-2000-0257 FU National Science Foundation [DMR 0804032, DMR 0805335]; US Department of Energy; State of Florida; Brazil CNPq; Brazil FAPESP FX This work was supported by the National Science Foundation Grants DMR 0804032 and DMR 0805335. Experimental work at the National High Magnetic Field Laboratory, Pulse Field Facility, Los Alamos National Laboratory, was further supported by the NSF, the US Department of Energy and the State of Florida. RFJ gratefully acknowledges the support from Brazil's CNPq and FAPESP. NR 28 TC 2 Z9 2 U1 3 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-4526 J9 PHYSICA B JI Physica B PD MAY 15 PY 2011 VL 406 IS 11 BP 2061 EP 2069 DI 10.1016/j.physb.2011.01.038 PG 9 WC Physics, Condensed Matter SC Physics GA 768QL UT WOS:000290951200002 ER PT J AU Yang, ST Henesian, MA Weiland, TL Vickers, JL Luthi, RL Bielecki, JP Wegner, PJ AF Yang, Steven T. Henesian, Mark A. Weiland, Timothy L. Vickers, James L. Luthi, Ronald L. Bielecki, John P. Wegner, Paul J. TI Noncritically phase-matched fourth harmonic generation of Nd:glass lasers in partially deuterated KDP crystals SO OPTICS LETTERS LA English DT Article ID FREQUENCY-CONVERSION; ABSORPTION; NM AB Noncritically phase-matched (NCPM) fourth harmonic generation (FHG) of Nd:glass laser radiation in partially deuterated dihydrogen phosphate (KD*P) crystals has been demonstrated. At an Nd: glass laser wavelength of 1053:0nm, NCPM FHG is achieved in 70% deuterated KD*P at a crystal temperature of 18.5 +/- 0.1 degrees C. Tuning the fundamental laser wavelength from 1052.9 to 1053.nm, FHG in KD*P is NCPM by changing the crystal temperature from 17.9 degrees C to 20.5 degrees C. When driven with 2.4 J of second harmonic radiation in a 3 ns flat-top pulse, corresponding to 1 GW/cm(2) 2 omega drive intensity, 1: 9 J of fourth harmonic radiation was generated in a 6mm long KD*P crystal, yielding a second to fourth harmonic energy conversion efficiency of 79%. C1 [Yang, Steven T.; Henesian, Mark A.; Weiland, Timothy L.; Vickers, James L.; Luthi, Ronald L.; Bielecki, John P.; Wegner, Paul J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Yang, ST (reprint author), Lawrence Livermore Natl Lab, 7000 E Ave, Livermore, CA 94550 USA. EM yang9@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. NR 11 TC 23 Z9 25 U1 0 U2 8 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 0146-9592 EI 1539-4794 J9 OPT LETT JI Opt. Lett. PD MAY 15 PY 2011 VL 36 IS 10 BP 1824 EP 1826 PG 3 WC Optics SC Optics GA 765NW UT WOS:000290716000028 PM 21593903 ER PT J AU Mikaelian, KO AF Mikaelian, Karnig O. TI Extended model for Richtmyer-Meshkov mix SO PHYSICA D-NONLINEAR PHENOMENA LA English DT Article DE Richtmyer-Meshkov; Shocks; Turbulence; Mix ID RAYLEIGH-TAYLOR INSTABILITY; ACCELERATION; DEPENDENCE; INTERFACE; FLUIDS; LAWS AB Mixing between two adjacent fluids has important consequences for inertial fusion capsule implosions and for supernova explosions. Consider an interface with small, random perturbations between two fluids of densities rho(A) and rho(B). When a shock passes through the interface, those perturbations grow and the two fluids begin mixing in a process called Richtmyer-Meshkov (RM) mix, in analogy with Rayleigh-Taylor (RT) mix generated when the system undergoes a constant acceleration. Around the interface a time-dependent mixing width h evolves from the initial value h(0) and grows very large for strong shocks. If the interface sees a second shock, also called a reshock, the mixing is again intensified. In this paper we examine four RM experiments on shock-generated turbulent mix and find them to be in good agreement with our earlier simple model in which the growth rate h of the mixing layer following a shock or reshock is constant and given by 2 alpha A Delta v. Here A is the Atwood number (rho(B) - rho(A))/(rho(B) + rho(A)), Delta v is the jump in velocity induced by the shock or reshock, and alpha is the constant measured in RT experiments: alpha(bubble) approximate to 0.05-0.07, alpha(spike) approximate to (1.8-2.5)alpha(bubble) for A approximate to 0.7-1.0. We then extend the model to t > t* or, equivalently, h > h* when the growth rate begins to decay and exhibit Is t We ascribe this changeover to loss of memory of the direction of the shock or reshock, signaling the transition from highly directional to isotropic turbulence. In the simplest extension of the model, h*/h(0) is independent of Delta v and depends only on A: h*/h(0) approximate to 2.5 - 3.5 for A approximate to 0.7 - 1.0. (C) 2011 Elsevier B.V. All rights reserved. C1 Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Mikaelian, KO (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM mikaelian1@llnl.gov FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 33 TC 8 Z9 10 U1 1 U2 16 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-2789 J9 PHYSICA D JI Physica D PD MAY 15 PY 2011 VL 240 IS 11 BP 935 EP 942 DI 10.1016/j.physd.2011.01.008 PG 8 WC Mathematics, Applied; Physics, Multidisciplinary; Physics, Mathematical SC Mathematics; Physics GA 766XT UT WOS:000290820600004 ER PT J AU Du, D Wang, J Wang, LM Lu, DL Smith, JN Timchalk, C Lin, YH AF Du, Dan Wang, Jun Wang, Limin Lu, Donglai Smith, Jordan N. Timchalk, Charles Lin, Yuehe TI Magnetic Electrochemical Sensing Platform for Biomonitoring of Exposure to Organophosphorus Pesticides and Nerve Agents Based on Simultaneous Measurement of Total Enzyme Amount and Enzyme Activity SO ANALYTICAL CHEMISTRY LA English DT Article ID PHOSPHORYLATED ACETYLCHOLINESTERASE; HUMAN SERUM; BUTYRYLCHOLINESTERASE; ASSAY; IMMOBILIZATION; BIOMARKER; CHOLINESTERASES; AMPLIFICATION; IMMUNOSENSOR; IMMUNOASSAYS AB We report a new approach for electrochemical quantification of enzymatic inhibition and phosphorylation for biomonitoring of exposure to organophosphorus (OP) pesticides and nerve agents based on a magnetic bead (MB) immunosensing platform. The principle of this approach is based on the combination of ME immunocapture-based enzyme activity assay and competitive immunoassay of the total amount of enzyme for simultaneous detection of enzyme inhibition and phosphorylation in biological fluids. Butyrylcholinesterase (BChE) was chosen as a model enzyme. In competitive immunoassay, the target BChE in a sample competes with the BChE immobilized on the Alas to bind to the limited sites of anti-BChE antibody labeled with quantum dots (QD anti-BChE), followed by stripping voltammetric analysis of the bound QD conjugate on the MBs. This assay shows a linear response over the total BChE concentration range of 0.1-20 nM. Simultaneous real time BChE activity was measured on an electrochemical carbon nanotube-based sensor coupled with a microflow injection system after immunocapture by the MB anti-BChE conjugate. Therefore, the formed phosphorylated BChE adduct (OP BChE) can be estimated by the difference values of the total amount of BChE (including active and OP-inhibited) and active BChE from established calibration curves. This approach not only eliminates the difficulty in screening of low-dose OP exposure (less than 20% inhibition of BChE) because of individual variation of BChE values but also avoids the drawback of the scarce availability of OP BChE antibody. It is sensitive enough to detect 0.5 nM OP BChE, which is less than 2% BChE inhibition. This method offers a new method for rapid, accurate, selective, and inexpensive quantification of OP-BChE and enzyme inhibition for biomonitoring of OP and nerve agent exposures. C1 [Du, Dan; Wang, Jun; Wang, Limin; Lu, Donglai; Smith, Jordan N.; Timchalk, Charles; Lin, Yuehe] Pacific NW Natl Lab, Richland, WA 99352 USA. [Du, Dan] Cent China Normal Univ, Coll Chem, Minist Educ, Key Lab Pesticide & Chem Biol, Wuhan 430079, Peoples R China. RP Wang, J (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM jun.wang@pnl.gov; yuehe.lin@pnl.gov RI Lin, Yuehe/D-9762-2011; Du, Dan (Annie)/G-3821-2012 OI Lin, Yuehe/0000-0003-3791-7587; FU National Institutes of Health through the National Institute of Neurological Disorders and Stroke, NIH [U01 NS058161-01]; CDC/NIOSH [R01 OH008173-01]; National Natural Science Foundation of China [21075047]; Program for Chenguang Young Scientist for Wuhan [200950431184]; Special Fund for Basic Scientific Research of Central Colleges [CCNU10A02005]; Department of Energy's Office of Biological and Environmental Research at Pacific Northwest National Laboratory; DOE [DE-AC05-76RL01830] FX The work was performed at Pacific Northwest National Laboratory (PNNL) and supported partially by grant number U01 NS058161-01 from the National Institutes of Health CounterACT Program through the National Institute of Neurological Disorders and Stroke, NIH, and CDC/NIOSH Grant R01 OH008173-01. This work was also supported partially by the National Natural Science Foundation of China (21075047), the Program for Chenguang Young Scientist for Wuhan (200950431184), and the Special Fund for Basic Scientific Research of Central Colleges (CCNU10A02005). A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. PNNL is operated by Battelle for DOE under Contract DE-AC05-76RL01830. The authors thank Alice Dohnalkova for the TEM experiment and Mark H. Engelhard for the XPS analysis. NR 32 TC 41 Z9 41 U1 7 U2 65 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 J9 ANAL CHEM JI Anal. Chem. PD MAY 15 PY 2011 VL 83 IS 10 BP 3770 EP 3777 DI 10.1021/ac200217d PG 8 WC Chemistry, Analytical SC Chemistry GA 762HO UT WOS:000290466000022 PM 21462919 ER PT J AU Dresel, PE Wellman, DM Cantrell, KJ Truex, MJ AF Dresel, P. Evan Wellman, Dawn M. Cantrell, Kirk J. Truex, Michael J. TI Review: Technical and Policy Challenges in Deep Vadose Zone Remediation of Metals and Radionuclides SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Review ID IN-SITU REMEDIATION; PERMEABLE REACTIVE BARRIER; ZERO-VALENT IRON; CONTAMINATED SOILS; ELECTROKINETIC REMEDIATION; HYDROGEN-SULFIDE; GEOCHEMICAL CONDITIONS; ENHANCED REMEDIATION; URANYL INCORPORATION; CALCIUM POLYSULFIDE AB Contamination in deep vadose zone environments is isolated from exposure so direct contact is not a factor in its risk to human health and the environment. Instead, movement of contamination to the groundwater creates the potential for exposure and risk to receptors. Limiting flux from contaminated vadose zone is key for protection of groundwater resources, thus the deep vadose zone is not necessarily considered a resource requiring restoration. Contaminant discharge to the groundwater must be maintained low enough by natural attenuation (e.g., adsorption processes or radioactive decay) or through remedial actions (e.g., contaminant mass reduction or mobility reduction) to meet the groundwater concentration goals. This paper reviews the major processes for deep vadose zone metal and radionuclide remediation that form the practical constraints on remedial actions. Remediation of metal and radionuclide contamination in the deep vadose zone is complicated by heterogeneous contaminant distribution and the saturation-dependent preferential flow in heterogeneous sediments. Thus, efforts to remove contaminants have generally been unsuccessful although partial removal may reduce downward flux. Contaminant mobility may be reduced through abiotic and biotic reactions or through physical encapsulation. Hydraulic controls may limit aqueous transport. Delivering amendments to the contaminated zone and verifying performance are challenges for remediation. C1 [Dresel, P. Evan] Future Farming Syst Res Div, Dept Primary Ind, Bendigo, Vic 3554, Australia. [Dresel, P. Evan; Wellman, Dawn M.; Cantrell, Kirk J.; Truex, Michael J.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Dresel, PE (reprint author), Future Farming Syst Res Div, Dept Primary Ind, Bendigo Delivery Ctr, POB 3100, Bendigo, Vic 3554, Australia. EM evan.dresel@dpi.vic.gov.au FU U.S. Department of Energy (DOE); Environmental Management [EM-32]; Office of Groundwater and Soil Remediation FX This research was supported by the U.S. Department of Energy (DOE) Environmental Management EM-32, Office of Groundwater and Soil Remediation. Pacific Northwest National Laboratory is operated for the Department of Energy by Battelle Memorial Institute. The authors would like to especially thank Mike Perkins of Pacific Northwest National Laboratory for his process conceptualizations and production of the graphics contained within this manuscript. The paper has benefited greatly from the peer review comments. NR 138 TC 20 Z9 21 U1 12 U2 88 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAY 15 PY 2011 VL 45 IS 10 BP 4207 EP 4216 DI 10.1021/es101211t PG 10 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 761UQ UT WOS:000290426900009 PM 21395250 ER PT J AU Salazar, JM Zitney, SE Diwekar, UM AF Salazar, Juan M. Zitney, Stephen E. Diwekar, Urmila M. TI Minimization of Water Consumption under Uncertainty for a Pulverized Coal Power Plant SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article AB Coal-fired power plants are large water consumers. Water consumption in thermoelectric generation is strongly associated with evaporation losses and makeup streams on cooling and contaminant removal systems. Thus, minimization of water consumption requires optimal operating conditions and parameters, while fulfilling the environmental constraints. Several uncertainties affect the operation of the plants, and this work studies those associated with weather. Air conditions (temperature and humidity) were included as uncertain factors for pulverized coal (PC) power plants. Optimization under uncertainty for these large-scale complex processes with black-box models cannot be solved with conventional stochastic programming algorithms because of the large computational expense. Employment of the novel better optimization of nonlinear uncertain systems (BONUS) algorithm, dramatically decreased the computational requirements of the stochastic optimization. Operating conditions including reactor temperatures and pressures; reactant ratios and conditions; and steam flow rates and conditions were calculated to obtain the minimum water consumption under the above-mentioned uncertainties. Reductions of up to 6.3% in water consumption were obtained for the fall season when process variables were set to optimal values. Additionally, the proposed methodology allowed the analysis of other performance parameters like gas emissions and cycle efficiency which were also improved. C1 [Salazar, Juan M.; Diwekar, Urmila M.] Vishwamitra Res Inst, Ctr Uncertain Syst Tools Optimizat & Management, Clarendon Hills, IL 60514 USA. [Zitney, Stephen E.] Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Diwekar, UM (reprint author), Vishwamitra Res Inst, Ctr Uncertain Syst Tools Optimizat & Management, Clarendon Hills, IL 60514 USA. EM urmila@vri-custom.org FU National Energy Technology Laboratory under the RDS [DE-06-485AA-VRI] FX This technical effort was performed with financial support of the National Energy Technology Laboratory's ongoing research in Process and Dynamic Systems Research under the RDS contract DE-06-485AA-VRI. NR 15 TC 4 Z9 4 U1 1 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAY 15 PY 2011 VL 45 IS 10 BP 4645 EP 4651 DI 10.1021/es1043062 PG 7 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 761UQ UT WOS:000290426900067 PM 21517062 ER PT J AU Moran, JJ Newburn, MK Alexander, ML Sams, RL Kelly, JF Kreuzer, HW AF Moran, James J. Newburn, Matt K. Alexander, M. Lizabeth Sams, Robert L. Kelly, James F. Kreuzer, Helen W. TI Laser ablation isotope ratio mass spectrometry for enhanced sensitivity and spatial resolution in stable isotope analysis SO RAPID COMMUNICATIONS IN MASS SPECTROMETRY LA English DT Article ID CARBON ISOTOPES; DIET CHANGES; TREE-RINGS; TAIL-HAIR; GC-IRMS; PTR-MS; DELTA-C-13; C-13; QUANTITIES; DENSITY AB Stable isotope analysis permits the tracking of physical, chemical, and biological reactions and source materials at a wide variety of spatial scales. We present a laser ablation isotope ratio mass spectrometry (LA-IRMS) method that enables delta(13)C measurement of solid samples at 50 mu m spatial resolution. The method does not require sample pretreatment to physically separate spatial zones. We use laser ablation of solid samples followed by quantitative combustion of the ablated particulates to convert sample carbon into CO(2). Cryofocusing of the resulting CO(2) coupled with modulation in the carrier flow rate permits coherent peak introduction into an isotope ratio mass spectrometer, with only 65 ng carbon required per measurement. We conclusively demonstrate that the measured CO(2) is produced by combustion of laser-ablated aerosols from the sample surface. We measured delta(13)C for a series of solid compounds using laser ablation and traditional solid sample analysis techniques. Both techniques produced consistent isotopic results but the laser ablation method required over two orders of magnitude less sample. We demonstrated that LA-IRMS sensitivity coupled with its 50 mu m spatial resolution could be used to measure delta(13)C values along a length of hair, making multiple sample measurements over distances corresponding to a single day's growth. This method will be highly valuable in cases where the delta(13)C analysis of small samples over prescribed spatial distances is required. Suitable applications include forensic analysis of hair samples, investigations of tightly woven microbial systems, and cases of surface analysis where there is a sharp delineation between different components of a sample. Copyright (C) 2011 John Wiley & Sons, Ltd. C1 [Moran, James J.; Newburn, Matt K.; Alexander, M. Lizabeth; Sams, Robert L.; Kelly, James F.; Kreuzer, Helen W.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Moran, JJ (reprint author), Pacific NW Natl Lab, POB 999,MSIN P7-50, Richland, WA 99352 USA. EM James.Moran@pnl.gov OI Moran, James/0000-0001-9081-9017 FU U.S. Department of Energy [DE-AC05-76RL01830] FX The research was conducted under the Laboratory Directed Research and Development Program at Pacific Northwest National Laboratory, a multiprogram laboratory operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830. A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. We are grateful to Charlie and Terri Thompson for providing the sample of horse hair used in our spatial resolution study. NR 35 TC 13 Z9 13 U1 4 U2 42 PU WILEY-BLACKWELL PI MALDEN PA COMMERCE PLACE, 350 MAIN ST, MALDEN 02148, MA USA SN 0951-4198 J9 RAPID COMMUN MASS SP JI Rapid Commun. Mass Spectrom. PD MAY 15 PY 2011 VL 25 IS 9 BP 1282 EP 1290 DI 10.1002/rcm.4985 PG 9 WC Biochemical Research Methods; Chemistry, Analytical; Spectroscopy SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy GA 762DN UT WOS:000290452600020 PM 21488126 ER PT J AU Hulot, SL Cale, EM Korber, BT Letvin, NL AF Hulot, Sandrine L. Cale, Evan M. Korber, Bette T. Letvin, Norman L. TI Vaccine-Induced CD8(+) T Lymphocytes of Rhesus Monkeys Recognize Variant Forms of an HIV Epitope but Do Not Mediate Optimal Functional Activity SO JOURNAL OF IMMUNOLOGY LA English DT Article ID HUMAN-IMMUNODEFICIENCY-VIRUS; MAJOR HISTOCOMPATIBILITY COMPLEX; DISEASE PROGRESSION; PRIMARY INFECTION; IMMUNE-RESPONSES; DNA VACCINATION; ESCAPE VARIANTS; CELL RESPONSES; AIDS VACCINE; TYPE-1 AB The sequence diversity of HIV-1 presents a challenge for the development of an effective HIV-1 vaccine, because such a vaccine must confer protection against diverse forms of the virus. The present studies were initiated to explore how vaccine-induced clonal populations of CD8 (+) T lymphocytes of rhesus monkeys recognize variants of an HIV-1 envelope epitope sequence. Evaluating a subset of variants of a selected epitope peptide that retain their binding to the MHC class I molecule of rhesus monkeys that presents this epitope peptide, we show that vaccine-elicited CD8(+) T lymphocytes comparably recognize the wild-type and a number of variant epitope peptides as determined by tetramer binding assays. In fact, the same clonal populations of CD8(+) T lymphocytes recognize the wild-type and variant epitope peptides. However, functional assays show that many of these variant epitope peptides stimulate suboptimal cytokine production by the vaccine-elicited CD8(+) T lymphocytes. These findings suggest that vaccine-induced CD8(+) T lymphocyte populations may recognize diverse forms of a viral epitope, but may not function optimally to confer protection against viruses expressing many of those variant sequences. The Journal of Immunology, 2011, 186: 5663-5674. C1 [Letvin, Norman L.] Harvard Univ, Sch Med, Beth Israel Deaconess Med Ctr, Div Viral Pathogenesis,Ctr Life Sci, Boston, MA 02215 USA. [Korber, Bette T.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Letvin, NL (reprint author), Harvard Univ, Sch Med, Beth Israel Deaconess Med Ctr, Div Viral Pathogenesis,Ctr Life Sci, 10th Floor,Room 1043,330 Brookline Ave, Boston, MA 02215 USA. EM nletvin@bidmc.harvard.edu OI Korber, Bette/0000-0002-2026-5757 FU National Institute of Allergy and Infectious Diseases Center for HIV/AIDS Vaccine Immunology [AI067854] FX This work was supported by the National Institute of Allergy and Infectious Diseases Center for HIV/AIDS Vaccine Immunology (Grant AI067854). NR 48 TC 4 Z9 4 U1 0 U2 2 PU AMER ASSOC IMMUNOLOGISTS PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814 USA SN 0022-1767 J9 J IMMUNOL JI J. Immunol. PD MAY 15 PY 2011 VL 186 IS 10 BP 5663 EP 5674 DI 10.4049/jimmunol.1100287 PG 12 WC Immunology SC Immunology GA 758GJ UT WOS:000290150700017 PM 21490161 ER PT J AU Lamendella, R Domingo, JWS Ghosh, S Martinson, J Oerther, DB AF Lamendella, Regina Domingo, Jorge W. Santo Ghosh, Shreya Martinson, John Oerther, Daniel B. TI Comparative fecal metagenomics unveils unique functional capacity of the swine gut SO BMC MICROBIOLOGY LA English DT Article ID GASTROINTESTINAL-TRACT; MICROBIAL DIVERSITY; PIG FARMS; GENE; COMMUNITIES; ANNOTATION; EVOLUTION; RESOURCE; TRACKING; PROJECT AB Background: Uncovering the taxonomic composition and functional capacity within the swine gut microbial consortia is of great importance to animal physiology and health as well as to food and water safety due to the presence of human pathogens in pig feces. Nonetheless, limited information on the functional diversity of the swine gut microbiome is available. Results: Analysis of 637, 722 pyrosequencing reads (130 megabases) generated from Yorkshire pig fecal DNA extracts was performed to help better understand the microbial diversity and largely unknown functional capacity of the swine gut microbiome. Swine fecal metagenomic sequences were annotated using both MG-RAST and JGI IMG/M-ER pipelines. Taxonomic analysis of metagenomic reads indicated that swine fecal microbiomes were dominated by Firmicutes and Bacteroidetes phyla. At a finer phylogenetic resolution, Prevotella spp. dominated the swine fecal metagenome, while some genes associated with Treponema and Anareovibrio species were found to be exclusively within the pig fecal metagenomic sequences analyzed. Functional analysis revealed that carbohydrate metabolism was the most abundant SEED subsystem, representing 13% of the swine metagenome. Genes associated with stress, virulence, cell wall and cell capsule were also abundant. Virulence factors associated with antibiotic resistance genes with highest sequence homology to genes in Bacteroidetes, Clostridia, and Methanosarcina were numerous within the gene families unique to the swine fecal metagenomes. Other abundant proteins unique to the distal swine gut shared high sequence homology to putative carbohydrate membrane transporters. Conclusions: The results from this metagenomic survey demonstrated the presence of genes associated with resistance to antibiotics and carbohydrate metabolism suggesting that the swine gut microbiome may be shaped by husbandry practices. C1 [Domingo, Jorge W. Santo] US EPA, Natl Risk Management Res Lab, Cincinnati, OH 45268 USA. [Lamendella, Regina; Ghosh, Shreya; Oerther, Daniel B.] Univ Cincinnati, Dept Civil & Environm Engn, Cincinnati, OH 45220 USA. [Martinson, John] US EPA, Natl Exposure Res Lab, Cincinnati, OH 45268 USA. [Lamendella, Regina] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Oerther, Daniel B.] Missouri Univ Sci & Technol, Dept Civil & Environm Engn, Rolla, MO 65409 USA. RP Domingo, JWS (reprint author), US EPA, Natl Risk Management Res Lab, Cincinnati, OH 45268 USA. EM santodomingo.jorge@epa.gov RI Oerther, Daniel/H-6543-2014 OI Oerther, Daniel/0000-0002-6724-3205 FU U.S. Environmental Protection Agency, through its Office of Research and Development; United States Environmental Protection Agency; National Science Foundation FX The U.S. Environmental Protection Agency, through its Office of Research and Development, funded and managed, or partially funded and collaborated in, the research described herein. It has been subjected to the Agency's administrative review and has been approved for external publication. Any opinions expressed in this paper are those of the author(s) and do not necessarily reflect the views of the Agency, therefore, no official endorsement should be inferred. Any mention of trade names or commercial products does not constitute endorsement or recommendation for use. This work was also partly funded by the United States Environmental Protection Agency Traineeship and National Science Foundation grant to DBO. NR 42 TC 109 Z9 118 U1 10 U2 109 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2180 J9 BMC MICROBIOL JI BMC Microbiol. PD MAY 15 PY 2011 VL 11 AR 103 DI 10.1186/1471-2180-11-103 PG 17 WC Microbiology SC Microbiology GA 783MX UT WOS:000292088700001 PM 21575148 ER PT J AU Cohen, ML Malone, BD AF Cohen, Marvin L. Malone, Brad D. TI Wave function engineering: Other phases of Si for photovoltaic applications SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 30th International Conference on the Physics of Semiconductors (ICPS-30) CY JUL 25-30, 2010 CL Seoul, SOUTH KOREA ID AB-INITIO CALCULATION; TRANSMISSION ELECTRON-MICROSCOPY; HOLE EXCITATIONS; OPTICAL-SPECTRA; TOTAL-ENERGY; SILICON; SEMICONDUCTORS; INSULATORS; PSEUDOPOTENTIALS AB We present first-principles electronic structural calculations of the quasiparticle and optical spectra of two silicon phases, Si-XII and the recently predicted phase of Si in the body-centered-tetragonal structure. The quasiparticle spectra calculated within the GW approximation predict that both of these materials are indirect bandgap semiconductors with small bandgaps. The optical spectra of these materials are obtained by solving the Bethe-Salpeter equation taking into account electron-hole interactions. Comparison is made to other phases of silicon commonly used in photovoltaic applications. The results suggest the possible utility of these materials as photovoltaics. (C) 2011 American Institute of Physics. [doi:10.1063/1.3575641] C1 [Cohen, Marvin L.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Cohen, ML (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM mlcohen@berkeley.edu NR 29 TC 9 Z9 9 U1 0 U2 5 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 15 PY 2011 VL 109 IS 10 AR 102402 DI 10.1063/1.3575641 PG 5 WC Physics, Applied SC Physics GA 783WU UT WOS:000292115900003 ER PT J AU He, L Xiu, FX Wang, Y Fedorov, AV Huang, G Kou, XF Lang, MR Beyermann, WP Zou, J Wang, KL AF He, Liang Xiu, Faxian Wang, Yong Fedorov, Alexei V. Huang, Guan Kou, Xufeng Lang, Murong Beyermann, Ward P. Zou, Jin Wang, Kang L. TI Epitaxial growth of Bi2Se3 topological insulator thin films on Si (111) SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID SINGLE DIRAC CONE; SURFACE-STATES; BI2TE3; OSCILLATIONS AB In this paper, we report the epitaxial growth of Bi2Se3 thin films on Si (1 1 1) substrate, using molecular beam epitaxy (MBE). We show that the as-grown samples have good crystalline quality, and their surfaces exhibit terracelike quintuple layers. Angel-resolved photoemission experiments demonstrate single-Dirac-conelike surface states. These results combined with the temperature-and thickness-dependent magneto-transport measurements, suggest the presence of a shallow impurity band. Below a critical temperature of similar to 100K, the surface states of a 7 nm thick film contribute up to 50% of the total conduction. (C) 2011 American Institute of Physics. [doi:10.1063/1.3585673] C1 [He, Liang; Xiu, Faxian; Wang, Yong; Huang, Guan; Kou, Xufeng; Lang, Murong; Wang, Kang L.] Univ Calif Los Angeles, Dept Elect Engn, Los Angeles, CA 90095 USA. [Wang, Yong; Zou, Jin] Univ Queensland, Ctr Microcopy & Microanal, Brisbane, Qld 4072, Australia. [Fedorov, Alexei V.] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source Div, Berkeley, CA 94720 USA. [Beyermann, Ward P.] Univ Calif Riverside, Dept Phys, Riverside, CA 92521 USA. RP He, L (reprint author), Univ Calif Los Angeles, Dept Elect Engn, Los Angeles, CA 90095 USA. EM heliang@ee.ucla.edu RI Wang, Yong/A-7766-2010; Xiu, Faxian/B-4985-2012; He, Liang/E-5935-2012; Zou, Jin/B-3183-2009; OI Wang, Yong/0000-0002-9893-8296; Zou, Jin/0000-0001-9435-8043; Kou, Xufeng/0000-0002-8860-5105 NR 30 TC 62 Z9 62 U1 9 U2 81 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 15 PY 2011 VL 109 IS 10 AR 103702 DI 10.1063/1.3585673 PG 6 WC Physics, Applied SC Physics GA 783WU UT WOS:000292115900078 ER PT J AU Morris, CL Ables, E Alrick, KR Aufderheide, MB Barnes, PD Buescher, KL Cagliostro, DJ Clark, DJ Espinoza, CJ Ferm, EN Gallegos, RA Gardner, SD Gomez, JJ Greene, GA Hanson, A Hartouni, EP Hogan, GE King, NSP Kwiatkowski, K Liljestrand, RP Mariam, FG Merrill, FE Morgan, DV Morley, KB Mottershead, CT Murray, MM Pazuchanics, PD Pearson, JE Sarracino, JS Saunders, A Scaduto, J von Wittenau, AES Soltz, RA Sterbenz, S Thompson, RT Vixie, K Wilke, MD Wright, DM Zumbro, JD AF Morris, C. L. Ables, E. Alrick, K. R. Aufderheide, M. B. Barnes, P. D., Jr. Buescher, K. L. Cagliostro, D. J. Clark, D. J. Espinoza, C. J. Ferm, E. N. Gallegos, R. A. Gardner, S. D. Gomez, J. J. Greene, G. A. Hanson, A. Hartouni, E. P. Hogan, G. E. King, N. S. P. Kwiatkowski, K. Liljestrand, R. P. Mariam, F. G. Merrill, F. E. Morgan, D. V. Morley, K. B. Mottershead, C. T. Murray, M. M. Pazuchanics, P. D. Pearson, J. E. Sarracino, J. S. Saunders, A. Scaduto, J. von Wittenau, A. E. Schach Soltz, R. A. Sterbenz, S. Thompson, R. T. Vixie, K. Wilke, M. D. Wright, D. M. Zumbro, J. D. TI Flash radiography with 24 GeV/c protons SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID MULTIPLE COULOMB SCATTERING; ACCELERATOR; IONIZATION; PARTICLES; DIAGNOSIS; FACILITY; NUCLEAR; MODEL; TOOL AB The accuracy of density measurements and position resolution in flash (40 ns) radiography of thick objects with 24 Gev/c protons is investigated. A global model fit to step wedge data is shown to give a good description spanning the periodic table. The parameters obtained from the step wedge data are used to predict transmission through the French Test Object (FTO), a test object of nested spheres, to a precision better than 1%. Multiple trials have been used to show that the systematic errors are less than 2%. Absolute agreement between the average radiographic measurements of the density and the known density is 1%. Spatial resolution has been measured to be 200 mu m at the center of the FTO. These data verify expectations of the benefits provided by high energy hadron radiography for thick objects. (C) 2011 American Institute of Physics. [doi:10.1063/1.3580262] C1 [Morris, C. L.; Alrick, K. R.; Buescher, K. L.; Cagliostro, D. J.; Clark, D. J.; Espinoza, C. J.; Ferm, E. N.; Gallegos, R. A.; Gomez, J. J.; Hogan, G. E.; King, N. S. P.; Kwiatkowski, K.; Liljestrand, R. P.; Mariam, F. G.; Merrill, F. E.; Morley, K. B.; Mottershead, C. T.; Murray, M. M.; Pazuchanics, P. D.; Pearson, J. E.; Sarracino, J. S.; Saunders, A.; Sterbenz, S.; Vixie, K.; Wilke, M. D.; Zumbro, J. D.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. [Ables, E.; Aufderheide, M. B.; Barnes, P. D., Jr.; Hartouni, E. P.; von Wittenau, A. E. Schach; Soltz, R. A.; Wright, D. M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Gardner, S. D.; Morgan, D. V.; Wilke, M. D.] Natl Secur Technol LLC, Los Alamos, NM 87544 USA. [Greene, G. A.; Hanson, A.; Thompson, R. T.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Morris, CL (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA. EM cmorris@lanl.gov OI Morris, Christopher/0000-0003-2141-0255; Hartouni, Edward/0000-0001-9869-4351; Merrill, Frank/0000-0003-0603-735X NR 49 TC 21 Z9 26 U1 0 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 15 PY 2011 VL 109 IS 10 AR 104905 DI 10.1063/1.3580262 PG 10 WC Physics, Applied SC Physics GA 783WU UT WOS:000292115900150 ER PT J AU Schreiber, DK Choi, YS Liu, YZ Chiaramonti, AN Seidman, DN Petford-Long, AK AF Schreiber, Daniel K. Choi, Young-Suk Liu, Yuzi Chiaramonti, Ann N. Seidman, David N. Petford-Long, Amanda K. TI Effects of elemental distributions on the behavior of MgO-based magnetic tunnel junctions SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ATOM-PROBE TOMOGRAPHY; FORMATION MECHANISM; MAGNETORESISTANCE; BARRIERS AB Three-dimensional atom-probe tomography and transmission electron microscopy have been utilized to study the effects of Ta getter presputtering and either a Mg or Ru free-layer cap on the elemental distributions and properties of MgO-based magnetic tunnel junctions after annealing. Annealing the samples resulted in crystallization of the amorphous CoFeB layer and diffusion of the majority of the boron away from the crystallized CoFeB layers. The Ta getter presputter is found to reduce the segregation of boron at the MgO/CoFeB interface after annealing, improving the tunneling magnetoresistance of the tunnel junction. This effect is observed for samples with either a Ru free-layer cap or a Mg free-layer cap and is thought to be a result of a reduced oxygen concentration within the MgO due to the effect of Ta getter presputtering. A Ru free-layer cap provides superior magnetic and magnetotransport properties compared to a Mg free-layer cap. Mg from the Mg free-layer cap is observed to diffuse toward the MgO tunnel barrier upon annealing, degrading both the crystalline quality of the CoFeB and magnetic isolation of the CoFeB free-layer from the CoFeB reference-layer. Lateral variations in the B distribution within the CoFeB free-layer are observed in the samples with a Ru free-layer cap, which are associated with crystalline and amorphous grains. The B-rich, amorphous grains are found to be depleted in Fe, while the B-poor crystalline grains are slightly enriched in Fe. (C) 2011 American Institute of Physics. [doi :10.1063/1.3583569] C1 [Schreiber, Daniel K.; Seidman, David N.; Petford-Long, Amanda K.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Schreiber, Daniel K.; Liu, Yuzi; Chiaramonti, Ann N.; Petford-Long, Amanda K.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Choi, Young-Suk] Canon ANELVA Corp, Elect Devices Engn Headquarters, Kawasaki, Kanagawa 2158550, Japan. [Seidman, David N.] Northwestern Univ, NUCAPT, Evanston, IL 60208 USA. RP Schreiber, DK (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. EM young-suk.choi@hitachigst.com RI Seidman, David/B-6697-2009; Chiaramonti, Ann/E-7459-2013; Petford-Long, Amanda/P-6026-2014; Liu, Yuzi/C-6849-2011 OI Chiaramonti, Ann/0000-0001-9933-3267; Petford-Long, Amanda/0000-0002-3154-8090; NR 51 TC 10 Z9 10 U1 0 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 15 PY 2011 VL 109 IS 10 AR 103909 DI 10.1063/1.3583569 PG 8 WC Physics, Applied SC Physics GA 783WU UT WOS:000292115900098 ER PT J AU Novikov, SV Staddon, CR Foxon, CT Yu, KM Broesler, R Hawkridge, M Liliental-Weber, Z Denlinger, J Demchenko, I Luckert, F Edwards, PR Martin, RW Walukiewicz, W AF Novikov, S. V. Staddon, C. R. Foxon, C. T. Yu, K. M. Broesler, R. Hawkridge, M. Liliental-Weber, Z. Denlinger, J. Demchenko, I. Luckert, F. Edwards, P. R. Martin, R. W. Walukiewicz, W. TI Growth by molecular beam epitaxy of amorphous and crystalline GaNAs alloys with band gaps from 3.4 to 0.8 eV for solar energy conversion devices SO JOURNAL OF CRYSTAL GROWTH LA English DT Article; Proceedings Paper CT 16th International Conference on Molecular Beam Epitaxy (ICMBE) CY AUG 22-27, 2010 CL Berlin, GERMANY DE Molecular beam epitaxy; Nitrides; Semiconducting III-V materials ID LAYERS AB Using low temperature MBE, we have shown that it is possible to grow amorphous GaN1-xAsx layers with a variable As content (0 < x < 0.8) on both crystalline (sapphire and silicon) and amorphous (glass and Pyrex glass) substrates. Despite the fact that the samples with high As content are amorphous, we observe a gradual continuous decrease of bandgap from similar to 3.4 to similar to 0.8 eV with increase in As content. To the best of our knowledge this is the first demonstration of homogeneous amorphous GaN-based alloys over a wide composition range. The large band gap range of the amorphous phase of GaNAs covers much of the solar spectrum. The amorphous nature of the GaNAs alloys is particularly advantageous since low cost substrates such as glass and Pyrex glass can be used for solar cell fabrication. (C) 2010 Elsevier B.V. All rights reserved. C1 [Novikov, S. V.; Staddon, C. R.; Foxon, C. T.] Univ Nottingham, Sch Phys & Astron, Nottingham NG7 2RD, England. [Yu, K. M.; Broesler, R.; Hawkridge, M.; Liliental-Weber, Z.; Walukiewicz, W.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Denlinger, J.; Demchenko, I.] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. [Luckert, F.; Edwards, P. R.; Martin, R. W.] Univ Strathclyde, Dept Phys, SUPA, Glasgow G4 0NG, Lanark, Scotland. RP Novikov, SV (reprint author), Univ Nottingham, Sch Phys & Astron, Nottingham NG7 2RD, England. EM Sergei.Novikov@Nottingham.ac.uk RI Liliental-Weber, Zuzanna/H-8006-2012; Yu, Kin Man/J-1399-2012; martin, rob/A-7127-2010; Edwards, Paul/C-1594-2009; OI Yu, Kin Man/0000-0003-1350-9642; martin, rob/0000-0002-6119-764X; Edwards, Paul/0000-0001-7671-7698; Novikov, Sergei/0000-0002-3725-2565 NR 8 TC 8 Z9 8 U1 0 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-0248 J9 J CRYST GROWTH JI J. Cryst. Growth PD MAY 15 PY 2011 VL 323 IS 1 SI SI BP 60 EP 63 DI 10.1016/j.jcrysgro.2010.11.064 PG 4 WC Crystallography; Materials Science, Multidisciplinary; Physics, Applied SC Crystallography; Materials Science; Physics GA 784RD UT WOS:000292175000016 ER PT J AU Kartal, G Eryilmaz, OL Krumdick, G Erdemir, A Timur, S AF Kartal, G. Eryilmaz, O. L. Krumdick, G. Erdemir, A. Timur, S. TI Kinetics of electrochemical boriding of low carbon steel SO APPLIED SURFACE SCIENCE LA English DT Article DE Electrochemical boriding; Growth kinetics; Activation energy; Boride layer thickness ID MOLTEN-SALTS; GROWTH-KINETICS; ALLOYING ELEMENTS; LAYERS; IRON; MECHANISM; PHASE AB In this study, the growth kinetics of the boride layers forming on low carbon steel substrates was investigated during electrochemical boriding which was performed at a constant current density of 200 mA/cm(2) in a borax based electrolyte at temperatures ranging from 1123K to 1273K for periods of 5-120 min. After boriding, the presence of both FeB and Fe(2)B phases were confirmed by the X-ray diffraction method. Cross-sectional microscopy revealed a very dense and thick morphology for both boride phases. Micro hardness testing of the borided steel samples showed a significant increase in the hardness of the borided surfaces (i.e., up to (1700 +/- 200) HV), while the hardness of un-borided steel samples was approximately (200 +/- 20) HV. Systematic studies over a wide range of boriding time and temperature confirmed that the rate of the boride layer formation is strongly dependent on boriding duration and has a parabolic character. The activation energy of boride layer growth for electrochemical boriding was determined as (172.75 +/- 8.6) kJ/mol. (C) 2011 Elsevier B. V. All rights reserved. C1 [Kartal, G.; Timur, S.] Istanbul Tech Univ, Dept Met & Mat Engn, TR-34469 Istanbul, Turkey. [Eryilmaz, O. L.; Krumdick, G.; Erdemir, A.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. RP Kartal, G (reprint author), Istanbul Tech Univ, Dept Met & Mat Engn, TR-34469 Istanbul, Turkey. EM kartalgu@itu.edu.tr RI Timur, Servet/J-2893-2012 FU U.S. Department of Energy [DE-FG02-07ER46453, DE-FG02-07ER46471] FX The authors would like to thank Prof. Dr. Suheyla Aydin for her helps on the processing of kinetic data. The XRD experiments were carried out in part in the Frederick Seitz Materials Research Laboratory Central Facilities, University of Illinois, which are partially supported by the U.S. Department of Energy under grants DE-FG02-07ER46453 and DE-FG02-07ER46471. NR 37 TC 27 Z9 32 U1 2 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-4332 J9 APPL SURF SCI JI Appl. Surf. Sci. PD MAY 15 PY 2011 VL 257 IS 15 BP 6928 EP 6934 DI 10.1016/j.apsusc.2011.03.034 PG 7 WC Chemistry, Physical; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA 749ZN UT WOS:000289512500097 ER PT J AU Gao, F Yu, KM Mendelsberg, RJ Anders, A Walukiewicz, W AF Gao, F. Yu, K. M. Mendelsberg, R. J. Anders, A. Walukiewicz, W. TI Preparation of high transmittance ZnO:Al film by pulsed filtered cathodic arc technology and rapid thermal annealing SO APPLIED SURFACE SCIENCE LA English DT Article DE ZnO:Al films; Cathodic arc deposition; Rapid thermal annealing; Transmittance; Resistivity ID ZNOAL THIN-FILMS; ZINC-OXIDE FILMS; OPTICAL-PROPERTIES; LASER DEPOSITION; AL AB Approximately 200nm thick ZnO:Al films with high visible and infrared transmittance properties were prepared on glass substrates by the pulsed filtered cathodic arc technique and rapid thermal annealing. The as-deposited and annealed films have a poly-crystalline hexagonal wurtzite type structure. As the annealing temperature increases from 500 degrees C to 650 degrees C, the visible transmittance remains nearly constant (similar to 85%) while the infrared (780-2500 nm) transmittance considerably improves from 22% for the as-deposited film to 58% at 600 degrees C and 71% at 650 degrees C at 2500nm for the annealed films. However, the electrical properties of the films worsen after high-temperature annealing, and resistivity increases from 2.5x10(-4) Omega cm for the as-deposited film to 3.6x10(-3) Omega cm and 1.2x10(-2) Omega cm for the films annealed at 600 and 650 degrees C, respectively. The high-temperature annealing improved the crystallinity and transmittance of the films. Nevertheless, these improvements may lead to the segregation and oxidation of aluminum atoms, as well as the reduction of oxygen vacancies, thereby degrading the electrical properties of the films. (C) 2011 Elsevier B.V. All rights reserved. C1 [Gao, F.] Shaanxi Normal Univ, Coll Phys & Informat Technol, Xian 710062, Peoples R China. [Gao, F.; Yu, K. M.; Mendelsberg, R. J.; Anders, A.; Walukiewicz, W.] Lawrence Berkeley Natl Lab, Berkeley, CA USA. RP Gao, F (reprint author), Shaanxi Normal Univ, Coll Phys & Informat Technol, 199 Changan S Rd, Xian 710062, Peoples R China. EM feigao@snnu.edu.cn RI Yu, Kin Man/J-1399-2012; Anders, Andre/B-8580-2009 OI Yu, Kin Man/0000-0003-1350-9642; Anders, Andre/0000-0002-5313-6505 FU Office of Building Technology; Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering of the U.S. Department of Energy [DE-AC02-05CH11231]; Hong Kong, Natural Science Foundation of China [61040057]; Fundamental Research Funds for the Central Universities of China [GK000902052] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Building Technology, and by the Director of the Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. Fei Gao acknowledges the financial support of Dr. Chongben He from Hong Kong, Natural Science Foundation of China (Grant No. 61040057), and the Fundamental Research Funds for the Central Universities of China (GK000902052). NR 16 TC 5 Z9 6 U1 0 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-4332 J9 APPL SURF SCI JI Appl. Surf. Sci. PD MAY 15 PY 2011 VL 257 IS 15 BP 7019 EP 7022 DI 10.1016/j.apsusc.2011.03.013 PG 4 WC Chemistry, Physical; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA 749ZN UT WOS:000289512500110 ER PT J AU Saillard, M Hall, SR Audin, L Farber, DL Regard, V Herail, G AF Saillard, M. Hall, S. R. Audin, L. Farber, D. L. Regard, V. Herail, G. TI Andean coastal uplift and active tectonics in southern Peru: Be-10 surface exposure dating of differentially uplifted marine terrace sequences (San Juan de Marcona, similar to 15.4 degrees S) SO GEOMORPHOLOGY LA English DT Article DE Marine terrace; 10-Beryllium; CRN dating; Uplift rate; Slip rate; Peru; Nazca Ridge ID SEA-LEVEL CHANGES; NORTHERN CHILE; NAZCA RIDGE; FORE-ARC; CRUSTAL DEFORMATION; HUON-PENINSULA; CARNEGIE RIDGE; ATACAMA DESERT; SUMBA-ISLAND; NEW-ZEALAND AB Along the San Juan de Marcona Bay of southern Peru, two spectacular sequences of preserved marine terraces record net Quaternary uplift. Previous geomorphic analysis of these paleo-shorelines has revealed evidence of upper plate deformation and regional uplift. However, in the absence of a robust absolute dating method, these studies contain substantial uncertainties concerning the numerical dating of these marine markers and thus the corresponding calculated surface uplift rates. However, field mapping, surveying the neotectonic features and Be-10 dating of abraded surfaces contained within two sequences of marine terraces along this margin should allow for the robust calculation of Pleistocene uplift rates. The San Juan de Marcona Bay lies on the southern flank of the subducting and south-migrating aseismic Nazca Ridge where the maximum rates of coastal uplift are expected. In this locality, we measure high uplift rates ranging from 0.4 m/ka to 0.9 m/ka during the Pleistocene. Margin-parallel normal faults displace several marine terraces and influence the development of bays, thereby contributing to the configuration of paleo-and present-day coastlines. The faults have relatively low slip rates, <0.1 m/ka over 400 ka, and have been inactive for the last 80 ka. The presence and activity of these normal faults can be directly linked to subduction zone processes, with the release and accommodation of short-term coseismic compression during megathrust subduction-zone events. In contrast, the regional permanent uplift is probably controlled by post-seismic and/or interseismic strain accumulation over longer time-scales due to inelastic behavior of the upper plate. Since at least the latest Pliocene, the San Juan de Marcona area has experienced long-term regional tectonic uplift that has increased since about 800 ka due to the southward migration of the subducting Nazca Ridge. Based on migration velocity and geometry of the ridge, the influence of the Nazca Ridge on the uplift of the forearc should account for similar to 0.4 m/ka within 145 km south of the ridge axis. Hence, most of the post-400 ka mean uplift rate of the San Juan de Marcona area could be explained by the Nazca Ridge subduction. (C) 2011 Elsevier B.V. All rights reserved. C1 [Saillard, M.; Audin, L.; Regard, V.; Herail, G.] Univ Toulouse, F-31400 Toulouse, France. [Saillard, M.; Audin, L.; Regard, V.; Herail, G.] UPS OMP, F-31400 Toulouse, France. [Saillard, M.; Audin, L.; Regard, V.; Herail, G.] LMTG, F-31400 Toulouse, France. [Saillard, M.; Audin, L.; Regard, V.; Herail, G.] IRD, F-31400 Toulouse, France. [Saillard, M.; Audin, L.; Regard, V.; Herail, G.] CNRS, F-31400 Toulouse, France. [Hall, S. R.; Farber, D. L.] Univ Calif Santa Cruz, Dept Earth Sci, Santa Cruz, CA 95060 USA. [Farber, D. L.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Saillard, M (reprint author), Univ Toulouse, 14 Av Edouard Belin, F-31400 Toulouse, France. EM saillard@lmtg.obs-mip.fr RI Farber, Daniel/F-9237-2011; Regard, Vincent/B-2585-2010; laurence, audin/D-7727-2013 OI Regard, Vincent/0000-0002-5250-6068; laurence, audin/0000-0002-4510-479X FU NSF [0345895] FX This research project thanks the Institut de Recherche pour le Developpement (IRD), NSF EAR grant 0345895 and IGPP-LLNL. Special thanks to Jose Machare and INGEMMET (Lima, Peru) for their support in this study. We thank the three anonymous reviewers for the work they did to considerably improve the manuscript. NR 83 TC 23 Z9 23 U1 0 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-555X EI 1872-695X J9 GEOMORPHOLOGY JI Geomorphology PD MAY 15 PY 2011 VL 128 IS 3-4 BP 178 EP 190 DI 10.1016/j.geomorph.2011.01.004 PG 13 WC Geography, Physical; Geosciences, Multidisciplinary SC Physical Geography; Geology GA 747SC UT WOS:000289338700006 ER PT J AU van der List, PIM Oldenbroek, SJL Lugthart, EN van Albada, GA Gamez, P Haasnoot, JG Teat, SJ Roubeau, O Mutikainen, I Reedijk, J AF van der List, Peerke I. M. Oldenbroek, Sebastien J. -L. Lugthart, Elza N. van Albada, Gerard A. Gamez, Patrick Haasnoot, Jaap G. Teat, Simon J. Roubeau, Olivier Mutikainen, Ilpo Reedijk, Jan TI Coordination network solids based on Cu(II) coordination compounds with 1,4-bis-(1,2,4-triazol-1-yl)-butane as a flexible alkyl spacer ligand: Synthesis, characterization and X-ray structures SO INORGANICA CHIMICA ACTA LA English DT Article DE Copper(II); Flexible spacer; Crystal structure; Framework; Coordination polymers ID BRIDGED COPPER(II) COMPOUNDS; CRYSTAL-STRUCTURES; BIS(2-BENZIMIDAZOLYL)ALKANE LIGANDS; SPECTROSCOPIC PROPERTIES; MAGNETIC-PROPERTIES; TRIAZOLE LIGAND; SQUARE-PLANAR; COMPLEXES; POLYMERS; ANION AB The coordination chemistry of three selected copper(II) salts with the flexible ligand 1,4-bis(1,2,4-triazol-1-yl) butane (abbreviated as btb) is described. This ligand acts as a bidentate ligand, bridging copper(II) ions, thereby generating polymers in 2D and 3D network solids. (C) 2011 Elsevier B.V. All rights reserved. C1 [van der List, Peerke I. M.; Oldenbroek, Sebastien J. -L.; Lugthart, Elza N.; van Albada, Gerard A.; Gamez, Patrick; Haasnoot, Jaap G.; Reedijk, Jan] Leiden Univ, Leiden Inst Chem, NL-2300 RA Leiden, Netherlands. [Teat, Simon J.] Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. [Gamez, Patrick] Univ Barcelona, Dept Quim Inorgan, ICREA, E-08028 Barcelona, Spain. [Roubeau, Olivier] CSIC, Inst Ciencia Mat Aragon, E-50009 Zaragoza, Spain. [Roubeau, Olivier] Univ Zaragoza, E-50009 Zaragoza, Spain. [Mutikainen, Ilpo] Univ Helsinki, Dept Chem, Inorgan Chem Lab, Helsinki 00014, Finland. [Reedijk, Jan] King Saud Univ, Dept Chem, Riyadh 11451, Saudi Arabia. RP Reedijk, J (reprint author), Leiden Univ, Leiden Inst Chem, POB 9502, NL-2300 RA Leiden, Netherlands. EM reedijk@chem.leidenuniv.nl RI Reedijk, Jan/F-1992-2010; Gamez, Patrick/B-3610-2012; Roubeau, Olivier/A-6839-2010 OI Reedijk, Jan/0000-0002-6739-8514; Gamez, Patrick/0000-0003-2602-9525; Roubeau, Olivier/0000-0003-2095-5843 FU Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX This work was performed in the framework of the freshmen students research project "Leren Onderzoeken 1" (Learning Research 1) in the B.Sc programme "Molecular Science and Technology", a recently started concept in the joint Academic programme of Delft University of Technology and Leiden University. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 42 TC 2 Z9 2 U1 3 U2 12 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0020-1693 J9 INORG CHIM ACTA JI Inorg. Chim. Acta PD MAY 15 PY 2011 VL 370 IS 1 BP 164 EP 169 DI 10.1016/j.ica.2011.01.052 PG 6 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 750NX UT WOS:000289556300023 ER PT J AU Klaehn, JR Peterman, DR Harrup, MK Luther, TA Daniels, LM AF Klaehn, John R. Peterman, Dean R. Harrup, Mason K. Luther, Thomas A. Daniels, Lee M. TI Bis(o-trifluoromethylphenyl)dithiophosphinic methyl ester SO INORGANICA CHIMICA ACTA LA English DT Article DE Synthesis; Characterization; Dithiophosphinic acid; Dithiophosphinic ester; X-ray crystal determination ID SUBSTITUTED DITHIOPHOSPHINIC ACIDS; SECONDARY PHOSPHINE OXIDES; BINARY EXTRACTANT SYSTEMS; METAL-COMPLEXES; COBALT/NICKEL RECOVERY; TRIVALENT ACTINIDES; SOLVENT-EXTRACTION; SEPARATION; CYANEX-301; LANTHANIDES AB When bis(o-trifluoromethylphenyl) dithiophosphinic acid (1) is dissolved in methanol, crystals of bis(o-trifluoromethylphenyl) dithiophosphinic methyl ester (2) are formed. The structure of dithiophosphinic methyl ester (2) has been characterized via single-crystal X-ray diffraction and multinuclear NMR studies. Compound 2 is remarkable in that the dithiophosphinic (PS(2)) core is preserved during this transformation. The transformation to 2 suggests that the o-trifluoromethylphenyl groups on phosphorus assist in retaining the PS(2) core, possibly by steric hindrance. Published by Elsevier B. V. C1 [Klaehn, John R.; Peterman, Dean R.; Harrup, Mason K.; Luther, Thomas A.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Daniels, Lee M.] Rigaku Amer Corp, The Woodlands, TX 77381 USA. RP Klaehn, JR (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM john.klaehn@inl.gov RI Klaehn, John/C-6011-2017 OI Klaehn, John/0000-0002-7077-4509 FU United States Department of Energy and the Laboratory Directed Research and Development (LDRD) at the Idaho National Laboratory (INL) [DE-AC07-05ID14517] FX This work was supported by the United States Department of Energy and the Laboratory Directed Research and Development (LDRD) program at the Idaho National Laboratory (INL) through contract DE-AC07-05ID14517. NR 37 TC 2 Z9 2 U1 0 U2 7 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0020-1693 J9 INORG CHIM ACTA JI Inorg. Chim. Acta PD MAY 15 PY 2011 VL 370 IS 1 BP 519 EP 522 DI 10.1016/j.ica.2011.01.023 PG 4 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 750NX UT WOS:000289556300075 ER PT J AU Tonks, M Millett, P AF Tonks, Michael Millett, Paul TI Phase field simulations of elastic deformation-driven grain growth in 2D copper polycrystals SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Grain boundary migration; Elastic deformation; Phase field model ID COMPUTER-SIMULATION; BOUNDARY MIGRATION; DYNAMICS; MODEL AB In this work, a phase field grain growth model coupled with a spectral stress calculation method is used to investigate the effect of applied elastic deformation on grain growth in 2D copper polycrystals with isotropic grain boundary properties. The applied deformation accelerates the grain growth compared to a relaxed polycrystal, though the effect of the deformation decreases rapidly with time. The softest grain orientations with respect to the applied deformation grow at the expense of other orientations, though they have higher elastic energy density. Due to a rapid decrease in the elastic energy stored in the system, the GB energy eventually dominates the growth leading to a linear change in the average grain area with time. Increasing the magnitude of the applied deformation accelerates the growth, while increasing the temperature accelerates the growth but decreases the effect of the applied deformation. Published by Elsevier B.V. C1 [Tonks, Michael; Millett, Paul] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Tonks, M (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM Michael.Tonks@inl.gov FU US Department of Energy, Office of Nuclear Energy; Battelle Energy Alliance, LLC with the US Department of Energy [DE-AC07-051D14517, INL/JOU-10-20202] FX The authors wish to thank Dieter Wolf of Argonne National Labaratory for his guidance during the initial stages of this work and Bulent Bluer of Idaho National Laboratory for his suggestions on grain growth conditions. This work was supported by the US Department of Energy, Office of Nuclear Energy, Advanced Modeling and Simulation program. This manuscript has been authored by Battelle Energy Alliance, LLC under Contract No. DE-AC07-051D14517 with the US Department of Energy (INL/JOU-10-20202). NR 15 TC 8 Z9 9 U1 3 U2 13 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD MAY 15 PY 2011 VL 528 IS 12 BP 4086 EP 4091 DI 10.1016/j.msea.2011.02.007 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA 748KL UT WOS:000289389400019 ER PT J AU Zhu, HY Dong, L Chen, Y AF Zhu, Haiyang Dong, Lin Chen, Yi TI Effect of titania structure on the properties of its supported copper oxide catalysts SO JOURNAL OF COLLOID AND INTERFACE SCIENCE LA English DT Article DE Copper oxide; Anatase; Rutile; Surface interaction; Surface structure ID MOLYBDENUM HYDRODESULFURIZATION CATALYSTS; CE0.5ZR0.5O2 SOLID-SOLUTION; O-XYLENE; SELECTIVE OXIDATION; PHTHALIC-ANHYDRIDE; VANADIUM-OXIDE; LIQUID-PHASE; ANATASE; REDUCTION; SURFACE AB Anatase and rutile have the same chemical composition as TiO(2) but different crystalline structures (space group of D(4h)(19) - l4(1) for anatase and D(4h)(14) - P4(2) for rutile, respectively), which result in different surface structures and can be used ideally to investigate the effects of support and surface structure on the properties of their supported catalysts. In this work, anatase- or rutile-supported copper oxide catalysts (signed as Cu-A and Cu-R, thereafter) prepared by the impregnation method were characterized by X-ray diffraction (XRD), Brunauer-Emmett-Teller (BET) surface area, X-ray photoelectron spectroscopy (XPS), and H(2) temperature-programmed reduction (H(2)-TPR) to study the support effect of titania on the physicochemical properties and catalytic properties for the NO reduction by CO of these supported copper oxide catalysts. The results indicated that (1) copper oxide presented different dispersion capacities on anatase or rutile; (2) dispersed copper oxide species on anatase and rutile also showed different reduction behaviors; i.e., one-step reduction for dispersed copper oxide species in Cu-A and stepwise reduction for that in Cu-R; (3) the NO + CO activity test suggested dispersed copper oxide and small CuO particles on rutile are the main active species under the current reaction conditions and copper oxide supported on rutile is more active than that on anatase, which might result from Cu(+) species in Cu-R sample formed during the reaction due to its stepwise reduction behavior. (C) 2011 Elsevier Inc. All rights reserved. C1 [Zhu, Haiyang; Dong, Lin; Chen, Yi] Nanjing Univ, Sch Chem & Chem Engn, Key Lab Mesoscop Chem MOE, Nanjing 210093, Peoples R China. RP Zhu, HY (reprint author), Pacific NW Natl Lab, Inst Interfacial Catalysis, POB 999,MSIN K8-87, Richland, WA 99352 USA. EM haiyangz79@gmail.com; donglin@nju.edu.cn RI Dong, Lin/N-6988-2014 FU National Natural Science Foundation of China [20873060, 20973091]; National 973 Program of China [2010CB732300] FX The financial support of the National Natural Science Foundation of China (Nos. 20873060, 20973091) and the National 973 Program of China (No. 2010CB732300) is gratefully acknowledged. NR 47 TC 16 Z9 16 U1 1 U2 13 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9797 J9 J COLLOID INTERF SCI JI J. Colloid Interface Sci. PD MAY 15 PY 2011 VL 357 IS 2 BP 497 EP 503 DI 10.1016/j.jcis.2011.02.012 PG 7 WC Chemistry, Physical SC Chemistry GA 745QA UT WOS:000289179500033 PM 21392779 ER PT J AU Chick, LA Meinhardt, KD Simner, SP Kirby, BW Powell, MR Canfield, NL AF Chick, Larry A. Meinhardt, Kerry D. Simner, Steve P. Kirby, Brent W. Powell, Mike R. Canfield, Nathan L. TI Factors affecting limiting current in solid oxide fuel cells or debunking the myth of anode diffusion polarization SO JOURNAL OF POWER SOURCES LA English DT Article DE Solid oxide fuel cell; Limiting current; Diffusion polarization; Concentration polarization; Tortuosity; Button cell ID SOFC ANODES; PERFORMANCE; IMPEDANCE; RECONSTRUCTION; MODEL AB Limiting current densities for solid oxide fuel cells were measured using both button cells and a flow-through cell. The cell anodes were supplied with mixtures of humidified hydrogen and various inert gasses. It was demonstrated that the true limiting current in flow-through cells is reached when either: the hydrogen is nearly or completely depleted at the anode-electrolyte interface near the outlet: or when the concentration of steam at that interface becomes high enough to interfere with adsorption or transport of the remaining hydrogen near the triple-phase boundaries. Choice of inert gas had no effect on limiting currents in the flow-through tests, indicating that diffusion within the porous anode had no significant effect on cell performance at high currents. In the button cells, the apparent limiting currents were significantly changed by the choice of inert gas, indicating that they were determined by diffusion through the bulk gas within the support tube. It was concluded that the apparent limiting currents measured in button cells are influenced more by parameters of the experimental setup, such as the proximity of the fuel tube outlet, than by the physical properties of the anode. (C) 2011 Elsevier B.V. All rights reserved. C1 [Chick, Larry A.; Meinhardt, Kerry D.; Simner, Steve P.; Kirby, Brent W.; Powell, Mike R.; Canfield, Nathan L.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Simner, Steve P.] Savannah River Remediat LLC, Aiken, SC 29808 USA. RP Chick, LA (reprint author), Pacific NW Natl Lab, 904 Battelle Blvd, Richland, WA 99352 USA. EM larry.chick@pnl.gov NR 20 TC 8 Z9 8 U1 1 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 J9 J POWER SOURCES JI J. Power Sources PD MAY 15 PY 2011 VL 196 IS 10 SI SI BP 4475 EP 4482 DI 10.1016/j.jpowsour.2011.01.035 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 745AR UT WOS:000289136800007 ER PT J AU Abernathy, H Gemmen, R Gerdes, K Koslowske, M Tao, T AF Abernathy, Harry Gemmen, Randall Gerdes, Kirk Koslowske, Mark Tao, Thomas TI Basic properties of a liquid tin anode solid oxide fuel cell SO JOURNAL OF POWER SOURCES LA English DT Article DE Solid oxide fuel cell; Oxygen diffusion; Tin; Liquid metal anode; Direct coal fuel cell ID OXYGEN; METALS; DIFFUSIVITY; SOLUBILITY; SN; PRESSURE; HYDROGEN; ALLOYS AB An unconventional high temperature fuel cell system, the liquid tin anode solid oxide fuel cell (LTA-SOFC), is discussed. A thermodynamic analysis of a solid oxide fuel cell with a liquid metal anode is developed. Pertinent thermochemical and thermophysical properties of liquid tin in particular are detailed. An experimental setup for analysis of LTA-SOFC anode kinetics is described, and data for a planar cell under hydrogen indicated an effective oxygen diffusion coefficient of 5.3 x 10(-5) cm(2) s(-1) at 800 degrees C and 8.9 x 10(-5) cm(2) s(-1) 900 degrees C. This value is similar to previously reported literature values for liquid tin. The oxygen conductivity through the tin, calculated from measured diffusion coefficients and theoretical oxygen solubility limits, is found to be on the same order of that of yttria-stabilized zirconia (YSZ), a traditional SOFC electrolyte material. As such, the ohmic loss due to oxygen transport through the tin layer must be considered in practical system cell design since the tin layer will usually be at least as thick as the electrolyte. (C) 2011 Elsevier B.V. All rights reserved. C1 [Abernathy, Harry; Gemmen, Randall; Gerdes, Kirk] Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Koslowske, Mark; Tao, Thomas] CellTech Power LLC, Westborough, MA 01581 USA. RP Abernathy, H (reprint author), Natl Energy Technol Lab, 3610 Collins Ferry Rd,POB 880, Morgantown, WV 26507 USA. EM Harry.Abernathy@netl.doe.gov NR 45 TC 28 Z9 29 U1 2 U2 27 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 J9 J POWER SOURCES JI J. Power Sources PD MAY 15 PY 2011 VL 196 IS 10 SI SI BP 4564 EP 4572 DI 10.1016/j.jpowsour.2010.12.089 PG 9 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 745AR UT WOS:000289136800017 ER PT J AU Ahluwalia, RK Wang, X Kwon, J Rousseau, A Kalinoski, J James, B Marcinkoski, J AF Ahluwalia, R. K. Wang, X. Kwon, J. Rousseau, A. Kalinoski, J. James, B. Marcinkoski, J. TI Performance and cost of automotive fuel cell systems with ultra-low platinum loadings SO JOURNAL OF POWER SOURCES LA English DT Article DE Polymer electrolyte fuel cells; Automotive fuel cell stacks; Electrocatalysts; Air management; Heat rejection; Cost and performance ID VEHICLES; ECONOMY; STACKS AB Anautomotive polymer-electrolyte fuel cell (PEFC) system with ultra-low platinum loading (0.15 mg-Pt cm(-2)) has been analyzed to determine the relationship between its design-point efficiency and the system efficiency at part loads, efficiency over drive cycles, stack and system costs, and heat rejection. The membrane electrode assemblies in the reference PEFC stack use nanostructured, thin-film ternary catalysts supported on organic whiskers and a modified perfluorosulfonic acid membrane. The analyses show that the stack Pt content can be reduced by 50% and the projected high-volume manufacturing cost by >45% for the stack and by 25% for the system, if the design-point system efficiency is lowered from 50% to 40%. The resulting penalties in performance are a <1% reduction in the system peak efficiency; a 2-4% decrease in the system efficiency on the urban, highway, and LA92 drive cycles: and a 6.3% decrease in the fuel economy of the modeled hybrid fuel-cell vehicle on the combined cycle used by EPA for emission and fuel economy certification. The stack heat load, however, increases by 50% at full power (80 kW(e)) but by only 23% at the continuous power (61.5 kW(e)) needed to propel the vehicle on a 6.5% grade at 55 mph. The reduced platinum and system cost advantages of further lowering the design-point efficiency from 40% to 35% are marginal. The analyses indicate that thermal management in the lower efficiency systems is very challenging and that the radiator becomes bulky if the stack temperature cannot be allowed to increase to 90-95 degrees C under driving conditions where heat rejection is difficult. (C) 2011 Elsevier B.V. All rights reserved. C1 [Ahluwalia, R. K.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Kalinoski, J.; James, B.] Directed Technol Inc, Arlington, VA USA. [Marcinkoski, J.] US DOE, Washington, DC USA. RP Ahluwalia, RK (reprint author), Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM walia@anl.gov FU U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy FX This work was supported by the Fuel Cell Technologies Program of the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy. NR 21 TC 22 Z9 22 U1 1 U2 26 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 J9 J POWER SOURCES JI J. Power Sources PD MAY 15 PY 2011 VL 196 IS 10 SI SI BP 4619 EP 4630 DI 10.1016/j.jpowsour.2011.01.059 PG 12 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 745AR UT WOS:000289136800027 ER PT J AU Jung, K Kim, CS Pettit, FS Meier, GH AF Jung, Keeyoung Kim, Chang-Soo Pettit, Frederick S. Meier, Gerald H. TI Interfacial failure via encapsulation of external particulates in an outward-growing thermal oxide SO JOURNAL OF POWER SOURCES LA English DT Article DE Syngas; Oxidation; Chromia former; Buckling; Numerical analysis; Finite element analysis ID NI-BASE SUPERALLOY; BARRIER COATINGS; CYCLIC OXIDATION; DEPOSITS; MECHANISMS; SPALLATION; SCALES; DELAMINATION; TEMPERATURE; CORROSION AB A Cr2O3-forming Ni-base superalloy and this alloy coated with a Pt-modified aluminide coating were exposed to SiO2 powder and cyclically oxidized at 950 degrees C. The uncoated alloy showed a considerable amount of spallation and buckling whereas the Pt-NiAl coated alloy remained protective throughout hundred 1 h-cycles. The interfacial failure is mainly ascribed to the increased thermal strain by the encapsulation of external SiO2 particulates in an outward-growing Cr2O3 layer. However, the particles were not embedded in the thermally grown oxide of the Pt-NiAl coated alloy due to the slow inward-growing characteristics of Al2O3 scales. The buckling of the Cr2O3 scale with embedded SiO2 was analyzed with (1) a classical buckling criterion using the instantaneous coefficients of thermal expansion of the constituents. and (2) finite element analyses (FEA) to estimate the local interfacial shear stresses. It turns out that the thermal strain with embedded SiO2 is larger than the experimentally determined critical thermal strain (epsilon(b))explaining the buckling of the oxide scale observed in the experiment. The FEA results demonstrate that local shear stresses at the metal/oxide interface are significantly amplified near the SiO2 particles showing that the buckling of oxide can be readily initiated especially in the vicinity of the embedded particles. (C) 2011 Elsevier B.V. All rights reserved. C1 [Jung, Keeyoung; Pettit, Frederick S.; Meier, Gerald H.] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Jung, Keeyoung; Pettit, Frederick S.; Meier, Gerald H.] Univ Pittsburgh, Dept Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA. [Kim, Chang-Soo] Univ Wisconsin, Dept Mat, Milwaukee, WI 53211 USA. RP Jung, K (reprint author), Natl Energy Technol Lab, 626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA. EM jung.keeyoung@gmail.com FU U.S. DOE; National Energy Technology Laboratory (NETL) [04-01-SR-116, DE-FE0004000]; college of engineering and applied science FX This work at the University of Pittsburgh was performed in support of the U.S. DOE and the National Energy Technology Laboratory (NETL) under the UTSR subcontract 04-01-SR-116 and the RES contract DE-FE0004000, respectively. The work performed at the University of Wisconsin at Milwaukee was supported by the start-up fund from the college of engineering and applied science for C.-S. Kim. The authors gratefully acknowledge GE Energy for providing specimens. NR 35 TC 3 Z9 3 U1 0 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 J9 J POWER SOURCES JI J. Power Sources PD MAY 15 PY 2011 VL 196 IS 10 SI SI BP 4686 EP 4694 DI 10.1016/j.jpowsour.2010.12.104 PG 9 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 745AR UT WOS:000289136800034 ER PT J AU Nelson, GJ Peracchio, AA Chiu, WKS AF Nelson, George J. Peracchio, Aldo A. Chiu, Wilson K. S. TI Analytical investigations of varying cross section microstructures on charge transfer in solid oxide fuel cell electrodes SO JOURNAL OF POWER SOURCES LA English DT Article DE Solid oxide fuel cell; Heterogeneous functional materials; Transport phenomena; Electrode microstructure ID MONTE-CARLO SIMULATIONS; COMPOSITE ELECTRODES; SOFC ELECTRODES; INTERMEDIATE TEMPERATURE; AIR CATHODES; ANODE; POLARIZATION; PERFORMANCE; RECONSTRUCTION; CONDUCTIVITY AB An extended surface modeling concept (electrochemical fin) is applied to charge transport within the SOFC electrode microstructure using an analytical modeling approach analogous to thermal fin analysis. This model is distinct from similar approaches applied to SOFC electrode microstructure in its application of a governing equation that allows for variable cross-section geometry. The model presented is capable of replicating experimentally observed electrode behavior inclusive of sensitivity to microstructural geometry, which stands in contrast to existing models that apply governing equations analogous to a constant cross-section thermal fin equation. Insights learned from this study include: the establishment of a suite of dimensionless parameters and performance metrics that can be applied to assess electrode microstructure, the definition of microstructure-related transport regimes relevant to electrode design, and correlations that allow performance predictions for electrodes that provide cell structural support. Of particular note, the variable cross-section modeling approach motivates the definition of a sintering quality parameter that quantifies the degree of constriction within the conducting network of the electrode, a phenomenon that exerts influence over electrode polarization. One-dimensional models are presented for electrochemical fins of several cross-sectional geometries with the ultimate goal of developing a general tool that enables the prompt performance evaluation of electrode microstructures. Such a tool would facilitate SOFC microstructural design by focusing more detailed modeling efforts on the most promising microstructures. (C) 2011 Elsevier B.V. All rights reserved. C1 [Nelson, George J.; Peracchio, Aldo A.; Chiu, Wilson K. S.] Univ Connecticut, Dept Mech Engn, HeteroFoaM Ctr, DOE Energy Frontier Res Ctr, Storrs, CT 06269 USA. RP Chiu, WKS (reprint author), Univ Connecticut, Dept Mech Engn, HeteroFoaM Ctr, DOE Energy Frontier Res Ctr, 191 Auditorium Rd,Unit 3139, Storrs, CT 06269 USA. EM wchiu@engr.uconn.edu FU U.S. Department of Energy, Office of Science. Office of Basic Energy Sciences [DE-SC0001061] FX Financial support from an Energy Frontier Research Center on Science Based Nano-Structure Design and Synthesis of Heterogeneous Functional Materials for Energy Systems (HeteroFoaM Center) funded by the U.S. Department of Energy, Office of Science. Office of Basic Energy Sciences (Award DE-SC0001061) is gratefully acknowledged. The authors are grateful to Prof. Anil V. Virkar at the University of Utah and Prof. Brice N. Cassenti at the University of Connecticut for invaluable discussions on SOFC microstructure and analytical solution methods, respectively. NR 25 TC 22 Z9 22 U1 1 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 J9 J POWER SOURCES JI J. Power Sources PD MAY 15 PY 2011 VL 196 IS 10 SI SI BP 4695 EP 4704 DI 10.1016/j.jpowsour.2010.12.103 PG 10 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 745AR UT WOS:000289136800035 ER PT J AU Cunsolo, A Leu, BM Said, AH Cai, YQ AF Cunsolo, A. Leu, B. M. Said, A. H. Cai, Y. Q. TI Structural and microscopic relaxations in glycerol: An inelastic x-ray scattering study SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID GLASS-FORMING LIQUIDS; BRILLOUIN-SCATTERING; DYNAMICS; TRANSITION; PRESSURE; BEHAVIOR; SYSTEMS; WATER AB The THz dynamics of liquid glycerol has been probed by inelastic x-ray scattering at different pressure spanning the 0.66-3 Kbar range. A comparison with ultrasound absorption results available in literature leads us to identify the presence of two different relaxations, a structural (slow) relaxation and a microscopic (fast) one. Although the former has been already thoroughly studied in glycerol by lower frequency spectroscopic techniques, no hints on the latter are so far available in literature. We observe that the characteristic timescale of this fast relaxation ranges in the sub-picosecond, tends to decrease with increasing the wave-vector and seems rather insensitive to pressure changes. Finally, the timescale and strength of the fast relaxation have a direct link revealing the microscopic, single particle, nature of the involved process. (C) 2011 American Institute of Physics. [doi:10.1063/1.3587104] C1 [Cunsolo, A.; Cai, Y. Q.] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Leu, B. M.; Said, A. H.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Cunsolo, A (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source 2, POB 5000, Upton, NY 11973 USA. EM acunsolo@bnl.gov RI Cunsolo, Alessandro/C-7617-2013; Cai, Yong/C-5036-2008 OI Cai, Yong/0000-0002-9957-6426 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; NSF [DMR-0115852] FX The authors feel indebted to the Advanced Photon Source for granting beam-time for the experiment and to T. Roberts for his valuable help in the setup of HP assembly. The use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The construction of HERIX was partially supported by the NSF under Grant No. DMR-0115852. NR 34 TC 5 Z9 5 U1 0 U2 8 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 14 PY 2011 VL 134 IS 18 AR 184502 DI 10.1063/1.3587104 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 763WH UT WOS:000290589900026 PM 21568516 ER PT J AU Harmon, ME Bond-Lamberty, B Tang, JW Vargas, R AF Harmon, Mark E. Bond-Lamberty, Ben Tang, Jianwu Vargas, Rodrigo TI Heterotrophic respiration in disturbed forests: A review with examples from North America SO JOURNAL OF GEOPHYSICAL RESEARCH-BIOGEOSCIENCES LA English DT Review ID COARSE WOODY DEBRIS; SOIL ORGANIC-MATTER; NET PRIMARY PRODUCTION; BLACK SPRUCE CHRONOSEQUENCE; LEAF-LITTER DECOMPOSITION; CARBON-DIOXIDE FLUX; OLD-GROWTH FORESTS; LONG-TERM CARBON; TEMPERATURE SENSITIVITY; CLIMATE-CHANGE AB Heterotrophic respiration (R-H) is a major process releasing carbon to the atmosphere and is essential to understanding carbon dynamics in terrestrial ecosystems. Here we review what is known about this flux as related to forest disturbance using examples from North America. The global R-H flux from soils has been estimated at 53-57 Pg C yr(-1), but this does not include contributions from other sources (i.e., dead wood, heart-rots). Disturbance-related inputs likely account for 20-50% of all R-H losses in forests, and disturbances lead to a reorganization of ecosystem carbon pools that influences how RH changes over succession. Multiple controls on R-H related to climate, the material being decomposed, and the decomposers involved have been identified, but how each potentially interacts with disturbance remains an open question. An emerging paradigm of carbon dynamics suggests the possibility of multiple periods of carbon sinks and sources following disturbance; a large contributing factor is the possibility that postdisturbance R-H does not always follow the monotonic decline assumed in the classic theory. Without a better understanding and modeling of R-H and its controlling factors, it will be difficult to estimate, forecast, understand, and manage carbon balances of regions in which disturbance frequency and severity are changing. Meeting this challenge will require (1) improved field data on processes and stores, (2) an improved understanding of the physiological and environmental controls of R-H, and (3) a more formal analysis of how model structure influences the R-H responses that can be predicted. C1 [Harmon, Mark E.] Oregon State Univ, Dept Forest Ecosyst & Soc, Corvallis, OR 97331 USA. [Tang, Jianwu] Marine Biol Lab, Ecosyst Ctr, Woods Hole, MA 02543 USA. [Vargas, Rodrigo] Ctr Invest Cient & Educ Super Ensenada, Dept Biol Conservac, Ensenada 22860, Baja California, Mexico. [Bond-Lamberty, Ben] Univ Maryland, Joint Global Change Res Inst, Pacific NW Natl Lab, College Pk, MD 20740 USA. RP Harmon, ME (reprint author), Oregon State Univ, Dept Forest Ecosyst & Soc, Corvallis, OR 97331 USA. EM mark.harmon@oregonstate.edu; bondlamberty@pnl.gov; jtang@mbl.edu; rvargas@cicese.mx RI Bond-Lamberty, Ben/C-6058-2008; Tang, Jianwu/K-6798-2014; Vargas, Rodrigo/C-4720-2008 OI Bond-Lamberty, Ben/0000-0001-9525-4633; Tang, Jianwu/0000-0003-2498-9012; Vargas, Rodrigo/0000-0001-6829-5333 FU U.S. Geologic Survey; Kaye and Ward Richardson Endowment FX This manuscript was a product of the Disturbance Working Group of the North American Carbon Program. Support was provided by the U.S. Geologic Survey and the Kaye and Ward Richardson Endowment. NR 150 TC 48 Z9 49 U1 8 U2 79 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-8953 EI 2169-8961 J9 J GEOPHYS RES-BIOGEO JI J. Geophys. Res.-Biogeosci. PD MAY 14 PY 2011 VL 116 AR G00K04 DI 10.1029/2010JG001495 PG 17 WC Environmental Sciences; Geosciences, Multidisciplinary SC Environmental Sciences & Ecology; Geology GA 764HY UT WOS:000290621700001 ER PT J AU Hunke, EC Comeau, D AF Hunke, Elizabeth C. Comeau, Darin TI Sea ice and iceberg dynamic interaction SO JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS LA English DT Article ID SOUTHERN-OCEAN; ROSS SEA; MODEL; DRIFT; ANTARCTICA; THICKNESS; CLIMATE; WINDS AB A model of iceberg motion has been implemented in the Los Alamos sea ice model (CICE). Individual bergs are tracked under the influence of winds, currents, sea surface tilt, Coriolis, and sea ice forcing. In turn, sea ice is affected by the presence of icebergs, primarily as obstacles that cause the sea ice to ridge on the upstream side or create open water on the downstream side of the bergs. Open water formed near icebergs due to sea ice ridging and blocking of sea ice advection increases level and ridged ice downstream of the bergs through increased frazil ice formation. Resulting anomalies in sea ice area and thickness (compared with a simulation without icebergs) are transported with the sea ice flow, expanding over time. Although local changes in the sea ice distribution may be important for smaller-scale studies, these anomalies are small compared with the total volume of sea ice and their effect on climate-scale variables appears to be insignificant. C1 [Hunke, Elizabeth C.] Los Alamos Natl Lab, Div Theoret, Fluid Dynam & Solid Mech Grp, Los Alamos, NM 87545 USA. [Comeau, Darin] Univ Arizona, Program Appl Math, Tucson, AZ 85721 USA. RP Hunke, EC (reprint author), Los Alamos Natl Lab, Div Theoret, Fluid Dynam & Solid Mech Grp, MS B216, Los Alamos, NM 87545 USA. EM eclare@lanl.gov FU Biological and Environmental Research Division of the U.S. Department of Energy Office of Science; U.S. Department of Energy [DE-AC52-06NA25396] FX This work was performed within the Climate, Ocean and Sea Ice Modeling (COSIM) project at Los Alamos National Laboratory, whose funding from the Biological and Environmental Research Division of the U.S. Department of Energy Office of Science is gratefully acknowledged. Marika Holland and David Bailey graciously provided the NCAR CCSM3 ocean forcing data set, and we thank Todd Arbetter of the National Ice Center for providing observed iceberg positions. Los Alamos National Laboratory is operated by the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. NR 31 TC 6 Z9 6 U1 1 U2 8 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0148-0227 J9 J GEOPHYS RES-OCEANS JI J. Geophys. Res.-Oceans PD MAY 14 PY 2011 VL 116 AR C05008 DI 10.1029/2010JC006588 PG 9 WC Oceanography SC Oceanography GA 764JB UT WOS:000290624600003 ER PT J AU Vaidya, NK Wu, JH AF Vaidya, Naveen K. Wu, Jianhong TI HIV epidemic in Far-Western Nepal: effect of seasonal labor migration to India SO BMC PUBLIC HEALTH LA English DT Article ID HUMAN-IMMUNODEFICIENCY-VIRUS; COST-EFFECTIVENESS; HIV/AIDS EPIDEMIC; TRANSMISSION; INFECTION; SPREAD; MODELS; POPULATION; MIGRANTS; DISEASE AB Background: Because of limited work opportunities in Nepal and the open-border provision between Nepal and India, a seasonal labor migration of males from Far-Western Nepal to India is common. Unsafe sexual activities of these migrants in India, such as frequent visits to brothels, lead to a high HIV prevalence among them and to a potential transmission upon their return home to Nepal. The present study aims to evaluate the role of such seasonal labor-migration to India on HIV transmission in Far-Western Nepal and to assess prevention programs. Methods: An HIV epidemic model was developed for a population in Far-Western Nepal. The model was fitted to the data to estimate the back and forth mobility rates of labor-migrants to India, the HIV prevalence among migrants and the HIV transmission rate in Far-Western Nepal. HIV prevalence, new infections, disease deaths and HIV infections recruited from India were calculated. Prevention programs targeting the general population and the migrants were evaluated. Results: Without any intervention programs, Far-Western Nepal will have about 7,000 HIV infected individuals returning from India by 2015, and 12,000 labor-migrants living with HIV in India. An increase of condom use among the general population from 39% to 80% will reduce new HIV infections due to sexual activity in Far-Western Nepal from 239 to 77. However, such a program loses its effectiveness due to the recruitment of HIV infections via returning migrants from India. The reduction of prevalence among migrants from 2.2% to 1.1% can bring general prevalence down to 0.4% with only 3,500 recruitments of HIV infections from India. Conclusion: Recruitment of HIV infections from India via seasonal labor-migrants is the key factor contributing to the HIV epidemic in Far-Western Nepal. Prevention programs focused on the general population are ineffective. Our finding highlights the urgency of developing prevention programs which reduce the prevalence of HIV among migrants for a successful control of the HIV epidemic in Far-Western Nepal. C1 [Wu, Jianhong] York Univ, Dept Math & Stat, Ctr Dis Modeling, Toronto, ON M3J 2R7, Canada. [Vaidya, Naveen K.] Univ Western Ontario, Dept Appl Math, London, ON N6A 5B9, Canada. [Vaidya, Naveen K.] Los Alamos Natl Lab, Theoret Biol & Biophys Grp, Los Alamos, NM USA. RP Wu, JH (reprint author), York Univ, Dept Math & Stat, Ctr Dis Modeling, Toronto, ON M3J 2R7, Canada. EM wujh@yorku.ca FU York University, Canada; Los Alamos National Laboratory, USA; Canada Research Chair Program; Natural Sciences and Engineering Research Council of Canada; Mathematics for Information Technology and Complex Systems FX This work began when NKV was at York University. The work of NKV has been partially supported by Susan Mann Scholarship Award of York University, Canada and Postdoctoral Research Program at Los Alamos National Laboratory, USA. The work of JW has been supported in part by The Canada Research Chair Program, by Natural Sciences and Engineering Research Council of Canada, and by Mathematics for Information Technology and Complex Systems. Authors would like to thank the reviewers for useful comments. NR 44 TC 7 Z9 7 U1 0 U2 1 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2458 J9 BMC PUBLIC HEALTH JI BMC Public Health PD MAY 13 PY 2011 VL 11 AR 310 DI 10.1186/1471-2458-11-310 PG 11 WC Public, Environmental & Occupational Health SC Public, Environmental & Occupational Health GA 779PF UT WOS:000291791100001 PM 21569469 ER PT J AU Kasaikina, MV Lobanov, AV Malinouski, MY Lee, BC Seravalli, J Fomenko, DE Turanov, AA Finney, L Vogt, S Park, TJ Miller, RA Hatfield, DL Gladyshev, VN AF Kasaikina, Marina V. Lobanov, Alexei V. Malinouski, Mikalai Y. Lee, Byung Cheon Seravalli, Javier Fomenko, Dmitri E. Turanov, Anton A. Finney, Lydia Vogt, Stefan Park, Thomas J. Miller, Richard A. Hatfield, Dolph L. Gladyshev, Vadim N. TI Reduced Utilization of Selenium by Naked Mole Rats Due to a Specific Defect in GPx1 Expression SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID LONGEST-LIVING RODENT; GLUTATHIONE-PEROXIDASE; HETEROCEPHALUS-GLABER; OXIDATIVE STRESS; MICE; CELLS; SELENOCYSTEINE; RESISTANCE; CANCER; SELENOPROTEINS AB Naked mole rat (MR) Heterocephalus glaber is a rodent model of delayed aging because of its unusually long life span (> 28 years). It is also not known to develop cancer. In the current work, tissue imaging by x-ray fluorescence microscopy and direct analyses of trace elements revealed low levels of selenium in the MR liver and kidney, whereas MR and mouse brains had similar selenium levels. This effect was not explained by uniform selenium deficiency because methionine sulfoxide reductase activities were similar in mice and MR. However, glutathione peroxidase activity was an order of magnitude lower in MR liver and kidney than in mouse tissues. In addition, metabolic labeling of MR cells with (75)Se revealed a loss of the abundant glutathione peroxidase 1 (GPx1) band, whereas other selenoproteins were preserved. To characterize the MR selenoproteome, we sequenced its liver transcriptome. Gene reconstruction revealed standard selenoprotein sequences except for GPx1, which had an early stop codon, and SelP, which had low selenocysteine content. When expressed in HEK 293 cells, MR GPx1 was present in low levels, and its expression could be rescued neither by removing the early stop codon nor by replacing its SECIS element. In addition, GPx1 mRNA was present in lower levels in MR liver than in mouse liver. To determine if GPx1 deficiency could account for the reduced selenium content, we analyzed GPx1 knock-out mice and found reduced selenium levels in their livers and kidneys. Thus, MR is characterized by the reduced utilization of selenium due to a specific defect in GPx1 expression. C1 [Kasaikina, Marina V.; Lobanov, Alexei V.; Malinouski, Mikalai Y.; Lee, Byung Cheon; Turanov, Anton A.; Gladyshev, Vadim N.] Brigham & Womens Hosp, Dept Med, Div Genet, Boston, MA 02115 USA. [Kasaikina, Marina V.; Lobanov, Alexei V.; Malinouski, Mikalai Y.; Lee, Byung Cheon; Turanov, Anton A.; Gladyshev, Vadim N.] Harvard Univ, Sch Med, Boston, MA 02115 USA. [Kasaikina, Marina V.; Malinouski, Mikalai Y.; Lee, Byung Cheon; Seravalli, Javier; Fomenko, Dmitri E.; Gladyshev, Vadim N.] Univ Nebraska, Dept Biochem, Lincoln, NE 68588 USA. [Kasaikina, Marina V.; Malinouski, Mikalai Y.; Lee, Byung Cheon; Seravalli, Javier; Fomenko, Dmitri E.; Gladyshev, Vadim N.] Univ Nebraska, Redox Biol Ctr, Lincoln, NE 68588 USA. [Finney, Lydia] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. [Vogt, Stefan] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Park, Thomas J.] Univ Illinois, Dept Biol Sci, Chicago, IL 60607 USA. [Miller, Richard A.] Univ Michigan, Ann Arbor, MI 48109 USA. [Hatfield, Dolph L.] NCI, Mol Biol Selenium Sect, Lab Canc Prevent, Ctr Canc Res,NIH, Bethesda, MD 20892 USA. RP Gladyshev, VN (reprint author), Brigham & Womens Hosp, Dept Med, Div Genet, New Res Bldg,Rm 435,77 Ave Louis Pasteur, Boston, MA 02115 USA. EM vgladyshev@rics.bwh.harvard.edu RI Gladyshev, Vadim/A-9894-2013; Vogt, Stefan/B-9547-2009; Vogt, Stefan/J-7937-2013 OI Vogt, Stefan/0000-0002-8034-5513; Vogt, Stefan/0000-0002-8034-5513 FU National Institutes of Health [GM061603, CA080946, AG021518]; Center for Cancer Research, NCI, National Institutes of Health; Department of Energy Office of Science [DE-AC02-06CH11357] FX This work was supported, in whole or in part, by National Institutes of Health Grants GM061603, CA080946, and AG021518 (to V. N. G.) and the Intramural Research Program of the Center for Cancer Research, NCI, National Institutes of Health (to D. L. H.). This work was also supported by the Department of Energy Office of Science under Contract DE-AC02-06CH11357. NR 47 TC 15 Z9 15 U1 2 U2 12 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 J9 J BIOL CHEM JI J. Biol. Chem. PD MAY 13 PY 2011 VL 286 IS 19 BP 17005 EP 17014 DI 10.1074/jbc.M110.216267 PG 10 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 760CZ UT WOS:000290301900051 PM 21372135 ER PT J AU Porta, M Lookman, T AF Porta, Marcel Lookman, Turab TI Effects of tricritical points and morphotropic phase boundaries on the piezoelectric properties of ferroelectrics SO PHYSICAL REVIEW B LA English DT Article ID SOLID-SOLUTION SYSTEM; THERMODYNAMIC THEORY; PB(ZRXTI1-X)O-3 CERAMICS; TRANSITIONS; PBZR1-XTIXO3; COEFFICIENTS; CRYSTALS; BEHAVIOR AB The longitudinal piezoelectric coefficient d*(33) of a PZT-like ferroelectric is computed in the full composition-temperature parameter space using sets of parameters that control the position of the tricritical points and the degree of tilting of the morphotropic phase boundary separating the ferroelectric rhombohedral phase from the ferroelectric tetragonal phase. The system is modeled using a Ginzburg-Landau expansion of the free energy in terms of the electric polarization up to sixth order, including all the symmetry-allowed terms. We obtain two regions of the phase diagram with a large piezoelectric response. In the polar direction, d*(33) is large in the vicinity of the paraelectric to ferroelectric line of phase transitions, whereas in a nonpolar direction d*(33) is large in the vicinity of the morphotropic phase boundary. We find that a given degree of tilting of the morphotropic phase boundary can be obtained from free energies with different degrees of anisotropy, and therefore the titling and anisotropy are not directly related. On the other hand, the piezoelectric response is larger when the two tricritical points of the phase diagram are farther apart from each other than when they collapse onto a single tricritical point. C1 [Porta, Marcel] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. Univ Toronto, Dept Mat Sci & Engn, Toronto, ON M5S 3E4, Canada. RP Porta, M (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Porta Tena, Marcel/0000-0001-7582-9671; Lookman, Turab/0000-0001-8122-5671 FU US DOE [DE-AC52-06NA25396]; NSERC of Canada FX We acknowledge fruitful discussions with X. Ren. This work was supported by the US DOE under Contract No. DE-AC52-06NA25396 and NSERC of Canada. NR 27 TC 25 Z9 25 U1 0 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 13 PY 2011 VL 83 IS 17 AR 174108 DI 10.1103/PhysRevB.83.174108 PG 7 WC Physics, Condensed Matter SC Physics GA 765LL UT WOS:000290707500001 ER PT J AU Schmitt, F Moritz, B Johnston, S Mo, SK Hashimoto, M Moore, RG Lu, DH Motoyama, E Greven, M Devereaux, TP Shen, ZX AF Schmitt, F. Moritz, B. Johnston, S. Mo, S. -K. Hashimoto, M. Moore, R. G. Lu, D. -H. Motoyama, E. Greven, M. Devereaux, T. P. Shen, Z. -X. TI High-energy anomaly in Nd2-xCexCuO4 investigated by angle-resolved photoemission spectroscopy and quantum Monte Carlo simulations SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTORS; CORRELATED ELECTRONS AB Recent high-binding-energy angle-resolved photoemission spectroscopy (ARPES) experiments reveal a change in band dispersion in the high-temperature superconducting cuprates (HTSCs) known as the high-energy anomaly (HEA). Despite considerable experimental and theoretical attention, the origin of the HEA remains a topic of some controversy. In this paper we present systematic and comprehensive experimental evidence on the origin of the HEA from ARPES measurements on the electron-doped HTSC material Nd2-xCexCuO4 at a number of dopings across the phase diagram and over the entire Brillouin zone (BZ). Comparing these new experimental findings to quantum Monte Carlo simulations of the single-band Hubbard model across the BZ and for various dopings demonstrates that this simple model qualitatively reproduces the key experimental features of the HEA and points to significant self-energy and band renormalization effects accompanying strong electron correlations as its origin rather than coupling to any one emergent bosonic mode, e. g., antiferromagnetic spin fluctuations. We conclude from comparison to this simple model that the HEA in these systems should be regarded as a crossover from a coherent quasiparticle band at low binding energies, emergent from the upper Hubbard band in electron-doped HTSCs due to doping and modified by subsequent strong band renormalization effects, to oxygen valence bands at higher binding energy that would be revealed in simulations explicitly incorporating these important orbital degrees of freedom. C1 [Schmitt, F.; Hashimoto, M.; Shen, Z. -X.] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. [Schmitt, F.; Moritz, B.; Johnston, S.; Hashimoto, M.; Devereaux, T. P.; Shen, Z. -X.] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA. [Moritz, B.] Univ N Dakota, Dept Phys & Astrophys, Grand Forks, ND 58202 USA. [Johnston, S.] Univ Waterloo, Dept Phys & Astron, Waterloo, ON N2L 3G1, Canada. [Johnston, S.] IFW Dresden, Inst Solid State Res, D-01171 Dresden, Germany. [Mo, S. -K.; Hashimoto, M.] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. [Moore, R. G.; Lu, D. -H.; Shen, Z. -X.] Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Motoyama, E.; Devereaux, T. P.; Shen, Z. -X.] Stanford Univ, Geballe Lab Adv Mat, Stanford, CA 94305 USA. [Greven, M.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. RP Schmitt, F (reprint author), Stanford Univ, Dept Appl Phys, Via Pueblo Mall, Stanford, CA 94305 USA. RI Mo, Sung-Kwan/F-3489-2013; Moritz, Brian/D-7505-2015; Johnston, Steven/J-7777-2016 OI Mo, Sung-Kwan/0000-0003-0711-8514; Moritz, Brian/0000-0002-3747-8484; FU Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-76-SFO0515]; NSF [DMR-0705086]; Natural Sciences and Engineering Research Council of Canada; Foundation for Fundamental Research on Matter; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX We thank C. Kim and W.-S. Lee for valuable discussions. This work was supported in part by the Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Contract No. DE-AC02-76-SFO0515. The crystal growth work was supported by the aforementioned contract and by the NSF under Grant No. DMR-0705086. SJ would like to acknowledge financial support from the Natural Sciences and Engineering Research Council of Canada and the Foundation for Fundamental Research on Matter. Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a national user facility operated by Stanford University on behalf of the US Department of Energy, Office of Basic Energy Sciences. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. Computational results were made possible in part by the resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. Three of the authors (BM, SJ, and TPD) wish to thank the Walther-Meissner-Institut for its hospitality during part of this work. NR 42 TC 5 Z9 5 U1 0 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 13 PY 2011 VL 83 IS 19 AR 195123 DI 10.1103/PhysRevB.83.195123 PG 10 WC Physics, Condensed Matter SC Physics GA 765MM UT WOS:000290711300003 ER PT J AU Sanchez, PD Lees, JP Poireau, V Prencipe, E Tisserand, V Tico, JG Grauges, E Martinelli, M Milanes, DA Palano, A Pappagallo, M Eigen, G Stugu, B Sun, L Brown, DN Kerth, LT Kolomensky, YG Lynch, G Osipenkov, IL Koch, H Schroeder, T Asgeirsson, DJ Hearty, C Mattison, TS McKenna, JA Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Yushkov, AN Bondioli, M Curry, S Kirkby, D Lankford, AJ Mandelkern, M Martin, EC Stoker, DP Atmacan, H Gary, JW Liu, F Long, O Vitug, GM Campagnari, C Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Heusch, CA Kroseberg, J Lockman, WS Martinez, AJ Schalk, T Schumm, BA Seiden, A Winstrom, LO Cheng, CH Doll, DA Echenard, B Hitlin, DG Ongmongkolkul, P Porter, FC Rakitin, AY Andreassen, R Dubrovin, MS Meadows, BT Sokoloff, MD Bloom, PC Ford, WT Gaz, A Nagel, M Nauenberg, U Smith, JG Wagner, SR Ayad, R Toki, WH Jasper, H Petzold, A Spaan, B Kobel, MJ Schubert, KR Schwierz, R Bernard, D Verderi, M Clark, PJ Playfer, S Watson, JE Andreotti, M Bettoni, D Bozzi, C Calabrese, R Cecchi, A Cibinetto, G Fioravanti, E Franchini, P Garzia, I Luppi, E Munerato, M Negrini, M Petrella, A Piemontese, L Baldini-Ferroli, R Calcaterra, A de Sangro, R Finocchiaro, G Nicolaci, M Pacetti, S Patteri, P Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Guido, E Lo Vetere, M Monge, MR Passaggio, S Patrignani, C Robutti, E Bhuyan, B Prasad, V Lee, CL Morii, M Edwards, AJ Adametz, A Marks, J Uwer, U Bernlochner, FU Ebert, M Lacker, HM Lueck, T Volk, A Dauncey, PD Tibbetts, M Behera, PK Mallik, U Chen, C Cochran, J Crawley, HB Meyer, WT Prell, S Rosenberg, EI Rubin, AE Gritsan, AV Guo, ZJ Arnaud, N Davier, M Derkach, D da Costa, JF Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Perez, A Roudeau, P Schune, MH Serrano, J Sordini, V Stocchi, A Wang, L Wormser, G Lange, DJ Wright, DM Bingham, I Chavez, CA Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Sigamani, M Cowan, G Paramesvaran, S Wren, AC Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Hafner, A Alwyn, KE Bailey, D Barlow, RJ Jackson, G Lafferty, GD Anderson, J Cenci, R Jawahery, A Roberts, DA Simi, G Tuggle, JM Dallapiccola, C Salvati, E Cowan, R Dujmic, D Sciolla, G Zhao, M Lindemann, D Patel, PM Robertson, SH Schram, M Biassoni, P Lazzaro, A Lombardo, V Palombo, F Stracka, S Cremaldi, L Godang, R Kroeger, R Sonnek, P Summers, DJ Nguyen, X Simard, M Taras, P De Nardo, G Monorchio, D Onorato, G Sciacca, C Raven, G Snoek, HL Jessop, CP Knoepfel, KJ LoSecco, JM Wang, WF Corwin, LA Honscheid, K Kass, R Blount, NL Brau, J Frey, R Igonkina, O Kolb, JA Rahmat, R Sinev, NB Strom, D Strube, J Torrence, E Castelli, G Feltresi, E Gagliardi, N Margoni, M Morandin, M Posocco, M Rotondo, M Simonetto, F Stroili, R Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Hamon, O Leruste, P Marchiori, G Ocariz, J Prendki, J Sitt, S Biasini, M Manoni, E Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Cervelli, A Forti, F Giorgi, MA Lusiani, A Neri, N Paoloni, E Rizzo, G Walsh, JJ Pegna, DL Lu, C Olsen, J Smith, AJS Telnov, AV Anulli, F Baracchini, E Cavoto, G Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Gioi, LL Mazzoni, MA Piredda, G Renga, F Buenger, C Hartmann, T Leddig, T Schroder, H Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S de Monchenault, GH Vasseur, G Yeche, C Allen, MT Aston, D Bard, DJ Bartoldus, R Benitez, JF Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Field, RC Sevilla, MF Fulsom, BG Gabareen, AM Graham, MT Grenier, P Hast, C Innes, WR Kelsey, MH Kim, H Kim, P Kocian, ML Leith, DWGS Lewis, P Li, S Lindquist, B Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Nelson, S O'Grady, CP Ofte, I Perl, M Pulliam, T Ratcliff, BN Roodman, A Salnikov, AA Santoro, V Schindler, RH Schwiening, J Snyder, A Su, D Sullivan, MK Sun, S Suzuki, K Thompson, JM Va'vra, J Wagner, AP Weaver, M Wisniewski, WJ Wittgen, M Wright, DH Wulsin, HW Yarritu, AK Young, CC Ziegler, V Chen, XR Park, W Purohit, MV White, RM Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Miyashita, TS Ahmed, S Alam, MS Ernst, JA Pan, B Saeed, MA Zain, SB Guttman, N Soffer, A Lund, P Spanier, SM Eckmann, R Ritchie, JL Ruland, AM Schilling, CJ Schwitters, RF Wray, BC Izen, JM Lou, XC Bianchi, F Gamba, D Pelliccioni, M Lanceri, L Vitale, L Lopez-March, N Martinez-Vidal, F Oyanguren, A Ahmed, H Albert, J Banerjee, S Choi, HHF Hamano, K King, GJ Kowalewski, R Lewczuk, MJ Lindsay, C Nugent, IM Roney, JM Sobie, RJ Gershon, TJ Harrison, PF Latham, TE Puccio, EMT Band, HR Dasu, S Flood, KT Pan, Y Prepost, R Vuosalo, CO Wu, SL AF Sanchez, P. del Amo Lees, J. P. Poireau, V. Prencipe, E. Tisserand, V. Garra Tico, J. Grauges, E. Martinelli, M. Milanes, D. A. Palano, A. Pappagallo, M. Eigen, G. Stugu, B. Sun, L. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lynch, G. Osipenkov, I. L. Koch, H. Schroeder, T. Asgeirsson, D. J. Hearty, C. Mattison, T. S. McKenna, J. A. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Yushkov, A. N. Bondioli, M. Curry, S. Kirkby, D. Lankford, A. J. Mandelkern, M. Martin, E. C. Stoker, D. P. Atmacan, H. Gary, J. W. Liu, F. Long, O. Vitug, G. M. Campagnari, C. Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Heusch, C. A. Kroseberg, J. Lockman, W. S. Martinez, A. J. Schalk, T. Schumm, B. A. Seiden, A. Winstrom, L. O. Cheng, C. H. Doll, D. A. Echenard, B. Hitlin, D. G. Ongmongkolkul, P. Porter, F. C. Rakitin, A. Y. Andreassen, R. Dubrovin, M. S. Meadows, B. T. Sokoloff, M. D. Bloom, P. C. Ford, W. T. Gaz, A. Nagel, M. Nauenberg, U. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Jasper, H. Petzold, A. Spaan, B. Kobel, M. J. Schubert, K. R. Schwierz, R. Bernard, D. Verderi, M. Clark, P. J. Playfer, S. Watson, J. E. Andreotti, M. Bettoni, D. Bozzi, C. Calabrese, R. Cecchi, A. Cibinetto, G. Fioravanti, E. Franchini, P. Garzia, I. Luppi, E. Munerato, M. Negrini, M. Petrella, A. Piemontese, L. Baldini-Ferroli, R. Calcaterra, A. de Sangro, R. Finocchiaro, G. Nicolaci, M. Pacetti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Guido, E. Lo Vetere, M. Monge, M. R. Passaggio, S. Patrignani, C. Robutti, E. Bhuyan, B. Prasad, V. Lee, C. L. Morii, M. Edwards, A. J. Adametz, A. Marks, J. Uwer, U. Bernlochner, F. U. Ebert, M. Lacker, H. M. Lueck, T. Volk, A. Dauncey, P. D. Tibbetts, M. Behera, P. K. Mallik, U. Chen, C. Cochran, J. Crawley, H. B. Meyer, W. T. Prell, S. Rosenberg, E. I. Rubin, A. E. Gritsan, A. V. Guo, Z. J. Arnaud, N. Davier, M. Derkach, D. da Costa, J. Firmino Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Perez, A. Roudeau, P. Schune, M. H. Serrano, J. Sordini, V. Stocchi, A. Wang, L. Wormser, G. Lange, D. J. Wright, D. M. Bingham, I. Chavez, C. A. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Sigamani, M. Cowan, G. Paramesvaran, S. Wren, A. C. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Hafner, A. Alwyn, K. E. Bailey, D. Barlow, R. J. Jackson, G. Lafferty, G. D. Anderson, J. Cenci, R. Jawahery, A. Roberts, D. A. Simi, G. Tuggle, J. M. Dallapiccola, C. Salvati, E. Cowan, R. Dujmic, D. Sciolla, G. Zhao, M. Lindemann, D. Patel, P. M. Robertson, S. H. Schram, M. Biassoni, P. Lazzaro, A. Lombardo, V. Palombo, F. Stracka, S. Cremaldi, L. Godang, R. Kroeger, R. Sonnek, P. Summers, D. J. Nguyen, X. Simard, M. Taras, P. De Nardo, G. Monorchio, D. Onorato, G. Sciacca, C. Raven, G. Snoek, H. L. Jessop, C. P. Knoepfel, K. J. LoSecco, J. M. Wang, W. F. Corwin, L. A. Honscheid, K. Kass, R. Blount, N. L. Brau, J. Frey, R. Igonkina, O. Kolb, J. A. Rahmat, R. Sinev, N. B. Strom, D. Strube, J. Torrence, E. Castelli, G. Feltresi, E. Gagliardi, N. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simonetto, F. Stroili, R. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Hamon, O. Leruste, Ph. Marchiori, G. Ocariz, J. Prendki, J. Sitt, S. Biasini, M. Manoni, E. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Cervelli, A. Forti, F. Giorgi, M. A. Lusiani, A. Neri, N. Paoloni, E. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Lu, C. Olsen, J. Smith, A. J. S. Telnov, A. V. Anulli, F. Baracchini, E. Cavoto, G. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Gioi, L. Li Mazzoni, M. A. Piredda, G. Renga, F. Buenger, C. Hartmann, T. Leddig, T. Schroeder, H. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. de Monchenault, G. Hamel Vasseur, G. Yeche, Ch. Allen, M. T. Aston, D. Bard, D. J. Bartoldus, R. Benitez, J. F. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Field, R. C. Sevilla, M. Franco Fulsom, B. G. Gabareen, A. M. Graham, M. T. Grenier, P. Hast, C. Innes, W. R. Kelsey, M. H. Kim, H. Kim, P. Kocian, M. L. Leith, D. W. G. S. Lewis, P. Li, S. Lindquist, B. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Nelson, S. O'Grady, C. P. Ofte, I. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Salnikov, A. A. Santoro, V. Schindler, R. H. Schwiening, J. Snyder, A. Su, D. Sullivan, M. K. Sun, S. Suzuki, K. Thompson, J. M. Va'vra, J. Wagner, A. P. Weaver, M. Wisniewski, W. J. Wittgen, M. Wright, D. H. Wulsin, H. W. Yarritu, A. K. Young, C. C. Ziegler, V. Chen, X. R. Park, W. Purohit, M. V. White, R. M. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Miyashita, T. S. Ahmed, S. Alam, M. S. Ernst, J. A. Pan, B. Saeed, M. A. Zain, S. B. Guttman, N. Soffer, A. Lund, P. Spanier, S. M. Eckmann, R. Ritchie, J. L. Ruland, A. M. Schilling, C. J. Schwitters, R. F. Wray, B. C. Izen, J. M. Lou, X. C. Bianchi, F. Gamba, D. Pelliccioni, M. Lanceri, L. Vitale, L. Lopez-March, N. Martinez-Vidal, F. Oyanguren, A. Ahmed, H. Albert, J. Banerjee, Sw. Choi, H. H. F. Hamano, K. King, G. J. Kowalewski, R. Lewczuk, M. J. Lindsay, C. Nugent, I. M. Roney, J. M. Sobie, R. J. Gershon, T. J. Harrison, P. F. Latham, T. E. Puccio, E. M. T. Band, H. R. Dasu, S. Flood, K. T. Pan, Y. Prepost, R. Vuosalo, C. O. Wu, S. L. CA BaBar Collaboration TI Searches for the baryon- and lepton-number violating decays B-0 -> Lambda(+)(c)l(-), B- -> Lambda l(-), and B- -> (Lambda)over-barl(-) SO PHYSICAL REVIEW D LA English DT Article ID ANNIHILATION AB Searches for B mesons decaying to final states containing a baryon and a lepton are performed, where the baryon is either Lambda(c) or Lambda and the lepton is a muon or an electron. These decays violate both baryon and lepton number and would be a signature of physics beyond the standard model. No significant signal is observed in any of the decay modes, and upper limits in the range (3.2-520) x 10(-8) are set on the branching fractions at the 90% confidence level. C1 [Sanchez, P. del Amo; Lees, J. P.; Poireau, V.; Prencipe, E.; Tisserand, V.] Univ Savoie, LAPP, CNRS, IN2P3, F-74941 Annecy Le Vieux, France. [Garra Tico, J.; Grauges, E.] Univ Barcelona, Fac Fis, Dept ECM, E-08028 Barcelona, Spain. [Martinelli, M.; Milanes, D. A.; Palano, A.; Pappagallo, M.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Martinelli, M.; Palano, A.; Pappagallo, M.] Univ Bari, Dipartimento Fis, I-70126 Bari, Italy. [Eigen, G.; Stugu, B.; Sun, L.] Univ Bergen, Inst Phys, N-5007 Bergen, Norway. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu. G.; Lynch, G.; Osipenkov, I. L.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. 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[Bellis, M.; Burchat, P. R.; Miyashita, T. S.] Stanford Univ, Stanford, CA 94305 USA. [Ahmed, S.; Alam, M. S.; Ernst, J. A.; Pan, B.; Saeed, M. A.; Zain, S. B.] SUNY Albany, Albany, NY 12222 USA. [Guttman, N.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Lund, P.; Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Eckmann, R.; Ritchie, J. L.; Ruland, A. M.; Schilling, C. J.; Schwitters, R. F.; Wray, B. C.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; Gamba, D.; Pelliccioni, M.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; Gamba, D.; Pelliccioni, M.] Univ Turin, Dipartimento Fis Sperimentale, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Lopez-March, N.; Martinez-Vidal, F.; Oyanguren, A.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Ahmed, H.; Albert, J.; Banerjee, Sw.; Choi, H. H. F.; Hamano, K.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lindsay, C.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.; Puccio, E. M. T.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Flood, K. T.; Pan, Y.; Prepost, R.; Vuosalo, C. O.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Carpinelli, M.] Univ Sassari, I-07100 Sassari, Italy. RP Oyanguren, A (reprint author), Univ Savoie, LAPP, CNRS, IN2P3, F-74941 Annecy Le Vieux, France. RI Oyanguren, Arantza/K-6454-2014; Neri, Nicola/G-3991-2012; Luppi, Eleonora/A-4902-2015; Kravchenko, Evgeniy/F-5457-2015; Calabrese, Roberto/G-4405-2015; Forti, Francesco/H-3035-2011; Rotondo, Marcello/I-6043-2012; de Sangro, Riccardo/J-2901-2012; Saeed, Mohammad Alam/J-7455-2012; Negrini, Matteo/C-8906-2014; Patrignani, Claudia/C-5223-2009; Monge, Maria Roberta/G-9127-2012; Martinez Vidal, F*/L-7563-2014; Kolomensky, Yury/I-3510-2015; Lo Vetere, Maurizio/J-5049-2012; Lusiani, Alberto/N-2976-2015; Morandin, Mauro/A-3308-2016; Lusiani, Alberto/A-3329-2016; Stracka, Simone/M-3931-2015; Di Lodovico, Francesca/L-9109-2016; Pappagallo, Marco/R-3305-2016; Calcaterra, Alessandro/P-5260-2015; Frey, Raymond/E-2830-2016; OI Oyanguren, Arantza/0000-0002-8240-7300; Neri, Nicola/0000-0002-6106-3756; Luppi, Eleonora/0000-0002-1072-5633; Calabrese, Roberto/0000-0002-1354-5400; Forti, Francesco/0000-0001-6535-7965; Rotondo, Marcello/0000-0001-5704-6163; de Sangro, Riccardo/0000-0002-3808-5455; Saeed, Mohammad Alam/0000-0002-3529-9255; Negrini, Matteo/0000-0003-0101-6963; Patrignani, Claudia/0000-0002-5882-1747; Monge, Maria Roberta/0000-0003-1633-3195; Martinez Vidal, F*/0000-0001-6841-6035; Kolomensky, Yury/0000-0001-8496-9975; Lo Vetere, Maurizio/0000-0002-6520-4480; Lusiani, Alberto/0000-0002-6876-3288; Morandin, Mauro/0000-0003-4708-4240; Lusiani, Alberto/0000-0002-6876-3288; Stracka, Simone/0000-0003-0013-4714; Di Lodovico, Francesca/0000-0003-3952-2175; Pappagallo, Marco/0000-0001-7601-5602; Calcaterra, Alessandro/0000-0003-2670-4826; Frey, Raymond/0000-0003-0341-2636; Raven, Gerhard/0000-0002-2897-5323 FU DOE; NSF (U.S.); NSERC (Canada); CEA; CNRS-IN2P3 (France); BMBF; DFG (Germany); INFN (Italy); FOM (The Netherlands); NFR (Norway); MES (Russia); MICIIN (Spain); STFC (United Kingdom); European Union; A. P. Sloan Foundation (U.S.); Binational Science Foundation (U.S.-Israel) FX We are grateful for the excellent luminosity and machine conditions provided by our PEP-II colleagues, and for the substantial dedicated effort from the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and kind hospitality. This work is supported by DOE and NSF (U.S.), NSERC (Canada), CEA and CNRS-IN2P3 (France), BMBF and DFG (Germany), INFN (Italy), FOM (The Netherlands), NFR (Norway), MES (Russia), MICIIN (Spain), STFC (United Kingdom). Individuals have received support from the Marie Curie EIF (European Union), the A. P. Sloan Foundation (U.S.), and the Binational Science Foundation (U.S.-Israel). NR 24 TC 8 Z9 8 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 13 PY 2011 VL 83 IS 9 AR 091101 DI 10.1103/PhysRevD.83.091101 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 765OS UT WOS:000290718800001 ER PT J AU Boehly, TR Goncharov, VN Seka, W Barrios, MA Celliers, PM Hicks, DG Collins, GW Hu, SX Marozas, JA Meyerhofer, DD AF Boehly, T. R. Goncharov, V. N. Seka, W. Barrios, M. A. Celliers, P. M. Hicks, D. G. Collins, G. W. Hu, S. X. Marozas, J. A. Meyerhofer, D. D. TI Velocity and Timing of Multiple Spherically Converging Shock Waves in Liquid Deuterium SO PHYSICAL REVIEW LETTERS LA English DT Article ID NATIONAL IGNITION FACILITY; LASER AB The fuel entropy and required drive energy for an inertial confinement fusion implosion are set by a sequence of shocks that must be precisely timed to achieve ignition. This Letter reports measurements of multiple spherical shock waves in liquid deuterium that facilitate timing inertial confinement fusion shocks to the required precision. These experiments produced the highest shock velocity observed in liquid deuterium (U(s) = 135 km/s at similar to 2500 GPa) and also the first observation of convergence effects on the shock velocity. Simulations model the shock-timing results well when a nonlocal transport model is used in the coronal plasma. C1 [Boehly, T. R.; Goncharov, V. N.; Seka, W.; Hu, S. X.; Marozas, J. A.; Meyerhofer, D. D.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA. [Barrios, M. A.; Celliers, P. M.; Hicks, D. G.; Collins, G. W.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Meyerhofer, D. D.] Univ Rochester, Dept Mech Engn, Rochester, NY 14623 USA. [Meyerhofer, D. D.] Univ Rochester, Dept Phys, Rochester, NY 14623 USA. RP Boehly, TR (reprint author), Univ Rochester, Laser Energet Lab, 250 E River Rd, Rochester, NY 14623 USA. RI Hu, Suxing/A-1265-2007; Collins, Gilbert/G-1009-2011; Goncharov, Valeri/H-4471-2011; Hicks, Damien/B-5042-2015 OI Hu, Suxing/0000-0003-2465-3818; Hicks, Damien/0000-0001-8322-9983 FU U.S. Department of Energy Office of Inertial Confinement Fusion [DE-FC52-08NA28302]; University of Rochester; New York State Energy Research and Development Authority FX This work was supported by the U.S. Department of Energy Office of Inertial Confinement Fusion under Cooperative Agreement No. DE-FC52-08NA28302, the University of Rochester, and the New York State Energy Research and Development Authority. The support of DOE does not constitute an endorsement by DOE of the views expressed in this article. NR 19 TC 30 Z9 30 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 13 PY 2011 VL 106 IS 19 AR 195005 DI 10.1103/PhysRevLett.106.195005 PG 4 WC Physics, Multidisciplinary SC Physics GA 765SI UT WOS:000290728500009 PM 21668170 ER PT J AU Albert, F Anderson, SG Gibson, DJ Marsh, RA Wu, SS Siders, CW Barty, CPJ Hartemann, FV AF Albert, F. Anderson, S. G. Gibson, D. J. Marsh, R. A. Wu, S. S. Siders, C. W. Barty, C. P. J. Hartemann, F. V. TI Design of narrow-band Compton scattering sources for nuclear resonance fluorescence SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID ELECTRON AB The design of narrow-band Compton scattering sources for specific applications using nuclear resonance fluorescence (NRF) is presented. NRF lines are extremely narrow (Delta E/E similar to 10(-6)) and require spectrally narrow sources to be excited selectively and efficiently. This paper focuses on the theory of spectral broadening mechanisms involved during Compton scattering of laser photons from relativistic electron beams. It is shown that in addition to the electron beam emittance, energy spread, and the laser parameters, nonlinear processes during the laser-electron interaction can have a detrimental effect on the gamma-ray source bandwidth, including a newly identified weakly nonlinear phase shift accumulated over the effective interaction duration. Finally, a design taking these mechanisms into consideration is outlined. C1 [Albert, F.] Lawrence Livermore Natl Lab, NIF, Livermore, CA 94550 USA. RP Albert, F (reprint author), Lawrence Livermore Natl Lab, NIF, 7000 East Ave, Livermore, CA 94550 USA. EM albert6@llnl.gov RI Albert, Felicie/G-2645-2013 FU U.S. Department of Energy [DE-AC52-07NA27344]; U.S. Department of Homeland Security [HSHQDC-09-X-00554/0001]; Laboratory Directed Research and Development Program at LLNL [09-SI-004] FX The authors acknowledge useful discussions with D. P. McNabb. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, and supported by the U.S. Department of Homeland Security under DNDO Contract No. HSHQDC-09-X-00554/0001. We also acknowledge support from the Laboratory Directed Research and Development Program at LLNL under tracking code 09-SI-004. NR 22 TC 26 Z9 26 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD MAY 13 PY 2011 VL 14 IS 5 AR 050703 DI 10.1103/PhysRevSTAB.14.050703 PG 11 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 765TC UT WOS:000290730500001 ER PT J AU Biersmith, BH Hammel, M Geisbrecht, ER Bouyain, S AF Biersmith, Bridget H. Hammel, Michal Geisbrecht, Erika R. Bouyain, Samuel TI The Immunoglobulin-like Domains 1 and 2 of the Protein Tyrosine Phosphatase LAR Adopt an Unusual Horseshoe-like Conformation SO JOURNAL OF MOLECULAR BIOLOGY LA English DT Article DE cell adhesion; receptor protein tyrosine phosphatase; heparan sulfate proteoglycans; immunoglobulin-like domains; crystal structure ID MOTOR AXON GUIDANCE; LIGAND-BINDING MODULE; X-RAY-SCATTERING; CRYSTAL-STRUCTURE; MICE LACKING; SULFATE PROTEOGLYCAN; DROSOPHILA EMBRYO; STRUCTURAL BASIS; CELL-ADHESION; PTP-SIGMA AB Neurogenesis depends on exquisitely regulated interactions between macromolecules on the cell surface and in the extracellular matrix. In particular, interactions between proteoglycans and members of the type Ha subgroup of receptor protein tyrosine phosphatases underlie crucial developmental processes such as the formation of synapses at the neuromuscular junction and the migration of axons to their appropriate targets. We report the crystal structures of the first and second immunoglobulin-like domains of the Drosophila type Ha receptor Dlar and its mouse homolog LAR. These two domains adopt an unusual antiparallel arrangement that has not been reported in tandem repeats of immunoglobulin-like domains and that is presumably conserved in all type Ha receptor protein tyrosine phosphatases. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Bouyain, Samuel] Univ Missouri, Sch Biol Sci, Div Mol Biol & Biochem, Kansas City, MO 64110 USA. [Biersmith, Bridget H.; Geisbrecht, Erika R.] Univ Missouri, Sch Biol Sci, Div Cell Biol & Biophys, Kansas City, MO 64110 USA. [Hammel, Michal] Univ Calif Berkeley, Lawrence Berkeley Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Bouyain, S (reprint author), Univ Missouri, Sch Biol Sci, Div Mol Biol & Biochem, 5100 Rockhill Rd, Kansas City, MO 64110 USA. EM bouyains@umkc.edu FU National Institute Of General Medical Sciences [R01GM088806]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [W-31-109-Eng-38]; U.S. Department of Energy FX The authors thank Brian Geisbrecht for helpful comments on the manuscript. This work was supported by the National Institute Of General Medical Sciences (award number R01GM088806). Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract no. W-31-109-Eng-38. Data were collected at Southeast Regional Collaborative Access Team beamlines at the Advanced Photon Source, Argonne National Laboratory. X-ray scattering technologies at the Lawrence Berkeley National Laboratory SIBYLS beamline of the Advanced Light Source are supported, in part, by the U.S. Department of Energy program Integrated Diffraction Analysis Technologies (IDAT). NR 47 TC 13 Z9 15 U1 0 U2 0 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-2836 J9 J MOL BIOL JI J. Mol. Biol. PD MAY 13 PY 2011 VL 408 IS 4 BP 616 EP 627 DI 10.1016/j.jmb.2011.03.013 PG 12 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 762SK UT WOS:000290501200003 PM 21402080 ER PT J AU Close, D Johnson, SJ Sdano, MA McDonald, SM Robinson, H Formosa, T Hill, CP AF Close, Devin Johnson, Sean J. Sdano, Matthew A. McDonald, Seth M. Robinson, Howard Formosa, Tim Hill, Christopher P. TI Crystal Structures of the S. cerevisiae Spt6 Core and C-Terminal Tandem SH2 Domain SO JOURNAL OF MOLECULAR BIOLOGY LA English DT Article DE protein structure; protein function; gene expression; crystallography ID RNA-POLYMERASE-II; TRANSCRIPTION ELONGATION-FACTORS; PROTEIN-STRUCTURE; SACCHAROMYCES-CEREVISIAE; IN-VIVO; OB-FOLD; BINDING; COMPLEX; CHROMATIN; PHOSPHORYLATION AB The conserved and essential eukaryotic protein Spt6 functions in transcription elongation, chromatin maintenance, and RNA processing. Spt6 has three characterized functions. It is a histone chaperone capable of reassembling nucleosomes, a central component of transcription elongation complexes, and is required for recruitment of RNA processing factors to elongating RNA polymerase II (RNAPII). Here, we report multiple crystal structures of the 168-kDa Spt6 protein from Saccharomyces cerevisiae that together represent essentially all of the ordered sequence. Our two structures of the similar to 900-residue core region reveal a series of putative nucleic acid and protein-protein interaction domains that fold into an elongated form that resembles the bacterial protein Tex. The similarity to a bacterial transcription factor suggests that the core domain performs nucleosomeindependent activities, and as with Tex, we find that Spt6 binds DNA. Unlike Tex, however, the Spt6 Si domain does not contribute to this activity. Crystal structures of the Spt6 C-terminal region reveal a tandem SH2 domain structure composed of two closely associated SH2 folds. One of these SH2 folds is cryptic, while the other shares striking structural similarity with metazoan SH2 domains and possesses structural features associated with the ability to bind phosphorylated substrates including phosphotyrosine. Binding studies with phosphopeptides that mimic the RNAPII C-terminal domain revealed affinities typical of other RNAPII C-terminal domain-binding proteins but did not indicate a specific interaction. Overall, these findings provide a structural foundation for understanding how Spt6 encodes several distinct functions within a single polypeptide chain. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Close, Devin; Sdano, Matthew A.; McDonald, Seth M.; Formosa, Tim; Hill, Christopher P.] Univ Utah, Dept Biochem, Salt Lake City, UT 84112 USA. [Johnson, Sean J.] Utah State Univ, Dept Chem & Biochem, Logan, UT 84322 USA. [Robinson, Howard] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. RP Hill, CP (reprint author), Univ Utah, Dept Biochem, Salt Lake City, UT 84112 USA. EM chris@biochem.utah.edu RI Johnson, Sean/G-8191-2012 FU National Cancer Institute [P30CA042014]; Offices of Biological and Environmental Research; U.S. Department of Energy; National Center for Research Resources of the National Institutes of Health (NIH); Department of Energy, Office of Biological and Environmental Research; NIH, National Center for Research Resources; Biomedical Technology Program; National Institute of General Medical Sciences; NIH [RO1 GM076242]; [GM074368] FX We thank Hua Xin and Charisse Kettelkamp for technical assistance and Heidi Schubert for advice with the crystallographic analysis. Portions of this work were performed in Core Facilities at the University of Utah, which were supported by P30CA042014 from the National Cancer Institute. Some of the X-ray diffraction data for this study were measured at the National Synchrotron Light Source (NSLS). Financial support for NSLS comes principally from the Offices of Biological and Environmental Research and of Basic Energy Sciences of the U.S. Department of Energy and from the National Center for Research Resources of the National Institutes of Health (NIH). Portions of this research were performed at the Stanford Synchrotron Radiation Laboratory (SSRL), a national user facility operated by Stanford University on behalf of the U.S. Department of Energy, Office of Basic Energy Sciences. The SSRL Structural Molecular Biology Program is supported by the Department of Energy, Office of Biological and Environmental Research, and the NIH, National Center for Research Resources, Biomedical Technology Program, and the National Institute of General Medical Sciences. S.J.J. was supported by a postdoctoral fellowship (GM074368). This work was supported by NIH grant RO1 GM076242. NR 64 TC 20 Z9 20 U1 1 U2 3 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-2836 EI 1089-8638 J9 J MOL BIOL JI J. Mol. Biol. PD MAY 13 PY 2011 VL 408 IS 4 BP 697 EP 713 DI 10.1016/j.jmb.2011.03.002 PG 17 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 762SK UT WOS:000290501200009 PM 21419780 ER PT J AU Blankenship, RE Tiede, DM Barber, J Brudvig, GW Fleming, G Ghirardi, M Gunner, MR Junge, W Kramer, DM Melis, A Moore, TA Moser, CC Nocera, DG Nozik, AJ Ort, DR Parson, WW Prince, RC Sayre, RT AF Blankenship, Robert E. Tiede, David M. Barber, James Brudvig, Gary W. Fleming, Graham Ghirardi, Maria Gunner, M. R. Junge, Wolfgang Kramer, David M. Melis, Anastasios Moore, Thomas A. Moser, Christopher C. Nocera, Daniel G. Nozik, Arthur J. Ort, Donald R. Parson, William W. Prince, Roger C. Sayre, Richard T. TI Comparing Photosynthetic and Photovoltaic Efficiencies and Recognizing the Potential for Improvement SO SCIENCE LA English DT Review ID CO2 CONCENTRATING MECHANISMS; SOLAR-ENERGY; CARBON FIXATION; QUANTUM YIELD; CHLOROPHYLL; CONVERSION; BIOFUELS; CYCLE; HYDROGENASES; MICROALGAE AB Comparing photosynthetic and photovoltaic efficiencies is not a simple issue. Although both processes harvest the energy in sunlight, they operate in distinctly different ways and produce different types of products: biomass or chemical fuels in the case of natural photosynthesis and nonstored electrical current in the case of photovoltaics. In order to find common ground for evaluating energy-conversion efficiency, we compare natural photosynthesis with present technologies for photovoltaic-driven electrolysis of water to produce hydrogen. Photovoltaic-driven electrolysis is the more efficient process when measured on an annual basis, yet short-term yields for photosynthetic conversion under optimal conditions come within a factor of 2 or 3 of the photovoltaic benchmark. We consider opportunities in which the frontiers of synthetic biology might be used to enhance natural photosynthesis for improved solar energy conversion efficiency. C1 [Blankenship, Robert E.] Washington Univ, Dept Biol, St Louis, MO 63130 USA. [Blankenship, Robert E.] Washington Univ, Dept Chem, St Louis, MO 63130 USA. [Tiede, David M.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Barber, James] Univ London Imperial Coll Sci Technol & Med, Div Mol Biosci, London SW7 2AZ, England. [Barber, James] Politecn Torino, Dept Mat Sci & Engn, I-10129 Turin, Italy. [Brudvig, Gary W.] Yale Univ, Dept Chem, New Haven, CT 06520 USA. [Fleming, Graham] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Fleming, Graham] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Ghirardi, Maria] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. [Gunner, M. R.] CUNY, Dept Phys, New York, NY 10031 USA. [Junge, Wolfgang] Univ Osnabruck, Div Biophys, D-49069 Osnabruck, Germany. [Kramer, David M.] Michigan State Univ, Biochem & Mol Biol & DOE Plant Res Lab, E Lansing, MI 48824 USA. [Melis, Anastasios] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Moore, Thomas A.] Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA. [Moser, Christopher C.] Univ Penn, Dept Biochem & Biophys, Philadelphia, PA 19104 USA. [Nocera, Daniel G.] MIT, Dept Chem, Cambridge, MA 02139 USA. [Nozik, Arthur J.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Ort, Donald R.] Univ Illinois, USDA, ARS, Photosynth Res Unit, Urbana, IL 61801 USA. [Parson, William W.] Univ Washington, Dept Biochem, Seattle, WA 98195 USA. [Prince, Roger C.] ExxonMobil Biomed Sci, Annandale, NJ 08801 USA. [Sayre, Richard T.] Donald Danforth Plant Sci Ctr, St Louis, MO 63132 USA. RP Blankenship, RE (reprint author), Washington Univ, Dept Biol, Campus Box 1137, St Louis, MO 63130 USA. EM blankenship@wustl.edu; tiede@anl.gov RI Junge, Wolfgang/F-6289-2012; Nozik, Arthur/A-1481-2012; Nozik, Arthur/P-2641-2016; OI Sayre, Richard/0000-0002-3153-7084 FU Council on Chemical and Biochemical Sciences of the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX This article evolved from presentations and discussions at the workshop "What is the Efficiency of Photosynthesis?" held in May 2009 in Albuquerque, New Mexico, sponsored by the Council on Chemical and Biochemical Sciences of the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. The authors thank the members of the Council for their encouragement and assistance in developing this workshop. In addition, the authors are indebted to the agencies responsible for funding their individual research efforts, without which this work would not have been possible. NR 64 TC 518 Z9 524 U1 79 U2 700 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 J9 SCIENCE JI Science PD MAY 13 PY 2011 VL 332 IS 6031 BP 805 EP 809 DI 10.1126/science.1200165 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 763CD UT WOS:000290529900037 PM 21566184 ER PT J AU Pratt, EJ Hunt, B Gadagkar, V Yamashita, M Graf, MJ Balatsky, AV Davis, JC AF Pratt, E. J. Hunt, B. Gadagkar, V. Yamashita, M. Graf, M. J. Balatsky, A. V. Davis, J. C. TI Interplay of Rotational, Relaxational, and Shear Dynamics in Solid He-4 SO SCIENCE LA English DT Article ID SUPERSOLIDITY; TRANSITION; HELIUM AB Using a high-sensitivity torsional oscillator (TO) technique, we mapped the rotational and relaxational dynamics of solid helium-4 (He-4) throughout the parameter range of the proposed supersolidity. We found evidence that the same microscopic excitations controlling the torsional oscillator motions are generated independently by thermal and mechanical stimulation. Moreover, a measure for the relaxation times of these excitations diverges smoothly without any indication for a critical temperature or critical velocity of a supersolid transition. Finally, we demonstrated that the combined temperature-velocity dependence of the TO response is indistinguishable from the combined temperature-strain dependence of the solid's shear modulus. This implies that the rotational responses of solid He-4 attributed to supersolidity are associated with generation of the same microscopic excitations as those produced by direct shear strain. C1 [Pratt, E. J.; Hunt, B.; Gadagkar, V.; Davis, J. C.] Cornell Univ, Dept Phys, Atom & Solid State Phys Lab, Ithaca, NY 14853 USA. [Pratt, E. J.] Univ Calif Santa Barbara, Kavli Inst Theoret Phys, Santa Barbara, CA 93016 USA. [Hunt, B.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Yamashita, M.] Kyoto Univ, Dept Phys, Kyoto 6068502, Japan. [Graf, M. J.; Balatsky, A. V.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Graf, M. J.; Balatsky, A. V.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Davis, J. C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Davis, J. C.] Univ St Andrews, Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland. RP Davis, JC (reprint author), Cornell Univ, Dept Phys, Atom & Solid State Phys Lab, Ithaca, NY 14853 USA. EM jcdavis@ccmr.cornell.edu RI YAMASHITA, MINORU/D-6556-2011; Pratt, Ethan/E-8714-2011; Hunt, Benjamin/C-3395-2017 OI Hunt, Benjamin/0000-0002-5008-8042 FU National Science Foundation [DMR-0806629, NSF PHY05-51164]; U.S. Department of Energy [DE-AC52-06NA25396]; Laboratory Directed Research and Development program FX We are grateful for discussions and communications with J. Beamish, D. M. Ceperley, M. H. W. Chan, J. Day, A. T. Dorsey, R. B. Hallock, H. Kojima, D. M. Lee, A. J. Leggett, E. Mueller, D. R. Nelson, J. M. Parpia, N. V. Prokof'ev, J. D. Reppy, P. C. E. Stamp, B. Svistunov, and M. Troyer. These studies were supported by the National Science Foundation under grants DMR-0806629 and NSF PHY05-51164 to the Kavli Institute for Theoretical Physics. Work at Los Alamos was supported by U.S. Department of Energy grant DE-AC52-06NA25396 to the Center for Integrated Nanotechnologies and through the Laboratory Directed Research and Development program. NR 34 TC 21 Z9 21 U1 1 U2 6 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 J9 SCIENCE JI Science PD MAY 13 PY 2011 VL 332 IS 6031 BP 821 EP 824 DI 10.1126/science.1203080 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 763CD UT WOS:000290529900040 PM 21566187 ER PT J AU Larsen, PE Sreedasyam, A Trivedi, G Podila, GK Cseke, LJ Collart, FR AF Larsen, Peter E. Sreedasyam, Avinash Trivedi, Geetika Podila, Gopi K. Cseke, Leland J. Collart, Frank R. TI Using next generation transcriptome sequencing to predict an ectomycorrhizal metabolome SO BMC SYSTEMS BIOLOGY LA English DT Article ID ARBUSCULAR MYCORRHIZAL SYMBIOSIS; FUNGUS LACCARIA-BICOLOR; RNA-SEQ; NITROGEN-FIXATION; ORGANIC NITROGEN; PINUS-SYLVESTRIS; POPULUS-TREMULA; GENE; PHOSPHATE; PLANTS AB Background: Mycorrhizae, symbiotic interactions between soil fungi and tree roots, are ubiquitous in terrestrial ecosystems. The fungi contribute phosphorous, nitrogen and mobilized nutrients from organic matter in the soil and in return the fungus receives photosynthetically-derived carbohydrates. This union of plant and fungal metabolisms is the mycorrhizal metabolome. Understanding this symbiotic relationship at a molecular level provides important contributions to the understanding of forest ecosystems and global carbon cycling. Results: We generated next generation short-read transcriptomic sequencing data from fully-formed ectomycorrhizae between Laccaria bicolor and aspen (Populus tremuloides) roots. The transcriptomic data was used to identify statistically significantly expressed gene models using a bootstrap-style approach, and these expressed genes were mapped to specific metabolic pathways. Integration of expressed genes that code for metabolic enzymes and the set of expressed membrane transporters generates a predictive model of the ectomycorrhizal metabolome. The generated model of mycorrhizal metabolome predicts that the specific compounds glycine, glutamate, and allantoin are synthesized by L. bicolor and that these compounds or their metabolites may be used for the benefit of aspen in exchange for the photosynthetically-derived sugars fructose and glucose. Conclusions: The analysis illustrates an approach to generate testable biological hypotheses to investigate the complex molecular interactions that drive ectomycorrhizal symbiosis. These models are consistent with experimental environmental data and provide insight into the molecular exchange processes for organisms in this complex ecosystem. The method used here for predicting metabolomic models of mycorrhizal systems from deep RNA sequencing data can be generalized and is broadly applicable to transcriptomic data derived from complex systems. C1 [Larsen, Peter E.; Collart, Frank R.] Argonne Natl Lab, Biosci Div, Lemont, IL 60490 USA. [Sreedasyam, Avinash; Trivedi, Geetika; Podila, Gopi K.; Cseke, Leland J.] Univ Alabama, Dept Biol Sci, Huntsville, AL 35899 USA. RP Larsen, PE (reprint author), Argonne Natl Lab, Biosci Div, Lemont, IL 60490 USA. EM plarsen@anl.gov OI Collart, Frank/0000-0001-6942-4483 FU U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 67 TC 23 Z9 24 U1 10 U2 76 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1752-0509 J9 BMC SYST BIOL JI BMC Syst. Biol. PD MAY 13 PY 2011 VL 5 AR 70 DI 10.1186/1752-0509-5-70 PG 14 WC Mathematical & Computational Biology SC Mathematical & Computational Biology GA 780TL UT WOS:000291882000001 PM 21569493 ER PT J AU Barton, NR Bernier, JV Knap, J Sunwoo, AJ Cerreta, EK Turner, TJ AF Barton, Nathan R. Bernier, Joel V. Knap, Jaroslaw Sunwoo, Anne J. Cerreta, Ellen K. Turner, Todd J. TI A call to arms for task parallelism in multi-scale materials modeling SO INTERNATIONAL JOURNAL FOR NUMERICAL METHODS IN ENGINEERING LA English DT Article DE solids; materials science; multiscale; plasticity; parallelization; finite element methods ID SITU ADAPTIVE TABULATION; POLYCRYSTALLINE SOLIDS; COMPONENT ARCHITECTURE; DEFORMATION-BEHAVIOR; CRYSTAL PLASTICITY; STRAIN RATES; SIMULATION; TITANIUM; TEXTURE; ALLOY AB Simulations based on multi-scale material models enabled by adaptive sampling have demonstrated speedup factors exceeding an order of magnitude. The use of these methods in parallel computing is hampered by dynamic load imbalance, with load imbalance measurably reducing the achieved speedup. Here we discuss these issues in the context of task parallelism, showing results achieved to date and discussing possibilities for further improvement. In some cases, the task parallelism methods employed to date are able to restore much of the potential wall-clock speedup. The specific application highlighted here focuses on the connection between microstructure and material performance using a polycrystal plasticity-based multi-scale method. However, the parallel load balancing issues are germane to a broad class of multi-scale problems. Copyright (C) 2011 John Wiley & Sons, Ltd. C1 [Barton, Nathan R.; Bernier, Joel V.; Sunwoo, Anne J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Knap, Jaroslaw] USA, Res Lab, Aberdeen Proving Ground, MD 21005 USA. [Cerreta, Ellen K.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Turner, Todd J.] USAF, Res Lab, Wright Patterson AFB, OH 45433 USA. RP Barton, NR (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM barton22@llnl.gov FU agency of the United States government; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344 (LLNL-JRNL-426324)] FX This document was prepared as an account of work sponsored by an agency of the United States government. Neither the United States government nor Lawrence Livermore National Security, LLC, nor any of their employees makes any warranty, expressed or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States government or Lawrence Livermore National Security, LLC. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States government or Lawrence Livermore National Security, LLC, and shall not be used for advertising or product endorsement purposes.; This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 (LLNL-JRNL-426324). We gratefully acknowledge the contributions of the members of the Babel and Co-op teams, the cooperation of the Ale3d development team, the resources provided by Livermore Computing, and DOD support of ongoing research through James Mackiewicz. NR 69 TC 12 Z9 12 U1 0 U2 9 PU WILEY-BLACKWELL PI MALDEN PA COMMERCE PLACE, 350 MAIN ST, MALDEN 02148, MA USA SN 0029-5981 J9 INT J NUMER METH ENG JI Int. J. Numer. Methods Eng. PD MAY 13 PY 2011 VL 86 IS 6 BP 744 EP 764 DI 10.1002/nme.3071 PG 21 WC Engineering, Multidisciplinary; Mathematics, Interdisciplinary Applications SC Engineering; Mathematics GA 748CZ UT WOS:000289368900004 ER PT J AU Iqbal, U Albaghdadi, H Nieh, MP Tuor, UI Mester, Z Stanimirovic, D Katsaras, J Abulrob, A AF Iqbal, Umar Albaghdadi, Homam Nieh, Mu-Ping Tuor, Ursula I. Mester, Zoltan Stanimirovic, Danica Katsaras, John Abulrob, Abedelnasser TI Small unilamellar vesicles: a platform technology for molecular imaging of brain tumors SO NANOTECHNOLOGY LA English DT Article ID HUMAN GLIOBLASTOMA CELLS; IN-VIVO; KINETIC-ANALYSIS; ANGIOGENESIS; LIPOSOMES; RECEPTOR; TIME; IDENTIFICATION; NANOPARTICLES; ANTIBODIES AB Molecular imaging enables the non-invasive investigation of cellular and molecular processes. Although there are challenges to overcome, the development of targeted contrast agents to increase the sensitivity of molecular imaging techniques is essential for their clinical translation. In this study, spontaneously forming, small unilamellar vesicles (sULVs) (30 nm diameter) were used as a platform to build a bimodal (i.e., optical and magnetic resonance imaging (MRI)) targeted contrast agent for the molecular imaging of brain tumors. sULVs were loaded with a gadolinium (Gd) chelated lipid (Gd-DPTA-BOA), functionalized with targeting antibodies (anti-EGFR monoclonal and anti-IGFBP7 single domain), and incorporated a near infrared dye (Cy5.5). The resultant sULVs were characterized in vitro using small angle neutron scattering (SANS), phantom MRI and dynamic light scattering (DLS). Antibody targeted and nontargeted Gd loaded sULVs labeled with Cy5.5 were assessed in vivo in a brain tumor model in mice using time domain optical imaging and MRI. The results demonstrated that a spontaneously forming, nanosized ULVs loaded with a high payload of Gd can selectively target and image, using MR and optical imaging, brain tumor vessels when functionalized with anti-IGFBP7 single domain antibodies. The unique features of these targeted sULVs make them promising molecular MRI contrast agents. C1 [Iqbal, Umar; Albaghdadi, Homam; Stanimirovic, Danica; Abulrob, Abedelnasser] Natl Res Council Canada, Inst Biol Sci, Ottawa, ON K1A 0R6, Canada. [Nieh, Mu-Ping; Katsaras, John] Natl Res Council Canada, Canadian Neutron Beam Ctr, Chalk River Labs, Chalk River, ON K0J 1J0, Canada. [Nieh, Mu-Ping] Univ Connecticut, Dept Chem Mat & Biomol Engn, Inst Mat Sci, Storrs, CT 06269 USA. [Tuor, Ursula I.] Natl Res Council Canada, Inst Biodiagnost W, Calgary, AB T2N 4N1, Canada. [Mester, Zoltan] Natl Res Council Canada, Inst Natl Measurements Stand, Ottawa, ON K1A 0R6, Canada. [Katsaras, John] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN USA. RP Iqbal, U (reprint author), Natl Res Council Canada, Inst Biol Sci, 1200 Montreal Rd, Ottawa, ON K1A 0R6, Canada. EM Abedelnasser.abulrob@nrc.gc.ca RI Mester, Zoltan/F-3154-2013; OI Mester, Zoltan/0000-0002-2377-2615; Nieh, Mu-Ping/0000-0003-4462-8716; Katsaras, John/0000-0002-8937-4177 NR 41 TC 9 Z9 11 U1 1 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD MAY 13 PY 2011 VL 22 IS 19 AR 195102 DI 10.1088/0957-4484/22/19/195102 PG 15 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 739WE UT WOS:000288750800002 PM 21436507 ER PT J AU Draganic, IN Seely, DG Havener, CC AF Draganic, I. N. Seely, D. G. Havener, C. C. TI Low-energy charge transfer between C5+ and atomic hydrogen SO PHYSICAL REVIEW A LA English DT Article ID MERGED-BEAMS MEASUREMENTS; ELECTRON-CAPTURE; CROSS-SECTIONS; X-RAY; IONS; COLLISIONS; EXCHANGE; IONIZATION; H-2 AB Charge transfer with carbon ions has been identified as important in both magnetic fusion plasma devices and, more recently, in solar wind interactions with comets, planets, or neutrals in the heliosphere. A merged-beams technique is used to measure the absolute total charge-transfer cross section for C5+ and atomic H over four orders of magnitude in collision energy, from 12 000 to 0.64 eV/u. The present measurements are compared with previous measurements using an atomic hydrogen target and benchmark available classical trajectory Monte Carlo and molecular-orbital close-coupling calculations. An observed increasing cross section below 10 eV/u is attributed to trajectory effects due to the ion-induced dipole attraction between reactants. C1 [Draganic, I. N.; Havener, C. C.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Seely, D. G.] Albion Coll, Dept Phys, Albion, MI 49224 USA. RP Draganic, IN (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. FU Office of Fusion Energy Sciences; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the US Department of Energy; NASA [NNH07ZDA001]; ORNL FX This research is supported by the Office of Fusion Energy Sciences and the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the US Department of Energy. I.N.D is supported by the NASA Solar & Heliospheric Physics Program (Grant No. NNH07ZDA001) and acknowledges support from the ORNL Postdoctoral Research Associates Program administered jointly by the Oak Ridge Institute for Science and Education and Oak Ridge National Laboratory. NR 27 TC 9 Z9 9 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 J9 PHYS REV A JI Phys. Rev. A PD MAY 12 PY 2011 VL 83 IS 5 AR 054701 DI 10.1103/PhysRevA.83.054701 PG 4 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 762ZE UT WOS:000290520300015 ER PT J AU Jansen, GR Hjorth-Jensen, M Hagen, G Papenbrock, T AF Jansen, G. R. Hjorth-Jensen, M. Hagen, G. Papenbrock, T. TI Toward open-shell nuclei with coupled-cluster theory SO PHYSICAL REVIEW C LA English DT Article ID EFFECTIVE-FIELD THEORY; CHIRAL LAGRANGIANS; SYSTEMS; FORCES; STATE; O-16 AB We develop a method based on equation-of-motion coupled-cluster theory to describe properties of open-shell nuclei with A +/- 2 nucleons outside a closed shell. We perform proof-of-principle calculations for the ground states of the helium isotopes He3-6 and the first excited 2(+) state in He-6. The comparison with exact results from matrix diagonalization in small model spaces demonstrates the accuracy of the coupled-cluster methods. Three-particle-one-hole excitations of He-4 play an important role for the accurate description of He-6. For the open-shell nucleus He-6, the computational cost of the method is comparable with the coupled-cluster singles-and-doubles approximation while its accuracy is similar to the coupled-cluster with singles, doubles, and triples excitations. C1 [Jansen, G. R.; Hjorth-Jensen, M.] Univ Oslo, Dept Phys, N-0316 Oslo, Norway. [Jansen, G. R.; Hjorth-Jensen, M.] Univ Oslo, Ctr Math Applicat, N-0316 Oslo, Norway. [Hagen, G.; Papenbrock, T.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Hagen, G.; Papenbrock, T.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Papenbrock, T.] GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany. [Papenbrock, T.] Tech Univ Darmstadt, Inst Kernphys, D-64289 Darmstadt, Germany. RP Jansen, GR (reprint author), Univ Oslo, Dept Phys, POB 1048, N-0316 Oslo, Norway. RI Hagen, Gaute/I-6146-2012; OI Hagen, Gaute/0000-0001-6019-1687; Jansen, Gustav R./0000-0003-3558-0968; Papenbrock, Thomas/0000-0001-8733-2849 FU US Department of Energy (University of Tennessee) [DE-FG02-96ER40963]; UNEDF SciDAC [DE-FC02-07ER41457]; Research Council of Norway; Alexander von Humboldt Stiftung FX We thank Oyvind Jensen for several discussions. T.P. thanks the Institut fur Kernphysik, Technische Universitat Darmstadt, and the GSI Helmholtzzentrum fur Schwerionenforschung for their hospitality. This work was supported in part by the US Department of Energy, Grants No. DE-FG02-96ER40963 (University of Tennessee), and No. DE-FC02-07ER41457 (UNEDF SciDAC), the Research Council of Norway, and the Alexander von Humboldt Stiftung. This research used computational resources of the Notur project in Norway and the National Center for Computational Sciences at Oak Ridge National Laboratory. NR 46 TC 44 Z9 44 U1 2 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 12 PY 2011 VL 83 IS 5 AR 054306 DI 10.1103/PhysRevC.83.054306 PG 9 WC Physics, Nuclear SC Physics GA 762ZR UT WOS:000290522200003 ER PT J AU Aaltonen, T Gonzalez, BA Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Apollinari, G Appel, JA Apresyan, A Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Auerbach, B Aurisano, A Azfar, F Badgett, W Barbaro-Galtieri, A Barnes, VE Barnett, BA Barria, P Bartos, P Bauce, M Bauer, G Bedeschi, F Beecher, D Behari, S Bellettini, G Bellinger, J Benjamin, D Beretvas, A Bhatti, A Binkley, M Bisello, D Bizjak, I Bland, KR Blumenfeld, B Bocci, A Bodek, A Bortoletto, D Boudreau, J Boveia, A Brau, B Brigliadori, L Brisuda, A Bromberg, C Brucken, E Bucciantonio, M Budagov, J Budd, HS Budd, S Burkett, K Busetto, G Bussey, P Buzatu, A Calancha, C Camarda, S Campanelli, M Campbell, M Canelli, F Canepa, A Carls, B Carlsmith, D Carosi, R Carrillo, S Carron, S Casal, B Casarsa, M Castro, A Catastini, P Cauz, D Cavaliere, V Cavalli-Sforza, M Cerri, A Cerrito, L Chen, YC Chertok, M Chiarelli, G Chlachidze, G Chlebana, F Cho, K Chokheli, D Chou, JP Chung, WH Chung, YS Ciobanu, CI Ciocci, MA Clark, A Compostella, G Convery, ME Conway, J Corbo, M Cordelli, M Cox, CA Cox, DJ Crescioli, F Almenar, CC Cuevas, J Culbertson, R Dagenhart, D d'Ascenzo, N Datta, M de Barbaro, P De Cecco, S De Lorenzo, G Dell'Orso, M Deluca, C Demortier, L Deng, J Deninno, M Devoto, F d'Errico, M Di Canto, A Di Ruzza, B Dittmann, JR D'Onofrio, M Donati, S Dong, P Dorigo, M Dorigo, T Ebina, K Elagin, A Eppig, A Erbacher, R Errede, D Errede, S Ershaidat, N Eusebi, R Fang, HC Farrington, S Feindt, M Fernandez, P Ferrazza, C Field, R Flanagan, G Forrest, R Frank, MJ Franklin, M Freeman, JC Funakoshi, Y Furic, I Gallinaro, M Galyardt, J Garcia, JE Garfinkel, AF Garosi, P Gerberich, H Gerchtein, E Giagu, S Giakoumopoulou, V Giannetti, P Gibson, K Ginsburg, CM Giokaris, N Giromini, P Giunta, M Giurgiu, G Glagolev, V Glenzinski, D Gold, M Goldin, D Goldschmidt, N Golossanov, A Gomez, G Gomez-Ceballos, G Goncharov, M Gonzalez, O Gorelov, I Goshaw, AT Goulianos, K Grinstein, S Grosso-Pilcher, C Group, RC da Costa, JG Gunay-Unalan, Z Haber, C Hahn, SR Halkiadakis, E Hamaguchi, A Han, JY Happacher, F Hara, K Hare, D Hare, M Harr, RF Hatakeyama, K Hays, C Heck, M Heinrich, J Herndon, M Hewamanage, S Hidas, D Hocker, A Hopkins, W Horn, D Hou, S Hughes, RE Hurwitz, M Husemann, U Hussain, N Hussein, M Huston, J Introzzi, G Iori, M Ivanov, A James, E Jang, D Jayatilaka, B Jeon, EJ Jha, MK Jindariani, S Johnson, W Jones, M Joo, KK Jun, SY Junk, TR Kamon, T Karchin, PE Kato, Y Ketchum, W Keung, J Khotilovich, V Kilminster, B Kim, DH Kim, HS Kim, HW Kim, JE Kim, MJ Kim, SB Kim, SH Kim, YK Kimura, N Kirby, M Klimenko, S Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kreps, M Kroll, J Krop, D Krumnack, N Kruse, M Krutelyov, V Kuhr, T Kurata, M Kwang, S Laasanen, AT Lami, S Lammel, S Lancaster, M Lander, RL Lannon, K Lath, A Latino, G LeCompte, T Lee, E Lee, HS Lee, JS Lee, SW Leo, S Leone, S Lewis, JD Limosani, A Lin, CJ Linacre, J Lindgren, M Lipeles, E Lister, A Litvintsev, DO Liu, C Liu, Q Liu, T Lockwitz, S Lockyer, NS Loginov, A Lucchesi, D Lueck, J Lujan, P Lukens, P Lungu, G Lys, J Lysak, R Madrak, R Maeshima, K Makhoul, K Maksimovic, P Malik, S Manca, G Manousakis-Katsikakis, A Margaroli, F Marino, C Martinez, M Martinez-Ballarin, R Mastrandrea, P Mathis, M Mattson, ME Mazzanti, P McFarland, KS McIntyre, P McNulty, R Mehta, A Mehtala, P Menzione, A Mesropian, C Miao, T Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Mondragon, MN Moon, CS Moore, R Morello, MJ Morlock, J Fernandez, PM Mukherjee, A Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nakano, I Napier, A Nett, J Neu, C Neubauer, MS Nielsen, J Nodulman, L Norniella, O Nurse, E Oakes, L Oh, SH Oh, YD Oksuzian, I Okusawa, T Orava, R Ortolan, L Griso, SP Pagliarone, C Palencia, E Papadimitriou, V Paramonov, AA Patrick, J Pauletta, G Paulini, M Paus, C Pellett, DE Penzo, A Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pondrom, L Potamianos, K Poukhov, O Prokoshin, F Pronko, A Ptohos, F Pueschel, E Punzi, G Pursley, J Rahaman, A Ramakrishnan, V Ranjan, N Rao, K Redondo, I Renton, P Rescigno, M Rimondi, F Ristori, L Robson, A Rodrigo, T Rodriguez, T Rogers, E Rolli, S Roser, R Rossi, M Rubbo, F Ruffini, F Ruiz, A Russ, J Rusu, V Safonov, A Sakumoto, WK Sakurai, Y Santi, L Sartori, L Sato, K Saveliev, V Savoy-Navarro, A Schlabach, P Schmidt, A Schmidt, EE Schmidt, MP Schmitt, M Schwarz, T Scodellaro, L Scribano, A Scuri, F Sedov, A Seidel, S Seiya, Y Semenov, A Sforza, F Sfyrla, A Shalhout, SZ Shears, T Shepard, PF Shimojima, M Shiraishi, S Shochet, M Shreyber, I Simonenko, A Sinervo, P Sissakian, A Sliwa, K Smith, JR Snider, FD Soha, A Somalwar, S Sorin, V Squillacioti, P Stancari, M Stanitzki, M St Denis, R Stelzer, B Stelzer-Chilton, O Stentz, D Strologas, J Strycker, GL Sudo, Y Sukhanov, A Suslov, I Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thome, J Thompson, GA Thomson, E Ttito-Guzman, P Tkaczyk, S Toback, D Tokar, S Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Tu, Y Ukegawa, F Uozumi, S Varganov, A Vazquez, F Velev, G Vellidis, C Vidal, M Vila, I Vilar, R Vizan, J Vogel, M Volpi, G Wagner, P Wagner, RL Wakisaka, T Wallny, R Wang, SM Warburton, A Waters, D Weinberger, M Wester, WC Whitehouse, B Whiteson, D Wicklund, AB Wicklund, E Wilbur, S Wick, F Williams, HH Wilson, JS Wilson, P Winer, BL Wittich, P Wolbers, S Wolfe, H Wright, T Wu, X Wu, Z Yamamoto, K Yamaoka, J Yang, T Yang, UK Yang, YC Yao, WM Yeh, GP Yi, K Yoh, J Yorita, K Yoshida, T Yu, GB Yu, I Yu, SS Yun, JC Zanetti, A Zeng, Y Zucchelli, S AF Aaltonen, T. Alvarez Gonzalez, B. Amerio, S. Amidei, D. Anastassov, A. Annovi, A. Antos, J. Apollinari, G. Appel, J. A. Apresyan, A. Arisawa, T. Artikov, A. Asaadi, J. Ashmanskas, W. Auerbach, B. Aurisano, A. Azfar, F. Badgett, W. Barbaro-Galtieri, A. Barnes, V. E. Barnett, B. A. Barria, P. Bartos, P. Bauce, M. Bauer, G. Bedeschi, F. Beecher, D. Behari, S. Bellettini, G. Bellinger, J. Benjamin, D. Beretvas, A. Bhatti, A. Binkley, M. Bisello, D. Bizjak, I. Bland, K. R. Blumenfeld, B. Bocci, A. Bodek, A. Bortoletto, D. Boudreau, J. Boveia, A. Brau, B. Brigliadori, L. Brisuda, A. Bromberg, C. Brucken, E. Bucciantonio, M. Budagov, J. Budd, H. S. Budd, S. Burkett, K. Busetto, G. Bussey, P. Buzatu, A. Calancha, C. Camarda, S. Campanelli, M. Campbell, M. Canelli, F. Canepa, A. Carls, B. Carlsmith, D. Carosi, R. Carrillo, S. Carron, S. Casal, B. Casarsa, M. Castro, A. Catastini, P. Cauz, D. Cavaliere, V. Cavalli-Sforza, M. Cerri, A. Cerrito, L. Chen, Y. C. Chertok, M. Chiarelli, G. Chlachidze, G. 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Glagolev, V. Glenzinski, D. Gold, M. Goldin, D. Goldschmidt, N. Golossanov, A. Gomez, G. Gomez-Ceballos, G. Goncharov, M. Gonzalez, O. Gorelov, I. Goshaw, A. T. Goulianos, K. Grinstein, S. Grosso-Pilcher, C. Group, R. C. da Costa, J. Guimaraes Gunay-Unalan, Z. Haber, C. Hahn, S. R. Halkiadakis, E. Hamaguchi, A. Han, J. Y. Happacher, F. Hara, K. Hare, D. Hare, M. Harr, R. F. Hatakeyama, K. Hays, C. Heck, M. Heinrich, J. Herndon, M. Hewamanage, S. Hidas, D. Hocker, A. Hopkins, W. Horn, D. Hou, S. Hughes, R. E. Hurwitz, M. Husemann, U. Hussain, N. Hussein, M. Huston, J. Introzzi, G. Iori, M. Ivanov, A. James, E. Jang, D. Jayatilaka, B. Jeon, E. J. Jha, M. K. Jindariani, S. Johnson, W. Jones, M. Joo, K. K. Jun, S. Y. Junk, T. R. Kamon, T. Karchin, P. E. Kato, Y. Ketchum, W. Keung, J. Khotilovich, V. Kilminster, B. Kim, D. H. Kim, H. S. Kim, H. W. Kim, J. E. Kim, M. J. Kim, S. B. Kim, S. H. Kim, Y. K. Kimura, N. Kirby, M. Klimenko, S. Kondo, K. Kong, D. J. Konigsberg, J. Kotwal, A. V. 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Scribano, A. Scuri, F. Sedov, A. Seidel, S. Seiya, Y. Semenov, A. Sforza, F. Sfyrla, A. Shalhout, S. Z. Shears, T. Shepard, P. F. Shimojima, M. Shiraishi, S. Shochet, M. Shreyber, I. Simonenko, A. Sinervo, P. Sissakian, A. Sliwa, K. Smith, J. R. Snider, F. D. Soha, A. Somalwar, S. Sorin, V. Squillacioti, P. Stancari, M. Stanitzki, M. St Denis, R. Stelzer, B. Stelzer-Chilton, O. Stentz, D. Strologas, J. Strycker, G. L. Sudo, Y. Sukhanov, A. Suslov, I. Takemasa, K. Takeuchi, Y. Tang, J. Tecchio, M. Teng, P. K. Thom, J. Thome, J. Thompson, G. A. Thomson, E. Ttito-Guzman, P. Tkaczyk, S. Toback, D. Tokar, S. Tollefson, K. Tomura, T. Tonelli, D. Torre, S. Torretta, D. Totaro, P. Trovato, M. Tu, Y. Ukegawa, F. Uozumi, S. Varganov, A. Vazquez, F. Velev, G. Vellidis, C. Vidal, M. Vila, I. Vilar, R. Vizan, J. Vogel, M. Volpi, G. Wagner, P. Wagner, R. L. Wakisaka, T. Wallny, R. Wang, S. M. Warburton, A. Waters, D. Weinberger, M. Wester, W. C., III Whitehouse, B. Whiteson, D. Wicklund, A. B. Wicklund, E. Wilbur, S. Wick, F. Williams, H. H. Wilson, J. S. Wilson, P. Winer, B. L. Wittich, P. Wolbers, S. Wolfe, H. Wright, T. Wu, X. Wu, Z. Yamamoto, K. Yamaoka, J. Yang, T. Yang, U. K. Yang, Y. C. Yao, W-M. Yeh, G. P. Yi, K. Yoh, J. Yorita, K. Yoshida, T. Yu, G. B. Yu, I. Yu, S. S. Yun, J. C. Zanetti, A. Zeng, Y. Zucchelli, S. CA CDF Collaboration TI Search for Production of Heavy Particles Decaying to Top Quarks and Invisible Particles in p(p)over-bar Collisions at root s=1.96 TeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID PHYSICS AB We present a search for a new particle T' decaying to top quark via T' -> t + X, where X is an invisible particle. In a data sample with 4.8 fb(-1) of integrated luminosity collected by the CDF II detector at Fermilab in p (p) over bar collisions with root s = 1.96 TeV, we search for pair production of T' in the lepton + jets channel, p (p) over bar -> t (t) over bar + X + X -> lvbqq'b + X + X. We interpret our results primarily in terms of a model where T' are exotic fourth generation quarks and X are dark matter particles. Current direct and indirect bounds on such exotic quarks restrict their masses to be between 300 and 600 GeV/c(2), the dark matter particle mass being anywhere below m(T'). The data are consistent with standard model expectations, and we set 95% confidence level limits on the generic production of T'(T) over bar -> t (t) over bar + X + X. For the dark matter model we exclude T' at 95% confidence level up to m(T)' = 360 GeV/c(2) for m(X) <= 100 GeV/c(2). C1 [Aaltonen, T.; Brucken, E.; Devoto, F.; Mehtala, P.; Orava, R.] Univ Helsinki, Dept Phys, Div High Energy Phys, FIN-00014 Helsinki, Finland. [Aaltonen, T.; Brucken, E.; Devoto, F.; Mehtala, P.; Orava, R.] Helsinki Inst Phys, FIN-00014 Helsinki, Finland. [Carrillo, S.; Chen, Y. C.; Hou, S.; Mitra, A.; Teng, P. K.; Vazquez, F.; Wang, S. M.] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. 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[Asaadi, J.; Aurisano, A.; Elagin, A.; Eusebi, R.; Goldin, D.; Khotilovich, V.; Krutelyov, V.; Lee, E.; Lee, S. W.; McIntyre, P.; Nett, J.; Safonov, A.; Toback, D.; Weinberger, M.] Texas A&M Univ, College Stn, TX 77843 USA. [Cauz, D.; Dorigo, M.; Pagliarone, C.; Pauletta, G.; Penzo, A.; Rossi, M.; Santi, L.; Zanetti, A.] Ist Nazl Fis Nucl Trieste Udine, I-34100 Trieste, Italy. [Pauletta, G.; Santi, L.] Univ Trieste Udine, I-33100 Udine, Italy. [Hara, K.; Kim, S. H.; Kurata, M.; Miyake, H.; Nagai, Y.; Sato, K.; Shimojima, M.; Sudo, Y.; Takemasa, K.; Takeuchi, Y.; Tomura, T.; Ukegawa, F.] Univ Tsukuba, Tsukuba, Ibaraki 305, Japan. [Hare, M.; Napier, A.; Rolli, S.; Sliwa, K.; Whitehouse, B.] Tufts Univ, Medford, MA 02155 USA. [Group, R. C.; Neu, C.; Oksuzian, I.] Univ Virginia, Charlottesville, VA 22906 USA. [Arisawa, T.; Ebina, K.; Funakoshi, Y.; Kimura, N.; Kondo, K.; Naganoma, J.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo 169, Japan. [Harr, R. F.; Mattson, M. E.] Wayne State Univ, Detroit, MI 48201 USA. [Bellinger, J.; Carlsmith, D.; Chung, W. H.; Herndon, M.; Pondrom, L.; Pursley, J.; Ramakrishnan, V.] Univ Wisconsin, Madison, WI 53706 USA. [Auerbach, B.; Almenar, C. Cuenca; Husemann, U.; Lockwitz, S.; Loginov, A.; Schmidt, M. P.; Stanitzki, M.] Yale Univ, New Haven, CT 06520 USA. RP Aaltonen, T (reprint author), Univ Helsinki, Dept Phys, Div High Energy Phys, FIN-00014 Helsinki, Finland. RI Moon, Chang-Seong/J-3619-2014; Scodellaro, Luca/K-9091-2014; Grinstein, Sebastian/N-3988-2014; Paulini, Manfred/N-7794-2014; Russ, James/P-3092-2014; Chiarelli, Giorgio/E-8953-2012; unalan, zeynep/C-6660-2015; vilar, rocio/P-8480-2014; Garcia, Jose /H-6339-2015; Cavalli-Sforza, Matteo/H-7102-2015; ciocci, maria agnese /I-2153-2015; Introzzi, Gianluca/K-2497-2015; Piacentino, Giovanni/K-3269-2015; Ruiz, Alberto/E-4473-2011; Lysak, Roman/H-2995-2014; Robson, Aidan/G-1087-2011; De Cecco, Sandro/B-1016-2012; St.Denis, Richard/C-8997-2012; manca, giulia/I-9264-2012; Amerio, Silvia/J-4605-2012; Punzi, Giovanni/J-4947-2012; Zeng, Yu/C-1438-2013; Annovi, Alberto/G-6028-2012; Ivanov, Andrew/A-7982-2013; Warburton, Andreas/N-8028-2013; Kim, Soo-Bong/B-7061-2014; Martinez Ballarin, Roberto/K-9209-2015; Gorelov, Igor/J-9010-2015; Prokoshin, Fedor/E-2795-2012; Canelli, Florencia/O-9693-2016 OI Moon, Chang-Seong/0000-0001-8229-7829; Scodellaro, Luca/0000-0002-4974-8330; Grinstein, Sebastian/0000-0002-6460-8694; Paulini, Manfred/0000-0002-6714-5787; Russ, James/0000-0001-9856-9155; Chiarelli, Giorgio/0000-0001-9851-4816; unalan, zeynep/0000-0003-2570-7611; ciocci, maria agnese /0000-0003-0002-5462; Introzzi, Gianluca/0000-0002-1314-2580; Piacentino, Giovanni/0000-0001-9884-2924; Ruiz, Alberto/0000-0002-3639-0368; Punzi, Giovanni/0000-0002-8346-9052; Annovi, Alberto/0000-0002-4649-4398; Ivanov, Andrew/0000-0002-9270-5643; Warburton, Andreas/0000-0002-2298-7315; Martinez Ballarin, Roberto/0000-0003-0588-6720; Gorelov, Igor/0000-0001-5570-0133; Prokoshin, Fedor/0000-0001-6389-5399; Canelli, Florencia/0000-0001-6361-2117 FU U.S. Department of Energy; National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A.P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; World Class University, the National Research Foundation of Korea; Science and Technology Facilities Council and the Royal Society, UK; Institut National de Physique Nucleaire et Physique des Particules/CNRS; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion; Programa Consolider-Ingenio 2010, Spain; Slovak RD Agency; Academy of Finland FX We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the Ministry of Education, Culture, Sports, Science and Technology of Japan; the Natural Sciences and Engineering Research Council of Canada; the National Science Council of the Republic of China; the Swiss National Science Foundation; the A.P. Sloan Foundation; the Bundesministerium fur Bildung und Forschung, Germany; the World Class University Program, the National Research Foundation of Korea; the Science and Technology Facilities Council and the Royal Society, UK; the Institut National de Physique Nucleaire et Physique des Particules/CNRS; the Russian Foundation for Basic Research; the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain; the Slovak R&D Agency; and the Academy of Finland. NR 21 TC 28 Z9 28 U1 2 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 12 PY 2011 VL 106 IS 19 AR 191801 DI 10.1103/PhysRevLett.106.191801 PG 7 WC Physics, Multidisciplinary SC Physics GA 762YV UT WOS:000290519100001 ER PT J AU Chernyak, VY Knoester, J Tretiak, S AF Chernyak, Vladimir Y. Knoester, Jasper Tretiak, Sergei TI Tribute to Shaul Mukamel SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Editorial Material C1 [Chernyak, Vladimir Y.] Wayne State Univ, Detroit, MI 48202 USA. [Knoester, Jasper] Univ Groningen, NL-9700 AB Groningen, Netherlands. [Tretiak, Sergei] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Chernyak, VY (reprint author), Wayne State Univ, Detroit, MI 48202 USA. RI Tretiak, Sergei/B-5556-2009; Chernyak, Vladimir/F-5842-2016 OI Tretiak, Sergei/0000-0001-5547-3647; Chernyak, Vladimir/0000-0003-4389-4238 NR 0 TC 0 Z9 0 U1 0 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 12 PY 2011 VL 115 IS 18 BP 5037 EP 5038 DI 10.1021/jp202931j PG 2 WC Chemistry, Physical SC Chemistry GA 757ZA UT WOS:000290127100001 PM 21542650 ER PT J AU Graham, MW Chmeliov, J Ma, YZ Shinohara, H Green, AA Hersam, MC Valkunas, L Fleming, GR AF Graham, M. W. Chmeliov, J. Ma, Y. -Z. Shinohara, H. Green, A. A. Hersam, M. C. Valkunas, L. Fleming, G. R. TI Exciton Dynamics in Semiconducting Carbon Nanotubes SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID SPECTROSCOPY; WALL AB We report a femtosecond transient absorption spectroscopic study on the (6, 5) single-walled carbon nanotubes and the (7, 5) inner tubes of a dominant double-walled carbon nanotube species. We found that the dynamics of exciton relaxation probed at the first transition-allowed state (E-11) of a given tube type exhibits a markedly slower decay when the second transition-allowed state (E-22) is excited than that measured by exciting its first transition-allowed state (E-11). A linear intensity dependence of the maximal amplitude of the transient absorption signal is found for the E-22 excitation, whereas the corresponding amplitude scales linearly with the square root of the E-11 excitation intensity. Theoretical modeling of these experimental findings was performed by developing a continuum model and a stochastic model with explicit consideration of the annihilation of coherent excitons. Our detailed numerical simulations show that both models can reproduce reasonably well the initial portion of decay kinetics measured upon the E-22 and E-11 excitation of the chosen tube species, but the stochastic model gives qualitatively better agreement with the intensity dependence observed experimentally than those obtained with the continuum model. C1 [Chmeliov, J.; Valkunas, L.] Ctr Phys Sci & Technol, LT-02300 Vilnius, Lithuania. [Chmeliov, J.; Valkunas, L.] Vilnius State Univ, Dept Theoret Phys, Fac Phys, LT-10222 Vilnius, Lithuania. [Graham, M. W.; Ma, Y. -Z.; Fleming, G. R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Graham, M. W.; Ma, Y. -Z.; Fleming, G. R.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Ma, Y. -Z.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Shinohara, H.] Nagoya Univ, Dept Chem, Chikusa Ku, Nagoya, Aichi 4648602, Japan. [Shinohara, H.] Nagoya Univ, Inst Adv Res, Chikusa Ku, Nagoya, Aichi 4648602, Japan. [Green, A. A.; Hersam, M. C.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. RP Valkunas, L (reprint author), Ctr Phys Sci & Technol, Savanoriu Ave 231, LT-02300 Vilnius, Lithuania. EM Leonas.Valkunas@ff.vu.lt RI Hersam, Mark/B-6739-2009; Chmeliov, Jevgenij/P-1782-2015; Ma, Yingzhong/L-6261-2016; OI Chmeliov, Jevgenij/0000-0002-7591-1373; Ma, Yingzhong/0000-0002-8154-1006; Green, Alexander/0000-0003-2058-1204 FU Lithuanian Scientific Council; NSF; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; Natural Sciences and Engineering Research Council of Canada FX This research was supported by the global grant of the Lithuanian Scientific Council according to the operational programme for the human resources development and by the NSF. Y.-Z.M, also acknowledges the support by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. M.W.G. thanks Natural Sciences and Engineering Research Council of Canada for a postgraduate scholarship. Density gradient processing was supported by the National Science Foundation, the Office of Naval Research, and the Nanoelectronics Research Initiative. NR 34 TC 26 Z9 26 U1 0 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 12 PY 2011 VL 115 IS 18 BP 5201 EP 5211 DI 10.1021/jp106250a PG 11 WC Chemistry, Physical SC Chemistry GA 757ZA UT WOS:000290127100016 PM 21090793 ER PT J AU Velizhanin, KA Piryatinski, A AF Velizhanin, Kirill A. Piryatinski, Andrei TI Probing Interband Coulomb Interactions in Semiconductor Nanostructures with 2D Double-Quantum Coherence Spectroscopy SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID MULTIPLE EXCITON GENERATION; CARRIER-MULTIPLICATION; SOLAR-CELLS; OPTICAL-PROPERTIES; DOTS; NANOCRYSTALS; ENERGY; PBSE; BIEXCITONS; EFFICIENCY AB Employing the interband exciton scattering model, we have derived a closed set of equations determining the 2D double-quantum coherence signal sensitive to the interband Coulomb interactions (i.e., many-body Coulomb interactions leading to the couplings between exciton and biexciton bands) in semiconductor nanostructures such as nanocrystals, quantum wires, wells, and carbon nanotubes. Our general analysis of 2D double-quantum coherence resonances has demonstrated that the interband Coulomb interactions lead to new cross-peaks whose appearance can be interpreted as a result of exciton and biexciton state mixing. The presence of the strongly coupled resonant states and weakly coupled background of off-resonant states can significantly simplify cross-peak analysis by eliminating the congested background spectrum. Our simulations of the 2D double-quantum coherence signal in PbSe NCs have validated this approach. C1 [Velizhanin, Kirill A.; Piryatinski, Andrei] Los Alamos Natl Lab, Ctr Nonlinear Studies, Div Theoret, Los Alamos, NM 87545 USA. RP Piryatinski, A (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies, Div Theoret, Los Alamos, NM 87545 USA. EM apiryat@lanl.gov RI Piryatinski, Andrei/B-5543-2009; Velizhanin, Kirill/C-4835-2008 FU Office of Basic Energy Sciences, US Department of Energy; Los Alamos LDRD FX This work was supported by the Office of Basic Energy Sciences, US Department of Energy, and Los Alamos LDRD funds. We also acknowledge the support provided by CNLS. We wish to thank Shaul Mukamel for directing our attention to investigate the sensitivity of the 2D double-quantum coherence technique to the interband Coulomb interactions. NR 49 TC 6 Z9 6 U1 0 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 12 PY 2011 VL 115 IS 18 BP 5372 EP 5382 DI 10.1021/jp109453y PG 11 WC Chemistry, Physical SC Chemistry GA 757ZA UT WOS:000290127100035 PM 21391697 ER PT J AU Nelson, T Fernandez-Alberti, S Chernyak, V Roitberg, AE Tretiak, S AF Nelson, Tammie Fernandez-Alberti, Sebastian Chernyak, Vladimir Roitberg, Adrian E. Tretiak, Sergei TI Nonadiabatic Excited-State Molecular Dynamics Modeling of Photoinduced Dynamics in Conjugated Molecules SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID DENSITY-FUNCTIONAL THEORY; DEPENDENT HARTREE-FOCK; OPTICAL-EXCITATIONS; ABSORPTION-SPECTRA; NONLINEAR POLARIZABILITIES; SEMICONDUCTOR NANOCRYSTALS; PHENYLACETYLENE DENDRIMERS; ELECTRONIC EXCITATIONS; SEMIEMPIRICAL METHODS; NANOSCALE SYSTEMS AB Nonadiabatic dynamics generally defines the entire evolution of electronic excitations in optically active molecular materials. It is commonly associated with a number of fundamental and complex processes such as intraband relaxation, energy transfer, and light harvesting influenced by the spatial evolution of excitations and transformation of photoexcitation energy into electrical energy via charge separation (e.g., charge injection at interfaces). To treat ultrafast excited-state dynamics and exciton/charge transport we have developed a nonadiabatic excited-state molecular dynamics (NA-ESMD) framework incorporating quantum transitions. Our calculations rely on the use of the Collective Electronic Oscillator (CEO) package accounting for many-body effects and actual potential energy surfaces of the excited states combined with Tully's fewest switches algorithm for surface hopping for probing nonadiabatic processes. This method is applied to model the photoinduced dynamics of distyrylbenzene (a small oligomer of polyphenylene vinylene, PPV). Our analysis shows intricate details of photoinduced vibronic relaxation and identifies specific slow and fast nuclear motions that are strongly coupled to the electronic degrees of freedom, namely, torsion and bond length alternation, respectively. Nonadiabatic relaxation of the highly excited mA(g) state is predicted to occur on a femtosecond time scale at room temperature and on a picosecond time scale at low temperature. C1 [Nelson, Tammie; Tretiak, Sergei] Los Alamos Natl Lab, Ctr Nonlinear Studies, Div Theoret, Los Alamos, NM 87545 USA. [Nelson, Tammie; Tretiak, Sergei] Los Alamos Natl Lab, Ctr Integrated Nanotechnol CINT, Los Alamos, NM 87545 USA. [Fernandez-Alberti, Sebastian] Univ Nacl Quilmes, Bernal, Argentina. [Chernyak, Vladimir] Wayne State Univ, Dept Chem, Detroit, MI 48202 USA. [Roitberg, Adrian E.] Univ Florida, Dept Phys, Quantum Theory Project, Gainesville, FL 32611 USA. [Roitberg, Adrian E.] Univ Florida, Dept Chem, Quantum Theory Project, Gainesville, FL 32611 USA. RP Tretiak, S (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies, Div Theoret, Los Alamos, NM 87545 USA. EM serg@lanl.gov RI Roitberg, Adrian/A-2378-2009; Tretiak, Sergei/B-5556-2009; Chernyak, Vladimir/F-5842-2016 OI Tretiak, Sergei/0000-0001-5547-3647; Chernyak, Vladimir/0000-0003-4389-4238 FU U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES); CONICET; UNQ; NSF [CHE-0239120, CHE-0808910]; U.S. Department of Energy [DE-ACS2-06NA25396]; Center for Integrated Nanotechnology (CINT); Center for Nonlinear Studies (CNLS) FX T.N. and ST. acknowledge support of the Center for Energy Efficient Materials (CEEM), an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES). This work was partially supported by CONICET, UNQ, NSF Grants CHE-0239120 and CHE-0808910. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-ACS2-06NA25396. We acknowledge support of the Center for Integrated Nanotechnology (CINT) and Center for Nonlinear Studies (CNLS). NR 114 TC 87 Z9 87 U1 7 U2 68 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 12 PY 2011 VL 115 IS 18 BP 5402 EP 5414 DI 10.1021/jp109522g PG 13 WC Chemistry, Physical SC Chemistry GA 757ZA UT WOS:000290127100038 PM 21218841 ER PT J AU Li, H Wu, C Malinin, SV Tretiak, S Chernyak, VY AF Li, Hao Wu, Chao Malinin, Sergey V. Tretiak, Sergei Chernyak, Vladimir Y. TI Exciton Scattering on Symmetric Branching Centers in Conjugated Molecules SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID ENERGY-LOSS SPECTROSCOPY; ELECTRONIC EXCITATIONS; OPTICAL-EXCITATIONS; NANOSCALE SYSTEMS; BINDING-ENERGY; POLYMERS; DENDRIMERS; PHOTOVOLTAICS; OLIGOMERS; STATES AB The capability of the exciton scattering approach, an efficient methodology for excited states in branched conjugated molecules, is extended to include symmetric triple and quadruple joints that connect linear segments on the basis of the phenylacetylene backbone. The obtained scattering matrices that characterize these vertices are used in application of our approach to several test structures, where we find excellent agreement with the transition energies computed by the reference quantum chemistry. We introduce topological charges, associated with the scattering matrices, which help to formulate useful relations between the number of excitations in the exciton band and the number of repeat units. The obtained features of the scattering phases are analyzed in terms of the observed excited state electronic structure. C1 [Tretiak, Sergei] Los Alamos Natl Lab, Ctr Nonlinear Studies, Div Theoret, Los Alamos, NM 87545 USA. [Tretiak, Sergei] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Li, Hao; Malinin, Sergey V.; Chernyak, Vladimir Y.] Wayne State Univ, Dept Chem, Detroit, MI 48202 USA. [Wu, Chao] Univ Notre Dame, Dept Chem & Biomol Engn, Notre Dame, IN 46556 USA. RP Tretiak, S (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies, Div Theoret, Los Alamos, NM 87545 USA. EM serg@lanl.gov; chernyak@chem.wayne.edu RI wu, chao/A-1303-2011; Li, Hao/B-4756-2013; Tretiak, Sergei/B-5556-2009; Chernyak, Vladimir/F-5842-2016 OI wu, chao/0000-0002-8573-7196; Tretiak, Sergei/0000-0001-5547-3647; Chernyak, Vladimir/0000-0003-4389-4238 FU National Science Foundation [CHE-0808910]; U.S. Department of Energy [DE-AC50-06NA25396]; Los Alamos LDRD funds; Center for Integrated Nanotechnology (CINT); Center for Nonlinear Studies (CNLS) FX This material is based upon work supported by the National Science Foundation under Grant No. CHE-0808910. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract DE-AC50-06NA25396. We acknowledge support of Los Alamos LDRD funds, Center for Integrated Nanotechnology (CINT), and Center for Nonlinear Studies (CNLS). NR 56 TC 6 Z9 6 U1 0 U2 5 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 12 PY 2011 VL 115 IS 18 BP 5465 EP 5475 DI 10.1021/jp110317d PG 11 WC Chemistry, Physical SC Chemistry GA 757ZA UT WOS:000290127100045 PM 21194223 ER PT J AU Karadimitriou, ME Kavousanaki, EG Dani, KM Fromer, NA Perakis, IE AF Karadimitriou, M. E. Kavousanaki, E. G. Dani, K. M. Fromer, N. A. Perakis, I. E. TI lStrong Electronic Correlation Effects in Coherent Multidimensional Nonlinear Optical Spectroscopy SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID FERMI-EDGE SINGULARITY; QUANTUM HALL SYSTEM; HARTREE-FOCK APPROXIMATION; COLLECTIVE EXCITATIONS; LANDAU-LEVEL; MANY-BODY; TRANSFORMATION APPROACH; SEMICONDUCTOR OPTICS; ULTRAFAST DYNAMICS; VIRTUAL EXCITATION AB We discuss a many-body theory of the coherent ultrafast nonlinear optical response of systems with a strongly correlated electronic ground state that responds unadiabatically to photoexcitation. We introduce a truncation of quantum kinetic density matrix equations of motion that does not rely on an expansion in terms of the interactions and thus applies to strongly correlated systems. For this we expand in terms of the optical field, separate out contributions to the time-evolved many-body state due to correlated and uncorrelated multiple optical transitions, and use "Hubbard operator" density matrices to describe the exact dynamics of the individual contributions within a subspace of strongly coupled states, including "pure dephasing". Our purpose is to develop a quantum mechanical tool capable of exploring how, by coherently photoexciting selected modes, one can trigger nonlinear dynamics of strongly coupled degrees of freedom. Such dynamics could lead to photoinduced phase transitions. We apply our theory to the nonlinear response of a two-dimensional electron gas (2DEG) in a magnetic field. We coherently photoexcite the two lowest Landau level (LL) excitations using three time-delayed optical pulses. We identify some striking temporal and spectral features due to dynamical coupling of the two LLs facilitated by inter-Landau-level magnetoplasmon and magnetoroton excitations and compare to three-pulse four-wave-mixing (FINM) experiments. We show that these features depend sensitively on the dynamics of four particle correlations between an electron-hole pair and a magnetoplasmon/magnetoroton, reminiscent of exciton-exciton correlations in undoped semiconductors. Our results shed light into unexplored coherent dynamics and relaxation of the quantum Hall system (QHS) and can provide new insight into non-equilibrium co-operative phenomena in strongly correlated systems. C1 [Karadimitriou, M. E.; Perakis, I. E.] Univ Crete, Dept Phys, Iraklion 71003, Crete, Greece. [Karadimitriou, M. E.; Perakis, I. E.] Fdn Res & Technol Hellas, Inst Elect Struct & Laser, Iraklion 71110, Crete, Greece. [Kavousanaki, E. G.] Univ Konstanz, Dept Phys, D-78464 Constance, Germany. [Dani, K. M.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Fromer, N. A.] CALTECH, Pasadena, CA 91125 USA. RP Perakis, IE (reprint author), Univ Crete, Dept Phys, Iraklion 71003, Crete, Greece. EM ilias@physics.uoc.gr RI Perakis, Ilias/G-9186-2011; Kavousanaki, Eleftheria/D-5712-2015; Dani, Keshav/B-7490-2015 OI Kavousanaki, Eleftheria/0000-0003-1805-6638; Dani, Keshav/0000-0003-3917-6305 FU EU FX This work was supported by the EU ITN program ICARUS. NR 90 TC 3 Z9 3 U1 2 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 12 PY 2011 VL 115 IS 18 BP 5634 EP 5647 DI 10.1021/jp1118794 PG 14 WC Chemistry, Physical SC Chemistry GA 757ZA UT WOS:000290127100063 PM 21395320 ER PT J AU Agapov, RL Malkovskiy, AV Sokolov, AP Foster, MD AF Agapov, Rebecca L. Malkovskiy, Andrey V. Sokolov, Alexei P. Foster, Mark D. TI Prolonged Blinking with TERS Probes SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ENHANCED RAMAN-SCATTERING; ATOMIC LAYER DEPOSITION; SINGLE-MOLECULE; SEPARATION DEPENDENCE; CARBON NANOTUBES; IN-SITU; SPECTROSCOPY; SERS; FILMS; NANOPARTICLES AB Tip-enhanced Raman spectroscopy (TERS), an emerging technique combining scanning probe microscopy (SPM) and Raman spectroscopy, provides the sensitivity and selectivity necessary for chemical imaging with nanoscale resolution. We demonstrate that coating the fragile plasmonic structures used to enhance the electric field with a protective layer improves significantly its mechanical, chemical, and thermal stability without loss of the extreme optical enhancement that appears as a "blinking" phenomenon. This observation provides important information on the mechanism of blinking. The fact that TERS blinking from a polymer layer is preserved when the analyte is separated from the plasmonic nanostructure by a 3 nm thick coating proves that chemical enhancement and charge transfer do not play a significant role in the blinking. Rather, thermally activated diffusion appears to be the dominant mechanism. While extreme enhancement persists only for minutes for an unprotected silver-coated tip, it persists for tens of hours with plasmonic structures coated by an ultrathin layer of alumina (Al(2)O(3)), opening broader opportunities for the study of blinking and for chemical imaging and sensing based on plasmonic structures. C1 [Agapov, Rebecca L.; Malkovskiy, Andrey V.; Foster, Mark D.] Univ Akron, Dept Polymer Sci, Akron, OH 44325 USA. [Sokolov, Alexei P.] Univ Tennessee, ORNL, Div Chem Sci, Knoxville, TN 37996 USA. [Sokolov, Alexei P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Foster, MD (reprint author), Univ Akron, Dept Polymer Sci, Akron, OH 44325 USA. EM mfoster@uakron.edu FU U.S. Army Research Laboratory; U.S. Army Research Office [W911NF-07-1-0470, W91NF-09-1-0424] FX This material is based upon work supported by, or in part by, the U.S. Army Research Laboratory and the U.S. Army Research Office under grants W911NF-07-1-0470 and W91NF-09-1-0424. The authors gratefully acknowledge Dr. Bojie Wang for help with TEM and SEM imaging and Dr. Edward Evans for assistance with physical vapor depositions. NR 56 TC 12 Z9 13 U1 0 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 12 PY 2011 VL 115 IS 18 BP 8900 EP 8905 DI 10.1021/jp111762u PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 757ZB UT WOS:000290127200005 ER PT J AU Tarakeshwar, P Finkelstein-Shapiro, D Hurst, SJ Rajh, T Mujica, V AF Tarakeshwar, Pilarisetty Finkelstein-Shapiro, Daniel Hurst, Sarah J. Rajh, Tijana Mujica, Vladimiro TI Surface-Enhanced Raman Scattering on Semiconducting Oxide Nanoparticles: Oxide Nature, Size, Solvent, and pH Effects SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID NOBLE-METAL NANOPARTICLES; DENSITY-FUNCTIONAL THEORY; TIO2 NANOPARTICLES; VIBRATIONAL FREQUENCIES; ELECTROMAGNETIC THEORY; SPECTROSCOPY SERS; ELECTRON-TRANSFER; SILVER ELECTRODE; CHARGE-TRANSFER; HARTREE-FOCK AB Semiconducting oxide nanoparticles have proven to be excellent in detecting extremely low-concentrations of molecules through surface-enhanced Raman scattering (SERS) effects. While the enhancement of the Raman activities arises from a large increase in polarizability due to charge transfer from the molecule to the semiconducting nanoparticle, little is known about how the oxide composition, nanoparticle size, solvent, or pH affects the observed Raman activities. In the current study, we examine these effects by carrying out extensive computational investigations of semiconducting TiO(2), SnO(2) and Fe(2)O(3) nanoparticles and their complexes with both catechol and dopamine. An increase in the size of the oxide cluster or a decrease in the pH of the system under observation leads to enhanced Raman activities; the variation of the activities in different solvents is very much dependent on the nature of the vibrational modes. The marked increase in the Raman activities of molecules adsorbed on SnO(2) or Fe(2)O(3) over that of molecules adsorbed on TiO(2) seems to indicate that these oxide nanoparticles would be useful substrates for SERS sensors. Our results also indicate that the Raman activities of some of the TiO(2) modes are magnified upon adsorption of molecules, which concurs with some very recent experimental observations. All these results are consistent with a recently proposed theoretical model of SERS on semiconducting substrates. Further, this work has implications on the development of molecular sensing, dye-sensitized solar cells, and photocatalysis. C1 [Tarakeshwar, Pilarisetty; Mujica, Vladimiro] Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA. [Finkelstein-Shapiro, Daniel; Mujica, Vladimiro] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Hurst, Sarah J.; Rajh, Tijana; Mujica, Vladimiro] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Tarakeshwar, P (reprint author), Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA. EM tarakesh@asu.edu; vmujica@asu.edu RI Petrosko, Sarah/A-3606-2013; Tarakeshwar, P./B-6609-2008; OI Tarakeshwar, P./0000-0002-0893-0670; Finkelstein Shapiro, Daniel/0000-0001-8015-5376 NR 91 TC 40 Z9 41 U1 8 U2 104 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 12 PY 2011 VL 115 IS 18 BP 8994 EP 9004 DI 10.1021/jp202590e PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 757ZB UT WOS:000290127200020 ER PT J AU Andersen, A Kathmann, SM Lilga, MA Albrecht, KO Hallen, RT Mei, DH AF Andersen, Amity Kathmann, Shawn M. Lilga, Michael A. Albrecht, Karl O. Hallen, Richard T. Mei, Donghai TI Adsorption of Potassium on MoS2(100) Surface: A First-Principles Investigation SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SPACE GAUSSIAN PSEUDOPOTENTIALS; MOLYBDENUM-DISULFIDE; ALCOHOLS SYNTHESIS; ALKALI PROMOTERS; AB-INITIO; MOS2; CATALYSTS; SYNGAS; CO; K2CO3/MOS2 AB Potassium- (K-) promoted MoS2 catalyst is a very promising catalyst used for synthesis of mixed higher alcohols from syngas. Herein, periodic density functional theory calculations were performed to investigate the interaction of potassium with the Mo and S edges of the MoS2(100) surface. Both neutral K- and charged "K+"-promoted MoS2(100) systems at different sulfur coverages were studied. Our calculations indicate that the adsorbed K atom readily donates its single 4s valence electron to the MoS2 structure, and the neutral K and charged K+ systems show similar adsorption behavior. Isolated K atom/ion tends to maximize its interactions with the available S atoms on the edge surface, preferring the 4-fold S hollow site on fully sulfided Mo and S edges and the interstitial sites where K atom/ion binds with 2-4 S atoms on the edge surface. The presence of K atoms/ions affects the electronic and magnetic properties of the edge surface. As the K coverage increases, the average adsorption energy of the K atoms, surface work function, and amount of 4s electron transfer from the K atoms to the MoS2(100) surface all decrease, suggesting an increased metallization of the K adlayer. The tendency to form a chainlike K adlayer along the interstitial gap area of two edges is found. The K-K distances in the K chains of the adlayer are 3.2-3.7 angstrom, which is notably less than that of bulk K metal. Density of states analysis for the K-saturated MoS2(100) surface suggests enhanced involvement of broad K 3d states beginning just above the Fermi level. The K promotional effects on the selectivity of mixed alcohol synthesis from CO hydrogenation can be rationalized as an increase in the surface basicity due to the increasing surface electron charge donated by K doping. The adsorbed K atoms/ions also provide active sites that facilitate CO hydrogenation, block Mo and S edge sites for CO dissociation leading to hydrocarbon formation, and limit H-2 dissociative adsorption at the edge surface via the s-type electron repulsion from the transferred K 4s electron. C1 [Andersen, Amity] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Kathmann, Shawn M.; Mei, Donghai] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Lilga, Michael A.; Albrecht, Karl O.; Hallen, Richard T.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Andersen, A (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. EM amity.andersen@pnl.gov; donghai.mei@pnl.gov RI Mei, Donghai/D-3251-2011; Mei, Donghai/A-2115-2012 OI Mei, Donghai/0000-0002-0286-4182 FU CRADA [PNNL/297]; Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory FX This work was funded by a CRADA project (PNNL/297) with Range Fuels. The research was performed by use of EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. We thank Dr. Roger Rousseau for his insight into the intricacies of the MoS2 system, its interaction with alkali metals, and the application of electronic structure methods. We also thank Ron Stites and Karl Kharas at Range Fuels for their insightful discussions concerning alkali-promoted MoS2 as an alcohol synthesis catalyst. NR 74 TC 23 Z9 23 U1 7 U2 82 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 12 PY 2011 VL 115 IS 18 BP 9025 EP 9040 DI 10.1021/jp110069r PG 16 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 757ZB UT WOS:000290127200023 ER PT J AU Si, H Peng, LJ Morris, JR Pan, BC AF Si, H. Peng, L. J. Morris, James R. Pan, B. C. TI Theoretical Prediction of Hydrogen Storage on ZnO Sheet SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID GRAPHENE; PSEUDOPOTENTIALS; NANOSTRUCTURES; ADSORPTION; SIMULATION; SYSTEMS; FILMS AB Using first-principles calculations, we investigate the adsorption behavior of hydrogen on the planar hexagonal ZnO sheet. Our calculations find that the planar ZnO monolayer preferably adsorbs hydrogen molecules, where a hydrogen molecule attaches to one oxygen atom with binding energy of similar to 0.13 eV. This implies that the interaction between a hydrogen molecule and the ZnO sheet is stronger than that between a hydrogen molecule and graphene. We predict that each oxygen atom in a ZnO sheet can adsorb two hydrogen molecules on opposite sides of the sheet, and thus the gravimetric density for hydrogen storage on ZnO sheet is evaluated to be about 4.7 wt % at zero temperature. Furthermore, our calculations show that the gravimetric density for hydrogen storage on ZnO sheet reaches 1.5-2.1 wt % at 298 K and 5 MPa. This suggests that, despite their weight, ZnO sheets may have potential applications in hydrogen storage. C1 [Si, H.; Pan, B. C.] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. [Si, H.; Pan, B. C.] Univ Sci & Technol China, Dept Phys, Hefei 230026, Anhui, Peoples R China. [Morris, James R.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Peng, L. J.; Morris, James R.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Pan, BC (reprint author), Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. EM bcpan@ustc.edu.cn RI sriram, dodda/F-1952-2011; Morris, J/I-4452-2012; Pan, Bicai/A-1235-2010 OI Morris, J/0000-0002-8464-9047; FU National Basic Research Program of China [2009CB939901]; U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division FX This work is supported by National Basic Research Program of China (2009CB939901). The HP-LHPC of USTC (University of Science and Technology of China) is acknowledged for computational support. Research was also sponsored by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division (L.J.P. and J.RM.). NR 39 TC 11 Z9 11 U1 5 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 12 PY 2011 VL 115 IS 18 BP 9053 EP 9058 DI 10.1021/jp111394v PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 757ZB UT WOS:000290127200026 ER PT J AU Formo, EV Wu, ZL Mahurin, SM Dai, S AF Formo, Eric V. Wu, Zili Mahurin, Shannon M. Dai, Sheng TI In Situ High Temperature Surface Enhanced Raman Spectroscopy for the Study of Interface Phenomena: Probing a Solid Acid on Alumina SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DIFFUSE-REFLECTANCE SPECTROSCOPY; ATOMIC LAYER DEPOSITION; METAL-OXIDE CATALYSTS; VIBRATIONAL INVESTIGATIONS; STRUCTURAL DETERMINATION; KEGGIN STRUCTURE; VANADIUM-OXIDE; MOLYBDENUM(VI); DFT; UV AB Herein, we utilize surface enhanced Raman spectroscopy (SERS) for the in situ analyses of catalyst structure while operating at elevated temperatures in various atmospheres. In order to accomplish this, robust SERS substrates were generated by depositing an ultrathin protective coating of alumina on top of silver nanowires (NWs) via atomic layer deposition (ALD). In situ studies were then conducted by analyzing the effects of heating a solid acid, phosphotungstic nioa acid (PTA), on the alumina surface in either an oxygen or hydrogen environment at temperatures up to 400 degrees C. Interestingly, the distance-dependent decay of the enhancement factor of the SERS signal from the underlying NWs allowed us to probe with great detail the interfacial region between the PTA and the alumina surface. The ability to analyze the area closest to the alumina surface was further confirmed by assembling vanadia onto the substrate and monitoring the intensity differences between the V - O Al and outer V = O bonds. C1 [Formo, Eric V.; Wu, Zili; Dai, Sheng] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Wu, Zili; Mahurin, Shannon M.; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Wu, ZL (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM wuzl@ornl.gov; dais@ornl.gov RI Wu, Zili/F-5905-2012; Dai, Sheng/K-8411-2015 OI Wu, Zili/0000-0002-4468-3240; Dai, Sheng/0000-0002-8046-3931 FU Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy [DE-AC05-00OR22725] FX This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at the Oak Ridge National Laboratory by the Office of Basic Energy Sciences, U.S. Department of Energy. Further, a portion of this research, performed by Shannon M. Mahurin, was conducted through The Division of Chemical Sciences, Office of Basic Energy Sciences, U.S. Department of Energy. XPS measurements were conducted using the SHaRE facilities, sponsored at Oak Ridge National Laboratory by the Office of Basic Energy Sciences, U.S. Department of Energy. The research was supported in part by the appointment of E. V. Formo to the ORNL Postdoctoral Research Associates Program, administered jointly by ORNL and the Oak Ridge Associated Universities. The Oak Ridge National Laboratory is managed by UT-Battelle, LLC for the U.S. Department of Energy under contract DE-AC05-00OR22725. NR 32 TC 10 Z9 10 U1 5 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 12 PY 2011 VL 115 IS 18 BP 9068 EP 9073 DI 10.1021/jp1119525 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 757ZB UT WOS:000290127200028 ER PT J AU Botiz, I Schaller, RD Verduzco, R Darling, SB AF Botiz, Ioan Schaller, Richard D. Verduzco, Rafael Darling, Seth B. TI Optoelectronic Properties and Charge Transfer in Donor-Acceptor All-Conjugated Diblock Copolymers SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID POLYMER SOLAR-CELLS; LIGHT-EMITTING-DIODES; COIL BLOCK-COPOLYMER; RADICAL POLYMERIZATION; REGIOREGULAR POLY(3-HEXYLTHIOPHENE); PHOTOVOLTAIC APPLICATIONS; POLYFLUORENE COPOLYMER; ORGANIC SEMICONDUCTORS; SIDE-CHAINS; BAND-GAP AB All-conjugated block copolymers, which can self-assemble into well-ordered morphologies, provide exciting opportunities to rationally design and control the nanoscale organization of electron-donor and electron-acceptor moieties in optoelectronic active layers. Here we report on the steady-state and time-resolved optical characterization of block copolymer films and solutions containing poly(3-hexylthiophene) as the donor block and poly(9,9-dioctylfluorene) with and without copolymerization with benzothiadiazole as the acceptor block. Transient absorption measurements suggest rapid charge transfer occurs in both systems, with higher efficiency observed in the latter composition. These results indicate that this class of materials has promise in preparing highly ordered bulk heterojunction all-polymer organic photovoltaic devices. C1 [Botiz, Ioan; Schaller, Richard D.; Darling, Seth B.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Schaller, Richard D.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Verduzco, Rafael] Rice Univ, Dept Chem & Biomol Engn, Houston, TX 77005 USA. RP Darling, SB (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. EM darling@anl.gov RI Botiz, Ioan/I-3209-2012 OI Botiz, Ioan/0000-0002-8555-1084 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Welch Foundation [C-1750]; Louis Owen Foundation; Rice University School of Engineering; Oak Ridge National Laboratory; U.S. Department of Energy FX I.B. and S.B.D. thank Yu-Chih Tseng for stimulating discussions. Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. R.V. acknowledges financial support from the Welch Foundation (Grant # C-1750), the Louis Owen Foundation, and Rice University School of Engineering start-up funds. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, U.S. Department of Energy. NR 81 TC 45 Z9 45 U1 2 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 12 PY 2011 VL 115 IS 18 BP 9260 EP 9266 DI 10.1021/jp201344p PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 757ZB UT WOS:000290127200051 ER PT J AU DeFusco, A Ivanic, J Schmidt, MW Gordon, MS AF DeFusco, Albert Ivanic, Joseph Schmidt, Michael W. Gordon, Mark S. TI Solvent-Induced Shifts in Electronic Spectra of Uracil SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID FRAGMENT POTENTIAL METHOD; ASTERISK EXCITED-STATE; REACTION FIELD-THEORY; NUCLEIC-ACID BASES; CONFIGURATION-INTERACTION; CONICAL INTERSECTIONS; PERTURBATION-THEORY; MOLECULAR-DYNAMICS; AQUEOUS-SOLUTION; PI-ASTERISK AB Highly accurate excitation spectra are predicted for the low-lying n-pi* and pi-pi* states of uracil for both the gas phase and in water employing the complete active space self-consistent field (CASSCF) and multiconfigurational quaside-generate perturbation theory (MCQDPT) methods. Implementation of the effective fragment potential (EFP) solvent method with CASSCF and MCQDPT enables the prediction of highly accurate solvated spectra, along with a direct interpretation of solvent shifts in terms of intermolecular interactions between solvent and solute. Solvent shifts of the n-pi* and pi-pi* ye excited states arise mainly from a change in the electrostatic interaction between solvent and solute upon photoexcitation. Polarization (induction) interactions contribute about 0.1 eV to the solvent-shifted excitation. The blue shift of the n-pi* state is found to be 0.43 eV and the red shift of the pi-pi* state is found to be -0.26 eV. Furthermore, the spectra show that in solution the pi-pi* state is 0.4 eV lower in energy than the n-pi* state. C1 [DeFusco, Albert; Schmidt, Michael W.; Gordon, Mark S.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [DeFusco, Albert; Schmidt, Michael W.; Gordon, Mark S.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Ivanic, Joseph] NCI, Adv Biomed Comp Ctr, Informat Syst Program, SAIC Frederick Inc, Frederick, MD 21702 USA. RP Gordon, MS (reprint author), Iowa State Univ, Dept Chem, Ames, IA 50011 USA. EM mark@si.msg.chem.iastate.edu FU National Science Foundation; Department of Energy FX This work was supported in part by a National Science Foundation Petascale Applications grant and in part by a Department of Energy Computational and Theoretical Chemistry grant. NR 57 TC 37 Z9 37 U1 2 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 12 PY 2011 VL 115 IS 18 BP 4574 EP 4582 DI 10.1021/jp112230f PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 757YZ UT WOS:000290126900002 PM 21491886 ER PT J AU Koh, CJ Liu, CL Harmon, CW Strasser, D Golan, A Kostko, O Chambreau, SD Vaghjiani, GL Leone, SR AF Koh, Christine J. Liu, Chen-Lin Harmon, Christopher W. Strasser, Daniel Golan, Amir Kostko, Oleg Chambreau, Steven D. Vaghjiani, Ghanshyam L. Leone, Stephen R. TI Soft Ionization of Thermally Evaporated Hypergolic Ionic Liquid Aerosols SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID VACUUM-ULTRAVIOLET PHOTOIONIZATION; MASS-SPECTROMETRY; GAS-PHASE; SOLAR-CELLS; VAPORIZATION; NANOPARTICLES; ELECTROLYTES; CONDUCTIVITY; VOLATILITY; VAPOR AB Isolated ion pairs of a conventional ionic liquid, 1-Ethyl-3-Methyl-Imidazolium Bis(trifluoromethylsulfonyl)imide ([Emim(+)]-[Tf2N-]), and a reactive hypergolic ionic liquid, 1-Butyl-3-Methyl-Imidazolium Dicyanamide ([Bmim(+)][Dca(-)]), are generated by vaporizing ionic liquid submicrometer aerosol particles for the first time; the vaporized species are investigated by dissociative ionization with tunable vacuum ultraviolet (VUV) light, exhibiting clear intact cations, Emim(+) and Bmim(+), presumably originating from intact ion pairs. Mass spectra of ion pair vapor from an effusive source of the hypergolic ionic liquid show substantial reactive decomposition due to the internal energy of the molecules emanating from the source. Photoionization efficiency curves in the near ionization region of isolated ion pairs of [Emim(+)][Tf2N-] ionic liquid vapor are compared for an aerosol source and an effusive source, revealing changes in the appearance energy due to the amount of internal energy in the ion pairs. The aerosol source has a shift to higher threshold energy (similar to 0.3 eV), attributed to reduced internal energy of the isolated ion pairs. The method of ionic liquid submicrometer aerosol particle vaporization, for reactive ionic liquids such as hypergolic species, is a convenient, thermally "cooler" source of isolated intact ion pairs in the gas phase compared to effusive sources. C1 [Koh, Christine J.; Strasser, Daniel; Leone, Stephen R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Koh, Christine J.; Strasser, Daniel; Leone, Stephen R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Liu, Chen-Lin; Harmon, Christopher W.; Golan, Amir; Kostko, Oleg; Leone, Stephen R.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Chambreau, Steven D.] ERC Inc, Edwards AFB, CA 93524 USA. [Vaghjiani, Ghanshyam L.] USAF, Res Lab, Edwards AFB, CA 93524 USA. RP Leone, SR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM srl@berkeley.edu RI Kostko, Oleg/B-3822-2009 OI Kostko, Oleg/0000-0003-2068-4991 FU U.S. Air Force Office of Scientific Research [FA9550-10-1-0163, FA9300-06-C-0023]; Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors gratefully acknowledge funding from the U.S. Air Force Office of Scientific Research for supporting C.J.K, D.S., and S.R.L. (Grant No. FA9550-10-1-0163), and for S.D.C. and G.L.V. (Grant No. FA9300-06-C-0023). This work at the ALS was supported by the Director, Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 (C.-L.L., C.W.H., A.G., OK, and S.R.L.). The authors thank Dr. Musahid Ahmed and Dr. Kevin Wilson of the Chemical Dynamics beamline for help in the measurements. NR 45 TC 14 Z9 14 U1 1 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 12 PY 2011 VL 115 IS 18 BP 4630 EP 4635 DI 10.1021/jp200633b PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 757YZ UT WOS:000290126900009 PM 21506546 ER PT J AU Shkrob, IA AF Shkrob, Ilya A. TI General Impossibility to "Prescribe" Diffusion for a Geminate Pair in a Central Force Field and Peculiarities of Geminate Dynamics in Ionic Liquids SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID SMOLUCHOWSKI EQUATION; ULTRAFAST DYNAMICS; RECOMBINATION; PHOTODETACHMENT AB Given the difficulty of obtaining analytical solutions for the diffusion of interacting geminate pairs of (ion) radicals in liquids, it is common, following the original treatment of Mozumder, to "prescribe" this diffusion. A demonstration is given that such a prescription is impossible for any interaction potential other than the Coulomb potential. This demonstration suggests the inadequacy of this common approach to modeling geminate pair and spur dynamics in the largest emerging class of organic solvents: room-temperature ionic liquids. C1 Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Shkrob, IA (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM shkrob@anl.gov FU US-DOE Office of Science, Division of Chemical Sciences, Geosciences and Biosciences [DE-AC02-06CH11357] FX The author thanks A. Mozumder, G. Wipff, and A. F. Wagner for stimulating discussions. This work was supported by the US-DOE Office of Science, Division of Chemical Sciences, Geosciences and Biosciences under Contracts Nos. DE-AC02-06CH11357. Programmatic support via the DOE SISGR "An Integrated Basic Research Program for Advanced Nuclear Energy Separations Systems Based on Ionic Liquids" is gratefully acknowledged. NR 19 TC 0 Z9 0 U1 0 U2 3 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 12 PY 2011 VL 115 IS 18 BP 4636 EP 4639 DI 10.1021/jp201461b PG 4 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 757YZ UT WOS:000290126900010 PM 21504172 ER PT J AU Atta-Fynn, R Bylaska, EJ Schenter, GK de Jong, WA AF Atta-Fynn, Raymond Bylaska, Eric J. Schenter, Gregory K. de Jong, Wibe A. TI Hydration Shell Structure and Dynamics of Curium(III) in Aqueous Solution: First Principles and Empirical Studies SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID NORM-CONSERVING PSEUDOPOTENTIALS; LOCALIZED WANNIER FUNCTIONS; ABSORPTION FINE-STRUCTURE; MOLECULAR-DYNAMICS; WATER-EXCHANGE; CANONICAL ENSEMBLE; LANTHANIDE IONS; SIMULATIONS; CM(III); SPECTRA AB Results of ab initio molecular dynamics (AIMD), quantum mechanics/molecular mechanics (QM/MM), and classical molecular dynamics (CMD) simulations of Cm(3+) in liquid water at a temperature of 300 K are reported. The AIMD simulation was based on the Car-Parrinello MD scheme and GGA-PBE formulation of density functional theory. Two QM/MM simulations were performed by treating Cm(3+) and the water molecules in the first shell quantum mechanically using the PBE (QM/MM-PBE) and the hybrid PBE0 density functionals (QM/MM-PBE0). Two CMD simulations were carried out using ab initio derived pair plus three-body potentials (CMD-3B) and empirical Lennard-Jones pair potential (CMD-LJ). The AIMD and QM/MM-PBE simulations predict average first shell hydration numbers of 8, both of which disagree with recent experimental EXAFS and TRLFS value of 9. On the other hand, the average first shell hydration numbers obtained in the QM/MM-PBE0 and CMD simulations was 9, which agrees with experiment. All the simulations predicted an average first shell and second shell Cm-O bond distance of 2.49-2.53 angstrom and 4.67-4.75 angstrom respectively, both of which are in fair agreement with corresponding experimental values of 2.45-2.48 and 4.65 angstrom. The geometric arrangement of the 8-fold and 9-fold coordinated first shell structures corresponded to the square antiprism and tricapped trigonal prisms, respectively. The second shell hydration number for AIMD QM/MM-PBE, QM/MM-PBE0, CMD-3B, and CMD-LJ, were 15.8, 17.2, 17.7, 17.4, and 16.4 respectively, which indicates second hydration shell overcoordination compared to a recent EXAFS experimental value of 13. Save the EXAFS spectra CMD-LJ simulation, all the computed EXAFS spectra agree fairly well with experiment and a clear distinction could not be made between configurations with 8-fold and 9-fold coordinated first shells. The mechanisms responsible for the first shell associative and dissociative ligand exchange in the classical simulations have been analyzed. The first shell mean residence time was predicted to be on the nanosecond time scale. The computed diffusion constants of Cm(3+) and water are in good agreement with experimental data. C1 [Atta-Fynn, Raymond; Bylaska, Eric J.; de Jong, Wibe A.] Pacific NW Natl Lab, WR Wiley Environm Mol Sci Lab, Richland, WA 99352 USA. [Schenter, Gregory K.] Pacific NW Natl Lab, Chem & Mat Sci Div, Richland, WA 99352 USA. RP Atta-Fynn, R (reprint author), Pacific NW Natl Lab, WR Wiley Environm Mol Sci Lab, POB 999, Richland, WA 99352 USA. EM raymond.attafynn@pnl.gov RI DE JONG, WIBE/A-5443-2008; Schenter, Gregory/I-7655-2014; Atta-Fynn, Raymond/G-1526-2016 OI DE JONG, WIBE/0000-0002-7114-8315; Schenter, Gregory/0000-0001-5444-5484; Atta-Fynn, Raymond/0000-0002-1389-9540 FU U.S. Department of Energy's Office of Biological and Environmental Research and located at the Pacific Northwest National Laboratory; BES Heavy Element Chemistry program; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy FX R.A.-F. would like to thank D. F. Johnson and C. Mundy for stimulating discussions and N. Govind for technical help. The authors would like to acknowledge Patrick Nichols for providing the initial pseudopotential for Cm3+ and L. Soderholm and her group for graciously making the experimental EXAFS data available to us. This research was performed using the Molecular Science Computing Capability in the William R. Wiley Environmental Molecular Science Laboratory, a national scientific user facility sponsored by the U.S. Department of Energy's Office of Biological and Environmental Research and located at the Pacific Northwest National Laboratory, operated for the Department of Energy by Battelle. This work was supported by the BES Heavy Element Chemistry program and the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. NR 69 TC 29 Z9 30 U1 4 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 12 PY 2011 VL 115 IS 18 BP 4665 EP 4677 DI 10.1021/jp201043f PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 757YZ UT WOS:000290126900014 PM 21500828 ER PT J AU Dupuis, M Chen, ST Raugei, S DuBois, DL Bullock, RM AF Dupuis, Michel Chen, Shentan Raugei, Simone DuBois, Daniel L. Bullock, R. Morris TI Comment on "New Insights in the Electrocatalytic Proton Reduction and Hydrogen Oxidation by Bioinspired Catalysts: A DFT Investigation" SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID MOLECULAR CATALYSTS; H-2 OXIDATION; COMPLEXES; ENERGIES; MODEL; 2ND AB In the title paper, Vetere et al. reported a computational investigation of the mechanism of H(2) oxidation/proton reduction using a model of nickel-based electrocatalysts that incorporates pendant amines in cyclic phosphorus ligands. These catalysts are attracting considerable attention owing to their high turnover rates and relatively low overpotentials. These authors interpreted the results of their calculations as evidence for a symmetric bond cleavage of H2 leading directly to two protonated amines in concert with a two-electron reduction of the Ni(II) site to form a Ni(0) diproton state. Proton reduction would involve a reverse symmetric bond formation. We report here an analysis that refutes the interpretation by these authors. We give, for the same model system, the structure of a heterolytic cleavage transition state consistent with the presence of the Ni(II) center acting as a Lewis acid and the pendant amines acting as Lewis bases. We present the associated intrinsic reaction coordinate (IRC) pathway connecting the dihydrogen (eta(2)-H(2)) adduct and a hydride-proton state. We report also the transition state and associated IRC for the proton rearrangement from a hydride-proton state to a diproton state. Finally, we complete the characterization of the transition state reported by Vetere et al. through a determination of the corresponding IRC. In summary, H2 oxidation/proton reduction with this class of catalysts involves a heterolytic bond breaking/formation. C1 [Dupuis, Michel; Chen, Shentan; Raugei, Simone; DuBois, Daniel L.; Bullock, R. Morris] Pacific NW Natl Lab, Ctr Mol Electrocatalysis, Chem & Mat Sci Div, Richland, WA 99352 USA. RP Dupuis, M (reprint author), Pacific NW Natl Lab, Ctr Mol Electrocatalysis, Chem & Mat Sci Div, Richland, WA 99352 USA. RI chen, shentan/H-4924-2011; Bullock, R. Morris/L-6802-2016 OI Bullock, R. Morris/0000-0001-6306-4851 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; U.S. Department of Energy [DE-AC06-76RLO 1830]; Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory; National Energy Research Scientific Computing Center (NERSC) at Lawrence Berkeley National Laboratory FX This research was carried out in the Center for Molecular Electrocatalysis, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Pacific Northwest National Laboratory is operated for the U.S. Department of Energy by Battelle under Contract No. DE-AC06-76RLO 1830. Computational resources were provided at W. R. Wiley Environmental Molecular Science Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory and the National Energy Research Scientific Computing Center (NERSC) at Lawrence Berkeley National Laboratory. NR 17 TC 22 Z9 22 U1 0 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 12 PY 2011 VL 115 IS 18 BP 4861 EP 4865 DI 10.1021/jp111479z PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 757YZ UT WOS:000290126900034 PM 21504191 ER PT J AU Galardini, M Mengoni, A Brilli, M Pini, F Fioravanti, A Lucas, S Lapidus, A Cheng, JF Goodwin, L Pitluck, S Land, M Hauser, L Woike, T Mikhailova, N Ivanova, N Daligault, H Bruce, D Detter, C Tapia, R Han, C Teshima, H Mocali, S Bazzicalupo, M Biondi, EG AF Galardini, Marco Mengoni, Alessio Brilli, Matteo Pini, Francesco Fioravanti, Antonella Lucas, Susan Lapidus, Alla Cheng, Jan-Fang Goodwin, Lynne Pitluck, Samuel Land, Miriam Hauser, Loren Woike, Tanja Mikhailova, Natalia Ivanova, Natalia Daligault, Hajnalka Bruce, David Detter, Chris Tapia, Roxanne Han, Cliff Teshima, Hazuki Mocali, Stefano Bazzicalupo, Marco Biondi, Emanuele G. TI Exploring the symbiotic pangenome of the nitrogen-fixing bacterium Sinorhizobium meliloti SO BMC GENOMICS LA English DT Article DE Sinorhizobium meliloti nodulation; symbiosis; comparative genomics; pangenome; panregulon ID RHIZOBIUM-LEGUMINOSARUM; COMPARATIVE GENOMICS; SEQUENCE-ANALYSIS; PAN-GENOME; NODULATION; GENES; IDENTIFICATION; BIOSYNTHESIS; RECOGNITION; TRANSPORTER AB Background: Sinorhizobium meliloti is a model system for the studies of symbiotic nitrogen fixation. An extensive polymorphism at the genetic and phenotypic level is present in natural populations of this species, especially in relation with symbiotic promotion of plant growth. AK83 and BL225C are two nodule-isolated strains with diverse symbiotic phenotypes; BL225C is more efficient in promoting growth of the Medicago sativa plants than strain AK83. In order to investigate the genetic determinants of the phenotypic diversification of S. meliloti strains AK83 and BL225C, we sequenced the complete genomes for these two strains. Results: With sizes of 7.14 Mbp and 6.97 Mbp, respectively, the genomes of AK83 and BL225C are larger than the laboratory strain Rm1021. The core genome of Rm1021, AK83, BL225C strains included 5124 orthologous groups, while the accessory genome was composed by 2700 orthologous groups. While Rm1021 and BL225C have only three replicons (Chromosome, pSymA and pSymB), AK83 has also two plasmids, 260 and 70 Kbp long. We found 65 interesting orthologous groups of genes that were present only in the accessory genome, consequently responsible for phenotypic diversity and putatively involved in plant-bacterium interaction. Notably, the symbiosis inefficient AK83 lacked several genes required for microaerophilic growth inside nodules, while several genes for accessory functions related to competition, plant invasion and bacteroid tropism were identified only in AK83 and BL225C strains. Presence and extent of polymorphism in regulons of transcription factors involved in symbiotic interaction were also analyzed. Our results indicate that regulons are flexible, with a large number of accessory genes, suggesting that regulons polymorphism could also be a key determinant in the variability of symbiotic performances among the analyzed strains. Conclusions: In conclusions, the extended comparative genomics approach revealed a variable subset of genes and regulons that may contribute to the symbiotic diversity. C1 [Galardini, Marco; Mengoni, Alessio; Pini, Francesco; Fioravanti, Antonella; Bazzicalupo, Marco; Biondi, Emanuele G.] Univ Florence, Dept Evolutionary Biol, I-50125 Florence, Italy. [Brilli, Matteo] Univ Lyon 1, CNRS, Lab Biometrie & Biol Evolut, UMR 5558, F-69365 Lyon, France. [Lucas, Susan; Cheng, Jan-Fang; Pitluck, Samuel; Woike, Tanja; Mikhailova, Natalia; Ivanova, Natalia; Daligault, Hajnalka; Bruce, David; Detter, Chris; Tapia, Roxanne; Han, Cliff; Teshima, Hazuki] Joint Genome Inst, DOE, Walnut Creek, CA USA. [Lapidus, Alla] Fox Chase Canc Ctr, Philadelphia, PA 19111 USA. [Goodwin, Lynne] Los Alamos Natl Lab, Los Alamos, NM USA. [Land, Miriam; Hauser, Loren] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Mocali, Stefano] Agrobiol & Pedol Ctr ABP, Agr Res Council, I-50121 Florence, Italy. [Biondi, Emanuele G.] CNRS, Interdisciplinary Res Inst, Villenenuve Dascq, France. RP Mengoni, A (reprint author), Univ Florence, Dept Evolutionary Biol, Via Romana 17, I-50125 Florence, Italy. EM alessio.mengoni@unifi.it RI Brilli, Matteo/F-4674-2011; Galardini, Marco/F-7610-2011; Hauser, Loren/H-3881-2012; Mengoni, Alessio/G-5336-2013; Lapidus, Alla/I-4348-2013; Land, Miriam/A-6200-2011; Pini, Francesco/E-9630-2015; OI Lapidus, Alla/0000-0003-0427-8731; Land, Miriam/0000-0001-7102-0031; Pini, Francesco/0000-0001-5323-8395; Mocali, Stefano/0000-0002-1173-7206; Mengoni, Alessio/0000-0002-1265-8251; Brilli, Matteo/0000-0001-9891-4617; Galardini, Marco/0000-0003-2018-8242 FU Office of Science of the U.S. Department of Energy, Office of Science [796808, DE-AC02-05CH11231]; Italian Ministry of Research [TCKNJL] FX This work was supported by the Office of Science of the U.S. Department of Energy, Office of Science, project number 796808 under Contract No. DE-AC02-05CH11231. Additional founding was provided by the Italian Ministry of Research (PRIN 2008 research grant contract No. TCKNJL, "Il pangenoma di Sinorhizobium meliloti: L'uso della genomica per il miglioramento agronomico dell'erba medica"). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 69 TC 44 Z9 44 U1 1 U2 28 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD MAY 12 PY 2011 VL 12 AR 235 DI 10.1186/1471-2164-12-235 PG 15 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA 781NQ UT WOS:000291940500001 PM 21569405 ER PT J AU Du Frane, WL Stern, LA Weitemeyer, KA Constable, S Pinkston, JC Roberts, JJ AF Du Frane, Wyatt L. Stern, Laura A. Weitemeyer, Karen A. Constable, Steven Pinkston, John C. Roberts, Jeffery J. TI Electrical properties of polycrystalline methane hydrate SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID GAS HYDRATE; SEA-FLOOR; SEDIMENTS; OLIVINE; ICE AB Electromagnetic (EM) remote-sensing techniques are demonstrated to be sensitive to gas hydrate concentration and distribution and complement other resource assessment techniques, particularly seismic methods. To fully utilize EM results requires knowledge of the electrical properties of individual phases and mixing relations, yet little is known about the electrical properties of gas hydrates. We developed a pressure cell to synthesize gas hydrate while simultaneously measuring in situ frequency-dependent electrical conductivity (sigma). Synthesis of methane (CH(4)) hydrate was verified by thermal monitoring and by post run cryogenic scanning electron microscope imaging. Impedance spectra (20 Hz to 2 MHz) were collected before and after synthesis of polycrystalline CH(4) hydrate from polycrystalline ice and used to calculate s. We determined the sigma of CH(4) hydrate to be 5 x 10(-5) S/m at 0 degrees C with activation energy (E(a)) of 30.6 kJ/mol (-15 to 15 degrees C). After dissociation back into ice, sigma measurements of samples increased by a factor of similar to 4 and E(a) increased by similar to 50%, similar to the starting ice samples. Citation: Du Frane, W. L., L. A. Stern, K. A. Weitemeyer, S. Constable, J. C. Pinkston, and J. J. Roberts (2011), Electrical properties of polycrystalline methane hydrate, Geophys. Res. Lett., 38, L09313, doi:10.1029/2011GL047243. C1 [Du Frane, Wyatt L.; Roberts, Jeffery J.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Stern, Laura A.; Pinkston, John C.] US Geol Survey, Menlo Pk, CA 94025 USA. [Weitemeyer, Karen A.; Constable, Steven] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA. RP Du Frane, WL (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. EM dufrane2@llnl.gov RI Constable, Steven/B-8959-2008; Du Frane, Wyatt/D-6879-2013 FU DOE [DE-NT0005668]; USGS Gas Hydrates [DE-NT0006147]; U.S. Department of Energy; LLNL [DE-AC52-07NA27344] FX The authors thank W. Durham (MIT) and D. Lockner, W. Waite, and S. Kirby (USGS) for helpful discussions and advice, and J. Lemire (SIO) for help with the cell fabrication and design. We also thank R. Evans (WHOI) and another anonymous reviewer. Support for this work was provided by DOE contract DE-NT0005668. Partial support was also provided by Interagency Agreement DE-NT0006147 between the USGS Gas Hydrates Project and the U.S. Department of Energy's Methane Hydrates R&D Program. Prepared by LLNL under contract DE-AC52-07NA27344. NR 25 TC 5 Z9 5 U1 0 U2 8 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAY 11 PY 2011 VL 38 AR L09313 DI 10.1029/2011GL047243 PG 5 WC Geosciences, Multidisciplinary SC Geology GA 764IR UT WOS:000290623600004 ER PT J AU Bradshaw, DH Di Rosa, MD AF Bradshaw, Douglas H. Di Rosa, Michael D. TI Vacuum field energy and spontaneous emission in anomalously dispersive cavities SO PHYSICAL REVIEW A LA English DT Article ID GRAVITATIONAL-WAVE DETECTORS; DIELECTRIC MEDIA; QUANTIZATION; PROPAGATION AB Anomalously dispersive cavities, particularly white-light cavities, may have larger bandwidth to finesse ratios than their normally dispersive counterparts. Partly for this reason, they have been proposed for use in laser interferometer gravitational-wave observatory (LIGO)-like gravity-wave detectors and in ring-laser gyroscopes. In this paper we analyze the quantum noise associated with anomalously dispersive cavity modes. The vacuum field energy associated with a particular cavity mode is proportional to the cavity-averaged group velocity of that mode. For anomalously dispersive cavities with group index values between 1 and 0, this means that the total vacuum field energy associated with a particular cavity mode must exceed h omega/2. For white-light cavities in particular, the group index approaches zero and the vacuum field energy of a particular spatial mode may be significantly enhanced. We predict enhanced spontaneous emission rates into anomalously dispersive cavity modes and broadened laser linewidths when the linewidth of intracavity emitters is broader than the cavity linewidth. C1 [Bradshaw, Douglas H.; Di Rosa, Michael D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Bradshaw, DH (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM bradshaw@lanl.gov FU Los Alamos Laboratory FX We would like to thank Ivan Deutsch, Peter Milonni, and Karen Tate for help in the development of this work. In addition, we express gratitude for a Los Alamos Laboratory Directed Research and Development grant, which funded much of this work. NR 29 TC 3 Z9 3 U1 0 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD MAY 11 PY 2011 VL 83 IS 5 AR 053816 DI 10.1103/PhysRevA.83.053816 PG 9 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 762KU UT WOS:000290476900005 ER PT J AU Fan, C Ren, Y Liu, CT Liaw, PK Yan, HG Egami, T AF Fan, C. Ren, Y. Liu, C. T. Liaw, P. K. Yan, H. G. Egami, T. TI Atomic migration and bonding characteristics during a glass transition investigated using as-cast Zr-Cu-Al SO PHYSICAL REVIEW B LA English DT Article ID SUPERCOOLED LIQUIDS; METALLIC GLASSES; TEMPERATURE AB The glass transition involves only a minor change in the internal energy, and yet the physical and mechanical properties of the glass change dramatically. Atomic bonding behavior is critical to understanding these interesting changes. In order to determine the evolution of the atomic structure through the glass transition, we employed in situ synchrotron x-ray scattering measurements as a function of temperature on a model material-Zr-Cu-Al metallic glass. Based upon the study of pair distribution function and the characterization of the free volume in terms of atomic bonding lengths, we found that the relative change of the quantity, Delta N/N (N represents the number of atom pairs), with significantly longer interatomic distances for the nearest atomic pairs, increases abruptly above the glass transition temperature (T-g). These phenomena are interpreted in terms of the tight-bond cluster model developed recently. C1 [Fan, C.; Yan, H. G.] Hunan Univ, Coll Mat Sci & Engn, Changsha 410082, Hunan, Peoples R China. [Ren, Y.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Liu, C. T.] City Univ Hong Kong, Coll Sci & Engn, Kowloon, Hong Kong, Peoples R China. [Liaw, P. K.; Egami, T.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Fan, C (reprint author), Hunan Univ, Coll Mat Sci & Engn, Changsha 410082, Hunan, Peoples R China. EM fan@hnu.edu.cn FU NSFC [50971057]; NSF [DMR-0231320, CMMI-0900271, DMR-0909037]; DOE [W-7405-ENG-36]; Office of Science, Office of Basic Energy Sciences (OBES); US DOE [DE-AC02-CH11357]; Division of Materials Science and Engineering, Office of Basic Energy Sciences, Department of Energy FX C. Fan thanks J. J. Wall for his help in technical discussion. This work was supported by the NSFC (Grant No. 50971057) and benefited by the NSF (Grants No. DMR-0231320, No. CMMI-0900271, and No. DMR-0909037). Use of NPDF at Los Alamos National Lab was supported by DOE Grant No. W-7405-ENG-36 and use of the Advanced Photon Source was supported by the Office of Science, Office of Basic Energy Sciences (OBES), and the US DOE (DE-AC02-CH11357). T. Egami was supported by the Division of Materials Science and Engineering, Office of Basic Energy Sciences, Department of Energy. NR 25 TC 10 Z9 11 U1 1 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 11 PY 2011 VL 83 IS 19 AR 195207 DI 10.1103/PhysRevB.83.195207 PG 6 WC Physics, Condensed Matter SC Physics GA 762LB UT WOS:000290478200003 ER PT J AU Lei, HC Petrovic, C AF Lei, Hechang Petrovic, C. TI Anisotropy in transport and magnetic properties of K0.64Fe1.44Se2 SO PHYSICAL REVIEW B LA English DT Article ID TEMPERATURE-DEPENDENCE; CRITICAL CURRENTS; SUPERCONDUCTIVITY; NBSE2 AB We report a study of the anisotropy in transport and magnetic properties of K0.64Fe1.44Se2.00 single crystals. The anisotropy in resistivity is up by one order of magnitude between 1.8 and 300 K. The magnetic susceptibility exhibits weak temperature dependence in the normal state with no significant anomalies with decreasing temperature. The lower critical fields H-c1 of K0.64Fe1.44Se2.00 are only about 3 Oe and the anisotropy of H-c1,(c)/H-c1,(ab) is about 1. The critical currents for H parallel to ab and H parallel to c are about 10-10(3) A/cm(2), which is smaller than in iron pnictides and in FeTe1-xSex, and nearly isotropic. C1 [Lei, Hechang; Petrovic, C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Lei, HC (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RI Petrovic, Cedomir/A-8789-2009; LEI, Hechang/H-3278-2016 OI Petrovic, Cedomir/0000-0001-6063-1881; FU US Department of Energy (DOE) [DE-AC02-98CH10886]; Center for Emergent Superconductivity; US DOE, Office for Basic Energy Science FX We thank John Warren for help with scanning electron microscopy measurements. The work at Brookhaven National Laboratory is supported by the the US Department of Energy (DOE) under Contract No. DE-AC02-98CH10886 and in part by the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the US DOE, Office for Basic Energy Science. NR 46 TC 36 Z9 36 U1 3 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 11 PY 2011 VL 83 IS 18 AR 184504 DI 10.1103/PhysRevB.83.184504 PG 4 WC Physics, Condensed Matter SC Physics GA 762KW UT WOS:000290477500002 ER PT J AU Morozovska, AN Eliseev, EA Tagantsev, AK Bravina, SL Chen, LQ Kalinin, SV AF Morozovska, A. N. Eliseev, E. A. Tagantsev, A. K. Bravina, S. L. Chen, Long-Qing Kalinin, S. V. TI Thermodynamics of electromechanically coupled mixed ionic-electronic conductors: Deformation potential, Vegard strains, and flexoelectric effect SO PHYSICAL REVIEW B LA English DT Article ID PIEZORESPONSE FORCE MICROSCOPY; INTERCALATION-INDUCED STRESS; FERROELECTRIC THIN-FILMS; CHEMICAL EXPANSION; BATTERY CATHODE; POLARIZATION; TRANSPORT; ELECTROSTRICTION; DIFFUSION; CERAMICS AB Strong coupling among external voltage, electrochemical potentials, concentrations of electronic and ionic species, and strains is a ubiquitous feature of solid statemixed ionic-electronic conductors (MIECs), the materials of choice in devices ranging from electroresistive and memristive elements to ion batteries and fuel cells. Here, we analyze in detail the electromechanical coupling mechanisms and derive generalized bias-concentration-strain equations for MIECs including contributions of concentration-driven chemical expansion, deformation potential, and flexoelectric effect. This analysis is extended toward the bias-induced strains in the uniform and scanning-probe-microscopy-like geometries. Notably, the contribution of the electron-phonon and flexoelectric coupling to the local surface displacement of the mixed ionic-electronic conductor caused by the electric field scanning probe microscope tip has not been considered previously. The developed thermodynamic approach allows evolving the theoretical description of mechanical phenomena induced by the electric fields (electromechanical response) in solid state ionics toward analytical theory and phase-field modeling of the MIECs in different geometries and under varying electrical, chemical, and mechanical boundary conditions. C1 [Morozovska, A. N.; Eliseev, E. A.] Natl Acad Sci Ukraine, Inst Semicond Phys, UA-03028 Kiev, Ukraine. [Eliseev, E. A.] Natl Acad Sci Ukraine, Inst Problems Mat Sci, UA-03142 Kiev, Ukraine. [Tagantsev, A. K.] Ecole Polytech Fed Lausanne, Swiss Fed Inst Technol, Ceram Lab, CH-1015 Lausanne, Switzerland. [Bravina, S. L.] Natl Acad Sci Ukraine, Inst Phys, UA-03028 Kiev, Ukraine. [Chen, Long-Qing] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Kalinin, S. V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Kalinin, S. V.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Morozovska, AN (reprint author), Natl Acad Sci Ukraine, Inst Semicond Phys, 41 Prospekt Nauki, UA-03028 Kiev, Ukraine. EM morozo@i.com.ua; sergei2@ornl.gov RI Tagantsev, Alexander/E-3707-2010; Kalinin, Sergei/I-9096-2012; Chen, LongQing/I-7536-2012 OI Kalinin, Sergei/0000-0001-5354-6152; Chen, LongQing/0000-0003-3359-3781 FU Ukraine State Agency on Science, Innovation and Informatization [UU30/004]; National Science Foundation [DMR-0908718, DMR-0820404]; Materials Science and Engineering Division, Office of Basic Energy Sciences, U.S. DOE; Swiss National Science Foundation FX The authors are grateful to V. Kharton (U. Aveiro) for useful discussions and valuable advice. A.N.M. is very thankful to the referee for important improvements in the paper and calculation details. The research of A.N.M., E. A. E., and L. Q. C. was sponsored in part by the Ukraine State Agency on Science, Innovation and Informatization (Grant No. UU30/004) and the National Science Foundation (Grants No. DMR-0908718 and No. DMR-0820404). This research was supported in part (S. V. K.) by the Materials Science and Engineering Division, Office of Basic Energy Sciences, U.S. DOE. A. K. T. acknowledges the Swiss National Science Foundation for financial support. NR 92 TC 45 Z9 45 U1 2 U2 67 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 11 PY 2011 VL 83 IS 19 AR 195313 DI 10.1103/PhysRevB.83.195313 PG 10 WC Physics, Condensed Matter SC Physics GA 762LB UT WOS:000290478200005 ER PT J AU del-Castillo-Negrete, D Chacon, L AF del-Castillo-Negrete, D. Chacon, L. TI Local and Nonlocal Parallel Heat Transport in General Magnetic Fields SO PHYSICAL REVIEW LETTERS LA English DT Article ID ANISOTROPIC DIFFUSION; LINES AB A novel approach for the study of parallel transport in magnetized plasmas is presented. The method avoids numerical pollution issues of grid-based formulations and applies to integrable and chaotic magnetic fields with local or nonlocal parallel closures. In weakly chaotic fields, the method gives the fractal structure of the devil's staircase radial temperature profile. In fully chaotic fields, the temperature exhibits self-similar spatiotemporal evolution with a stretched-exponential scaling function for local closures and an algebraically decaying one for nonlocal closures. It is shown that, for both closures, the effective radial heat transport is incompatible with the quasilinear diffusion model. C1 [del-Castillo-Negrete, D.; Chacon, L.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP del-Castillo-Negrete, D (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM delcastillod@ornl.gov OI del-Castillo-Negrete, Diego/0000-0001-7183-801X FU Office of Applied Scientific Computing Research; Office of Fusion Energy Sciences of the U. S. Department of Energy at Oak Ridge National Laboratory [DE-AC05-00OR22725] FX This work was sponsored by the Office of Applied Scientific Computing Research and the Office of Fusion Energy Sciences of the U. S. Department of Energy at Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. NR 18 TC 18 Z9 18 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 11 PY 2011 VL 106 IS 19 AR 195004 DI 10.1103/PhysRevLett.106.195004 PG 4 WC Physics, Multidisciplinary SC Physics GA 762KC UT WOS:000290474100013 PM 21668169 ER PT J AU Micklitz, T Levchenko, A AF Micklitz, Tobias Levchenko, Alex TI Thermalization of Nonequilibrium Electrons in Quantum Wires SO PHYSICAL REVIEW LETTERS LA English DT Article ID FERMI LIQUID AB We study the problem of energy relaxation in a one-dimensional electron system. The leading thermalization mechanism is due to three-particle collisions. We show that for the case of spinless electrons in a single channel quantum wire the corresponding collision integral can be transformed into an exactly solvable problem. The latter is known as the Schrodinger equation for a quantum particle moving in a Poschl-Teller potential. The spectrum for the resulting eigenvalue problem allows for bound-state solutions, which can be identified with the zero modes of the collision integral, and a continuum of propagating modes, which are separated by a gap from the bound states. The inverse gap gives the time scale at which counterpropagating electrons thermalize. C1 [Micklitz, Tobias] Free Univ Berlin, Dahlem Ctr Complex Quantum Syst, D-14195 Berlin, Germany. [Micklitz, Tobias] Free Univ Berlin, Inst Theoret Phys, D-14195 Berlin, Germany. [Levchenko, Alex] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Levchenko, Alex] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. RP Micklitz, T (reprint author), Free Univ Berlin, Dahlem Ctr Complex Quantum Syst, D-14195 Berlin, Germany. FU U.S. DOE, Office of Science [DEAC02-06CH11357] FX We are sincerely grateful to K. A. Matveev for discussions which stimulated this project and thank P. Brouwer, A. Imambekov, L. Glazman, A. Kamenev, T. Karzig, F. von Oppen, and Z. Ristivojevic for useful communication. The work at Argonne National Laboratory was supported by the U.S. DOE, Office of Science, under Contract No. DEAC02-06CH11357. NR 24 TC 21 Z9 21 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 11 PY 2011 VL 106 IS 19 AR 196402 DI 10.1103/PhysRevLett.106.196402 PG 4 WC Physics, Multidisciplinary SC Physics GA 762KC UT WOS:000290474100016 PM 21668178 ER PT J AU Grenier, P Alimonti, G Barbero, M Bates, R Bolle, E Borri, M Boscardin, M Buttar, C Capua, M Cavalli-Sforza, M Cobal, M Cristofoli, A Dalla Betta, F Darbo, G Da Via, C Devetak, E DeWilde, B Di Girolamo, B Dobos, D Einsweiler, K Esseni, D Fazio, S Fleta, C Freestone, J Gallrapp, C Garcia-Sciveres, M Gariano, G Gemme, C Giordani, MP Gjersdal, H Grinstein, S Hansen, T Hansen, TE Hansson, P Hasi, J Helle, K Hoeferkamp, M Hugging, F Jackson, P Jakobs, K Kalliopuska, J Karagounis, M Kenney, C Kohler, M Kocian, M Kok, A Kolya, S Korokolov, I Kostyukhin, V Kruger, H La Rosa, A Lai, CH Lietaer, N Lozano, M Mastroberardino, A Micelli, A Nellist, C Oja, A Oshea, V Padilla, C Palestri, P Parker, S Parzefall, U Pater, J Pellegrini, G Pernegger, H Piemonte, C Pospisil, S Povoli, M Roe, S Rohne, O Ronchin, S Rovani, A Ruscino, E Sandaker, H Seidel, S Selmi, L Silverstein, D Sjobaek, K Slavicek, T Stapnes, S Stugu, B Stupak, J Su, D Susinno, G Thompson, R Tsung, JW Tsybychev, D Watts, SJ Wermes, N Young, C Zorzi, N AF Grenier, P. Alimonti, G. Barbero, M. Bates, R. Bolle, E. Borri, M. Boscardin, M. Buttar, C. Capua, M. Cavalli-Sforza, M. Cobal, M. Cristofoli, A. G.-F. Dalla Betta Darbo, G. Da Via, C. Devetak, E. DeWilde, B. Di Girolamo, B. Dobos, D. Einsweiler, K. Esseni, D. Fazio, S. Fleta, C. Freestone, J. Gallrapp, C. Garcia-Sciveres, M. Gariano, G. Gemme, C. Giordani, M. -P. Gjersdal, H. Grinstein, S. Hansen, T. Hansen, T. -E. Hansson, P. Hasi, J. Helle, K. Hoeferkamp, M. Huegging, F. Jackson, P. Jakobs, K. Kalliopuska, J. Karagounis, M. Kenney, C. Koehler, M. Kocian, M. Kok, A. Kolya, S. Korokolov, I. Kostyukhin, V. Krueger, H. La Rosa, A. Lai, C. H. Lietaer, N. Lozano, M. Mastroberardino, A. Micelli, A. Nellist, C. Oja, A. Oshea, V. Padilla, C. Palestri, P. Parker, S. Parzefall, U. Pater, J. Pellegrini, G. Pernegger, H. Piemonte, C. Pospisil, S. Povoli, M. Roe, S. Rohne, O. Ronchin, S. Rovani, A. Ruscino, E. Sandaker, H. Seidel, S. Selmi, L. Silverstein, D. Sjobaek, K. Slavicek, T. Stapnes, S. Stugu, B. Stupak, J. Su, D. Susinno, G. Thompson, R. Tsung, J. -W. Tsybychev, D. Watts, S. J. Wermes, N. Young, C. Zorzi, N. TI Test beam results of 3D silicon pixel sensors for the ATLAS upgrade SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE ATLAS upgrade; Silicon sensors; 3D sensors; Radiation hard detectors ID DETECTORS; TRACKING AB Results on beam tests of 3D silicon pixel sensors aimed at the ATLAS Insertable B-Layer and High Luminosity LHC (HL-LHC) upgrades are presented. Measurements include charge collection, tracking efficiency and charge sharing between pixel cells, as a function of track incident angle, and were performed with and without a 1.6 T magnetic field oriented as the ATLAS inner detector solenoid field. Sensors were bump-bonded to the front-end chip currently used in the ATLAS pixel detector. Full 3D sensors, with electrodes penetrating through the entire wafer thickness and active edge, and double-sided 3D sensors with partially overlapping bias and read-out electrodes were tested and showed comparable performance. (C) 2011 Elsevier B.V. All rights reserved. C1 [Helle, K.; Sandaker, H.; Stugu, B.] Univ Bergen, N-5020 Bergen, Norway. [Barbero, M.; Huegging, F.; Karagounis, M.; Kostyukhin, V.; Krueger, H.; Tsung, J. -W.; Wermes, N.] Univ Bonn, D-5300 Bonn, Germany. [Capua, M.; Fazio, S.; Mastroberardino, A.; Susinno, G.] INFN Grp Collegato Cosenza, Rome, Italy. [Di Girolamo, B.; Dobos, D.; Gallrapp, C.; La Rosa, A.; Pernegger, H.; Roe, S.] CERN, CH-1211 Geneva 23, Switzerland. [Pospisil, S.; Slavicek, T.] Czech Tech Univ, Prague, Czech Republic. [Jakobs, K.; Koehler, M.; Parzefall, U.] Univ Freiburg, D-7800 Freiburg, Germany. [Darbo, G.; Gariano, G.; Gemme, C.; Rovani, A.; Ruscino, E.] INFN Sez Genova, Genoa, Italy. [Bates, R.; Buttar, C.; Oshea, V.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. [Parker, S.] Univ Hawaii, Honolulu, HI 96822 USA. [Cavalli-Sforza, M.; Korokolov, I.; Padilla, C.] IFAE Barcelona, Barcelona, Spain. [Grinstein, S.] ICREA IFAE Barcelona, Barcelona, Spain. [Einsweiler, K.; Garcia-Sciveres, M.] Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Alimonti, G.] INFN Sez Milano, Milan, Italy. [Borri, M.; Da Via, C.; Freestone, J.; Kolya, S.; Lai, C. H.; Nellist, C.; Pater, J.; Thompson, R.; Watts, S. J.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Hoeferkamp, M.; Seidel, S.] Univ New Mexico, Albuquerque, NM 87131 USA. [Bolle, E.; Gjersdal, H.; Rohne, O.; Sjobaek, K.; Stapnes, S.] Univ Oslo, N-0316 Oslo, Norway. [Devetak, E.; DeWilde, B.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Stony Brook, NY USA. [G.-F. Dalla Betta; Povoli, M.] INFN Grp Collegato Trento, Trento, Italy. [G.-F. Dalla Betta; Povoli, M.] DISI Univ Trento, Trento, Italy. [Capua, M.; Fazio, S.; Mastroberardino, A.; Susinno, G.] Univ Calabria, I-87030 Commenda Di Rende, Italy. [Cobal, M.; Cristofoli, A.; Esseni, D.; Giordani, M. -P.; Micelli, A.; Palestri, P.; Selmi, L.] INFN Grp Collegato Udine, Udine, Italy. [Cobal, M.; Cristofoli, A.; Esseni, D.; Giordani, M. -P.; Micelli, A.; Palestri, P.; Selmi, L.] Univ Udine, I-33100 Udine, Italy. [Fleta, C.; Lozano, M.; Pellegrini, G.] CSIC, CNM, IMB, Barcelona, Spain. [Boscardin, M.; Piemonte, C.; Ronchin, S.; Zorzi, N.] FBK Irst, Trento, Italy. [Kalliopuska, J.; Oja, A.] VTT, Espoo, Finland. EM grenier@slac.stanford.edu RI Capua, Marcella/A-8549-2015; O'Shea, Val/G-1279-2010; Fleta, Celeste/D-7303-2014; Pellegrini, Giulio/F-4921-2011; Zorzi, Nicola/M-3141-2014; Grinstein, Sebastian/N-3988-2014; Buttar, Craig/D-3706-2011; Fazio, Salvatore /G-5156-2010; Dalla Betta, Gian-Franco/I-1783-2012; La Rosa, Alessandro/I-1856-2013; Cavalli-Sforza, Matteo/H-7102-2015; Lozano, Manuel/C-3445-2011; Boscardin, Maurizio/A-4420-2014 OI Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; O'Shea, Val/0000-0001-7183-1205; Fleta, Celeste/0000-0002-6591-6744; Pellegrini, Giulio/0000-0002-1606-3546; Zorzi, Nicola/0000-0002-6650-3925; Grinstein, Sebastian/0000-0002-6460-8694; Dalla Betta, Gian-Franco/0000-0001-5516-9282; La Rosa, Alessandro/0000-0001-6291-2142; Lozano, Manuel/0000-0001-5826-5544; FU US Department of Energy FX We are very grateful to the ATLAS test beam coordinator Henric Wilkens, and to the EUDET, CERN SPS and North Area teams for their dedicated support and work. This work was supported in part by the US Department of Energy. NR 19 TC 19 Z9 19 U1 2 U2 11 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAY 11 PY 2011 VL 638 IS 1 BP 33 EP 40 DI 10.1016/j.nima.2011.01.181 PG 8 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 757JZ UT WOS:000290082600006 ER PT J AU Harkness, LJ Boston, AJ Boston, HC Cole, P Cresswell, JR Filmer, F Jones, M Judson, DS Nolan, PJ Oxley, DC Sampson, JA Scraggs, DP Slee, MJ Bimson, WE Kemp, GJ Groves, J Headspith, J Lazarus, I Simpson, J Cooper, RJ AF Harkness, L. J. Boston, A. J. Boston, H. C. Cole, P. Cresswell, J. R. Filmer, F. Jones, M. Judson, D. S. Nolan, P. J. Oxley, D. C. Sampson, J. A. Scraggs, D. P. Slee, M. J. Bimson, W. E. Kemp, G. J. Groves, J. Headspith, J. Lazarus, I. Simpson, J. Cooper, R. J. TI An investigation of the performance of a coaxial HPGe detector operating in a magnetic resonance imaging field SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Germanium detector; Semiconductor; Magnetic field; MRI ID ESCAPE SUPPRESSED SPECTROMETER; POSITRON-EMISSION-TOMOGRAPHY; COMPUTED-TOMOGRAPHY; CAMERA; SYSTEM; HEAD AB Nuclear medical imaging modalities such as positron emission tomography and single photon emission computed tomography are used to probe physiological functions of the body by detecting gamma rays emitted from biologically targeted radiopharmaceuticals. A system which is capable of simultaneous data acquisition for nuclear medical imaging and magnetic resonance imaging is highly sought after by the medical imaging community. Such a device could provide a more complete medical insight into the functions of the body within a well-defined structural context. However, acquiring simultaneous nuclear/MRI sequences are technically challenging due to the conventional photomultiplier tube readout employed by most existing scintillator detector systems. A promising solution is a nuclear imaging device composed of semiconductor detectors that can be operated with a standard MRI scanner. However, the influence of placing a semiconductor detector such as high purity germanium (HPGe) within or close to the bore of an MRI scanner, where high magnetic fields are present, is not well understood. In this paper, the performance of a HPGe detector operating in a high strength static (B(s)) MRI field along with fast switching gradient fields and radiofrequency from the MRI system has been assessed. The influence of the B(s) field on the energy resolution of the detector has been investigated for various positions and orientations of the detector within the magnetic field. The results have then been interpreted in terms of the influence of the B(s) field on the charge collection properties. MRI images have been acquired with the detector situated at the entrance of the MRI bore to investigate the effects of simultaneous data acquisition on detector performance and MRI imaging. (C) 2011 Elsevier B.V. All rights reserved. C1 [Harkness, L. J.; Boston, A. J.; Boston, H. C.; Cole, P.; Cresswell, J. R.; Filmer, F.; Jones, M.; Judson, D. S.; Nolan, P. J.; Oxley, D. C.; Sampson, J. A.; Scraggs, D. P.; Slee, M. J.] Univ Liverpool, Dept Phys, Liverpool L69 7ZE, Merseyside, England. [Bimson, W. E.; Kemp, G. J.] Univ Liverpool, MARIARC, Liverpool L69 3GE, Merseyside, England. [Groves, J.; Headspith, J.; Lazarus, I.; Simpson, J.] STFC Daresbury Lab, Warrington WA4 4AD, Cheshire, England. [Cooper, R. J.] Oak Ridge Natl Lab, Joint Inst Heavy Ion Res, Oak Ridge, TN 37831 USA. RP Harkness, LJ (reprint author), Univ Liverpool, Dept Phys, Liverpool L69 7ZE, Merseyside, England. EM ljh@ns.ph.liv.ac.uk OI Kemp, Graham/0000-0002-8324-9666 FU Science and Technology Facilities Council (STFC); Engineering and Physical Sciences Research Council (EPSRC) FX The authors would like to acknowledge financial support for this work from the Science and Technology Facilities Council (STFC) and the Engineering and Physical Sciences Research Council (EPSRC). NR 25 TC 1 Z9 1 U1 0 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAY 11 PY 2011 VL 638 IS 1 BP 67 EP 73 DI 10.1016/j.nima.2011.02.034 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 757JZ UT WOS:000290082600011 ER PT J AU Bauer, DA Burke, S Cooley, J Crisler, M Cushman, P DeJongh, F Duong, L Ferril, R Golwala, SR Hall, J Holmgren, D Mahapatra, R Nelson, H Reisetter, A Sander, J Savage, C AF Bauer, D. A. Burke, S. Cooley, J. Crisler, M. Cushman, P. DeJongh, F. Duong, L. Ferril, R. Golwala, S. R. Hall, J. Holmgren, D. Mahapatra, R. Nelson, H. Reisetter, A. Sander, J. Savage, C. TI The CDMS II Data Acquisition System SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE DAQ; Data acquisition; CDMS; Dark matter; WIMP; Soudan ID DARK-MATTER SEARCH AB The Data Acquisition System for the CDMS II dark matter experiment was designed and built when the experiment moved to its new underground installation at the Soudan Lab. The combination of remote operation and increased data load necessitated a completely new design. Elements of the original LabView system remained as stand-alone diagnostic programs, but the main data processing moved to a VME-based system with custom electronics for signal conditioning, trigger formation and buffering. The data rate was increased 100-fold and the automated cryogenic system was linked to the data acquisition. A modular server framework with associated user interfaces was implemented in Java to allow control and monitoring of the entire experiment remotely. (C) 2011 Elsevier B.V. All rights reserved. C1 [Cushman, P.; Duong, L.; Reisetter, A.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Golwala, S. R.] CALTECH, Dept Phys, Pasadena, CA 91125 USA. [Bauer, D. A.; Crisler, M.; DeJongh, F.; Hall, J.; Holmgren, D.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Cooley, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Mahapatra, R.; Sander, J.] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Burke, S.; Ferril, R.; Nelson, H.; Savage, C.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. RP Cushman, P (reprint author), Univ Minnesota, Sch Phys & Astron, 116 Church St SE, Minneapolis, MN 55455 USA. EM prisca@physics.umn.edu RI Hall, Jeter/F-6108-2013; OI Holmgren, Donald/0000-0001-6701-7737 NR 3 TC 1 Z9 1 U1 1 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAY 11 PY 2011 VL 638 IS 1 BP 127 EP 133 DI 10.1016/j.nima.2011.02.059 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 757JZ UT WOS:000290082600019 ER PT J AU Huang, XJ Miao, HJ Nelson, J Turner, J Steinbrener, J Shapiro, D Kirz, J Jacobsen, C AF Huang, Xiaojing Miao, Huijie Nelson, Johanna Turner, Joshua Steinbrener, Jan Shapiro, David Kirz, Janos Jacobsen, Chris TI Anti-contamination device for cryogenic soft X-ray diffraction microscopy SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE X-ray Imaging; Cryogenic X-ray microscopy; Diffraction microscopy; Anti-contamination ID BIOLOGICAL SPECIMENS; COMPUTED-TOMOGRAPHY; RESOLUTION; CELLS; YEAST; WHOLE AB Cryogenic microscopy allows one to view frozen hydrated biological and soft matter specimens with good structural preservation and a high degree of stability against radiation damage. We describe a liquid nitrogen-cooled anti-contamination device for cryogenic X-ray diffraction microscopy. The anti-contaminator greatly reduces the buildup of ice layers on the specimen due to condensation of residual water vapor in the experimental vacuum chamber. We show by coherent X-ray diffraction measurements that this leads to fivefold reduction of background scattering, which is important for far-field X-ray diffraction microscopy of biological specimens. Published by Elsevier B.V. C1 [Huang, Xiaojing; Miao, Huijie; Nelson, Johanna; Turner, Joshua; Steinbrener, Jan; Jacobsen, Chris] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Shapiro, David; Kirz, Janos] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. [Jacobsen, Chris] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Jacobsen, Chris] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Huang, XJ (reprint author), UCL, London Ctr Nanotechnol, London WC1H 0AH, England. EM xiaojing.huang@ucl.ac.uk RI Huang, Xiaojing/K-3075-2012; Jacobsen, Chris/E-2827-2015; Nelson Weker, Johanna/J-4159-2015 OI Huang, Xiaojing/0000-0001-6034-5893; Jacobsen, Chris/0000-0001-8562-0353; Nelson Weker, Johanna/0000-0001-6856-3203 FU Division of Materials Sciences and Engineering, Office of Basic Energy Sciences [DE-FG02-07ER46128]; National Institutes for Health [5R21EB6134]; U.S. Department of Energy [DE-AC02-05CH11231] FX We thank the Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, at the Department of Energy for support of X-ray diffraction microscopy methods and instrumentation development under contract DE-FG02-07ER46128. We also thank the National institute for General Medical Services at the National Institutes for Health for support of the application of this method to biological imaging under contract 5R21EB6134. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Finally, we thank Stefano Marchesini and George Meigs of ALS for the fruitful discussions related to this project, and Richard Celestre and Tony Warwick of ALS for help and advice. NR 32 TC 1 Z9 1 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAY 11 PY 2011 VL 638 IS 1 BP 171 EP 175 DI 10.1016/j.nima.2011.02.085 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 757JZ UT WOS:000290082600025 PM 21547016 ER PT J AU Tan, K Lawler, J AF Tan, Kemin Lawler, Jack TI The structure of the Ca2+-binding, glycosylated F-spondin domain of F-spondin - A C2-domain variant in an extracellular matrix protein SO BMC STRUCTURAL BIOLOGY LA English DT Article ID PATTERN-RECOGNITION MOLECULE; CRYSTAL-STRUCTURE; PRECURSOR PROTEIN; FLOOR PLATE; C2 DOMAINS; BINDING; MINDIN; LIGAND; GROWTH; CELLS AB Background: F-spondin is a multi-domain extracellular matrix (ECM) protein and a contact-repellent molecule that directs axon outgrowth and cell migration during development. The reelin_N domain and the F-spondin domain (FS domain) comprise a proteolytic fragment that interacts with the cell membrane and guides the projection of commissural axons to floor plate. The FS domain is found in F-spondins, mindins, M-spondin and amphiF-spondin. Results: We present the crystal structure of human F-spondin FS domain at 1.95 angstrom resolution. The structure reveals a Ca2+-binding C2 domain variant with an 8-stranded antiparallel beta-sandwich fold. Though the primary sequences of the FS domains of F-spondin and mindin are less than 36% identical, their overall structures are very similar. The unique feature of F-spondin FS domain is the presence of three disulfide bonds associated with the N- and C-termini of the domain and a highly conserved N-linked glycosylation site. The integrin-binding motif found in mindin is not conserved in the F-spondin FS domain. Conclusion: The structure of the F-spondin FS domain completes the structural studies of the multiple-domain ECM molecule. The homology of its core structure to a common Ca2+- and lipid-binding C2 domain suggests that the F-spondin FS domain may be responsible for part of the membrane targeting of F-spondin in its regulation of axon development. The structural properties of the FS domain revealed in this study pave the way for further exploration into the functions of F-spondin. C1 [Tan, Kemin] Argonne Natl Lab, Midwest Ctr Struct Genom, Argonne, IL 60439 USA. [Tan, Kemin] Argonne Natl Lab, Struct Biol Ctr, Biosci Div, Argonne, IL 60439 USA. [Lawler, Jack] Beth Israel Deaconess Med Ctr, Dept Pathol, Div Expt Pathol, Boston, MA 02215 USA. [Lawler, Jack] Harvard Univ, Sch Med, Boston, MA 02215 USA. RP Tan, K (reprint author), Argonne Natl Lab, Midwest Ctr Struct Genom, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ktan@anl.gov; jlawler@bidmc.harvard.edu FU National Heart, Lung and Blood Institute of the National Institutes of Health [HL49081] FX This work was support by a grant (HL49081) from the National Heart, Lung and Blood Institute of the National Institutes of Health. The authors wish to thank Mark Duquette for technical assistance, Gekleng Chhor for proofreading, Drs. Hui Lu and Wonhwa Cho of University of Illinois at Chicago for helpful discussion and Drs. Frank Rotella and Marianne Schiffer of Argonne National Laboratory for critical reading of the manuscript. NR 39 TC 2 Z9 3 U1 0 U2 1 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1472-6807 J9 BMC STRUCT BIOL JI BMC Struct. Biol. PD MAY 10 PY 2011 VL 11 AR 22 DI 10.1186/1472-6807-11-22 PG 9 WC Biophysics SC Biophysics GA 779QB UT WOS:000291793500001 PM 21569239 ER PT J AU Lee, JS Kim, YM Kwon, JH Sim, JS Shin, H Sohn, BH Jia, QX AF Lee, Jang-Sik Kim, Yong-Mu Kwon, Jeong-Hwa Sim, Jae Sung Shin, Hyunjung Sohn, Byeong-Hyeok Jia, Quanxi TI Multilevel Data Storage Memory Devices Based on the Controlled Capacitive Coupling of Trapped Electrons SO ADVANCED MATERIALS LA English DT Article ID FIELD-EFFECT TRANSISTORS; THIN-FILM TRANSISTORS; NONVOLATILE MEMORY; FLASH MEMORY; NANOCRYSTAL MEMORIES; ORGANIC ELECTRONICS; LOW-COST; SEMICONDUCTORS; RETENTION; FUTURE AB Multiple data storage memory devices based on the controlled capacitive coupling of trapped electrons are fabricated using highly ordered arrays of metal nanoparticles. Results are presented from metal nanoparticle-based memory devices with controlled nanoparticle charge trapping elements, which undergo gate-voltage-adjustable multilevel memory states. Experimental and theoretical analysis for multilevel data manipulations and visualization of memory states are done on the nanometer scale. C1 [Lee, Jang-Sik; Kim, Yong-Mu; Shin, Hyunjung] Kookmin Univ, Sch Adv Mat Engn, Seoul 136702, South Korea. [Kwon, Jeong-Hwa; Sohn, Byeong-Hyeok] Seoul Natl Univ, Dept Chem, Seoul 151747, South Korea. [Kwon, Jeong-Hwa; Sohn, Byeong-Hyeok] Seoul Natl Univ, NANO Syst Inst, Seoul 151747, South Korea. [Sim, Jae Sung] Samsung Elect Co Ltd, Memory Business, Hwasung City 449711, Kyungki Do, South Korea. [Jia, Quanxi] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Lee, JS (reprint author), Kookmin Univ, Sch Adv Mat Engn, Seoul 136702, South Korea. EM jangsik@kookmin.ac.kr RI Shin, Hyunjung/D-5107-2009; Lee, Jang-Sik/A-6629-2008; Jia, Q. X./C-5194-2008 OI Shin, Hyunjung/0000-0003-1284-9098; Lee, Jang-Sik/0000-0002-1096-1783; FU Korea government (MEST) [2010-0014925, 2010-0015014]; MEST [2008-0059952, 2009-0077593]; ERC, NRF/MEST [R11-2005-048-00000-0]; Korea Ministry of Knowledge Economy; World Gold Council [RP05-06]; NRF [2010-0000039]; NRF/MEST [R0A-2007-000-20105-0] FX J.S.L. is grateful to Prof. Charles M. Lieber for his valuable comments on this manuscript. This work was supported by the National Research Foundation (NRF) grant funded by the Korea government (MEST) (2010-0014925, 2010-0015014). In addition, this work was supported by the NRF grant funded by the MEST (2008-0059952, 2009-0077593), by the ERC program of NRF/MEST (R11-2005-048-00000-0), by the "SystemIC2010" project of Korea Ministry of Knowledge Economy, and by the G.R.O.W. project of World Gold Council (RP05-06). B. H. S. acknowledges the support of NRF (2010-0000039) and S. H. acknowledges the support of the NRF/MEST (R0A-2007-000-20105-0). NR 50 TC 50 Z9 51 U1 5 U2 69 PU WILEY-BLACKWELL PI MALDEN PA COMMERCE PLACE, 350 MAIN ST, MALDEN 02148, MA USA SN 0935-9648 J9 ADV MATER JI Adv. Mater. PD MAY 10 PY 2011 VL 23 IS 18 BP 2064 EP + DI 10.1002/adma.201004150 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 771MY UT WOS:000291164200003 PM 21538583 ER PT J AU Hupalo, M Liu, XJ Wang, CZ Lu, WC Yao, YX Ho, KM Tringides, MC AF Hupalo, Myron Liu, Xiaojie Wang, Cai-Zhuang Lu, Wen-Cai Yao, Yon-Xin Ho, Kai-Ming Tringides, Michael C. TI Metal Nanostructure Formation on Graphene: Weak versus Strong Bonding SO ADVANCED MATERIALS LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; SILICON-CARBIDE; FILMS AB Graphene is an exciting material with numerous potential applications. To understand metal graphene interaction two different metals were studied. Two large Pb islands nucleate at 78K indicating fast diffusion and weak interaction(right). On the contrary, for Dysprosium a high island density is observed confirming slow diffusion and strong interaction(left). C1 [Hupalo, Myron; Liu, Xiaojie; Wang, Cai-Zhuang; Yao, Yon-Xin; Ho, Kai-Ming; Tringides, Michael C.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. [Hupalo, Myron; Liu, Xiaojie; Wang, Cai-Zhuang; Yao, Yon-Xin; Ho, Kai-Ming; Tringides, Michael C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Liu, Xiaojie; Lu, Wen-Cai] Jilin Univ, Inst Theoret Chem, State Key Lab Theoret & Computat Chem, Changchun 130021, Jilin, Peoples R China. [Lu, Wen-Cai] Qingdao Univ, Coll Phys, Qingdao 266071, Shandong, Peoples R China. [Lu, Wen-Cai] Qingdao Univ, Lab Fiber Mat & Modern Text, Growing Base State Key Lab, Qingdao 266071, Shandong, Peoples R China. RP Tringides, MC (reprint author), Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. EM tringides@ameslab.gov RI Yao, Yongxin/B-7320-2008 FU US Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering, National Energy Research Supercomputing Center (NERSC) in Berkeley, CA [DE-AC02-07CH11358]; China Scholarship Council [2009617104]; National Natural Science Foundation of China [20773047, 21043001] FX Work at Ames Laboratory was supported by the US Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering, including a grant of computer time at the National Energy Research Supercomputing Center (NERSC) in Berkeley, CA under Contract No. DE-AC02-07CH11358. X.J.L. acknowledges the support from China Scholarship Council (File NO.2009617104). W. C. L. acknowledges the support by the National Natural Science Foundation of China (Nos. 20773047 and 21043001). NR 29 TC 42 Z9 42 U1 2 U2 46 PU WILEY-BLACKWELL PI MALDEN PA COMMERCE PLACE, 350 MAIN ST, MALDEN 02148, MA USA SN 0935-9648 J9 ADV MATER JI Adv. Mater. PD MAY 10 PY 2011 VL 23 IS 18 BP 2082 EP + DI 10.1002/adma.201100412 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 771MY UT WOS:000291164200006 PM 21432915 ER PT J AU Huang, DM Mauger, SA Friedrich, S George, SJ Dumitriu-LaGrange, D Yoon, S Moule, AJ AF Huang, David M. Mauger, Scott A. Friedrich, Stephan George, Simon J. Dumitriu-LaGrange, Daniela Yoon, Sook Moule, Adam J. TI The Consequences of Interface Mixing on Organic Photovoltaic Device Characteristics SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID HETEROJUNCTION SOLAR-CELLS; LIGHT-EMITTING-DIODES; ENERGY-LEVEL ALIGNMENT; CONJUGATED POLYMERS; THIN-FILMS; MORPHOLOGY; EFFICIENCY; PERFORMANCE; LAYER; POLYTHIOPHENES AB Organic bulk-heterojunction solar cells are being developed as a low-cost alternative to inorganic photovoltaics. A key step to producing high-effi ciency bulk-heterojunction devices is fi lm curing using either heat or a solvent atmosphere. All of the literature examining the curing process have assumed that improvement of the bulk-heterojunction morphology is the reason for the increased fi lling factor, short-circuit current density, and effi ciency following heat or solvent treatment. We show in this article that heat treatment causes the donor polymer (P3HT) and polymer electrode (PEDOT: PSS) to mix physically to form an interface layer. This interface layer is composed of a mixture of P3HT and PSS in which the P3HT is oxidized to P3HT +. This mixed layer affects the open-circuit voltage and compensation voltage by limiting the dark current. This result implies that a simplistic description of the P3HT/PEDOT: PSS contact as a sharp interface between bulk P3HT and bulk PEDOT: PSS cannot adequately capture its electrical characteristics. C1 [Huang, David M.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5005, Australia. [Mauger, Scott A.; Dumitriu-LaGrange, Daniela; Yoon, Sook; Moule, Adam J.] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [Friedrich, Stephan] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [George, Simon J.] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Biol & Environm Xray Facil, Berkeley, CA 94720 USA. RP Huang, DM (reprint author), Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5005, Australia. EM amoule@ucdavis.edu RI Huang, David/E-6830-2010; Moule, Adam/B-9484-2013 OI Huang, David/0000-0003-2048-4500; Moule, Adam/0000-0003-1354-3517 FU US Department of Energy EERE Solar America Initiative [DE-FG36-08GO18018]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was supported by the US Department of Energy EERE Solar America Initiative under Contract No. DE-FG36-08GO18018. The authors thank LANL for neutron reflectometry measurement time at the LANSCE-SPEAR facility and measurement help obtained from Erik Watkins and Jarek Majewski. We thank the ALS for providing beam time. Part of this work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. We also thank Louise Berben for support with GCMS measurements. NR 52 TC 59 Z9 59 U1 0 U2 42 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1616-301X J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD MAY 10 PY 2011 VL 21 IS 9 BP 1657 EP 1665 DI 10.1002/adfm.201002014 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 763CG UT WOS:000290530500015 ER PT J AU Bennartz, R Fan, JW Rausch, J Leung, LR Heidinger, AK AF Bennartz, Ralf Fan, Jiwen Rausch, John Leung, L. Ruby Heidinger, Andrew K. TI Pollution from China increases cloud droplet number, suppresses rain over the East China Sea SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID LIQUID WATER PATH; WINTER MONSOON; STRATOCUMULUS; PRECIPITATION; AEROSOLS; DRIZZLE; CLIMATOLOGY; SYSTEM AB Rapid economic growth over the last 30 years in China has led to a significant increase in aerosol loading, which is mainly due to the increased emissions of its precursors such as SO2 and NOx. Here we show that these changes significantly affect wintertime clouds and precipitation over the East China Sea downwind of major emission sources. Satellite observations show an increase of cloud droplet number concentration from less than 200 cm(-3) in the 1980s to more than 300 cm(-3) in 2005. In the same time period, precipitation frequency reported by voluntary ship observers was reduced from more than 30% to less than 20% of the time. A back trajectory analysis showed the pollution in the investigation area to originate from the Shanghai-Nanjing and Jinan industrial areas. A model sensitivity study was performed, isolating the effects of changes in emissions of the aerosol precursors SO2 and NOx on clouds and precipitation using a state-of-the-art mesocale model including chemistry and aerosol indirect effects. Similar changes in cloud droplet number concentration over the East China Sea were obtained when the current industrial emissions in China were reduced to the 1980s levels. Simulated changes in precipitation were somewhat smaller than the observed changes but still significant. Citation: Bennartz, R., J. Fan, J. Rausch, L. R. Leung, and A. K. Heidinger (2011), Pollution from China increases cloud droplet number, suppresses rain over the East China Sea, Geophys. Res. Lett., 38, L09704, doi: 10.1029/2011GL047235. C1 [Bennartz, Ralf; Rausch, John] Univ Wisconsin, Atmospher & Ocean Sci Dept, Madison, WI 53706 USA. [Fan, Jiwen; Leung, L. Ruby] Pacific NW Natl Lab, Richland, WA 99352 USA. [Heidinger, Andrew K.] NOAA, Ctr Satellite Applicat & Res, NESDIS, Camp Springs, MD 20746 USA. RP Bennartz, R (reprint author), Univ Wisconsin, Atmospher & Ocean Sci Dept, 1225 W Dayton St, Madison, WI 53706 USA. EM bennartz@aos.wisc.edu RI Fan, Jiwen/E-9138-2011; Bennartz, Ralf/F-3760-2010; Heidinger, Andrew/F-5591-2010 OI Heidinger, Andrew/0000-0001-7631-109X FU NASA [NNX08AF92G]; Department of Energy (DOE) [ER64840]; US Department of Energy [DE-AC06-76RLO1830] FX This project was partly supported by NASA grant NNX08AF92G and the Department of Energy (DOE) Regional and Global Climate Modeling (RCGM) Program Grant ER64840 to the first author as well as by the bilateral agreement between DOE and China's Ministry of Sciences and Technology that supports regional climate research at PNNL. PNNL is operated for the US Department of Energy by Battelle Memorial Institute under contract DE-AC06-76RLO1830. We thank Chun Zhao and Yi Gao at PNNL for providing the emission data used in our model simulations and Andi Walther of UW-Madison/CIMSS for his help in processing the satellite observations. The views and opinions contained in this report are those of the authors and should not be construed as an official National Oceanic and Atmospheric Administration or U.S. Government position, policy, or decision. NR 24 TC 10 Z9 11 U1 2 U2 20 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAY 10 PY 2011 VL 38 AR L09704 DI 10.1029/2011GL047235 PG 6 WC Geosciences, Multidisciplinary SC Geology GA 764IP UT WOS:000290623400003 ER PT J AU McCauley, AP Rosa, FSS Rodriguez, AW Joannopoulos, JD Dalvit, DAR Johnson, SG AF McCauley, Alexander P. Rosa, F. S. S. Rodriguez, Alejandro W. Joannopoulos, John D. Dalvit, D. A. R. Johnson, Steven G. TI Structural anisotropy and orientation-induced Casimir repulsion in fluids SO PHYSICAL REVIEW A LA English DT Article ID MU-M; FORCES; TORQUE; RANGE AB In this work we theoretically consider the Casimir force between two periodic arrays of nanowires (both in vacuum, and on a substrate separated by a fluid) at separations comparable to the period. Specifically, we compute the dependence of the exact Casimir force between the arrays under both lateral translations and rotations. Although typically the force between such structures is well characterized by the proximity force approximation (PFA), we find that in the present case the microstructure modulates the force in a way qualitatively inconsistent with PFA. We find instead that effective-medium theory, in which the slabs are treated as homogeneous, anisotropic dielectrics, gives a surprisingly accurate picture of the force, down to separations of half the period. This includes a situation for identical, fluid-separated slabs in which the exact force changes sign with the orientation of the wire arrays, whereas PFA predicts attraction. We discuss the possibility of detecting these effects in experiments, concluding that this effect is strong enough to make detection possible in the near future. C1 [McCauley, Alexander P.; Joannopoulos, John D.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Rosa, F. S. S.] Univ Paris 11, Lab Charles Fabry, Inst Opt, CNRS, F-91127 Palaiseau, France. [Rosa, F. S. S.; Dalvit, D. A. R.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Rodriguez, Alejandro W.; Johnson, Steven G.] MIT, Dept Math, Cambridge, MA 02139 USA. [Rodriguez, Alejandro W.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02139 USA. RP McCauley, AP (reprint author), MIT, Dept Phys, Cambridge, MA 02139 USA. FU Army Research Office through the ISN [W911NF-07-D-0004]; DARPA [N66001-09-1-2070-DOD]; DOE/NNSA [DE-AC52-06NA25396] FX We thank D. Woolf, J. Munday, F. Intravaia, and M. Maghrebi for useful discussions, and R. Zhao and K. Berggren for helpful references. This work was supported by the Army Research Office through the ISN under Contract No. W911NF-07-D-0004, and by DARPA under Contract No. N66001-09-1-2070-DOD and under DOE/NNSA Contract No. DE-AC52-06NA25396. NR 59 TC 7 Z9 7 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 J9 PHYS REV A JI Phys. Rev. A PD MAY 10 PY 2011 VL 83 IS 5 AR 052503 DI 10.1103/PhysRevA.83.052503 PG 11 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 761YD UT WOS:000290438300003 ER PT J AU Bernstein, DP Brauer, B Kukreja, R Stohr, J Hauet, T Cucchiara, J Mangin, S Katine, JA Tyliszczak, T Chou, KW Acremann, Y AF Bernstein, David P. Braeuer, Bjoern Kukreja, Roopali Stoehr, Joachim Hauet, Thomas Cucchiara, Julien Mangin, Stephane Katine, Jordan A. Tyliszczak, Tolek Chou, Kang W. Acremann, Yves TI Nonuniform switching of the perpendicular magnetization in a spin-torque-driven magnetic nanopillar SO PHYSICAL REVIEW B LA English DT Article AB Time-resolved scanning transmission x-ray microscopy measurements were performed to study the current-induced magnetization switching mechanism in nanopillars exhibiting strong perpendicular magnetic anisotropy. This technique provides both short-time (70 ps) and high-spatial (25 nm) resolutions. Direct imaging of the magnetization demonstrates that, after an incubation time of similar to 1.3 ns, a 100 x 300 nm(2) ellipsoidal device switches in similar to 1 ns via a central domain nucleation and opposite propagation of two domain walls toward the edges. High domain-wall velocities on the order of 100 m/s are measured. Micromagnetic simulations are shown to be in good agreement with experimental results and provide insight into magnetization dynamics during the incubation and reversal periods. C1 [Bernstein, David P.; Braeuer, Bjoern; Kukreja, Roopali; Stoehr, Joachim] Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Hauet, Thomas; Cucchiara, Julien; Mangin, Stephane] Nancy Univ, UPV Metz, CNRS, Inst Jean Lamour, Vandoeuvre Les Nancy, France. [Hauet, Thomas; Katine, Jordan A.] Hitachi Global Storage Technol, San Jose, CA 95119 USA. [Tyliszczak, Tolek; Chou, Kang W.] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. [Acremann, Yves] ETH, Solid State Phys Lab, Zurich, Switzerland. RP Bernstein, DP (reprint author), Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. OI Mangin, stephane/0000-0001-6046-0437 FU US Department of Energy, Office of Science, Office of Basic Energy Science [DE-AC02-76SF00515]; German Research Foundation (DFG); Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX The authors would like to thank Olav Hellwig for his help with the PMA deposition process, H. Tomita, Y. Suzuki, A. Kent, and E. E. Fullerton for discussions, and the US Department of Energy, Office of Science, Office of Basic Energy Science for its continued support under Contract No. DE-AC02-76SF00515. B. B. acknowledges support from the German Research Foundation (DFG). The ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 19 TC 24 Z9 24 U1 0 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 10 PY 2011 VL 83 IS 18 AR 180410 DI 10.1103/PhysRevB.83.180410 PG 4 WC Physics, Condensed Matter SC Physics GA 761YJ UT WOS:000290439000001 ER PT J AU Stafford, RL Tang, MY Sawaya, MR Phillips, ML Bowie, JU AF Stafford, Ryan L. Tang, Ming-Yun Sawaya, Michael R. Phillips, Martin L. Bowie, James U. TI Crystal Structure of the Central Coiled-Coil Domain from Human Liprin-beta 2 SO BIOCHEMISTRY LA English DT Article ID LIPRIN-ALPHA; NEUROTRANSMITTER RELEASE; SYNAPSE FORMATION; ACTIVE ZONE; PROTEIN; ORGANIZATION; ELEGANS; PROGRAM; SPECIFICITY; PREDICTION AB Liprins are a conserved family of scaffolding proteins important for the proper regulation and development of neuronal synapses. Humans have four liprin-alpha s and two liprin-beta s which all contain long coiled-coil domains followed by three tandem SAM domains. Complex interactions between the coiled-coil and SAM domains are thought to create liprin scaffolds, but the structural and biochemical properties of these domains remain largely uncharacterized. In this study we find that the human liprin-beta 2 coiled-coil forms an extended dimer. Several protease-resistant subdomains within the liprin-beta 1 and liprin-beta 2 coiled-coils were also identified. A 2.0 angstrom crystal structure of the central, protease-resistant core of the liprin-beta 2 coiled-coil reveals a parallel helix orientation. These studies represent an initial step toward determining the overall architecture of liprin scaffolds and understanding the molecular basis for their synaptic functions. C1 [Stafford, Ryan L.; Tang, Ming-Yun; Sawaya, Michael R.; Phillips, Martin L.; Bowie, James U.] Univ Calif Los Angeles, Dept Chem & Biochem, UCLA DOE Inst Genom & Prote, Inst Mol Biol, Los Angeles, CA 90095 USA. RP Bowie, JU (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, UCLA DOE Inst Genom & Prote, Inst Mol Biol, Boyer Hall,611 Charles E Young Dr, Los Angeles, CA 90095 USA. EM bowie@mbi.ucla.edu FU NIH [R01GM093393, F32GM084615, P20 RR-016464] FX This work was supported by NIH Grant R01GM093393 to J.U.B. and a NIH Ruth L. Kirschstein Postdoctoral Fellowship F32GM084615 to R.L.S.; We thank Julian Whitelegge and Sara Bassilian (UCLA Pasarow Mass Spectrometry Laboratory) for assistance with mass spectrometry experiments and Kathy Schegg (UNR INBRE Nevada Proteomics Center; NIH Grant Number P20 RR-016464) for Edman sequencing. NR 42 TC 3 Z9 4 U1 0 U2 2 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD MAY 10 PY 2011 VL 50 IS 18 BP 3807 EP 3815 DI 10.1021/bi200141e PG 9 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 757AK UT WOS:000290056000022 PM 21462929 ER PT J AU Abazov, VM Abbott, B Acharya, BS Adams, M Adams, T Alexeev, GD Alkhazov, G Alton, A Alverson, G Alves, GA Ancu, LS Aoki, M Arov, M Askew, A Asman, B Atramentov, O Avila, C BackusMayes, J Badaud, F Bagby, L Baldin, B Bandurin, DV Banerjee, S Barberis, E Baringer, P Barreto, J Bartlett, JF Bassler, U Bazterra, V Beale, S Bean, A Begalli, M Begel, M Belanger-Champagne, C Bellantoni, L Beri, SB Bernardi, G Bernhard, R Bertram, I Besancon, M Beuselinck, R Bezzubov, VA Bhat, PC Bhatnagar, V Blazey, G Blessing, S Bloom, K Boehnlein, A Boline, D Bolton, TA Boos, EE Borissov, G Bose, T Brandt, A Brandt, O Brock, R Brooijmans, G Bross, A Brown, D Brown, J Bu, XB Buehler, M Buescher, V Bunichev, V Burdin, S Burnett, TH Buszello, CP Calpas, B Camacho-Perez, E Carrasco-Lizarraga, MA Casey, BCK Castilla-Valdez, H Chakrabarti, S Chakraborty, D Chan, KM Chandra, A Chen, G Chevalier-Thery, S Cho, DK Cho, SW Choi, S Choudhary, B Christoudias, T Cihangir, S Claes, D Clutter, J Cooke, M Cooper, WE Corcoran, M Couderc, F Cousinou, MC Croc, A Cutts, D Das, A Davies, G De, K de Jong, SJ De La Cruz-Burelo, E Deliot, F Demarteau, M Demina, R Denisov, D Denisov, SP Desai, S DeVaughan, K Diehl, HT Diesburg, M Dominguez, A Dorland, T Dubey, A Dudko, LV Duggan, D Duperrin, A Dutt, S Dyshkant, A Eads, M Edmunds, D Ellison, J Elvira, VD Enari, Y Evans, H Evdokimov, A Evdokimov, VN Facini, G Ferbel, T Fiedler, F Filthaut, F Fisher, W Fisk, HE Fortner, M Fox, H Fuess, S Gadfort, T Garcia-Bellido, A Gavrilov, V Gay, P Geist, W Geng, W Gerbaudo, D Gerber, CE Gershtein, Y Ginther, G Golovanov, G Goussiou, A Grannis, PD Greder, S Greenlee, H Greenwood, ZD Gregores, EM Grenier, G Gris, P Grivaz, JF Grohsjean, A Grunendahl, S Grunewald, MW Guo, F Gutierrez, G Gutierrez, P Haas, A Hagopian, S Haley, J Han, L Harder, K Harel, A Hauptman, JM Hays, J Head, T Hebbeker, T Hedin, D Hegab, H Heinson, AP Heintz, U Hensel, C Heredia-De La Cruz, I Herner, K Hildreth, MD Hirosky, R Hoang, T Hobbs, JD Hoeneisen, B Hohlfeld, M Hossain, S Hubacek, Z Huske, N Hynek, V Iashvili, I Illingworth, R Ito, AS Jabeen, S Jaffre, M Jain, S Jamin, D Jesik, R Johns, K Johnson, M Johnston, D Jonckheere, A Jonsson, P Joshi, J Juste, A Kaadze, K Kajfasz, E Karmanov, D Kasper, PA Katsanos, I Kehoe, R Kermiche, S Khalatyan, N Khanov, A Kharchilava, A Kharzheev, YN Khatidze, D Kirby, MH Kohli, JM Kozelov, AV Kraus, J Kumar, A Kupco, A Kurca, T Kuzmin, VA Kvita, J Lammers, S Landsberg, G Lebrun, P Lee, HS Lee, SW Lee, WM Lellouch, J Li, L Li, QZ Lietti, SM Lim, JK Lincoln, D Linnemann, J Lipaev, VV Lipton, R Liu, Y Liu, Z Lobodenko, A Lokajicek, M Love, P Lubatti, HJ Luna-Garcia, R Lyon, AL Maciel, AKA Mackin, D Madar, R Magana-Villalba, R Malik, S Malyshev, VL Maravin, Y Martinez-Ortega, J McCarthy, R McGivern, CL Meijer, MM Melnitchouk, A Menezes, D Mercadante, PG Merkin, M Meyer, A Meyer, J Miconi, F Mondal, NK Muanza, GS Mulhearn, M Nagy, E Naimuddin, M Narain, M Nayyar, R Neal, HA Negret, JP Neustroev, P Novaes, SF Nunnemann, T Obrant, G Orduna, J Osman, N Osta, J Garzon, GJOY Owen, M Padilla, M Pangilinan, M Parashar, N Parihar, V Park, SK Parsons, J Partridge, R Parua, N Patwa, A Penning, B Perfilov, M Peters, K Peters, Y Petrillo, G Petroff, P Piegaia, R Piper, J Pleier, MA Podesta-Lerma, PLM Podstavkov, VM Pol, ME Polozov, P Popov, AV Prewitt, M Price, D Protopopescu, S Qian, J Quadt, A Quinn, B Rangel, MS Ranjan, K Ratoff, PN Razumov, I Renkel, P Rijssenbeek, M Ripp-Baudot, I Rizatdinova, F Rominsky, M Royon, C Rubinov, P Ruchti, R Safronov, G Sajot, G Sanchez-Hernandez, A Sanders, MP Sanghi, B Santos, AS Savage, G Sawyer, L Scanlon, T Schamberger, RD Scheglov, Y Schellman, H Schliephake, T Schlobohm, S Schwanenberger, C Schwienhorst, R Sekaric, J Severini, H Shabalina, E Shary, V Shchukin, AA Shivpuri, RK Simak, V Sirotenko, V Skubic, P Slattery, P Smirnov, D Smith, KJ Snow, GR Snow, J Snyder, S Soldner-Rembold, S Sonnenschein, L Sopczak, A Sosebee, M Soustruznik, K Spurlock, B Stark, J Stolin, V Stoyanova, DA Strauss, M Strom, D Stutte, L Suter, L Svoisky, P Takahashi, M Tanasijczuk, A Taylor, W Titov, M Tokmenin, VV Tsai, YT Tsybychev, D Tuchming, B Tully, C Tuts, PM Uvarov, L Uvarov, S Uzunyan, S Van Kooten, R van Leeuwen, WM Varelas, N Varnes, EW Vasilyev, IA Verdier, P Vertogradov, LS Verzocchi, M Vesterinen, M Vilanova, D Vint, P Vokac, P Wahl, HD Wang, MHLS Warchol, J Watts, G Wayne, M Weber, M Welty-Rieger, L White, A Wicke, D Williams, MRJ Wilson, GW Wimpenny, SJ Wobisch, M Wood, DR Wyatt, TR Xie, Y Xu, C Yacoob, S Yamada, R Yang, WC Yasuda, T Yatsunenko, YA Ye, Z Yin, H Yip, K Youn, SW Yu, J Zelitch, S 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Luna-Garcia, R. Lyon, A. L. Maciel, A. K. A. Mackin, D. Madar, R. Magana-Villalba, R. Malik, S. Malyshev, V. L. Maravin, Y. Martinez-Ortega, J. McCarthy, R. McGivern, C. L. Meijer, M. M. Melnitchouk, A. Menezes, D. Mercadante, P. G. Merkin, M. Meyer, A. Meyer, J. Miconi, F. Mondal, N. K. Muanza, G. S. Mulhearn, M. Nagy, E. Naimuddin, M. Narain, M. Nayyar, R. Neal, H. A. Negret, J. P. Neustroev, P. Novaes, S. F. Nunnemann, T. Obrant, G. Orduna, J. Osman, N. Osta, J. Otero Y Garzon, G. J. Owen, M. Padilla, M. Pangilinan, M. Parashar, N. Parihar, V. Park, S. K. Parsons, J. Partridge, R. Parua, N. Patwa, A. Penning, B. Perfilov, M. Peters, K. Peters, Y. Petrillo, G. Petroff, P. Piegaia, R. Piper, J. Pleier, M. -A. Podesta-Lerma, P. L. M. Podstavkov, V. M. Pol, M. -E. Polozov, P. Popov, A. V. Prewitt, M. Price, D. Protopopescu, S. Qian, J. Quadt, A. Quinn, B. Rangel, M. S. Ranjan, K. Ratoff, P. N. Razumov, I. Renkel, P. Rijssenbeek, M. Ripp-Baudot, I. Rizatdinova, F. Rominsky, M. Royon, C. Rubinov, P. Ruchti, R. Safronov, G. Sajot, G. Sanchez-Hernandez, A. Sanders, M. P. Sanghi, B. Santos, A. S. Savage, G. Sawyer, L. Scanlon, T. Schamberger, R. D. Scheglov, Y. Schellman, H. Schliephake, T. Schlobohm, S. Schwanenberger, C. Schwienhorst, R. Sekaric, J. Severini, H. Shabalina, E. Shary, V. Shchukin, A. A. Shivpuri, R. K. Simak, V. Sirotenko, V. Skubic, P. Slattery, P. Smirnov, D. Smith, K. J. Snow, G. R. Snow, J. Snyder, S. Soeldner-Rembold, S. Sonnenschein, L. Sopczak, A. Sosebee, M. Soustruznik, K. Spurlock, B. Stark, J. Stolin, V. Stoyanova, D. A. Strauss, M. Strom, D. Stutte, L. Suter, L. Svoisky, P. Takahashi, M. Tanasijczuk, A. Taylor, W. Titov, M. Tokmenin, V. V. Tsai, Y. -T. Tsybychev, D. Tuchming, B. Tully, C. Tuts, P. M. Uvarov, L. Uvarov, S. Uzunyan, S. Van Kooten, R. van Leeuwen, W. M. Varelas, N. Varnes, E. W. Vasilyev, I. A. Verdier, P. Vertogradov, L. S. Verzocchi, M. Vesterinen, M. Vilanova, D. Vint, P. Vokac, P. Wahl, H. D. Wang, M. H. L. S. Warchol, J. Watts, G. Wayne, M. Weber, M. Welty-Rieger, L. White, A. Wicke, D. Williams, M. R. J. Wilson, G. W. Wimpenny, S. J. Wobisch, M. Wood, D. R. Wyatt, T. R. Xie, Y. Xu, C. Yacoob, S. Yamada, R. Yang, W. -C. Yasuda, T. Yatsunenko, Y. A. Ye, Z. Yin, H. Yip, K. Youn, S. W. Yu, J. Zelitch, S. Zhao, T. Zhou, B. Zhu, J. Zielinski, M. Zieminska, D. Zivkovic, L. CA D0 Collaboration TI Measurement of color flow in t(t)over-bar events from p(p)over-bar collisions at root s=1.96 TeV SO PHYSICAL REVIEW D LA English DT Article ID DETECTOR AB We present the first measurement of the color representation of the hadronically decaying W boson in t (t) over bar events, from 5.3 fb(-1) of integrated luminosity collected with the D0 experiment. A novel calorimeter-based vectorial variable, "jet pull," is used, sensitive to the color-flow structure of the final state. We find that the fraction of uncolored W bosons is 0.56 +/- 0.42(stat + syst), in agreement with the standard model. C1 [Otero Y Garzon, G. J.; Piegaia, R.; Tanasijczuk, A.] Univ Buenos Aires, Buenos Aires, DF, Argentina. [Alves, G. A.; Maciel, A. K. A.; Pol, M. -E.; Rangel, M. S.] Ctr Brasileiro Pesquisas Fis, LAFEX, Rio De Janeiro, Brazil. [Barreto, J.; Begalli, M.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Santo Andre, Brazil. [Lietti, S. M.; Novaes, S. F.; Santos, A. S.] Univ Estadual Paulista, Inst Fis Teor, BR-01405 Sao Paulo, Brazil. [Beale, S.; Liu, Z.; Taylor, W.] Simon Fraser Univ, Vancouver, BC, Canada. [Beale, S.; Liu, Z.; Taylor, W.] York Univ, Toronto, ON M3J 2R7, Canada. [Han, L.; Liu, Y.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Avila, C.; Negret, J. P.] Univ Los Andes, Bogota, Colombia. [Kvita, J.; Soustruznik, K.] Charles Univ Prague, Fac Math & Phys, Ctr Particle Phys, Prague, Czech Republic. [Hubacek, Z.; Hynek, V.; Simak, V.; Vokac, P.] Czech Tech Univ, CR-16635 Prague, Czech Republic. 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[Abbott, B.; Gutierrez, P.; Hossain, S.; Severini, H.; Skubic, P.; Strauss, M.; Svoisky, P.] Univ Oklahoma, Norman, OK 73019 USA. [Hegab, H.; Khanov, A.; Rizatdinova, F.] Oklahoma State Univ, Stillwater, OK 74078 USA. [Cho, D. K.; Cutts, D.; Heintz, U.; Jabeen, S.; Khatidze, D.; Landsberg, G.; Narain, M.; Pangilinan, M.; Parihar, V.; Partridge, R.; Zivkovic, L.] Brown Univ, Providence, RI 02912 USA. [Brandt, A.; De, K.; Sosebee, M.; Spurlock, B.; White, A.; Yu, J.] Univ Texas Arlington, Arlington, TX 76019 USA. [Kehoe, R.; Renkel, P.] So Methodist Univ, Dallas, TX 75275 USA. [Chandra, A.; Corcoran, M.; Mackin, D.; Prewitt, M.] Rice Univ, Houston, TX 77005 USA. [Buehler, M.; Hirosky, R.; Mulhearn, M.; Zelitch, S.] Univ Virginia, Charlottesville, VA 22901 USA. [BackusMayes, J.; Burnett, T. H.; Dorland, T.; Goussiou, A.; Lubatti, H. J.; Schlobohm, S.; Watts, G.; Zhao, T.] Univ Washington, Seattle, WA 98195 USA. RP Abazov, VM (reprint author), Univ Buenos Aires, Buenos Aires, DF, Argentina. RI Fisher, Wade/N-4491-2013; De, Kaushik/N-1953-2013; Ancu, Lucian Stefan/F-1812-2010; Deliot, Frederic/F-3321-2014; Sharyy, Viatcheslav/F-9057-2014; Lokajicek, Milos/G-7800-2014; Kupco, Alexander/G-9713-2014; Kozelov, Alexander/J-3812-2014; Christoudias, Theodoros/E-7305-2015; Gerbaudo, Davide/J-4536-2012; Li, Liang/O-1107-2015; Dudko, Lev/D-7127-2012; Perfilov, Maxim/E-1064-2012; Boos, Eduard/D-9748-2012; Gutierrez, Phillip/C-1161-2011; Novaes, Sergio/D-3532-2012; Santos, Angelo/K-5552-2012; Mercadante, Pedro/K-1918-2012; Bolton, Tim/A-7951-2012; bu, xuebing/D-1121-2012; Alves, Gilvan/C-4007-2013; Yip, Kin/D-6860-2013; Merkin, Mikhail/D-6809-2012 OI De, Kaushik/0000-0002-5647-4489; Ancu, Lucian Stefan/0000-0001-5068-6723; Sharyy, Viatcheslav/0000-0002-7161-2616; Christoudias, Theodoros/0000-0001-9050-3880; Gerbaudo, Davide/0000-0002-4463-0878; Li, Liang/0000-0001-6411-6107; Dudko, Lev/0000-0002-4462-3192; Novaes, Sergio/0000-0003-0471-8549; Yip, Kin/0000-0002-8576-4311; FU DOE; NSF (USA); CEA; CNRS/IN2P3 (France); FASI, Rosatom; RFBR (Russia); CNPq; FAPERJ; FAPESP; FUNDUNESP (Brazil); DAE; DST (India); Colciencias (Colombia); CONACyT (Mexico); KRF; KOSEF (Korea); CONICET; UBACyT (Argentina); FOM (The Netherlands); STFC; Royal Society (United Kingdom); MSMT; GACR (Czech Republic); CRC; NSERC (Canada); BMBF; DFG (Germany); SFI (Ireland); Swedish Research Council (Sweden); CAS; CNSF (China) FX We thank Jason Gallicchio, Matthew Schwartz, Steve Mrenna, Peter Skands, and Jay Wacker for discussions and guidance. We thank the staffs at Fermilab and collaborating institutions, and acknowledge support from the DOE and NSF (USA); CEA and CNRS/IN2P3 (France); FASI, Rosatom, and RFBR (Russia); CNPq, FAPERJ, FAPESP, and FUNDUNESP (Brazil); DAE and DST (India); Colciencias (Colombia); CONACyT (Mexico); KRF and KOSEF (Korea); CONICET and UBACyT (Argentina); FOM (The Netherlands); STFC and the Royal Society (United Kingdom); MSMT and GACR (Czech Republic); CRC Program and NSERC (Canada); BMBF and DFG (Germany); SFI (Ireland); The Swedish Research Council (Sweden); and CAS and CNSF (China). NR 21 TC 7 Z9 7 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 J9 PHYS REV D JI Phys. Rev. D PD MAY 10 PY 2011 VL 83 IS 9 AR 092002 DI 10.1103/PhysRevD.83.092002 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 761YV UT WOS:000290440300001 ER PT J AU Fox, PJ Liu, J Weiner, N AF Fox, Patrick J. Liu, Jia Weiner, Neal TI Integrating out astrophysical uncertainties SO PHYSICAL REVIEW D LA English DT Article ID DARK-MATTER SEARCH; DAMA/LIBRA; SIGNATURE; LIMITS AB Underground searches for dark matter involve a complicated interplay of particle physics, nuclear physics, atomic physics, and astrophysics. We attempt to remove the uncertainties associated with astrophysics by developing the means to map the observed signal in one experiment directly into a predicted rate at another. We argue that it is possible to make experimental comparisons that are completely free of astrophysical uncertainties by focusing on integral quantities, such as g(v(min)) = integral(vmin) dv f(v)/v and integral(vthresh) dvvg(v). Direct comparisons are possible when the vmin space probed by different experiments overlap. As examples, we consider the possible dark matter signals at CoGeNT, DAMA, and CRESST-Oxygen. We find that the expected rate from CoGeNT in the XENON10 experiment is higher than observed, unless scintillation light output is low. Moreover, we determine that S2-only analyses are constraining, unless the charge yields Q(y) < 2.4 electrons/keV. For DAMA to be consistent with XENON10, we find for q(Na) = 0.3 that the modulation rate must be extremely high (greater than or similar to 70% for m(chi) = 7 GeV), while for higher quenching factors, it makes an explicit prediction (0.8-0.9 cpd/kg) for the modulation to be observed at CoGeNT. Finally, we find CDMS-Si, even with a 10 keV threshold, as well as XENON10, even with low scintillation, would have seen significant rates if the excess events at CRESST arise from elastic WIMP scattering, making it very unlikely to be the explanation of this anomaly. C1 [Fox, Patrick J.] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Fox, Patrick J.; Weiner, Neal] Inst Adv Study, Sch Nat Sci, Princeton, NJ 08540 USA. [Liu, Jia; Weiner, Neal] NYU, Ctr Cosmol & Particle Phys, Dept Phys, New York, NY 10003 USA. RP Fox, PJ (reprint author), Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. RI LIU, JIA/O-7813-2016 OI LIU, JIA/0000-0001-7386-0253 FU NSF [PHY-0449818]; DOE [DE-FG02-06ER41417]; Amborse Monell Foundation; United States Department of Energy [DE-AC02-07CH11359] FX We thank Juan Collar, Rafael Lang, David Moore, and Peter Sorensen for useful comments on the manuscript. N. W. is supported by NSF Grant No. PHY-0449818 and DOE OJI Grant No. DE-FG02-06ER41417, as well as by the Amborse Monell Foundation. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. P. F. and N. W. would like to thank the Aspen Center for Physics where this work was initiated. NR 56 TC 101 Z9 101 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 10 PY 2011 VL 83 IS 10 AR 103514 DI 10.1103/PhysRevD.83.103514 PG 12 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 761YY UT WOS:000290440600004 ER PT J AU Ozer, MM Moon, EJ Eguiluz, AG Weitering, HH AF Oezer, Mustafa M. Moon, Eun Ju Eguiluz, Adolfo G. Weitering, Hanno H. TI Plasmon Response of a Quantum-Confined Electron Gas Probed by Core-Level Photoemission SO PHYSICAL REVIEW LETTERS LA English DT Article ID THIN METAL-FILMS; SPECTRA; EXCITATIONS; MAGNESIUM; MG AB We demonstrate the existence of quantized "bulk'' plasmons in ultrathin magnesium films on Si( 111) by analyzing plasmon-loss satellites in core-level photoemission spectra, recorded as a function of the film thickness d. Remarkably, the plasmon energy is shown to vary as 1/d(2) all the way down to three atomic layers. The loss spectra are dominated by the n = 1 and n = 2 normal modes, consistent with the excitation of plasmons involving quantized electronic subbands. With decreasing film thickness, spectral weight is gradually transferred from the plasmon modes to the low-energy single-particle excitations. These results represent striking manifestations of the role of quantum confinement on plasmon resonances in precisely controlled nanostructures. C1 [Oezer, Mustafa M.; Eguiluz, Adolfo G.; Weitering, Hanno H.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Moon, Eun Ju; Eguiluz, Adolfo G.; Weitering, Hanno H.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Ozer, MM (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM hanno@utk.edu RI Moon, Eun Ju/C-7856-2014 FU American Chemical Society; National Science Foundation [DMR 0906025, OCI-0904972]; Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, U.S. Department of Energy FX Acknowledgment is made to the Donors of the American Chemical Society Petroleum Research Fund for partial support of this research. Additional funding was provided by the National Science Foundation under Grants No. DMR 0906025 and No. OCI-0904972 and by the Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, U.S. Department of Energy. NR 19 TC 8 Z9 8 U1 1 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 10 PY 2011 VL 106 IS 19 AR 197601 DI 10.1103/PhysRevLett.106.197601 PG 4 WC Physics, Multidisciplinary SC Physics GA 761YA UT WOS:000290437900011 PM 21668200 ER PT J AU Tamam, L Ocko, BM Reichert, H Deutsch, M AF Tamam, L. Ocko, B. M. Reichert, H. Deutsch, M. TI Checkerboard Self-Patterning of an Ionic Liquid Film on Mercury SO PHYSICAL REVIEW LETTERS LA English DT Article ID X-RAY REFLECTIVITY; NORMAL-ALKANES; SURFACE; MOLECULES AB A-resolution studies of room temperature ionic liquid (RTIL) interfaces are scarce, in spite of their long-recognized importance for the science and many applications of RTILs. We present an A-resolution x-ray study of a Langmuir film of an RTIL on mercury. At low (high) coverage [90 (50) angstrom A(2)/molecule] a mono-(bi) layer of surface-parallel molecules is found. The molecules self-assemble in a lateral ionic checkerboard pattern, unlike the uniform-charge, alternate-ion layers of this RTIL at its bulk-solid interface. A 2D-smectic order is found, with molecules packed in parallel stripes, forming long-range order normal to, but none along, the stripes. C1 [Tamam, L.; Deutsch, M.] Bar Ilan Univ, Dept Phys, IL-52900 Ramat Gan, Israel. [Tamam, L.; Deutsch, M.] Bar Ilan Univ, Inst Nanotechnol, IL-52900 Ramat Gan, Israel. [Ocko, B. M.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Reichert, H.] European Synchrotron Radiat Facil, F-38043 Grenoble, France. RP Tamam, L (reprint author), Bar Ilan Univ, Dept Phys, IL-52900 Ramat Gan, Israel. EM moshe.deautsch@biu.ac.il FU DOE [DE-AC02-76CH0016] FX Jerusalem, for support, and NSLS, Brookhaven National Laboratory (supported by DOE Contract No. DE-AC02-76CH0016) for beamtime. NR 30 TC 19 Z9 19 U1 3 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 10 PY 2011 VL 106 IS 19 AR 197801 DI 10.1103/PhysRevLett.106.197801 PG 4 WC Physics, Multidisciplinary SC Physics GA 761YA UT WOS:000290437900012 PM 21668201 ER PT J AU Barth, AJ Nguyen, ML Malkan, MA Filippenko, AV Li, WD Gorjian, V Joner, MD Bennert, VN Botyanszki, J Cenko, SB Childress, M Choi, J Comerford, JM Cucciara, A da Silva, R Duchene, G Fumagalli, M Ganeshalingam, M Gates, EL Gerke, BF Griffith, CV Harris, C Hintz, EG Hsiao, E Kandrashoff, MT Keel, WC Kirkman, D Kleiser, IKW Laney, CD Lee, J Lopez, L Lowe, TB Moody, JW Morton, A Nierenberg, AM Nugent, P Pancoast, A Rex, J Rich, RM Silverman, JM Smith, GH Sonnenfeld, A Suzuki, N Tytler, D Walsh, JL Woo, JH Yang, YZ Zeisse, C AF Barth, Aaron J. Nguyen, My L. Malkan, Matthew A. Filippenko, Alexei V. Li, Weidong Gorjian, Varoujan Joner, Michael D. Bennert, Vardha Nicola Botyanszki, Janos Cenko, S. Bradley Childress, Michael Choi, Jieun Comerford, Julia M. Cucciara, Antonino da Silva, Robert Duchene, Gaspard Fumagalli, Michele Ganeshalingam, Mohan Gates, Elinor L. Gerke, Brian F. Griffith, Christopher V. Harris, Chelsea Hintz, Eric G. Hsiao, Eric Kandrashoff, Michael T. Keel, William C. Kirkman, David Kleiser, Io K. W. Laney, C. David Lee, Jeffrey Lopez, Liliana Lowe, Thomas B. Moody, J. Ward Morton, Alekzandir Nierenberg, A. M. Nugent, Peter Pancoast, Anna Rex, Jacob Rich, R. Michael Silverman, Jeffrey M. Smith, Graeme H. Sonnenfeld, Alessandro Suzuki, Nao Tytler, David Walsh, Jonelle L. Woo, Jong-Hak Yang, Yizhe Zeisse, Carl TI BROAD-LINE REVERBERATION IN THE KEPLER-FIELD SEYFERT GALAXY Zw 229-015 SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: active; galaxies: individual (Zw 229-015); galaxies: nuclei ID ACTIVE GALACTIC NUCLEI; AGN MONITORING PROJECT; BLACK-HOLE MASS; ALL-SKY SURVEY; RADIATION PRESSURE; LUMINOSITY RELATIONSHIP; RECOMBINATION LINES; VELOCITY DISPERSION; POWER SPECTRA; REGION SIZES AB The Seyfert 1 galaxy Zw 229-015 is among the brightest active galaxies being monitored by the Kepler mission. In order to determine the black hole mass in Zw 229-015 from H beta reverberation mapping, we have carried out nightly observations with the Kast Spectrograph at the Lick 3 m telescope during the dark runs from 2010 June through December, obtaining 54 spectroscopic observations in total. We have also obtained nightly V-band imaging with the Katzman Automatic Imaging Telescope at Lick Observatory and with the 0.9 m telescope at the Brigham Young University West Mountain Observatory over the same period. We detect strong variability in the source, which exhibited more than a factor of two change in broad H beta flux. From cross-correlation measurements, we find that the H beta light curve has a rest-frame lag of 3.86(-0.90)(+0.69) days with respect to the V-band continuum variations. We also measure reverberation lags for H alpha and H gamma and find an upper limit to the H delta lag. Combining the H beta lag measurement with a broad H beta width of sigma(line) = 1590 +/- 47 km s(-1) measured from the rms variability spectrum, we obtain a virial estimate of M-BH = 1.00(-0.24)(+0.19) x 10(7) M-circle dot for the black hole in Zw 229-015. As a Kepler target, Zw 229-015 will eventually have one of the highest-quality optical light curves ever measured for any active galaxy, and the black hole mass determined from reverberation mapping will serve as a benchmark for testing relationships between black hole mass and continuum variability characteristics in active galactic nuclei. C1 [Barth, Aaron J.; Nguyen, My L.; Walsh, Jonelle L.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Malkan, Matthew A.; Rich, R. Michael] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90024 USA. [Filippenko, Alexei V.; Li, Weidong; Cenko, S. Bradley; Choi, Jieun; Duchene, Gaspard; Ganeshalingam, Mohan; Kandrashoff, Michael T.; Kleiser, Io K. W.; Morton, Alekzandir; Nugent, Peter; Rex, Jacob; Silverman, Jeffrey M.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Gorjian, Varoujan] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Joner, Michael D.; Hintz, Eric G.; Laney, C. David; Moody, J. Ward] Brigham Young Univ, Dept Phys & Astron, Provo, UT 84602 USA. [Bennert, Vardha Nicola; Harris, Chelsea; Nierenberg, A. M.; Pancoast, Anna; Sonnenfeld, Alessandro] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Botyanszki, Janos; Childress, Michael; Cucciara, Antonino; Hsiao, Eric; Nugent, Peter; Suzuki, Nao] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Comerford, Julia M.] Univ Texas Austin, Dept Astron, Austin, TX 78712 USA. [da Silva, Robert; Smith, Graeme H.] Univ Calif Santa Cruz, Univ Calif Observ, Lick Observ, Santa Cruz, CA 95064 USA. [Duchene, Gaspard] UJF Grenoble 1, CNRS, INSU, IPAG,UMR 5274, F-38041 Grenoble, France. [Fumagalli, Michele] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. [Gerke, Brian F.] SLAC Natl Accelerator Lab, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. [Griffith, Christopher V.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Keel, William C.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Kirkman, David; Lee, Jeffrey; Lopez, Liliana; Tytler, David; Zeisse, Carl] Univ Calif San Diego, Ctr Astrophys & Space Sci, La Jolla, CA 92093 USA. [Woo, Jong-Hak] Seoul Natl Univ, Astron Program, Dept Phys & Astron, Seoul 151742, South Korea. [Yang, Yizhe] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Yang, Yizhe] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. RP Barth, AJ (reprint author), Univ Calif Irvine, Dept Phys & Astron, 4129 Frederick Reines Hall, Irvine, CA 92697 USA. EM barth@uci.edu RI Woo, Jong-Hak/A-2790-2014; Fumagalli, Michele/K-9510-2015; OI Fumagalli, Michele/0000-0001-6676-3842; Barth, Aaron/0000-0002-3026-0562 FU NSF [AST-0548198, AST-0908886, AST-0618209, NSF-0642621]; TABASGO Foundation; Gary and Cynthia Bengier; Richard and Rhoda Goldman Fund; Sun Microsystems, Inc.; Hewlett-Packard Company; Auto-Scope Corporation; Lick Observatory; University of California; Sylvia & Jim Katzman Foundation; Packard Fellowship; Ministry of Education, Science and Technology [2010-0021558]; NASA; Marc J. Staley for a Graduate Fellowship FX Research by A.J.B., M.L.N., and J.L.W. at UC Irvine has been supported by NSF CAREER grant AST-0548198. A.V.F.'s group is grateful for the financial support of NSF grant AST-0908886, the TABASGO Foundation, Gary and Cynthia Bengier, and the Richard and Rhoda Goldman Fund; also, J.M.S. thanks Marc J. Staley for a Graduate Fellowship. KAIT and its ongoing operation were made possible by donations from Sun Microsystems, Inc., the Hewlett-Packard Company, Auto-Scope Corporation, Lick Observatory, the NSF, the University of California, the Sylvia & Jim Katzman Foundation, and the TABASGO Foundation. The West Mountain Observatory 0.9 m telescope has been supported by NSF grant AST-0618209. M. D. J., C. D. L., E. G. H., and J. W. M. thank the Department of Physics and Astronomy at Brigham Young University for continued support of research efforts at the West Mountain Observatory. Tommaso Treu's research group at UCSB has been supported by NSF CAREER grant NSF-0642621 and a Packard Fellowship. Research by J. H. W. has been supported by the Basic Science Research Program through the National Research Foundation of Korea funded by the Ministry of Education, Science and Technology (2010-0021558). We thank Rick Edelson for discussions that motivated this project. We are grateful to the Lick Observatory staff for their assistance in obtaining the spectroscopic observations, and to the staff of the Maidanak Observatory for obtaining data for this project. We also thank Tabitha Buehler, Carl Melis, Dovi Poznanski, X. Prochaska, and Ben Zuckerman for contributing observations. This research has made use of the NASA/IPAC Extragalactic Database (NED) which is operated by the Jet Propulsion Laboratory, California Institute of Technology, under contract with NASA. NR 48 TC 38 Z9 38 U1 0 U2 9 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X J9 ASTROPHYS J JI Astrophys. J. PD MAY 10 PY 2011 VL 732 IS 2 AR 121 DI 10.1088/0004-637X/732/2/121 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 755ML UT WOS:000289935900061 ER PT J AU Bhattacharya, S Heitmann, K White, M Lukic, Z Wagner, C Habib, S AF Bhattacharya, Suman Heitmann, Katrin White, Martin Lukic, Zarija Wagner, Christian Habib, Salman TI MASS FUNCTION PREDICTIONS BEYOND Lambda CDM SO ASTROPHYSICAL JOURNAL LA English DT Article DE large-scale structure of universe; methods: numerical ID LARGE-SCALE BIAS; MATTER POWER SPECTRUM; COSMIC STRUCTURE FORMATION; PEAK-BACKGROUND SPLIT; N-BODY SIMULATIONS; COLD DARK-MATTER; GRAVITATIONAL-INSTABILITY; COSMOLOGICAL CONSTRAINTS; PRECISION DETERMINATION; INITIAL CONDITIONS AB The statistics of dark matter halos is an essential component of precision cosmology. The mass distribution of halos, as specified by the halo mass function, is a key input for several cosmological probes. The sizes of N-body simulations are now such that, for the most part, results need no longer be statistics-limited, but are still subject to various systematic uncertainties. Discrepancies in the results of simulation campaigns for the halo mass function remain in excess of statistical uncertainties and of roughly the same size as the error limits set by near-future observations; we investigate and discuss some of the reasons for these differences. Quantifying error sources and compensating for them as appropriate, we carry out a high-statistics study of dark matter halos from 67 N-body simulations to investigate the mass function and its evolution for a reference Lambda CDM cosmology and for a set of wCDM cosmologies. For the reference Lambda CDM cosmology (close to WMAP5), we quantify the breaking of universality in the form of the mass function as a function of redshift, finding an evolution of as much as 10% away from the universal form between redshifts z = 0 and z = 2. For cosmologies very close to this reference we provide a fitting formula to our results for the (evolving) Lambda CDM mass function over a mass range of 6 x 10(11)-3 x 10(15) M-circle dot to an estimated accuracy of about 2%. The set of wCDM cosmologies is taken from the Coyote Universe simulation suite. The mass functions from this suite (which includes a Lambda CDM cosmology and others with w similar or equal to -1) are described by the fitting formula for the reference Lambda CDM case at an accuracy level of 10%, but with clear systematic deviations. We argue that, as a consequence, fitting formulae based on a universal form for the mass function may have limited utility in high-precision cosmological applications. C1 [Bhattacharya, Suman; Lukic, Zarija; Habib, Salman] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Heitmann, Katrin] Los Alamos Natl Lab, ISR Div, Los Alamos, NM 87545 USA. [White, Martin] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [White, Martin] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Wagner, Christian] Univ Barcelona, ICC, E-08028 Barcelona, Spain. RP Bhattacharya, S (reprint author), Los Alamos Natl Lab, Div Theoret, T-2, Los Alamos, NM 87545 USA. RI White, Martin/I-3880-2015 OI White, Martin/0000-0001-9912-5070 FU DOE [W-7405-ENG-36]; LDRD program at Los Alamos National Laboratory; NASA FX A special acknowledgment is due to supercomputing time awarded to us under the LANL Institutional Computing initiative. Part of this research was supported by the DOE under contract W-7405-ENG-36 and by a DOE HEP Dark Energy R&D award. S. B., S. H., K. H., Z.L., and C. W. acknowledge support from the LDRD program at Los Alamos National Laboratory. K. H. and Z.L. were supported in part by NASA. M. W. was supported in part by NASA and the DOE. K. H., S. H., and M. W. thank the Aspen Center of Physics where part of this work was completed. S. B. and Z.L. acknowledge useful discussions with Darren Reed. We thank the referee for a careful reading of the manuscript and for a number of useful insights and suggestions. NR 66 TC 76 Z9 76 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 10 PY 2011 VL 732 IS 2 AR 122 DI 10.1088/0004-637X/732/2/122 PG 17 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 755ML UT WOS:000289935900062 ER PT J AU Feldmann, R Gnedin, NY Kravtsov, AV AF Feldmann, R. Gnedin, N. Y. Kravtsov, A. V. TI HOW UNIVERSAL IS THE Sigma(SFR)-Sigma(H2) RELATION? SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: evolution; methods: numerical; stars: formation ID GIANT MOLECULAR CLOUDS; STAR-FORMATION LAW; KENNICUTT-SCHMIDT RELATION; COSMOLOGICAL SIMULATIONS; INTERSTELLAR MATTER; LINEAR-REGRESSION; GALAXIES; GAS; HYDROGEN; M33 AB It is a well-established empirical fact that the surface density of the star formation rate, Sigma(SFR), strongly correlates with the surface density of molecular hydrogen, Sigma(H2), at least when averaged over large (similar to kpc) scales. Much less is known, however, about whether (and how) the Sigma(SFR)-Sigma(H2) relation depends on environmental parameters, such as the metallicity or the UV radiation field in the interstellar medium (ISM). Furthermore, observations indicate that the scatter in the Sigma(SFR)-Sigma(H2) relation increases rapidly with decreasing averaging scale. How the scale-dependent scatter is generated and how one recovers a tight similar to kpc scale Sigma(SFR)-Sigma(H2) relation in the first place is still largely debated. Here, these questions are explored with hydrodynamical simulations that follow the formation and destruction of H-2, include radiative transfer of UV radiation, and resolve the ISM on similar to 60 pc scales. We find that within the considered range of H-2 surface densities (10-100 M-circle dot pc(-2)), the Sigma(SFR)-Sigma(H2) relation is steeper in environments of low-metallicity and/or high-radiation fields (compared to the Galaxy), that the star formation rate (SFR) at a given H-2 surface density is larger, and the scatter is increased. Deviations from a "universal" Sigma(SFR)-Sigma(H2) relation should be particularly relevant for high-redshift galaxies or for low-metallicity dwarfs at z similar to 0. We also find that the use of time-averaged SFRs produces a large, scale-dependent scatter in the Sigma(SFR)-Sigma(H2) relation. Given the plethora of observational data expected from upcoming surveys such as ALMA, the scale-scatter relation may indeed become a valuable tool for determining the physical mechanisms connecting star formation and H-2 formation. C1 [Feldmann, R.; Gnedin, N. Y.] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA. [Feldmann, R.; Gnedin, N. Y.; Kravtsov, A. V.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Gnedin, N. Y.; Kravtsov, A. V.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Kravtsov, A. V.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. RP Feldmann, R (reprint author), Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA. EM feldmann@fnal.gov FU NSF [AST-0507596, AST-0708154]; Kavli Institute for Cosmological Physics at the University of Chicago through NSF [PHY-0551142]; Fermilab; Kavli Institute for Cosmological Physics; University of Chicago FX The authors thank A. Leroy and F. Bigiel for stimulating discussions and the anonymous referee for comments that helped improve the manuscript. The authors are grateful to the Aspen Center for Physics and to the participants and organizers of the workshop "Star Formation in Galaxies: From Recipes to Real Physics." N.Y.G. and A. V. K. were supported by the NSF grants AST-0507596 and AST-0708154, and by the Kavli Institute for Cosmological Physics at the University of Chicago through the NSF grant PHY-0551142 and an endowment from the Kavli Foundation. The simulations used in this work have been performed on the Joint Fermilab-KICP Supercomputing Cluster, supported by grants from Fermilab, Kavli Institute for Cosmological Physics, and the University of Chicago. This work made extensive use of the NASA Astrophysics Data System and arXiv.org preprint server. NR 48 TC 36 Z9 36 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X J9 ASTROPHYS J JI Astrophys. J. PD MAY 10 PY 2011 VL 732 IS 2 AR 115 DI 10.1088/0004-637X/732/2/115 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 755ML UT WOS:000289935900055 ER PT J AU Gu, MF Beiersdorfer, P Lepson, JK AF Gu, M. F. Beiersdorfer, P. Lepson, J. K. TI EMISSION LINE SPECTRA OF Al IV-Al XI IN THE EXTREME ULTRAVIOLET REGION 40-170 angstrom SO ASTROPHYSICAL JOURNAL LA English DT Article DE line: identification; methods: analytical; methods: laboratory; Sun: corona ID PERTURBATION-THEORY APPROACH; L-SHELL IONS; ELECTRON-BEAM; ATOMIC DATABASE; RAY REGION; OB STARS; SPECTROSCOPY; FE; ABUNDANCES; SPECTROMETER AB We measured wavelengths and intensities of L-shell emission lines of aluminum in the extreme ultraviolet wavelength band. We identify 75 features of Al IV through Al XI between 40 and 170 angstrom. The strongest features are due to 3 -> 2 transitions; features from 4 -> 2, 5 -> 2, and 6 -> 2 transitions are also included. Calculations made with the Flexible Atomic Code using the configuration-interaction method and many-body perturbation theory are presented and compared to the experimental results. C1 [Gu, M. F.; Lepson, J. K.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Beiersdorfer, P.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. RP Gu, MF (reprint author), Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. EM lepson@ssl.berkeley.edu FU NASA [NNH07AF81I, NNX07AH98G]; Department of Energy [DE-AC5.2-07NA27344] FX This work was supported by NASA's Astronomy and Physics Research and Analysis program grant NNH07AF81I and by NASA's Solar and Heliospherical Physics grant NNX07AH98G (U. C. Berkeley). Work at the Lawrence Livermore National Laboratory was performed under the auspices of the Department of Energy under Contract No. DE-AC5.2-07NA27344. NR 36 TC 13 Z9 13 U1 0 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X J9 ASTROPHYS J JI Astrophys. J. PD MAY 10 PY 2011 VL 732 IS 2 AR 91 DI 10.1088/0004-637X/732/2/91 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 755ML UT WOS:000289935900031 ER PT J AU Rettura, A Mei, S Stanford, SA Raichoor, A Moran, S Holden, B Rosati, P Ellis, R Nakata, F Nonino, M Treu, T Blakeslee, JP Demarco, R Eisenhardt, P Ford, HC Fosbury, RAE Illingworth, G Huertas-Company, M Jee, MJ Kodama, T Postman, M Tanaka, M White, RL AF Rettura, A. Mei, S. Stanford, S. A. Raichoor, A. Moran, S. Holden, B. Rosati, P. Ellis, R. Nakata, F. Nonino, M. Treu, T. Blakeslee, J. P. Demarco, R. Eisenhardt, P. Ford, H. C. Fosbury, R. A. E. Illingworth, G. Huertas-Company, M. Jee, M. J. Kodama, T. Postman, M. Tanaka, M. White, R. L. TI EARLY-TYPE GALAXIES AT z similar to 1.3. III. ON THE DEPENDENCE OF FORMATION EPOCHS AND STAR FORMATION HISTORIES ON STELLAR MASS AND ENVIRONMENT SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmology: observations; galaxies: clusters: general; galaxies: elliptical and lenticular, cD; galaxies: evolution; galaxies: formation; galaxies: star formation ID ORIGINS DEEP SURVEY; GOODS-SOUTH FIELD; COLOR-MAGNITUDE RELATION; HIGH-REDSHIFT CLUSTERS; MORPHOLOGY-DENSITY RELATION; BAND LUMINOSITY FUNCTION; ELLIPTIC GALAXIES; FUNDAMENTAL PLANE; VLT/FORS2 SPECTROSCOPY; INTERMEDIATE REDSHIFT AB We study the environmental dependence of stellar population properties at z similar to 1.3. We derive galaxy properties (stellar masses, ages, and star formation histories) for samples of massive, red, passive early-type galaxies (ETGs) in two high-redshift clusters, RXJ0849+4452 and RXJ0848+4453 (with redshifts of z = 1.26 and 1.27, respectively), and compare them with those measured for the RDCS1252.9-2927 cluster at z = 1.24 and with those measured for a similarly mass-selected sample of field contemporaries drawn from the GOODS-South field. Robust estimates of the aforementioned parameters have been obtained by comparing a large grid of composite stellar population models with extensive 8- to 10-band photometric coverage, from the rest-frame far-ultraviolet to the infrared. We find no variations of the overall stellar population properties among the different samples of cluster ETGs. However, when comparing cluster versus field stellar population properties we find that, even if the ages are similar and depend only on galaxy mass, the ones in the field do employ longer timescales to assemble their final mass. We find that, approximately 1Gyr after the onset of star formation, the majority (75%) of cluster galaxies have already assembled most (> 80%) of their final mass, while, by the same time, fewer (35%) field ETGs have. Thus, we conclude that while galaxy mass regulates the timing of galaxy formation, the environment regulates the timescale of their star formation histories. C1 [Rettura, A.; Stanford, S. A.; Jee, M. J.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Rettura, A.; Moran, S.] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Rettura, A.] Univ Calif Riverside, Dept Phys & Astron, Riverside, CA 92521 USA. [Mei, S.; Ford, H. C.; Huertas-Company, M.] Univ Paris Denis Diderot, F-75205 Paris 13, France. [Mei, S.; Raichoor, A.; Huertas-Company, M.] Observ Paris, GEPI, Sect Meudon, Meudon, France. [Stanford, S. A.] Lawrence Livermore Natl Lab, Inst Geophys & Planetary Phys, Livermore, CA 94551 USA. [Holden, B.; Illingworth, G.] Univ Calif Santa Cruz, UCO Lick Observ, Santa Cruz, CA 92065 USA. [Rosati, P.; Fosbury, R. A. E.] European So Observ, D-85748 Garching, Germany. [Ellis, R.] CALTECH, Pasadena, CA 91125 USA. [Nakata, F.] Natl Inst Nat Sci, Natl Astron Observ Japan, Subaru Telescope, Hilo, HI 96720 USA. [Nonino, M.] INAF Osservatorio Astron Trieste, I-34131 Trieste, Italy. [Treu, T.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Blakeslee, J. P.] Natl Res Council Canada, Herzberg Inst Astrophys, Victoria, BC V9E 2E7, Canada. [Demarco, R.] Univ Concepcion, Dept Astron, Concepcion, Chile. [Eisenhardt, P.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Kodama, T.; Postman, M.; White, R. L.] Natl Inst Nat Sci, Natl Astron Observ Japan, Mitaka, Tokyo 1818588, Japan. [Tanaka, M.] Univ Tokyo, Inst Phys & Math Universe, Kashiwa, Chiba 2778583, Japan. RP Rettura, A (reprint author), Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. OI Fosbury, Robert/0000-0001-9975-8003; Nonino, Mario/0000-0001-6342-9662; Blakeslee, John/0000-0002-5213-3548 FU NASA [NAS 5-32865, GO-10574.01-A, 20694, NAS5-26555]; W. M. Keck Foundation; BASAL Center for Astrophysics and Associated Technologies; FONDECYT [1100540] FX ACS was developed under NASA contract NAS 5-32865. This research has been supported by the NASA HST grant GO-10574.01-A, and Spitzer program 20694. The Space Telescope Science Institute is operated by AURA Inc., under NASA contract NAS5-26555. Some of the data presented herein were obtained at the W. M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California and the National Aeronautics and Space Administration. The Observatory was made possible by the generous financial support of the W. M. Keck Foundation. The authors wish to recognize and acknowledge the very significant cultural role and reverence that the summit of Mauna Kea has always had within the indigenous Hawaiian community. They are most fortunate to have the opportunity to conduct observations from this mountain. Some data were based on observations obtained at the Gemini Observatory, which is operated by the AURA, Inc., under a cooperative agreement with the NSF on behalf of the Gemini partnership: the National Science Foundation (United States), the Science and Technology Facilities Council (UK), the National Research Council (Canada), CONICYT (Chile), the Australian Research Council (Australia), Ministerio da Ciencia e Tecnologia (Brazil), and Ministerio de Ciencia, Tecnologia e Innovacion Productiva (Argentina), Gemini Science Program ID: GN-2006A-Q-78. R.D. acknowledges the support provided by the BASAL Center for Astrophysics and Associated Technologies and by FONDECYT grant N. 1100540. NR 90 TC 24 Z9 24 U1 0 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 10 PY 2011 VL 732 IS 2 AR 94 DI 10.1088/0004-637X/732/2/94 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 755ML UT WOS:000289935900034 ER PT J AU Sullivan, M Kasliwal, MM Nugent, PE Howell, DA Thomas, RC Ofek, EO Arcavi, I Blake, S Cooke, J Gal-Yam, A Hook, IM Mazzali, P Podsiadlowski, P Quimby, R Bildsten, L Bloom, JS Cenko, SB Kulkarni, SR Law, N Poznanski, D AF Sullivan, M. Kasliwal, M. M. Nugent, P. E. Howell, D. A. Thomas, R. C. Ofek, E. O. Arcavi, I. Blake, S. Cooke, J. Gal-Yam, A. Hook, I. M. Mazzali, P. Podsiadlowski, P. Quimby, R. Bildsten, L. Bloom, J. S. Cenko, S. B. Kulkarni, S. R. Law, N. Poznanski, D. TI THE SUBLUMINOUS AND PECULIAR TYPE Ia SUPERNOVA PTF 09dav SO ASTROPHYSICAL JOURNAL LA English DT Article DE supernovae: general; supernovae: individual (PTF09dav) ID WHITE-DWARF MODELS; LIGHT CURVES; LOW-LUMINOSITY; LOW-RESOLUTION; MAXIMUM LIGHT; LEGACY SURVEY; HIGH-REDSHIFT; K-CORRECTIONS; FAINT TYPE; SN 2008HA AB PTF 09dav is a peculiar subluminous Type Ia supernova (SN) discovered by the Palomar Transient Factory (PTF). Spectroscopically, it appears superficially similar to the class of subluminous SN1991bg-like SNe, but it has several unusual features which make it stand out from this population. Its peak luminosity is fainter than any previously discovered SN1991bg-like SN Ia (M-B similar to -15.5), but without the unusually red optical colors expected if the faint luminosity were due to extinction. The photospheric optical spectra have very unusual strong lines of Sc II and Mg I, with possible Sr ii, together with stronger than average Ti ii and low velocities of similar to 6000 km s(-1). The host galaxy of PTF09dav is ambiguous. The SN lies either on the extreme outskirts (similar to 41 kpc) of a spiral galaxy or in an very faint (M-R >= -12.8) dwarf galaxy, unlike other 1991bg-like SNe which are invariably associated with massive, old stellar populations. PTF 09dav is also an outlier on the light-curve-width-luminosity and color-luminosity relations derived for other subluminous SNe Ia. The inferred Ni-56 mass is small (0.019 +/- 0.003 M-circle dot), as is the estimated ejecta mass of 0.36 M-circle dot. Taken together, these properties make PTF 09dav a remarkable event. We discuss various physical models that could explain PTF 09dav. Helium shell detonation or deflagration on the surface of a CO white dwarf can explain some of the features of PTF 09dav, including the presence of Sc and the low photospheric velocities, but the observed Si and Mg are not predicted to be very abundant in these models. We conclude that no single model is currently capable of explaining all of the observed signatures of PTF 09dav. C1 [Sullivan, M.; Ofek, E. O.; Blake, S.; Podsiadlowski, P.] Univ Oxford, Dept Phys Astrophys, Oxford OX1 3RH, England. [Kasliwal, M. M.; Cooke, J.; Quimby, R.; Kulkarni, S. R.] CALTECH, Cahill Ctr Astrophys, Pasadena, CA 91125 USA. [Nugent, P. E.; Thomas, R. C.; Poznanski, D.] Univ Calif Berkeley, Lawrence Berkeley Lab, Computat Cosmol Ctr, Berkeley, CA 94720 USA. [Howell, D. A.] Las Cumbres Observ Global Telescope Network, Goleta, CA 93117 USA. [Howell, D. A.; Bildsten, L.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Arcavi, I.; Gal-Yam, A.] Weizmann Inst Sci, Fac Phys, Dept Particle Phys & Astrophys, IL-76100 Rehovot, Israel. [Hook, I. M.] INAF Osservatorio Roma, I-00040 Monte Porzio Catone, Roma, Italy. [Mazzali, P.] Max Planck Inst Astrophys, D-85741 Garching, Germany. [Mazzali, P.] Scuola Normale Super Pisa, I-56126 Pisa, Italy. [Mazzali, P.] Natl Inst Astrophys OAPd, I-35122 Padua, Italy. [Bildsten, L.] Univ Calif Santa Barbara, Kavli Inst Theoret Phys, Santa Barbara, CA 93106 USA. [Bloom, J. S.; Cenko, S. B.; Poznanski, D.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Law, N.] Univ Toronto, Dunlap Inst Astron & Astrophys, Toronto, ON M5S 3H4, Canada. RP Sullivan, M (reprint author), Univ Oxford, Dept Phys Astrophys, Keble Rd, Oxford OX1 3RH, England. EM sullivan@astro.ox.ac.uk OI Sullivan, Mark/0000-0001-9053-4820 FU Royal Society; Einstein fellowship; NASA; National Science Foundation [PHY 05-51164, AST 07-07633]; Gary and Cynthia Bengier; Richard and Rhoda Goldman Foundation; W. M. Keck Foundation; Israeli Science Foundation; Binational Science Foundation (BSF); Weizmann-UK; EU/FP7 Marie Curie IRG fellowship; Peter Award; Patricia Gruber Award FX We acknowledge useful discussions with Brian Schmidt and Dan Kasen. We thank Richard Ellis for providing the P200/DBSP spectrum. M. S. acknowledges support from the Royal Society. E.O.O. is supported by an Einstein fellowship and NASA grants. L. B. is supported by the National Science Foundation under grants PHY 05-51164 and AST 07-07633. S. B. C. acknowledges generous support from Gary and Cynthia Bengier and the Richard and Rhoda Goldman Foundation. D. P. is supported by an Einstein fellowship. The WHT is operated on the island of La Palma by the Isaac Newton Group in the Spanish Observatorio del Roque de los Muchachos of the Instituto de Astrofisica de Canarias. Observations obtained with the Samuel Oschin Telescope and the 60 inch Telescope at the Palomar Observatory as part of the Palomar Transient Factory project, a scientific collaboration between the California Institute of Technology, Columbia University, Las Cumbres Observatory, the Lawrence Berkeley National Laboratory, the National Energy Research Scientific Computing Center, the University of Oxford, and the Weizmann Institute of Science. Some of the data presented herein were obtained at the W. M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California, and the National Aeronautics and Space Administration. The Observatory was made possible by the generous financial support of the W. M. Keck Foundation. This research has made use of the NASA/IPAC Extragalactic Database (NED) which is operated by the Jet Propulsion Laboratory, California Institute of Technology, under contract with the National Aeronautics and Space Administration. The Weizmann Institute participation of in PTF is supported in part by grants from the Israeli Science Foundation to A. G. Weizmann-Caltech collaborative work on PTF is supported by a grant from the Binational Science Foundation (BSF) to A. G. and S. R. K. Collaborative work by A. G. and M. S. is supported by a grant from the Weizmann-UK "making connection" program. Collaborative work of A. G. and P. A. M. is supported by a Weizmann-Minerva grant. A. G. is supported by an EU/FP7 Marie Curie IRG fellowship and a research grant from the Peter and Patricia Gruber Awards. NR 80 TC 28 Z9 28 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X J9 ASTROPHYS J JI Astrophys. J. PD MAY 10 PY 2011 VL 732 IS 2 AR 118 DI 10.1088/0004-637X/732/2/118 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 755ML UT WOS:000289935900058 ER PT J AU Knoops, HCM Elam, JW Libera, JA Kessels, WMM AF Knoops, Harm C. M. Elam, Jeffrey W. Libera, Joseph A. Kessels, Wilhelmus M. M. TI Surface Loss in Ozone-Based Atomic Layer Deposition Processes SO CHEMISTRY OF MATERIALS LA English DT Article DE ALD; ozone; loss; recombination; decomposition ID OXIDE THIN-FILMS; MANGANESE OXIDE; CATALYTIC DECOMPOSITION; REACTION-MECHANISM; MASS-SPECTROMETRY; TEMPERATURE; GROWTH; SPECTROSCOPY; COEFFICIENT; MORPHOLOGY AB The recombinative surface loss of O(3) was investigated and its effects on the initial growth, film uniformity, and film conformality in atomic layer deposition (ALD) processes were illustrated. To determine O(3) recombination probabilities over a wide range, a method was developed using high aspect ratio capillaries at the inlet to a mass spectrometer. Using this method, we measured O(3) recombination probabilities ranging from < 10(-6) to < 10(-3) depending on the composition and temperature of the capillary surface. We utilized these measurements to understand dramatic variations in O(3) loss observed during the initial growth of O(3)-based ALD Pt on Al(2)O(3) and vice versa. Next, we studied the uniformity of O(3)-based ALD using ZnO ALD as a model system. Changes in the spatial uniformity of the ALD ZnO films and the O(3) concentration in the reactor as a function of the O(3) exposure were explained by a transition from reaction- to recombination-limited growth. This explanation was validated using a simple plug-flow model. Finally, we estimated the maximum aspect ratios that can be coated for a given O(3) recombination probability in O(3)-based ALD processes using reasonable cycle times. C1 [Knoops, Harm C. M.] M2i, Mat Innovat Inst, NL-2600 GA Delft, Netherlands. [Knoops, Harm C. M.; Kessels, Wilhelmus M. M.] Eindhoven Univ Technol, NL-5600 MB Eindhoven, Netherlands. [Elam, Jeffrey W.; Libera, Joseph A.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. RP Knoops, HCM (reprint author), M2i, Mat Innovat Inst, POB 5008, NL-2600 GA Delft, Netherlands. EM H.C.M.Knoops@tue.nl OI Knoops, Harm/0000-0003-2284-4477 FU Materials innovation institute M2i [MC3.06278]; U.S. Department of Energy; EERE-Solar Energy Technologies Program [FWP-4911A]; U.S. Department of Energy Office of Science Laboratory, UChicago Argonne, LLC [DE-AC02-06CH11357] FX This work was sponsored by the Materials innovation institute M2i (www.m2i.nl) under project number MC3.06278. The work at Argonne was supported by the U.S. Department of Energy, EERE-Solar Energy Technologies Program under FWP-4911A. Argonne National Laboratory is a U.S. Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. NR 38 TC 34 Z9 35 U1 1 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 J9 CHEM MATER JI Chem. Mat. PD MAY 10 PY 2011 VL 23 IS 9 BP 2381 EP 2387 DI 10.1021/cm2001144 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 757DC UT WOS:000290063600014 ER PT J AU Dachraoui, W Yang, T Liu, C King, G Hadermann, J Van Tendeloo, G Llobet, A Greenblatt, M AF Dachraoui, Walid Yang, Tao Liu, Chang King, Graham Hadermann, Joke Van Tendeloo, Gustaaf Llobet, Anna Greenblatt, Martha TI Short-Range Layered A-Site Ordering in Double Perovskites NaLaBB ' O-6 (B = Mn, Fe; B ' = Nb, Ta) SO CHEMISTRY OF MATERIALS LA English DT Article DE double perovskite; layered ordering; electron microscopy; magnetic ID MAGNETIC-PROPERTIES; CATIONS; SB; DIFFRACTION; CUPRATE; SR AB The new compounds NaLaFeTaO6, NaLaFeNbO6, NaLaMnTaO6, and NaLaMnNbO6 have been synthesized and characterized with a combination of transmission electron microscopy, X-ray powder diffraction (XRPD), neutron powder diffraction (NPD), and magnetization measurements. Through electron microscopy study, a local layered order of the A-cations has been detected without the typical occurrence of rock salt order at the B-cation site. Satellite reflections in the electron diffraction related to the local layered order are not visible on the XRPD or NPD patterns. The occurrence of local layered order is supported by pair distribution function analysis, which also reveals the presence of uncorrelated displacements of the Nb and Ta cations. The octahedra are tilted according to the system a(-)b(+)a(-), and the coordinates were refined from XRPD and NPD with a disordered cation distribution in the space group Pnma. The magnetic exchange interactions in NaLaFeTaO6 and NaLaFeNbO6 are antiferromagnetic, while they are ferromagnetic in NaLaMnTaO6 and NaLaMnNbO6. Long-range magnetic ordering is not observed down to 4 K for any of the compositions. C1 [Yang, Tao; Liu, Chang; Greenblatt, Martha] Rutgers State Univ, Dept Chem & Chem Biol, Piscataway, NJ 08854 USA. [Dachraoui, Walid; Hadermann, Joke; Van Tendeloo, Gustaaf] Univ Antwerp, EMAT, B-2020 Antwerp, Belgium. [Liu, Chang] Jilin Univ, State Key Lab Inorgan Synth & Preparat Chem, Coll Chem, Changchun 130012, Peoples R China. [King, Graham; Llobet, Anna] Los Alamos Natl Lab, Manuel Lujan Jr Neutron Scattering Ctr, Los Alamos, NM 87545 USA. RP Greenblatt, M (reprint author), Rutgers State Univ, Dept Chem & Chem Biol, 610 Taylor Rd Piscataway, Piscataway, NJ 08854 USA. EM martha@rutchem.rutgers.edu RI King, Graham/E-3632-2010; Llobet, Anna/B-1672-2010; Hadermann, Joke/F-4644-2011 OI King, Graham/0000-0003-1886-7254; FU NSF-DMR [0541911]; European Union [026019]; DOE Office of Basic Energy Sciences; DOE [DE-AC52 06NA25396]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was partially supported by NSF-DMR 0541911 grant (M.G., T.Y.). W.D., J.H., and G.V.T. acknowledge financial support from the European Union under the Framework 6 program under a contract for an Integrated Infrastructure Initiative, Reference 026019 ESTEEM. This work has benefited from the use of HIPD at the Lujan Center at Los Alamos Neutron Science Center, funded by DOE Office of Basic Energy Sciences. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE Contract DE-AC52 06NA25396. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 28 TC 12 Z9 12 U1 5 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 J9 CHEM MATER JI Chem. Mat. PD MAY 10 PY 2011 VL 23 IS 9 BP 2398 EP 2406 DI 10.1021/cm200226u PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 757DC UT WOS:000290063600016 ER PT J AU Hu, YY Liu, XP Ma, X Rawal, A Prozorov, T Akinc, M Mallapragada, SK Schmidt-Rohr, K AF Hu, Y. -Y. Liu, X. P. Ma, X. Rawal, A. Prozorov, T. Akinc, M. Mallapragada, S. K. Schmidt-Rohr, K. TI Biomimetic Self-Assembling Copolymer-Hydroxyapatite Nanocomposites with the Nanocrystal Size Controlled by Citrate SO CHEMISTRY OF MATERIALS LA English DT Article DE bioinspired materials; biocompatibility; bone; crystal control; hybrid materials; nuclear magnetic resonance ID CALCIUM-PHOSPHATE NANOCOMPOSITES; CITRIC-ACID; NMR-SPECTROSCOPY; BONE; MINERALIZATION; COMPOSITES; COLLAGEN; POLYMER; NUCLEATION; MICROSCOPY AB Citrate binds strongly to the surface of calcium phosphate (apatite) nanocrystals in bone and is thought to prevent crystal thickening. In this work, citrate added as a regulatory element enabled molecular control of the size and stability of hydroxyapatite (HAp) nanocrystals in synthetic nanocomposites, fabricated with self-assembling block copolymer templates. The decrease of the HAp crystal size within the polymer matrix with increasing citrate concentration was documented by solid-state nuclear magnetic resonance (NMR) techniques and wide-angle X-ray diffraction (XRD), while the shapes of HAp nanocrystals were determined by transmission electron microscopy (TEM). Advanced NMR techniques were used to characterize the interfacial species and reveal enhanced interactions between mineral and organic matrix, concomitant with the size effects. The surface-to-volume ratios determined by NMR spectroscopy and long-range (31)P{(1)H} dipolar dephasing show that 2, 10, and 40 mM citrate changes the thicknesses of the HAp crystals from 4 nm without citrate to 2.9, 2.8, and 2.3 nm, respectively. With citrate concentrations comparable to those in body fluids, HAp nanocrystals of sizes and morphologies similar to those in avian and bovine bones have been produced. C1 [Hu, Y. -Y.; Liu, X. P.; Ma, X.; Rawal, A.; Prozorov, T.; Akinc, M.; Mallapragada, S. K.; Schmidt-Rohr, K.] Ames Lab, Ames, IA 50011 USA. RP Schmidt-Rohr, K (reprint author), Ames Lab, Ames, IA 50011 USA. EM srohr@iastate.edu RI Mallapragada, Surya/F-9375-2012; Hu, Yan-Yan/A-1795-2015 OI Hu, Yan-Yan/0000-0003-0677-5897 FU U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering; Iowa State University [DE-AC02-07CH11358] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering. The research was performed at the Ames Laboratory. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract DE-AC02-07CH11358. Thanks to Dr. Jennifer O'Donnell (Iowa State University) for helping to perform the SANS experiments, and to Dr. Bosiljka Njegic for help with the TOC figure. NR 48 TC 43 Z9 44 U1 7 U2 74 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 J9 CHEM MATER JI Chem. Mat. PD MAY 10 PY 2011 VL 23 IS 9 BP 2481 EP 2490 DI 10.1021/cm200355n PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 757DC UT WOS:000290063600025 ER PT J AU Polaske, NW McGrath, DV McElhanon, JR AF Polaske, Nathan W. McGrath, Dominic V. McElhanon, James R. TI Thermally Reversible Dendronized Linear AB Step-Polymers via "Click" Chemistry SO MACROMOLECULES LA English DT Article ID DIELS-ALDER REACTION; BEARING FURAN MOIETIES; ONE-POT SYNTHESIS; HIGHLY EFFICIENT; CROSS-LINKING; COPOLYMERS; DENDRIMERS; ADDUCTS; POLYMERIZATION; BISMALEIMIDES AB The synthesis and characterization of thermally labile dendronized linear AB step-polymers is described. First through third generation dendritic AB monomers 14a-c containing both a furan and furan-protected maleimide functionality were prepared by the Cu(I)-catalyzed azide-alkyne cycloaddition reaction followed by polymerization via the thermally reversible furan-maleimide Diels-Alder reaction. The assembly, disassembly, and reassembly behavior of linear dendronized step-polymers 16a-c was studied by GPC. C1 [Polaske, Nathan W.; McGrath, Dominic V.] Univ Arizona, Dept Chem, Tucson, AZ 85721 USA. [McElhanon, James R.] Sandia Natl Labs, Organ Mat Dept, Albuquerque, NM 87185 USA. RP McGrath, DV (reprint author), Univ Arizona, Dept Chem, Tucson, AZ 85721 USA. EM mcgrath@email.arizona.edu; jrmcelh@sandia.gov RI McGrath, Dominic/A-7675-2012 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation [DE-AC04-94AL85000] FX Research supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. Certain trade names and company products are identified in order to specify experimental procedures adequately. In no case does such identification imply recommendation or endorsement by the National Institute of Standards and Technology, nor does it imply that the products are necessarily the best available for the purpose. NR 63 TC 21 Z9 21 U1 4 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 J9 MACROMOLECULES JI Macromolecules PD MAY 10 PY 2011 VL 44 IS 9 BP 3203 EP 3210 DI 10.1021/ma200296t PG 8 WC Polymer Science SC Polymer Science GA 757CE UT WOS:000290060900003 ER PT J AU Guedj, J Bazzoli, C Neumann, AU Mentre, F AF Guedj, Jeremie Bazzoli, Caroline Neumann, Avidan U. Mentre, France TI Design evaluation and optimization for models of hepatitis C viral dynamics SO STATISTICS IN MEDICINE LA English DT Article DE design evaluation; design optimization; hepatitis C; non-linear mixed effect models; ordinary differential equations; viral kinetics ID MIXED-EFFECTS MODELS; FISHER INFORMATION MATRIX; PEGINTERFERON ALPHA-2A; VIRUS-INFECTION; HIV DYNAMICS; KINETICS; PHARMACOKINETICS; IDENTIFIABILITY; INTERFERON; STANDARD AB Mathematical modeling of hepatitis C viral (HCV) kinetics is widely used for understanding viral pathogenesis and predicting treatment outcome. The standard model is based on a system of five non-linear ordinary differential equations (ODE) that describe both viral kinetics and changes in drug concentration after treatment initiation. In such complex models parameter estimation is challenging and requires frequent sampling measurements on each individual. By borrowing information between study subjects, non-linear mixed effect models can deal with sparser sampling from each individual. However, the search for optimal designs in this context has been limited by the numerical difficulty of evaluating the Fisher information matrix (FIM). Using the software PFIM, we show that a linearization of the statistical model avoids most of the computational burden, while providing a good approximation to the FIM. We then compare the precision of the parameters that can be expected using five study designs from the literature. We illustrate the usefulness of rationalizing data sampling by showing that, for a given level of precision, optimal design could reduce the total number of measurements by up 50 per cent. Our approach can be used by a statistician or a clinician aiming at designing an HCV viral kinetics study. Copyright (C) 2011 John Wiley & Sons, Ltd. C1 [Guedj, Jeremie] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Neumann, Avidan U.] Bar Ilan Univ, Everard & Mina Goodman Fac Life Sci, IL-52900 Ramat Gan, Israel. [Bazzoli, Caroline; Mentre, France] INSERM, UMR 738, F-75018 Paris, France. [Bazzoli, Caroline; Mentre, France] Univ Paris Diderot, F-75018 Paris, France. [Neumann, Avidan U.] Santa Fe Inst, Santa Fe, NM 87501 USA. RP Guedj, J (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM jeremie.guedj@gmail.com RI Guedj, Jeremie/A-6842-2017 OI Guedj, Jeremie/0000-0002-5534-5482 FU French Ministry of Foreign Affairs; Israel Science Foundation [ISF 939/2008]; US Department of Energy [RR06555, P20-RR18754] FX We thank L. Murillo, A. Smith and A. S. Perelson (LANL) for helpful comments; we are also grateful to both anonymous reviewers and the AE for very insightful remarks. This work was supported by the French Ministry of Foreign Affairs, the Israel Science Foundation (ISF 939/2008) and the US Department of Energy under contract RR06555 and P20-RR18754. NR 38 TC 9 Z9 9 U1 0 U2 2 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0277-6715 J9 STAT MED JI Stat. Med. PD MAY 10 PY 2011 VL 30 IS 10 BP 1045 EP 1056 DI 10.1002/sim.4191 PG 12 WC Mathematical & Computational Biology; Public, Environmental & Occupational Health; Medical Informatics; Medicine, Research & Experimental; Statistics & Probability SC Mathematical & Computational Biology; Public, Environmental & Occupational Health; Medical Informatics; Research & Experimental Medicine; Mathematics GA 756GT UT WOS:000290000400001 PM 21337592 ER PT J AU Diaz-San Segundo, F Weiss, M Perez-Martin, E Koster, MJ Zhu, J Grubman, MJ de los Santos, T AF Diaz-San Segundo, Fayna Weiss, Marcelo Perez-Martin, Eva Koster, Marla J. Zhu, James Grubman, Marvin J. de los Santos, Teresa TI Antiviral activity of bovine type III interferon against foot-and-mouth disease virus SO VIROLOGY LA English DT Article DE FMDV; Interferon; Bovine interferon lambda; IFN-lambda; IL28B; Interferon stimulated genes; Antiviral activity ID RAPIDLY PROTECTS SWINE; IFN-LAMBDA; ALPHA/BETA INTERFERON; EXPRESSION; REPLICATION; CELLS; COMBINATION; INFECTIONS; INDUCTION; SYSTEM AB Foot-and-mouth disease (FMD) is one of the most serious threats to the livestock industry. Despite the availability of a vaccine, recent outbreaks in disease-free countries have demonstrated that development of novel FMD control strategies is imperative. Here we report the identification and characterization of bovine (bo) interferon lambda 3 (IFN-lambda 3), a member of the type III IFN family. Expression of bolFN-lambda 3 using a replication-defective human adenovirus type 5 vector (Ad5-bolFN-lambda 3) yielded a glycosylated secreted protein with antiviral activity against FMD virus (FMDV) and vesicular stomatitis virus in bovine cell culture. Inoculation of cattle with Ad5-bolFN-lambda 3 induced systemic antiviral activity and up-regulation of IFN stimulated gene expression in multiple tissues susceptible to FMDV infection. Our results demonstrate that the type III IFN family is conserved in bovines and bolFN-lambda 3 has potential for further development as a biotherapeutic candidate to inhibit FMDV or other viruses in cattle. Published by Elsevier Inc. C1 [Diaz-San Segundo, Fayna; Weiss, Marcelo; Perez-Martin, Eva; Koster, Marla J.; Zhu, James; Grubman, Marvin J.; de los Santos, Teresa] ARS, Plum Isl Anim Dis Ctr, N Atlantic Area, USDA, Greenport, NY 11944 USA. [Diaz-San Segundo, Fayna; Weiss, Marcelo; Perez-Martin, Eva] PIADC Res Participat Program, Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA. RP de los Santos, T (reprint author), ARS, Plum Isl Anim Dis Ctr, N Atlantic Area, USDA, Greenport, NY 11944 USA. EM teresa.delosantos@ars.usda.gov RI Weiss, Marcelo/I-1274-2012 OI Weiss, Marcelo/0000-0001-7902-3210 FU Plum Island Animal Disease Research Participation Program; CRIS [1940-32000-053-00D ARS]; USDA (Teresa de los Santos and Marvin J. Grubman); Department of Homeland Security [60-1940-9-028, 60-1940-7-047] FX This research was supported in part by the Plum Island Animal Disease Research Participation Program administered by the Oak Ridge Institute for Science and Education through an interagency agreement between the U.S. Department of Energy and the U.S. Department of Agriculture (appointments of Fayna Diaz-San Segundo, Marcelo Weiss and Eva Perez-Martin), by CRIS project number 1940-32000-053-00D ARS, USDA (Teresa de los Santos and Marvin J. Grubman) and by reimbursable agreements with the Department of Homeland Security 60-1940-9-028 Task 3a (Teresa de los Santos) and 60-1940-7-047 (Marvin J. Grubman). We thank Dr Jonathan Arzt for advice in bovine necropsies, Camila Dias, Betty Bishop, Traci Turecek and Beatriz Garbelotti Matias for technical support and Dr Zhiqiang Lu for DNA sequencing. We are also thankful to the Plum Island animal caretakers for their superb assistance with animal experiments. NR 45 TC 13 Z9 13 U1 3 U2 6 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0042-6822 J9 VIROLOGY JI Virology PD MAY 10 PY 2011 VL 413 IS 2 BP 283 EP 292 DI 10.1016/j.virol.2011.02.023 PG 10 WC Virology SC Virology GA 757CS UT WOS:000290062400015 PM 21435672 ER PT J AU Turner, DZ Nakshatrala, KB Hjelmstad, KD AF Turner, D. Z. Nakshatrala, K. B. Hjelmstad, K. D. TI A stabilized formulation for the advection-diffusion equation using the Generalized Finite Element Method SO INTERNATIONAL JOURNAL FOR NUMERICAL METHODS IN FLUIDS LA English DT Article DE advection-diffusion equation; Generalized Finite Element Method; eXtended finite element method; stabilized methods; partition of unity framework; non-polynomial enrichment functions ID ESSENTIAL BOUNDARY-CONDITIONS; MESH-FREE METHODS; BUBBLE FUNCTIONS; MULTISCALE AB This paper presents a stable formulation for the advection-diffusion equation based on the Generalized (or eXtended) Finite Element Method, GFEM (or X-FEM). Using enrichment functions that represent the exponential character of the exact solution, smooth numerical solutions are obtained for problems with steep gradients and high Peclet numbers in one-and two-dimensions. In contrast with traditional stabilized methods that require the construction of stability parameters and stabilization terms, the present work avoids numerical instabilities by improving the classical Galerkin solution with enrichment functions (that need not be polynomials) using GFEM, which is an instance of the partition of unity framework. This work also presents a strategy for constructing enrichment functions for problems involving complex geometries by employing a global-local-type approach. Representative numerical results are presented to illustrate the performance of the proposed method. Copyright (C) 2010 John Wiley & Sons, Ltd. C1 [Turner, D. Z.] Sandia Natl Labs, Computat Thermal & Fluid Mech Dept, Albuquerque, NM 87112 USA. [Nakshatrala, K. B.] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. [Hjelmstad, K. D.] Arizona State Univ, Coll Technol & Innovat, Mesa, AZ 85212 USA. RP Turner, DZ (reprint author), Sandia Natl Labs, Computat Thermal & Fluid Mech Dept, Mail Stop 0836,POB 5800, Albuquerque, NM 87112 USA. EM dzturne@sandia.gov RI Nakshatrala, Kalyana Babu/C-5813-2012; Turner, Daniel/E-7008-2012; Nakshatrala, Kalyana/F-2490-2014 FU Department of Energy [DOE DE-FC02-07ER64323]; UIUC FX Contract/grant sponsor: Department of Energy; contract/grant number: DOE DE-FC02-07ER64323; The research reported herein was partly supported (D.Z.T.) by the Computational Science and Engineering Fellowship at UIUC, and (K.B.N.) by the Department of Energy through a SciDAC-2 project (Grant No. DOE DE-FC02-07ER64323). This support is gratefully acknowledged. The opinions expressed in this paper are those of the authors and do not necessarily reflect that of the sponsors. NR 49 TC 12 Z9 12 U1 1 U2 7 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0271-2091 EI 1097-0363 J9 INT J NUMER METH FL JI Int. J. Numer. Methods Fluids PD MAY 10 PY 2011 VL 66 IS 1 BP 64 EP 81 DI 10.1002/fld.2248 PG 18 WC Computer Science, Interdisciplinary Applications; Mathematics, Interdisciplinary Applications; Mechanics; Physics, Fluids & Plasmas SC Computer Science; Mathematics; Mechanics; Physics GA 748DK UT WOS:000289370000005 ER PT J AU Shen, CP Qiu, JM Christlieb, A AF Shen, Chaopeng Qiu, Jing-Mei Christlieb, Andrew TI Adaptive mesh refinement based on high order finite difference WENO scheme for multi-scale simulations SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Adaptive mesh refinement (AMR); WENO; High order finite difference; Multiscale simulations ID SHOCK-CAPTURING SCHEMES; DISCONTINUOUS GALERKIN METHODS; COMPRESSIBLE EULER EQUATIONS; TIME CONSERVATION ELEMENT; EFFICIENT IMPLEMENTATION; HYPERBOLIC SYSTEMS; LAWS; DISCRETIZATIONS; ALGORITHMS; ERROR AB In this paper, we propose a finite difference AMR-WENO method for hyperbolic conservation laws. The proposed method combines the adaptive mesh refinement (AMR) framework 14,51 with the high order finite difference weighted essentially non-oscillatory (WENO) method in space and the total variation diminishing (TVD) Runge-Kutta (RK) method in time (WENO-RK) [18,10] by a high order coupling. Our goal is to realize mesh adaptivity in the AMR framework, while maintaining very high (higher than second) order accuracy of the WENO-RK method in the finite difference setting. The high order coupling of AMR and WENO-RK is accomplished by high order prolongation in both space (WENO interpolation) and time (Hermite interpolation) from coarse to fine grid solutions, and at ghost points. The resulting AMR-WENO method is accurate, robust and efficient, due to the mesh adaptivity and very high order spatial and temporal accuracy. We have experimented with both the third and the fifth order AMR-WENO schemes. We demonstrate the accuracy of the proposed scheme using smooth test problems, and their quality and efficiency using several 1D and 2D nonlinear hyperbolic problems with very challenging initial conditions. The AMR solutions are observed to perform as well as, and in some cases even better than, the corresponding uniform fine grid solutions. We conclude that there is significant improvement of the fifth order AMR-WENO over the third order one, not only in accuracy for smooth problems, but also in its ability in resolving complicated solution structures, due to the very low numerical diffusion of high order schemes. In our work, we found that it is difficult to design a robust AMR-WENO scheme that is both conservative and high order (higher than second order), due to the mass inconsistency of coarse and fine grid solutions at the initial stage in a finite difference scheme. Resolving these issues as well as conducting comprehensive evaluation of computational efficiency constitute our future work. (C) 2011 Elsevier Inc. All rights reserved. C1 [Shen, Chaopeng] Michigan State Univ, Dept Civil & Environm Engn, E Lansing, MI 48824 USA. [Qiu, Jing-Mei] Colorado Sch Mines, Dept Math & Comp Sci, Golden, CO 80401 USA. [Christlieb, Andrew] Michigan State Univ, Dept Math, E Lansing, MI 48824 USA. RP Shen, CP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Computat Res Div, Berkeley, CA 94720 USA. EM cshen@lbl.gov; jingqiu@mines.edu; Christlieb@math.msu.edu OI Shen, Chaopeng/0000-0002-0685-1901 FU NOAA Center of Excellence for Great Lakes and Human Health; Air Force Office of Scientific Computing; National Science Foundation FX We thank Dr. Chi-Wang Shu for incisive suggestions and generous help. We thank Dr. Randy Leveque for constructive advice We thank the anonymous reviewers, as well as Dr. W. Nicolas G. Hitchon whose useful comments and suggestions led to the improved version of the manuscript. The first author was supported by NOAA Center of Excellence for Great Lakes and Human Health. The second and third authors were supported by Air Force Office of Scientific Computing and the National Science Foundation. NR 35 TC 29 Z9 31 U1 0 U2 12 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 J9 J COMPUT PHYS JI J. Comput. Phys. PD MAY 10 PY 2011 VL 230 IS 10 BP 3780 EP 3802 DI 10.1016/j.jcp.2011.02.008 PG 23 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 751DK UT WOS:000289597500009 ER PT J AU Jakeman, JD Archibald, R Xiu, DB AF Jakeman, John D. Archibald, Richard Xiu, Dongbin TI Characterization of discontinuities in high-dimensional stochastic problems on adaptive sparse grids SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Adaptive sparse grids; Stochastic partial differential equations; Multivariate discontinuity detection; Generalized polynomial chaos method; High-dimensional approximation ID PARTIAL-DIFFERENTIAL-EQUATIONS; RANDOM INPUT DATA; COLLOCATION METHOD; POLYNOMIAL CHAOS; EDGE-DETECTION; UNCERTAINTY AB In this paper we present a set of efficient algorithms for detection and identification of discontinuities in high dimensional space. The method is based on extension of polynomial annihilation for discontinuity detection in low dimensions. Compared to the earlier work, the present method poses significant improvements for high dimensional problems. The core of the algorithms relies on adaptive refinement of sparse grids. It is demonstrated that in the commonly encountered cases where a discontinuity resides on a small subset of the dimensions, the present method becomes "optimal", in the sense that the total number of points required for function evaluations depends linearly on the dimensionality of the space. The details of the algorithms will be presented and various numerical examples are utilized to demonstrate the efficacy of the method. (C) 2011 Elsevier Inc. All rights reserved. C1 [Jakeman, John D.] Australian Natl Univ, Dept Math, Canberra, ACT 0200, Australia. [Archibald, Richard] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Xiu, Dongbin] Purdue Univ, Dept Math, W Lafayette, IN 47907 USA. RP Jakeman, JD (reprint author), Australian Natl Univ, Dept Math, Canberra, ACT 0200, Australia. EM john.jakeman@anu.edu.au; ArchibaldRK@ORNL.gov; dxiu@purdue.edu RI Archibald, Rick/I-6238-2016 OI Archibald, Rick/0000-0002-4538-9780 FU US Government [DE-AC05-00OR22725]; AFOSR [FA9550-08-1-0353]; DOE/NNSA [DE-FC52-08NA28617]; NSF [DMS-0645035, IIS-0914447] FX The submitted manuscript has been authored by contractors [UT-Battelle LLC, manager of Oak Ridge National Laboratory (ORNL)] of the US Government under Contract No. DE-AC05-00OR22725. Accordingly, the US Government retains a non-exclusive, royalty-free license to publish or reproduce the published form of this contribution, or allow others to do so, for US Government purposes. Dongbin Xiu was partially supported by AFOSR FA9550-08-1-0353, DOE/NNSA DE-FC52-08NA28617, and NSF CAREER DMS-0645035 and IIS-0914447. NR 35 TC 14 Z9 14 U1 1 U2 8 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 J9 J COMPUT PHYS JI J. Comput. Phys. PD MAY 10 PY 2011 VL 230 IS 10 BP 3977 EP 3997 DI 10.1016/j.jcp.2011.02.022 PG 21 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 751DK UT WOS:000289597500019 ER PT J AU Daval, D Sissmann, O Menguy, N Saldi, GD Guyot, F Martinez, I Corvisier, J Garcia, B Machouk, I Knauss, KG Hellmann, R AF Daval, Damien Sissmann, Olivier Menguy, Nicolas Saldi, Giuseppe D. Guyot, Francois Martinez, Isabelle Corvisier, Jerome Garcia, Bruno Machouk, Imene Knauss, Kevin G. Hellmann, Roland TI Influence of amorphous silica layer formation on the dissolution rate of olivine at 90 degrees C and elevated pCO(2) SO CHEMICAL GEOLOGY LA English DT Article DE Olivine; Carbonation; CO2 sequestration; Passivation; Kinetic modeling ID AQUEOUS MINERAL CARBONATION; BASALTIC GLASS DISSOLUTION; ALBITE-WATER SYSTEM; FORSTERITE DISSOLUTION; CO2 SEQUESTRATION; WOLLASTONITE CARBONATION; NUMERICAL-SIMULATION; SATURATION STATE; HIGH-RESOLUTION; NEAR-SURFACE AB For mitigating against rising levels of atmospheric CO2, carbonation of M2+-bearing silicates has been proposed as a possible option for sequestering CO2 over long time spans. Due to its rapid far-from-equilibrium dissolution rate and its widespread occurrence in mafic and ultramafic rocks, olivine has been suggested as a potentially good candidate for achieving this goal, although the efficacy of the carbonation reaction still needs to be assessed. With this as a goal, the present study aims at measuring the carbonation rate of San Carlos olivine in batch experiments at 90 degrees C and pCO(2) of 20 and 25 MPa. When the reaction was initiated in pure water, the kinetics of olivine dissolution was controlled by the degree of saturation of the bulk solution with respect to amorphous silica. This yet unrecognized effect for olivine was responsible for a decrease of the dissolution rate by over two orders of magnitude. In long-term (45 days) carbonation experiments with a high surface area to solution volume ratio (SA/V=24,600 m(-1)), the final composition of the solution was close to equilibrium with respect to SiO2(am), independent of the initial concentration of dissolved salts (NaCl and NaClO4, ranging between 0 and 1 m), and with an aqueous Mg/Si ratio close to that of olivine. No secondary phase other than a ubiquitous thin (<= 40 nm), Si-rich amorphous layer was observed. These results are at odds with classic kinetic modeling of the process. Due to experimental uncertainties, it was not possible to determine precisely the dissolution rate of olivine after 45 days. but the long term alteration of olivine was indirectly estimated to be at least 4 orders of magnitude slower than predicted. Taken together, these results suggest that the formation of amorphous silica layers plays an important role in controlling the rate of olivine dissolution by passivating the surface of olivine, an effect which has yet to be quantified and incorporated into standard reactive-transport codes. Published by Elsevier B.V. C1 [Daval, Damien; Saldi, Giuseppe D.; Knauss, Kevin G.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Daval, Damien; Sissmann, Olivier; Guyot, Francois; Martinez, Isabelle] Ctr Rech Stockage Geol CO2, Inst Phys Globe Paris, F-75238 Paris 05, France. [Daval, Damien; Sissmann, Olivier; Corvisier, Jerome] Ecole Normale Super, Geol Lab, CNRS, UMR 8538, F-75005 Paris, France. [Menguy, Nicolas; Guyot, Francois; Machouk, Imene] Univ Paris 06, Inst Mineral & Phys Milieux Condenses, CNRS, F-75252 Paris, France. [Garcia, Bruno] IFP Energies Nouvelles, F-92852 Rueil Malmaison, France. [Hellmann, Roland] Univ Grenoble 1, Lab Geophys Interne & Tectonophys, CNRS, OSUG,UMR C5559, F-38041 Grenoble 9, France. RP Daval, D (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Earth Sci, MS 90R-1116,1 Cyclotron Rd, Berkeley, CA 94720 USA. EM ddaval@lbl.gov RI Daval, Damien/H-1116-2011; MENGUY, Nicolas/F-5607-2012; knauss, kevin/K-2827-2012; 3G, Direction Geologie/C-1699-2013; GUYOT, Francois/C-3824-2016; IMPMC, Geobio/F-8819-2016; IFPEN, Publications/A-8028-2008 OI MENGUY, Nicolas/0000-0003-4613-2490; GUYOT, Francois/0000-0003-4622-2218; NR 80 TC 102 Z9 102 U1 12 U2 88 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 J9 CHEM GEOL JI Chem. Geol. PD MAY 9 PY 2011 VL 284 IS 1-2 BP 193 EP 209 DI 10.1016/j.chemgeo.2011.02.021 PG 17 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 768YJ UT WOS:000290975500016 ER PT J AU Guzman, J Boswell-Koller, CN Beeman, JW Bustillo, KC Conry, T Dubon, OD Hansen, WL Levander, AX Liao, CY Lieten, RR Sawyer, CA Sherburne, MP Shin, SJ Stone, PR Watanabe, M Yu, KM Ager, JW Chrzan, DC Haller, EE AF Guzman, J. Boswell-Koller, C. N. Beeman, J. W. Bustillo, K. C. Conry, T. Dubon, O. D. Hansen, W. L. Levander, A. X. Liao, C. Y. Lieten, R. R. Sawyer, C. A. Sherburne, M. P. Shin, S. J. Stone, P. R. Watanabe, M. Yu, K. M. Ager, J. W., III Chrzan, D. C. Haller, E. E. TI Reversible phase changes in Ge-Au nanoparticles SO APPLIED PHYSICS LETTERS LA English DT Article ID NANOCRYSTALS; MEMORY AB We demonstrate a reversible phase transition in nanoparticles composed of a binary eutectic alloy, Ge-Au. The structure, 9 nm diameter nanoparticles embedded in silica, can be switched from bilobe to mixed using a 30 ns ultraviolet laser pulse. The structure can be switched back to bilobe by heating at 80 degrees C. The bilobe/mixed switching can be performed on the same sample at least ten times. Synchrotron X-ray diffraction studies reveal that the bilobe structure contains crystalline Ge and Au while the mixed structure consists of crystalline Ge and beta Ge-Au. (C) 2011 American Institute of Physics. [doi:10.1063/1.3584850] C1 [Guzman, J.; Boswell-Koller, C. N.; Beeman, J. W.; Bustillo, K. C.; Conry, T.; Dubon, O. D.; Hansen, W. L.; Levander, A. X.; Liao, C. Y.; Lieten, R. R.; Sawyer, C. A.; Sherburne, M. P.; Shin, S. J.; Stone, P. R.; Yu, K. M.; Ager, J. W., III; Chrzan, D. C.; Haller, E. E.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Guzman, J.; Boswell-Koller, C. N.; Bustillo, K. C.; Conry, T.; Dubon, O. D.; Levander, A. X.; Liao, C. Y.; Sawyer, C. A.; Sherburne, M. P.; Shin, S. J.; Stone, P. R.; Chrzan, D. C.; Haller, E. E.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Watanabe, M.] Univ Calif Berkeley, Lawrence Berkeley Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. RP Haller, EE (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM eehaller@lbl.gov RI Yu, Kin Man/J-1399-2012; OI Yu, Kin Man/0000-0003-1350-9642; Ager, Joel/0000-0001-9334-9751 FU Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation (NSF) [DMR-0902179]; Berkeley Graduate Fellowship; Intel Ph.D. Fellowship; U.S. NSF [DMR-0902179]; U.S. Department of Energy [DE-AC02-05CH11231] FX The work at the Lawrence Berkeley National Laboratory was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 [Raman spectroscopy and Rutherford backscattering spectrometry] and by the National Science Foundation (NSF) under Contract No. DMR-0902179 [Sample fabrication]. J.G. acknowledges support from the Berkeley Graduate Fellowship, the Intel Ph.D. Fellowship, and U.S. NSF Grant No. DMR-0902179. S.J.S. was supported by the NSF IGERT program. P. R. S. acknowledges fellowship support from the NSF. Electron microscopy experiments were performed as a user project at the National Center for Electron Microscopy, Lawrence Berkeley National Laboratory, which is supported by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Synchrotron X-ray diffraction experiments were performed at SSRL, a national user facility operated by Stanford University on behalf of the U. S. Department of Energy, Office of Basic Energy Sciences. The authors thank Apurva Mehta for his expert support at SSRL. NR 17 TC 6 Z9 6 U1 0 U2 25 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. 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Rubinov, R. Ruchti, R. Safronov, G. Sajot, G. Sanchez-Hernandez, A. Sanders, M. P. Sanghi, B. Santos, A. S. Savage, G. Sawyer, L. Scanlon, T. Schamberger, R. D. Scheglov, Y. Schellman, H. Schliephake, T. Schlobohm, S. Schwanenberger, C. Schwienhorst, R. Sekaric, J. Severini, H. Shabalina, E. Shary, V. Shchukin, A. A. Shivpuri, R. K. Simak, V. Sinthuprasith, T. Sirotenko, V. Skubic, R. Slattery, R. Smirnov, D. Smith, K. J. Snow, G. R. Snow, J. Snyder, S. Soldner-Rembold, S. Sonnenschein, L. Sopczak, A. Sosebee, M. Soustruznik, K. Spurlock, B. Stark, J. Stolin, V. Stoyanova, D. A. Strauss, M. Strom, D. Stutte, L. Suter, L. Svoisky, R. Takahashi, M. Tanasijczuk, A. Taylor, W. Titov, M. Tokmenin, V. V. Tsai, Y. -T. Tsybychev, D. Tuchming, B. Tully, C. Tuts, P. M. Uvarov, L. Uvarov, S. Uzunyan, S. Van Kooten, R. van Leeuwen, W. M. Varelas, N. Varnes, E. W. Vasilyev, I. A. Verdier, P. Vertogradov, L. S. Verzocchi, M. Vesterinen, M. Vilanova, D. Vint, R. Vokac, R. Wahl, H. D. Wang, M. H. L. S. Warchol, J. Watts, G. Wayne, M. Weber, M. Welty-Rieger, L. White, A. Wicke, D. Williams, M. R. J. Wilson, G. W. Wimpenny, S. J. Wobisch, M. Wood, D. R. Wyatt, T. R. Xie, Y. Xu, C. Yacoob, S. Yamada, R. Yang, W. -C. Yasuda, T. Yatsunenko, Y. A. Ye, Z. Yin, H. Yip, K. Youn, S. W. Yu, J. Zelitch, S. Zhao, T. Zhou, B. Zhu, J. Zielinski, M. Zieminska, D. Zivkovic, L. CA DO Collaboration TI Search for W' -> tb resonances with left- and right-handed couplings to fermions D0 Collaboration SO PHYSICS LETTERS B LA English DT Article DE Wprime; Resonances; Top quark; Bottom quark; Left-right couplings ID IDENTIFICATION; EVENTS AB We present a search for the production of a heavy gauge boson, W', that decays to third-generation quarks, by DO Collaboration in p (p) over bar) collisions at root s = 1.96 TeV. We set 95% confidence level upper limits on the production cross section times branching fraction. For the first time, we set limits for arbitrary combinations of left-and right-handed couplings of the W' boson to fermions. For couplings with the same strength as for the standard model W boson, we set the following limits, assuming that there are right-handed neutrinos nu(R) for all three generations with M(W') > m(nu(R)): M(W') > 863 GeV for purely left-handed couplings, M(W') > 885 GeV for purely right-handed couplings, and M(W') > 916 GeV if both left-and right-handed couplings are present. The limit for right-handed couplings improves for M(W') < m(nu(R)) to M(W') > 890 GeV. (C) 2011 Elsevier B.V. All rights reserved. C1 [Abazov, V. M.; Alexeev, G. D.; Golovanov, G.; Kharzheev, Y. N.; Malyshev, V. L.; Tokmenin, V. V.; Vertogradov, L. S.; Yatsunenko, Y. A.] Joint Inst Nucl Res, Dubna, Russia. [Piegaia, R.; Tanasijczuk, A.] Univ Buenos Aires, Buenos Aires, DF, Argentina. [Alves, G. A.; Maciel, A. K. A.] Ctr Brasileiro Pesquisas Fis, LAFEX, Rio De Janeiro, Brazil. 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[Lobodenko, A.; Neustroev, R.; Obrant, G.; Scheglov, Y.; Uvarov, L.; Uvarov, S.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Asman, B.; Belanger-Champagne, C.; Buszello, C. P.] Stockholm Univ, S-10691 Stockholm, Sweden. [Asman, B.; Belanger-Champagne, C.; Buszello, C. P.] Uppsala Univ, Uppsala, Sweden. [Bertram, I.; Borissov, G.; Burdin, S.; Fox, H.; Love, P.; Ratoff, Rn.; Sopczak, A.; Williams, M. R. J.] Univ Lancaster, Lancaster LA1 4YB, England. [Beuselinck, R.; Christoudias, T.; Davies, G.; Hays, J.; Jesik, R.; Jonsson, P.; Osman, N.; Scanlon, T.; Vint, R.] Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England. [Harder, K.; Head, T.; Owen, M.; Peters, K.; Peters, Y.; Schwanenberger, C.; Soldner-Rembold, S.; Suter, L.; Takahashi, M.; Vesterinen, M.; Wyatt, T. R.; Yang, W. -C.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Das, A.; Johns, K.; Varnes, E. W.] Univ Arizona, Tucson, AZ 85721 USA. [Ellison, J.; Heinson, A. P.; Li, L.; Padilla, M.; Wimpenny, S. J.] Univ Calif Riverside, Riverside, CA 92521 USA. [Adams, T.; Askew, A.; Bandurin, D. V.; Blessing, S.; Hagopian, S.; Hoang, T.; Wahl, H. D.] Florida State Univ, Tallahassee, FL 32306 USA. [Aoki, M.; Bagby, L.; Baldin, B.; Bartlett, J. F.; Bellantoni, L.; Bhat, Rc.; Boehnlein, A.; Bross, A.; Bu, X. B.; Casey, B. C. K.; Cihangir, S.; Cooke, M.; Cooper, W. E.; Demarteau, M.; Denisov, D.; Desai, S.; Diehl, H. T.; Diesburg, M.; Elvira, V. D.; Fisk, H. E.; Fuess, S.; Ginther, G.; Greenlee, H.; Gruenendahl, S.; Gutierrez, G.; Illingworth, R.; Ito, A. S.; Johnson, M.; Jonckheere, A.; Kasper, Ra.; Khalatyan, N.; Lee, W. M.; Li, Q. Z.; Lyon, A. L.; Penning, B.; Podstavkov, V. M.; Rominsky, M.; Rubinov, R.; Sanghi, B.; Savage, G.; Sirotenko, V.; Stutte, L.; Verzocchi, M.; Weber, M.; Xie, Y.; Yamada, R.; Yasuda, T.; Ye, Z.; Yin, H.; Youn, S. W.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Adams, M.; Bazterra, V.; Gerber, C. E.; Strom, D.; Varelas, N.] Univ Illinois, Chicago, IL 60607 USA. [Blazey, G.; Chakraborty, D.; Fortner, M.; Hedin, D.; Menezes, D.; Uzunyan, S.] No Illinois Univ, De Kalb, IL 60115 USA. [Kirby, M. H.; Schellman, H.; Welty-Rieger, L.; Yacoob, S.] Northwestern Univ, Evanston, IL 60208 USA. [Evans, H.; Lammers, S.; Parua, N.; Price, D.; Van Kooten, R.; Zieminska, D.] Indiana Univ, Bloomington, IN 47405 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, IN 46323 USA. [Chan, K. M.; Hildreth, M. D.; Osta, J.; Ruchti, R.; Smirnov, D.; Warchol, J.; Wayne, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Hauptman, J. M.; Lee, S. W.; Pol, M. -E.; Range, M. S.] Iowa State Univ, Ames, IA 50011 USA. [Baringer, P.; Bean, A.; Carrasco-Lizarraga, M. A.; Chen, G.; Clutter, J.; McGivern, C. L.; Sekaric, J.; Wilson, G. W.] Univ Kansas, Lawrence, KS 66045 USA. [Bolton, T. A.; Kaadze, K.; Maravin, Y.] Kansas State Univ, Manhattan, KS 66506 USA. [Arov, M.; Greenwood, Z. D.; Sawyer, L.; Wobisch, M.] Louisiana Tech Univ, Ruston, LA 71272 USA. [Bose, T.] Boston Univ, Boston, MA 02215 USA. [Alverson, G.; Barberis, E.; Facini, G.; Haley, J.; Wood, D. R.] Northeastern Univ, Boston, MA 02115 USA. [Alton, A.; Herner, K.; Neal, H. A.; Qian, J.; Xu, C.; Zhou, B.; Zhu, J.] Univ Michigan, Ann Arbor, MI 48109 USA. [Brock, R.; Edmunds, D.; Fisher, W.; Geng, W.; Kraus, J.; Linnemann, J.; Piper, J.; Schwienhorst, R.] Michigan State Univ, E Lansing, MI 48824 USA. [Melnitchouk, A.; Quinn, B.] Univ Mississippi, University, MS 38677 USA. [Bloom, K. B. K.; Claes, D.; DeVaughan, K.; Dominguez, A.; Dyshkant, A.; Johnston, D.; Katsanos, I.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE 68588 USA. [Atramentov, O.; Duggan, D.; Gershtein, Y.] Rutgers State Univ, Piscataway, NJ 08855 USA. [Gerbaudo, D.; Tully, C.] Princeton Univ, Princeton, NJ 08544 USA. [Lashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Smith, K. J.] SUNY Buffalo, Buffalo, NY 14260 USA. [Brooijmans, G.; Haas, A.; Parsons, J.; Tuts, P. M.] Columbia Univ, New York, NY 10027 USA. [Demina, R.; Ferbel, T.; Garcia-Bellido, A.; Ginther, G.; Harel, A.; Petrillo, G.; Slattery, R.; Tsai, Y. -T.; Wang, M. H. L. S.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Boline, D.; Chakrabarti, S.; Grannis, R. P.; Guo, F.; Hobbs, J. D.; McCarthy, R.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.] SUNY Stony Brook, Stony Brook, NY 11794 USA. [Beget, M.; Evdokimov, A.; Gadfort, T.; Patwa, A.; Pleier, M. -A.; Protopopescu, S.; Snyder, S.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Snow, J.] Langston Univ, Langston, OK 73050 USA. [Abbott, B.; Gutierrez, P.; Hossain, S.; Severini, H.; Skubic, R.; Strauss, M.; Svoisky, R.] Univ Oklahoma, Norman, OK 73019 USA. [Hegab, H.; Khanov, A.; Rizatdinova, F.] Oklahoma State Univ, Stillwater, OK 74078 USA. [Cho, D. K.; Cutts, D.; Heintz, U.; Jabeen, S.; Khatidze, D.; Landsberg, G.; Narain, M.; Pangilinan, M.; Parihar, V.; Partridge, R.; Sinthuprasith, T.; Zivkovic, L.] Brown Univ, Providence, RI 02912 USA. [Brandt, A.; De, K.; Sosebee, M.; Spurlock, B.; White, A.; Yu, J.] Univ Texas Arlington, Arlington, TX 76019 USA. [Kehoe, R.; Renkel, R.] So Methodist Univ, Dallas, TX 75275 USA. [Chandra, A.; Corcoran, M.; Mackin, D.; Prewitt, M.] Rice Univ, Houston, TX 77005 USA. [Buehler, M.; Hirosky, Ba. R.; Mulhearn, M.; Zelitch, S.] Univ Virginia, Charlottesville, VA 22901 USA. [BackusMayes, J.; Burnett, T. H.; Dorland, T.; Eads, M.; Goussiou, A.; Lubatti, H. J.; Schlobohm, S.; Watts, G.; Zhao, T.] Univ Washington, Seattle, WA 98195 USA. RP Abazov, VM (reprint author), Joint Inst Nucl Res, Dubna, Russia. RI Perfilov, Maxim/E-1064-2012; Boos, Eduard/D-9748-2012; Novaes, Sergio/D-3532-2012; Santos, Angelo/K-5552-2012; Mercadante, Pedro/K-1918-2012; Alves, Gilvan/C-4007-2013; Yip, Kin/D-6860-2013; Gutierrez, Phillip/C-1161-2011; Bolton, Tim/A-7951-2012; bu, xuebing/D-1121-2012; Merkin, Mikhail/D-6809-2012; Dudko, Lev/D-7127-2012; Fisher, Wade/N-4491-2013; De, Kaushik/N-1953-2013; Ancu, Lucian Stefan/F-1812-2010; Deliot, Frederic/F-3321-2014; Sharyy, Viatcheslav/F-9057-2014; Lokajicek, Milos/G-7800-2014; Kupco, Alexander/G-9713-2014; Kozelov, Alexander/J-3812-2014; Christoudias, Theodoros/E-7305-2015; Gerbaudo, Davide/J-4536-2012; Li, Liang/O-1107-2015 OI Novaes, Sergio/0000-0003-0471-8549; Yip, Kin/0000-0002-8576-4311; Dudko, Lev/0000-0002-4462-3192; De, Kaushik/0000-0002-5647-4489; Ancu, Lucian Stefan/0000-0001-5068-6723; Sharyy, Viatcheslav/0000-0002-7161-2616; Christoudias, Theodoros/0000-0001-9050-3880; Gerbaudo, Davide/0000-0002-4463-0878; Li, Liang/0000-0001-6411-6107 FU DOE (USA); NSF (USA); CEA (France); CNRS/IN2P3 (France); FASI (Russia); Rosatom (Russia); RFBR (Russia); CNPq (Brazil); FAPERJ (Brazil); FAPESP (Brazil); FUNDUNESP (Brazil); DAE (India); DST (India); Colciencias (Colombia); CONACyT (Mexico); KRF (Korea); KOSEF (Korea); CONICET (Argentina); UBACyT (Argentina); FOM (The Netherlands); STFC (United Kingdom); Royal Society (United Kingdom); MSMT (Czech Republic); GACR (Czech Republic); CRC (Canada); NSERC (Canada); BMBF (Germany); DFG (Germany); SFI (Ireland); Swedish Research Council (Sweden); CAS (China); CNSF (China) FX We thank the staffs at Fermilab and collaborating institutions, and acknowledge support from the DOE and NSF (USA); CEA and CNRS/IN2P3 (France); FASI, Rosatom and RFBR (Russia); CNPq, FAPERJ, FAPESP and FUNDUNESP (Brazil); DAE and DST (India); Colciencias (Colombia); CONACyT (Mexico); KRF and KOSEF (Korea); CONICET and UBACyT (Argentina); FOM (The Netherlands); STFC and The Royal Society (United Kingdom); MSMT and GACR (Czech Republic); CRC Program and NSERC (Canada); BMBF and DFG (Germany); SFI (Ireland); The Swedish Research Council (Sweden); and CAS and CNSF (China). NR 21 TC 38 Z9 38 U1 5 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAY 9 PY 2011 VL 699 IS 3 BP 145 EP 150 DI 10.1016/j.physletb.2011.03.066 PG 6 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 766JK UT WOS:000290778200003 ER PT J AU Kondo, N Takahashi, A Mori, E Noda, T Zdzienicka, MZ Thompson, LH Helleday, T Suzuki, M Kinashi, Y Masunaga, S Ono, K Hasegawa, M Ohnishi, T AF Kondo, Natsuko Takahashi, Akihisa Mori, Eiichiro Noda, Taichi Zdzienicka, Malgorzata Z. Thompson, Larry H. Helleday, Thomas Suzuki, Minoru Kinashi, Yuko Masunaga, Shinichiro Ono, Koji Hasegawa, Masatoshi Ohnishi, Takeo TI FANCD1/BRCA2 Plays Predominant Role in the Repair of DNA Damage Induced by ACNU or TMZ SO PLOS ONE LA English DT Article ID DOUBLE-STRAND BREAKS; FANCONI-ANEMIA; HOMOLOGOUS RECOMBINATION; MALIGNANT GLIOMA; MOLECULAR TARGET; MAMMALIAN-CELLS; LIGASE IV; PROTEIN; BRCA2; TEMOZOLOMIDE AB Nimustine (ACNU) and temozolomide (TMZ) are DNA alkylating agents which are commonly used in chemotherapy for glioblastomas. ACNU is a DNA cross-linking agent and TMZ is a methylating agent. The therapeutic efficacy of these agents is limited by the development of resistance. In this work, the role of the Fanconi anemia (FA) repair pathway for DNA damage induced by ACNU or TMZ was examined. Cultured mouse embryonic fibroblasts were used: FANCA(-/-), FANCC(-/-), FANCA(-/-)C(-/-), FANCD2(-/-) cells and their parental cells, and Chinese hamster ovary and lung fibroblast cells were used: FANCD1/BRCA2mt, FANCG(-/-) and their parental cells. Cell survival was examined after a 3 h ACNU or TMZ treatment by using colony formation assays. All FA repair pathways were involved in ACNU-induced DNA damage. However, FANCG and FANCD1/BRCA2 played notably important roles in the repair of TMZ-induced DNA damage. The most effective molecular target correlating with cellular sensitivity to both ACNU and TMZ was FANCD1/BRCA2. In addition, it was found that FANCD1/BRCA2 small interference RNA efficiently enhanced cellular sensitivity toward ACNU and TMZ in human glioblastoma A172 cells. These findings suggest that the down-regulation of FANCD1/BRCA2 might be an effective strategy to increase cellular chemo-sensitization towards ACNU and TMZ. C1 [Kondo, Natsuko; Suzuki, Minoru; Kinashi, Yuko; Masunaga, Shinichiro; Ono, Koji] Kyoto Univ, Inst Res Reactor, Particle Radiat Oncol Res Ctr, Osaka 59004, Japan. [Takahashi, Akihisa] Gunma Univ, Adv Sci Res Leaders Dev Unit, Gunma, Japan. [Mori, Eiichiro; Hasegawa, Masatoshi; Ohnishi, Takeo] Nara Med Univ, Dept Radiat Oncol, Sch Med, Nara, Japan. [Noda, Taichi] Nara Med Univ, Dept Dermatol, Sch Med, Nara, Japan. [Zdzienicka, Malgorzata Z.] UMK Coll Med, Dept Mol Cell Genet, Bydgoszcz, Poland. [Thompson, Larry H.] Lawrence Livermore Natl Lab, BBR Program, Livermore, CA USA. [Helleday, Thomas] Stockholm Univ, Dept Genet Microbiol & Toxicol, S-10691 Stockholm, Sweden. RP Kondo, N (reprint author), Kyoto Univ, Inst Res Reactor, Particle Radiat Oncol Res Ctr, Osaka 59004, Japan. EM tohnishi@naramed-u.ac.jp RI Helleday, Thomas/D-5224-2013; OI Helleday, Thomas/0000-0002-7384-092X FU Ministry of Education, Culture, Sports, Science and Technology of Japan; Central Research Institute of the Electric Power Industry in Japan; Japan Space Forum FX This work was supported by Grants-in-Aid for Scientific Research from the Ministry of Education, Culture, Sports, Science and Technology of Japan. This work was also funded in part by a grant from the Central Research Institute of the Electric Power Industry in Japan, and by a grant for Exploratory Research for Space Utilization from the Japan Space Forum. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 37 TC 13 Z9 13 U1 0 U2 9 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 185 BERRY ST, STE 1300, SAN FRANCISCO, CA 94107 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 9 PY 2011 VL 6 IS 5 AR e19659 DI 10.1371/journal.pone.0019659 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 761GX UT WOS:000290386800030 PM 21573016 ER PT J AU Choi, WS Jeong, DW Seo, SSA Lee, YS Kim, TH Jang, SY Lee, HN Myung-Whun, K AF Choi, Woo Seok Jeong, D. W. Seo, S. S. A. Lee, Y. S. Kim, T. H. Jang, S. Y. Lee, H. N. Myung-Whun, K. TI Charge states and magnetic ordering in LaMnO3/SrTiO3 superlattices SO PHYSICAL REVIEW B LA English DT Article ID THIN-FILMS; LAMNO3; INTERFACES; TRANSITION; PHASE AB We investigated themagnetic and optical properties of [(LaMnO3)(n)/( SrTiO3)(8)](20) (n = 1, 2, and 8) superlattices grown by pulsed-laser deposition. We found that a weak ferromagnetic and semiconducting state developed in all superlattices. An analysis of the optical conductivity showed that the LaMnO3 layers in the superlattices were slightly doped. The amount of doping was almost identical regardless of the LaMnO3 layer thickness up to eight unit cells, suggesting that the effect is not limited to the interface. On the other hand, the magnetic ordering became less stable as the LaMnO3 layer thickness decreased, probably due to a dimensional effect. C1 [Choi, Woo Seok; Seo, S. S. A.; Lee, H. N.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Choi, Woo Seok; Jeong, D. W.; Kim, T. H.; Jang, S. Y.] Seoul Natl Univ, Dept Phys & Astron, ReCFI, Seoul 151747, South Korea. [Lee, Y. S.] Soongsil Univ, Dept Phys, Seoul 156743, South Korea. [Myung-Whun, K.] Chonbuk Natl Univ, Dept Phys, Jeonju 561756, South Korea. [Myung-Whun, K.] Chonbuk Natl Univ, IPIT, Jeonju 561756, South Korea. RP Choi, WS (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM hnlee@ornl.gov; mwkim@chonbuk.ac.kr RI Seo, Sung Seok/B-6964-2008; Lee, Ho Nyung/K-2820-2012; Choi, Woo Seok/G-8783-2014; Kim, Tae Heon/C-5935-2015 OI Seo, Sung Seok/0000-0002-7055-5314; Lee, Ho Nyung/0000-0002-2180-3975; Kim, Tae Heon/0000-0003-4835-0707 FU Korean government (MEST) [2009-0069982, 2009-0080567, 2010-0020416, 2010-0014488]; MEST; Pohang University of Science and Technology; Materials Sciences and Engineering Division, US Department of Energy FX The authors are grateful for valuable discussion with J.-S. Chung and H. M. Christen. This research was supported by the National Research Foundation of Korea (NRF) grants funded by the Korean government (MEST) (Grants No. 2009-0069982, No. 2009-0080567, No 2010-0020416, and No. 2010-0014488). The experiments at Pohang Accelerator Laboratory were supported in part by MEST and Pohang University of Science and Technology. The work at Oak Ridge National Laboratory was sponsored by the Materials Sciences and Engineering Division, US Department of Energy. NR 32 TC 29 Z9 29 U1 0 U2 55 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 9 PY 2011 VL 83 IS 19 AR 195113 DI 10.1103/PhysRevB.83.195113 PG 6 WC Physics, Condensed Matter SC Physics GA 761HC UT WOS:000290387400006 ER PT J AU Gray, AX Karel, J Minar, J Bordel, C Ebert, H Braun, J Ueda, S Yamashita, Y Ouyang, L Smith, DJ Kobayashi, K Hellman, F Fadley, CS AF Gray, A. X. Karel, J. Minar, J. Bordel, C. Ebert, H. Braun, J. Ueda, S. Yamashita, Y. Ouyang, L. Smith, D. J. Kobayashi, K. Hellman, F. Fadley, C. S. TI Hard x-ray photoemission study of near-Heusler FexSi1-x alloys SO PHYSICAL REVIEW B LA English DT Article ID AUGER-ELECTRON-SPECTROSCOPY; PHOTOELECTRON-SPECTROSCOPY; MAGNETIC-PROPERTIES; BINDING ENERGIES; EPITAXIAL-GROWTH; SURFACE; SYSTEMS; FE3SI; FILMS; FE AB The structural and electronic properties of epitaxial and amorphous FexSi1-x alloys with x = 0.72 and 0.67 near the binary Heusler composition of x = 0.75 were determined using hard x-ray photoelectron spectroscopy (HXPS). By performing the measurements at a photon energy of 5950.3 eV, the bulk-sensitivity of the measurement is enhanced by a factor of 4-7 compared to conventional soft x-ray photoelectron spectroscopy at about 1000 keV. HXPS probes, on average, as far as 76 angstrom into the FexSi1-x samples. Via core-level spectra, it is found in the amorphous alloy that, in spite of the disordered structure that could lead to a broad distribution of chemical environments, the Si environment is mostly unique. Valence-band spectra reveal a clear distinction between the contributions of the two inequivalent Fe sites of the most highly ordered (x = 0.72, D0(3)) epitaxial sample. The valence-band spectra are compared to results of fully relativistic coherent potential approximation calculations performed in the framework of the one-step model of photoemission, which reveal details of the atomic-orbital makeup of various features, and generally exhibit good agreement with experiment. C1 [Gray, A. X.; Fadley, C. S.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Gray, A. X.; Hellman, F.; Fadley, C. S.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Karel, J.; Hellman, F.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Minar, J.; Ebert, H.; Braun, J.] Univ Munich, Dept Chem & Biochem, D-81377 Munich, Germany. [Bordel, C.; Hellman, F.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bordel, C.] Univ Rouen, INSA Rouen, CNRS, Grp Phys Mat,UMR 6634, F-76801 St Etienne, France. [Ueda, S.; Yamashita, Y.; Kobayashi, K.] Natl Inst Mat Sci, NIMS Beamline Stn SPring 8, Sayo, Hyogo 6795198, Japan. [Ouyang, L.; Smith, D. J.] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA. RP Gray, AX (reprint author), Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. RI Gray, Alexander/F-9267-2011; Minar, Jan/E-9598-2012; MSD, Nanomag/F-6438-2012; UEDA, Shigenori/H-2991-2011; Minar, Jan/O-3186-2013; Karel, Julie/J-5305-2014; YAMASHITA, Yoshiyuki/H-2704-2011 OI Minar, Jan/0000-0001-9735-8479; Minar, Jan/0000-0001-9735-8479; FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-05CH11231]; Ministry of Education, Culture, Sports, Science and Technology (MEXT), Japan; Deutsche Forschungsgemeinschaft [EBE-154/18, EBE-154/20, MI-1327/1] FX Research was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-05CH11231 (A.X.G., J.K., C.B., F.H., and C.S.F.), by the Nanotechnology Network Project, the Ministry of Education, Culture, Sports, Science and Technology (MEXT), Japan (S.U., Y.Y., and K.K.), and by Deutsche Forschungsgemeinschaft under Projects EBE-154/18, EBE-154/20, and MI-1327/1 (J.M., H.E., and J.B.). NR 44 TC 7 Z9 7 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 9 PY 2011 VL 83 IS 19 AR 195112 DI 10.1103/PhysRevB.83.195112 PG 10 WC Physics, Condensed Matter SC Physics GA 761HC UT WOS:000290387400005 ER PT J AU Wang, Y Zhang, F Stumpf, R Lin, P Chou, MY AF Wang, Yan Zhang, Feng Stumpf, R. Lin, Pei Chou, M. Y. TI Catalytic effect of near-surface alloying on hydrogen interaction on the aluminum surface SO PHYSICAL REVIEW B LA English DT Article ID SODIUM ALANATE; STORAGE MATERIALS; DOPED NAALH4; TI; HYDRIDES; H-2; AL; DECOMPOSITION; ABSORPTION; DESORPTION AB A small amount of catalyst, such as Ti, was found to greatly improve the kinetics of hydrogen reactions in the prototypical hydrogen storage compound sodium alanate (NaAlH(4)). We propose a near-surface alloying mechanism for the rehydrogenation cycle based on a detailed analysis of available experimental data as well as first-principles calculations. The calculated results indicate that the catalyst remains at subsurface sites near the Al surface, reducing the dissociation energy barrier of H(2). The binding between Ti and Al modifies the surface charge distribution, which facilitates hydrogen adsorption and enhances hydrogen mobility on the surface. C1 [Wang, Yan; Zhang, Feng; Lin, Pei; Chou, M. Y.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Stumpf, R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Wang, Y (reprint author), Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. RI Zhang, Feng/D-1450-2012; Chou, Mei-Yin/D-3898-2012 FU Department of Energy [DE-FG02-05ER46229]; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX This work is supported by the Department of Energy under Grant No. DE-FG02-05ER46229. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 34 TC 16 Z9 17 U1 2 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 9 PY 2011 VL 83 IS 19 AR 195419 DI 10.1103/PhysRevB.83.195419 PG 5 WC Physics, Condensed Matter SC Physics GA 761HC UT WOS:000290387400018 ER PT J AU Song, HC Bass, SA Heinz, U Hirano, T Shen, C AF Song, Huichao Bass, Steffen A. Heinz, Ulrich Hirano, Tetsufumi Shen, Chun TI 200 A GeV Au plus Au Collisions Serve a Nearly Perfect Quark-Gluon Liquid SO PHYSICAL REVIEW LETTERS LA English DT Article ID HEAVY-ION COLLISIONS; ELLIPTIC FLOW; PLASMA; COLLABORATION; PERSPECTIVE; MATTER AB A new robust method to extract the specific shear viscosity (eta/s)(QGP) of a quark-gluon plasma (QGP) at temperatures T-c < T <= 2T(c) from the centrality dependence of the eccentricity-scaled elliptic flow v(2)/epsilon measured in ultrarelativistic heavy-ion collisions is presented. Coupling viscous fluid dynamics for the QGP with a microscopic transport model for hadronic freeze-out we find for 200 A GeV Au + Au collisions that v(2)/epsilon is a universal function of multiplicity density (1/S)(dN(ch)/dy) that depends only on the viscosity but not on the model used for computing the initial fireball eccentricity epsilon. Comparing with measurements we find 1 < 4 pi(eta/s)(QGP) < 2.5 where the uncertainty range is dominated by model uncertainties for the values of epsilon used to normalize the measured v(2). C1 [Song, Huichao; Hirano, Tetsufumi] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Heinz, Ulrich; Shen, Chun] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Bass, Steffen A.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Hirano, Tetsufumi] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. RP Song, HC (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. FU U.S. Department of Energy [DE-AC02-05CH11231, DE-FG02-05ER41367, DE-SC0004286, DE-SC0004104]; Japan Society for the Promotion of Science [22740151, 213383] FX We gratefully acknowledge fruitful discussions with P. Huovinen, A. Poskanzer, S. Voloshin, and A. Tang. This work was supported by the U.S. Department of Energy under Grants No. DE-AC02-05CH11231, No. DE-FG02-05ER41367, No. DE-SC0004286, and (within the framework of the JET Collaboration) No. DE-SC0004104. T. H. acknowledges support through Grant-in-Aid for Scientific Research No. 22740151 and through the Excellent Young Researchers Oversea Visit Program (No. 213383) of the Japan Society for the Promotion of Science. NR 57 TC 206 Z9 210 U1 1 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 9 PY 2011 VL 106 IS 19 AR 192301 DI 10.1103/PhysRevLett.106.192301 PG 4 WC Physics, Multidisciplinary SC Physics GA 761FW UT WOS:000290383500004 PM 21668145 ER PT J AU Raufaste, C Jamtveit, B John, T Meakin, P Dysthe, DK AF Raufaste, Christophe Jamtveit, Bjorn John, Timm Meakin, Paul Dysthe, Dag Kristian TI The mechanism of porosity formation during solvent-mediated phase transformations SO PROCEEDINGS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES LA English DT Article DE porosity; dissolution-precipitation; recrystallization; fluid-solid interaction ID PSEUDOMORPHIC REPLACEMENT; MINERAL REPLACEMENT; ALKALI FELDSPARS; CRYSTALLIZATION; KINETICS; SYSTEM; MODEL; POLYMORPHISM; KCL-KBR-H2O; DISSOLUTION AB Solvent-mediated solid-solid phase transformations often result in the formation of a porous medium, which may be stable on long time scales or undergo ripening and consolidation. We have studied replacement processes in the KBr-KCl-H(2)O system using both in situ and ex situ experiments. The replacement of a KBr crystal by a K(Br,Cl) solid solution in the presence of an aqueous solution is facilitated by the generation of a surprisingly stable, highly anisotropic and connected pore structure that pervades the product phase. This pore structure ensures efficient solute transport from the bulk solution to the reacting KBr and K(Br,Cl) surfaces. The compositional profile of the K(Br,Cl) solid solution exhibits striking discontinuities across disc-like cavities in the product phase. Similar transformation mechanisms are probably important in controlling phase-transformation processes and rates in a variety of natural and man-made systems. C1 [Raufaste, Christophe; Jamtveit, Bjorn; John, Timm; Meakin, Paul; Dysthe, Dag Kristian] Univ Oslo, N-0316 Oslo, Norway. [Raufaste, Christophe] Univ Nice Sophia Antipolis, Phys Mat Condensee Lab, CNRS, UMR Parc Valrose 6622, F-06108 Nice 2, France. [John, Timm] Univ Munster, Inst Mineral, D-48149 Munster, Germany. [Meakin, Paul] Idaho Natl Lab, Ctr Adv Modeling & Simulat, Idaho Falls, ID 83415 USA. [Meakin, Paul] Inst Energy Technol, N-2007 Kjeller, Norway. RP Raufaste, C (reprint author), Univ Oslo, POB 1048, N-0316 Oslo, Norway. EM christophe.raufaste@unice.fr RI Dysthe, Dag Kristian/F-2247-2011; OI Dysthe, Dag Kristian/0000-0001-8336-5061; Jamtveit, Bjorn/0000-0001-5700-1803 FU Norwegian Research Council FX C.R. thanks Muriel Erambert for her help with the microprobe. Andrew Putnis is thanked for insightful discussions over many years. This study was funded by a Center of Excellence grant from the Norwegian Research Council to PGP. NR 41 TC 21 Z9 21 U1 2 U2 18 PU ROYAL SOC PI LONDON PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND SN 1364-5021 J9 P ROY SOC A-MATH PHY JI Proc. R. Soc. A-Math. Phys. Eng. Sci. PD MAY 8 PY 2011 VL 467 IS 2129 BP 1408 EP 1426 DI 10.1098/rspa.2010.0469 PG 19 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 741GP UT WOS:000288852500010 ER PT J AU Frischknecht, AL Yethiraj, A AF Frischknecht, Amalie L. Yethiraj, Arun TI Two- and three-body interactions among nanoparticles in a polymer melt SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; DIRECTIONAL ATTRACTIVE FORCES; INTEGRAL-EQUATION THEORY; MOLECULAR-DYNAMICS SIMULATIONS; COLLOIDAL PARTICLES; NANOCOMPOSITE MELTS; FLUIDS; MIXTURES; THERMODYNAMICS; NONUNIFORM AB We perform direct three-dimensional density functional theory (DFT) calculations of two-and three-body interactions in polymer nanocomposites. The nanoparticles are modeled as hard spheres, immersed in a hard-sphere homopolymer melt of freely jointed chains. The two-particle potential of mean force obtained from the DFT is in near quantitative agreement with the potential of mean force obtained from self-consistent polymer reference interaction site model theory. Three-body interactions among three nanoparticles are found to be significant, such that it is not possible to describe these systems with a polymer-mediated two-body interaction calculated from the potential of mean force. (C) 2011 American Institute of Physics. [doi:10.1063/1.3585979] C1 [Frischknecht, Amalie L.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Yethiraj, Arun] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA. RP Frischknecht, AL (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. EM alfrisc@sandia.gov RI Frischknecht, Amalie/N-1020-2014; OI Frischknecht, Amalie/0000-0003-2112-2587; Yethiraj, Arun/0000-0002-8579-449X FU Office of Science of the Department of Energy [DE-AC05-00OR22725]; US Department of Energy, Center for Integrated Nanotechnologies at Los Alamos National Laboratory [DE-AC52-06NA25396]; Sandia National Laboratories [DE-AC04-94AL85000] FX This research used resources of the Oak Ridge Leadership Computing Facility, located in the National Center for Computational Sciences at Oak Ridge National Laboratory, which is supported by the Office of Science of the Department of Energy under Contract DE-AC05-00OR22725. Additionally, this work was performed in part at the US Department of Energy, Center for Integrated Nanotechnologies at Los Alamos National Laboratory (Contract DE-AC52-06NA25396) and Sandia National Laboratories (Contract DE-AC04-94AL85000). NR 56 TC 13 Z9 13 U1 2 U2 23 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 7 PY 2011 VL 134 IS 17 AR 174901 DI 10.1063/1.3585979 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 761JD UT WOS:000290393200043 PM 21548703 ER PT J AU Reinhold, CO Yoshida, S Dunning, FB AF Reinhold, C. O. Yoshida, S. Dunning, F. B. TI Electric-field-induced dissociation of heavy Rydberg ion-pair states SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID HALF-CYCLE PULSES; CHARGE-TRANSFER; CLASSICAL-THEORY; HYDROGEN-ATOMS; CROSS-SECTIONS; WAVE-PACKETS; IONIZATION; MOLECULES; SODIUM AB A classical trajectory Monte Carlo approach is used to simulate the dissociation of H(+) center dot center dot center dot F(-) and K(+) center dot center dot center dot Cl(-) heavy Rydberg ion pairs induced by a ramped electric field, a technique used experimentally to detect and probe ion-pair states. Simulations that include the effects of the strong short-range repulsive interaction associated with ion-pair scattering are in good agreement with experimental results for Stark wavepackets probed by a ramped field, demonstrating that many of the characteristics of field-induced dissociation can be well described using a quasi-classical model. The data also show that states with a given value of principal quantum number (i.e., binding energy) can dissociate over a broad range of applied fields, the exact field being governed by the initial orbital angular momentum and orientation of the state. (C) 2011 American Institute of Physics. [doi:10.1063/1.3581832] C1 [Reinhold, C. O.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Reinhold, C. O.] Univ Tennessee, Dept Phys, Knoxville, TN 37996 USA. [Yoshida, S.] Vienna Univ Technol, Inst Theoret Phys, A-1040 Vienna, Austria. [Dunning, F. B.] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Dunning, F. B.] Rice Univ, Rice Quantum Inst, Houston, TX 77005 USA. RP Reinhold, CO (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. EM reinhold@ornl.gov OI Reinhold, Carlos/0000-0003-0100-4962 FU National Science Foundation (NSF) [0964819]; Robert A. Welch Foundation [C-0734]; U.S. Department of Energy (DOE) OBES [ACO5-00OR22725]; FWF (Austria) [SFB016] FX Research supported by the National Science Foundation (NSF) under Grant No. 0964819, the Robert A. Welch Foundation under Grant No. C-0734, the U.S. Department of Energy (DOE) OBES through Contract No. ACO5-00OR22725 to ORNL managed by UT-Batelle, LLC, and the FWF (Austria) under Contract No. SFB016. NR 39 TC 8 Z9 9 U1 3 U2 18 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 7 PY 2011 VL 134 IS 17 AR 174305 DI 10.1063/1.3581832 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 761JD UT WOS:000290393200025 PM 21548685 ER PT J AU Schwerdtfeger, CA DePrince, AE Mazziotti, DA AF Schwerdtfeger, Christine A. DePrince, A. Eugene, III Mazziotti, David A. TI Testing the parametric two-electron reduced-density-matrix method with improved functionals: Application to the conversion of hydrogen peroxide to oxywater SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID CONTRACTED SCHRODINGER-EQUATION; COUPLED-CLUSTER METHODS; CONFIGURATION-INTERACTION; APPROXIMATE SOLUTION; ELECTRON CORRELATION; N-REPRESENTABILITY; WAVE-FUNCTIONS; WATER OXIDE; BASIS-SETS; MOLECULES AB Parametrization of the two-electron reduced density matrix (2-RDM) has recently enabled the direct calculation of electronic energies and 2-RDMs at the computational cost of configuration interaction with single and double excitations. While the original Kollmar energy functional yields energies slightly better than those from coupled cluster with single-double excitations, a general family of energy functionals has recently been developed whose energies approach those from coupled cluster with triple excitations [D. A.Mazziotti, Phys. Rev. Lett. 101, 253002 (2008)]. In this paper we test the parametric 2-RDM method with one of these improved functionals through its application to the conversion of hydrogen peroxide to oxywater. Previous work has predicted the barrier from oxywater to hydrogen peroxide with zero-point energy correction to be 3.3-to-3.9 kcal/mol from coupled cluster with perturbative triple excitations [CCSD(T)] and -2.3 kcal/mol from complete active-space second-order perturbation theory (CASPT2) in augmented polarized triple-zeta basis sets. Using a larger basis set than previously employed for this reaction-an augmented polarized quadruple-zeta basis set (aug-cc-pVQZ)-with extrapolation to the complete basis-set limit, we examined the barrier with two parametric 2-RDM methods and three coupled cluster methods. In the basis-set limit the M parametric 2-RDM method predicts an activation energy of 2.1 kcal/mol while the CCSD(T) barrier becomes 4.2 kcal/mol. The dissociation energy of hydrogen peroxide to hydroxyl radicals is also compared to the activation energy for oxywater formation. We report energies, optimal geometries, dipole moments, and natural occupation numbers. Computed 2-RDMs nearly satisfy necessary N-representability conditions. (C) 2011 American Institute of Physics. [doi:10.1063/1.3585568] C1 [Schwerdtfeger, Christine A.; DePrince, A. Eugene, III; Mazziotti, David A.] Univ Chicago, Dept Chem, Chicago, IL 60637 USA. [DePrince, A. Eugene, III] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Mazziotti, DA (reprint author), Univ Chicago, Dept Chem, 5735 S Ellis Ave, Chicago, IL 60637 USA. EM damazz@uchicago.edu FU NSF; Henry-Camille Dreyfus Foundation; David-Lucile Packard Foundation; Microsoft Corporation FX C.A.S. thanks Professor Barbara Finlayson-Pitts for helpful discussions. D. A. M. gratefully acknowledges the NSF, the Henry-Camille Dreyfus Foundation, the David-Lucile Packard Foundation, and the Microsoft Corporation for their support. NR 65 TC 18 Z9 18 U1 0 U2 2 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 7 PY 2011 VL 134 IS 17 AR 174102 DI 10.1063/1.3585568 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 761JD UT WOS:000290393200008 PM 21548668 ER PT J AU Van Wesep, RG Chen, H Zhu, WG Zhang, ZY AF Van Wesep, Robert G. Chen, Hua Zhu, Wenguang Zhang, Zhenyu TI Communication: Stable carbon nanoarches in the initial stages of epitaxial growth of graphene on Cu(111) SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID AUGMENTED-WAVE METHOD; FILMS; PALLADIUM; SURFACE; CHAIN AB To fully exploit the device potential of graphene, reliable production of large-area, high-quality samples is required. Epitaxial growth on metal substrates have shown promise in this regard, but further improvement would be facilitated by a more complete understanding of the atomistic processes involved in the early growth stages. Using first-principles calculations within density functional theory, we have investigated the energetics and kinetics of graphene nucleation and growth on a Cu(111) surface. Our calculations have revealed an energetic preference for the formation of stable one-dimensional carbon nanoarches consisting of 3-13 atoms when compared to two-dimensional compact islands of equal sizes. We also estimate the critical cluster size that marks the transition from nanoarch dominance to island dominance in the growth sequence. Our findings may provide the structural link between nucleated carbon dimers and larger carbon nanodomes, and are expected to stimulate future experimental efforts. (C) 2011 American Institute of Physics. [doi:10.1063/1.3587239] C1 [Van Wesep, Robert G.; Chen, Hua; Zhu, Wenguang; Zhang, Zhenyu] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Zhu, Wenguang] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Zhang, Zhenyu] Univ Sci & Technol China, ICQD HFNL, Hefei 230026, Anhui, Peoples R China. RP Van Wesep, RG (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RI Zhu, Wenguang/F-4224-2011; Chen, Hua/H-3092-2013 OI Zhu, Wenguang/0000-0003-0819-595X; Chen, Hua/0000-0003-0676-3079 FU US National Science Foundation [0906025]; UTK/ORNL Distinguished Graduate Fellowship; UT/ORNL Joint Institute for Advanced Materials (JIAM fellowship); Division of Materials Science and Engineering; Office of Basic Energy Sciences; US Department of Energy; National Natural Science Foundation of China [11034006] FX This work was supported by US National Science Foundation (Grant No. 0906025), UTK/ORNL Distinguished Graduate Fellowship, the UT/ORNL Joint Institute for Advanced Materials (JIAM fellowship), the Division of Materials Science and Engineering, Office of Basic Energy Sciences, US Department of Energy, and National Natural Science Foundation of China (Grant No. 11034006). The calculations were performed at National Energy Research Scientific Computing Center (NERSC) of US Department of Energy. NR 38 TC 32 Z9 32 U1 1 U2 40 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 7 PY 2011 VL 134 IS 17 AR 171105 DI 10.1063/1.3587239 PG 4 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 761JD UT WOS:000290393200005 PM 21548665 ER PT J AU Gok, R Mellors, RJ Sandvol, E Pasyanos, M Hauk, T Takedatsu, R Yetirmishli, G Teoman, U Turkelli, N Godoladze, T Javakishvirli, Z AF Goek, R. Mellors, R. J. Sandvol, E. Pasyanos, M. Hauk, T. Takedatsu, R. Yetirmishli, G. Teoman, U. Turkelli, N. Godoladze, T. Javakishvirli, Z. TI Lithospheric velocity structure of the Anatolian plateau-Caucasus-Caspian region SO JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH LA English DT Article ID SURFACE-WAVE DISPERSION; CONTINENT-CONTINENT COLLISION; TURKISH-IRANIAN PLATEAU; SURROUNDING REGIONS; RECEIVER FUNCTIONS; EASTERN TURKEY; CRUSTAL STRUCTURE; ACTIVE TECTONICS; STRUCTURE BENEATH; JOINT INVERSION AB The Anatolian plateau-Caucasus-Caspian region is an area of complex lithospheric structure accompanied by large variations in seismic wave velocities. Despite the complexity of the region, little is known about the detailed lithospheric structure. Using data from 31 new, permanent broadband seismic stations along with results from a previous 29 temporary seismic stations and 3 existing global seismic stations in the region, a 3-D velocity model is developed using joint inversion of teleseismic receiver functions and surface waves. Both group and phase dispersion curves (Love and Rayleigh) were derived from regional and teleseismic events. Additional Rayleigh wave group dispersion curves were determined using ambient noise correlation. Receiver functions were calculated using P arrivals from 789 teleseismic (30 degrees-90 degrees) earthquakes. The stacked receiver functions and surface wave dispersion curves were jointly inverted to yield the absolute shear wave velocity to a depth of 100 km at each station. The depths of major discontinuities (sediment-basement, crust-mantle, and lithosphere-asthenosphere) were inferred from the velocity-depth profiles at the location of each station. Distinct spatial variations in crustal and upper mantle shear velocities were observed. The Kura basin showed slow (similar to 2.7-2.9 km/s) upper crustal (0-11 km) velocities but elevated (similar to 3.8-3.9 km/s) velocities in the lower crust. The Anatolian plateau varied from similar to 3.1-3.2 in the upper crust to similar to 3.5-3.7 in the lower crust, while velocities in the Arabian plate (south of the Bitlis suture) were slightly faster (upper crust between 3.3 and 3.4 km/s and lower crust between 3.8 and 3.9 km/s). The depth of the Moho, which was estimated from the shear velocity profiles, was 35 km in the Arabian plate and increased northward to 54 km at the southern edge of the Greater Caucasus. Moho depths in the Kura and at the edge of the Caspian showed more spatial variability but ranged between 35 and 45 km. Upper mantle velocities were slow under the Anatolian plateau but increased to the south under the Arabian plate and to the east (4.3-4.4 km/s) under the Kura basin and Greater Caucasus. The areas of slow mantle coincided with the locations of Holocene volcanoes. Differences between Rayleigh and Love dispersions at long wavelengths reveal a pronounced variation in anisotropy between the Anatolian plateau and the Kura basin. C1 [Goek, R.; Pasyanos, M.; Hauk, T.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Mellors, R. J.; Takedatsu, R.] San Diego State Univ, Dept Geol Sci, San Diego, CA 92182 USA. [Sandvol, E.] Univ Missouri, Dept Geol Sci, Columbia, MO 65201 USA. [Yetirmishli, G.] Republ Seism Survey Ctr, AZ-1001 Baku, Azerbaijan. [Teoman, U.; Turkelli, N.] Bogazici Univ, Kandilli Observ, TR-34684 Istanbul, Turkey. [Teoman, U.; Turkelli, N.] Bogazici Univ, Earthquake Res Inst, Dept Geophys, TR-34684 Istanbul, Turkey. [Godoladze, T.; Javakishvirli, Z.] Ilia State Univ, Earth Res Inst, GE-0177 Tbilisi, Rep of Georgia. RP Gok, R (reprint author), Lawrence Livermore Natl Lab, 7000 E Ave, Livermore, CA 94550 USA. EM gok1@llnl.gov RI Pasyanos, Michael/C-3125-2013; Mellors, Robert/K-7479-2014; Gok, Rengin/O-6639-2014; Yetirmishli, Gurban/C-4257-2017 OI Mellors, Robert/0000-0002-2723-5163; Yetirmishli, Gurban/0000-0002-0542-2443 FU Air Force Research Laboratory [FA8718-07-C-0007]; Lawrence Livermore National Laboratory under U.S. Department of Energy [DE-AC52-07NA27344] FX We would like to thank our Turkish, Azeri, and Georgian collaborators for their hospitality during our trips to the region. We would like to thank Rob Reilinger and Keith Priestley for discussions about the region. Special thanks to Nancy McGee for her insightful contribution. This project is funded by Air Force Research Laboratory contract FA8718-07-C-0007 to San Diego State University. This project was supported by the Lawrence Livermore National Laboratory under the auspices of the U.S. Department of Energy under contract DE-AC52-07NA27344. This is LLNL contribution LLNL-JRNL-468943. NR 56 TC 24 Z9 24 U1 1 U2 11 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9313 EI 2169-9356 J9 J GEOPHYS RES-SOL EA JI J. Geophys. Res.-Solid Earth PD MAY 7 PY 2011 VL 116 AR B05303 DI 10.1029/2009JB000837 PG 14 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 761PW UT WOS:000290410900001 ER PT J AU de Leeuw, G Andreas, EL Anguelova, MD Fairall, CW Lewis, ER O'Dowd, C Schulz, M Schwartz, SE AF de Leeuw, Gerrit Andreas, Edgar L. Anguelova, Magdalena D. Fairall, C. W. Lewis, Ernie R. O'Dowd, Colin Schulz, Michael Schwartz, Stephen E. TI PRODUCTION FLUX OF SEA SPRAY AEROSOL SO REVIEWS OF GEOPHYSICS LA English DT Review ID CENTRAL ARCTIC-OCEAN; SIZE-SEGREGATED SIMULATION; SURFACE MICROWAVE EMISSION; CLOUD CONDENSATION NUCLEI; PRIMARY MARINE AEROSOL; WAVE-FIELD CONDITIONS; AIR-QUALITY MODELS; NORTH POLAR WATERS; WHITECAP COVERAGE; BREAKING WAVES AB Knowledge of the size- and composition-dependent production flux of primary sea spray aerosol (SSA) particles and its dependence on environmental variables is required for modeling cloud microphysical properties and aerosol radiative influences, interpreting measurements of particulate matter in coastal areas and its relation to air quality, and evaluating rates of uptake and reactions of gases in sea spray drops. This review examines recent research pertinent to SSA production flux, which deals mainly with production of particles with r(80) (equilibrium radius at 80% relative humidity) less than 1 mu m and as small as 0.01 mu m. Production of sea spray particles and its dependence on controlling factors has been investigated in laboratory studies that have examined the dependences on water temperature, salinity, and the presence of organics and in field measurements with micrometeorological techniques that use newly developed fast optical particle sizers. Extensive measurements show that water-insoluble organic matter contributes substantially to the composition of SSA particles with r(80) < 0.25 mu m and, in locations with high biological activity, can be the dominant constituent. Order-of-magnitude variation remains in estimates of the size-dependent production flux per white area, the quantity central to formulations of the production flux based on the whitecap method. This variation indicates that the production flux may depend on quantities such as the volume flux of air bubbles to the surface that are not accounted for in current models. Variation in estimates of the whitecap fraction as a function of wind speed contributes additional, comparable uncertainty to production flux estimates. C1 [de Leeuw, Gerrit] Finnish Meteorol Inst, Climate Change Unit, FI-00101 Helsinki, Finland. [de Leeuw, Gerrit] Univ Helsinki, Dept Phys, Helsinki, Finland. [de Leeuw, Gerrit] TNO Built Environm & Geosci, Dept Air Qual & Climate, Utrecht, Netherlands. [Andreas, Edgar L.] NW Res Associates Inc, Seattle Div, Lebanon, NH 03766 USA. [Anguelova, Magdalena D.] USN, Res Lab, Washington, DC 20375 USA. [Fairall, C. W.] NOAA Earth Syst Res Lab, Boulder, CO 80305 USA. [Lewis, Ernie R.; Schwartz, Stephen E.] Brookhaven Natl Lab, Upton, NY 11973 USA. [O'Dowd, Colin] Natl Univ Ireland, Ctr Climate & Air Pollut Studies, Environm Change Inst, Galway, Ireland. [O'Dowd, Colin] Natl Univ Ireland, Sch Phys, Galway, Ireland. [Schulz, Michael] Lab Sci Climat & Environm, Gif Sur Yvette, France. RP de Leeuw, G (reprint author), Finnish Meteorol Inst, Climate Change Unit, Erik Palmenin Aukio 1, FI-00101 Helsinki, Finland. EM gerrit.leeuw@fmi.fi RI Schwartz, Stephen/C-2729-2008; O'Dowd , Colin/K-8904-2012; Schulz, Michael/A-6930-2011 OI Schwartz, Stephen/0000-0001-6288-310X; O'Dowd , Colin/0000-0002-3068-2212; Schulz, Michael/0000-0003-4493-4158 FU EU (European Union) [GOCE-018332, SIP4-CT-2004-516099]; EUCAARI [036833-2]; MACC (Monitoring Atmospheric Composition and Climate); Irish EPA and HEA PRTLI4 program; U.S. Office of Naval Research [N000140810411, 61153N]; U.S. Department of Energy (Office of Science, OBER) [DE-AC02-98CH10886]; NOAA's (National Oceanic and Atmospheric Administration) Office of Climate Observations; NOAA FX The work of G. de Leeuw and C. O'Dowd was supported by the EU (European Union) FP6 projects MAP (Marine Aerosol Production, project GOCE-018332), EUCAARI (European Integrated Project on Aerosol Cloud Climate and Air Quality Interactions) project 036833-2, and MACC (Monitoring Atmospheric Composition and Climate: FP7 Collaborative Project). Work by C. O'Dowd was further supported by the Irish EPA and HEA PRTLI4 program and the EU FP6 project GEMS (Global and Regional Earth-System (Atmosphere) Monitoring Using Satellite and In Situ Data, contract SIP4-CT-2004-516099). The U.S. Office of Naval Research supported E. Andreas's work on this project with award N000140810411. Work by E. R. Lewis and S. E. Schwartz was supported by the U.S. Department of Energy's Atmospheric System Research Program (Office of Science, OBER, contract DE-AC02-98CH10886). Work by M. D. Anguelova was supported by the U.S. Office of Naval Research, NRL program element 61153N. Work by C. W. Fairall was supported by NOAA's (National Oceanic and Atmospheric Administration) Office of Climate Observations and NOAA's Health of the Atmosphere Program. We thank three anonymous reviewers for helpful comments and suggestions. NR 132 TC 132 Z9 132 U1 12 U2 109 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 8755-1209 J9 REV GEOPHYS JI Rev. Geophys. PD MAY 7 PY 2011 VL 49 AR RG2001 DI 10.1029/2010RG000349 PG 39 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 761XS UT WOS:000290436600001 ER PT J AU Smith, AM McCullers, JA Adler, FR AF Smith, Amber M. McCullers, Jonathan A. Adler, Frederick R. TI Mathematical model of a three-stage innate immune response to a pneumococcal lung infection SO JOURNAL OF THEORETICAL BIOLOGY LA English DT Article DE Bacterial dynamics model; Streptococcus pneumoniae infection; Acute inflammation; Dose-dependence; Immune response modeling ID PULMONARY ALVEOLAR MACROPHAGES; STREPTOCOCCUS-PNEUMONIAE; INFLAMMATORY RESPONSE; EPITHELIAL-CELLS; INFLUENZA INFECTION; BACTERIAL PATHOGENS; CYTOKINE PRODUCTION; HOST-DEFENSE; MICE; NEUTROPHIL AB Pneumococcal pneumonia is a leading cause of death and a major source of human morbidity. The initial immune response plays a central role in determining the course and outcome of pneumococcal disease. We combine bacterial titer measurements from mice infected with Streptococcus pneumoniae with mathematical modeling to investigate the coordination of immune responses and the effects of initial inoculum on outcome. To evaluate the contributions of individual components, we systematically build a mathematical model from three subsystems that describe the succession of defensive cells in the lung: resident alveolar macrophages, neutrophils and monocyte-derived macrophages. The alveolar macrophage response, which can be modeled by a single differential equation, can by itself rapidly clear small initial numbers of pneumococci. Extending the model to include the neutrophil response required additional equations for recruitment cytokines and host cell status and damage. With these dynamics, two outcomes can be predicted: bacterial clearance or sustained bacterial growth. Finally, a model including monocyte-derived macrophage recruitment by neutrophils suggests that sustained bacterial growth is possible even in their presence. Our model quantifies the contributions of cytotoxicity and immune-mediated damage in pneumococcal pathogenesis. Published by Elsevier Ltd. C1 [Smith, Amber M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [McCullers, Jonathan A.] St Jude Childrens Res Hosp, Dept Infect Dis, Memphis, TN 38105 USA. [Adler, Frederick R.] Univ Utah, Dept Math & Biol, Salt Lake City, UT 84112 USA. RP Smith, AM (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM asmith@lanl.gov FU National Science Foundation [DMS-0354259]; NIH [N01-AI-50020]; James S. McDonnell Foundation; PHS [AI-66349]; ALSAC; US Department of Energy FX This material is based upon work supported by the National Science Foundation under Grant DMS-0354259 (AMS), NIH Contract N01-AI-50020 (AMS), the 21st Century Science Initiative Grant from the James S. McDonnell Foundation (AMS, FRA), and PHS Grant AI-66349 and ALSAC (JAM). Portions were done under the auspices of the US Department of Energy (AMS). NR 71 TC 25 Z9 26 U1 1 U2 6 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-5193 J9 J THEOR BIOL JI J. Theor. Biol. PD MAY 7 PY 2011 VL 276 IS 1 BP 106 EP 116 DI 10.1016/j.jtbi.2011.01.052 PG 11 WC Biology; Mathematical & Computational Biology SC Life Sciences & Biomedicine - Other Topics; Mathematical & Computational Biology GA 750JW UT WOS:000289543400013 PM 21300073 ER PT J AU Man, JKS Oh, Y Nakayama, K AF Man, J. Ka Shing Oh, Yongseok Nakayama, K. TI Role of high-spin hyperon resonances in the reaction of gamma p -> K+K+Xi(-) SO PHYSICAL REVIEW C LA English DT Article ID BARYON RESONANCES; QUARK-MODEL; DECAYS; CHROMODYNAMICS AB The recent data taken by the CLAS Collaboration at the Thomas Jefferson National Accelerator Facility for the reaction of gamma p -> K+K+Xi(-) are reanalyzed within a relativistic meson-exchange model of hadronic interactions. The present model is an extension of the one developed in an earlier work by Nakayama, Oh, and Haberzettl [Phys. Rev. C 74, 035205 (2006)]. In particular, the role of the spin-5/2 and -7/2 hyperon resonances, which were not included in the previous model, is investigated in the present study. It is shown that the contribution of the Sigma(2030) hyperon having spin-7/2 and positive parity has a key role to bring the model predictions into a fair agreement with the measured data for the K+Xi(-) invariant mass distribution. C1 [Man, J. Ka Shing; Nakayama, K.] Univ Georgia, Dept Phys & Astron, Athens, GA 30602 USA. [Oh, Yongseok] Kyungpook Natl Univ, Dept Phys, Taegu 702701, South Korea. [Oh, Yongseok] Thomas Jefferson Natl Accelerator Facil, Excited Baryon Anal Ctr, Newport News, VA 23606 USA. [Oh, Yongseok] POSTECH, Asia Pacific Ctr Theoret Phys, Pohang 790784, South Korea. [Nakayama, K.] Forschungszentrum Julich, Inst Kernphys, D-52425 Julich, Germany. RP Man, JKS (reprint author), Univ Georgia, Dept Phys & Astron, Athens, GA 30602 USA. EM yohphy@knu.ac.kr; nakayama@uga.edu RI Oh, Yongseok/A-2504-2008 OI Oh, Yongseok/0000-0001-9822-8975 FU FFE [41788390 (COSY-58)]; Ministry of Education, Science and Technology [2010-0009381] FX We are grateful to L. Guo and T.-S. H. Lee for fruitful discussions. We also thank V. Pascalutsa and O. Scholten for discussions on high-spin fields. Y.O. is grateful to the Excited Baryon Analysis Center of the Thomas Jefferson National Accelerator Facility, where part of this work was done. We also acknowledge the University of Georgia Research Computing Center for providing the necessary computing resources. This work was supported by the FFE Grant No. 41788390 (COSY-58) and by Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science and Technology (Grant No. 2010-0009381). NR 31 TC 14 Z9 14 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 6 PY 2011 VL 83 IS 5 AR 055201 DI 10.1103/PhysRevC.83.055201 PG 7 WC Physics, Nuclear SC Physics GA 760FF UT WOS:000290309200005 ER PT J AU Borovsky, JE Denton, MH AF Borovsky, Joseph E. Denton, Michael H. TI A survey of the anisotropy of the outer electron radiation belt during high-speed-stream-driven storms SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article ID ION-CYCLOTRON WAVES; COROTATING INTERACTION REGIONS; PITCH-ANGLE DISTRIBUTIONS; QUASI-LINEAR DIFFUSION; GEOMAGNETIC STORMS; SOLAR-WIND; GEOSYNCHRONOUS ORBIT; RELATIVISTIC ELECTRONS; ENERGETIC PARTICLES; MAGNETIC STORMS AB Electron measurements on board six spacecraft in geosynchronous orbit are superposed-epoch analyzed for 42 high-speed-stream-driven storms. Using pitch angle-resolved fluxes in the range 30 keV to 1.7 MeV, the evolution of the outer electron radiation belt and the suprathermal tail of the electron plasma sheet are studied. The outer electron radiation belt exhibits perpendicular-dominated anisotropies on the dayside and parallel-dominated anisotropies on the nightside consistent with shell splitting in a distorted magnetosphere. The magnitudes of the radiation-belt anisotropies are weak prior to storm onset and become very large during the storms. The magnitudes of the anisotropies lessen with time as the storm ages and the radiation belt heats, probably owing to a weakening of the magnetic field distortion as the storm ages. When a calm before the storm occurs, the dayside radiation belt approaches isotropy, probably owing to pitch angle scattering in the outer plasmasphere that fills during the calm. If no calm before the storm occurs, the dayside radiation belt is strongly perpendicular dominated. The local-time pattern of anisotropy in storms is very different for the suprathermal tail of the electron plasma sheet, which tends to be perpendicular on the nightside and isotropic elsewhere. The magnitudes of the anisotropies of the suprathermal tail are a factor of similar to 10 weaker than the anisotropies of the outer electron radiation belt. C1 [Borovsky, Joseph E.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Denton, Michael H.] Univ Lancaster, Dept Phys, Lancaster LA1 4YB, England. RP Borovsky, JE (reprint author), Los Alamos Natl Lab, ISR-1,Mail Stop D466, Los Alamos, NM 87545 USA. EM jborovsky@lanl.gov OI Denton, Michael/0000-0002-1748-3710 FU NASA; National Science Foundation; STFC [ST/G002401/1] FX The authors thank Rod Christensen for producing pitch-angle-resolved fluxes. The authors thank Tom Cayton, Reiner Friedel, and Jim Wild for their help. Research at Los Alamos was supported by the NASA Targeted Research and Technology Program and by the National Science Foundation GEM Program. Research at Lancaster was supported by STFC grant ST/G002401/1. NR 66 TC 11 Z9 11 U1 0 U2 1 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAY 6 PY 2011 VL 116 AR A05201 DI 10.1029/2010JA016151 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 761RJ UT WOS:000290415500001 ER PT J AU Adelstein, N Mun, BS Ray, HL Ross, PN Neaton, JB De Jonghe, LC AF Adelstein, Nicole Mun, B. Simon Ray, Hannah L. Ross, Philip N., Jr. Neaton, Jeffrey B. De Jonghe, Lutgard C. TI Structure and electronic properties of cerium orthophosphate: Theory and experiment SO PHYSICAL REVIEW B LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; CORRELATED SYSTEMS; BAND-STRUCTURE; BASIS-SET; XPS; SEMICONDUCTORS; CONDUCTION; SPECTRA; METALS AB Using a combination of density functional theory (DFT) calculations and experiments, we determine the structural and electronic properties of cerium orthophosphate (CePO4), a promising proton-conducting electrolyte for fuel cell applications. To better account for strongly-localized Ce 4f electrons, we use a DFT + U approach, where the exchange-correlation functional is augmented with an adjustable effective Hubbard-like parameter U. We find that the calculated structural properties are in good agreement with x-ray diffraction measurements, largely independent of the value of U used. However, the electronic structure is much more sensitive to U, and values of U = 2.5-3 eV for Ce 4f states provide excellent agreement between the calculated density of states and measured photoemission spectra near the valence-band edge, validating the efficacy of a DFT + U-based approach for this system. With a judicious choice of U determined from photoemission experiments, this work provides a natural starting point for future studies of charge transport and charged defect formation and migration in this important class of compounds. C1 [Adelstein, Nicole; Ray, Hannah L.; Ross, Philip N., Jr.; De Jonghe, Lutgard C.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Sci Mat, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Lab, Mol Foundry, Berkeley, CA 94720 USA. [Adelstein, Nicole; Ray, Hannah L.; De Jonghe, Lutgard C.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Mun, B. Simon] Hanyang Univ, Dept Appl Phys, ERICA, Gyeonggi 426791, South Korea. RP Adelstein, N (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Sci Mat, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RI Mun, Bongjin /G-1701-2013; Neaton, Jeffrey/F-8578-2015 OI Neaton, Jeffrey/0000-0001-7585-6135 FU Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the US Department of Energy [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231]; NERSC; Office of Science of the US Department of Energy [DE-AC03-76SF00098]; Korea government MEST [2009-0068720] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the US Department of Energy under Contract No. DE-AC02-05CH11231. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. We also gratefully acknowledge computational support from NERSC, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC03-76SF00098. B. S. Mun would like to thank the support of the Korea Research Foundation KRF grant funded by the Korea government MEST Grant No. 2009-0068720. NR 37 TC 14 Z9 14 U1 2 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 6 PY 2011 VL 83 IS 20 AR 205104 DI 10.1103/PhysRevB.83.205104 PG 7 WC Physics, Condensed Matter SC Physics GA 760EV UT WOS:000290308000002 ER PT J AU Liu, YH Velthuis, SGET Jiang, JS Choi, Y Bader, SD Parizzi, AA Ambaye, H Lauter, V AF Liu, Yaohua Velthuis, S. G. E. Te Jiang, J. S. Choi, Y. Bader, S. D. Parizzi, A. A. Ambaye, H. Lauter, V. TI Magnetic structure in Fe/Sm-Co exchange spring bilayers with intermixed interfaces SO PHYSICAL REVIEW B LA English DT Article ID PERMANENT-MAGNETS; REFLECTOMETER; NEUTRONS; MEDIA AB The depth profile of the intrinsic magnetic properties in an Fe/Sm-Co bilayer fabricated under nearly optimal spring-magnet conditions was determined by complementary studies of polarized neutron reflectometry and micromagnetic simulations. We found that at the Fe/Sm-Co interface, the magnetic properties change gradually at the length scale of 8 nm. In this intermixed interfacial region, the saturation magnetization and magnetic anisotropy are lower and the exchange stiffness is higher than values estimated from the model based on a mixture of Fe and Sm-Co phases. Therefore, the intermixed interface yields superior exchange coupling between the Fe and Sm-Co layers, but at the cost of average magnetization. C1 [Liu, Yaohua; Velthuis, S. G. E. Te; Jiang, J. S.; Choi, Y.; Bader, S. D.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Parizzi, A. A.; Ambaye, H.; Lauter, V.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. RP Liu, YH (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM yhliu@anl.gov; tevelthuis@anl.gov RI Bader, Samuel/A-2995-2013; te Velthuis, Suzanne/I-6735-2013; Liu, Yaohua/B-2529-2009; Ambaye, Haile/D-1503-2016 OI te Velthuis, Suzanne/0000-0002-1023-8384; Liu, Yaohua/0000-0002-5867-5065; Ambaye, Haile/0000-0002-8122-9952 FU US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-06CH11357]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX We thank Gian P. Felcher for helpful discussions. Research at Argonne was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award No. DE-AC02-06CH11357. Research at Oak Ridge National Laboratory's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 25 TC 17 Z9 18 U1 1 U2 27 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 6 PY 2011 VL 83 IS 17 AR 174418 DI 10.1103/PhysRevB.83.174418 PG 7 WC Physics, Condensed Matter SC Physics GA 760EH UT WOS:000290306400005 ER PT J AU Zhang, JL Jiao, L Balakirev, FF Wang, XC Jin, CQ Yuan, HQ AF Zhang, J. L. Jiao, L. Balakirev, F. F. Wang, X. C. Jin, C. Q. Yuan, H. Q. TI Upper critical field and its anisotropy in LiFeAs SO PHYSICAL REVIEW B LA English DT Article ID SUPERCONDUCTORS AB The upper critical field mu H-0(c2)(T-c) of LiFeAs single crystals has been determined by measuring the electrical resistivity using the facilities of pulsed magnetic field at Los Alamos. We found that mu H-0(c2)(T-c) of LiFeAs shows a moderate anisotropy among the layered iron-based superconductors; its anisotropic parameter gamma monotonically decreases with decreasing temperature and approaches gamma similar or equal to 1.5 as T -> 0. The upper critical field reaches 15 T (H parallel to c) and 24.2 T (H parallel to ab) at T = 1.4 K, which values are much smaller than those of other iron-based high T-c superconductors. The temperature dependence of mu H-0(c2)(T-c) can be described by the Werthamer-Helfand-Hohenberg (WHH) method, showing orbitally and (likely) spin-paramagnetically limited upper critical fields for H parallel to c and H parallel to ab, respectively. C1 [Zhang, J. L.; Jiao, L.; Yuan, H. Q.] Zhejiang Univ, Dept Phys, Hangzhou 310027, Zhejiang, Peoples R China. [Balakirev, F. F.] Los Alamos Natl Lab, NHMFL, Los Alamos, NM 87545 USA. [Wang, X. C.; Jin, C. Q.] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Inst Phys, Beijing 100080, Peoples R China. RP Zhang, JL (reprint author), Zhejiang Univ, Dept Phys, Hangzhou 310027, Zhejiang, Peoples R China. EM hqyuan@zju.edu.cn FU National Science Foundation of China; National Basic Research Program of China (973 Program); PCSIRT of the Ministry of Education of China; Zhejiang Provincial Natural Science Foundation of China; Fundamental Research Funds for the Central Universities; National Science Foundation; Department of Energy; State of Florida FX This work was supported by the National Science Foundation of China, the National Basic Research Program of China (973 Program), the PCSIRT of the Ministry of Education of China, Zhejiang Provincial Natural Science Foundation of China, and the Fundamental Research Funds for the Central Universities. Work at NHMFL-LANL was performed under the auspices of the National Science Foundation, the Department of Energy, and the State of Florida. NR 27 TC 33 Z9 34 U1 2 U2 27 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 6 PY 2011 VL 83 IS 17 AR 174506 DI 10.1103/PhysRevB.83.174506 PG 5 WC Physics, Condensed Matter SC Physics GA 760EH UT WOS:000290306400008 ER PT J AU Boughezal, R AF Boughezal, Radja TI Constraints on heavy colored scalars from Tevatron's Higgs exclusion limit SO PHYSICAL REVIEW D LA English DT Article ID LOW-ENERGY THEOREMS; BOSON PRODUCTION; HADRON COLLIDERS; DECAYS; LHC; QCD AB The null search for the Higgs boson at the Tevatron implies strong constraints on heavy colored particles that increase the gluon-fusion induced production rate of the Higgs. We investigate the implications of the Tevatron exclusion limit on example extensions of the standard model that contain a new scalar state transforming as either an adjoint or a fundamental under the QCD gauge group. The bounds on the adjoint (fundamental) scalar mass exceed 200 GeV (100 GeV) for natural choices of scalar-sector parameters. C1 Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. RP Boughezal, R (reprint author), Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. FU US Department of Energy, Division of High Energy Physics [DE-AC02-06CH11357] FX Work supported by the US Department of Energy, Division of High Energy Physics, under Contract No. DE-AC02-06CH11357. NR 31 TC 5 Z9 5 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 J9 PHYS REV D JI Phys. Rev. D PD MAY 6 PY 2011 VL 83 IS 9 AR 093003 DI 10.1103/PhysRevD.83.093003 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 760FJ UT WOS:000290309600001 ER PT J AU Aaltonen, T Gonzalez, BA Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Apollinari, G Appel, JA Apresyan, A Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Auerbach, B Aurisano, A Azfar, F Badgett, W Barbaro-Galtieri, A Barnes, VE Barnett, BA Barria, P Bartos, P Bauce, M Bauer, G Bedeschi, F Beecher, D Behari, S Bellettini, G Bellinger, J Benjamin, D Beretvas, A Bhatti, A Binkley, M Bisello, D Bizjak, I Bland, KR Blumenfeld, B Bocci, A Bodek, A Bortoletto, D Boudreau, J Boveia, A Brau, B Brigliadori, L Brisuda, A Bromberg, C Brucken, E Bucciantonio, M Budagov, J Budd, HS Budd, S Burkett, K Busetto, G Bussey, P Buzatu, A Calancha, C Camarda, S Campanelli, M Campbell, M Canelli, F Canepa, A Carls, B Carlsmith, D Carosi, R Carrillo, S Carron, S Casal, B Casarsa, M Castro, A Catastini, P Cauz, D Cavaliere, V Cavalli-Sforza, M Cerri, A Cerrito, L Chen, YC Chertok, M Chiarelli, G Chlachidze, G Chlebana, F Cho, K Chokheli, D Chou, JP Chung, WH Chung, YS Ciobanu, CI Ciocci, MA Clark, A Compostella, G Convery, ME Conway, J Corbo, M Cordelli, M Cox, CA Cox, DJ Crescioli, F Almenar, CC Cuevas, J Culbertson, R Dagenhart, D d'Ascenzo, N Datta, M de Barbaro, P De Cecco, S De Lorenzo, G Dell'Orso, M Deluca, C Demortier, L Deng, J Deninno, M Devoto, F d'Errico, M Di Canto, A Di Ruzza, B Dittmann, JR D'Onofrio, M Donati, S Dong, P Dorigo, M Dorigo, T Ebina, K Elagin, A Eppig, A Erbacher, R Errede, D Errede, S Ershaidat, N Eusebi, R Fang, HC Farrington, S Feindt, M Fernandez, JP Ferrazza, C Field, R Flanagan, G Forrest, R Frank, MJ Franklin, M Freeman, JC Funakoshi, Y Furic, I Gallinaro, M Galyardt, J Garcia, JE Garfinkel, AF Garosi, P Gerberich, H Gerchtein, E Giagu, S Giakoumopoulou, V Giannetti, P Gibson, K Ginsburg, CM Giokaris, N Giromini, P Giunta, M Giurgiu, G Glagolev, V Glenzinski, D Gold, M Goldin, D Goldschmidt, N Golossanov, A Gomez, G Gomez-Ceballos, G Goncharov, M Gonzalez, O Gorelov, I Goshaw, AT Goulianos, K Gresele, A Grinstein, S Grosso-Pilcher, C Group, RC da Costa, JG Gunay-Unalan, Z Haber, C Hahn, SR Halkiadakis, E Hamaguchi, A Han, JY Happacher, F Hara, K Hare, D Hare, M Harr, RF Hatakeyama, K Hays, C Heck, M Heinrich, J Herndon, M Hewamanage, S Hidas, D Hocker, A Hopkins, W Horn, D Hou, S Hughes, RE Hurwitz, M Husemann, U Hussain, N Hussein, M Huston, J Introzzi, G Iori, M Ivanov, A James, E Jang, D Jayatilaka, B Jeon, EJ Jha, MK Jindariani, S Johnson, W Jones, M Joo, KK Jun, SY Junk, TR Kamon, T Karchin, PE Kato, Y Ketchum, W Keung, J Khotilovich, V Kilminster, B Kim, DH Kim, HS Kim, HW Kim, JE Kim, MJ Kim, SB Kim, SH Kim, YK Kimura, N Kirby, M Klimenko, S Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kreps, M Kroll, J Krop, D Krumnack, N Kruse, M Krutelyov, V Kuhr, T Kurata, M Kwang, S Laasanen, AT Lami, S Lammel, S Lancaster, M Lander, RL Lannon, K Lath, A Latino, G Lazzizzera, I LeCompte, T Lee, E Lee, HS Lee, JS Lee, SW Leo, S Leone, S Lewis, JD Lin, CJ Linacre, J Lindgren, M Lipeles, E Lister, A Litvintsev, DO Liu, C Liu, Q Liu, T Lockwitz, S Lockyer, NS Loginov, A Lucchesi, D Lueck, J Lujan, P Lukens, P Lungu, G Lys, J Lysak, R Madrak, R Maeshima, K Makhoul, K Maksimovic, P Malik, S Manca, G Manousakis-Katsikakis, A Margaroli, F Marino, C Martinez, M Martinez-Ballarin, R Mastrandrea, P Mathis, M Mattson, ME Mazzanti, P McFarland, KS McIntyre, P McNulty, R Mehta, A Mehtala, P Menzione, A Mesropian, C Miao, T Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Mondragon, MN Moon, CS Moore, R Morello, MJ Morlock, J Fernandez, PM Mukherjee, A Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nakano, I Napier, A Nett, J Neu, C Neubauer, MS Nielsen, J Nodulman, L Norniella, O Nurse, E Oakes, L Oh, SH Oh, YD Oksuzian, I Okusawa, T Orava, R Ortolan, L Griso, SP Pagliarone, C Palencia, E Papadimitriou, V Paramonov, AA Patrick, J Pauletta, G Paulini, M Paus, C Pellett, DE Penzo, A Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pondrom, L Potamianos, K Poukhov, O Prokoshin, F Pronko, A Ptohos, F Pueschel, E Punzi, G Pursley, J Rahaman, A Ramakrishnan, V Ranjan, N Redondo, I Renton, P Rescigno, M Rimondi, F Ristori, L Robson, A Rodrigo, T Rodriguez, T Rogers, E Rolli, S Roser, R Rossi, M Rubbo, F Ruffini, F Ruiz, A Russ, J Rusu, V Safonov, A Sakumoto, WK Sakurai, Y Santi, L Sartori, L Sato, K Saveliev, V Savoy-Navarro, A Schlabach, P Schmidt, A Schmidt, EE Schmidt, MP Schmitt, M Schwarz, T Scodellaro, L Scribano, A Scuri, F Sedov, A Seidel, S Seiya, Y Semenov, A Sforza, F Sfyrla, A Shalhout, SZ Shears, T Shepard, PF Shimojima, M Shiraishi, S Shochet, M Shreyber, I Simonenko, A Sinervo, P Sissakian, A Sliwa, K Smith, JR Snider, FD Soha, A Somalwar, S Sorin, V Squillacioti, P Stancari, M Stanitzki, M Denis, RS Stelzer, B Stelzer-Chilton, O Stentz, D Strologas, J Strycker, GL Sudo, Y Sukhanov, A Suslov, I Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thome, J Thompson, GA Thomson, E Ttito-Guzman, P Tkaczyk, S Toback, D Tokar, S Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Tu, Y Ukegawa, F Uozumi, S Varganov, A Vazquez, F Velev, G Vellidis, C Vidal, M Vila, I Vilar, R Vizan, J Vogel, M Volpi, G Wagner, P Wagner, RL Wakisaka, T Wallny, R Wang, SM Warburton, A Waters, D Weinberger, M Wester, WC Whitehouse, B Whiteson, D Wicklund, AB Wicklund, E Wilbur, S Wick, F Williams, HH Wilson, JS Wilson, P Winer, BL Wittich, P Wolbers, S Wolfe, H Wright, T Wu, X Wu, Z Yamamoto, K Yamaoka, J Yang, T Yang, UK Yang, YC Yao, WM Yeh, GP Yi, K Yoh, J Yorita, K Yoshida, T Yu, GB Yu, I Yu, SS Yun, JC Zanetti, A Zeng, Y Zucchelli, S AF Aaltonen, T. Alvarez Gonzalez, B. Amerio, S. Amidei, D. Anastassov, A. Annovi, A. Antos, J. Apollinari, G. Appel, J. A. Apresyan, A. Arisawa, T. Artikov, A. Asaadi, J. Ashmanskas, W. Auerbach, B. Aurisano, A. Azfar, F. Badgett, W. Barbaro-Galtieri, A. Barnes, V. E. Barnett, B. A. Barria, P. Bartos, P. Bauce, M. Bauer, G. Bedeschi, F. Beecher, D. Behari, S. Bellettini, G. Bellinger, J. Benjamin, D. Beretvas, A. Bhatti, A. Binkley, M. Bisello, D. Bizjak, I. Bland, K. R. Blumenfeld, B. Bocci, A. Bodek, A. Bortoletto, D. Boudreau, J. Boveia, A. Brau, B. Brigliadori, L. Brisuda, A. Bromberg, C. Brucken, E. Bucciantonio, M. Budagov, J. Budd, H. S. Budd, S. Burkett, K. Busetto, G. Bussey, P. Buzatu, A. Calancha, C. Camarda, S. Campanelli, M. Campbell, M. Canelli, F. Canepa, A. Carls, B. Carlsmith, D. Carosi, R. Carrillo, S. Carron, S. Casal, B. Casarsa, M. Castro, A. Catastini, P. Cauz, D. Cavaliere, V. Cavalli-Sforza, M. Cerri, A. Cerrito, L. Chen, Y. C. Chertok, M. Chiarelli, G. Chlachidze, G. 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Scribano, A. Scuri, F. Sedov, A. Seidel, S. Seiya, Y. Semenov, A. Sforza, F. Sfyrla, A. Shalhout, S. Z. Shears, T. Shepard, P. F. Shimojima, M. Shiraishi, S. Shochet, M. Shreyber, I. Simonenko, A. Sinervo, P. Sissakian, A. Sliwa, K. Smith, J. R. Snider, F. D. Soha, A. Somalwar, S. Sorin, V. Squillacioti, P. Stancari, M. Stanitzki, M. Denis, R. St. Stelzer, B. Stelzer-Chilton, O. Stentz, D. Strologas, J. Strycker, G. L. Sudo, Y. Sukhanov, A. Suslov, I. Takemasa, K. Takeuchi, Y. Tang, J. Tecchio, M. Teng, P. K. Thom, J. Thome, J. Thompson, G. A. Thomson, E. Ttito-Guzman, P. Tkaczyk, S. Toback, D. Tokar, S. Tollefson, K. Tomura, T. Tonelli, D. Torre, S. Torretta, D. Totaro, P. Trovato, M. Tu, Y. Ukegawa, F. Uozumi, S. Varganov, A. Vazquez, F. Velev, G. Vellidis, C. Vidal, M. Vila, I. Vilar, R. Vizan, J. Vogel, M. Volpi, G. Wagner, P. Wagner, R. L. Wakisaka, T. Wallny, R. Wang, S. M. Warburton, A. Waters, D. Weinberger, M. Wester, W. C., III Whitehouse, B. Whiteson, D. Wicklund, A. B. Wicklund, E. Wilbur, S. Wick, F. Williams, H. H. Wilson, J. S. Wilson, P. Winer, B. L. Wittich, P. Wolbers, S. Wolfe, H. Wright, T. Wu, X. Wu, Z. Yamamoto, K. Yamaoka, J. Yang, T. Yang, U. K. Yang, Y. C. Yao, W. -M. Yeh, G. P. Yi, K. Yoh, J. Yorita, K. Yoshida, T. Yu, G. B. Yu, I. Yu, S. S. Yun, J. C. Zanetti, A. Zeng, Y. Zucchelli, S. TI Measurements of Direct CP Violating Asymmetries in Charmless Decays of Strange Bottom Mesons and Bottom Baryons SO PHYSICAL REVIEW LETTERS LA English DT Article ID PHYSICS AB We report measurements of direct CP-violating asymmetries in charmless decays of neutral bottom hadrons to pairs of charged hadrons with the upgraded Collider Detector at the Fermilab Tevatron. Using a data sample corresponding to 1 fb(-1) of integrated luminosity, we obtain the first measurements of direct CP violation in bottom strange mesons, A(CP)(B-s(0) -> K- pi(+)) = +0.39 + 0.15(stat) +/- 0.08(syst), and bottom baryons, A(CP)(Lambda(0)(b) -> p pi(-)) = 0.03 +/- 0.17(stat) +/- 0.05(syst) and A(CP)(Lambda(0)(b) -> pK(-)) = +0.37 +/- 0.17(stat) +/- 0.03dsyst_. In addition, we measure CP violation in B-0 -> K+ pi(-) decays with 3.5 sigma significance, A(CP)(B-0 -> K+ pi(-)) = -0.086 +/- 0.023(stat) +/- 0.009(syst), in agreement with the current world average. Measurements of branching fractions of B-s(0) -> K+K- and B-0 -> pi(+)pi- decays are also updated. C1 [Carrillo, S.; Chen, Y. C.; Hou, S.; Mitra, A.; Teng, P. K.; Wang, S. M.] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [LeCompte, T.; Nodulman, L.; Paramonov, A. A.; Wicklund, A. B.] Argonne Natl Lab, Argonne, IL 60439 USA. 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[Ferrazza, C.; Trovato, M.] Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Boudreau, J.; Gibson, K.; Liu, C.; Rahaman, A.; Ristori, L.; Shepard, P. F.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Apresyan, A.; Barnes, V. E.; Bortoletto, D.; Flanagan, G.; Garfinkel, A. F.; Jones, M.; Laasanen, A. T.; Liu, Q.; Margaroli, F.; Potamianos, K.; Ranjan, N.; Sedov, A.] Purdue Univ, W Lafayette, IN 47907 USA. [Bodek, A.; Budd, H. S.; Chung, Y. S.; de Barbaro, P.; Han, J. Y.; McFarland, K. S.; Sakumoto, W. K.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Demortier, L.; Gallinaro, M.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10065 USA. [De Cecco, S.; Giagu, S.; Iori, M.; Mastrandrea, P.; Rescigno, M.] Ist Nazl Fis Nucl, I-00185 Rome, Italy. [Giagu, S.; Iori, M.] Univ Roma La Sapienza, I-00185 Rome, Italy. [Halkiadakis, E.; Hare, D.; Hidas, D.; Lath, A.; Somalwar, S.] Rutgers State Univ, Piscataway, NJ 08855 USA. [Asaadi, J.; Aurisano, A.; Elagin, A.; Eusebi, R.; Goldin, D.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Lee, E.; Lee, S. W.; McIntyre, P.; Nett, J.; Safonov, A.; Toback, D.; Weinberger, M.] Texas A&M Univ, College Stn, TX 77843 USA. [Cauz, D.; Dorigo, M.; Pagliarone, C.; Pauletta, G.; Penzo, A.; Roser, R.; Rossi, M.; Santi, L.; Totaro, P.; Zanetti, A.] Ist Nazl Fis Nucl, I-34100 Trieste, Italy. [Pauletta, G.; Santi, L.; Totaro, P.] Univ Trieste, I-33100 Udine, Italy. [Hara, K.; Kim, S. H.; Kurata, M.; Miyake, H.; Nagai, Y.; Sato, K.; Shimojima, M.; Sudo, Y.; Takemasa, K.; Takeuchi, Y.; Tomura, T.; Ukegawa, F.] Univ Tsukuba, Tsukuba, Ibaraki 305, Japan. [Hare, M.; Napier, A.; Rolli, S.; Sliwa, K.; Whitehouse, B.] Tufts Univ, Medford, MA 02155 USA. [Group, R. C.; Neu, C.; Oksuzian, I.] Univ Virginia, Charlottesville, VA 22906 USA. [Arisawa, T.; Ebina, K.; Funakoshi, Y.; Kimura, N.; Kondo, K.; Naganoma, J.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo 169, Japan. [Harr, R. F.; Karchin, P. E.; Mattson, M. E.] Wayne State Univ, Detroit, MI 48201 USA. [Bellinger, J.; Carlsmith, D.; Chung, W. H.; Herndon, M.; Pondrom, L.; Pursley, J.; Ramakrishnan, V.] Univ Wisconsin, Madison, WI 53706 USA. [Auerbach, B.; Almenar, C. Cuenca; Husemann, U.; Lockwitz, S.; Loginov, A.; Schmidt, M. P.; Stanitzki, M.] Yale Univ, New Haven, CT 06520 USA. RP Aaltonen, T (reprint author), Acad Sinica, Inst Phys, Taipei 11529, Taiwan. RI Grinstein, Sebastian/N-3988-2014; Martinez Ballarin, Roberto/K-9209-2015; Gorelov, Igor/J-9010-2015; Prokoshin, Fedor/E-2795-2012; Canelli, Florencia/O-9693-2016; Moon, Chang-Seong/J-3619-2014; Scodellaro, Luca/K-9091-2014; Paulini, Manfred/N-7794-2014; Russ, James/P-3092-2014; Chiarelli, Giorgio/E-8953-2012; unalan, zeynep/C-6660-2015; Lazzizzera, Ignazio/E-9678-2015; Garcia, Jose /H-6339-2015; Cavalli-Sforza, Matteo/H-7102-2015; ciocci, maria agnese /I-2153-2015; Introzzi, Gianluca/K-2497-2015; Piacentino, Giovanni/K-3269-2015; Ivanov, Andrew/A-7982-2013; St.Denis, Richard/C-8997-2012; Warburton, Andreas/N-8028-2013; Kim, Soo-Bong/B-7061-2014; Lysak, Roman/H-2995-2014; Ruiz, Alberto/E-4473-2011; Robson, Aidan/G-1087-2011; De Cecco, Sandro/B-1016-2012; manca, giulia/I-9264-2012; Amerio, Silvia/J-4605-2012; Punzi, Giovanni/J-4947-2012; Zeng, Yu/C-1438-2013; Annovi, Alberto/G-6028-2012 OI Vidal Marono, Miguel/0000-0002-2590-5987; Hays, Chris/0000-0003-2371-9723; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Dorigo, Mirco/0000-0002-0681-6946; Gallinaro, Michele/0000-0003-1261-2277; Brucken, Jens Erik/0000-0001-6066-8756; Torre, Stefano/0000-0002-7565-0118; Di Canto, Angelo/0000-0003-1233-3876; Lami, Stefano/0000-0001-9492-0147; Casarsa, Massimo/0000-0002-1353-8964; Margaroli, Fabrizio/0000-0002-3869-0153; Latino, Giuseppe/0000-0002-4098-3502; Group, Robert/0000-0002-4097-5254; iori, maurizio/0000-0002-6349-0380; Grinstein, Sebastian/0000-0002-6460-8694; Volpi, Guido/0000-0003-1058-8883; Jun, Soon Yung/0000-0003-3370-6109; Toback, David/0000-0003-3457-4144; Martinez Ballarin, Roberto/0000-0003-0588-6720; Gorelov, Igor/0000-0001-5570-0133; Prokoshin, Fedor/0000-0001-6389-5399; Canelli, Florencia/0000-0001-6361-2117; Simonenko, Alexander/0000-0001-6580-3638; Lancaster, Mark/0000-0002-8872-7292; Nielsen, Jason/0000-0002-9175-4419; Moon, Chang-Seong/0000-0001-8229-7829; Scodellaro, Luca/0000-0002-4974-8330; Paulini, Manfred/0000-0002-6714-5787; Russ, James/0000-0001-9856-9155; Chiarelli, Giorgio/0000-0001-9851-4816; unalan, zeynep/0000-0003-2570-7611; Lazzizzera, Ignazio/0000-0001-5092-7531; ciocci, maria agnese /0000-0003-0002-5462; Introzzi, Gianluca/0000-0002-1314-2580; Piacentino, Giovanni/0000-0001-9884-2924; Ivanov, Andrew/0000-0002-9270-5643; Warburton, Andreas/0000-0002-2298-7315; Ruiz, Alberto/0000-0002-3639-0368; Punzi, Giovanni/0000-0002-8346-9052; Annovi, Alberto/0000-0002-4649-4398 FU U.S. Department of Energy; National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A. P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; World Class University; National Research Foundation of Korea; Science and Technology Facilities Council; Royal Society, UK; Institut National de Physique Nucleaire et Physique des Particules/CNRS; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion; Programa Consolider-Ingenio 2010, Spain; Slovak RD Agency; Academy of Finland FX We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the Ministry of Education, Culture, Sports, Science and Technology of Japan; the Natural Sciences and Engineering Research Council of Canada; the National Science Council of the Republic of China; the Swiss National Science Foundation; the A. P. Sloan Foundation; the Bundesministerium fur Bildung und Forschung, Germany; the World Class University Program, the National Research Foundation of Korea; the Science and Technology Facilities Council and the Royal Society, UK; the Institut National de Physique Nucleaire et Physique des Particules/CNRS; the Russian Foundation for Basic Research; the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain; the Slovak R&D Agency; and the Academy of Finland. NR 35 TC 35 Z9 35 U1 2 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 6 PY 2011 VL 106 IS 18 AR 181802 DI 10.1103/PhysRevLett.106.181802 PG 8 WC Physics, Multidisciplinary SC Physics GA 760DT UT WOS:000290304800008 PM 21635084 ER PT J AU Brown, CRD Hoarty, DJ James, SF Swatton, D Hughes, SJ Morton, JW Guymer, TM Hill, MP Chapman, DA Andrew, JE Comley, AJ Shepherd, R Dunn, J Chen, H Schneider, M Brown, G Beiersdorfer, P Emig, J AF Brown, C. R. D. Hoarty, D. J. James, S. F. Swatton, D. Hughes, S. J. Morton, J. W. Guymer, T. M. Hill, M. P. Chapman, D. A. Andrew, J. E. Comley, A. J. Shepherd, R. Dunn, J. Chen, H. Schneider, M. Brown, G. Beiersdorfer, P. Emig, J. TI Measurements of Electron Transport in Foils Irradiated with a Picosecond Time Scale Laser Pulse SO PHYSICAL REVIEW LETTERS LA English DT Article ID SOLID INTERACTIONS; THERMAL TRANSPORT; TARGETS; MODEL AB The heating of solid foils by a picosecond time scale laser pulse has been studied by using x-ray emission spectroscopy. The target material was plastic foil with a buried layer of a spectroscopic tracer material. The laser pulse length was either 0.5 or 2 ps, which resulted in a laser irradiance that varied over the range 10(16)-10(19) W/cm(2). Time-resolved measurements of the buried layer emission spectra using an ultrafast x-ray streak camera were used to infer the density and temperature conditions as a function of laser parameters and depth of the buried layer. Comparison of the data to different models of electron transport showed that they are consistent with a model of electron transport that predicts the bulk of the target heating is due to return currents. C1 [Brown, C. R. D.; Hoarty, D. J.; James, S. F.; Swatton, D.; Hughes, S. J.; Morton, J. W.; Guymer, T. M.; Hill, M. P.; Chapman, D. A.; Andrew, J. E.; Comley, A. J.] AWE Aldermaston, Directorate Sci & Technol, Reading RG7 4PR, Berks, England. [Shepherd, R.; Dunn, J.; Chen, H.; Schneider, M.; Brown, G.; Beiersdorfer, P.; Emig, J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Brown, CRD (reprint author), AWE Aldermaston, Directorate Sci & Technol, Reading RG7 4PR, Berks, England. RI Hill, Matthew/C-4365-2013 OI Hill, Matthew/0000-0002-0307-0624 NR 29 TC 31 Z9 31 U1 1 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 6 PY 2011 VL 106 IS 18 AR 185003 DI 10.1103/PhysRevLett.106.185003 PG 4 WC Physics, Multidisciplinary SC Physics GA 760DT UT WOS:000290304800014 PM 21635097 ER PT J AU McKenna, P Robinson, APL Neely, D Desjarlais, MP Carroll, DC Quinn, MN Yuan, XH Brenner, CM Burza, M Coury, M Gallegos, P Gray, RJ Lancaster, KL Li, YT Lin, XX Tresca, O Wahlstrom, CG AF McKenna, P. Robinson, A. P. L. Neely, D. Desjarlais, M. P. Carroll, D. C. Quinn, M. N. Yuan, X. H. Brenner, C. M. Burza, M. Coury, M. Gallegos, P. Gray, R. J. Lancaster, K. L. Li, Y. T. Lin, X. X. Tresca, O. Wahlstrom, C. -G. TI Effect of Lattice Structure on Energetic Electron Transport in Solids Irradiated by Ultraintense Laser Pulses SO PHYSICAL REVIEW LETTERS LA English DT Article ID LIQUID-METALS; PLASMAS AB The effect of lattice structure on the transport of energetic (MeV) electrons in solids irradiated by ultraintense laser pulses is investigated using various allotropes of carbon. We observe smooth electron transport in diamond, whereas beam filamentation is observed with less ordered forms of carbon. The highly ordered lattice structure of diamond is shown to result in a transient state of warm dense carbon with metalliclike conductivity, at temperatures of the order of 1-100 eV, leading to suppression of electron beam filamentation. C1 [McKenna, P.; Carroll, D. C.; Quinn, M. N.; Yuan, X. H.; Brenner, C. M.; Coury, M.; Gallegos, P.; Gray, R. J.; Tresca, O.] Univ Strathclyde, Dept Phys, SUPA, Glasgow G4 0NG, Lanark, Scotland. [Robinson, A. P. L.; Neely, D.; Brenner, C. M.; Gallegos, P.; Lancaster, K. L.] STFC Rutherford Appleton Lab, Cent Laser Facil, Didcot OX11 0QX, Oxon, England. [Desjarlais, M. P.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Burza, M.; Wahlstrom, C. -G.] Lund Univ, Dept Phys, S-22100 Lund, Sweden. [Li, Y. T.; Lin, X. X.] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. RP McKenna, P (reprint author), Univ Strathclyde, Dept Phys, SUPA, Glasgow G4 0NG, Lanark, Scotland. EM paul.mckenna@strath.ac.uk RI yuan, xiaohui/O-4622-2015; McKenna, Paul/B-9764-2009; OI yuan, xiaohui/0000-0001-8924-4682; McKenna, Paul/0000-0001-8061-7091; Brenner, Ceri/0000-0003-0347-4415 FU EPSRC [EP/E048668/1, EP/E035728/1]; HiPER; Swedish Research Council; National Basic Research Program of China (program 973) [2007CB815101] FX We acknowledge the expert support of the staff at the Central Laser Facility of the Rutherford Appleton Laboratory and the use of computing resources provided by the STFC e-Science Facility. We also acknowledge discussions with Professor R. Bingham and Professor A. R. Bell. This work is supported by EPSRC (Grants No. EP/E048668/1 and No. EP/E035728/1), the HiPER project, the Swedish Research Council, and by the National Basic Research Program of China (program 973; Grant No. 2007CB815101). NR 15 TC 31 Z9 32 U1 0 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 6 PY 2011 VL 106 IS 18 AR 185004 DI 10.1103/PhysRevLett.106.185004 PG 4 WC Physics, Multidisciplinary SC Physics GA 760DT UT WOS:000290304800015 PM 21635098 ER PT J AU Pan, ZH Camacho, J Upton, MH Fedorov, AV Howard, CA Ellerby, M Valla, T AF Pan, Z. -H. Camacho, J. Upton, M. H. Fedorov, A. V. Howard, C. A. Ellerby, M. Valla, T. TI Electronic Structure of Superconducting KC8 and Nonsuperconducting LiC6 Graphite Intercalation Compounds: Evidence for a Graphene-Sheet-Driven Superconducting State SO PHYSICAL REVIEW LETTERS LA English DT Article ID INTERLAYER STATES; SELF-ENERGY; PHOTOEMISSION; SURFACE AB We have performed photoemission studies of the electronic structure in LiC6 and KC8, a non-superconducting and a superconducting graphite intercalation compound, respectively. We have found that the charge transfer from the intercalant layers to graphene layers is larger in KC8 than in LiC6, opposite of what might be expected from their chemical composition. We have also measured the strength of the electron-phonon interaction on the graphene-derived Fermi surface to carbon derived phonons in both materials and found that it follows a universal trend where the coupling strength and superconductivity monotonically increase with the filling of graphene pi* states. This correlation suggests that both graphene-derived electrons and graphene-derived phonons are crucial for superconductivity in graphite intercalation compounds. C1 [Pan, Z. -H.; Camacho, J.; Valla, T.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Upton, M. H.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60192 USA. [Fedorov, A. V.] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. [Howard, C. A.; Ellerby, M.] UCL, London Ctr Nanotechnol, London WC1E 6BT, England. [Howard, C. A.; Ellerby, M.] UCL, Dept Phys & Astron, London WC1E 6BT, England. RP Pan, ZH (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM valla@bnl.gov FU U.S. DOE [DE-AC02-98CH10886, DE-AC03-76SF00098]; UK Engineering and Physical Science Research Council FX We acknowledge useful discussions with M. Calandra, M. Dean, M. Khodas, E. Rotenberg, M. Strongin, and A. Walters. Work at Brookhaven is supported by the U.S. DOE under Contract No. DE-AC02-98CH10886. Work at University College London is supported by the UK Engineering and Physical Science Research Council. ALS is operated by the U.S. DOE under Contract No. DE-AC03-76SF00098. NR 27 TC 42 Z9 42 U1 4 U2 34 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 6 PY 2011 VL 106 IS 18 AR 187002 DI 10.1103/PhysRevLett.106.187002 PG 4 WC Physics, Multidisciplinary SC Physics GA 760DT UT WOS:000290304800023 PM 21635120 ER PT J AU Tetard, L Passian, A Eslami, S Jalili, N Farahi, RH Thundat, T AF Tetard, L. Passian, A. Eslami, S. Jalili, N. Farahi, R. H. Thundat, T. TI Virtual Resonance and Frequency Difference Generation by van der Waals Interaction SO PHYSICAL REVIEW LETTERS LA English DT Article ID HOLOGRAPHY; MICROSCOPY AB The ability to explore the interior of materials for the presence of inhomogeneities was recently demonstrated by mode synthesizing atomic force microscopy [L. Tetard, A. Passian, and T. Thundat, Nature Nanotech. 5, 105 (2009).]. Proposing a semiempirical nonlinear force, we show that difference frequency omega(-) generation, regarded as the simplest synthesized mode, occurs optimally when the force is tuned to van der Waals form. From a parametric study of the probe-sample excitation, we show that the predicted omega(-) oscillation agrees well with experiments. We then introduce the concept of virtual resonance to show that probe oscillations at omega(-) can efficiently be enhanced. C1 [Tetard, L.; Passian, A.; Farahi, R. H.; Thundat, T.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Tetard, L.; Passian, A.; Thundat, T.] Univ Tennessee, Dept Phys, Knoxville, TN 37996 USA. [Eslami, S.; Jalili, N.] Northeastern Univ, Dept Mech Engn, Boston, MA 02115 USA. RP Tetard, L (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM passianan@ornl.gov FU Oak Ridge National Laboratory (ORNL) BioEnergy Science Center (BESC); Office of Biological and Environmental Research in the DOE Office of Science; U.S. DOE [DE-AC05-00OR22725] FX This research was sponsored by the Oak Ridge National Laboratory (ORNL) BioEnergy Science Center (BESC). The BioEnergy Science Center is a U.S. Department of Energy (DOE) Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. ORNL is managed by UT-Battelle, LLC, for the U.S. DOE under Contract No. DE-AC05-00OR22725. NR 13 TC 17 Z9 17 U1 0 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 6 PY 2011 VL 106 IS 18 AR 180801 DI 10.1103/PhysRevLett.106.180801 PG 4 WC Physics, Multidisciplinary SC Physics GA 760DT UT WOS:000290304800005 PM 21635079 ER PT J AU Chambers, SD Svec, F Frechet, JMJ AF Chambers, Stuart D. Svec, Frantisek Frechet, Jean M. J. TI Incorporation of carbon nanotubes in porous polymer monolithic capillary columns to enhance the chromatographic separation of small molecules SO JOURNAL OF CHROMATOGRAPHY A LA English DT Article DE Porous polymer monolith; Carbon nanotubes; Poly(glycidyl methacrylate-co-ethylene dimethacrylate); Reversed phase chromatography; Small molecules ID PERFORMANCE LIQUID-CHROMATOGRAPHY; REVERSED-PHASE CHROMATOGRAPHY; ANION-EXCHANGE CHROMATOGRAPHY; STABLE FREE-RADICALS; STATIONARY PHASES; GOLD NANOPARTICLES; MACROPOROUS POLY(STYRENE-CO-DIVINYLBENZENE); ION CHROMATOGRAPHY; GAS-CHROMATOGRAPHY; ELECTROCHROMATOGRAPHY AB Multiwalled carbon nanotubes have been entrapped in monolithic poly(glycidyl methacrylate-co-ethylene dimethacrylate) capillary columns to afford stationary phases with enhanced liquid chromatographic performance for small molecules in the reversed phase. While the column with no nanotubes exhibited an efficiency of only 1800 plates/m, addition of a small amount of nanotubes to the polymerization mixture increased the efficiency to over 15,000 and 35,000 plates/m at flow rates of 1 and 0.15 mu L/min, respectively. Alternatively, the native glycidyl methacrylate-based monolith was functionalized with ammonia and, then, shortened carbon nanotubes, bearing carboxyl functionalities, were attached to the pore surface through the aid of electrostatic interactions with the amine functionalities. Reducing the pore size of the monolith enhanced the column efficiency for the retained analyte, benzene. to 30,000 plates/m at a flow rate of 0.25 mu L/min. Addition of tetrahydrofuran to the typical aqueous acetonitrile eluents improved the peak shape and increased the column efficiency to 44,000 plates/m calculated for the retained benzene peak. (C) 2011 Elsevier B.V. All rights reserved. C1 [Chambers, Stuart D.; Frechet, Jean M. J.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Svec, Frantisek; Frechet, Jean M. J.] EO Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Frechet, JMJ (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM frechet1@gmail.com OI Frechet, Jean /0000-0001-6419-0163 FU National Institute of Health [GM48364]; Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-05CH11231] FX Financial support of S.D.C. and J.M.J.F. by a grant of the National Institute of Health (GM48364) is gratefully acknowledged. All experimental and characterization work performed at the Molecular Foundry, Lawrence Berkeley National Laboratory and F.S. were supported by the Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. NR 64 TC 88 Z9 90 U1 12 U2 110 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0021-9673 EI 1873-3778 J9 J CHROMATOGR A JI J. Chromatogr. A PD MAY 6 PY 2011 VL 1218 IS 18 BP 2546 EP 2552 DI 10.1016/j.chroma.2011.02.055 PG 7 WC Biochemical Research Methods; Chemistry, Analytical SC Biochemistry & Molecular Biology; Chemistry GA 757EN UT WOS:000290068100011 PM 21420096 ER PT J AU Wang, LM Du, D Lu, DL Lin, CT Smith, JN Timchalk, C Liu, FQ Wang, J Lin, YH AF Wang, Limin Du, Dan Lu, Donglai Lin, Chiann-Tso Smith, Jordan N. Timchalk, Charles Liu, Fengquan Wang, Jun Lin, Yuehe TI Enzyme-linked immunosorbent assay for detection of organophosphorylated butyrylcholinesterase: A biomarker of exposure to organophosphate agents SO ANALYTICA CHIMICA ACTA LA English DT Article DE Sandwich ELISA; Organophosphorylated butyrylcholinesterase; Butyrylcholinesterase; Organophosphate insecticides and nerve agents ID CHEMICAL WARFARE AGENTS; CHROMATOGRAPHY-MASS-SPECTROMETRY; PHOSPHORYLATED ACETYLCHOLINESTERASE; NERVE AGENTS; STEREOSPECIFIC REACTIVATION; RETROSPECTIVE DETECTION; PESTICIDES; SARIN; PRODUCTS; UREA AB A sandwich enzyme-linked immunosorbent assay (sELISA) has been developed for detection of organophosphorylated butyrylcholinesterase (OP-BChE), a potential biomarker for human exposure to organophosphate insecticides and nerve agents. A pair of antibodies specific to OP-BChE adduct were identified through systematic screening of several anti BChE antibodies (anti-BChE) and antiphosphoserine antibodies (anti-P(ser)) from different sources. The selected anti-BChE (set as capture antibody) antibodies recognize both phosphorylated and nonphosphorylated BChE. These antibodies can therefore be used to capture both BChE and OP-BChE from the sample matrices. The anti-P(ser) (set as detecting antibody) was used to recognize the OP moiety of OP-BChE adducts. With the combination of the selected antibody pair, several key parameters (such as the concentration of anti-BChE and anti-P(ser), and the blocking agent) were optimized to enhance the sensitivity and selectivity of the sELISA. Under the optimal conditions, the sELISA has shown a wide linear range from 0.03 nM to 30 nM, with a detection limit of 0.03 nM. Furthermore, the sELISA was successfully applied to detect OP-BChE using in vitro biological samples such as rat plasma spiked with OP-BChE with excellent adduct recovery (z > 99%). These results demonstrate that this novel approach holds great promise to develop an ELISA kit and offers a simple and cost-effective tool for screening/evaluating exposure to organophosphate insecticides and nerve agents. (C) 2011 Elsevier B.V. All rights reserved. C1 [Wang, Limin; Liu, Fengquan] Nanjing Agr Univ, Key Lab Monitoring & Management Crop Dis & Pest I, Minist Agr, Dept Plant Pathol,Coll Plant Protect, Nanjing 210095, Peoples R China. [Wang, Limin; Du, Dan; Lu, Donglai; Lin, Chiann-Tso; Smith, Jordan N.; Timchalk, Charles; Wang, Jun; Lin, Yuehe] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Liu, FQ (reprint author), Nanjing Agr Univ, Key Lab Monitoring & Management Crop Dis & Pest I, Minist Agr, Dept Plant Pathol,Coll Plant Protect, Nanjing 210095, Peoples R China. EM fqliu20011@sina.com; jun.wang@pnl.gov RI Lin, Yuehe/D-9762-2011; Du, Dan (Annie)/G-3821-2012 OI Lin, Yuehe/0000-0003-3791-7587; FU National Institutes of Health through the National Institute of Neurological Disorders and Stroke, NIH [U01 NS058161-01]; National Science & Technology Pillar Program [2009BADB9B03]; DOE [DE-AC05-76L01830]; China Scholarship Council FX This work was conducted at Pacific Northwest National Laboratory (PNNL) and supported by Grant U01 NS058161-01 from the National Institutes of Health CounterACT Program through the National Institute of Neurological Disorders and Stroke, NIH. This work was also supported partially by Key Projects in the National Science & Technology Pillar Program (2009BADB9B03). The contents of this publication are solely the responsibility of the authors and do not necessarily represent the official views of the federal government. PNNL is operated for DOE by Battelle under Contract DE-AC05-76L01830. L.W. would like to acknowledge the fellowship from the China Scholarship Council and the fellowship from PNNL. NR 49 TC 10 Z9 10 U1 0 U2 25 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0003-2670 J9 ANAL CHIM ACTA JI Anal. Chim. Acta PD MAY 5 PY 2011 VL 693 IS 1-2 BP 1 EP 6 DI 10.1016/j.aca.2011.03.013 PG 6 WC Chemistry, Analytical SC Chemistry GA 767VO UT WOS:000290886800001 PM 21504805 ER PT J AU Zhu, K Jang, SR Frank, AJ AF Zhu, Kai Jang, Song-Rim Frank, Arthur J. TI Impact of High Charge-Collection Efficiencies and Dark Energy-Loss Processes on Transport, Recombination, and Photovoltaic Properties of Dye-Sensitized Solar Cells SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID BAND-EDGE MOVEMENT; CONVERSION EFFICIENCY; DIFFUSION LENGTH; TIO2 NANOTUBES; ELECTRON-DIFFUSION; IMPEDANCE; ARRAYS; PHOTOCURRENT; KINETICS; SYSTEM AB We report on the relationships between the energy-loss processes in the dark, charge-collection efficiency and photocurrent density voltage characteristics of dye-sensitized solar cells (DSSCs). The charge-collection efficiencies (eta(cc)) of the DSSCs with different electrolytes were close to 100%. Despite the high eta(cc) values, the DSSCs showed significant loss of photocurrent density and power density resulting from dark processes associated with the exchange current density J(0) at the TiO(2)/electrolyte interface, series resistance of the cells, and diode ideality factor. Even in DSSCs with high eta(cc) values, making recombination slower and transport faster in the dark would reduce these losses. The opposing effects of J(0) and light absorption properties of DSSCs were found to determine the optimum film thickness (L(opt)) for the highest output power density. These effects also explain why L(opt) is generally much less than the electron diffusion length. C1 [Zhu, Kai; Jang, Song-Rim; Frank, Arthur J.] Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. RP Zhu, K (reprint author), Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. EM Kai.Zhu@nrel.gov; Arthur.Frank@nrel.gov FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences; Division of Photovoltaics, Office of Utility Technologies, U.S. Department of Energy [DEAC36-08GO28308] FX This work was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences (A.J.F.) and the Division of Photovoltaics, Office of Utility Technologies, (K.Z., S.-R.J), U.S. Department of Energy, under Contract No. DEAC36-08GO28308. NR 41 TC 60 Z9 61 U1 0 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 5 PY 2011 VL 2 IS 9 BP 1070 EP 1076 DI 10.1021/jz200290c PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 761CM UT WOS:000290372900026 ER PT J AU Blanchard, JW Belieres, JP Alam, TM Yarger, JL Holland, GP AF Blanchard, John W. Belieres, Jean-Philippe Alam, Todd M. Yarger, Jeffery L. Holland, Gregory P. TI NMR Determination of the Diffusion Mechanisms in Triethylamine-Based Protic Ionic Liquids SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID BRONSTED ACID-BASE; FUEL-CELLS; CHEMICAL-EXCHANGE; ELECTROLYTES; CONDUCTIVITY; TRANSPORT; MEMBRANES; SOLVENTS AB Protic ionic liquids (PILs) are highly conductive fluids that have emerged as alternative solvents for electrochemical applications including fuel cells. In the present contribution, the transport properties for a set of triethylamine (TEA)-based PILs were explored with pulsed field gradient stimulated echo (PFG-STE) NMR spectroscopy to obtain the self-diffusion coefficient (D) of the individual molecular species that comprise each system. We report self-diffusion coefficients from measurements conducted in two different laboratories for PILs that were produced by two distinct synthetic routes, a conventional route and a strictly anhydrous route. The PLLs of interest are comprised of TEA cations and different anions, methane sulfonate (MS), bis(trifluoromethylsulfonyl)imide (TFSI), tetrachloroaluminate (AlCl(4)(-)), and bis(perfluoroethylsulfonypimide (BETI). In contrast with previous reports, the PFG-STE diffusion measurements presented here show no proton decoupled (Grotthuss mechanism) mobility in these PILs. Additionally, it is shown that the presence of moderate amounts of water (similar to 1000 ppm) can have a marked influence on D of the acidic proton. C1 [Blanchard, John W.; Yarger, Jeffery L.; Holland, Gregory P.] Arizona State Univ, Magnet Resonance Res Ctr, Dept Chem & Biochem, Tempe, AZ 85287 USA. [Belieres, Jean-Philippe] Boeing Commercial Airplanes, Fuels Res, Seattle, WA 98124 USA. [Alam, Todd M.] Sandia Natl Labs, Dept Nanostruct & Elect Mat, Albuquerque, NM 87185 USA. RP Yarger, JL (reprint author), Arizona State Univ, Magnet Resonance Res Ctr, Dept Chem & Biochem, Tempe, AZ 85287 USA. EM jyarger@gmail.com; greg.holland@asu.edu RI Yarger, Jeff/L-8748-2014; OI Yarger, Jeff/0000-0002-7385-5400; Blanchard, John/0000-0002-1621-6637 FU Defense Air Force Office of Scientific Research (AFOSR) [FA9550-10-1-0275]; National Science Foundation, Division of Materials Research [DMR-0805197]; DOE-BES [DE-SC0001057]; U.S. Department of Energy [DE-AC04-94AL85000]; Arnold and Mabel Beckman Foundation FX The Department of Defense Air Force Office of Scientific Research (AFOSR) under Award No. FA9550-10-1-0275 and the National Science Foundation, Division of Materials Research (DMR-0805197) supported this work. J.L.Y. and NMR. support was also provided in part from the National Nuclear, Security Administration Carnegie/DOE Alliance Center (NNSA CDAC) and EFree, an Energy Frontier Research Center funded by DOE-BES under Award DE-SC0001057. The NMR work at Sandia (TMA) was funded by the DOE BES program. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear security Administration under Contract DE-AC04-94AL85000. J.W.B. was supported in part by a scholarship from the 2007 Beckman Scholars Program from the Arnold and Mabel Beckman Foundation. The authors would like to thank Dr. Brian Cherry for help with NMR instrumentation and student training and Prof. Austen Angell for scientific discussion regarding ionic liquids. NR 31 TC 21 Z9 22 U1 4 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 5 PY 2011 VL 2 IS 9 BP 1077 EP 1081 DI 10.1021/jz200357j PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 761CM UT WOS:000290372900027 ER PT J AU Shuai, DM Wang, CM Genc, A Werth, CJ AF Shuai, Danmeng Wang, Chongmin Genc, Arda Werth, Charles J. TI A New Geometric Method Based on Two-Dimensional Transmission Electron Microscopy for Analysis of Interior versus Exterior Pd Loading on Hollow Carbon Nanofibers SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID MATERIALS SCIENCE; NANOTUBES; NANOPARTICLES; TOMOGRAPHY; PARTICLES; LOCALIZATION AB Hollow carbon nanofibers (CNFs) are being explored as catalyst supports because of their unique properties. Internal versus external loading of metal nanoparticles impacts catalytic performance; we developed a fast and accurate geometric analysis method based on two-dimensional transmission electron microscopy (2D TEM) images to estimate Pd internal versus external loading percentages. Three different Pd-loaded CNF catalysts were prepared using methods reported in the literature to yield different amounts of Pd inside loading. Results indicate the percentage of inside-loaded Pd increases as expected in the three samples (from 22.7 +/- 17.8%, to 47.2 +/- 22.8%, to 71.4 +/- 19.7%, based on Pd nanoparticle number). We compared percent inside loading values for one segment of a Pd-loaded CNF using our method and three-dimensional scanning transmission electron microscopy (3D STEM), and observed adequate agreement (27.8% vs 32.7%). Our geometric analysis method is proposed as a more straightforward and fast way to evaluate metal nanoparticles on tubular supports. C1 [Shuai, Danmeng; Werth, Charles J.] Univ Illinois, Dept Civil & Environm Engn, Urbana, IL 61801 USA. [Wang, Chongmin] Pacific NW Natl Lab, Richland, WA 99354 USA. [Genc, Arda] USA NanoPort, FEI Co, Hillsboro, OR 97124 USA. [Shuai, Danmeng; Werth, Charles J.] Univ Illinois, Ctr Adv Mat Purificat Water Syst, Urbana, IL 61801 USA. RP Werth, CJ (reprint author), Univ Illinois, Dept Civil & Environm Engn, Urbana, IL 61801 USA. EM werth@illinois.edu RI Shuai, Danmeng/E-2212-2011 OI Shuai, Danmeng/0000-0003-3817-4092 FU National Science Foundation [CTS-0120978]; DOE [DE-AC06-76RLO 1830] FX This work was supported by Water CAMPWS, a Science and Technology Center program of the National Science Foundation under agreement number CTS-0120978. 2D TEM analysis was carried out in part at the Frederick Seitz Materials Research Laboratory Central Facilities, University of Illinois. We thank Changyong Zhang for helping to arrange 3D STEM analysis at Pacific Northwest National Laboratory. The 3D STEM images were conducted at the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a DOE User Facility operated by Battelle for the DOE Office of Biological and Environmental Research. Pacific Northwest National Laboratory is operated for the DOE under Contract DE-AC06-76RLO 1830. NR 19 TC 2 Z9 2 U1 0 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 5 PY 2011 VL 2 IS 9 BP 1082 EP 1087 DI 10.1021/jz2003815 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 761CM UT WOS:000290372900028 ER PT J AU Baer, MD Mundy, CJ AF Baer, Marcel D. Mundy, Christopher J. TI Toward an Understanding of the Specific Ion Effect Using Density Functional Theory SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID LIQUID-VAPOR INTERFACE; MOLECULAR-DYNAMICS SIMULATIONS; FREE-ENERGY; AIR/WATER INTERFACE; 1ST PRINCIPLES; SALT-SOLUTIONS; WATER; SURFACE; SOLVATION; IODIDE AB Although it is now accepted that some anions adsorb at the air water interface following a reverse Hofmeister series [Kunz, W.; Hen le, J.; Ninham, B. W. Curr. Opinion Colloid Interface Sci. 2004, 9, 19-37; Tobias, D. J.; Hemminger,. C. Science 2008, 319, 1197-1198], the nature of the microscopic interactions driving ions to interfaces is currently the subject of active research. We use extensive density functional theory (DFT)-based interaction potentials to study the free energy of transfer of iodide from the interior to the surface in both a cluster and the extended air-water interface. Our research supports a picture that empirical polarizable interaction potentials may overestimate surface adsorption for iodide. These results, in conjunction with previous theoretical and experimental studies on iodide solvation, have implications toward the necessary interactions that give rise to the specific ion effect at the air water interface. C1 [Baer, Marcel D.; Mundy, Christopher J.] Pacific NW Natl Lab, Div Chem & Mat Sci, Richland, WA 99352 USA. RP Mundy, CJ (reprint author), Pacific NW Natl Lab, Div Chem & Mat Sci, POB 999, Richland, WA 99352 USA. EM chris.mundy@pnl.gov RI Baer, Marcel/K-7664-2012 FU U.S. Department of Energy (DOE) Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences; Office of Science of the U.S. DOE [DE-AC0500OR22725]; PNNL FX This work was supported by the U.S. Department of Energy (DOE) Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences. Pacific Northwest National Laboratory (PNNL) is operated for the Department of Energy by Battelle. The extended slab calculations were performed under the auspices of our INCITE 2008-2011 award using the CRAY XTS at Oak Ridge National Laboratory (ORNL) that is supported by the Office of Science of the U.S. DOE under Contract No. DE-AC0500OR22725. Cluster calculations were performed using the CRAY XTS at NERSC at Lawrence Berkeley National Laboratory. Bulk studies were performed using NWICE at the Environmental Molecular Sciences Laboratory at PNNL. M.D.B. is grateful for the support of the Linus Pauling Distinguished Postdoctoral Fellowship Program at PNNL. We also acknowledge insightful conversations with Profs. Doug Tobias and Yan Levin and useful discussions with our PNNL colleagues, Dr. Greg Schenter, Dr. Shawn Kathmann, and Dr. Liem Dang. NR 51 TC 60 Z9 60 U1 4 U2 50 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 5 PY 2011 VL 2 IS 9 BP 1088 EP 1093 DI 10.1021/jz200333b PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 761CM UT WOS:000290372900029 ER PT J AU Feng, EH Jones, RE AF Feng, Edward H. Jones, Reese E. TI Carbon nanotube cantilevers for next-generation sensors SO PHYSICAL REVIEW B LA English DT Article ID MOLECULAR-DYNAMICS; YOUNGS MODULUS; RESONATORS; SYSTEMS; TEMPERATURE AB Researchers continue to make smaller force sensors and mechanical resonators in an effort to enhance force sensitivity and achieve higher resonant frequencies. We explore the single wall carbon nanotube cantilever as the ultimate limit of this trend. Using molecular dynamics simulations to calculate the thermal vibrational spectrum of tip displacements, we find that the quality factor of the cantilever is independent of its length. This leads to the surprising result that the intrinsic signal-to-noise ratio for a carbon nanotube cantilever improves with increased length. We discuss qualitative reasons why this result will also hold in a real carbon nanotube device. C1 [Feng, Edward H.; Jones, Reese E.] Sandia Natl Labs, Livermore, CA 94551 USA. RP Feng, EH (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA. EM ehfeng@sandia.gov FU Sandia National Laboratories FX We would like to acknowledge the support of the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract No. DE-ACO4-94AL85000. NR 34 TC 8 Z9 8 U1 1 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 5 PY 2011 VL 83 IS 19 AR 195412 DI 10.1103/PhysRevB.83.195412 PG 6 WC Physics, Condensed Matter SC Physics GA 759NR UT WOS:000290255000010 ER PT J AU Feygenson, M Teng, X Inderhees, SE Yiu, Y Du, W Han, W Wen, J Xu, Z Podlesnyak, AA Niedziela, JL Hagen, M Qiu, Y Brown, CM Zhang, L Aronson, MC AF Feygenson, M. Teng, X. Inderhees, S. E. Yiu, Y. Du, W. Han, W. Wen, J. Xu, Z. Podlesnyak, A. A. Niedziela, J. L. Hagen, M. Qiu, Y. Brown, C. M. Zhang, L. Aronson, M. C. TI Low-energy magnetic excitations in Co/CoO core/shell nanoparticles SO PHYSICAL REVIEW B LA English DT Article ID INELASTIC NEUTRON-SCATTERING; BRILLOUIN LIGHT-SCATTERING; PAIR DISTRIBUTION FUNCTION; FERROMAGNETIC-RESONANCE; SPIN DYNAMICS; FERRITE NANOPARTICLES; EXCHANGE BIAS; COBALT OXIDE; LINE WIDTH; COO AB We have used inelastic neutron scattering measurements to study the magnetic excitations of Co core/CoO shell nanoparticles for energies from 0 to 50 meV. Above the blocking temperature T-B, broad quasielastic scattering is observed, corresponding to the reorientation of the Co core moments and to paramagnetic CoO scattering. Below T-B, two nearly dispersionless inelastic peaks are found, whose energies increase with decreasing temperature as order parameters, controlled by the nanoparticle Neel temperature T-N = 235 K, and saturating as T -> 0 at 2.7 and 6.7 meV, respectively. Similar excitations were observed in a powdered single crystal of CoO, indicating that both are intrinsic excitations of CoO, resulting from the exchange splitting of single-ion states for T <= TN. Pronounced finite-size effects are observed for the scattering from the CoO nanoparticle shells, whose thicknesses range from 1.7 to 4.5 nm. These include an enhanced excitation linewidth, as well as a response that is not only spread over a much wider range of wave vectors, but is also significantly more intense in the nanoparticles than in bulk CoO. C1 [Feygenson, M.; Yiu, Y.; Wen, J.; Xu, Z.; Aronson, M. C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Teng, X.; Han, W.; Zhang, L.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Teng, X.; Du, W.] Univ New Hampshire, Dept Chem Engn, Durham, NH 03824 USA. [Inderhees, S. E.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yiu, Y.; Aronson, M. C.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Podlesnyak, A. A.; Niedziela, J. L.; Hagen, M.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Qiu, Y.; Brown, C. M.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Qiu, Y.] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. RP Feygenson, M (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM feygenson@bnl.gov RI Wen, Jinsheng/F-4209-2010; Instrument, CNCS/B-4599-2012; Yiu, Yuen/A-4353-2010; xu, zhijun/A-3264-2013; Podlesnyak, Andrey/A-5593-2013; Zhang, Lihua/F-4502-2014; Feygenson, Mikhail /H-9972-2014; Du, Wenxin/P-9195-2014; Brown, Craig/B-5430-2009 OI Wen, Jinsheng/0000-0001-5864-1466; Yiu, Yuen/0000-0002-1466-6191; xu, zhijun/0000-0001-7486-2015; Podlesnyak, Andrey/0000-0001-9366-6319; Feygenson, Mikhail /0000-0002-0316-3265; Brown, Craig/0000-0002-9637-9355 FU US Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH1886, DE-AC02-98CH10886]; NSF [DMR-0454672]; Scientific User Facilities Division, Department of Energy, Office of Basic Energy Sciences; University of New Hampshire FX We are grateful to S. Shapiro for useful discussions, and to Jack Simonson for assistance with magnetization measurements. Work at BNL was carried out under the auspices of the US Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-98CH1886 (M. F. and M. C. A.), and at the Brookhaven Center for Functional Nanomaterials under Contract No. DE-AC02-98CH10886. Work at NIST is supported in part by the NSF under Agreement No. DMR-0454672. Work at the Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Department of Energy, Office of Basic Energy Sciences. X. T. and W. D. are partially supported by the University of New Hampshire. NR 84 TC 9 Z9 9 U1 6 U2 51 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 5 PY 2011 VL 83 IS 17 AR 174414 DI 10.1103/PhysRevB.83.174414 PG 10 WC Physics, Condensed Matter SC Physics GA 759NO UT WOS:000290254500004 ER PT J AU Abouzaid, E Arenton, M Barker, AR Barrio, M Bellantoni, L Blucher, E Bock, GJ Bown, C Cheu, E Coleman, R Corcoran, MD Cox, B Erwin, AR Escobar, CO Glazov, A Golossanov, A Gomes, RA Gouffon, P Graham, J Hamm, J Hsiung, YB Jensen, DA Kessler, R Kotera, K LaDue, J Ledovskoy, A McBride, PL Monnier, E Nguyen, H Niclasen, R Phillips, DG Prasad, V Qi, XR Ramberg, EJ Ray, RE Ronquest, M Roodman, A Santos, E Shanahan, P Shawhan, PS Slater, W Smith, D Solomey, N Swallow, EC Taegar, SA Toale, PA Tschirhart, R Wah, YW Wang, J White, HB Whitmore, J Wilking, MJ Winstein, B Winston, R Worcester, ET Yamanaka, T Zimmerman, ED Zukanovich, RF AF Abouzaid, E. Arenton, M. Barker, A. R. Barrio, M. Bellantoni, L. Blucher, E. Bock, G. J. Bown, C. Cheu, E. Coleman, R. Corcoran, M. D. Cox, B. Erwin, A. R. Escobar, C. O. Glazov, A. Golossanov, A. Gomes, R. A. Gouffon, P. Graham, J. Hamm, J. Hsiung, Y. B. Jensen, D. A. Kessler, R. Kotera, K. LaDue, J. Ledovskoy, A. McBride, P. L. Monnier, E. Nguyen, H. Niclasen, R. Phillips, D. G., II Prasad, V. Qi, X. R. Ramberg, E. J. Ray, R. E. Ronquest, M. Roodman, A. Santos, E. Shanahan, P. Shawhan, P. S. Slater, W. Smith, D. Solomey, N. Swallow, E. C. Taegar, S. A. Toale, P. A. Tschirhart, R. Wah, Y. W. Wang, J. White, H. B. Whitmore, J. Wilking, M. J. Winstein, B. Winston, R. Worcester, E. T. Yamanaka, T. Zimmerman, E. D. Zukanovich, R. F. TI Precise measurements of direct CP violation, CPT symmetry, and other parameters in the neutral kaon system SO PHYSICAL REVIEW D LA English DT Article ID PARTICLE PHYSICS; CROSS SECTIONS; KLOE DETECTOR; DECAYS; MESON; REGENERATION; AMPLITUDE; LIFETIME AB We present precise tests of CP and CPT symmetry based on the full data set of K -> pi pi decays collected by the KTeV experiment at Fermi National Accelerator Laboratory during 1996, 1997, and 1999. This data set contains 16 x 10(6) K -> pi(0)pi(0) and 69 x 10(6) K -> pi(+)pi(-) decays. We measure the direct CP violation parameter Re(epsilon'/epsilon) = (19.2 +/- 2.1) x 10(-4). We find the K-L -> K-S mass difference Delta m = (5270 +/- 12) x 10(6) (h) over tilde s(-1) and the K-S lifetime tau(S) = (89.62 +/- 0.05) x 10(-12) s. We also measure several parameters that test CPT invariance. We find the difference between the phase of the indirect CP violation parameter epsilon and the superweak phase: phi(epsilon) - phi(SW) =(0.40 +/- 0.56)degrees. We measure the difference of the relative phases between the CP violating and CP conserving decay amplitudes for K -> pi(+)pi(-) (phi(+-)) and for K -> pi(0)pi(0) (phi(00)): Delta phi = (0.30 +/- 0.35)degrees. From these phase measurements, we place a limit on the mass difference between K-0 and (K) over bar (0): Delta M < 4.8 x 10(-19) GeV/c(2) at 95% C.L. These results are consistent with those of other experiments, our own earlier measurements, and CPT symmetry. C1 [Abouzaid, E.; Barrio, M.; Blucher, E.; Bown, C.; Glazov, A.; Graham, J.; Kessler, R.; Monnier, E.; Prasad, V.; Roodman, A.; Shawhan, P. S.; Solomey, N.; Swallow, E. C.; Wah, Y. W.; Winstein, B.; Winston, R.; Worcester, E. T.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Cheu, E.; Taegar, S. A.; Wang, J.] Univ Arizona, Tucson, AZ 85721 USA. [Slater, W.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Escobar, C. O.; Gomes, R. A.] Univ Estadual Campinas, BR-13083970 Campinas, SP, Brazil. [Barker, A. R.; LaDue, J.; Niclasen, R.; Toale, P. A.; Wilking, M. J.; Zimmerman, E. D.] Univ Colorado, Boulder, CO 80309 USA. [Swallow, E. C.] Elmhurst Coll, Elmhurst, IL 60126 USA. [Bellantoni, L.; Bock, G. J.; Coleman, R.; Hsiung, Y. B.; Jensen, D. A.; McBride, P. L.; Nguyen, H.; Qi, X. R.; Ramberg, E. J.; Ray, R. E.; Shanahan, P.; Tschirhart, R.; White, H. B.; Whitmore, J.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Kotera, K.; Yamanaka, T.] Osaka Univ, Osaka 5600043, Japan. [Corcoran, M. D.] Rice Univ, Houston, TX 77005 USA. [Gouffon, P.; Santos, E.; Zukanovich, R. F.] Univ Sao Paulo, BR-05315970 Sao Paulo, Brazil. [Arenton, M.; Cox, B.; Golossanov, A.; Ledovskoy, A.; Phillips, D. G., II; Ronquest, M.; Smith, D.] Univ Virginia, Dept Phys, Charlottesville, VA 22901 USA. [Arenton, M.; Cox, B.; Golossanov, A.; Ledovskoy, A.; Phillips, D. G., II; Ronquest, M.; Smith, D.] Univ Virginia, Inst Nucl & Particle Phys, Charlottesville, VA 22901 USA. [Erwin, A. R.; Hamm, J.] Univ Wisconsin, Madison, WI 53706 USA. [Glazov, A.] DESY, D-2000 Hamburg, Germany. [Monnier, E.] CNRS, CPP Marseille, F-75700 Paris, France. RP Abouzaid, E (reprint author), Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. RI Gomes, Ricardo/B-6899-2008; Zukanovich Funchal, Renata/C-5829-2013; Moura Santos, Edivaldo/K-5313-2016; Gouffon, Philippe/I-4549-2012; Inst. of Physics, Gleb Wataghin/A-9780-2017; OI Gomes, Ricardo/0000-0003-0278-4876; Zukanovich Funchal, Renata/0000-0001-6749-0022; Moura Santos, Edivaldo/0000-0002-2818-8813; Gouffon, Philippe/0000-0001-7511-4115; HSIUNG, YEE/0000-0003-4801-1238 FU U.S. Department of Energy; National Science Foundation; Ministry of Education and Science of Japan; Fundacao de Amparo a Pesquisa do Estado de Sao Paulo-FAPESP; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico-CNPq; CAPES-Ministerio Educacao FX We gratefully acknowledge the support and effort of the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported in part by the U.S. Department of Energy, The National Science Foundation, The Ministry of Education and Science of Japan, Fundacao de Amparo a Pesquisa do Estado de Sao Paulo-FAPESP, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico-CNPq, and CAPES-Ministerio Educacao. NR 41 TC 34 Z9 34 U1 1 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 J9 PHYS REV D JI Phys. Rev. D PD MAY 5 PY 2011 VL 83 IS 9 AR 092001 DI 10.1103/PhysRevD.83.092001 PG 28 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 759NV UT WOS:000290255600001 ER PT J AU Ketko, MH Kamath, G Potoff, JJ AF Ketko, MaryBeth H. Kamath, Ganesh Potoff, Jeffrey J. TI Development of an Optimized Intermolecular Potential for Sulfur Dioxide SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID UNITED-ATOM DESCRIPTION; MOLECULAR-DYNAMICS SIMULATION; VAPOR-LIQUID-EQUILIBRIA; PHASE-EQUILIBRIA; IONIC LIQUID; TRANSFERABLE POTENTIALS; FORCE-FIELD; SO2; MODELS; CO2 AB A new force field for sulfur dioxide, capable of predicting accurately the vapor-liquid equilibria, critical properties, vapor pressure, and heats of vaporization is presented. The new force field reproduces the saturated liquid densities, vapor pressures and heats of vaporization to within 0.5, 2, and 2% of experiment, respectively. The predicted critical properties and the normal boiling point are in excellent agreement with experimental results. Pair distribution functions are calculated for the S S, S-O, and O-O interactions are in close agreement with neutron and X-ray scattering experiments. In addition to the new force field, similar calculations are performed for four SO(2) intermolecular potentials proposed by Sokolic et al. (Sokolic, F.; Guissani, Y.; Guillot, B. J. Phys. Chem. 1985, 89, 3023], which show that these models work reasonably well near the state point where they were originally parametrized, but large errors in the predicted coexistence properties are displayed at higher and lower temperatures. Comparison of the radial distribution functions show the local structure is only weakly affected by the different force field parameters. C1 [Ketko, MaryBeth H.; Potoff, Jeffrey J.] Wayne State Univ, Dept Chem Engn & Mat Sci, Detroit, MI 48202 USA. [Kamath, Ganesh] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37830 USA. RP Potoff, JJ (reprint author), Wayne State Univ, Dept Chem Engn & Mat Sci, Detroit, MI 48202 USA. EM jpotoff@wayne.edu FU Wayne State University; NSF [CBET-0730768]; ORISE/ORAU FX Financial support from a Wayne State University Undergraduate Research and Creative Projects Grant (M.B.H.K.), NSF CBET-0730768 (J.J.P.) and ORISE/ORAU (G.K.) is gratefully acknowledged. The authors acknowledge CPU time provided by Grid Computing at Wayne State University. NR 42 TC 22 Z9 22 U1 2 U2 28 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 5 PY 2011 VL 115 IS 17 BP 4949 EP 4954 DI 10.1021/jp2010524 PG 6 WC Chemistry, Physical SC Chemistry GA 754AV UT WOS:000289824300006 PM 21476503 ER PT J AU Cao, Y Jin, XS Levin, EJ Huang, H Zong, YN Quick, M Weng, J Pan, YP Love, J Punta, M Rost, B Hendrickson, WA Javitch, JA Rajashankar, KR Zhou, M AF Cao, Yu Jin, Xiangshu Levin, Elena J. Huang, Hua Zong, Yinong Quick, Matthias Weng, Jun Pan, Yaping Love, James Punta, Marco Rost, Burkhard Hendrickson, Wayne A. Javitch, Jonathan A. Rajashankar, Kanagalaghatta R. Zhou, Ming TI Crystal structure of a phosphorylation-coupled saccharide transporter SO NATURE LA English DT Article ID COLI MANNITOL PERMEASE; BACTERIAL PHOSPHOTRANSFERASE SYSTEM; MAJOR FACILITATOR SUPERFAMILY; ESCHERICHIA-COLI; MEMBRANE TOPOLOGY; CARBOHYDRATE TRANSPORTERS; CHITIN DISACCHARIDE; SUBSTRATE-BINDING; ENZYME-II; PHOSPHOENOLPYRUVATE AB Saccharides have a central role in the nutrition of all living organisms. Whereas several saccharide uptake systems are shared between the different phylogenetic kingdoms, the phosphoenolpyruvate-dependent phosphotransferase system exists almost exclusively in bacteria. This multi-component system includes an integral membrane protein EIIC that transports saccharides and assists in their phosphorylation. Here we present the crystal structure of an EIIC from Bacillus cereus that transports diacetylchitobiose. The EIIC is a homodimer, with an expansive interface formed between the amino-terminal halves of the two protomers. The carboxy-terminal half of each protomer has a large binding pocket that contains a diacetylchitobiose, which is occluded from both sides of the membrane with its site of phosphorylation near the conserved His 250 and Glu 334 residues. The structure shows the architecture of this important class of transporters, identifies the determinants of substrate binding and phosphorylation, and provides a framework for understanding the mechanism of sugar translocation. C1 [Cao, Yu; Levin, Elena J.; Huang, Hua; Weng, Jun; Pan, Yaping; Zhou, Ming] Columbia Univ, Coll Phys & Surg, Dept Physiol & Cellular Biophys, New York, NY 10032 USA. [Jin, Xiangshu] Columbia Univ, Howard Hughes Med Inst, Dept Biochem & Mol Biophys, Ctr Computat Biol & Bioinformat, New York, NY 10032 USA. [Zong, Yinong] Sanford Burnham Inst, La Jolla, CA 92037 USA. [Quick, Matthias; Javitch, Jonathan A.] Columbia Univ, Dept Psychiat, New York, NY 10032 USA. [Quick, Matthias; Javitch, Jonathan A.] Columbia Univ, Ctr Mol Recognit, New York, NY 10032 USA. [Quick, Matthias; Javitch, Jonathan A.] New York State Psychiat Inst & Hosp, Div Mol Therapeut, New York, NY 10032 USA. [Love, James; Punta, Marco; Rost, Burkhard; Hendrickson, Wayne A.] New York Struct Biol Ctr, New York Consortium Membrane Prot Struct, New York, NY 10027 USA. [Punta, Marco; Rost, Burkhard] Tech Univ Munich, Dept Comp Sci, D-85748 Munich, Germany. [Punta, Marco; Rost, Burkhard] Tech Univ Munich, Inst Adv Study, D-85748 Munich, Germany. [Javitch, Jonathan A.] Columbia Univ, Dept Pharmacol, New York, NY 10032 USA. [Rajashankar, Kanagalaghatta R.] Cornell Univ, Dept Chem & Chem Biol, NE CAT, Adv Photon Source, Argonne, IL 60439 USA. RP Zhou, M (reprint author), Columbia Univ, Coll Phys & Surg, Dept Physiol & Cellular Biophys, 630 W 168th St, New York, NY 10032 USA. EM mz2140@columbia.edu FU US National Institutes of Health [DK088057, GM098878, GM05026-sub0007, T32HL087745]; [GM05026] FX Data for this study were measured at beamlines X4A, X4C, X25 and X29 of the National Synchrotron Light Source and the NE-CAT 24ID-C and E at the Advanced Photon Source. This work was supported by the US National Institutes of Health (DK088057, GM098878 and GM05026-sub0007 to M.Z., and T32HL087745 to E.J.L.). M.Z. is a Pew Scholar in Biomedical Sciences. The NYCOMPS central facility was supported by GM05026 to W.A.H. as part of the Protein Structure Initiative (PSI-2) established by the National Institute of General Medical Sciences. The authors would like to thank B. Honig for support and M. Saier, B. Erni, R. Kaback and D.-N. Wang for comments on the manuscript and helpful discussions. M.Z. is grateful to R. MacKinnon for advice and encouragement. NR 50 TC 41 Z9 41 U1 2 U2 24 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 J9 NATURE JI Nature PD MAY 5 PY 2011 VL 473 IS 7345 BP 50 EP U58 DI 10.1038/nature09939 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 759CQ UT WOS:000290218300028 PM 21471968 ER PT J AU Alam, TM Dreyer, DR Bielwaski, CW Ruoff, RS AF Alam, Todd M. Dreyer, Daniel R. Bielwaski, Christopher W. Ruoff, Rodney S. TI Measuring Molecular Dynamics and Activation Energies for Quaternary Acyclic Ammonium and Cyclic Pyrrolidinium Ionic Liquids Using N-14 NMR Spectroscopy SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID QUADRUPOLE COUPLING-CONSTANTS; ROTATIONAL FRICTION COEFFICIENTS; PHYSICOCHEMICAL PROPERTIES; TEMPERATURE-DEPENDENCE; PHYSICAL-PROPERTIES; NUCLEAR-RELAXATION; BOUNDARY-CONDITION; CORRELATION TIMES; SELF-DIFFUSION; C-13 AB The N-14 NMR spin-lattice (R-1) and spin-spin (R-2) relaxation rates were determined as a function of temperature for a series of tetra-alkyl acyclic ammonium and cyclic pyrrolidinium ionic liquids (ILs). Through the use of the R-2/R-1, ratio method, it was shown that for the majority of these ILs, the reorientational dynamics are not in the extreme narrowing regime, but instead are in the dispersive relaxation regime, thus allowing a unique solution for the correlation time to be determined. The temperature variation of the R-2 relaxation rate, along with the temperature variation of the calculated correlation times, allowed activation energies for the reorientational dynamics to be measured and compared. In addition, these NMR relaxation experiments enabled the N-14 quadrupolar coupling product to be extracted, which revealed surprising temperature dependence. Collectively, the N-14 NMR results allow the impact of cation and anion identity on the local reorientational dynamics of these ILs to be delineated. C1 [Alam, Todd M.] Sandia Natl Labs, Dept Elect & Nanostruct Mat, Albuquerque, NM 87185 USA. [Dreyer, Daniel R.; Bielwaski, Christopher W.] Univ Texas Austin, Dept Chem & Biochem, Austin, TX 78712 USA. [Ruoff, Rodney S.] Univ Texas Austin, Dept Mech Engn, Austin, TX 78712 USA. [Ruoff, Rodney S.] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA. RP Alam, TM (reprint author), Sandia Natl Labs, Dept Elect & Nanostruct Mat, POB 5800, Albuquerque, NM 87185 USA. EM tmalam@sandia.gov RI Ruoff, Rodney/K-3879-2015 FU U.S. DOE, Office of Basic Energy Sciences [DE-SC001951, ER46657]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This research was funded by the U.S. DOE, Office of Basic Energy Sciences, under Award ID DE-SC001951 and ER46657. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 65 TC 17 Z9 17 U1 3 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 5 PY 2011 VL 115 IS 17 BP 4307 EP 4316 DI 10.1021/jp200630k PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 754AX UT WOS:000289824500021 PM 21456554 ER PT J AU Ghorai, S Laskin, A Tivanski, AV AF Ghorai, Suman Laskin, Alexander Tivanski, Alexei V. TI Spectroscopic Evidence of Keto-Enol Tautomerism in Deliquesced Malonic Acid Particles SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID SOLUBLE DICARBOXYLIC-ACIDS; CARBOXYLIC-ACIDS; HYGROSCOPIC PROPERTIES; CHEMICAL-COMPOSITION; RAMAN-SPECTROSCOPY; AEROSOL-PARTICLES; PHASE-TRANSITION; AMMONIUM-SULFATE; FT-IR; WATER AB Scanning transmission X-ray microscopy combined with near-edge X-ray absorption fine structure spectroscopy (STXM/NEXAFS) and optical microscopy coupled with Fourier transform infrared spectroscopy (micro-FTIR) have been applied to observe hygroscopic growth and chemical changes in malonic acid particles deposited on substrates. The extent of the hygroscopic growth of particles has been quantified in terms of the corresponding water-to-solute ratios (WSR) based on STXM/NEXAFS and micro-FTIR data sets. WSR values derived separately from two applied methods displayed a remarkable agreement with previous data reported in the literature. Comparison of NEXAFS and FTIR spectra acquired at different relative humidity (RH) shows efficient keto enol tautomerization of malonic acid, with the enol form dominating at higher RI-I. The keto enol equilibrium constants were calculated using relevant peak intensities in the carbon and oxygen K-edge NEXAFS spectra as a function of RH. We report strong dependence of the equilibrium constant on RI-I, with measured values of 0.18 +/- 0.03, 1.11 +/- 0.14, and 2.33 +/- 0.37 corresponding to 2, 50, and 90% RH, respectively. Enols are important intermediates in aldol condensation reactions pertaining to formation and atmospheric aging of secondary organic aerosol (SOA). The present knowledge assumes that constituents of atmospheric deliquesced particles undergo aqueous chemistry with kinetic and equilibrium constants analogous to reactions in bulk solutions, which would estimate absolute dominance of the keto form of carboxylic acids. For instance, the keto enol equilibrium constant of malonic acid in diluted aqueous solution is <10(-4). Our results suggest that in deliquesced micrometer-size particles, carboxylic acids may exist in predominantly enol forms that need to be explicitly considered in atmospheric aerosol chemistry. C1 [Ghorai, Suman; Tivanski, Alexei V.] Univ Iowa, Dept Chem, Iowa City, IA 52242 USA. [Laskin, Alexander] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Tivanski, AV (reprint author), Univ Iowa, Dept Chem, Iowa City, IA 52242 USA. EM alexei-tivanski@uiowa.edu RI Laskin, Alexander/I-2574-2012 OI Laskin, Alexander/0000-0002-7836-8417 FU University of Iowa; Pacific Northwest National Laboratory (PNNL); Office of Science, Office of Basic Energy Sciences, the Division of Chemical Sciences, Geosciences, and Biosciences; Division of Materials Sciences of Department of Energy (DOE) at the ALS and LBNL [DE-AC03-76500098]; DOE's Office of Biological and Environmental Research and located at PNNL; U.S. Department of Energy by Battelle Memorial Institute [DE-AC06-76RLO 1830] FX S.G. and A.V.T. gratefully acknowledge the University of Iowa for the financial support. A.L. acknowledges support by Laboratory Directed Research and Development funds of Pacific Northwest National Laboratory (PNNL). The STXM/NEXAFS experiments at the Advanced Light Source (ALS) of Lawrence Berkeley National Laboratory (LBNL) were supported by the Office of Science, Office of Basic Energy Sciences, the Division of Chemical Sciences, Geosciences, and Biosciences, and the Division of Materials Sciences of Department of Energy (DOE) at the ALS and LBNL under Contract No. DE-AC03-76500098. The micro-FTIR experiments were performed at the William R. Wiley Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at PNNL. Pacific Northwest National Laboratory is operated for the U.S. Department of Energy by Battelle Memorial Institute under Contract No. DE-AC06-76RLO 1830. We thank Dr. M. K. Gilles for helpful discussions regarding STXM/NEXAFS data interpretation, Dr. A. D. Kilcoyne for support at beamline 5.3.2, and Mr. P. L. Gassman and Dr. J. P. Cain for assistance with the micro-FTIR instrument. NR 52 TC 22 Z9 22 U1 3 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 5 PY 2011 VL 115 IS 17 BP 4373 EP 4380 DI 10.1021/jp112360x PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 754AX UT WOS:000289824500028 PM 21480651 ER PT J AU Petkovic, LM Utgikar, V Rashkeev, SN AF Petkovic, Lucia M. Utgikar, Vivek Rashkeev, Sergey N. TI Structural Stability and Catalytic Activity of Lanthanum-Based Perovskites SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; OXYGEN PERMEATION; COMBUSTION; OXIDES; PERFORMANCE; TECHNOLOGY; MEMBRANES; CATHODE AB Perovskite-type oxide materials with a general formula La(1-x)A(x)Fe(1-y) Co(y)O(3-delta), where A is an alkaline earth metal Sr or Ba, have been studied as cathode materials for catalytic reduction of oxygen in solid oxide fuel cells (SOFCs), as well as combustion catalysts. In this study, we use a combination of temperature-programmed reduction measurements, X-ray diffraction, carbon black catalytic oxidation measurements, and first-principles, density-functional-theory (DFT) calculations to elucidate the main processes that contribute to the structural stability and catalytic activity for soot oxidation of these materials. In particular, we investigate the dynamics of the structure reconstruction with oxygen loss during the regulated increase of the temperature. The calculations are in good qualitative agreement with catalytic experiments and allow us to identify special combinations of the perovskite chemical composition and local surface structures for which one could expect the highest catalytic activity for the soot oxidation process. C1 [Petkovic, Lucia M.; Rashkeev, Sergey N.] Idaho Natl Lab, Ctr Adv Modeling & Simulat, Idaho Falls, ID 83415 USA. [Utgikar, Vivek] Univ Idaho, Dept Chem Engn, Idaho Falls, ID 83402 USA. RP Petkovic, LM (reprint author), Idaho Natl Lab, Ctr Adv Modeling & Simulat, Idaho Falls, ID 83415 USA. RI Petkovic, Lucia/E-9092-2011 OI Petkovic, Lucia/0000-0002-0870-3355 FU INL; U.S. Department of Energy, Office of Nuclear Energy; U.S. Department of Energy [DE-AC07-05ID14517] FX We would like to acknowledge the INL Laboratory Directed Research and Development program and the U.S. Department of Energy, Office of Nuclear Energy, for financial support. This research was also supported in part by a grant of computer time from High Performance Computer Center at Idaho National Laboratory. Thanks to Dr. Harry W. Rollins for the XRD analyses. This manuscript has been authored by Battelle Energy Alliance, LLC under Contract No. DE-AC07-05ID14517 with the U.S. Department of Energy. NR 31 TC 10 Z9 10 U1 0 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 5 PY 2011 VL 115 IS 17 BP 8709 EP 8715 DI 10.1021/jp112422m PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 754AU UT WOS:000289824200031 ER PT J AU Powell, MR Sa, N Davenport, M Healy, K Vassiouk, I Letant, SE Baker, LA Siwy, ZS AF Powell, M. R. Sa, N. Davenport, M. Healy, K. Vassiouk, I. Letant, S. E. Baker, L. A. Siwy, Z. S. TI Noise Properties of Rectifying Nanopores SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SOLID-STATE NANOPORES; ION CURRENT; 1/F NOISE; CURRENT RECTIFICATION; DNA TRANSLOCATION; TRANSPORT; MEMBRANES; CHANNEL; DIODES AB Ion currents through three types of rectifying nanoporous structures are studied and compared: conically shaped polymer nanopores, glass nanopipettes, and silicon nitride nanopores. Time signals of ion currents are analyzed by the power spectrum. We focus on the low-frequency range where the power spectrum magnitude scales with frequency, f, as 1/f. Glass nanopipettes and polymer nanopores exhibit nonequilibrium 1/f noise; thus, the normalized power spectrum depends on the voltage polarity and magnitude. In contrast, 1/f noise in rectifying silicon nitride nanopores is of equilibrium character. Various mechanisms underlying the voltage-dependent 1/f noise are explored and discussed, including intrinsic pore wall dynamics and formation of vortices and nonlinear flow patterns in the pore. Experimental data are supported by modeling of ion currents based on the coupled Poisson-Nernst-Planck and Navier-Stokes equations. We conclude that the voltage-dependent 1/f noise observed in polymer and glass asymmetric nanopores might result from high and asymmetric electric fields, inducing secondary effects in the pore, such as enhanced water dissociation. C1 [Powell, M. R.; Davenport, M.; Healy, K.; Siwy, Z. S.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Sa, N.; Baker, L. A.] Indiana Univ, Dept Chem, Bloomington, IN 47405 USA. [Vassiouk, I.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Letant, S. E.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Siwy, ZS (reprint author), Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. EM zsiwy@uci.edu RI Baker, Lane/B-6452-2008; Vlassiouk, Ivan/F-9587-2010; SA, NIYA/E-8521-2017 OI Vlassiouk, Ivan/0000-0002-5494-0386; FU National Science Foundation [CHE 0747237]; UC System/National laboratories; Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX Single-ion irradiation at the Institute for Heavy Ions Research, Darmstadt, Germany is greatly acknowledged. The research was supported by the National Science Foundation (CHE 0747237) and the UC System/National laboratories collaboration program. This work was performed under the auspices of the U.S. Department of Energy by the Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 45 TC 18 Z9 18 U1 4 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 5 PY 2011 VL 115 IS 17 BP 8775 EP 8783 DI 10.1021/jp2016038 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 754AU UT WOS:000289824200039 ER PT J AU O'Bryan, G Yang, EL Zifer, T Wally, K Skinner, JL Vance, AL AF O'Bryan, G. Yang, E. L. Zifer, T. Wally, K. Skinner, J. L. Vance, A. L. TI Nanotube Surface Functionalization Effects in Blended Multiwalled Carbon Nanotube/PVDF Composites SO JOURNAL OF APPLIED POLYMER SCIENCE LA English DT Article DE nanocomposites; carbon nanotubes; dispersions; mixing AB A mixed fill system of multiwalled carbon nanotubes (MWCNT) and hydroxylated MWCNT (HO-MWCNT) in a poly(vinylidene fluoride) (PVDF) matrix was investigated to improve nanotube dispersion and enhance electrical percolation for the bulk nanocomposites. Nonfunctionalized MWCNT were blended at various concentrations into dimethylformamide solutions containing PVDF with 0, 5, or 10 wt % HO-MWCNT. Composite samples prepared from these solutions were examined by four-point probe resistivity measurements. The percolation threshold decreased from 0.49 wt % MWCNT in binary MWCNT/PVDF composites to 0.25 wt % for ternary composites containing MWCNT/HO-MWCNT/PVDF, with either 5 or 10 wt % HO-MWCNT. In the case of the ternary composite with 10 wt % HO-MWCNT, the lowest fill percent of MWCNT (0.25 wt %) measured a conductivity that was three orders of magnitude higher than the binary MWCNT/PVDF composite containing twice the concentration of MWCNT (0.5 wt %). (C) 2010 Wiley Periodicals, Inc. J Appl Polym Sci 120: 1379-1384, 2011 C1 [O'Bryan, G.; Yang, E. L.; Zifer, T.; Wally, K.; Skinner, J. L.; Vance, A. L.] Sandia Natl Labs, Dept Chem Mat, Livermore, CA 94551 USA. RP O'Bryan, G (reprint author), Sandia Natl Labs, Dept Chem Mat, Livermore, CA 94551 USA. EM gobryan@sandia.gov FU Sandia National Laboratories (for the United States Department of Energy) [DE-AC04-94-AL85000] FX Contract grant sponsor: Laboratory Directed Research and Development Program at Sandia National Laboratories (for the United States Department of Energy); contract grant number: DE-AC04-94-AL85000. NR 19 TC 13 Z9 14 U1 2 U2 23 PU WILEY-BLACKWELL PI MALDEN PA COMMERCE PLACE, 350 MAIN ST, MALDEN 02148, MA USA SN 0021-8995 J9 J APPL POLYM SCI JI J. Appl. Polym. Sci. PD MAY 5 PY 2011 VL 120 IS 3 BP 1379 EP 1384 DI 10.1002/app.33264 PG 6 WC Polymer Science SC Polymer Science GA 731XC UT WOS:000288142700017 ER PT J AU Black, M Messman, J Rawlins, J AF Black, Micah Messman, Jamie Rawlins, James TI Chain Transfer of Vegetable Oil Macromonomers in Acrylic Solution Copolymerization SO JOURNAL OF APPLIED POLYMER SCIENCE LA English DT Article DE macromonomers; copolymerization; renewable resources ID LINSEED OIL; EMULSION; SPECTROSCOPY; POLYMERS AB The use of vegetable oil macromonomers (VOMMs) as comonomers in emulsion polymerization enables good film coalescence without the use of solvents that constitute volatile organic compounds (VOCs). VOMMs are derived from renewable resources and offer the potential of post-application crosslinking via auto-oxidation. However, chain transfer reactions of VOMMs with initiator and/or polymer radicals during emulsion polymerization reduce the amount of allylic hydrogen atoms available for primary auto-oxidation during drying. Vegetable oils and derivatives were reacted with butyl acrylate and methyl methacrylate via solution polymerization, and the polymerization was monitored using in situ infrared spectroscopy to determine the extent of chain transfer. NMR spectroscopy was used to determine the loci of chain transfer and the molecular weight characteristics of the polymers were characterized by SEC. Solution polymerization was utilized because this limited temperature fluctuations and insolubility of the polymer. (C) 2010 Wiley Periodicals, Inc. J Appl Polym Sci 120: 1390-1396, 2011 C1 [Black, Micah; Rawlins, James] Univ So Mississippi, Sch Polymers & High Performance Mat, Hattiesburg, MS 39406 USA. [Messman, Jamie] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Messman, Jamie] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Rawlins, J (reprint author), Univ So Mississippi, Sch Polymers & High Performance Mat, Hattiesburg, MS 39406 USA. EM james.rawlins@usm.edu FU Cooperative State Research, Education, and Extension Service (U.S. Department of Agriculture) [2001-38202-10424, 2006-38202-16954] FX Contract grant sponsor: Cooperative State Research, Education, and Extension Service (U.S. Department of Agriculture); contract grant numbers: 2001-38202-10424, 2006-38202-16954. NR 18 TC 2 Z9 2 U1 2 U2 8 PU WILEY-BLACKWELL PI MALDEN PA COMMERCE PLACE, 350 MAIN ST, MALDEN 02148, MA USA SN 0021-8995 J9 J APPL POLYM SCI JI J. Appl. Polym. Sci. PD MAY 5 PY 2011 VL 120 IS 3 BP 1390 EP 1396 DI 10.1002/app.31546 PG 7 WC Polymer Science SC Polymer Science GA 731XC UT WOS:000288142700019 ER PT J AU Schmiedeshoff, GM Mun, ED Lounsbury, AW Tracy, SJ Palm, EC Hannahs, ST Park, JH Murphy, TP Bud'ko, SL Canfield, PC AF Schmiedeshoff, G. M. Mun, E. D. Lounsbury, A. W. Tracy, S. J. Palm, E. C. Hannahs, S. T. Park, J. -H. Murphy, T. P. Bud'ko, S. L. Canfield, P. C. TI Multiple regions of quantum criticality in YbAgGe SO PHYSICAL REVIEW B LA English DT Article ID HEAVY-FERMION YBAGGE; PHASE-DIAGRAM; FRUSTRATION; POINTS; METALS AB Dilation and thermopower measurements on YbAgGe, a heavy-fermion antiferromagnet, clarify and refine the magnetic-field temperature (H-T) phase diagram and reveal a field-induced phase with T-linear resistivity. On the low-H side of this phase we find evidence for a first-order transition and suggest that YbAgGe at 4.5 T may be close to a quantum critical end point. On the high-H side our results are consistent with a second-order transition suppressed to a quantum critical point near 7.2 T. We discuss these results in light of global phase diagrams proposed for Kondo lattice systems. C1 [Schmiedeshoff, G. M.; Lounsbury, A. W.; Tracy, S. J.] Occidental Coll, Dept Phys, Los Angeles, CA 90041 USA. [Mun, E. D.; Bud'ko, S. L.; Canfield, P. C.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Mun, E. D.; Bud'ko, S. L.; Canfield, P. C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Palm, E. C.; Hannahs, S. T.; Park, J. -H.; Murphy, T. P.] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. RP Schmiedeshoff, GM (reprint author), Occidental Coll, Dept Phys, Los Angeles, CA 90041 USA. RI Lounsbury, Amanda/L-9285-2013; Canfield, Paul/H-2698-2014; Hannahs, Scott/B-1274-2008 OI Lounsbury, Amanda/0000-0002-1246-5214; Hannahs, Scott/0000-0002-5840-7714 FU National Science Foundation [DMR-1006118]; US Department of Energy, Basic Energy Sciences [DE-AC02-07CH11358]; National Science Foundation; State of Florida; US Department of Energy FX This work was supported by the National Science Foundation under Grant No. DMR-1006118. Work at Ames Laboratory was supported by the US Department of Energy, Basic Energy Sciences, under Contract No. DE-AC02-07CH11358. Work at the National High Magnetic Field Laboratory was supported under the auspices of the National Science Foundation, the State of Florida, and the US Department of Energy. NR 35 TC 11 Z9 11 U1 3 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 4 PY 2011 VL 83 IS 18 AR 180408 DI 10.1103/PhysRevB.83.180408 PG 4 WC Physics, Condensed Matter SC Physics GA 800BU UT WOS:000293333600004 ER PT J AU Podesta, JJ AF Podesta, J. J. TI On the energy cascade rate of solar wind turbulence in high cross helicity flows SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article ID MAGNETOHYDRODYNAMIC TURBULENCE; 1 AU; 3RD-ORDER MOMENTS; INERTIAL-RANGE; MAGNETIC-FIELD; MHD TURBULENCE; DISSIPATION; SPECTRUM; PLASMA; PROTON AB Improved observations and analysis of solar wind fluctuations at 1 AU show that the total energy spectrum, kinetic plus magnetic, is in better agreement with the Kraichnan 3/2 scaling than with the Kolmogorov 5/3 scaling, consistent with simulations of incompressible MHD turbulence with a strong ambient magnetic field which exhibit a perpendicular energy spectrum proportional to k(perpendicular to)(-3/2). The Kraichnan scaling is especially clear in solar wind flows having large values of the normalized cross helicity sigma(c). In this study, a generalization of Boldyrev's theory that applies to turbulence with nonvanishing cross helicity is used to estimate the energy cascade rate for high cross helicity flows in the solar wind at 1 AU. The analysis of 85 intervals of solar wind data from the Wind spacecraft characterized by normalized cross helicities in the range |sigma(c)| > 0.88 yields typical values of the energy dissipation rate epsilon ranging from 100 to 2400 J/kg/s. This is roughly a factor of 4 or 5 smaller than estimates of the proton heating rate at 1 AU needed to account for the nonadiabatic solar wind expansion. The results suggest that the reduction in turbulent heating in high cross helicity flows creates a tangible deficit in the heating rate required by empirical models based on average solar wind properties. C1 Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Podesta, JJ (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM jpodesta@solar.stanford.edu FU NASA; NSF FX I am grateful to Jean Perez for computing the constant C0 using data from his numerical simulations. Helpful discussions with Joe Borovsky, Charles Smith, and Stas Boldyrev are also gratefully acknowledged. This research is supported by the NASA Solar and Heliospheric Physics Program, the NASA Heliospheric Guest Investigator Program, and the NSF SHINE Program. NR 61 TC 8 Z9 8 U1 0 U2 2 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0148-0227 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAY 4 PY 2011 VL 116 AR A05101 DI 10.1029/2010JA016306 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 761RE UT WOS:000290414900004 ER PT J AU Jin, YH Voss, BA Jin, A Long, H Noble, RD Zhang, W AF Jin, Yinghua Voss, Bret A. Jin, Athena Long, Hai Noble, Richard D. Zhang, Wei TI Highly CO2-Selective Organic Molecular Cages: What Determines the CO2 Selectivity SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID OCTAHEDRAL NANOCONTAINER MOLECULE; CARBON-DIOXIDE CAPTURE; ALKYNE METATHESIS; CONJUGATED POLYMERS; SORPTION PROPERTIES; HYDROGEN STORAGE; GAS-ADSORPTION; GUEST EXCHANGE; ONE-POT; MACROCYCLES AB A series of novel organic cage compounds 1-4 were successfully synthesized from readily available starting materials in one-pot in decent to excellent yields (46-90%) through a dynamic covalent chemistry approach (imine condensation reaction). Covalently cross-linked cage framework 14 was obtained through the cage-to-framework strategy via the Sonogashira coupling of cage 4 with the 1,4-diethynylbenzene linker molecule. Cage compounds 1-4 and framework 14 exhibited exceptional high ideal selectivity (36/1-138/1) in adsorption of CO2 over N-2 under the standard temperature and pressure (STP, 20 degrees C, 1 bar). Gas adsorption studies indicate that the high selectivity is provided not only by the amino group density (mol/g), but also by the intrinsic pore size of the cage structure (distance between the top and bottom panels), which can be tuned by judiciously choosing building blocks of different size. The systematic studies on the structure-property relationship of this novel class of organic cages are reported herein for the first time; they provide critical knowledge on the rational design principle of these cage-based porous materials that have shown great potential in gas separation and carbon capture applications. C1 [Jin, Yinghua; Jin, Athena; Zhang, Wei] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Voss, Bret A.; Noble, Richard D.] Univ Colorado, Dept Chem & Biol Engn, Boulder, CO 80309 USA. [Long, Hai] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Zhang, W (reprint author), Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA. EM Wei.Zhang@Colorado.edu RI Long, Hai/C-5838-2015 FU University of Colorado; CRCW; Office of Energy Efficiency and Renewable Energy of the U.S. Department of Energy [DE-AC36-08GO28308] FX We thank Dr. Richard Shoemaker for solid state NMR assistance, University of Colorado innovative seed grant, and CRCW Junior Faculty Development award for funding support. This research used capabilities of the National Renewable Energy Laboratory Computational Sciences Center, which is supported by the Office of Energy Efficiency and Renewable Energy of the U.S. Department of Energy under Contract No. DE-AC36-08GO28308. NR 63 TC 122 Z9 123 U1 19 U2 152 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 4 PY 2011 VL 133 IS 17 BP 6650 EP 6658 DI 10.1021/ja110846c PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA 760ZG UT WOS:000290363400032 PM 21473590 ER PT J AU Shavorskiy, A Aksoy, F Grass, ME Liu, Z Bluhm, H Held, G AF Shavorskiy, Andrey Aksoy, Funda Grass, Michael E. Liu, Zhi Bluhm, Hendrik Held, Georg TI A Step toward the Wet Surface Chemistry of Glycine and Alanine on Cu{110}: Destabilization and Decomposition in the Presence of Near-Ambient Water Vapor SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID TEMPERATURE-PROGRAMMED DESORPTION; CHIRAL CU(531) SURFACE; OXYGEN-COVERED CU(110); ADVANCED LIGHT-SOURCE; HETEROGENEOUS CATALYSIS; ADSORPTION FOOTPRINTS; ENANTIOPURE ALANINE; COPPER SURFACES; METAL-SURFACES; SPECTROSCOPY AB The coadsorption of water with organic molecules under near-ambient pressure and temperature conditions opens up new reaction pathways on model catalyst surfaces that are not accessible in conventional ultrahigh-vacuum surface-science experiments. The surface chemistry of glycine and alanine at the water-exposed Cu{110} interface was studied in situ using ambient-pressure photoemission and X-ray absorption spectroscopy techniques. At water pressures above 10(-5) Torr a significant pressure-dependent decrease in the temperature for dissociative desorption was observed for both amino acids, accompanied by the appearance of a new CN intermediate, which is not observed for lower pressures. The most likely reaction mechanisms involve dehydrogenation induced by O and/or OH surface species resulting from the dissociative adsorption of water. The linear relationship between the inverse decomposition temperature and the logarithm of water pressure enables determination of the activation energy for the surface reaction, between 213 and 232 kJ/mol, and a prediction of the decomposition temperature at the solid-liquid interface by extrapolating toward the equilibrium vapor pressure. Such experiments near the equilibrium vapor pressure provide important information about elementary surface processes at the solid-liquid interface, which can be retrieved neither under ultrahigh vacuum conditions nor from interfaces immersed in a solution. C1 [Shavorskiy, Andrey; Held, Georg] Univ Reading, Dept Chem, Reading RG6 6AD, Berks, England. [Aksoy, Funda; Grass, Michael E.; Liu, Zhi] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. [Aksoy, Funda] Nigde Univ, Fac Arts & Sci, Dept Phys, Nigde, Turkey. [Bluhm, Hendrik] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Held, G (reprint author), Univ Reading, Dept Chem, Reading RG6 6AD, Berks, England. EM g.held@reading.ac.uk RI Held, Georg/D-5468-2013; Liu, Zhi/B-3642-2009; OI Liu, Zhi/0000-0002-8973-6561; Held, Georg/0000-0003-0726-4183 FU European Community through the Marie Curie Early Stage Training Network "MONET" [MEST-CT-2005-020908]; EPSRC [EP/H015493/1]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the European Community through the Marie Curie Early Stage Training Network "MONET" (MEST-CT-2005-020908) and by the EPSRC through an overseas travel grant (No. EP/H015493/1). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 70 TC 17 Z9 17 U1 1 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 4 PY 2011 VL 133 IS 17 BP 6659 EP 6667 DI 10.1021/ja110910y PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA 760ZG UT WOS:000290363400033 PM 21473591 ER PT J AU Liu, C Sawaya, MR Cheng, PN Zheng, J Nowick, JS Eisenberg, D AF Liu, Cong Sawaya, Michael R. Cheng, Pin-Nan Zheng, Jing Nowick, James S. Eisenberg, David TI Characteristics of Amyloid-Related Oligomers Revealed by Crystal Structures of Macrocyclic beta-Sheet Mimics SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ALZHEIMERS-DISEASE; A-BETA; MODEL SYSTEMS; DIFFRACTION DATA; ALPHA-SYNUCLEIN; PLEATED SHEETS; PROTEIN; FIBRILS; TAU; PEPTIDE AB Protein amyloid oligomers have been strongly linked to amyloid diseases and can be intermediates to amyloid fibers. beta-Sheets have been identified in amyloid oligomers. However, because of their transient and highly polymorphic properties, the details of their self-association remain elusive. Here we explore oligomer structure using a model system: macrocyclic peptides. Key amyloidogenic sequences from A beta and tau were incorporated into macrocycles, thereby restraining them to beta-strands, but limiting the growth of the oligomers so they may crystallize and cannot fibrillate. We determined the atomic structures for four such oligomers, and all four reveal tetrameric interfaces in which beta-sheet dimers pair together by highly complementary, dry interfaces, analogous to steric zippers found in fibers, suggesting a common structure for amyloid oligomers and fibers. In amyloid fibers, the axes of the paired sheets are either parallel or antiparallel, whereas the oligomeric interfaces display a variety of sheet-to-sheet pairing angles, offering a structural explanation for the heterogeneity of amyloid oligomers. C1 [Liu, Cong; Sawaya, Michael R.; Eisenberg, David] Univ Calif Los Angeles, Inst Mol Biol, Howard Hughes Med Inst, UCLA DOE Inst Genom & Prote, Los Angeles, CA 90095 USA. [Cheng, Pin-Nan; Zheng, Jing; Nowick, James S.] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. RP Eisenberg, D (reprint author), Univ Calif Los Angeles, Inst Mol Biol, Howard Hughes Med Inst, UCLA DOE Inst Genom & Prote, Los Angeles, CA 90095 USA. EM david@mbi.ucla.edu RI Eisenberg, David/E-2447-2011; liu, cong/H-1103-2011 FU NIH [GM-49076, AG-029430]; NSF; HHMI FX We thank the NE-CAT beamline, the Advanced Photon Source for beam time and collection assistance. We thank NIH (GM-49076 and AG-029430), NSF, and HHMI for grant support. NR 61 TC 53 Z9 53 U1 0 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 4 PY 2011 VL 133 IS 17 BP 6736 EP 6744 DI 10.1021/ja200222n PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA 760ZG UT WOS:000290363400042 PM 21473620 ER PT J AU Joglekar, YN Saxena, A AF Joglekar, Yogesh N. Saxena, Avadh TI Robust PT-symmetric chain and properties of its Hermitian counterpart SO PHYSICAL REVIEW A LA English DT Article ID LATTICE; STATES AB We study the properties of a parity-and time-reversal-(PT) symmetric tight-binding chain of size N with position-dependent hopping amplitude. In contrast to the fragile PT-symmetric phase of a chain with constant hopping and imaginary impurity potentials, we show that, under very general conditions, our model is always in the PT-symmetric phase. We numerically obtain the energy spectrum and the density of states of such a chain, and show that they are widely tunable. By studying the size dependence of inverse participation ratios, we show that although the chain is not translationally invariant, most of its eigenstates are extended. Our results indicate that tight-binding models with non-Hermitian, PT-symmetric hopping have a robust PT-symmetric phase and rich dynamics which may be explored in coupled waveguides. C1 [Joglekar, Yogesh N.] IUPUI, Dept Phys, Indianapolis, IN 46202 USA. [Saxena, Avadh] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Joglekar, YN (reprint author), IUPUI, Dept Phys, Indianapolis, IN 46202 USA. FU U.S. Department of Energy FX Y.J. acknowledges useful discussions with Donald Priour and Ricardo Decca. This work was supported in part by the U.S. Department of Energy. NR 21 TC 32 Z9 32 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 J9 PHYS REV A JI Phys. Rev. A PD MAY 4 PY 2011 VL 83 IS 5 AR 050101 DI 10.1103/PhysRevA.83.050101 PG 4 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 759GU UT WOS:000290229500001 ER PT J AU Dominguez, F Marquet, C Xiao, BW Yuan, F AF Dominguez, Fabio Marquet, Cyrille Xiao, Bo-Wen Yuan, Feng TI Universality of unintegrated gluon distributions at small x SO PHYSICAL REVIEW D LA English DT Article ID DEUTERON-GOLD COLLISIONS; AZIMUTHAL CORRELATIONS; PA-COLLISIONS; LARGE NUCLEI; QCD; QUARK; GLASS AB We systematically study dijet production in various processes in the small-x limit and establish an effective k(t)-factorization for hard processes in a system with dilute probes scattering on a dense target. We find that the well-known Weizsacker-Williams gluon distribution can be directly probed in the quark-antiquark jet correlation in deep inelastic scattering and the dipole gluon distribution can be directly measured in the direct photon-jet correlation in pA collisions. In the large-N(c) limit, the unintegrated gluon distributions involved in other different dijet channels in pA collisions are shown to be related to two widely proposed ones: the Weizsacker-Williams gluon distribution and the dipole gluon distribution. C1 [Dominguez, Fabio] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Marquet, Cyrille] CERN, Dept Phys, Theory Unit, CH-1211 Geneva, Switzerland. [Xiao, Bo-Wen] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Xiao, Bo-Wen; Yuan, Feng] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Yuan, Feng] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. RP Dominguez, F (reprint author), Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA. RI Yuan, Feng/N-4175-2013 FU U.S. Department of Energy [DE-AC02-05CH11231, DE-AC02-98CH10886]; DOE [DE-SC0002145] FX We thank Al Mueller for stimulating discussions and critical reading of the manuscript. We thank Alberto Accardi, Emil Avsar, Markus Diehl, Volker Koch, Larry McLerran, Stephane Munier, Jianwei Qiu, Anna Stasto, Raju Venugopalan and Xin-Nian Wang for helpful conversations. This work was supported in part by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 and DOE O. J. I. Grant No. DE-SC0002145. We are grateful to RIKEN, Brookhaven National Laboratory and the U.S. Department of Energy (Contract No. DE-AC02-98CH10886) for providing the facilities essential for the completion of this work. We also thank the Institute for Nuclear Theory at the University of Washington for its hospitality and the Department of Energy for partial support during the completion of this work. NR 53 TC 128 Z9 128 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 J9 PHYS REV D JI Phys. Rev. D PD MAY 4 PY 2011 VL 83 IS 10 AR 105005 DI 10.1103/PhysRevD.83.105005 PG 27 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 759HD UT WOS:000290230400009 ER PT J AU Speck, T AF Speck, Thomas TI Effective free energy for pinned membranes SO PHYSICAL REVIEW E LA English DT Article ID SUPPORTED MEMBRANES; LATERAL DIFFUSION; ADHESION; BONDS; JUNCTIONS AB We consider membranes adhered through specific receptor-ligand bonds. Thermal undulations of the membrane induce effective interactions between adhesion sites. We derive an upper bound to the free energy that is independent of interaction details. To the lowest order in a systematic expansion we obtain two-body interactions that allow us to map the free energy onto a lattice gas with a constant density. The induced interactions alone are not strong enough to lead to a condensation of individual adhesion sites. A measure of the thermal roughness is shown to depend on the inverse square root of the density of adhesion sites, which is in good agreement with previous computer simulations. C1 [Speck, Thomas] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Speck, Thomas] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Speck, T (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RI Speck, Thomas/F-2624-2012; Physics, Komet/C-9533-2016 OI Speck, Thomas/0000-0002-6357-1180; FU Alexander von Humboldt Foundation; Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division and Chemical Sciences, Geosciences, and Biosciences Division of the US Department of Energy [DE-AC02-05CH11231] FX I thank Oded Farago for helpful discussions and a critical reading of the manuscript. Financial support from the Alexander von Humboldt Foundation and from the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division and Chemical Sciences, Geosciences, and Biosciences Division of the US Department of Energy under Contract No. DE-AC02-05CH11231 is gratefully acknowledged. NR 22 TC 6 Z9 6 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD MAY 4 PY 2011 VL 83 IS 5 AR 050901 DI 10.1103/PhysRevE.83.050901 PN 1 PG 4 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 759HF UT WOS:000290230600001 PM 21728477 ER PT J AU Zhou, SY Zhu, Y Langner, MC Chuang, YD Yu, P Yang, WL Gonzalez, AGC Tahir, N Rini, M Chu, YH Ramesh, R Lee, DH Tomioka, Y Tokura, Y Hussain, Z Schoenlein, RW AF Zhou, S. Y. Zhu, Y. Langner, M. C. Chuang, Y. -D. Yu, P. Yang, W. L. Gonzalez, A. G. Cruz Tahir, N. Rini, M. Chu, Y. -H. Ramesh, R. Lee, D. -H. Tomioka, Y. Tokura, Y. Hussain, Z. Schoenlein, R. W. TI Ferromagnetic Enhancement of CE-Type Spin Ordering in (Pr, Ca)MnO3 SO PHYSICAL REVIEW LETTERS LA English DT Article ID NEUTRON-DIFFRACTION; MANGANITES; TRANSITION; STATES; PR0.7CA0.3MNO3; PR1-XCAXMNO3; CHARGE AB We present resonant soft x-ray scattering results from small bandwidth manganites (Pr, Ca)MnO3, which show that the CE-type spin ordering (SO) at the phase boundary is stabilized only below the canted antiferromagnetic transition temperature and enhanced by ferromagnetism in the macroscopically insulating state (FM-I). Our results reveal the fragility of the CE-type ordering that underpins the colossal magnetoresistance effect in this system, as well as an unexpected cooperative interplay between FM-I and CE-type SO which is in contrast to the competitive interplay between the ferromagnetic metallic state and CE-type ordering. C1 [Zhou, S. Y.; Chuang, Y. -D.; Yang, W. L.; Gonzalez, A. G. Cruz; Tahir, N.; Hussain, Z.; Schoenlein, R. W.] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. [Zhou, S. Y.; Zhu, Y.; Langner, M. C.; Rini, M.; Ramesh, R.; Lee, D. -H.; Schoenlein, R. W.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Zhu, Y.] Univ Calif Davis, Dept Appl Sci, Davis, CA 95616 USA. [Yu, P.; Ramesh, R.; Lee, D. -H.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Tahir, N.] Natl Ctr Phys, Islamabad, Pakistan. [Chu, Y. -H.] Natl Chiao Tung Univ, Dept Mat Sci & Engn, Hsingchu 30010, Taiwan. [Tomioka, Y.] Natl Inst Adv Ind Sci & Technol, Nanoelect Res Inst, Tsukuba, Ibaraki 3058562, Japan. [Tokura, Y.] Univ Tokyo, Dept Appl Phys, Bunkyo Ku, Tokyo 1138656, Japan. [Tokura, Y.] RIKEN, Adv Sci Inst, CMRG, Wako, Saitama 3510198, Japan. [Tokura, Y.] RIKEN, Adv Sci Inst, CERG, Wako, Saitama 3510198, Japan. RP Zhou, SY (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. EM szhou@lbl.gov; ychuang@lbl.gov; rwschoenlein@lbl.gov RI Ying-Hao, Chu/A-4204-2008; Zhou, Shuyun/A-5750-2009; Schoenlein, Robert/D-1301-2014; Tokura, Yoshinori/C-7352-2009; Yang, Wanli/D-7183-2011; Yu, Pu/F-1594-2014 OI Ying-Hao, Chu/0000-0002-3435-9084; Schoenlein, Robert/0000-0002-6066-7566; Yang, Wanli/0000-0003-0666-8063; FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, the Materials Sciences and Engineering Division under the Department of Energy [DE-AC02-05CH11231]; NSC [099-2811-M-009-003] FX The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, the Materials Sciences and Engineering Division under the Department of Energy Contract No. DE-AC02-05CH11231. Y. H. C. is supported by NSC 099-2811-M-009-003. NR 22 TC 19 Z9 19 U1 7 U2 42 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 4 PY 2011 VL 106 IS 18 AR 186404 DI 10.1103/PhysRevLett.106.186404 PG 5 WC Physics, Multidisciplinary SC Physics GA 759GQ UT WOS:000290229100003 PM 21635110 ER PT J AU Hur, TB Phuoc, TX Chyu, MK Romanov, V AF Hur, Tae-Bong Phuoc, Tran X. Chyu, Minking K. Romanov, Vyacheslav TI Evolution of rheological properties of the nanofluids composed of laponite particles and Mg-Fe layered double hydroxide nanosheets SO POLYMER LA English DT Article DE Laser ablation; LDH nanosheet; Laponite ID DISPERSIONS; SUSPENSIONS; DELAMINATION; THIXOTROPY; EXCHANGE; ANION; CLAY AB The thixotropic clay suspensions composed of laponite particles and Mg-Fe layered double hydroxide nanosheets were examined. By adding a very small amount of the layered double hydroxide nanosheets overall theological properties of the host laponite suspension have been changed. Though the particle concentration of the mixture suspension is only about 1 wt%, the mixture quickly becomes a gel in a day by the electrostatic attraction between nano-materials. When a constant shear rate is applied to the mixture gel suspension, at short time, stress increases linearly with elastic deformation of the mixture. Beyond the maximum of stress, while the solid-like gel structure is being broken down with time of shearing, the stress increases again by reflecting shear enhanced association of solid phase. This is likely that the mixture suspension shows partially the behavior of memory effect. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Hur, Tae-Bong; Phuoc, Tran X.; Romanov, Vyacheslav] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Hur, Tae-Bong; Chyu, Minking K.] Univ Pittsburgh, Dept Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA. RP Hur, TB (reprint author), Univ Pittsburgh, Dept Geol & Planetary Sci, 4107 OHara St SRCC, Pittsburgh, PA 15260 USA. EM Tae.Hur@netl.doe.gov RI Romanov, Vyacheslav/C-6467-2008 OI Romanov, Vyacheslav/0000-0002-8850-3539 FU National Energy Technology Laboratory under the RES [DE-FE0004000]; DOE-NETL FX This technical effort was performed in support of the National Energy Technology Laboratory's ongoing research in Hydrophobic/Hydrophilic Interactions under the RES contract DE-FE0004000 and the EPACT program of DOE-NETL NR 24 TC 1 Z9 1 U1 3 U2 17 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 J9 POLYMER JI Polymer PD MAY 4 PY 2011 VL 52 IS 10 BP 2238 EP 2243 DI 10.1016/j.polymer.2011.03.022 PG 6 WC Polymer Science SC Polymer Science GA 758AJ UT WOS:000290131500017 ER PT J AU You, FQ Grossmann, IE Wassick, JM AF You, Fengqi Grossmann, Ignacio E. Wassick, John M. TI Multisite Capacity, Production, and Distribution Planning with Reactor Modifications: MILP Model, Bilevel Decomposition Algorithm versus Lagrangean Decomposition Scheme SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID SUPPLY CHAIN OPTIMIZATION; FLEXIBLE PROCESS NETWORKS; PROCESSING NETWORKS; DEMAND UNCERTAINTY; INVESTMENT MODEL; DESIGN; MANAGEMENT; EXPANSION; INDUSTRY; PLANTS AB We propose a multiperiod mixed-integer linear programming (MILP) model for the simultaneous capacity, production, and distribution planning for a multisite system including a number of production sites and markets. Multiple products are produced in several production trains that are located in different sites. The unique feature of the proposed model is that it considers the construction times of capacity modifications and takes into account the option of capacity transformation by modifying the reactor in a production train from producing one product family to producing another one. To solve the resulting large-scale MILP model, we present solution techniques based on Lagrangean decomposition and bilevel decomposition. Numerical examples are presented to illustrate the applicability of the model and the performance of the algorithms. It is shown that the bilevel decomposition is the superior solution approach in terms of faster computational times and smaller optimality gaps for the problem addressed in this work. C1 [You, Fengqi; Grossmann, Ignacio E.] Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA. [Wassick, John M.] Dow Chem Co USA, Midland, MI 48674 USA. RP Grossmann, IE (reprint author), Argonne Natl Lab, 9700 S Cass Ave,Bldg 240, Argonne, IL 60439 USA. EM grossmann@cmu.edu RI You, Fengqi/F-6894-2011; You, Fengqi/B-5040-2011 OI You, Fengqi/0000-0001-9609-4299 FU Dow Chemical Company; Pennsylvania Infrastructure Technology Alliance (PITA); National Science Foundation [CMMI-0556090] FX The authors gratefully acknowledge financial support from The Dow Chemical Company, the Pennsylvania Infrastructure Technology Alliance (PITA), and the National Science Foundation under Grant No. CMMI-0556090. NR 34 TC 28 Z9 28 U1 1 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD MAY 4 PY 2011 VL 50 IS 9 BP 4831 EP 4849 DI 10.1021/ie100559y PG 19 WC Engineering, Chemical SC Engineering GA 753HX UT WOS:000289764000004 ER PT J AU Ebner, AD Gray, ML Chisholm, NG Black, QT Mumford, DD Nicholson, MA Ritter, JA AF Ebner, A. D. Gray, M. L. Chisholm, N. G. Black, Q. T. Mumford, D. D. Nicholson, M. A. Ritter, J. A. TI Suitability of a Solid Amine Sorbent for CO2 Capture by Pressure Swing Adsorption SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID CARBON-DIOXIDE CAPTURE; EXPANDED MESOPOROUS SILICA; WATER-TOLERANT ADSORBENT; FLUE-GAS; SITE-ISOLATION; HIGH-CAPACITY; HYDROTALCITE; ALKALI; MCM-41; REGENERATION AB This study showed that a solid amine, composed of poly(ethylenimine) immobilized into a CARiACT G10 silica substrate, is a feasible sorbent for applications in a pressure swing adsorption (PSA) process for postcombustion CO2 capture. This deduction materialized from an extensive study of the behavior of this material over a wide range of industrially relevant conditions using thermogravimetric analysis. The temperature ranged from 40 to 100 degrees C, the CO2 partial pressure ranged from 1.2 to 100 vol % with the total pressure fixed at 1 atm, the relative humidity ranged from dry conditions to 2 vol %, and the number of consecutive adsorption and desorption cycles ranged from 4 to 76. The results revealed that this solid amine sorbent was very stable under the conditions investigated. Water vapor at a low relative humidity exhibited only a minor and reversible effect on both the thermodynamics and kinetics of the CO2 uptake and release. The isothermal CO2 working capacity ranged between 0.25 and 2.8 mol/kg, increased with increasing CO2 concentration, exhibited a maximum with increasing temperature, and produced a heat of adsorption/reaction of around 50.0 kJ/mol. It was also determined that the optimal operating temperature for a PSA process was around 80 degrees C for CO2 partial pressures > 10 kPa and 60-70 degrees C for CO2 partial pressures < 10 kPa. C1 [Ebner, A. D.; Chisholm, N. G.; Black, Q. T.; Mumford, D. D.; Nicholson, M. A.; Ritter, J. A.] Univ S Carolina, Dept Chem Engn, Columbia, SC 29208 USA. [Gray, M. L.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Ritter, JA (reprint author), Univ S Carolina, Dept Chem Engn, Columbia, SC 29208 USA. EM ritter@cec.sc.edu FU NSF Research Experience for Undergraduates (REU) Site in Chemical Engineering at the University of South Carolina [EEC-0851997]; Center for Strategic Approaches to the Generation of Electricity at the University of South Carolina FX The authors gratefully acknowledge financial support provided, in part, by the NSF Research Experience for Undergraduates (REU) Site in Chemical Engineering at the University of South Carolina under Grant EEC-0851997 and, in part, by the Center for Strategic Approaches to the Generation of Electricity at the University of South Carolina. NR 47 TC 56 Z9 58 U1 5 U2 75 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD MAY 4 PY 2011 VL 50 IS 9 BP 5634 EP 5641 DI 10.1021/ie2000709 PG 8 WC Engineering, Chemical SC Engineering GA 753HX UT WOS:000289764000074 ER PT J AU Markovskiy, ND Munoz, JA Lucas, MS Li, CW Delaire, O Stone, MB Abernathy, DL Fultz, B AF Markovskiy, N. D. Munoz, J. A. Lucas, M. S. Li, Chen W. Delaire, O. Stone, M. B. Abernathy, D. L. Fultz, B. TI Nonharmonic phonons in MgB2 at elevated temperatures SO PHYSICAL REVIEW B LA English DT Article ID SUPERCONDUCTING PROPERTIES; THERMAL-EXPANSION; PSEUDOPOTENTIALS; SPECTROSCOPY; SPECTRUM; DIBORIDE; BORON AB Inelastic neutron scattering was used to measure phonon spectra in MgB2 and Mg0.75Al0.25B2 from 7 to 750 K to investigate anharmonicity and adiabatic electron-phonon coupling. First-principles calculations of phonons with a linear response method were performed at multiple unit cell volumes, and the Helmholtz free energy was minimized to obtain the lattice parameters and phonon dynamics at elevated temperature in the quasiharmonic approximation. Most of the temperature dependence of the phonon density of states could be understood with the quasiharmonic approximation, although there was also significant thermal broadening of the phonon spectra. In comparison to Mg0.75Al0.25B2, in the energy range of 60 to 80 meV the experimental phonon spectra from MgB2 showed a nonmonotonic change with temperature around 500 K. This may originate from a change with temperature of the adiabatic electron-phonon coupling. C1 [Markovskiy, N. D.; Munoz, J. A.; Li, Chen W.; Fultz, B.] CALTECH, Dept Appl Phys & Mat Sci, Pasadena, CA 91125 USA. [Lucas, M. S.; Delaire, O.; Stone, M. B.; Abernathy, D. L.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Markovskiy, ND (reprint author), CALTECH, Dept Appl Phys & Mat Sci, Pasadena, CA 91125 USA. RI Munoz, Jorge/C-8427-2011; Stone, Matthew/G-3275-2011; Abernathy, Douglas/A-3038-2012; Li, Chen/D-1542-2010; BL18, ARCS/A-3000-2012 OI Stone, Matthew/0000-0001-7884-9715; Abernathy, Douglas/0000-0002-3533-003X; Li, Chen/0000-0002-0758-5334; FU Department of Energy through the Basic Energy Sciences [DE-FG02-03ER46055]; Scientific User Facilities Division; Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, DOE FX This work was supported by the Department of Energy through the Basic Energy Sciences Grant No. DE-FG02-03ER46055. The portions of this work conducted at Oak Ridge National Laboratory were supported by the Scientific User Facilities Division and by the Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, DOE. This work benefited from DANSE software developed under NSF Grant No. DMR-0520547. NR 52 TC 2 Z9 2 U1 1 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 4 PY 2011 VL 83 IS 17 AR 174301 DI 10.1103/PhysRevB.83.174301 PG 7 WC Physics, Condensed Matter SC Physics GA 934VC UT WOS:000303473800001 ER PT J AU Wang, KF Lei, HC Petrovic, C AF Wang, Kefeng Lei, Hechang Petrovic, C. TI Thermoelectric studies of KxFe2-ySe2 indicating a weakly correlated superconductor SO PHYSICAL REVIEW B LA English DT Article ID IRON; THERMOPOWER; CONDUCTIVITY; GRADIENT; ANGLE; DRAG AB We report thermal transport properties of a KxFe2-ySe2 superconducting single crystal. A peak anomaly in the thermal conductivity is observed at nearly T-C/2, attributed to phonons. The thermoelectric power above T-c exhibits nearly linear behavior and could be described well by the carrier diffusion mechanism in a wide temperature range. The zero-temperature extrapolated thermoelectric power is smaller than the value in typical strongly correlated superconductors, implying a large normalized Fermi temperature. These findings indicate that KxFe2-ySe2 is a weakly or intermediately correlated superconductor. C1 [Wang, Kefeng; Lei, Hechang; Petrovic, C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Wang, KF (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RI Wang, Kefeng/E-7683-2011; Petrovic, Cedomir/A-8789-2009; LEI, Hechang/H-3278-2016 OI Wang, Kefeng/0000-0002-8449-9720; Petrovic, Cedomir/0000-0001-6063-1881; FU US DOE [DE-AC02-98CH10886]; center for Emergent Supercondcutivity; Energy Frontier Research Center; US DOE, office for Basic Energy Science FX We acknowledge valuable discussions with Louis Taillefer. We thank John Warren for help with scanning electron microscope measurements. Work at Brookhaven is supported by the US DOE under Contract No. DE-AC02-98CH10886 and in part by the center for Emergent Supercondcutivity, and Energy Frontier Research Center funded by the US DOE, office for Basic Energy Science. NR 60 TC 21 Z9 21 U1 1 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 4 PY 2011 VL 83 IS 17 AR 174503 DI 10.1103/PhysRevB.83.174503 PG 6 WC Physics, Condensed Matter SC Physics GA 934VC UT WOS:000303473800003 ER PT J AU Atanasov, V Saxena, A AF Atanasov, Victor Saxena, Avadh TI Electronic properties of corrugated graphene: the Heisenberg principle and wormhole geometry in the solid state SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID QUANTUM-MECHANICS; SURFACES AB Adopting a purely two-dimensional relativistic equation for graphene's carriers contradicts the Heisenberg uncertainty principle since it requires setting the off-the-surface coordinate of a three-dimensional wavefunction to zero. Here we present a theoretical framework for describing graphene's massless relativistic carriers in accordance with this most fundamental of all quantum principles. A gradual confining procedure is used to restrict the dynamics onto a surface and normal to the surface parts, and in the process the embedding of this surface into the three-dimensional world is accounted for. As a result an invariant geometric potential arises in the surface part which scales linearly with the mean curvature and shifts the Fermi energy of the material proportional to bending. Strain induced modification of the electronic properties or 'straintronics' is clearly an important field of study in graphene. This opens an avenue to producing electronic devices: micro-and nano-electromechanical systems (MEMS and NEMS), where the electronic properties are controlled by geometric means and no additional alteration of graphene is necessary. The appearance of this geometric potential also provides us with clues as to how quantum dynamics looks in the curved space-time of general relativity. In this context we explore a two-dimensional cross-section of the wormhole geometry, realized with graphene as a solid state thought experiment. C1 [Atanasov, Victor] Univ Sofia, Dept Condensed Matter Phys, Sofia 1164, Bulgaria. [Saxena, Avadh] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Saxena, Avadh] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. RP Atanasov, V (reprint author), Univ Sofia, Dept Condensed Matter Phys, 5 Blvd J Boucher, Sofia 1164, Bulgaria. EM vatanaso@gmail.com; avadh@lanl.gov OI Atanasov, Victor/0000-0001-6587-409X FU US Department of Energy; ICTP, Trieste, Italy FX This work was supported in part by the US Department of Energy. VA also acknowledges support by ICTP, Trieste, Italy where this paper was completed. NR 22 TC 14 Z9 14 U1 0 U2 18 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAY 4 PY 2011 VL 23 IS 17 AR 175301 DI 10.1088/0953-8984/23/17/175301 PG 7 WC Physics, Condensed Matter SC Physics GA 750NR UT WOS:000289555700007 PM 21474883 ER PT J AU Melechko, AV Pearce, RC Hensley, DK Simpson, ML McKnight, TE AF Melechko, Anatoli V. Pearce, Ryan C. Hensley, Dale K. Simpson, Michael L. McKnight, Timothy E. TI Challenges in process integration of catalytic DC plasma synthesis of vertically aligned carbon nanofibres SO JOURNAL OF PHYSICS D-APPLIED PHYSICS LA English DT Article ID CHEMICAL-VAPOR-DEPOSITION; FIELD-EMISSION PROPERTIES; LOW-TEMPERATURE GROWTH; LARGE-SCALE SYNTHESIS; COVALENT FUNCTIONALIZATION; NANOELECTRODE ARRAYS; HIPPOCAMPAL SLICES; PATTERNED GROWTH; NANOTUBE GROWTH; FABRICATION AB The ability to synthesize free-standing, individual carbon nanofibres (CNFs) aligned perpendicularly to a substrate has enabled fabrication of a large array of devices with nanoscale functional elements, including electron field emission sources, electrochemical probes, neural interface arrays, scanning probes, gene delivery arrays and many others. This was made possible by development of a catalytic plasma process, with DC bias directing the alignment of nanofibres. Successful implementation of prototypical devices has uncovered numerous challenges in the integration of this synthesis process as one of the steps in device fabrication. This paper is dedicated to these engineering and fundamental difficulties that hinder further device development. Relatively high temperature for catalytic synthesis, electrical conductivity of the substrate to maintain DC discharge and other difficulties place restrictions on substrate material. Balancing non-catalytic carbon film deposition and substrate etching, non-uniformity of plasma due to growth of the high aspect ratio structures, plasma instabilities and other factors lead to challenges in controlling the plasma. Ultimately, controlling the atomistic processes at the catalyst nanoparticle (NP) and the behaviour of the NP is the central challenge of plasma nanosynthesis of vertically aligned CNFs. C1 [Melechko, Anatoli V.; Pearce, Ryan C.] N Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27695 USA. [Hensley, Dale K.; Simpson, Michael L.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [McKnight, Timothy E.] Oak Ridge Natl Lab, Measurement Sci & Syst Engn Div, Oak Ridge, TN 37831 USA. RP Melechko, AV (reprint author), N Carolina State Univ, Dept Mat Sci & Engn, Box 7907, Raleigh, NC 27695 USA. EM anatoli_melechko@ncsu.edu RI Melechko, Anatoli/B-8820-2008; Simpson, Michael/A-8410-2011; McKnight, Tim/H-3087-2011; Hensley, Dale/A-6282-2016 OI Simpson, Michael/0000-0002-3933-3457; McKnight, Tim/0000-0003-4326-9117; Hensley, Dale/0000-0001-8763-7765 FU Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX The challenges discussed here were encountered while working with Kate Klein, Michael Guillorn, Scott Retterer, Darryl Thomas, Teri Subic, Jason Fowlkes and others at Oak Ridge National Laboratory on realization of VACNF-based devices. AVM and MLS would like to acknowledge support from the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy (processing, analytical microscopy, experimental design and modelling). The microfabrication of devices was done through user projects at the Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, and sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 89 TC 5 Z9 5 U1 0 U2 15 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0022-3727 EI 1361-6463 J9 J PHYS D APPL PHYS JI J. Phys. D-Appl. Phys. PD MAY 4 PY 2011 VL 44 IS 17 AR 174008 DI 10.1088/0022-3727/44/17/174008 PG 11 WC Physics, Applied SC Physics GA 749ZP UT WOS:000289512700008 ER PT J AU Koirala, SR Gentry, RW Mulholland, PJ Perfect, E Schwartz, JS Sayler, GS AF Koirala, Shesh R. Gentry, Randall W. Mulholland, Patrick J. Perfect, Edmund Schwartz, John S. Sayler, Gary S. TI Persistence of hydrologic variables and reactive stream solute concentrations in an east Tennessee watershed SO JOURNAL OF HYDROLOGY LA English DT Article DE Spectral analysis; Wavelet analysis; Persistence; Reactive water chemistry; Time series ID WAVELET ANALYSIS; TIME-SERIES; CHEMISTRY; TRANSPORT; NUTRIENT; FLOW AB Time and frequency domain analyses were conducted on weekly time series of water chemistry (nitrate, sulfate and calcium concentrations) collected from November 1995 to December 2005 at the West Fork of Walker Branch in Oak Ridge, Tennessee to evaluate the extent of their persistence and the relationship of this persistence to discharge and rainfall. In this study, spectral and wavelet analyses provided a theoretical basis for insights into long-term water chemistry behavior. All water chemistry parameters showed some level of persistence that was influenced by rainfall and/or discharge. Short-term persistence (less than a year) was related to the persistence of rainfall and discharge, whereas long-term persistence (more than a year) was related to the persistence of discharge. The Walker Branch conceptual hydrology model is augmented by these results that relate characteristic periodicities with flowpaths through different zones: the vadose zone (< 20 week period), saturated zone (20-50 week period) and bedrock zone (> 50 week period) with implications for reactive chemistries within the watershed. (C) 2011 Elsevier B.V. All rights reserved. C1 [Koirala, Shesh R.; Gentry, Randall W.] Univ Tennessee, Inst Secure & Sustainable Environm, Knoxville, TN 37996 USA. [Koirala, Shesh R.; Gentry, Randall W.; Schwartz, John S.] Univ Tennessee, Knoxville, TN 37996 USA. [Mulholland, Patrick J.] Oak Ridge Natl Lab, Div Earth Sci, Oak Ridge, TN USA. [Perfect, Edmund] Univ Tennessee, Dept Earth & Planetary Sci, Knoxville, TN 37996 USA. [Gentry, Randall W.; Sayler, Gary S.] Univ Tennessee, Ctr Environm Biotechnol, Knoxville, TN 37996 USA. RP Koirala, SR (reprint author), Univ Tennessee, Inst Secure & Sustainable Environm, Knoxville, TN 37996 USA. EM skoirala@utk.edu RI Mulholland, Patrick/C-3142-2012; Gentry, Randall/J-8177-2012 OI Gentry, Randall/0000-0003-2477-8127 FU Center for Environmental Biotechnology; Inst. for a Secure and Sustainable Environment at the Univ. of Tennessee; US Department of Energy [DE-AC05-00OR22725]; Office of Science, Office of Biological and Environmental Research FX Funding for this research was also provided by the Center for Environmental Biotechnology and the Inst. for a Secure and Sustainable Environment at the Univ. of Tennessee. Data were collected as part of the long-term Walker Branch Watershed project at Oak Ridge National Laboratory and supported by the US Department of Energy's Program for Ecosystem Research, in the Office of Science, Office of Biological and Environmental Research. Oak Ridge National Laboratory is managed by University of Tennessee-Battelle LLC for the US Department of Energy under contract DE-AC05-00OR22725. NR 30 TC 2 Z9 2 U1 2 U2 18 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-1694 J9 J HYDROL JI J. Hydrol. PD MAY 3 PY 2011 VL 401 IS 3-4 BP 221 EP 230 DI 10.1016/j.jhydrol.2011.02.022 PG 10 WC Engineering, Civil; Geosciences, Multidisciplinary; Water Resources SC Engineering; Geology; Water Resources GA 758SR UT WOS:000290187300007 ER PT J AU Canton, SE Plesiat, E Bozek, JD Rude, BS Decleva, P Martin, F AF Canton, Sophie E. Plesiat, Etienne Bozek, John D. Rude, Bruce S. Decleva, Piero Martin, Fernando TI Direct observation of Young's double-slit interferences in vibrationally resolved photoionization of diatomic molecules SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE photoelectron spectroscopy; molecular spectroscopy; molecular ionization; density functional theory; quantum chemistry ID 2-CENTER INTERFERENCE; H-2; N-2; LOCALIZATION; DISSOCIATION; DIFFRACTION; SYMMETRY AB Vibrationally resolved valence-shell photoionization spectra of H(2), N(2) and CO have been measured in the photon energy range 20-300 eV using third-generation synchrotron radiation. Young's double-slit interferences lead to oscillations in the corresponding vibrational ratios, showing that the molecules behave as two-center electron-wave emitters and that the associated interferences leave their trace in the angle-integrated photoionization cross section. In contrast to previous work, the oscillations are directly observable in the experiment, thereby removing any possible ambiguity related to the introduction of external parameters or fitting functions. A straightforward extension of an original idea proposed by Cohen and Fano [Cohen HD, Fano U (1966) Phys Rev 150: 30] confirms this interpretation and shows that it is also valid for diatomic heteronuclear molecules. Results of accurate theoretical calculations are in excellent agreement with the experimental findings. C1 [Plesiat, Etienne; Martin, Fernando] Univ Autonoma Madrid, Dept Quim, E-28049 Madrid, Spain. [Canton, Sophie E.] Lund Univ, Max Lab, S-22100 Lund, Sweden. [Bozek, John D.] SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA. [Rude, Bruce S.] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. [Decleva, Piero] Univ Trieste, Dipartimento Sci Chim, I-34127 Trieste, Italy. [Decleva, Piero] CNR, Ist Officina Mat, I-34127 Trieste, Italy. [Martin, Fernando] IMDEA Nanociencia, Madrid 28049, Spain. RP Martin, F (reprint author), Univ Autonoma Madrid, Dept Quim, Modulo 13, E-28049 Madrid, Spain. EM fernando.martin@uam.es RI Bozek, John/E-9260-2010; Martin, Fernando/C-3972-2014; Plesiat, Etienne/M-6248-2014; Canton, Sophie/A-8432-2016 OI Bozek, John/0000-0001-7486-7238; Martin, Fernando/0000-0002-7529-925X; FU Ministerio de Ciencia e Innovacion (Spain) [FIS2010-15127, ACI2008-0777, CSD2007-00010]; European Cooperation in Science and Technology Action [CM0702]; DOE [DE-AC02-05CH11231] FX We thank Mare Nostrum Barcelona Supercomputing Center, Cineca and Centro de Computacion Cientifica - Universidad Autonoma de Madrid for allocation of computer time. Work partially supported by the Ministerio de Ciencia e Innovacion (Spain) project Nos. FIS2010-15127, ACI2008-0777 and CSD2007-00010, and the European Cooperation in Science and Technology Action CM0702. The ALS is supported by the DOE contract No. DE-AC02-05CH11231. NR 47 TC 57 Z9 57 U1 3 U2 32 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 3 PY 2011 VL 108 IS 18 BP 7302 EP 7306 DI 10.1073/pnas.1018534108 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 758YF UT WOS:000290203100012 ER PT J AU Ding, F Lu, CR Zhao, W Rajashankar, KR Anderson, DL Jardine, PJ Grimes, S Ke, AL AF Ding, Fang Lu, Changrui Zhao, Wei Rajashankar, Kanagalaghatta R. Anderson, Dwight L. Jardine, Paul J. Grimes, Shelley Ke, Ailong TI Structure and assembly of the essential RNA ring component of a viral DNA packaging motor SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE bacteriophage phi29; oligomeric RNA; molecular motor; gp16 ID BACTERIAL-VIRUS PHI29; PROHEAD RNA; BACTERIOPHAGE PHI-29; CRYSTAL-STRUCTURE; HEXAMERIC RNA; PRNA; ATPASE; MICROSCOPY; MACHINERY; MECHANISM AB Prohead RNA (pRNA) is an essential component in the assembly and operation of the powerful bacteriophage phi 29 DNA packaging motor. The pRNA forms a multimeric ring via intermolecular base-pairing interactions between protomers that serves to guide the assembly of the ring ATPase that drives DNA packaging. Here we report the quaternary structure of this rare multimeric RNA at 3.5 angstrom resolution, crystallized as tetrameric rings. Strong quaternary interactions and the inherent flexibility helped rationalize how free pRNA is able to adopt multiple oligomerization states in solution. These characteristics also allowed excellent fitting of the crystallographic pRNA protomers into previous prohead/pRNA cryo-EM reconstructions, supporting the presence of a pentameric, but not hexameric, pRNA ring in the context of the DNA packaging motor. The pentameric pRNA ring anchors itself directly to the phage prohead by interacting specifically with the fivefold symmetric capsid structures that surround the head-tail connector portal. From these contacts, five RNA superhelices project from the pRNA ring, where they serve as scaffolds for binding and assembly of the ring ATPase, and possibly mediate communication between motor components. Construction of structure-based designer pRNAs with little sequence similarity to the wild-type pRNA were shown to fully support the packaging of phi 29 DNA. C1 [Ding, Fang; Lu, Changrui; Ke, Ailong] Cornell Univ, Dept Mol Biol & Genet, Ithaca, NY 14853 USA. [Zhao, Wei; Anderson, Dwight L.; Jardine, Paul J.; Grimes, Shelley] Univ Minnesota, Dept Diagnost & Biol Sci, Minneapolis, MN 55455 USA. [Zhao, Wei; Anderson, Dwight L.; Jardine, Paul J.; Grimes, Shelley] Univ Minnesota, Inst Mol Virol, Minneapolis, MN 55455 USA. [Rajashankar, Kanagalaghatta R.] Argonne Natl Lab, NE Collaborat Access Team, Adv Photon Source, Argonne, IL 60439 USA. [Anderson, Dwight L.] Univ Minnesota, Dept Microbiol, Minneapolis, MN 55455 USA. RP Ke, AL (reprint author), Cornell Univ, Dept Mol Biol & Genet, Ithaca, NY 14853 USA. EM ak425@cornell.edu OI Lu, Changrui/0000-0002-2171-9888; Jardine, Paul/0000-0002-1090-0550 FU National Institutes of Health [GM-059604, DE-003606]; Ke lab [GM-059604, GM-086766] FX We thank the beam line staff at Advanced Photon Source ID24 and Macromolecular Diffraction at Cornell High Energy Synchrotron Source for assistance in data collection, Marc Morais for sharing EM maps, Kevin Weeks for sharing SHAPE reagents, and Rockney Atz and Marc Morais for helpful discussions and comments on the manuscript. Work in the Grimes lab was supported in part by Public Health Service Grants GM-059604 and DE-003606 from the National Institutes of Health, and the Ke lab by GM-059604 and GM-086766. NR 37 TC 31 Z9 31 U1 2 U2 9 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 3 PY 2011 VL 108 IS 18 BP 7357 EP 7362 DI 10.1073/pnas.1016690108 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 758YF UT WOS:000290203100022 PM 21471452 ER PT J AU Park, YS Malko, AV Vela, J Chen, Y Ghosh, Y Garcia-Santamaria, F Hollingsworth, JA Klimov, VI Htoon, H AF Park, Y. -S. Malko, A. V. Vela, J. Chen, Y. Ghosh, Y. Garcia-Santamaria, F. Hollingsworth, J. A. Klimov, V. I. Htoon, H. TI Near-Unity Quantum Yields of Biexciton Emission from CdSe/CdS Nanocrystals Measured Using Single-Particle Spectroscopy SO PHYSICAL REVIEW LETTERS LA English DT Article ID SEMICONDUCTOR NANOCRYSTALS; DOTS; BLINKING; PHOTOLUMINESCENCE; RECOMBINATION; SUPPRESSION; DYNAMICS AB Biexciton photoluminescence (PL) quantum yields (Q(2X)) of individual CdSe/CdS core-shell nanocrystal quantum dots with various shell thicknesses are derived from independent PL saturation and two-photon correlation measurements. We observe a near-unity Q(2X) for some nanocrystals with an ultrathick 19-monolayer shell. High Q(2X)'s are, however, not universal and vary widely among nominally identical nanocrystals indicating a significant dependence of Q(2X) upon subtle structural differences. Interestingly, our measurements indicate that high Q(2X)'s are not required to achieve complete suppression of PL intensity fluctuations in individual nanocrystals. C1 [Park, Y. -S.; Vela, J.; Chen, Y.; Ghosh, Y.; Garcia-Santamaria, F.; Hollingsworth, J. A.; Klimov, V. I.; Htoon, H.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Park, Y. -S.; Vela, J.; Chen, Y.; Ghosh, Y.; Hollingsworth, J. A.; Htoon, H.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Klimov, V. I.] Los Alamos Natl Lab, Ctr Adv Solar Photophys, Los Alamos, NM 87545 USA. [Malko, A. V.] Univ Texas Dallas, Dept Phys, Richardson, TX 75080 USA. RP Klimov, VI (reprint author), Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. EM klimov@lanl.gov; htoon@lanl.gov RI Park, Young-Shin/E-7181-2012; Vela, Javier/I-4724-2014; OI Vela, Javier/0000-0001-5124-6893; Park, Young-Shin/0000-0003-4204-1305; Klimov, Victor/0000-0003-1158-3179; Htoon, Han/0000-0003-3696-2896 FU CINT; Los Alamos National Laboratory; UT Dallas; Center for Advanced Solar Photophysics, an Energy Frontier Research Center of the OBES, Office of Science (OS), U.S. DOE; Chemical Sciences, Biosciences and Geosciences Division of OBES, U.S. DOE; Investigator Small Group, OBES, OS, U.S. DOE [2009LANL1096] FX This work was conducted, in part, at the Center for Integrated Nanotechnologies (CINT), a U. S. Department of Energy (DOE), Office of Basic Energy Sciences (OBES) user facility. We acknowledge D. Werder for performing transmission electron microscopy studies. Y. P. is supported by CINT. Y. G., J. V., Y. C. acknowledge Los Alamos National Laboratory Directed Research and Development Funds. Work of A. V. M was supported by UT Dallas start-up funds. V. I. K. is supported by the Center for Advanced Solar Photophysics, an Energy Frontier Research Center of the OBES, Office of Science (OS), U.S. DOE. F. G. is supported by the Chemical Sciences, Biosciences and Geosciences Division of OBES, U.S. DOE. H. H. and J. A. H. acknowledge a Single Investigator Small Group Research Grant (2009LANL1096), OBES, OS, U.S. DOE. NR 26 TC 105 Z9 105 U1 2 U2 72 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 3 PY 2011 VL 106 IS 18 AR 187401 DI 10.1103/PhysRevLett.106.187401 PG 4 WC Physics, Multidisciplinary SC Physics GA 758JI UT WOS:000290160200012 PM 21635124 ER PT J AU Sikorski, M Sandy, AR Narayanan, S AF Sikorski, M. Sandy, A. R. Narayanan, S. TI Depletion-Induced Structure and Dynamics in Bimodal Colloidal Suspensions SO PHYSICAL REVIEW LETTERS LA English DT Article ID PHASE-SEPARATION; SCATTERING DATA; MODEL; MIXTURES AB Combined small angle x-ray scattering and x-ray photon correlation spectroscopy studies of moderately concentrated bimodal hard-sphere colloidal suspensions in the fluid phase show that depletion-induced demixing introduces spatially heterogeneous dynamics with two distinct time scales. The adhesive nature, as well as the mobility, of the large particles is determined by the level of interaction within the monomodal domains. This interaction is driven by osmotic forces, which are governed by the relative concentration of the constituents. C1 [Sikorski, M.; Sandy, A. R.; Narayanan, S.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Narayanan, S (reprint author), Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Argonne, IL 60439 USA. EM sureshn@aps.anl.gov FU U.S. DOE, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We acknowledge S.-H. Lee and R. Ziegler for technical assistance. This work and the use of the APS are supported by the U.S. DOE, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 19 TC 14 Z9 14 U1 1 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 3 PY 2011 VL 106 IS 18 AR 188301 DI 10.1103/PhysRevLett.106.188301 PG 4 WC Physics, Multidisciplinary SC Physics GA 758JI UT WOS:000290160200014 PM 21635129 ER PT J AU Kim, J Holinga, GJ Somorjai, GA AF Kim, Joonyeong Holinga, George J. Somorjai, Gabor A. TI Curing Induced Structural Reorganization and Enhanced Reactivity of Amino-Terminated Organic Thin Films on Solid Substrates: Observations of Two Types of Chemically and Structurally Unique Amino Groups on the Surface SO LANGMUIR LA English DT Article ID SUM-FREQUENCY GENERATION; INTERFACIAL WATER-STRUCTURE; GAMMA-AMINOPROPYLTRIETHOXYSILANE; VIBRATIONAL SPECTROSCOPY; FLUORESCENCE MICROSCOPY; INFRARED-SPECTROSCOPY; SILICA SURFACES; COUPLING AGENTS; GLASS SURFACES; SILANE AB Infrared-visible sum frequency generation vibrational spectroscopy (SFG) was used to characterize the structure of 3-amino-propyltriethoxysilane (APTES) films deposited on solid substrates under controlled experimental conditions for the first time. Our SFG spectra in combination With complementary analytical data showed that APTES films undergo structural changes when cured at an elevated temperature. Before the films are cured, well-ordered hydrophobic ethoxy groups are dominantly present on the surface. A majority of hydrophilic surface amino groups are protonated, and they are either buried or randomly oriented at the interface. After the films are cured, chemically and structurally different neutral amino groups are detected on the surface. Unlike the protonated amino groups, a new class of neutral amino groups is ordered at the interface and shows enhanced reactivity. C1 [Kim, Joonyeong] SUNY Coll Buffalo, Dept Chem, Buffalo, NY 14222 USA. [Holinga, George J.; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Holinga, George J.; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Kim, J (reprint author), SUNY Coll Buffalo, Dept Chem, 1300 Elmwood Ave, Buffalo, NY 14222 USA. EM kimj@buffalostate.edu FU SUNY Research Foundation; Department of Chemistry, Buffalo State, SUNY; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by startup funds from the SUNY Research Foundation and Department of Chemistry, Buffalo State, SUNY, and the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. NR 44 TC 17 Z9 18 U1 6 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAY 3 PY 2011 VL 27 IS 9 BP 5171 EP 5175 DI 10.1021/la2007205 PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 753CN UT WOS:000289742500002 PM 21476532 ER PT J AU Kwon, KY Wang, E Nofal, M Lee, SW AF Kwon, Ki-Young Wang, Eddie Nofal, Michel Lee, Seung-Wuk TI Microscopic Study of Hydroxyapatite Dissolution As Affected by Fluoride Ions SO LANGMUIR LA English DT Article ID ATOMIC-FORCE MICROSCOPY; DENTAL-CARIES; SELECTIVE BINDING; CALCITE GROWTH; IN-SITU; ENAMEL; SURFACE; TOOTH; FLUOROSIS; CRYSTALS AB Fluoride ions play a critical role in preventing tooth decay. We investigated the microscopic effects of fluoride ions on hydroxyapatite (100) surface dissolution using in situ atomic force microscopy. In the presence of 10 mM NaF, individual surface step retraction velocities decreased by about a factor of 5 as compared to NaF-free conditions. Importantly, elongated hexagonal etch pits, which are characteristic of (100) surface dissolution, were no longer observed when NaF was present. The alteration of pit shape is more distinct at a higher NO concentration (SO mM) where triangular etch pits evolved during dissolution. Furthermore, in a fluoride concentration typical for tap water (10 mu M), we observed roughening of individual step lines, resulting in the formation of scalloped morphologies. Morphological changes to individual steps across a wide range of fluoride concentrations suggest that the cariostatic capabilities of fluoride ions originate from their strong interactions with molecular steps. C1 [Kwon, Ki-Young; Wang, Eddie; Nofal, Michel; Lee, Seung-Wuk] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Kwon, Ki-Young; Wang, Eddie; Nofal, Michel; Lee, Seung-Wuk] Univ Calif Berkeley, Phys Biosci Div, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Kwon, Ki-Young] Gyeongsang Natl Univ, Dept Chem, Jinju 660701, South Korea. [Kwon, Ki-Young] Gyeongsang Natl Univ, RINS, Jinju 660701, South Korea. RP Lee, SW (reprint author), Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. EM leesw@berkeley.edu OI Wang, Eddie/0000-0002-9814-0102 FU National Science Foundation [DMR-0747713]; National Research Foundation of Korea [NRF-2010-0006157] FX This work was supported by the National Science Foundation Early Career Development Award (DMR-0747713). K.-Y.K. acknowledges support from the National Research Foundation of Korea (NRF-2010-0006157). NR 43 TC 7 Z9 7 U1 6 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAY 3 PY 2011 VL 27 IS 9 BP 5335 EP 5339 DI 10.1021/la200325d PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 753CN UT WOS:000289742500021 PM 21456602 ER PT J AU Goertz, MP Goyal, N Montano, GA Bunker, BC AF Goertz, Matthew P. Goyal, Nikita Montano, Gabriel A. Bunker, Bruce C. TI Lipid Bilayer Reorganization under Extreme pH Conditions SO LANGMUIR LA English DT Article ID FLUORESCENCE MICROSCOPY; MEMBRANES; PHOSPHOLIPIDS; HYDROLYSIS; LIPOSOMES; DIFFUSION AB Supported lipid bilayers containing phosphatidylcholine headgroups are observed to undergo reorganization from a 2D fluid, lipid bilayer assembly into an array of complex 3D structures upon exposure to extreme pH environments. These conditions induce a combination of molecular packing and electrostatic interactions that can create dynamic morphologies of highly curved lipid membrane structures. This work demonstrates that fluid, single-component lipid bilayer assemblies can create complex morphologies, a phenomenon typically only associated with lipid bilayers of mixed composition. C1 [Goertz, Matthew P.; Bunker, Bruce C.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Goyal, Nikita; Montano, Gabriel A.] Los Alamos Natl Labs, Los Alamos, NM 87545 USA. RP Goertz, MP (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. EM mgoertz@sandia.gov FU U.S. Department of Energy [DE-AC04-94AL85000, DE-AC52-06NA25396] FX This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corp., a Lockheed-Martin Co., for the U.S. Department of Energy under Contract No. DE-AC04-94AL85000. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. NR 29 TC 9 Z9 9 U1 0 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAY 3 PY 2011 VL 27 IS 9 BP 5481 EP 5491 DI 10.1021/la2001305 PG 11 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 753CN UT WOS:000289742500039 PM 21462990 ER PT J AU Bouree, JE Mahan, AH AF Bouree, Jean-Eric Mahan, A. Harv TI Sixth international conference on hot-wire CVD (Cat-CVD) process Preface SO THIN SOLID FILMS LA English DT Editorial Material C1 [Bouree, Jean-Eric] Ecole Polytech, Lab Phys Interfaces & Couches Minces, F-91128 Palaiseau, France. [Mahan, A. Harv] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Bouree, JE (reprint author), Ecole Polytech, Lab Phys Interfaces & Couches Minces, F-91128 Palaiseau, France. EM jean-eric.bouree@polytechnique.edu; harv.mahan@nrel.gov NR 0 TC 1 Z9 1 U1 0 U2 3 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0040-6090 J9 THIN SOLID FILMS JI Thin Solid Films PD MAY 2 PY 2011 VL 519 IS 14 SI SI BP 4409 EP 4411 DI 10.1016/j.tsf.2011.01.002 PG 3 WC Materials Science, Multidisciplinary; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA 792DE UT WOS:000292719900001 ER PT J AU Mahan, AH Parilla, PA Moutinho, H To, B Dabney, MS Ginley, DS AF Mahan, A. Harv Parilla, Phil A. Moutinho, Helio To, Bobby Dabney, Matthew S. Ginley, David S. TI An alternative method to determine the steady state nucleation rate in thermally annealed HWCVD a-Si:H films SO THIN SOLID FILMS LA English DT Article; Proceedings Paper CT 6th International Conference on Hot-Wire CVD (CAT-CVD) Process CY SEP 13-17, 2010 CL Palaiseau, FRANCE SP Ecole Polytech ParisTech, CNRS-INSIS, Forschungszentrum Julich, Fraunhofer IST, GVD Corp, Gifu Univ, Ctr Innovat Photovolt Systems, ULVAC Inc, Mat Design Factory Co Ltd, Top Macoat Co Ltd, Universal Systems Co Ltd DE Amorphous silicon; Thermal annealing; Crystallization; Nucleation rate ID CHEMICAL-VAPOR-DEPOSITION; AMORPHOUS-SILICON; GRAIN NUCLEATION; CRYSTALLIZATION; RECRYSTALLIZATION; TEMPERATURE AB A determination of the steady state nucleation rate r(n) in thermally annealed a-Si:H has typically been performed using TEM, where the increase in grain density with isothermal sample anneal time can be directly observed for samples with small crystalline volume fractions. Using the classical model of crystallite nucleation and grain growth, this paper presents an alternative technique for determining rn using in situ XRD measurements of the crystallization time and EBSD measurements of the final grain size, the latter in fully annealed samples. HWCVD a-Si:H samples containing different as-grown film H contents C(H) have been examined by both techniques, and the agreement between these techniques is excellent. R(n) is seen to decrease with increasing as-grown film C(H). Differences in the values of r(n) are suggested as being due to variations in the transition rate per atom at the amorphous/crystalline interface. Published by Elsevier B.V. C1 [Mahan, A. Harv; Parilla, Phil A.; Moutinho, Helio; To, Bobby; Dabney, Matthew S.; Ginley, David S.] Natl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA. RP Mahan, AH (reprint author), Natl Renewable Energy Lab, Natl Ctr Photovolta, 1617 Cole Blvd, Golden, CO 80401 USA. EM harv.mahan@nrel.gov NR 12 TC 5 Z9 5 U1 0 U2 2 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0040-6090 J9 THIN SOLID FILMS JI Thin Solid Films PD MAY 2 PY 2011 VL 519 IS 14 SI SI BP 4455 EP 4458 DI 10.1016/j.tsf.2011.01.332 PG 4 WC Materials Science, Multidisciplinary; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA 792DE UT WOS:000292719900013 ER PT J AU Dillon, AC Riley, LA Jung, YS Ban, C Molina, D Mahan, AH Cavanagh, AS George, SM Lee, SH AF Dillon, A. C. Riley, L. A. Jung, Y. S. Ban, C. Molina, D. Mahan, A. H. Cavanagh, A. S. George, S. M. Lee, S-H TI HWCVD MoO3 nanoparticles and a-Si for next generation Li-ion anodes SO THIN SOLID FILMS LA English DT Article; Proceedings Paper CT 6th International Conference on Hot-Wire CVD (CAT-CVD) Process CY SEP 13-17, 2010 CL Palaiseau, FRANCE SP Ecole Polytech ParisTech, CNRS-INSIS, Forschungszentrum Julich, Fraunhofer IST, GVD Corp, Gifu Univ, Ctr Innovat Photovolt Systems, ULVAC Inc, Mat Design Factory Co Ltd, Top Macoat Co Ltd, Universal Systems Co Ltd DE Li-ion batteries; MoO3 nanoparticles; Amorphous silicon; Atomic layer deposition ID ATOMIC LAYER DEPOSITION; AMORPHOUS HYDROGENATED SILICON; OXIDE NANOPARTICLES; CARBON NANOTUBES; HIGH-CAPACITY; BATTERIES; ELECTRODES; NANOWIRES AB We have employed hot wire chemical vapor deposition (HWCVD) for the generation of MoO3 nanostructures at high density. Furthermore, the morphology of the nanoparticles is easily tailored by altering the HWCVD synthesis conditions. The MoO3 nanoparticles have been demonstrated as high-capacity Li-ion battery anodes for next-generation electric vehicles. Specifically, the MoO3 anodes have been shown to have approximately three times the Li-ion capacity of commercially employed graphite anodes in thick electrodes suitable for vehicular applications. However because the materials are high volume expansion materials (>= 100%), conformal Al2O3 coatings deposited with atomic layer deposition (ALD) were required before high rate capability was demonstrated. Recently, NREL is exploring high capacity Si anode materials that have a volume expansion of similar to 400%. It is assumed that new ALD coatings will need to be developed in order to stabilize Si as an anode material. Silicon is a superior choice for an anode material to the metal oxide structures due to both a higher capacity and a significantly lower hysteresis in the voltage vs. Li/Li+ for the charge/discharge profiles. (C) 2011 Published by Elsevier B.V. C1 [Dillon, A. C.; Riley, L. A.; Jung, Y. S.; Ban, C.; Molina, D.; Mahan, A. H.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Riley, L. A.; Molina, D.; Cavanagh, A. S.; George, S. M.; Lee, S-H] Univ Colorado, Boulder, CO 80309 USA. RP Dillon, AC (reprint author), Natl Renewable Energy Lab, 1617 Cole Blvd, Golden, CO 80401 USA. EM anne.dillon@nrel.gov RI Lee, Sehee/A-5989-2011; George, Steven/O-2163-2013; Jung, Yoon Seok/B-8512-2011 OI George, Steven/0000-0003-0253-9184; Jung, Yoon Seok/0000-0003-0357-9508 NR 20 TC 15 Z9 15 U1 6 U2 31 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0040-6090 J9 THIN SOLID FILMS JI Thin Solid Films PD MAY 2 PY 2011 VL 519 IS 14 SI SI BP 4495 EP 4497 DI 10.1016/j.tsf.2011.01.337 PG 3 WC Materials Science, Multidisciplinary; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA 792DE UT WOS:000292719900024 ER PT J AU Page, MR Iwaniczko, E Xu, YQ Roybal, L Hasoon, F Wang, Q Crandall, RS AF Page, M. R. Iwaniczko, E. Xu, Y. -Q. Roybal, L. Hasoon, F. Wang, Q. Crandall, R. S. TI Amorphous/crystalline silicon heterojunction solar cells with varying i-layer thickness SO THIN SOLID FILMS LA English DT Article; Proceedings Paper CT 6th International Conference on Hot-Wire CVD (CAT-CVD) Process CY SEP 13-17, 2010 CL Palaiseau, FRANCE SP Ecole Polytech ParisTech, CNRS-INSIS, Forschungszentrum Julich, Fraunhofer IST, GVD Corp, Gifu Univ, Ctr Innovat Photovolt Systems, ULVAC Inc, Mat Design Factory Co Ltd, Top Macoat Co Ltd, Universal Systems Co Ltd DE Catalytic CVD; Solar cell; Amorphous silicon; Heterojunction; Hot-wire deposition; Transient capacitance AB We study the effect on various properties of varying the intrinsic layer (i-layer) thickness of amorphous/ crystalline silicon heterojunction (SHJ) solar cells. Double-side monocrystalline silicon (c-Si) heterojunction solar cells are made using hot-wire chemical vapor deposition on high-lifetime n-type Czochralski wafers. We fabricate a series of SHJ solar cells with the amorphous silicon (a-Si:H) i-layer thickness at the front emitter varying from 3.2 nm (0.8xi) to similar to 96 nm (24xi). Our optimized i-layer thickness is about 4 nm (1xi). Our reference cell (1xi) performance has an efficiency of 17.1% with open-circuit voltage (V(oc)) of 684 mV, fill factor (FF) of 76%, and short-circuit current density (J(sc)) of 33.1 mA/cm(2). With an increase of i-layer thickness, V(oc) changes little, whereas the FF falls significantly after 12 nm (3xi) of i-layer. Transient capacitance measurements are used to probe the effect of the potential barrier at the n-type c-Si/a-Si interface on minority-carrier collection. We show that hole transport through the i-layer is field-driven transport rather than tunneling. (C) 2011 Published by Elsevier B.V. C1 [Page, M. R.; Iwaniczko, E.; Xu, Y. -Q.; Roybal, L.; Hasoon, F.; Wang, Q.; Crandall, R. S.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Page, MR (reprint author), Natl Renewable Energy Lab, 1617 Cole Blvd, Golden, CO 80401 USA. EM Matthew.Page@nrel.gov; Eugene.Iwaniczko@nrel.gov; Yueqin.Xu@nrel.gov; Lorenzo.Roybal@nrel.gov; Falah.Hasoon@nrel.gov; Qi.Wang@nrel.gov; Richard.Crandall@nrel.gov NR 5 TC 23 Z9 24 U1 0 U2 37 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0040-6090 J9 THIN SOLID FILMS JI Thin Solid Films PD MAY 2 PY 2011 VL 519 IS 14 SI SI BP 4527 EP 4530 DI 10.1016/j.tsf.2011.01.293 PG 4 WC Materials Science, Multidisciplinary; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA 792DE UT WOS:000292719900032 ER PT J AU Branz, HM Teplin, CW Romero, MJ Martin, IT Wang, Q Alberi, K Young, DL Stradins, P AF Branz, Howard M. Teplin, Charles W. Romero, Manuel J. Martin, Ina T. Wang, Qi Alberi, Kirstin Young, David L. Stradins, Paul TI Hot-wire chemical vapor deposition of epitaxial film crystal silicon for photovoltaics SO THIN SOLID FILMS LA English DT Article; Proceedings Paper CT 6th International Conference on Hot-Wire CVD (CAT-CVD) Process CY SEP 13-17, 2010 CL Palaiseau, FRANCE SP Ecole Polytech ParisTech, CNRS-INSIS, Forschungszentrum Julich, Fraunhofer IST, GVD Corp, Gifu Univ, Ctr Innovat Photovolt Systems, ULVAC Inc, Mat Design Factory Co Ltd, Top Macoat Co Ltd, Universal Systems Co Ltd DE Solar cells; Epitaxy; Film crystal silicon; Silicon; Hot-wire deposition; Modeling; Photovoltaics; Dislocations ID ALUMINUM-INDUCED CRYSTALLIZATION; HYDROGENATED AMORPHOUS-SILICON; LOW-TEMPERATURE; SOLAR-CELLS; BEAM EVAPORATION; SEED LAYERS; THIN-FILMS; SI FILMS; GLASS; GROWTH AB We have demonstrated that hot-wire chemical vapor deposition (HWCVD) is an excellent technique to produce high-quality epitaxial silicon at high rates, at substrate temperatures from 620 to 800 degrees C. Fast, scalable, inexpensive epitaxy of high-quality crystalline Si (c-Si) in this temperature range is a key element in creating cost-competitive film Si PV devices on crystalline seed layers on inexpensive substrates such as display glass and metal foil. We have improved both the quality and rate of our HWCVD Si epitaxy in this display-glass-compatible T range. We understand factors critical to high-quality epitaxial growth and obtain dislocation densities down to 6 x 10(4) cm(-2) by techniques that reduce the surface oxygen contamination at the moment growth is initiated. We have also developed and validated a model of the HWCVD silicon growth rate, based on fundamentals of reaction chemistry and ideal gas physics. This model enables us to predict growth rates and calculate the sticking coefficient of the Si radicals contributing to film formation between 300 and 800 degrees C. We obtain efficiencies up to 6.7% with a 2.5-micron absorber layer grown on heavily-doped 'dead' Si wafers although these cells still lack hydrogenation and light trapping. Open-circuit voltages up to 0.57 V are obtained on 2-mu m cells. Efficient film crystal silicon photovoltaics will require dislocation spacing more than 6 times the cell thickness, or else effective H passivation of the dislocations. (C) 2011 Elsevier B.V. All rights reserved. C1 [Branz, Howard M.; Teplin, Charles W.; Romero, Manuel J.; Martin, Ina T.; Wang, Qi; Alberi, Kirstin; Young, David L.; Stradins, Paul] Natl Renewable Energy Lab, Silicon Mat & Devices Grp, Golden, CO 80401 USA. RP Branz, HM (reprint author), Natl Renewable Energy Lab, Silicon Mat & Devices Grp, 1617 Cole Blvd, Golden, CO 80401 USA. EM howard.branz@nrel.gov RI Martin, Ina/J-9484-2012 NR 57 TC 31 Z9 31 U1 1 U2 33 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0040-6090 J9 THIN SOLID FILMS JI Thin Solid Films PD MAY 2 PY 2011 VL 519 IS 14 SI SI BP 4545 EP 4550 DI 10.1016/j.tsf.2011.01.335 PG 6 WC Materials Science, Multidisciplinary; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA 792DE UT WOS:000292719900037 ER PT J AU Martin, IT Teplin, CW Stradins, P Landry, M Shub, M Reedy, RC To, B Portugal, JV Mariner, JT AF Martin, Ina T. Teplin, Charles W. Stradins, Paul Landry, Marc Shub, Maxim Reedy, Robert C. To, Bobby Portugal, James V. Mariner, John T. TI High rate hot-wire chemical vapor deposition of silicon thin films using a stable TaC covered graphite filament SO THIN SOLID FILMS LA English DT Article; Proceedings Paper CT 6th International Conference on Hot-Wire CVD (CAT-CVD) Process CY SEP 13-17, 2010 CL Palaiseau, FRANCE SP Ecole Polytech ParisTech, CNRS-INSIS, Forschungszentrum Julich, Fraunhofer IST, GVD Corp, Gifu Univ, Ctr Innovat Photovolt Systems, ULVAC Inc, Mat Design Factory Co Ltd, Top Macoat Co Ltd, Universal Systems Co Ltd DE Hot-wire chemical vapor deposition; TaC; Filament; Silicidation ID TANTALUM FILAMENTS; CAT-CVD; TUNGSTEN; DIAMOND; SILICIDATION AB We grow silicon films by hot-wire/catalytic chemical vapor deposition using a new filament material: TaC-coated graphite rods. The filaments are 1.6 mm diameter rigid graphite rods with similar to 30 mu m thick TaC coatings. Whereas heated W or Ta wire filaments are reactive and embrittle in silane (SiH(4)), the TaC/graphite filament is stable. After >2 h of exposure to SiH(4) gas at a range of filament temperatures, the full length of a TaC/graphite filament retains its shiny golden color with no indication of swelling or degradation. In comparison, a W wire exposed to Sift, under the same conditions becomes swollen and discolored at the cold ends, indicating suicide formation. Scanning electron microscopy images of the filament material are nearly identical before and after SiH4 exposure at 1500-2000 degrees C. This temperature-independent chemical stability could enable added control of the gas phase chemistry during deposition that does not compromise the filament lifetime. The larger surface area of the 1.6 mm diameter TaC coated graphite filament (compared to the 0.5 mm W filament) allows for a similar to 2x increase in the deposition rate of Si thin films grown for photovoltaic applications. (C) 2011 Elsevier B.V. All rights reserved. C1 [Portugal, James V.; Mariner, John T.] Moment Performance Mat, Strongsville, OH 44149 USA. [Martin, Ina T.; Teplin, Charles W.; Stradins, Paul; Landry, Marc; Shub, Maxim; Reedy, Robert C.; To, Bobby] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Mariner, JT (reprint author), Moment Performance Mat, 22557 W Lunn Rd, Strongsville, OH 44149 USA. EM John.Mariner@Momentive.com RI Martin, Ina/J-9484-2012 NR 16 TC 5 Z9 5 U1 0 U2 10 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0040-6090 J9 THIN SOLID FILMS JI Thin Solid Films PD MAY 2 PY 2011 VL 519 IS 14 SI SI BP 4585 EP 4588 DI 10.1016/j.tsf.2011.01.322 PG 4 WC Materials Science, Multidisciplinary; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA 792DE UT WOS:000292719900047 ER PT J AU Biswas, K Du, MH AF Biswas, Koushik Du, Mao-Hua TI AX centers in II-VI semiconductors: Hybrid functional calculations SO APPLIED PHYSICS LETTERS LA English DT Article ID MOLECULAR-BEAM EPITAXY; AUGMENTED-WAVE METHOD; P-TYPE ZNSE; DOPING LIMITS; IMPURITY; FILMS AB Hybrid functional calculations predict significantly enhanced stability of AX centers against shallow acceptors in selected II-VI semiconductors (ZnO, ZnS, and ZnSe), as compared to the calculations based on local density approximation and generalized gradient approximation. The results agree well with the experimental observations on the p-type doping of ZnS and ZnSe. The improved description of the AX centers by hybrid functional calculations is due to the correction of the valence band maximum of the semiconductor. (C) 2011 American Institute of Physics. [doi:10.1063/1.3583661] C1 [Biswas, Koushik; Du, Mao-Hua] Oak Ridge Natl Lab, Ctr Radiat Detect Mat & Syst, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Biswas, K (reprint author), Oak Ridge Natl Lab, Ctr Radiat Detect Mat & Syst, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RI Du, Mao-Hua/B-2108-2010 OI Du, Mao-Hua/0000-0001-8796-167X FU U.S. DOE Office of Nonproliferation Research and Development [NA22] FX This work was supported by the U.S. DOE Office of Nonproliferation Research and Development NA22. NR 25 TC 16 Z9 16 U1 1 U2 14 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 2 PY 2011 VL 98 IS 18 AR 181913 DI 10.1063/1.3583661 PG 3 WC Physics, Applied SC Physics GA 761IU UT WOS:000290392300025 ER PT J AU Liu, XH Zhong, L Zhang, LQ Kushima, A Mao, SX Li, J Ye, ZZ Sullivan, JP Huang, JY AF Liu, Xiao Hua Zhong, Li Zhang, Li Qiang Kushima, Akihiro Mao, Scott X. Li, Ju Ye, Zhi Zhen Sullivan, John P. Huang, Jian Yu TI Lithium fiber growth on the anode in a nanowire lithium ion battery during charging SO APPLIED PHYSICS LETTERS LA English DT Article ID CELLS; ELECTRODE; DENSITY; STORAGE; METAL AB Lithium (Li) dendrite formation has been recognized as one of the major safety concerns for Li metal batteries but not for conventional Li ion batteries (LIBs) where Li metal is not used. With the advanced in situ transmission electron microscopy enabling direct observation of battery operation, we found that Li fibers with length up to 35 mu m grew on nanowire tip after charging. The Li fibers growth were highly directional, i.e., nucleating from the nanowire tip, and extending along the nanowire axis, which was attributed to the strong electric field enhancement effect induced by the sharp nanowire tip. This study reveals a potential safety concern of short-circuit failure for LIBs using nanowire anodes. (C) 2011 American Institute of Physics. [doi:10.1063/1.3585655] C1 [Liu, Xiao Hua; Sullivan, John P.; Huang, Jian Yu] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Zhong, Li; Zhang, Li Qiang; Mao, Scott X.] Univ Pittsburgh, Dept Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA. [Kushima, Akihiro; Li, Ju] Univ Penn, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [Zhang, Li Qiang; Ye, Zhi Zhen] Zhejiang Univ, Dept Mat Sci & Engn, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R China. RP Liu, XH (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. EM jhuang@sandia.gov RI Liu, Xiaohua/A-8752-2011; Huang, Jianyu/C-5183-2008; Li, Ju/A-2993-2008; Zhong, Li/I-3714-2014; Zhang, Liqiang/E-6539-2015; Kushima, Akihiro/H-2347-2011 OI Liu, Xiaohua/0000-0002-7300-7145; Li, Ju/0000-0002-7841-8058; Zhang, Liqiang/0000-0001-7482-0739; FU Laboratory Directed Research and Development (LDRD) at Sandia National Laboratories (SNL); Science of Precision Multifunctional Nanostructures for Electrical Energy Storage (NEES); U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DESC0001160]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; NSF through University of Pittsburgh [CMMI 08 010934]; Sandia National Laboratory; NSF [DMR-0520020, DMR-1008104]; AFOSR [FA9550-08-1-0325] FX Portions of this work was supported by a Laboratory Directed Research and Development (LDRD) project at Sandia National Laboratories (SNL) and partly by the Science of Precision Multifunctional Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center (EFRC) funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DESC0001160. The LDRD supported the development and fabrication of platforms. The NEES center supported the development of TEM techniques, and some of the additional platform development, and fabrication and materials characterization. CINT supported the TEM capability and the fabrication capabilities that were used for the TEM characterization; in addition, this work represents the efforts of several CINT users, primarily those with affiliation external to Sandia National Laboratories. This work was performed, in part, at the Sandia-Los Alamos Center for Integrated Nanotechnologies (CINT), a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Co., for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. S. M. would like to acknowledge NSF under Grant No. CMMI 08 010934 through University of Pittsburgh and Sandia National Laboratory support. J.L. and A. K. acknowledge support by NSF under Grant Nos. DMR-0520020 and DMR-1008104, and AFOSR under Grant No. FA9550-08-1-0325. NR 18 TC 33 Z9 34 U1 9 U2 76 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 2 PY 2011 VL 98 IS 18 AR 183107 DI 10.1063/1.3585655 PG 3 WC Physics, Applied SC Physics GA 761IU UT WOS:000290392300051 ER PT J AU Walter, AL Jeon, KJ Bostwick, A Speck, F Ostler, M Seyller, T Moreschini, L Kim, YS Chang, YJ Horn, K Rotenberg, E AF Walter, Andrew L. Jeon, Ki-Joon Bostwick, Aaron Speck, Florian Ostler, Markus Seyller, Thomas Moreschini, Luca Kim, Yong Su Chang, Young Jun Horn, Karsten Rotenberg, Eli TI Highly p-doped epitaxial graphene obtained by fluorine intercalation SO APPLIED PHYSICS LETTERS LA English DT Article ID SIC(0001); LAYERS AB We present a method for decoupling epitaxial graphene grown on SiC(0001) by intercalation of a layer of fluorine at the interface. The fluorine atoms do not enter into a covalent bond with graphene but rather saturate the substrate Si bonds. This configuration of the fluorine atoms induces a remarkably large hole density of p approximate to 4.5 x 10(13) cm(-2), equivalent to the location of the Fermi level at 0.79 eV above the Dirac point E-D. (C) 2011 American Institute of Physics. [doi:10.1063/1.3586256] C1 [Walter, Andrew L.; Bostwick, Aaron; Moreschini, Luca; Kim, Yong Su; Chang, Young Jun; Rotenberg, Eli] EO Lawrence Berkeley Natl Lab, ALS, Berkeley, CA 94720 USA. [Walter, Andrew L.; Chang, Young Jun; Horn, Karsten] Max Planck Gesell, Fritz Haber Inst, Dept Mol Phys, D-14195 Berlin, Germany. [Jeon, Ki-Joon] Univ Ulsan, Sch Elect Engn, Ulsan 680749, South Korea. [Speck, Florian; Ostler, Markus; Seyller, Thomas] Univ Erlangen Nurnberg, Lehrstuhl Tech Phys, D-91058 Erlangen, Germany. [Kim, Yong Su] Hanyang Univ, Dept Appl Phys, Ansan 426791, Gyeonggi Do, South Korea. RP Walter, AL (reprint author), EO Lawrence Berkeley Natl Lab, ALS, Berkeley, CA 94720 USA. EM al5walter@yahoo.com RI Seyller, Thomas/F-8410-2011; Walter, Andrew/B-9235-2011; Bostwick, Aaron/E-8549-2010; Rotenberg, Eli/B-3700-2009; Chang, Young Jun/N-3440-2014 OI Seyller, Thomas/0000-0002-4953-2142; Rotenberg, Eli/0000-0002-3979-8844; Chang, Young Jun/0000-0001-5538-0643 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; ESF; DFG FX The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Work in Erlangen was supported by the ESF and the DFG through the EUROCORES program EU-ROGRAPHENE. NR 26 TC 73 Z9 76 U1 4 U2 80 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 2 PY 2011 VL 98 IS 18 AR 184102 DI 10.1063/1.3586256 PG 3 WC Physics, Applied SC Physics GA 761IU UT WOS:000290392300075 ER PT J AU Parker, D Mazin, II AF Parker, David Mazin, I. I. TI Non-nesting spin-density-wave antiferromagnetism in FeAs from first principles SO PHYSICAL REVIEW B LA English DT Article AB The antiferromagnetic (AFM) state of FeAs is very different from that of the FeAs-based superconductor parent compounds, and it is rather complicated, with the Fe spins forming an incommensurate magnetic spiral pattern with a wavelength of about 15 A. To model this, we perform first-principles calculations and find the nearest-neighbor AFM ordering to be energetically favorable, with the lowest-energy pattern reproducing the experimentally found nearest-neighbor correlations. Other AFM orderings are also very stable, although higher in energy. Unlike in the superconductor parent compounds, the Fermi-surface geometry thus plays a small role. We calculate the bare Lindhard susceptibility in the AFM state and find that the observed spin-density-wave ordering vector Q similar or equal to (0,0,0.4) is not that given by this calculation. This is again unlike the superconductor parent compounds, which generally show a magnetic pattern matching the Lindhard susceptibility maximum. Thus in FeAs, the observed pattern must be due to a subtler mechanism. C1 [Parker, David] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Mazin, I. I.] USN, Res Lab, Washington, DC 20375 USA. RP Parker, D (reprint author), Oak Ridge Natl Lab, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. FU Office of Naval Research; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering FX This work was supported by the Office of Naval Research (I.I.M.) and by (D.P.) the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering. NR 13 TC 6 Z9 6 U1 2 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 2 PY 2011 VL 83 IS 18 AR 180403 DI 10.1103/PhysRevB.83.180403 PG 4 WC Physics, Condensed Matter SC Physics GA 757WR UT WOS:000290119700003 ER PT J AU Wan, XG Turner, AM Vishwanath, A Savrasov, SY AF Wan, Xiangang Turner, Ari M. Vishwanath, Ashvin Savrasov, Sergey Y. TI Topological semimetal and Fermi-arc surface states in the electronic structure of pyrochlore iridates SO PHYSICAL REVIEW B LA English DT Article ID QUANTUM SPIN HALL; FRUSTRATED MAGNETS; PHYSICS; INSULATORS; TRANSITION; LIQUIDS; LATTICE; OXIDES; PHASE AB We investigate novel phases that emerge from the interplay of electron correlations and strong spin-orbit interactions. We focus on describing the topological semimetal, a three-dimensional phase of a magnetic solid, and argue that it may be realized in a class of pyrochlore iridates (such as Y(2)Ir(2)O(7)) based on calculations using the LDA + U method. This state is a three-dimensional analog of graphene with linearly dispersing excitations and provides a condensed-matter realization of Weyl fermions that obeys a two-component Dirac equation. It also exhibits remarkable topological properties manifested by surface states in the form of Fermi arcs, which are impossible to realize in purely two-dimensional band structures. For intermediate correlation strengths, we find this to be the ground state of the pyrochlore iridates, coexisting with noncollinear magnetic order. A narrow window of magnetic "axion" insulator may also be present. An applied magnetic field is found to induce a metallic ground state. C1 [Wan, Xiangang; Savrasov, Sergey Y.] Nanjing Univ, Natl Lab Solid State Microstruct, Nanjing 210093, Peoples R China. [Wan, Xiangang; Savrasov, Sergey Y.] Nanjing Univ, Dept Phys, Nanjing 210093, Peoples R China. [Turner, Ari M.; Vishwanath, Ashvin] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Vishwanath, Ashvin] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Savrasov, Sergey Y.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. RP Wan, XG (reprint author), Nanjing Univ, Natl Lab Solid State Microstruct, Nanjing 210093, Peoples R China. RI Savrasov, Sergey/M-7157-2015 FU National Key Project for Basic Research of China [2011CB922101, 2010CB923404]; NSFC [10774067, 10974082]; DOE [SE-FC02-06ER25793]; Kavli Institute for Theoretical Physics; US Department of Energy [DE-AC02-05CH11231]; National Science Foundation [NSF-DMR 0645691] FX A.V. thanks L. Balents, J. Orenstein, and R. Ramesh for insightful discussions. X.W. acknowledges support by National Key Project for Basic Research of China (Grants No. 2011CB922101 and No. 2010CB923404) and NSFC under Grants No. 10774067 and No. 10974082. S.S. acknowledges support by DOE SciDAC Grant No. SE-FC02-06ER25793 and thanks Nanjing University for the kind hospitality during his visit to China. X.W. and S.S also acknowledge support from Kavli Institute for Theoretical Physics where this work was initiated. We also acknowledge support by the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under US Department of Energy Contract No. DE-AC02-05CH11231 (A.M.T.) as well as support by the National Science Foundation under grant NSF-DMR 0645691 (A.V.). NR 41 TC 1001 Z9 1013 U1 78 U2 367 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 2 PY 2011 VL 83 IS 20 AR 205101 DI 10.1103/PhysRevB.83.205101 PG 9 WC Physics, Condensed Matter SC Physics GA 757WY UT WOS:000290120500002 ER PT J AU Xiang, HJ Kan, EJ Whangbo, MH Lee, C Wei, SH Gong, XG AF Xiang, H. J. Kan, E. J. Whangbo, M. -H. Lee, C. Wei, Su-Huai Gong, X. G. TI Single-ion anisotropy, Dzyaloshinskii-Moriya interaction, and negative magnetoresistance the spin-1/2 pyrochlore R2V2O7 SO PHYSICAL REVIEW B LA English DT Article ID LU2V2O7 AB The electronic and magnetic properties of spin-1/2 pyrochlores R2V2O7 were investigated on the basis of density-functional calculations. Contrary to common belief, the spin-1/2 V4+ ions are found to have a substantial easy-axis single-ion anisotropy. We show that the magnon quantum Hall effect of Lu2V2O7 is a combined consequence of the easy-axis single-ion anisotropy and the Dzyaloshinskii-Moriya interaction of the spin-1/2 V4+ ions. We also show that the negative magnetoresistance observed for R2V2O7 arises from a different mechanism, i.e., the band gap decreases as the spin alignment becomes more parallel to each other. C1 [Xiang, H. J.; Gong, X. G.] Fudan Univ, Minist Educ, Key Lab Computat Phys Sci, Shanghai 200433, Peoples R China. [Xiang, H. J.; Gong, X. G.] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. [Kan, E. J.; Whangbo, M. -H.; Lee, C.] N Carolina State Univ, Dept Chem, Raleigh, NC 27695 USA. [Wei, Su-Huai] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Xiang, HJ (reprint author), Fudan Univ, Minist Educ, Key Lab Computat Phys Sci, Shanghai 200433, Peoples R China. RI Xiang, Hongjun/I-4305-2016; Kan, Erjun/A-4322-2009; gong, xingao/D-6532-2011 OI Xiang, Hongjun/0000-0002-9396-3214; Kan, Erjun/0000-0003-0433-4190; FU NSFC; Pujiang plan; Program for Professor of Special Appointment (Eastern Scholar); US DOE [DE-AC36-08GO28308, DE-FG02-86ER45259] FX Work at Fudan was partially supported by NSFC, Pujiang plan, and Program for Professor of Special Appointment (Eastern Scholar). Work at NREL was supported by US DOE under Contract No. DE-AC36-08GO28308, and that at NCSU by US DOE under Grant No. DE-FG02-86ER45259. NR 21 TC 21 Z9 21 U1 3 U2 26 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 2 PY 2011 VL 83 IS 17 AR 174402 DI 10.1103/PhysRevB.83.174402 PG 5 WC Physics, Condensed Matter SC Physics GA 757VU UT WOS:000290117000004 ER PT J AU Zhu, LJ Zhu, JX AF Zhu, Lijun Zhu, Jian-Xin TI Coherence scale of coupled Anderson impurities SO PHYSICAL REVIEW B LA English DT Article ID 2-IMPURITY KONDO MODEL; CRITICAL-POINT; LATTICE; TRANSITION; SYSTEMS AB For two coupled Anderson impurities, two energy scales are present to characterize the evolution from the local moment state of the impurities to either the interimpurity singlet or the Kondo singlet ground state. The high-energy scale is found to deviate from the single-ion Kondo temperature and rather scales as the Ruderman-Kittel-Kasuya-Yosida interaction when it becomes dominant. We find that the scaling behavior and the associated physical properties of this scale are consistent with those of a coherence scale defined in heavy fermion systems. C1 [Zhu, Lijun] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. RP Zhu, LJ (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Zhu, Jianxin/0000-0001-7991-3918 FU National Nuclear Security Administration of the US DOE at LANL [DE-AC52-06NA25396]; US DOE Office of Science; LANL; NSF [PHY05-51164] FX We would like to thank Qimiao Si, Joe D. Thompson, and Chandra M. Varma for helpful discussions. One of us (L.Z.) is also grateful to Chandra M. Varma for collaboration on related research. This work was supported by the National Nuclear Security Administration of the US DOE at LANL under Contract No. DE-AC52-06NA25396, the US DOE Office of Science, the LDRD Program at LANL, and in part by the NSF under Grant No. PHY05-51164. We also acknowledge the hospitality of Kavli Institute for Theoretical Physics (UCSB). NR 23 TC 14 Z9 15 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 2 PY 2011 VL 83 IS 19 AR 195103 DI 10.1103/PhysRevB.83.195103 PG 10 WC Physics, Condensed Matter SC Physics GA 757WW UT WOS:000290120300005 ER PT J AU Kang, ZB Qiu, JW Vogelsang, W Yuan, F AF Kang, Zhong-Bo Qiu, Jian-Wei Vogelsang, Werner Yuan, Feng TI Observation concerning the process dependence of the Sivers functions SO PHYSICAL REVIEW D LA English DT Article ID TRANSVERSE-SPIN ASYMMETRIES; DEEP-INELASTIC SCATTERING; FINAL-STATE INTERACTIONS; POLARIZED PROTON-BEAM; DRELL-YAN PROCESSES; SINGLE-SPIN; HARD-SCATTERING; QUANTUM CHROMODYNAMICS; PARTON DISTRIBUTIONS; ANALYZING POWER AB The k(perpendicular to) moment of a quark's Sivers function is known to be related to the corresponding twist-three quark-gluon correlation function T-q,T-F(x, x). The two functions have been extracted from data for single-spin asymmetries in semi-inclusive deep-inelastic scattering and in single-inclusive hadron production in pp collisions, respectively. Performing a consistent comparison of the extracted functions, we find that they show a "sign mismatch": while the magnitude of the functions is roughly consistent, the k(perpendicular to) moment of the Sivers function has opposite sign from that of T-q,T-F(x, x), both for up and for down quarks. Barring any inconsistencies in our theoretical understanding of the Sivers functions and their process dependence, the implication of this mismatch is that either the Sivers effect is not dominantly responsible for the observed single-spin asymmetries in pp collisions or the current semi-inclusive lepton scattering data do not sufficiently constrain the k(perpendicular to) moment of the quark Sivers functions. Both possibilities strengthen the case for further experimental investigations of single-spin asymmetries in high-energy pp and ep scattering. C1 [Kang, Zhong-Bo; Yuan, Feng] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Qiu, Jian-Wei] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Qiu, Jian-Wei] SUNY Stony Brook, CN Yang Inst Theoret Phys, Stony Brook, NY 11794 USA. [Qiu, Jian-Wei] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Vogelsang, Werner] Univ Tubingen, Inst Theoret Phys, D-72076 Tubingen, Germany. [Yuan, Feng] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Kang, ZB (reprint author), Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. EM zkang@bnl.gov; jqiu@bnl.gov; werner.vogelsang@uni-tuebingen.de; fyuan@lbl.gov RI Yuan, Feng/N-4175-2013; Kang, Zhongbo/P-3645-2014 FU U.S. Department of Energy [DE-FG02-87ER4037, DE-AC02-05CH11231, DE-AC02-98CH10886]; RIKEN, Brookhaven National Laboratory FX We thank H. Avakian, L. Gamberg, A. Metz, B. Musch, and A. Prokudin for discussions and comments. This work was supported in part by the U.S. Department of Energy under Grants No. DE-FG02-87ER4037 (J.Q.) and No. DE-AC02-05CH11231 (F.Y.). We are grateful to RIKEN, Brookhaven National Laboratory, and the U.S. Department of Energy (Contract No. DE-AC02-98CH10886) for supporting this work. NR 83 TC 82 Z9 82 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 J9 PHYS REV D JI Phys. Rev. D PD MAY 2 PY 2011 VL 83 IS 9 AR 094001 DI 10.1103/PhysRevD.83.094001 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 758KN UT WOS:000290163700001 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Fried, M Fruhwirth, R Ghete, VM Hammer, J Hansel, S Hoch, M Hormann, N Hrubec, J Jeitler, M Kasieczka, G Kiesenhofer, W Krammer, M Liko, D Mikulec, I Pernicka, M Rohringer, H Schofbeck, R Strauss, J Teischinger, F Wagner, P Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Benucci, L De Wolf, EA Janssen, X Maes, T Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Blekman, F Blyweert, S D'Hondt, J Devroede, O Suarez, RG Kalogeropoulos, A Maes, J Maes, M Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Charaf, O Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hammad, GH Hreus, T Marage, 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Hidas, D. Hits, D. Lath, A. Panwalkar, S. Patel, R. Richards, A. Rose, K. Schnetzer, S. Somalwar, S. Stone, R. Thomas, S. Cerizza, G. Hollingsworth, M. Spanier, S. Yang, Z. C. York, A. Asaadi, J. Eusebi, R. Gilmore, J. Gurrola, A. Kamon, T. Khotilovich, V. Montalvo, R. Nguyen, C. N. Osipenkov, I. Pivarski, J. Safonov, A. Sengupta, S. Tatarinov, A. Toback, D. Weinberger, M. Akchurin, N. Damgov, J. Jeong, C. Kovitanggoon, K. Lee, S. W. Roh, Y. Sill, A. Volobouev, I. Wigmans, R. Yazgan, E. Appelt, E. Brownson, E. Engh, D. Florez, C. Gabella, W. Lssah, M. Johns, W. Kurt, P. Maguire, C. Melo, A. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Balazs, M. Boutle, S. Cox, B. Francis, B. Hirosky, R. Ledovskoy, A. Lin, C. Neu, C. Yohay, R. Gollapinni, S. Harr, R. Karchin, P. E. Lamichhane, R. Mattson, M. Milstene, C. Sakharov, A. Anderson, M. Bachtis, M. Bellinger, J. N. Carlsmith, D. Dasu, S. Efron, J. Flood, K. Gray, L. Grogg, K. S. Grothe, M. Hall-Wilton, R. Herndon, M. Klabbers, P. Klukas, J. Lanaro, A. Lazaridis, C. Leonard, J. Loveless, R. Mohapatra, A. Reeder, D. Ross, I. Savin, A. Smith, W. H. Swanson, J. Weinberg, M. CA CMS Collaboration TI Measurement of W+W- production and search for the Higgs boson in pp collisions at root s=7 TeV SO PHYSICS LETTERS B LA English DT Article DE CMS; Physics; Software; Computing ID W-BOSON; COUPLINGS; LHC; LEP; TEVATRON; MASS AB A measurement of W+W- production in pp collisions at root s = 7 TeV and a search for the Higgs boson are reported. The W+W- candidates are selected in events with two leptons, either electrons or muons. The measurement is performed using LHC data recorded with the CMS detector, corresponding to an integrated luminosity of 36 pb(-1). The pp -> W+W- cross section is measured to be 41.1 +/- 15.3 (stat) +/- 5.8 (syst) +/- 4.5 (lumi) ph. consistent with the standard model prediction. Limits on WW gamma and WWZ anomalous triple gauge couplings are set. The search for the standard model Higgs boson in the W+W- decay mode does not reveal any evidence of excess above backgrounds. Limits are set on the production of the Higgs boson in the context of the standard model and in the presence of a sequential fourth family of fermions with high masses. In the latter context, a Higgs boson with mass between 144 and 207 GeV/c(2) is ruled out at 95% confidence level. (C) 2011 CERN. Published by Elsevier B.V. All rights reserved. C1 [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Fried, M.; Fruehwirth, R.; Ghete, V. M.; Hammer, J.; Haensel, S.; Hoch, M.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kasieczka, G.; Kiesenhofer, W.; Krammer, M.; Liko, D.; Mikulec, I.; Pernicka, M.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Teischinger, F.; Wagner, P.; Waltenberger, W.; Walzel, G.; Widl, E.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. 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[Braibant-Giacomelli, S.; Capiluppi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Navarria, El.; Rossi, A. M.; Rovelli, T.; Siroli, G.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Tricomi, A.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Lenzi, P.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Colafranceschi, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. 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T.; Nespolo, M.; Perrozzi, L.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bellan, P.; Bisello, D.; Carlin, R.; De Mattia, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Univ Padua, Padua, Italy. [Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Baesso, P.; Berzano, U.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.; Viviani, C.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Baesso, P.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.; Viviani, C.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Caponeri, B.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Santocchia, A.; Taroni, S.; Valdata, M.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Caponeri, B.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Taroni, S.; Valdata, M.] Univ Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Palmonari, F.; Segneri, G.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bernardini, J.; Fiori, F.; Messineo, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; D'Agnolo, R. T.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Di Marco, E.; Diemoz, M.; Franci, D.; Grassi, M.; Longo, E.; Nourbakhsh, S.; Organtini, G.; Pandolfi, F.; Paramatti, R.; Rahatlou, S.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Di Marco, E.; Franci, D.; Longo, E.; Organtini, G.; Pandolfi, F.; Rahatlou, S.] Univ Roma La Sapienza, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Botta, C.; Cartiglia, N.; Castello, R.; Costa, M.; Demaria, N.; Graziano, A.; Mariotti, C.; Marone, M.; Maselli, S.; Migliore, E.; Mila, G.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Romero, A.; Ruspa, M.; Sacchi, R.; Sola, V.; Solano, A.; Staiano, A.; Trocino, D.; Pereira, A. Vilela] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Romeo, F.; Amapane, N.; Argiro, S.; Botta, C.; Castello, R.; Costa, M.; Graziano, A.; Marone, M.; Migliore, E.; Mila, G.; Monaco, V.; Musich, M.; Pelliccioni, M.; Sacchi, R.; Sola, V.; Solano, A.; Trocino, D.; Pereira, A. Vilela] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Montanino, D.; Penzo, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Della Ricca, G.; Montanino, D.] Univ Trieste, Trieste, Italy. [Heo, S. G.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Chung, J.; Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Park, H.; Ro, S. R.; Son, D.; Son, D. C.; Son, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, Zero; Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Hong, B.; Jeong, M. S.; Jo, M.; Kim, H.; Kim, J. H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.; Rhee, H. B.; Seo, E.; Shin, S.; Sim, K. S.] Korea Univ, Seoul, South Korea. [Choi, M.; Kang, S.; Kim, H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Martisiute, D.; Petrov, P.; Sabonis, T.] Vilnius Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.; Tam, J.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. R.; Doesburg, R.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ahmed, I.; Asghar, M. I.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Cwiok, M.; Dorninik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Soltan Inst Nucl Studies, PL-00681 Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Musella, P.; Nayak, A.; Seixas, J.; Varela, J.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Belotelov, I.; Bunin, P.; Golutvin, I.; Kamenev, A.; Karjavin, V.; Kozlov, G.; Laney, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Toropin, A.; Troitsky, S.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Kaftanov, V.; Kossov, M.; Krokhotin, A.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Sarycheva, L.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Rusakov, S. V.; Vinogradov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Azhgirey, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Slabospitsky, S.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Arce, P.; Battilana, C.; Calvo, E.; Cepeda, M.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Diez Pardos, C.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Jorda, C.; Lobelle Pardo, P.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, Inst Fis Cantabria IFCA, CSIC, E-39005 Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Baillon, P.; Ball, A. H.; Barney, D.; Bell, A. J.; Benedetti, D.; Bernet, C.; Bialas, W.; Bloch, P.; Bocci, A.; Bolognesi, S.; Bona, M.; Breuker, H.; Brona, G.; Bunkowski, K.; Camporesi, T.; Cerminara, G.; Perez, J. A. Coarasa; Cure, B.; D'Enterria, D.; De Roeck, A.; Di Guida, S.; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Gaddi, A.; Gennai, S.; Georgiou, G.; Gerwig, H.; Gigi, D.; Gill, K.; Giordano, D.; Glege, E.; Garrido, R. Gomez-Reino; Gouzevitch, M.; Govoni, R.; Gowdy, S.; Guiducci, L.; Hansen, M.; Hard, C.; Harvey, J.; Hegeman, J.; Hegner, B.; Hoffmann, H. F.; Honma, A.; Innocente, V.; Janot, R.; Kaadze, K.; Karavakis, E.; Lecoq, P.; Lourenco, C.; Maeki, T.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Nesvold, E.; Nguyen, M.; Orimoto, T.; Orsini, L.; Perez, E.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Polese, G.; Racz, A.; Antunes, J. Rodrigues; Rolandi, G.; Rommerskirchen, T.; Rovelli, C.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Segoni, I.; Sharma, A.; Siegrist, P.; Simon, M.; Sphicas, P.; Spiropulu, M.; Stoeckli, F.; Stoye, M.; Tropea, P.; Tsirou, A.; Vichoudis, P.; Voutilainen, M.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Starodumov, A.] Paul Scherrer Inst, Villigen, Switzerland. [Bortignon, P.; Caminada, L.; Chen, Z.; Cittolin, S.; Dissertori, G.; Dittmar, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Herve, A.; Hintz, W.; Lecomte, P.; Lustermann, W.; Marchica, C.; del Arbol, P. Martinez Ruiz; Meridiani, P.; Milenovic, P.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pape, L.; Pauss, F.; Punz, T.; Rizzi, A.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Sawley, M. -C.; Stieger, B.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, M.; Wehrli, L.; Weng, J.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aguilo, E.; Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Otiougova, P.; Regenfus, C.; Robmann, P.; Schmidt, A.; Snoek, H.] Univ Zurich, Zurich, Switzerland. [Attikis, A.; Chang, Y. H.; Chen, K. H.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Volpe, R.; Wu, J. H.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Cukurova Univ, Adana, Turkey. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Topaksu, A. Kayis; Nart, A.; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Uzun, D.; Vergili, L. N.; Vergili, M.; Zorbilmez, C.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Akin, I. V.; Aliev, T.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Cuter, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yildirim, E.; Zeyrek, M.] Bogazici Univ, Istanbul, Turkey. [Deliomeroglu, M.; Demir, D.; Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Levchuk, L.] Univ Bristol, Bristol, Avon, England. [Bell, P.; Bostock, F.; Brooke, J. J.; Cheng, T. L.; Clement, E.; Cussans, D.; Frazier, R.; Goldstein, J.; Grimes, M.; Hansen, M.; Hartley, D.; Heath, G. P.; Heath, H. F.; Huckvale, B.; Jackson, J.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Ward, S.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Dzelalija, M.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Camanzi, B.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Univ London Imperial Coll Sci Technol & Med, London, England. [Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Camanzi, B.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Worm, S. D.; Buchmuller, O.; Gilbert, A.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.] Baylor Univ, Waco, TX 76798 USA. [Bose, T.; Jarrin, E. Carrera; Fantasia, C.; Heister, A.; St John, J.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Avetisyan, A.; Bhattacharya, S.; Chou, J. P.; Cutts, D.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Landsberg, G.; Narain, M.; Nguyen, D.; Segala, M.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Cox, P. T.; Dolen, J.; Erbacher, R.; Friis, E.; Kopecky, A.; Lander, R.; Liu, H.; Maruyama, S.; Miceli, T.; Nikolic, M.; Pellett, D.; Robles, J.; Salur, S.; Schwarz, T.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez; Veelken, C.] Univ Calif Davis, Davis, CA 95616 USA. [Babb, J.; Chandra, A.; Clare, R.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Kao, S. C.; Liu, F.; Liu, H.; Long, O. R.; Luthra, A.; Nguyen, H.; Shen, B. C.; Stringer, R.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Dusinberre, E.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pi, H.; Pieri, M.; Ranieri, R.; Sani, M.; Sharma, V.; Simon, S.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, R.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; Vlimant, J. R.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Gataullin, M.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Shin, K.; Timciuc, V.; Traczyk, P.; Veverka, J.; Wilkinson, R.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Akgun, B.; Carroll, R.; Ferguson, T.; Liyama, Y.; Jang, D. W.; Jun, S. Y.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Dinardo, M. E.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Gaz, A.; Heyburn, B.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.; Zang, S. L.] Univ Colorado, Boulder, CO 80309 USA. [Agostino, L.; Alexander, J.; Cassel, D.; Chatterjee, A.; Das, S.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Kaufman, G. Nicolas; Patterson, J. R.; Puigh, D.; Ryd, A.; Shi, X.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Biselli, A.; Cirino, G.; Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Atac, M.; Bakken, J. A.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Borcherding, F.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Cooper, W.; Eartly, D. P.; Elvira, V. D.; Esen, S.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Green, D.; Gunthoti, K.; Gutsche, O.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jensen, H.; Johnson, M.; Joshi, U.; Khatiwada, R.; Klima, B.; Kousouris, K.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Limon, P.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Mason, D.; McBride, P.; Miao, T.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Pordes, R.; Prokofyev, O.; Saoulidou, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Tan, P.; Taylor, L.; Tkaczyk, S.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. 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[Cole, R.; Cooper, S. I.; Cushman, P.; Dahmes, B.; De Benedetti, A.; Dudero, P. R.; Franzoni, G.; Haupt, J.; Klapoetke, K.; Kubota, Y.; Mans, J.; Rekovic, V.; Rusack, R.; Sasseville, M.; Singovsky, A.] Univ Minnesota, Minneapolis, MN USA. [Baden, A.; Cremaldi, L. M.; Godang, R.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, University, MS 38677 USA. [Bloom, K.; Bose, S.; Butt, J.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kelly, T.; Kravchenko, I.; Lazo-Flores, J.; Malbouisson, H.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Baur, U.; Godshalk, A.; Lashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Shipkowski, S. P.; Smith, K.; Alverson, G.] SUNY Buffalo, Buffalo, NY 14260 USA. [Barberis, E.; Baumgartel, D.; Boeriu, O.; Chasco, M.; Reucroft, S.; Swain, J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Kubik, A.; Odell, N.; Ofierzynski, R. 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[Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.; Yan, M.] Rockefeller Univ, New York, NY 10021 USA. [Barker, A.; Duggan, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hits, D.; Lath, A.; Panwalkar, S.; Patel, R.; Richards, A.; Rose, K.; Schnetzer, S.; Somalwar, S.; Stone, R.; Thomas, S.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Asaadi, J.; Eusebi, R.; Gilmore, J.; Gurrola, A.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Nguyen, C. N.; Osipenkov, I.; Pivarski, J.; Safonov, A.; Sengupta, S.; Tatarinov, A.; Toback, D.; Weinberger, M.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Damgov, J.; Jeong, C.; Kovitanggoon, K.; Lee, S. W.; Roh, Y.; Sill, A.; Volobouev, I.; Wigmans, R.; Yazgan, E.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Brownson, E.; Engh, D.; Florez, C.; Gabella, W.; Lssah, M.; Johns, W.; Kurt, P.; Maguire, C.; Melo, A.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN USA. [Arenton, M. W.; Balazs, M.; Boutle, S.; Cox, B.; Francis, B.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Yohay, R.] Univ Virginia, Charlottesville, VA USA. [Harr, R.; Karchin, P. E.; Lamichhane, R.; Mattson, M.; Milstene, C.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Anderson, M.; Bachtis, M.; Bellinger, J. N.; Carlsmith, D.; Dasu, S.; Efron, J.; Flood, K.; Gray, L.; Grogg, K. S.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Leonard, J.; Loveless, R.; Mohapatra, A.; Reeder, D.; Ross, I.; Savin, A.; Smith, W. H.; Swanson, J.; Weinberg, M.] Univ Wisconsin, Madison, WI 53706 USA. [Andreev, V.; Arisaka, K.; Cline, D.; Cousins, R.; Deisher, A.; Duris, J.; Erhan, S.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Tucker, J.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Palmonari, F.; Segneri, G.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. RP Tenchini, R (reprint author), Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. EM Roberto.Tenchini@cern.ch RI Tinoco Mendes, Andre David/D-4314-2011; Dudko, Lev/D-7127-2012; Mignerey, Alice/D-6623-2011; Ganjour, Serguei/D-8853-2011; Stahl, Achim/E-8846-2011; Hektor, Andi/G-1804-2011; lebert, thomas/H-4032-2011; Wulz, Claudia-Elisabeth/H-5657-2011; Chen, Jie/H-6210-2011; Bolton, Tim/A-7951-2012; Yang, Fan/B-2755-2012; Krammer, Manfred/A-6508-2010; Lokhtin, Igor/D-7004-2012; Kodolova, Olga/D-7158-2012; Varela, Joao/K-4829-2016; Menasce, Dario Livio/A-2168-2016; Bargassa, Pedrame/O-2417-2016; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Fassi, Farida/F-3571-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Gerbaudo, Davide/J-4536-2012; Flix, Josep/G-5414-2012; Ozdemir, Kadri/P-8058-2014; Azarkin, Maxim/N-2578-2015; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Haj Ahmad, Wael/E-6738-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Govoni, Pietro/K-9619-2016; Bedoya, Cristina/K-8066-2014; Matorras, Francisco/I-4983-2015; My, Salvatore/I-5160-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Arce, Pedro/L-1268-2014; Leonidov, Andrey/P-3197-2014; Russ, James/P-3092-2014; Dahms, Torsten/A-8453-2015; Grandi, Claudio/B-5654-2015; Ahmed, Ijaz/E-9144-2015; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; vilar, rocio/P-8480-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; Cerrada, Marcos/J-6934-2014; Calderon, Alicia/K-3658-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Marinho, Franciole/N-8101-2014; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Rolandi, Luigi (Gigi)/E-8563-2013; Zalewski, Piotr/H-7335-2013; Cavallo, Nicola/F-8913-2012; Ivanov, Andrew/A-7982-2013; Hill, Christopher/B-5371-2012; Troitsky, Sergey/C-1377-2014; Marlow, Daniel/C-9132-2014; Janssen, Xavier/E-1915-2013; Oguri, Vitor/B-5403-2013; Santoro, Alberto/E-7932-2014; Codispoti, Giuseppe/F-6574-2014; Gribushin, Andrei/J-4225-2012; de Jesus Damiao, Dilson/G-6218-2012; Montanari, Alessandro/J-2420-2012; Amapane, Nicola/J-3683-2012; tosi, mia/J-5777-2012; Petrushanko, Sergey/D-6880-2012; Raidal, Martti/F-4436-2012; Mercadante, Pedro/K-1918-2012; Della Ricca, Giuseppe/B-6826-2013; Kadastik, Mario/B-7559-2008; Mundim, Luiz/A-1291-2012; Santaolalla, Javier/C-3094-2013; Alves, Gilvan/C-4007-2013; Belyaev, Andrey/E-1540-2012; Katkov, Igor/E-2627-2012; Boos, Eduard/D-9748-2012; Snigirev, Alexander/D-8912-2012; Tomei, Thiago/E-7091-2012; Novaes, Sergio/D-3532-2012; Padula, Sandra /G-3560-2012; Fruhwirth, Rudolf/H-2529-2012; Azzi, Patrizia/H-5404-2012; Torassa, Ezio/I-1788-2012; Giacomelli, Paolo/B-8076-2009; Jeitler, Manfred/H-3106-2012; Venturi, Andrea/J-1877-2012 OI Tinoco Mendes, Andre David/0000-0001-5854-7699; Dudko, Lev/0000-0002-4462-3192; Stahl, Achim/0000-0002-8369-7506; Hektor, Andi/0000-0001-7873-8118; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Krammer, Manfred/0000-0003-2257-7751; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Varela, Joao/0000-0003-2613-3146; Heath, Helen/0000-0001-6576-9740; Menasce, Dario Livio/0000-0002-9918-1686; Bargassa, Pedrame/0000-0001-8612-3332; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Lloret Iglesias, Lara/0000-0002-0157-4765; Carrera, Edgar/0000-0002-0857-8507; Sguazzoni, Giacomo/0000-0002-0791-3350; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Fassi, Farida/0000-0002-6423-7213; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Gerbaudo, Davide/0000-0002-4463-0878; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Flix, Josep/0000-0003-2688-8047; Ozdemir, Kadri/0000-0002-0103-1488; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Haj Ahmad, Wael/0000-0003-1491-0446; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Govoni, Pietro/0000-0002-0227-1301; Bedoya, Cristina/0000-0001-8057-9152; Matorras, Francisco/0000-0003-4295-5668; My, Salvatore/0000-0002-9938-2680; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Arce, Pedro/0000-0003-3009-0484; Russ, James/0000-0001-9856-9155; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Cerrada, Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Marinho, Franciole/0000-0002-7327-0349; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Ivanov, Andrew/0000-0002-9270-5643; Hill, Christopher/0000-0003-0059-0779; Troitsky, Sergey/0000-0001-6917-6600; Codispoti, Giuseppe/0000-0003-0217-7021; de Jesus Damiao, Dilson/0000-0002-3769-1680; Montanari, Alessandro/0000-0003-2748-6373; Amapane, Nicola/0000-0001-9449-2509; Della Ricca, Giuseppe/0000-0003-2831-6982; Mundim, Luiz/0000-0001-9964-7805; Katkov, Igor/0000-0003-3064-0466; Tomei, Thiago/0000-0002-1809-5226; Novaes, Sergio/0000-0003-0471-8549; Azzi, Patrizia/0000-0002-3129-828X; FU FMSR (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN (China); CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences (Estonia); NICPB (Estonia); Academy of Finland (Finland); ME (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Korea); WCU (Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MST (Russia); MAE (Russia); MSTD (Serbia); MICINN (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK (Turkey); TAEK (Turkey); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme; European Research Council (European Union); Leventis Foundation; A.P. Sloan Foundation; Alexander von Humboldt Foundation; Associazione per lo Sviluppo Scientifico e Tecnologico del Piemonte (Italy); Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium) FX We wish to congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine. We thank the technical and administrative staff at CERN and other CMS institutes, and acknowledge support from: FMSR (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences and NICPB (Estonia); Academy of Finland, ME, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MST and MAE (Russia); MSTD (Serbia); MICINN and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK and TAEK (Turkey); STFC (United Kingdom); DOE and NSF (USA). Individuals have received support from the Marie-Curie programme and the European Research Council (European Union); the Leventis Foundation; the A.P. Sloan Foundation; the Alexander von Humboldt Foundation; the Associazione per lo Sviluppo Scientifico e Tecnologico del Piemonte (Italy); the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); and the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium). NR 52 TC 82 Z9 82 U1 2 U2 59 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAY 2 PY 2011 VL 699 IS 1-2 BP 25 EP 47 DI 10.1016/j.physletb.2011.03.056 PG 23 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 757CN UT WOS:000290061900006 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hammer, J Hansel, S Hartl, C Hoch, M Hormann, N Hrubec, J Jeitler, M Kasieczka, G Kiesenhofer, W Krammer, M Liko, D Mikulec, I Pernicka, M Rohringer, H Schofbeck, R Strauss, J Taurok, A Teischinger, F Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Benucci, L Cerny, K De Wolf, EA Janssen, X Maes, T Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Adler, V Beauceron, S Blekman, F Blyweert, S D'Hondt, J Devroede, O Suarez, RG Kalogeropoulos, A Maes, J Maes, M Tavernier, S Van Doninck, W Van Mulders, R Van Onsem, GP Villella, I Charaf, O 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Lazaridis, C. Leonard, J. Lomidze, D. Loveless, R. Mohapatra, A. Reeder, D. Ross, I. Savin, A. Smith, W. H. Swanson, J. Weinberg, M. CA CMS Collaboration TI First measurement of hadronic event shapes in pp collisions at root s=7 TeV SO PHYSICS LETTERS B LA English DT Article DE CMS; LHC; QCD; Event shapes ID TESTS AB Hadronic event shapes have been measured in proton-proton collisions at root s = 7 TeV, with a data sample collected with the CMS detector at the LHC. The sample corresponds to an integrated luminosity of 3.2 pb(-1). Event-shape distributions, corrected for detector response, are compared with five models of QCD multijet production. (C) 2011 CERN. Published by Elsevier B.V. All rights reserved. C1 [Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Foa, F.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Palmonari, F.; Sarkar, S.; Segneri, G.; Serban, A. 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[Braibant-Giacomelli, S.; Capiluppi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Meneghelli, M.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G.; Travaglini, R.; Rovelli, C.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Tricomi, A.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Genta, C.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Lenzi, P.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Colafranceschi, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. 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[Azzi, P.; Bacchetta, N.; Bellan, P.; Bellato, M.; Biasotto, M.; Branca, A.; Checchia, P.; Conti, E.; De Mattia, M.; Dorigo, T.; Fanzago, F.; Gasparini, F.; Giubilato, P.; Gresele, A.; Gulmini, M.; Kaminskiy, A.; Lacaprara, S.; Lazzizzer, I.; Margoni, M.; Mazzucato, M.; Meneguzzo, A. T.; Nespolo, M.; Perrozzi, L.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bellan, P.; De Mattia, M.; Gasparini, F.; Giubilato, P.; Kaminskiy, A.; Margoni, M.; Meneguzzo, A. T.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.] Univ Padua, Padua, Italy. [Gresele, A.; Lazzizzer, I.] Univ Trento Trento, Padua, Italy. [Berzano, U.; Riccardi, C.; Torre, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Riccardi, C.; Torre, P.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Caponeri, B.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Menichelli, M.; Nappi, A.; Santocchia, A.; Servoli, L.; Taroni, S.; Valdata, M.; Volpe, R.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Caponeri, B.; Fano, L.; Lariccia, P.; Lucaroni, A.; Nappi, A.; Santocchia, A.; Servoli, L.; Taroni, S.; Valdata, M.; Volpe, R.] Univ Perugia, I-06100 Perugia, Italy. [Bernardini, J.; Messineo, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; D'Agnolo, R. T.; Sarkar, S.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Di Marco, E.; Diemoz, M.; Franci, D.; Grassi, M.; Longo, E.; Organtini, G.; Palma, A.; Pandolfi, F.; Paramatti, R.; Rahatlou, S.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Di Marco, E.; Franci, D.; Longo, E.; Organtini, G.; Palma, A.; Pandolfi, F.; Rahatlou, S.] Univ Roma La Sapienza, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Botta, C.; Cartiglia, N.; Castello, R.; Costa, M.; Demaria, N.; Graziano, A.; Mariotti, C.; Marone, M.; Maselli, S.; Migliore, E.; Mila, G.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Romero, A.; Ruspa, M.; Sacchi, R.; Sola, V.; Solano, A.; Staiano, A.; Trocino, D.; Pereira, A. Vilela] Ist Nazl Fis Nucl, Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Botta, C.; Castello, R.; Costa, M.; Graziano, A.; Marone, M.; Migliore, E.; Mila, G.; Monaco, V.; Musich, M.; Pelliccioni, M.; Romero, A.; Sacchi, R.; Sola, V.; Solano, A.; Trocino, D.; Pereira, A. Vilela] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Ambroglini, F.; Belforte, S.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Montanino, D.; Penzo, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Riccardi, C.; Ambroglini, F.; Montanino, D.] Univ Trieste, Trieste, Italy. [Heo, S. G.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Chung, J.; Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, Dj.; Park, H.; Son, D.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, Zero; Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Hong, B.; Jo, M.; Kim, H.; Kim, J. H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.; Rhee, H. B.; Seo, E.; Shin, S.] Korea Univ, Seoul, South Korea. [Choi, M.; Kang, S.; Kim, H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Martisiute, D.; Petrov, P.; Sabonis, T.] Vilnius Univ, Vilnius, Lithuania. [Castilla Valdez, H.; De La Cruz Burelo, E.; Lopez-Fernandez, R.; Sanchez Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Allfrey, R.; Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ahmed, I.; Asghar, M. I.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Soltan Inst Nucl Studies, PL-00681 Warsaw, Poland. [Almeida, N.; David, A.; Faccioli, R.; Ferreira Parracho, P. G.; Gallinaro, M.; Martins, P.; Musella, P.; Nayak, A.; Ribeiro, P. Q.; Seixas, J.; Silva, P.; Varela, J.; Woehri, H. K.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Belotelov, I.; Bunin, P.; Finger, M.; Finger, M., Jr.; Golutvin, I.; Kamenev, A.; Karjavin, V.; Kozlov, G.; Laney, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Bondar, N.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Toropin, A.; Troitsky, S.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Kaftanov, V.; Kossov, M.; Krokhotin, A.; Lychkovskaya, N.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Sarycheva, L.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Azhgirey, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Slabospitsky, S.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Maestre, J. Alcaraz; Arce, P.; Battilana, C.; Calvo, E.; Cepeda, M.; Cerrada, M.; Colino, N.; De La Cruz, B.; Diez Pardos, C.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Redondo, I.; Romero, L.; Santaolalla, J.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chamizo Llatas, M.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Jorda, C.; Lobelle Pardo, P.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Ruiz Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, Inst Fis Cantabria IFSC, CSIC, E-39005 Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Baillon, P.; Ball, A. H.; Barney, D.; Bell, A. J.; Benedetti, D.; Bernet, C.; Bialas, W.; Bloch, P.; Bocci, A.; Bolognesi, S.; Breuker, H.; Brona, G.; Bunkowski, K.; Camporesi, T.; Cano, E.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Cure, B.; D'Enterria, D.; De Roeck, A.; Ramos, F. Duarte; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Gaddi, A.; Gennai, S.; Georgiou, G.; Gerwig, H.; Gigi, D.; Gill, K.; Giordano, D.; Glege, F.; Garrido, R. Gomez-Reino; Gouzevitch, M.; Govoni, P.; Gowdy, S.; Guiducci, L.; Hansen, M.; Harvey, J.; Hegeman, J.; Hegner, B.; Henderson, C.; Hesketh, G.; Hoffmann, H. F.; Honma, A.; Innocente, V.; Janot, P.; Karavakis, E.; Lecoq, P.; Leonidopoulos, C.; Lourenco, C.; Macpherson, A.; Maeki, T.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Nesvold, E.; Nguyen, M.; Orimoto, T.; Orsini, L.; Perez, E.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Polese, G.; Racz, A.; Rolandi, G.; Rommerskirchen, T.; Rovelli, C.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Segoni, I.; Sharma, A.; Siegrist, P.; Simon, M.; Sphicas, P.; Spiga, D.; Spiropulu, M.; Stoeckli, F.; Stoye, M.; Tropea, P.; Tsirou, A.; Tsyganov, A.; Veres, G. I.; Vichoudis, P.; Voutilainen, M.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Starodumov, A.] Paul Scherrer Inst, Villigen, Switzerland. [Bortignon, P.; Caminada, L.; Chen, Z.; Cittolin, S.; Dissertori, G.; Dittmar, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Herve, A.; Hintz, W.; Lecomte, P.; Lustermann, W.; Marchica, C.; del Arbol, P. Martinez Ruiz; Meridiani, P.; Milenovic, P.; Moortgat, F.; Nef, P.; Nessi-Tedaldi, F.; Pape, L.; Pauss, F.; Punz, T.; Rizzi, A.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Sawley, M. -C.; Stieger, B.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, M.; Wehrli, L.; Weng, J.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aguilo, E.; Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Milian; Regenfus, C.; Robmann, P.; Schmidt, A.; Snoek, H.; Wilke, L.; Adiguzel, A.; Belyaev, A.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Chen, W. T.; Dutta, S.; Go, A.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, M. H.; Liu, Z. K.; Lu, Y. J.; Wu, J. H.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Cuter, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Topaksu, A. Kayis; Nart, A.; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Tali, B.; Topakli, H.; Uzun, D.; Vergili, L. N.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Cuter, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Akin, I. V.; Aliev, T.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Cuter, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yildirim, E.; Zeyrek, M.] Bogazici Univ, Istanbul, Turkey. [Deliomeroglu, M.; Demir, D.; Gulmez, E.; Halu, A.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Levchuk, L.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Bell, P.; Bostock, E.; Brooke, J. J.; Cheng, T. L.; Clement, E.; Cussans, D.; Frazier, R.; Goldstein, J.; Grimes, M.; Hansen, M.; Hartley, D.; Heath, G. P.; Heath, H. F.; Huckvale, B.; Jackson, J.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Ward, S.] Univ Bristol, Bristol, Avon, England. [Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Camanzi, B.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Bailin, J.; Beuselinck, R.; Buchmuller, O.; Coiling, D.; Cripps, N.; Cutajar, M.; Davies, G.; Della Negra, M.; Fulcher, J.; Futyan, D.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Karapostoli, G.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rompotis, N.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Tourneur, S.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardrope, D.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Barrett, M.; Chadwick, M.; Cole, J. E.; Hobson, Rr.; Khan, A.; Kyberd, P.; Leslie, D.; Martin, W.; Reid, I. D.; Teodorescu, L.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.] Baylor Univ, Waco, TX 76798 USA. [Bose, T.; Jarrin, E. Carrera; Clough, A.; Fantasia, C.; Heister, A.; St John, J.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Avetisyan, A.; Bhattacharya, S.; Chou, J. P.; Cutts, D.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Landsberg, G.; Narain, M.; Nguyen, D.; Segala, M.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Borgia, M. A.; Breedon, R.; Sanchez, M. Calderon De La Barca; Cebra, D.; Chauhan, S.; Chertok, M.; Conway, J.; Cox, P. T.; Dolen, J.; Erbacher, R.; Friis, E.; Ko, W.; Kopecky, A.; Lander, R.; Liu, H.; Maruyama, S.; Miceli, T.; Nikolic, M.; Pellett, D.; Robles, J.; Salur, S.; Schwarz, T.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.] Univ Calif Davis, Davis, CA 95616 USA. [Sierra, R. Vasquez; Veelken, C.; Andreev, V.; Arisaka, K.; Cline, D.; Cousins, R.; Deisher, A.; Duris, J.; Erhan, S.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Tucker, J.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Giordano, E.; Hanson, G.; Jeng, G. Y.; Kao, S. C.; Liu, E.; Liu, H.; Luthra, A.; Nguyen, H.; Pasztor, G.; Satpathy, A.; Shen, B. C.; Stringer, R.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; C'erati, G. B.; Dusinberre, E.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Mangano, B.; Muelmenstaedt, J.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pi, H.; Pieri, M.; Ranieri, R.; Sani, M.; Sharma, V.; Simon, S.; Tu, Y.; Vartak, A.; Wuerthwein, F.; Yagil, A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; Vlimant, J. R.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Bornheim, A.; Bunn, J.; Chen, Y.; Gataullin, M.; Kcira, D.; Litvine, V.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Timciuc, V.; Traczyk, R.; Veverka, J.; Wilkinson, R.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Akgun, B.; Carroll, R.; Ferguson, T.; Liyama, Y.; Jang, D. W.; Jun, S. Y.; Liu, Y. F.; Paulini, M.; Russ, J.; Terentyev, N.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Dinardo, M. E.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Heyburn, B.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.; Zang, S. L.] Univ Colorado, Boulder, CO 80309 USA. [Agostino, L.; Alexander, J.; Chatterjee, A.; Eggert, N.; Fields, L. J.; Gibbons, L. K.; Heltsley, B.; Khukhunaishvili, A.; Kreis, B.; Kaufman, G. Nicolas; Patterson, J. R.; Puigh, D.; Riley, D.; Ryd, A.; Thom, J.; Thompson, J.; Vaughan, J.; Winstrom, L.] Cornell Univ, Ithaca, NY USA. [Biselli, A.; Cirino, G.; Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Atac, M.; Bakken, J. A.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Borcherding, F.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Demarteau, M.; Eartly, D. P.; Elvira, V. D.; Esen, S.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Green, D.; Gunthoti, K.; Gutsche, O.; Hahn, A.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; James, E.; Jensen, H.; Johnson, M.; Joshi, U.; Khatiwada, R.; Kilminster, B.; Klima, B.; Kousouris, K.; Kunori, S.; Kwan, S.; Limon, R.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Mason, D.; McBride, P.; McCauley, T.; Miao, T.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Popescu, S.; Pordes, R.; Prokofyev, O.; Saoulidou, N.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Tan, P.; Taylor, L.; Tkaczyk, S.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. 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EM Roberto.Tenchini@cern.ch RI de Jesus Damiao, Dilson/G-6218-2012; Montanari, Alessandro/J-2420-2012; Amapane, Nicola/J-3683-2012; tosi, mia/J-5777-2012; Petrushanko, Sergey/D-6880-2012; Raidal, Martti/F-4436-2012; Della Ricca, Giuseppe/B-6826-2013; Kadastik, Mario/B-7559-2008; Mundim, Luiz/A-1291-2012; Santaolalla, Javier/C-3094-2013; Alves, Gilvan/C-4007-2013; Rolandi, Luigi (Gigi)/E-8563-2013; Katkov, Igor/E-2627-2012; Boos, Eduard/D-9748-2012; Snigirev, Alexander/D-8912-2012; Servoli, Leonello/E-6766-2012; Tomei, Thiago/E-7091-2012; Novaes, Sergio/D-3532-2012; Padula, Sandra /G-3560-2012; Fruhwirth, Rudolf/H-2529-2012; Azzi, Patrizia/H-5404-2012; Torassa, Ezio/I-1788-2012; Giacomelli, Paolo/B-8076-2009; Jeitler, Manfred/H-3106-2012; Venturi, Andrea/J-1877-2012; Tinoco Mendes, Andre David/D-4314-2011; Mignerey, Alice/D-6623-2011; Ganjour, Serguei/D-8853-2011; Stahl, Achim/E-8846-2011; Hektor, Andi/G-1804-2011; Wulz, Claudia-Elisabeth/H-5657-2011; Chen, Jie/H-6210-2011; Bolton, Tim/A-7951-2012; Yang, Fan/B-2755-2012; buotempo, salvatore/B-5210-2012; Krammer, Manfred/A-6508-2010; Lokhtin, Igor/D-7004-2012; Kodolova, Olga/D-7158-2012; Dudko, Lev/D-7127-2012; Zalewski, Piotr/H-7335-2013; Ivanov, Andrew/A-7982-2013; Hill, Christopher/B-5371-2012; Troitsky, Sergey/C-1377-2014; Marlow, Daniel/C-9132-2014; Janssen, Xavier/E-1915-2013; Oguri, Vitor/B-5403-2013; Codispoti, Giuseppe/F-6574-2014; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Calderon, Alicia/K-3658-2014; de la Cruz, Begona/K-7552-2014; Varela, Joao/K-4829-2016; Ligabue, Franco/F-3432-2014; Fassi, Farida/F-3571-2016; Menasce, Dario Livio/A-2168-2016; Bargassa, Pedrame/O-2417-2016; Sguazzoni, Giacomo/J-4620-2015; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Gerbaudo, Davide/J-4536-2012; MERCIER, Damien/C-4151-2017; Lazzizzera, Ignazio/E-9678-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Flix, Josep/G-5414-2012; Ozdemir, Kadri/P-8058-2014; Azarkin, Maxim/N-2578-2015; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Haj Ahmad, Wael/E-6738-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; Bedoya, Cristina/K-8066-2014; Matorras, Francisco/I-4983-2015; My, Salvatore/I-5160-2015; Muelmenstaedt, Johannes/K-2432-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; Vogel, Helmut/N-8882-2014; Marinho, Franciole/N-8101-2014; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Russ, James/P-3092-2014; Ahmed, Ijaz/E-9144-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015 OI de Jesus Damiao, Dilson/0000-0002-3769-1680; Montanari, Alessandro/0000-0003-2748-6373; Amapane, Nicola/0000-0001-9449-2509; Della Ricca, Giuseppe/0000-0003-2831-6982; Mundim, Luiz/0000-0001-9964-7805; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Katkov, Igor/0000-0003-3064-0466; Servoli, Leonello/0000-0003-1725-9185; Tomei, Thiago/0000-0002-1809-5226; Novaes, Sergio/0000-0003-0471-8549; Azzi, Patrizia/0000-0002-3129-828X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Stahl, Achim/0000-0002-8369-7506; Hektor, Andi/0000-0001-7873-8118; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Krammer, Manfred/0000-0003-2257-7751; Dudko, Lev/0000-0002-4462-3192; Ivanov, Andrew/0000-0002-9270-5643; Hill, Christopher/0000-0003-0059-0779; Troitsky, Sergey/0000-0001-6917-6600; Codispoti, Giuseppe/0000-0003-0217-7021; Cerrada, Marcos/0000-0003-0112-1691; Sogut, Kenan/0000-0002-9682-2855; Varela, Joao/0000-0003-2613-3146; Faccioli, Pietro/0000-0003-1849-6692; Heath, Helen/0000-0001-6576-9740; Gallinaro, Michele/0000-0003-1261-2277; Tabarelli de Fatis, Tommaso/0000-0001-6262-4685; Lenzi, Piergiulio/0000-0002-6927-8807; Raval, Amita/0000-0003-0164-4337; Torassa, Ezio/0000-0003-2321-0599; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Fassi, Farida/0000-0002-6423-7213; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Bargassa, Pedrame/0000-0001-8612-3332; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; 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Bedoya, Cristina/0000-0001-8057-9152; Matorras, Francisco/0000-0003-4295-5668; My, Salvatore/0000-0002-9938-2680; Muelmenstaedt, Johannes/0000-0003-1105-6678; Rovelli, Tiziano/0000-0002-9746-4842; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Vogel, Helmut/0000-0002-6109-3023; Marinho, Franciole/0000-0002-7327-0349; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408 FU FMSR (Austria); FNRS; FWO (Belgium); CNPq; CAPES; CAPES, FAPERJ; FAPESP (Brazil); MES (Bulgaria); CERN; CAS; MoST; NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences and NICPB (Estonia); Academy of Finland; ME; HIP (Finland); CEA; CNRS/IN2P3 (France); BMBF; DFG; HGF (Germany); GSRT (Greece); OTKA; NKTH (Hungary); DAE; DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF; WCU (Korea); LAS (Lithuania); CINVESTAV; CONACYT; SEP; UASLPFAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MST; MAE (Russia); MSTD (Serbia); MICINN; CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK; TAEK (Turkey); STFC (United Kingdom); DOE; NSF (USA); Marie-Curie programme; European Research Council (European Union); Leventis Foundation; A.P. Sloan Foundation; Alexander von Humboldt Foundation; Associazione per lo Sviluppo Scientifico e Tecnologico del Piemonte (Italy); Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'industrie et dans l'Agriculture (FRIA - Belgium); Agentschap voor lnnovatie door Wetenschap en Technologie (IWT - Belgium) FX We wish to congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine. We thank the technical and administrative staff at CERN and other CMS institutes, and acknowledge support from: FMSR (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences and NICPB (Estonia); Academy of Finland, ME, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea): LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLPFAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MST and MAE (Russia); MSTD (Serbia); MICINN and CPAN (Spain): Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK and TAEK (Turkey); STFC (United Kingdom); DOE and NSF (USA). Individuals have received support from the Marie-Curie programme and the European Research Council (European Union); the Leventis Foundation; the A.P. Sloan Foundation; the Alexander von Humboldt Foundation; the Associazione per lo Sviluppo Scientifico e Tecnologico del Piemonte (Italy); the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'industrie et dans l'Agriculture (FRIA - Belgium); and the Agentschap voor lnnovatie door Wetenschap en Technologie (IWT - Belgium). NR 24 TC 41 Z9 41 U1 2 U2 38 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAY 2 PY 2011 VL 699 IS 1-2 BP 48 EP 67 DI 10.1016/j.physletb.2011.03.060 PG 20 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 757CN UT WOS:000290061900007 ER PT J AU Adamson, P Andreopoulos, C Armstrong, R Auty, DJ Ayres, DS Backhouse, C Barr, G Bishai, M Blake, A Bock, GJ Boehnlein, DJ Bogert, D Cavanaugh, S Cherdack, D Childress, S Choudhary, BC Coelho, JAB Coleman, SJ Corwin, L Cronin-Hennessy, D Danko, IZ de Jong, JK Devenish, NE Diwan, MV Dorman, M Escobar, CO Evans, JJ Falk, E Feldman, GJ Frohne, MV Gallagher, HR Gomes, RA Goodman, MC Gouffon, P Graf, N Gran, R Grant, N Grzelak, K Habig, A Harris, D Hartnell, J Hatcher, R Himmel, A Holin, A Huang, X Hylen, J Ilic, J Irwin, GM Isvan, Z Jaffe, DE James, C Jensen, D Kafka, T Kasahara, SMS Koizumi, G Kopp, S Kordosky, M Kreymer, A Lang, K Lefeuvre, G Ling, J Litchfield, PJ Litchfield, RP Loiacono, L Lucas, P Mann, WA Marshak, ML Mayer, N McGowan, AM Mehdiyev, R Meier, JR Messier, MD Michael, DG Miller, WH Mishra, SR Mitchell, J Moore, CD Moffin, J Mualem, L Mufson, S Musser, J Naples, D Nelson, JK Newman, HB Nichol, RJ Nowak, JA Oliver, WP Orchanian, M Ospanov, R Paley, J Patterson, RB Pawloski, G Pearce, GF Petyt, DA Phan-Budd, S Plunkett, RK Qiu, X Ratchford, J Raufer, TM Rebel, B Rodrigues, PA Rosenfeld, C Rubin, HA Sanchez, MC Schneps, J Schreiner, P Shanahan, P Smith, C Sousa, A Stamoulis, P Strait, M Tagg, N Talaga, RL Thomas, J Thomson, MA Tinti, G Toner, R Tzanakos, G Urheim, J Vahle, P Viren, B Weber, A Webb, RC White, C Whitehead, L Wojcicki, SG Yang, T Zwaska, R AF Adamson, P. Andreopoulos, C. Armstrong, R. Auty, D. J. Ayres, D. S. Backhouse, C. Barr, G. Bishai, M. Blake, A. Bock, G. J. Boehnlein, D. J. Bogert, D. Cavanaugh, S. Cherdack, D. Childress, S. Choudhary, B. C. Coelho, J. A. B. Coleman, S. J. Corwin, L. Cronin-Hennessy, D. Danko, I. Z. de Jong, J. K. Devenish, N. E. Diwan, M. V. Dorman, M. Escobar, C. O. Evans, J. J. Falk, E. Feldman, G. J. Frohne, M. V. Gallagher, H. R. Gomes, R. A. Goodman, M. C. Gouffon, P. Graf, N. Gran, R. Grant, N. Grzelak, K. Habig, A. Harris, D. Hartnell, J. Hatcher, R. Himmel, A. Holin, A. Huang, X. Hylen, J. Ilic, J. Irwin, G. M. Isvan, Z. Jaffe, D. E. James, C. Jensen, D. Kafka, T. Kasahara, S. M. S. Koizumi, G. Kopp, S. Kordosky, M. Kreymer, A. Lang, K. Lefeuvre, G. Ling, J. Litchfield, P. J. Litchfield, R. P. Loiacono, L. Lucas, P. Mann, W. A. Marshak, M. L. Mayer, N. McGowan, A. M. Mehdiyev, R. Meier, J. R. Messier, M. D. Michael, D. G. Miller, W. H. Mishra, S. R. Mitchell, J. Moore, C. D. Moffin, J. Mualem, L. Mufson, S. Musser, J. Naples, D. Nelson, J. K. Newman, H. B. Nichol, R. J. Nowak, J. A. Oliver, W. P. Orchanian, M. Ospanov, R. Paley, J. Patterson, R. B. Pawloski, G. Pearce, G. F. Petyt, D. A. Phan-Budd, S. Plunkett, R. K. Qiu, X. Ratchford, J. Raufer, T. M. Rebel, B. Rodrigues, P. A. Rosenfeld, C. Rubin, H. A. Sanchez, M. C. Schneps, J. Schreiner, P. Shanahan, P. Smith, C. Sousa, A. Stamoulis, P. Strait, M. Tagg, N. Talaga, R. L. Thomas, J. Thomson, M. A. Tinti, G. Toner, R. Tzanakos, G. Urheim, J. Vahle, P. Viren, B. Weber, A. Webb, R. C. White, C. Whitehead, L. Wojcicki, S. G. Yang, T. Zwaska, R. CA MINOS Collaboration TI Measurement of the Neutrino Mass Splitting and Flavor Mixing by MINOS SO PHYSICAL REVIEW LETTERS LA English DT Article ID LEPTON CHARGE AB Measurements of neutrino oscillations using the disappearance of muon neutrinos from the Fermilab NuMI neutrino beam as observed by the two MINOS detectors are reported. New analysis methods have been applied to an enlarged data sample from an exposure of 7.25 x 10(20) protons on target. A fit to neutrino oscillations yields values of vertical bar Delta m(2)vertical bar = (2.32(-0.08)(+0.12) x 10(-3) eV(2) for the atmospheric mass splitting and sin(2)(2 theta) > 0.90 (90% C.L.) for the mixing angle. Pure neutrino decay and quantum decoherence hypotheses are excluded at 7 and 9 standard deviations, respectively. C1 [Stamoulis, P.; Tzanakos, G.] Univ Athens, Dept Phys, GR-15771 Athens, Greece. [Bishai, M.; Diwan, M. V.; Jaffe, D. E.; Viren, B.; Whitehead, L.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Himmel, A.; Michael, D. G.; Mualem, L.; Newman, H. B.; Orchanian, M.; Patterson, R. B.] CALTECH, Lauritsen Lab, Pasadena, CA 91125 USA. [Blake, A.; Mitchell, J.; Thomson, M. A.; Toner, R.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Coelho, J. A. B.; Escobar, C. O.] Univ Estadual Campinas, IFGW UNICAMP, BR-13083970 Campinas, SP, Brazil. [Adamson, P.; Bock, G. J.; Boehnlein, D. J.; Bogert, D.; Childress, S.; Choudhary, B. C.; Harris, D.; Hatcher, R.; Hylen, J.; James, C.; Jensen, D.; Koizumi, G.; Kreymer, A.; Lucas, P.; Moore, C. D.; Moffin, J.; Plunkett, R. K.; Rebel, B.; Shanahan, P.; Zwaska, R.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Gomes, R. A.] Univ Fed Goias, Inst Fis, BR-74001970 Goiania, Go, Brazil. [Cavanaugh, S.; Feldman, G. J.; Sanchez, M. C.; Sousa, A.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Frohne, M. V.] Coll Holy Cross, Notre Dame, IN 46556 USA. [Graf, N.; Rubin, H. A.; White, C.] IIT, Div Phys, Chicago, IL 60616 USA. [Armstrong, R.; Corwin, L.; Mayer, N.; Messier, M. D.; Mufson, S.; Musser, J.; Paley, J.; Urheim, J.] Indiana Univ, Bloomington, IN 47405 USA. [Sanchez, M. C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Dorman, M.; Evans, J. J.; Holin, A.; Nichol, R. J.; Smith, C.; Thomas, J.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Cronin-Hennessy, D.; Kasahara, S. M. S.; Litchfield, P. J.; Marshak, M. L.; Meier, J. R.; Miller, W. H.; Nowak, J. A.; Petyt, D. A.; Strait, M.] Univ Minnesota, Minneapolis, MN 55455 USA. [Gran, R.; Habig, A.] Univ Minnesota, Dept Phys, Duluth, MN 55812 USA. [Tagg, N.] Otterbein Coll, Westerville, OH 43081 USA. [Backhouse, C.; Barr, G.; de Jong, J. K.; Litchfield, R. P.; Rodrigues, P. A.; Tinti, G.; Weber, A.] Univ Oxford, Subdept Particle Phys, Oxford OX1 3RH, England. [Danko, I. Z.; Isvan, Z.; Naples, D.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Andreopoulos, C.; Grant, N.; Hartnell, J.; Ilic, J.; Litchfield, P. J.; Pearce, G. F.; Raufer, T. M.] Rutherford Appleton Lab, Sci & Technol Facil Council, Didcot OX11 0QX, Oxon, England. [Gouffon, P.] Univ Sao Paulo, Inst Fis, BR-05315970 Sao Paulo, Brazil. [Ling, J.; Mishra, S. R.; Rosenfeld, C.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Irwin, G. M.; Pawloski, G.; Qiu, X.; Wojcicki, S. G.; Yang, T.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Auty, D. J.; Devenish, N. E.; Falk, E.; Hartnell, J.; Lefeuvre, G.] Univ Sussex, Dept Phys & Astron, Brighton BN1 9QH, E Sussex, England. [Webb, R. C.] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Kopp, S.; Lang, K.; Loiacono, L.; Mehdiyev, R.; Ospanov, R.; Ratchford, J.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Cherdack, D.; Gallagher, H. R.; Kafka, T.; Mann, W. A.; Oliver, W. P.; Schneps, J.] Tufts Univ, Dept Phys, Medford, MA 02155 USA. [Grzelak, K.] Univ Warsaw, Dept Phys, PL-00681 Warsaw, Poland. [Coleman, S. J.; Kordosky, M.; Nelson, J. K.; Vahle, P.] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. [Ayres, D. S.; Goodman, M. C.; Huang, X.; McGowan, A. M.; Paley, J.; Phan-Budd, S.; Sanchez, M. C.; Schreiner, P.; Talaga, R. L.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Adamson, P (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. RI Ling, Jiajie/I-9173-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Qiu, Xinjie/C-6164-2012; Gomes, Ricardo/B-6899-2008; Coelho, Joao/D-3546-2013; Tinti, Gemma/I-5886-2013; Evans, Justin/P-4981-2014; Gouffon, Philippe/I-4549-2012; Nowak, Jaroslaw/P-2502-2016 OI Hartnell, Jeffrey/0000-0002-1744-7955; Cherdack, Daniel/0000-0002-3829-728X; Weber, Alfons/0000-0002-8222-6681; Ling, Jiajie/0000-0003-2982-0670; COLEMAN, STEPHEN/0000-0002-4621-9169; Corwin, Luke/0000-0001-7143-3821; Gomes, Ricardo/0000-0003-0278-4876; Evans, Justin/0000-0003-4697-3337; Gouffon, Philippe/0000-0001-7511-4115; Nowak, Jaroslaw/0000-0001-8637-5433 FU U.S. DOE; UK STFC; U.S. NSF; State and University of Minnesota; University of Athens, Greece; Brazil FAPESP; Brazil CNPq; Brazil CAPES FX This work was supported by the U.S. DOE, the UK STFC, the U.S. NSF, the State and University of Minnesota, the University of Athens, Greece, and Brazil's FAPESP, CNPq, and CAPES. We are grateful to the Minnesota DNR, the crew of the Soudan Underground Laboratory, and the personnel of Fermilab for their contributions to this effort. NR 37 TC 168 Z9 168 U1 2 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 2 PY 2011 VL 106 IS 18 AR 181801 DI 10.1103/PhysRevLett.106.181801 PG 6 WC Physics, Multidisciplinary SC Physics GA 757PU UT WOS:000290101000002 PM 21635083 ER PT J AU Yu, R Zhu, JX Si, QM AF Yu, Rong Zhu, Jian-Xin Si, Qimiao TI Mott Transition in Modulated Lattices and Parent Insulator of (K, Tl)(y)FexSe2 Superconductors SO PHYSICAL REVIEW LETTERS LA English DT Article ID IRON AB The degree of electron correlations remains a central issue in the iron-based superconductors. The parent iron pnictides are antiferromagnetic, and their bad-metal behavior has been interpreted in terms of proximity to a Mott transition. We study such a transition in multiorbital models on modulated lattices containing an ordered pattern of iron vacancies, using a slave-rotor method. We show that the ordered vacancies lead to a band narrowing, which pushes the system to the Mott insulator side. This effect is proposed to underlie the insulating behavior observed in the parent compounds of the newly discovered (K, Tl)(y)FexSe2 superconductors. C1 [Yu, Rong; Si, Qimiao] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Yu, R (reprint author), Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. RI YU, RONG/C-1506-2012; Yu, Rong/K-5854-2012; Yu, Rong/H-3355-2016; OI Zhu, Jianxin/0000-0001-7991-3918 FU NSF [DMR-1006985]; Robert A. Welch Foundation [C-1411]; U.S. DOE [DE-AC52-06NA25396] FX We thank J. Dai, M. Fang, and T. Xiang for useful discussions. This work was supported by NSF Grant No. DMR-1006985 and the Robert A. Welch Foundation Grant No. C-1411 (R. Y. and Q. S.), and U.S. DOE at LANL under Contract No. DE-AC52-06NA25396 (J.-X.Z.). NR 35 TC 64 Z9 65 U1 1 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 2 PY 2011 VL 106 IS 18 AR 186401 DI 10.1103/PhysRevLett.106.186401 PG 4 WC Physics, Multidisciplinary SC Physics GA 757PU UT WOS:000290101000008 PM 21635107 ER PT J AU Lund, SM Friedman, A Bazouin, G AF Lund, Steven M. Friedman, Alex Bazouin, Guillaume TI Sheet beam model for intense space charge: Application to Debye screening and the distribution of particle oscillation frequencies in a thermal equilibrium beam SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID EMITTANCE GROWTH; ELECTRON-BEAMS; ION-BEAMS; RESONANCES; ANISOTROPY; PLASMAS; ENERGY AB A one-dimensional Vlasov-Poisson model for sheet beams is reviewed and extended to provide a simple framework for analysis of space-charge effects. Centroid and rms envelope equations including image-charge effects are derived and reasonable parameter equivalences with commonly employed 2D transverse models of unbunched beams are established. This sheet-beam model is then applied to analyze several problems of fundamental interest. A sheet-beam thermal equilibrium distribution in a continuous focusing channel is constructed and shown to have analogous properties to two- and three-dimensional thermal equilibrium models in terms of the equilibrium structure and Debye screening properties. The simpler formulation for sheet beams is exploited to explicitly calculate the distribution of particle oscillation frequencies within a thermal equilibrium beam. It is shown that as space-charge intensity increases, the frequency distribution becomes broad, suggesting that beams with strong space-charge can have improved stability relative to beams with weak space-charge. C1 [Lund, Steven M.; Friedman, Alex] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Bazouin, Guillaume] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. RP Lund, SM (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM smlund@llnl.gov; gbazouin@lbl.gov; af@llnl.gov FU U.S. Department of Energy at the Lawrence Livermore and Lawrence Berkeley National Laboratories [DE-AC52-07NA27344, DE-AC02-05CH11231] FX The authors wish to thank O. Anderson, J. Barnard, E. Lee, H. Okamoto, and E. Startsev for useful discussions. M. Campos Pinto helped verify aspects of results reported with Vlasov simulations which are not included herein. This research was performed under the auspices of the U.S. Department of Energy at the Lawrence Livermore and Lawrence Berkeley National Laboratories under Contracts No. DE-AC52-07NA27344 and No. DE-AC02-05CH11231. NR 52 TC 2 Z9 2 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD MAY 2 PY 2011 VL 14 IS 5 AR 054201 DI 10.1103/PhysRevSTAB.14.054201 PG 23 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 758IX UT WOS:000290158900003 ER PT J AU Yang, LY Li, YJ Guo, WM Krinsky, S AF Yang, Lingyun Li, Yongjun Guo, Weiming Krinsky, Samuel TI Multiobjective optimization of dynamic aperture SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID ACCELERATORS AB Dynamic aperture (DA) is one of the key nonlinear properties for a storage ring. Although there have been both analytical and numerical methods to find the aperture, the reverse problem of how to optimize it is still a challenging problem. A general and flexible way of optimizing the DA is highly demanded in accelerator design and operation. In this paper, we discuss the use of multiobjective optimization for DA. First we consider using objective functions based only on numerical tracking results. Data mining of these results demonstrated a correlation between DA and low-order nonlinear driving terms. Next we considered using objective functions which included both numerical tracking results and analytical estimates of low-order nonlinear driving terms. This resulted in faster convergence. The National Synchrotron Light Source II (NSLS-II) lattice was taken as an example to illustrate this method. This multiobjective approach is not limited by particular linear or nonlinear lattice settings, and can also be applied for optimizing other properties of a storage ring. C1 [Yang, Lingyun; Li, Yongjun; Guo, Weiming; Krinsky, Samuel] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. RP Yang, LY (reprint author), Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. FU Brookhaven Science Associates, LLC [DE-AC02-98CH10886]; Department of Energy FX We thank J. Bengtsson for his help on driving terms calculation, T. Tanabe for the kickmap of the damping wiggler, and M. Borland, L. Emery, D. Robin, and C. Steier for fruitful discussions. This work was supported by Brookhaven Science Associates, LLC under Contract No. DE-AC02-98CH10886 with the Department of Energy. NR 25 TC 15 Z9 15 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD MAY 2 PY 2011 VL 14 IS 5 AR 054001 DI 10.1103/PhysRevSTAB.14.054001 PG 10 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 758IX UT WOS:000290158900002 ER PT J AU Jain, A Lense, S Linehan, JC Raugei, S Cho, H DuBois, DL Shaw, WJ AF Jain, Avijita Lense, Sheri Linehan, John C. Raugei, Simone Cho, Herman DuBois, Daniel L. Shaw, Wendy J. TI Incorporating Peptides in the Outer-Coordination Sphere of Bioinspired Electrocatalysts for Hydrogen Production SO INORGANIC CHEMISTRY LA English DT Article ID PENDANT NITROGEN BASES; SOLID-PHASE SYNTHESIS; FE-ONLY HYDROGENASE; MOLECULAR CATALYSTS; CRYSTAL-STRUCTURE; H-2 PRODUCTION; ACTIVE-SITE; COMPUTATIONAL DESIGN; IRON(II) COMPLEXES; SOLUBLE POLYMERS AB Four new cyclic 1,5-diaza-3,7-diphosphacyclooctane ligands have been prepared and used to synthesize [Ni(p(2)(ph)N(2)(R))(2)](2+) complexes in which R is a mono- or dipeptide. These complexes represent a first step in the development of an outer-coordination sphere for this class of complexes that can mimic the outer-coordination sphere of the active sites of hydrogenase enzymes. Importantly, these complexes retain the electrocatalytic activity of the parent [Ni(P(2)(Ph)N(2)(Ph))(2)](2+) complex in an acetonitrile solution with turnover frequencies for hydrogen production ranging from 14 to 25 s(-1) in the presence of p-cyanoaniliniurn trifluoromethanesulfonate and from 135 to 1000 s(-1) in the presence of protonated dimethylformamide, with moderately low overpotentials, similar to 0.3 V. The addition of small amounts of water results in rate increases of 2-7 times. Unlike the parent complex, these complexes demonstrate dynamic structural transformations in solution. These results establish a building block from which larger peptide scaffolding can be added to allow the [Ni(p(2)(R)N(2)(R'))(2)](2+) molecular catalytic core to begin to mimic the multifunctional outer-coordination sphere of enzymes. C1 [Jain, Avijita; Lense, Sheri; Linehan, John C.; Raugei, Simone; Cho, Herman; DuBois, Daniel L.; Shaw, Wendy J.] Pacific NW Natl Lab, Chem & Mat Sci Div, Richland, WA 99354 USA. RP Shaw, WJ (reprint author), Pacific NW Natl Lab, Chem & Mat Sci Div, Richland, WA 99354 USA. EM wendy.shaw@pnl.gov FU U.S. Department of Energy Basic Energy Sciences, Chemical Sciences, Geosciences & Biosciences Division FX We thank Dr. John Roberts for useful discussion. This work was supported by the U.S. Department of Energy Basic Energy Sciences, Chemical Sciences, Geosciences & Biosciences Division. The Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy. NR 78 TC 47 Z9 47 U1 2 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 J9 INORG CHEM JI Inorg. Chem. PD MAY 2 PY 2011 VL 50 IS 9 BP 4073 EP 4085 DI 10.1021/ic1025872 PG 13 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 752RO UT WOS:000289710700027 PM 21456543 ER PT J AU Miller, MK Longstreth-Spoor, L Kelton, KF AF Miller, M. K. Longstreth-Spoor, L. Kelton, K. F. TI Detecting density variations and nanovoids SO ULTRAMICROSCOPY LA English DT Article; Proceedings Paper CT 52nd International Field Emission Symposium CY JUL 05-08, 2010 CL Sydney, AUSTRALIA DE Atom probe tomography; Voids; Radiation damage ID FIELD-ION MICROSCOPY; IRRADIATED TUNGSTEN AB A combination of simulated and experimental data has been used to investigate the size range of nanovoids that can be detected in atom probe tomography data. Simulated atom probe tomography data have revealed that nanovoids as small as 1 nm in diameter can be detected in atom probe tomography data with the use of iso-density surfaces. Iso-density surfaces may be used to quantify the size, morphology and number density of nanovoids and other variations in density in atom probe tomography data. Experimental data from an aluminum-yttrium-iron metallic glass ribbon have revealed the effectiveness of this approach. Combining iso-density surfaces with atom maps also permits the segregation of solute to the nanovoids to be investigated. Field ion microscopy and thin section atom maps have also been used to detect pores and larger voids. Published by Elsevier B.V. C1 [Miller, M. K.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Longstreth-Spoor, L.; Kelton, K. F.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. RP Miller, MK (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM millermk@ornl.gov FU United States Government [DE-AC05-00OR22725]; United States Department of Energy; Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy; ORNL; Office of Basic Energy Sciences, US Department of Energy FX This submission was sponsored by a contractor of the United States Government under Contract DE-AC05-00OR22725 with the United States Department of Energy. The United States Government retains, and the publisher, by accepting this submission for publication, acknowledges that the United States Government retains, a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this submission, or allow others to do so, for United States Government purposes.; MKM was sponsored by the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy. Atom probe tomography (MKM) was supported by ORNL's Shared Research Equipment (SHaRE) User Facility, which is sponsored by the Office of Basic Energy Sciences, US Department of Energy. NR 5 TC 10 Z9 10 U1 2 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3991 EI 1879-2723 J9 ULTRAMICROSCOPY JI Ultramicroscopy PD MAY PY 2011 VL 111 IS 6 BP 469 EP 472 DI 10.1016/j.ultramic.2011.01.027 PG 4 WC Microscopy SC Microscopy GA 894XN UT WOS:000300460900018 PM 21664542 ER PT J AU Miller, MK Zhang, Y AF Miller, M. K. Zhang, Y. TI Fabrication and characterization of APT specimens from high dose heavy ion irradiated materials SO ULTRAMICROSCOPY LA English DT Article; Proceedings Paper CT 52nd International Field Emission Symposium CY JUL 05-08, 2010 CL Sydney, AUSTRALIA DE Atom probe tomography; Ion irradiation; Radiation damage; Focused ion beam milling ID ATOM-PROBE TOMOGRAPHY; MICROSCOPY; TUNGSTEN; ALLOYS; DAMAGE AB The next generations of advanced energy systems will require materials that can withstand high doses of irradiation at elevated temperatures. Therefore, a methodology has been developed for the fabrication of high-dose ion-irradiated atom probe tomography specimens at a specific dose with the use of a focused ion beam milling system. The method also enables the precise ion dose of the atom probe tomography specimen to be estimated from the local concentration of the implanted ions. The method has been successfully applied to the characterization of the distribution of nanoclusters in a radiation-tolerant 14YWT nanostructured ferritic steel under ion irradiation to doses up to 400 displacements per atom. Published by Elsevier B.V. C1 [Miller, M. K.; Zhang, Y.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Miller, MK (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, POB 2008,MS 6136, Oak Ridge, TN 37831 USA. EM millermk@ornl.gov FU United States Government [DE-AC05-00OR22725]; United States Department of Energy [DE-AC05-76RL01830]; Office of Basic Energy Sciences, US Department of Energy; Department of Energy's Office of Biological and Environmental Research at Pacific Northwest National Laboratory (PNNL); Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, US Department of Energy FX This submission was sponsored by a contractor of the United States Government under contract DE-AC05-00OR22725 with the United States Department of Energy. The United States Government retains, and the publisher, by accepting this submission for publication, acknowledges that the United States Government retains, a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this submission, or allow others to do so, for United States Government purposes.; The authors thank K. Thomas for preparing the APT specimens and D.T. Hoelzer for providing the alloy used in this study. This research was sponsored by the Office of Basic Energy Sciences, US Department of Energy and by ORNL's Shared Research Equipment (SHaRE) User Facility, which is sponsored by the Office of Basic Energy Sciences, US Department of Energy. A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory (PNNL). Y. Zhang is grateful for the PECASE supported by the Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, US Department of Energy. PNNL is operated by Battelle for the US Department of Energy under Contract no. DE-AC05-76RL01830. NR 14 TC 12 Z9 12 U1 1 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3991 EI 1879-2723 J9 ULTRAMICROSCOPY JI Ultramicroscopy PD MAY PY 2011 VL 111 IS 6 BP 672 EP 675 DI 10.1016/j.ultramic.2010.12.036 PG 4 WC Microscopy SC Microscopy GA 894XN UT WOS:000300460900054 PM 21277681 ER PT J AU Kainerstorfer, JM Riley, JD Ehler, M Najafizadeh, L Amyot, F Hassan, M Pursley, R Demos, SG Chernomordik, V Pircher, M Smith, PD Hitzenberger, CK Gandjbakhche, AH AF Kainerstorfer, Jana M. Riley, Jason D. Ehler, Martin Najafizadeh, Laleh Amyot, Franck Hassan, Moinuddin Pursley, Randall Demos, Stavros G. Chernomordik, Victor Pircher, Michael Smith, Paul D. Hitzenberger, Christoph K. Gandjbakhche, Amir H. TI Quantitative principal component model for skin chromophore mapping using multi-spectral images and spatial priors SO BIOMEDICAL OPTICS EXPRESS LA English DT Article ID OPTICAL COHERENCE TOMOGRAPHY; IN-VIVO; HEMOGLOBIN OXYGENATION; LESION CLASSIFICATION; EPIDERMAL THICKNESS; COLOR IMAGE; SEGMENTATION; ABSORPTION; SIMULATION; FEATURES AB We describe a novel reconstruction algorithm based on Principal Component Analysis (PCA) applied to multi-spectral imaging data. Using numerical phantoms, based on a two layered skin model developed previously, we found analytical expressions, which convert qualitative PCA results into quantitative blood volume and oxygenation values, assuming the epidermal thickness to be known. We also evaluate the limits of accuracy of this method when the value of the epidermal thickness is not known. We show that blood volume can reliably be extracted (less than 6% error) even if the assumed thickness deviates 0.04mm from the actual value, whereas the error in blood oxygenation can be as large as 25% for the same deviation in thickness. This PCA based reconstruction was found to extract blood volume and blood oxygenation with less than 8% error, if the underlying structure is known. We then apply the method to in vivo multi-spectral images from a healthy volunteer's lower forearm, complemented by images of the same area using Optical Coherence Tomography (OCT) for measuring the epidermal thickness. Reconstruction of the imaging results using a two layered analytical skin model was compared to PCA based reconstruction results. A point wise correlation was found, showing the proof of principle of using PCA based reconstruction for blood volume and oxygenation extraction. (C) 2011 Optical Society of America C1 [Kainerstorfer, Jana M.; Riley, Jason D.; Najafizadeh, Laleh; Hassan, Moinuddin; Chernomordik, Victor; Gandjbakhche, Amir H.] Eunice Kennedy Shriver Natl Inst Child Hlth & Hum, NIH, Program Pediat Imaging & Tissue Sci, Sect Analyt & Funct Biophoton, Bethesda, MD 20892 USA. [Kainerstorfer, Jana M.; Pircher, Michael; Hitzenberger, Christoph K.] Med Univ Vienna, Ctr Med Phys & Biomed Engn, A-1090 Vienna, Austria. [Ehler, Martin] Eunice Kennedy Shriver Natl Inst Child Hlth & Hum, NIH, Program Phys Biol, Lab Integrat & Med Biophys,Sect Med Biophys, Bethesda, MD 20892 USA. [Najafizadeh, Laleh] Henry M Jackson Fdn, Rockville, MD 20852 USA. [Amyot, Franck] NINDS, NIH, Clin Neurosci Program, Bethesda, MD 20892 USA. [Pursley, Randall] NIH, Ctr Informat Technol, Div Computat Biosci, Signal Proc & Instrumentat Sect, Bethesda, MD 20892 USA. [Demos, Stavros G.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Smith, Paul D.] Natl Inst Biomed Imaging & Bioengn, NIH, Lab Cellular Imaging & Macromol Biophys, Biomed Instrumentat & Multiscale Imaging Sect, Bethesda, MD 20892 USA. RP Kainerstorfer, JM (reprint author), Eunice Kennedy Shriver Natl Inst Child Hlth & Hum, NIH, Program Pediat Imaging & Tissue Sci, Sect Analyt & Funct Biophoton, Bethesda, MD 20892 USA. EM kainersj@mail.nih.gov FU Eunice Kennedy Shriver National Institute of Child Health and Human Development FX The research was funded by the Intramural Research Program of the Eunice Kennedy Shriver National Institute of Child Health and Human Development. The Graduate Partnership Program at the National Institutes of Health and the Faculty of Physics at the University of Vienna / Austria are also acknowledged. NR 46 TC 10 Z9 10 U1 0 U2 8 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 2156-7085 J9 BIOMED OPT EXPRESS JI Biomed. Opt. Express PD MAY 1 PY 2011 VL 2 IS 5 BP 1040 EP 1058 PG 19 WC Biochemical Research Methods; Optics; Radiology, Nuclear Medicine & Medical Imaging SC Biochemistry & Molecular Biology; Optics; Radiology, Nuclear Medicine & Medical Imaging GA 886TY UT WOS:000299878000002 PM 21559118 ER PT J AU Rupnow, K Underwood, KD Compton, K AF Rupnow, Kyle Underwood, Keith D. Compton, Katherine TI Scientific Application Demands on a Reconfigurable Functional Unit Interface SO ACM TRANSACTIONS ON RECONFIGURABLE TECHNOLOGY AND SYSTEMS LA English DT Article DE Design; Performance; Reconfigurable functional units; communication interfaces; scientific applications ID SYSTEMS AB Modern scientific applications are large, complex, and highly parallel they are commonly executed on supercomputers with tens of thousands of processors. Yet these applications still commonly require weeks or even months to execute. Thus, single-thread performance remains a concern for highly parallel scientific applications. Adding a reconfigurable accelerator to each CPU could improve system performance; however, scientific applications have design constraints that differ from most application domains commonly accelerated by reconfigurable logic. In this article, we discuss the constraints imposed by scientific applications on the computation model, the accelerator architecture, and the accelerator's communication interface with the CPU. Based on these constraints and application analysis, we have previously proposed adding a Reconfigurable Functional Unit (RFU) to accelerate integer graphs that calculate complex memory addresses. In this work, we now propose a flexible multi-instruction interface technique that allows dataflow graphs implemented on the RFU to access a large number of inputs and outputs with minor CPU datapath modifications. We present an in-depth examination of the performance effects of different communication interfaces that use this technique, and select one that best matches the needs of Sandia's scientific applications. Although RFU execution overall improves performance, we also isolate two key negative performance effects introduced by aggregating CPU instructions into dataflow graphs: delayed issue and graph serialization. Finally, to demonstrate the marketability of an RFU beyond scientific applications, we reanalyze the proposed interfaces using the SPEC-fp benchmark suite. We show that although choosing an interface based on SPEC-fp needs is detrimental to Sandia application performance, choosing an interface based on Sandia demands works well for more general-purpose applications. C1 [Rupnow, Kyle; Compton, Katherine] Univ Wisconsin Madison, Dept Elect Engn, Madison, WI 53715 USA. [Rupnow, Kyle] Sandia Natl Labs, Livermore, CA 94550 USA. [Underwood, Keith D.] Intel Corp, Santa Clara, CA 95051 USA. RP Rupnow, K (reprint author), Univ Wisconsin Madison, Dept Elect Engn, Madison, WI 53715 USA. EM kjrupnow@gmail.com; keith.d.underwood@intel.com; kati@engr.wisc.edu RI Rupnow, Kyle/E-1635-2015 OI Rupnow, Kyle/0000-0003-2908-2225 FU United States Department of Energy's National Nuclear Security Administration [DEAC04-94AL85000] FX Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under contract DEAC04-94AL85000. NR 28 TC 4 Z9 4 U1 0 U2 1 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 1936-7406 EI 1936-7414 J9 ACM T RECONFIG TECHN JI ACM T. Reconfigurable Technol. Syst. PD MAY PY 2011 VL 4 IS 2 AR 19 DI 10.1145/1968502.1968510 PG 30 WC Computer Science, Hardware & Architecture SC Computer Science GA 879NQ UT WOS:000299337300008 ER PT J AU Raabe, BM Lovaglio, J Grover, GS Brown, SA Boucher, JF Yuan, Y Civil, JR Gillhouse, KA Stubbs, MN Hoggatt, AF Halliday, LC Fortman, JD AF Raabe, Brigitte M. Lovaglio, Jamie Grover, G. Scott Brown, Scott A. Boucher, Joseph F. Yuan, Yang Civil, Jacqueline R. Gillhouse, Kimberly A. Stubbs, Makeida N. Hoggatt, Amber F. Halliday, Lisa C. Fortman, Jeffrey D. TI Pharmacokinetics of Cefovecin in Cynomolgus Macaques (Macaca fascicularis), Olive Baboons (Papio anubis), and Rhesus Macaques (Macaca mulatta) SO JOURNAL OF THE AMERICAN ASSOCIATION FOR LABORATORY ANIMAL SCIENCE LA English DT Article ID MODEL; PARAMETERS; CATS; DOGS AB Cefovecin sodium is a long-acting, third-generation, cephalosporin antibiotic approved for the treatment of skin infections in dogs and cats. The pharmacokinetic properties of cefovecin were evaluated in cynomolgus macaques (Macaca fascicularis), olive baboons (Papio anubis), and rhesus macaques (Macaca mulatta) by using a single-dose (8 mg/kg SC) dosing regimen. Plasma cefovecin concentrations were determined by using ultra-performance liquid chromatography with tandem mass spectrometry, and a noncompartmental model was used to determine pharmacokinetic parameters. The half-life of cefovecin was 4.95 +/- 1.47 h in cynomolgus macaques, 9.17 +/- 1.84 h in olive baboons, and 8.40 +/- 2.53 h in rhesus macaques. These values are considerably lower than the half-lives previously published for dogs (133 h) and cats (166 h). The extended half-life of cefovecin in dogs and cats is speculated to be due to active reabsorption of drug in the kidney tubules because plasma clearance is well below the normal glomerular filtration rate. In nonhuman primates, renal clearance rates approximated plasma clearance rates, suggesting that active renal reabsorption of cefovecin does not occur in these species. The pharmacokinetic properties of cefovecin in nonhuman primates are vastly different from the pharmacokinetic properties in dogs and cats, precluding its use as a long-acting antibiotic in nonhuman primates. This study highlights the importance of performing pharmacokinetic studies prior to extralabel drug usage. C1 [Raabe, Brigitte M.; Lovaglio, Jamie; Hoggatt, Amber F.; Halliday, Lisa C.; Fortman, Jeffrey D.] Univ Illinois, Biol Resources Lab, Chicago, IL USA. [Lovaglio, Jamie] Battelle Toxicol NW, Richland, WA USA. [Grover, G. Scott; Brown, Scott A.; Boucher, Joseph F.; Yuan, Yang] Pfizer Anim Hlth, Vet Med Res & Dev, Kalamazoo, MI USA. [Civil, Jacqueline R.] Pfizer Anim Hlth, Vet Med Res & Dev, Sandwich, Kent, England. [Gillhouse, Kimberly A.; Stubbs, Makeida N.] Pfizer Inc, Global Res & Dev, Groton, CT 06340 USA. RP Raabe, BM (reprint author), Res Anim Resources Ctr, Madison, WI 53726 USA. EM bmraabe@wise.edu NR 18 TC 10 Z9 10 U1 0 U2 11 PU AMER ASSOC LABORATORY ANIMAL SCIENCE PI MEMPHIS PA 9190 CRESTWYN HILLS DR, MEMPHIS, TN 38125 USA SN 1559-6109 J9 J AM ASSOC LAB ANIM JI J. Amer. Assoc. Lab. Anim. Sci. PD MAY PY 2011 VL 50 IS 3 BP 389 EP 395 PG 7 WC Veterinary Sciences; Zoology SC Veterinary Sciences; Zoology GA 875JO UT WOS:000299026400014 PM 21640036 ER PT J AU Kumar, KS Patnaik, A AF Kumar, K. Senthil Patnaik, Archita TI Solvent-Polarity-Tunable Dimeric Association of a Fullerene (C-60)-N,N-Dimethylaminoazobenzene Dyad: Modulated Electronic Coupling of the Azo Chromophore with a Substituted 3D Fullerene SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE azo compounds; dimerization; electronic structure; fullerenes; supramolecular chemistry ID LANGMUIR-BLODGETT-FILMS; WATER-SOLUBLE FULLERENES; PERYLENE BISIMIDE DYES; SUPRAMOLECULAR ARCHITECTURES; AZOBENZENE DERIVATIVES; AROMATIC INTERACTIONS; PORPHYRIN-FULLERENE; CYANINE DYES; COLLOIDAL DISPERSIONS; AGGREGATE FORMATION AB The tunable self-assembly of a fullerene (C60)-N,N-dimethylaminoazobenzene (DPNME) molecular system as a function of solvent polarity in THF/water binary solvent is reported. Gradual increase of the volume fraction of the nonsolvent water in a 1 x 10(-5) M THF solution of DPNME at a mixed dielectric constant epsilon(mix) approximate to 42 resulted in initial redshifting of the 1(pi ->pi*) absorption band, which signified the 1D head-to-tail or J-type arrangement of the DPNME molecular system. Further increase in the solvent polarity to epsilon(mix) approximate to 66 evidenced formation of an antiparallel head-to-tail or H-type molecular arrangement in conjunction with the J-aggregates, thereby establishing a solvent-polarity-dependent dynamic equilibrium between the monomer <-> J-aggregate <-> H-aggregate. The controlled aggregation was governed by the synergetic effect of intermolecular donor-acceptor interaction between the electron-deficient fullerene ring and the electron-rich N,N-dimethylamino-substituted aromatic ring; typically, van der Waals and pi-pi interactions between the molecules constituting a pair of dimers were envisaged. An agreement between the semiempirically calculated drastically reduced oscillator strength of the DPNME H-dimer in the antiparallel configuration (0.69 vs. 1.29 in the monomeric DPNME) and the experimental electronic absorption spectra beyond epsilon(mix)=66 further strengthened this assignment to the hitherto forbidden antiparallel H-dimer. Complementing the above, the periodicity of molecular self-assembly dictated a monoclinic unit cell in the single-crystal XRD packing pattern with a C2/c space group; the molecules packed laterally with mutual interdigitation with the donor (E)-N,N-dimethyl-4-(p-tolyldiazenyl)aniline (AZNME) parts in an antiparallel fashion (contrary to the usual expectation for H-aggregates) with strong inter-and intrapair van der Waals and pi-pi interactions between the constituent fullerene moieties. Unlike those of porphyrin/phthalocyanine bowl-like donor-initiated architectures, a rare class of DPNME dyadic supramolecular self-assemblies was realized with pi-extended 2D fullerene networks, in which the linear geometry of the AZNME donor and the conformational rigidity of the fullerene acceptor played crucial roles. C1 [Kumar, K. Senthil; Patnaik, Archita] Indian Inst Technol, Dept Chem, Madras 600036, Tamil Nadu, India. RP Patnaik, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. EM archita59@yahoo.com FU Department of Science and Technology, New Delhi, India [SR/S2/CMP-57/2006]; IIT Madras for the SRF FX The authors are grateful to the Department of Science and Technology, New Delhi, India, for the financial support (Grant No. SR/S2/CMP-57/2006). K.S.K. thanks IIT Madras for the SRF grant. NR 148 TC 9 Z9 9 U1 4 U2 57 PU WILEY-BLACKWELL PI MALDEN PA COMMERCE PLACE, 350 MAIN ST, MALDEN 02148, MA USA SN 0947-6539 J9 CHEM-EUR J JI Chem.-Eur. J. PD MAY PY 2011 VL 17 IS 19 BP 5327 EP 5343 DI 10.1002/chem.201002981 PG 17 WC Chemistry, Multidisciplinary SC Chemistry GA 759BF UT WOS:000290214200016 PM 21404350 ER PT J AU Wang, YX Yang, F Gritsenko, MA Wang, YC Clauss, T Liu, T Shen, YF Monroe, ME Lopez-Ferrer, D Reno, T Moore, RJ Klemke, RL Camp, DG Smith, RD AF Wang, Yuexi Yang, Feng Gritsenko, Marina A. Wang, Yingchun Clauss, Therese Liu, Tao Shen, Yufeng Monroe, Matthew E. Lopez-Ferrer, Daniel Reno, Theresa Moore, Ronald J. Klemke, Richard L. Camp, David G., II Smith, Richard D. TI Reversed-phase chromatography with multiple fraction concatenation strategy for proteome profiling of human MCF10A cells SO PROTEOMICS LA English DT Article DE 2-D chromatography; Concatenation; Fractionation; High pH RP; Low pH RP; Technology ID TANDEM MASS-SPECTROMETRY; CYSTEINYL-PEPTIDE ENRICHMENT; STRONG CATION-EXCHANGE; LIQUID-CHROMATOGRAPHY; SHOTGUN PROTEOMICS; RETENTION PREDICTION; YEAST PROTEOME; PH GRADIENT; SEPARATION; MS/MS AB In this study, we evaluated a concatenated low pH (pH 3) and high pH (pH 10) reversed-phase liquid chromatography strategy as a first dimension for two-dimensional liquid chromatography tandem mass spectrometry ("shotgun") proteomic analysis of trypsin-digested human MCF10A cell sample. Compared with the more traditional strong cation exchange method, the use of concatenated high pH reversed-phase liquid chromatography as a first-dimension fractionation strategy resulted in 1.8- and 1.6-fold increases in the number of peptide and protein identifications (with two or more unique peptides), respectively. In addition to broader identifications, advantages of the concatenated high pH fractionation approach include improved protein sequence coverage, simplified sample processing, and reduced sample losses. The results demonstrate that the concatenated high pH reversed-phased strategy is an attractive alternative to strong cation exchange for two-dimensional shotgun proteomic analysis. C1 [Wang, Yuexi; Yang, Feng; Gritsenko, Marina A.; Clauss, Therese; Liu, Tao; Shen, Yufeng; Monroe, Matthew E.; Lopez-Ferrer, Daniel; Moore, Ronald J.; Camp, David G., II; Smith, Richard D.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. [Wang, Yingchun] Chinese Acad Sci, Key Lab Mol & Dev Biol, Inst Genet & Dev Biol, Beijing, Peoples R China. [Klemke, Richard L.] Univ Calif San Diego, Dept Pathol, La Jolla, CA 92093 USA. [Klemke, Richard L.] UC San Diego, Moores Canc Ctr, La Jolla, CA USA. RP Smith, RD (reprint author), Pacific NW Natl Lab, Div Biol Sci, POB 999,MS K8-98, Richland, WA 99352 USA. EM rds@pnl.gov RI Smith, Richard/J-3664-2012; Liu, Tao/A-9020-2013 OI Smith, Richard/0000-0002-2381-2349; Liu, Tao/0000-0001-9529-6550 FU NIH [GM068487, CA097022, RR018522]; DOE [DE-AC05-76RL01830] FX This research was supported by NIH grants GM068487 (R. L. K.), CA097022 (R. L. K.) and RR018522 (R. D. S.). Work was performed in the NIH NCRR P41 Biomedical Technology Research Center for Proteomics located in the Environmental Molecular Sciences Laboratory (EMSL), a US Department of Energy (DOE) Office of Biological and Environmental Science national scientific user facility at Pacific Northwest National Laboratory (PNNL) in Richland, Washington. PNNL is a multi-program national laboratory operated by Battelle for the DOE under Contract DE-AC05-76RL01830. The authors thank Dr. Andrew Alpert from PolyLC Inc., for his helpful input on SCX chromatography. NR 35 TC 134 Z9 137 U1 7 U2 54 PU WILEY-BLACKWELL PI MALDEN PA COMMERCE PLACE, 350 MAIN ST, MALDEN 02148, MA USA SN 1615-9853 J9 PROTEOMICS JI Proteomics PD MAY PY 2011 VL 11 IS 10 BP 2019 EP 2026 DI 10.1002/pmic.201000722 PG 8 WC Biochemical Research Methods; Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 762NM UT WOS:000290486200013 PM 21500348 ER PT J AU Ramirez, LM Cirnigliaro, CM Asselin, P Swaby, S Wielopolski, L Spungen, AM Bauman, WA AF Ramirez, L. M. Cirnigliaro, C. M. Asselin, P. Swaby, S. Wielopolski, L. Spungen, A. M. Bauman, W. A. TI Comparison of Regional and Total Body Skeletal Muscle Mass by BIA, DEXA, and Lower Extremity PBK in Persons with Spinal Cord Injury SO INTERNATIONAL JOURNAL OF OBESITY LA English DT Meeting Abstract CT 9th International Symposium on In Vivo Body Composition Studies CY MAY, 2011 CL Hangzhou, PEOPLES R CHINA C1 [Ramirez, L. M.; Asselin, P.; Swaby, S.; Spungen, A. M.; Bauman, W. A.] James J Peters VA Med Ctr, VA RR&D Ctr Excellence Med Consequences Spinal Co, Bronx, NY USA. [Cirnigliaro, C. M.] Kessler Inst Rehabil, W Orange, NJ USA. [Wielopolski, L.] Brookhaven Natl Lab, Upton, NY 11973 USA. NR 0 TC 0 Z9 0 U1 0 U2 1 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0307-0565 J9 INT J OBESITY JI Int. J. Obes. PD MAY PY 2011 VL 35 SU 2 BP S61 EP S61 PG 1 WC Endocrinology & Metabolism; Nutrition & Dietetics SC Endocrinology & Metabolism; Nutrition & Dietetics GA 836UZ UT WOS:000296141100204 ER PT J AU Li, LY Kim, S Wang, W Vijayakumar, M Nie, ZM Chen, BW Zhang, JL Xia, GG Hu, JZ Graff, G Liu, J Yang, ZG AF Li, Liyu Kim, Soowhan Wang, Wei Vijayakumar, M. Nie, Zimin Chen, Baowei Zhang, Jianlu Xia, Guanguang Hu, Jianzhi Graff, Gordon Liu, Jun Yang, Zhenguo TI A Stable Vanadium Redox-Flow Battery with High Energy Density for Large-Scale Energy Storage SO ADVANCED ENERGY MATERIALS LA English DT Article ID CELL ELECTROLYTE AB The all-vanadium redox flow battery is a promising technology for large-scale renewable and grid energy storage, but is limited by the low energy density and poor stability of the vanadium electrolyte solutions. A new vanadium redox flow battery with a significant improvement over the current technology is reported in this paper. This battery uses sulfate-chloride mixed electrolytes, which are capable of dissolving 2.5 M vanadium, representing about a 70% increase in energy capacity over the current sulfate system. More importantly, the new electrolyte remains stable over a wide temperature range of -5 to 50 C, potentially eliminating the need for electrolyte temperature control in practical applications. This development would lead to a significant reduction in the cost of energy storage, thus accelerating its market penetration. C1 [Li, Liyu; Kim, Soowhan; Wang, Wei; Vijayakumar, M.; Nie, Zimin; Chen, Baowei; Zhang, Jianlu; Xia, Guanguang; Hu, Jianzhi; Graff, Gordon; Liu, Jun; Yang, Zhenguo] Pacific NW Natl Lab, Richland, WA 99354 USA. RP Li, LY (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd,POB 999, Richland, WA 99354 USA. EM liyu.li@pnl.gov; zgary.yang@pnl.gov RI Murugesan, Vijayakumar/C-6643-2011; Wang, Wei/F-4196-2010; Hu, Jian Zhi/F-7126-2012 OI Murugesan, Vijayakumar/0000-0001-6149-1702; Wang, Wei/0000-0002-5453-4695; FU Office of Electricity Delivery & Energy Reliability; U.S. Department of Energy (DOE) [57558]; Pacific Northwest National Laboratory (PNNL); DOE's Office of Biological and Environmental Research (BER); DOE by Battelle [DE-AC05 - 76RL01830] FX This work was supported by the Office of Electricity Delivery & Energy Reliability (project manager: Dr. Imre Gyuk), U.S. Department of Energy (DOE) under contract #57558, and by Pacific Northwest National Laboratory (PNNL) LDRD program. The NMR work was carried out at the Environmental and Molecular Science Laboratory, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research (BER). PNNL is a multi-program laboratory operated for DOE by Battelle under Contract DE-AC05 - 76RL01830. NR 19 TC 204 Z9 207 U1 31 U2 196 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD MAY PY 2011 VL 1 IS 3 BP 394 EP 400 DI 10.1002/aenm.201100008 PG 7 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA 778TH UT WOS:000291728400014 ER PT J AU Wang, RX Wang, F Boroyevich, D Burgos, R Lai, RX Ning, PQ Rajashekara, K AF Wang, Ruxi Wang, Fei (Fred) Boroyevich, Dushan Burgos, Rolando Lai, Rixin Ning, Puqi Rajashekara, Kaushik TI A High Power Density Single-Phase PWM Rectifier With Active Ripple Energy Storage SO IEEE TRANSACTIONS ON POWER ELECTRONICS LA English DT Article DE Active energy storage; capacitive energy storage; high power density converter; ripple energy; single-phase rectifier ID CONVERTER; INVERTERS AB It is well known that single-phase pulse width modulation rectifiers have second-order harmonic currents and corresponding ripple voltages on the dc bus. The low-frequency harmonic current is normally filtered using a bulk capacitor in the bus, which results in low power density. However, pursuing high power density in converter design is a very important goal in the aerospace applications. This paper studies methods for reducing the energy storage capacitor for single-phase rectifiers. The minimum ripple energy storage requirement is derived independently of a specific topology. Based on the minimum ripple energy requirement, the feasibility of the active capacitor's reduction schemes is verified. Then, we propose a bidirectional buck-boost converter as the ripple energy storage circuit, which can effectively reduce the energy storage capacitance. The analysis and design are validated by simulation and experimental results. C1 [Wang, Ruxi; Boroyevich, Dushan] Virginia Polytech Inst & State Univ, Dept Elect & Comp Engn, Ctr Power Elect Syst, Blacksburg, VA 24060 USA. [Wang, Fei (Fred)] Univ Tennessee, Knoxville, TN 37996 USA. [Wang, Fei (Fred); Ning, Puqi] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Burgos, Rolando] ABB Corp Res, Raleigh, NC 27606 USA. [Lai, Rixin] GE Global Res Ctr, Niskayuna, NY 12309 USA. [Rajashekara, Kaushik] Rolls Royce Corp, Carmel, IN 46032 USA. RP Wang, RX (reprint author), Virginia Polytech Inst & State Univ, Dept Elect & Comp Engn, Ctr Power Elect Syst, Blacksburg, VA 24060 USA. EM ruxi@vt.edu FU Rolls-Royce Corporation; National Science Foundation [EEC-9731677] FX Manuscript received May 18, 2010; revised October 13, 2010; accepted October 17, 2010. Date of current version June 22, 2011. This work was supported in part by the Rolls-Royce Corporation and in part by the National Science Foundation under Award Number EEC-9731677. Recommended for publication by Associate Editor. NR 24 TC 109 Z9 113 U1 2 U2 14 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8993 J9 IEEE T POWER ELECTR JI IEEE Trans. Power Electron. PD MAY PY 2011 VL 26 IS 5 BP 1430 EP 1443 DI 10.1109/TPEL.2010.2090670 PG 14 WC Engineering, Electrical & Electronic SC Engineering GA 821WX UT WOS:000295006200017 ER PT J AU Rossi, A Schulze, S Klose, S Kann, DA Rau, A Krimm, HA Johannesson, G Panaitescu, A Yuan, F Ferrero, P Kruhler, T Greiner, J Schady, P Pandey, SB Amati, L Afonso, PMJ Akerlof, CW Arnold, LA Clemens, C Filgas, R Hartmann, DH Yoldas, AK McBreen, S McKay, TA Guelbenzu, AN Olivares, FE Paciesas, B Rykoff, ES Szokoly, G Updike, AC Yoldas, A AF Rossi, A. Schulze, S. Klose, S. Kann, D. A. Rau, A. Krimm, H. A. Johannesson, G. Panaitescu, A. Yuan, F. Ferrero, P. Kruehler, T. Greiner, J. Schady, P. Pandey, S. B. Amati, L. Afonso, P. M. J. Akerlof, C. W. Arnold, L. A. Clemens, C. Filgas, R. Hartmann, D. H. Yoldas, A. Kuepcue McBreen, S. McKay, T. A. Guelbenzu, A. Nicuesa Olivares, F. E. Paciesas, B. Rykoff, E. S. Szokoly, G. Updike, A. C. Yoldas, A. TI The Swift/Fermi GRB 080928 from 1 eV to 150 keV SO ASTRONOMY & ASTROPHYSICS LA English DT Article DE gamma-ray burst: individual: GRB 080928 ID GAMMA-RAY BURST; BLAST WAVE PHYSICS; OPTICAL AFTERGLOWS; LIGHT CURVES; ULTRARELATIVISTIC SHOCKS; PARTICLE-ACCELERATION; COLUMN DENSITIES; HOST GALAXIES; 1ST SURVEY; SWIFT-ERA AB We present the results of a comprehensive study of the gamma-ray burst 080928 and of its afterglow. GRB 080928 was a long burst detected by Swift/BAT and Fermi/GBM. It is one of the exceptional cases where optical emission had already been detected when the GRB itself was still radiating in the gamma-ray band. For nearly 100 s simultaneous optical, X-ray and gamma-ray data provide a coverage of the spectral energy distribution of the transient source from about 1 eV to 150 keV. In particular, we show that the SED during the main prompt emission phase agrees with synchrotron radiation. We constructed the optical/near-infrared light curve and the spectral energy distribution based on Swift/UVOT, ROTSE-IIIa (Australia), and GROND (La Silla) data and compared it to the X-ray light curve retrieved from the Swift/XRT repository. We show that its bumpy shape can be modeled by multiple energy-injections into the forward shock. Furthermore, we investigate whether the temporal and spectral evolution of the tail emission of the first strong flare seen in the early X-ray light curve can be explained by large-angle emission (LAE). We find that a nonstandard LAE model is required to explain the observations. Finally, we report on the results of our search for the GRB host galaxy, for which only a deep upper limit can be provided. C1 [Rossi, A.; Schulze, S.; Klose, S.; Kann, D. A.; Ferrero, P.; Guelbenzu, A. Nicuesa] Thuringer Landessternwarte Tautenburg, D-07778 Tautenburg, Germany. [Schulze, S.] Univ Iceland, Inst Sci, Ctr Astrophys & Cosmol, IS-107 Reykjavik, Iceland. [Rau, A.; Kruehler, T.; Greiner, J.; Schady, P.; Afonso, P. M. J.; Clemens, C.; Filgas, R.; Yoldas, A. Kuepcue; McBreen, S.; Olivares, F. E.; Szokoly, G.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Krimm, H. A.] Univ Space Res Assoc, CRESST, Greenbelt, MD 20771 USA. [Updike, A. C.] NASA, Goddard Space Flight Ctr, Observ Cosmol Lab, Greenbelt, MD 20771 USA. [Johannesson, G.] Stanford Univ, Hansen Expt Phys Lab, Stanford, CA 94305 USA. [Panaitescu, A.] Los Alamos Natl Lab, ISR 1, Los Alamos, NM 87545 USA. [Yuan, F.; Pandey, S. B.; Akerlof, C. W.; McKay, T. A.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Ferrero, P.] Inst Astrofis Canarias, Tenerife 38200, Spain. [Ferrero, P.] Univ La Laguna, Dept Astrofis, Tenerife 38205, Spain. [Kruehler, T.] Tech Univ Munich, D-85748 Garching, Germany. [Pandey, S. B.] ARIES, Naini Tal 263129, Uttaranchal, India. [Amati, L.] INAF IASF Bologna, I-40129 Bologna, Italy. [Arnold, L. A.] Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA. [Hartmann, D. H.; Updike, A. C.] Clemson Univ, Dept Phys & Astron, Clemson, SC 29634 USA. [Yoldas, A. Kuepcue; Yoldas, A.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [McBreen, S.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Paciesas, B.] Univ Alabama, NSSTC, Huntsville, AL 35805 USA. [Rykoff, E. S.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Szokoly, G.] Eotvos Lorand Univ, Inst Phys, H-1117 Budapest, Hungary. [Updike, A. C.] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. RP Rossi, A (reprint author), Thuringer Landessternwarte Tautenburg, Sternwarte 5, D-07778 Tautenburg, Germany. EM rossi@tls-tautenburg.de RI McKay, Timothy/C-1501-2009; Amati, Lorenzo/N-5586-2015; Johannesson, Gudlaugur/O-8741-2015; Rossi, Andrea/N-4674-2015; OI McKay, Timothy/0000-0001-9036-6150; Amati, Lorenzo/0000-0001-5355-7388; Johannesson, Gudlaugur/0000-0003-1458-7036; Rossi, Andrea/0000-0002-8860-6538; Kruehler, Thomas/0000-0002-8682-2384; Schulze, Steve/0000-0001-6797-1889 FU DFG [K1 766/11-3, K1 766/16-1, HA 1850/28-1]; BLANCEFLOR Boncompagni-Ludovisi, nee Bildt foundation; Thuringer Landessternwarte Tautenburg, Germany; Icelandic Research Fund FX The authors thank the anonymous referee for a very constructive report. A. Rossi and S.K. acknowledge support by DFG grant K1 766/11-3 and AR additionally from the BLANCEFLOR Boncompagni-Ludovisi, nee Bildt foundation. S.S., D.A.K. and P.F. acknowledge support by the Thuringer Landessternwarte Tautenburg, Germany, as well as DFG grant K1 766/16-1. T.K. acknowledges support by the DFG cluster of excellence "Origin and Structure of the Universe". S.S. acknowledges further support by a Grant of Excellence from the Icelandic Research Fund. A. Rossi acknowledges Frederic Daigne, Cristiano Guidorzi, Daniele Pierini, and Sandra Savaglio for helpful discussions. A. Rau and S.K. acknowledge Re'em Sari for helpful remarks. D.A.K. acknowledges A. Zeh for fitting scripts. Part of the funding for GROND (both hardware and personnel) was generously granted from the Leibniz-Prize to Prof. G. Hasinger (DFG grant HA 1850/28-1). This work made use of data supplied by the UK Swift Science Data Centre at the University of Leicester. NR 99 TC 26 Z9 26 U1 0 U2 3 PU EDP SCIENCES S A PI LES ULIS CEDEX A PA 17, AVE DU HOGGAR, PA COURTABOEUF, BP 112, F-91944 LES ULIS CEDEX A, FRANCE SN 1432-0746 J9 ASTRON ASTROPHYS JI Astron. Astrophys. PD MAY PY 2011 VL 529 AR A142 DI 10.1051/0004-6361/201015324 PG 17 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 811UD UT WOS:000294240700017 ER PT J AU Sorger, VJ Ye, ZL Oulton, RF Wang, Y Bartal, G Yin, XB Zhang, X AF Sorger, Volker J. Ye, Ziliang Oulton, Rupert F. Wang, Yuan Bartal, Guy Yin, Xiaobo Zhang, Xiang TI Experimental demonstration of low-loss optical waveguiding at deep sub-wavelength scales SO NATURE COMMUNICATIONS LA English DT Article ID MACH-ZEHNDER MODULATOR; GUIDES; COMMUNICATION; PLASMONICS; PHOTON AB Emerging communication applications call for a road map towards nanoscale photonic components and systems. Although metal-based nanostructures theoretically offer a solution to enable nanoscale photonics, the key demonstration of optical modes with deep sub-diffraction-limited confinement and significant propagation distances has not been experimentally achieved because of the trade-off between optical confinement and metallic losses. Here we report the first experimental demonstration of truly nanoscale guided waves in a metal-insulator-semiconductor device featuring low-loss and broadband operation. Near-field scanning optical microscopy reveals mode sizes down to 50x60 nm(2) at visible and nearinfrared wavelengths propagating more than 20 times the vacuum wavelength. Interference spectroscopy confirms that the optical mode hybridization between a surface plasmon and a dielectric mode concentrates the hybridized mode inside a nanometre thin gap. This nanoscale waveguide holds promise for next generation on-chip optical communication systems that integrate light sources, modulators or switches, nonlinear and quantum optics. C1 [Sorger, Volker J.; Ye, Ziliang; Oulton, Rupert F.; Wang, Yuan; Bartal, Guy; Yin, Xiaobo; Zhang, Xiang] Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr, Berkeley, CA 94720 USA. [Zhang, Xiang] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Zhang, X (reprint author), Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr, 3112 Etcheverry Hall, Berkeley, CA 94720 USA. EM xiang@berkeley.edu RI Yin, Xiaobo/A-4142-2011; Zhang, Xiang/F-6905-2011; Wang, Yuan/F-7211-2011; Ye, Ziliang/A-2104-2011 FU National Science Foundation Nano-Scale Science and Engineering Center (NSF-NSEC) [CMMI-0751621] FX We acknowledge financial support from the National Science Foundation Nano-Scale Science and Engineering Center (NSF-NSEC) under the award CMMI-0751621. NR 30 TC 120 Z9 120 U1 12 U2 107 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAY PY 2011 VL 2 AR 331 DI 10.1038/ncomms1315 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 819CI UT WOS:000294802600036 ER PT J AU Hansen, JF van Breugel, W Bringa, EM Eberly, B Graham, GA Remington, BA Taylor, EA Tielens, AGGM AF Hansen, J. F. van Breugel, W. Bringa, E. M. Eberly, B. Graham, G. A. Remington, B. A. Taylor, E. A. Tielens, A. G. G. M. TI A new method to generate dust with astrophysical properties SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Plasma generation (laser-produced, RF, x ray-produced); Plasma diagnostics - high speed photography; Plasma diagnostics - interferometry, spectroscopy and imaging; Detector design and construction technologies and materials ID LOW-EARTH-ORBIT; HYPERVELOCITY IMPACT; INTERSTELLAR-MEDIUM; MOLECULAR-DYNAMICS; GRAIN DESTRUCTION; SIZE DISTRIBUTION; SPACE DEBRIS; SHOCK-WAVES; SOLAR-CELLS; CHEMISTRY AB To model the size distribution and composition of interstellar and interplanetary dust grains, and their effect on a wide range of phenomena, it is vital to understand the mechanism of dust-shock interaction. We demonstrate a new laser experiment that subjects dust grains to pressure spikes similar to those of colliding astrophysical dust, and that accelerates the grains to astrophysical velocities. This new method generates much larger data sets than earlier methods; we show how large quantities (thousands) of grains are accelerated at once, rather than accelerating individual grains, as is the case of earlier methods using electric fields. We also measure the in-flight velocity (similar to 4.5 km/s) of hundreds of grains simultaneously by use of a particle image velocimetry (PIV) technique. C1 [Hansen, J. F.; van Breugel, W.; Bringa, E. M.; Eberly, B.; Graham, G. A.; Remington, B. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Taylor, E. A.] Open Univ, Milton Keynes MK7 6BJ, Bucks, England. [Tielens, A. G. G. M.] Leiden Univ, Leiden Observ, NL-2300 RA Leiden, Netherlands. [van Breugel, W.] Univ Calif, Off Undergrad Educ, Merced, CA 95343 USA. [van Breugel, W.] Univ Calif, Sch Nat Sci, Merced, CA 95343 USA. [Bringa, E. M.] Univ Nacl Cuyo, CONICET, RA-5500 Mendoza, Argentina. [Bringa, E. M.] Univ Nacl Cuyo, Inst Ciencias Basicas, RA-5500 Mendoza, Argentina. [Graham, G. A.] Nat Hist Museum, Dept Mineral, London SW7 5BD, England. [Taylor, E. A.] MMI Engn Ltd, Warrington WA4 6HL, Cheshire, England. RP Hansen, JF (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM hansen46@llnl.gov RI Bringa, Eduardo/F-8918-2011 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX LLNL-JRNL-471526. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 42 TC 4 Z9 4 U1 0 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAY PY 2011 VL 6 AR P05010 DI 10.1088/1748-0221/6/05/P05010 PG 18 WC Instruments & Instrumentation SC Instruments & Instrumentation GA 814YA UT WOS:000294491900011 ER PT J AU Commer, M Newman, GA Williams, KH Hubbard, SS AF Commer, Michael Newman, Gregory A. Williams, Kenneth H. Hubbard, Susan S. TI 3D induced-polarization data inversion for complex resistivity SO GEOPHYSICS LA English DT Article ID SPECTRAL INDUCED POLARIZATION; REMOVAL; GROUNDWATER; FREQUENCY; EARTH AB The conductive and capacitive material properties of the subsurface can be quantified through the frequency-dependent complex resistivity. However, the routine three-dimensional (3D) interpretation of voluminous induced polarization (IP) data sets still poses a challenge due to large computational demands and solution nonuniqueness. We have developed a flexible methodology for 3D (spectral) IP data inversion. Our inversion algorithm is adapted from a frequency-domain electromagnetic (EM) inversion method primarily developed for large-scale hydrocarbon and geothermal energy exploration purposes. The method has proven to be efficient by implementing the nonlinear conjugate gradient method with hierarchical parallelism and by using an optimal finite-difference forward modeling mesh design scheme. The method allows for a large range of survey scales, providing a tool for both exploration and environmental applications. We experimented with an image focusing technique to improve the poor depth resolution of surface data sets with small survey spreads. The algorithm's underlying forward modeling operator properly accounts for EM coupling effects; thus, traditionally used EM coupling correction procedures are not needed. The methodology was applied to both synthetic and field data. We tested the benefit of directly inverting EM coupling contaminated data using a synthetic large-scale exploration data set. Afterward, we further tested the monitoring capability of our method by inverting time-lapse data from an environmental remediation experiment near Rifle, Colorado. Similar trends observed in both our solution and another 2D inversion were in accordance with previous findings about the IP effects due to subsurface microbial activity. C1 [Commer, Michael; Newman, Gregory A.; Williams, Kenneth H.; Hubbard, Susan S.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Commer, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM MCommer@lbl.gov; GANewman@lbl.gov; KHWil-liams@lbl.gov; SSHubbard@lbl.gov RI Hubbard, Susan/E-9508-2010; Williams, Kenneth/O-5181-2014; Newman, Gregory/G-2813-2015; Commer, Michael/G-3350-2015 OI Williams, Kenneth/0000-0002-3568-1155; Commer, Michael/0000-0003-0015-9217 FU United States Department of Energy, Office of Basic Energy Sciences [DE-AC02-05CH11231]; Biological and Environmental Research Program [DE-AC02-05CH11231] FX This work was carried out at Lawrence Berkeley National Laboratory, with partial funding provided by the United States Department of Energy, Office of Basic Energy Sciences, under contract DE-AC02-05CH11231, and from the Biological and Environmental Research Program under Contract DE-AC02-05CH11231 to the LBNL Sustainable Systems Scientific Focus Area. We thank Mike Wilkins, Hila Elifantz, Paula Mouser, and Lucie N'Guessan for their assistance with field experiments. We further thank Andreas Kemna for providing the employed 2D imaging code, and we thank Adrian Flores-Orozco for help with using the 2D code. NR 35 TC 12 Z9 15 U1 0 U2 14 PU SOC EXPLORATION GEOPHYSICISTS PI TULSA PA 8801 S YALE ST, TULSA, OK 74137 USA SN 0016-8033 J9 GEOPHYSICS JI Geophysics PD MAY-JUN PY 2011 VL 76 IS 3 BP F157 EP F171 DI 10.1190/1.3560156 PG 15 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 802PC UT WOS:000293522500017 ER PT J AU Nihei, KT Nakagawa, S Reverdy, F Myer, LR Duranti, L Ball, G AF Nihei, Kurt T. Nakagawa, Seiji Reverdy, Frederic Myer, Larry R. Duranti, Luca Ball, Greg TI Phased array compaction cell for measurement of the transversely isotropic elastic properties of compacting sediments SO GEOPHYSICS LA English DT Article ID SEISMIC ANISOTROPY; PREFERRED ORIENTATION; WAVE VELOCITIES; SHALES; KAOLINITE; FABRICS; ROCKS AB Sediments undergoing compaction typically exhibit transversely isotropic (TI) elastic properties. We present a new experimental apparatus, the phased array compaction cell, for measuring the TI elastic properties of clay-rich sediments during compaction. This apparatus uses matched sets of P- and S-wave ultrasonic transducers located along the sides of the sample and an ultrasonic P-wave phased array source, together with a miniature P-wave receiver on the top and bottom ends of the sample. The phased array measurements are used to form plane P-waves that provide estimates of the phase velocities over a range of angles. From these measurements, the five TI elastic constants can be recovered as the sediment is compacted, without the need for sample unloading, recoring, or reorienting. This paper provides descriptions of the apparatus, the data processing, and an application demonstrating recovery of the evolving TI properties of a compacting marine sediment sample. C1 [Nihei, Kurt T.; Duranti, Luca; Ball, Greg] Chevron ETC, Chevron, CA USA. [Nakagawa, Seiji; Myer, Larry R.] Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Reverdy, Frederic] CEA, Gif Sur Yvette, France. RP Nihei, KT (reprint author), Chevron ETC, Chevron, CA USA. EM knih@chevron.com; snakagawa@lbl.gov; frederic.reverdy@cea.fr; lrmyer@lbl.gov; ludu@chevron.com; bagj@chevron.com RI Nakagawa, Seiji/F-9080-2015; Nihei, Kurt/K-1239-2016 OI Nakagawa, Seiji/0000-0002-9347-0903; FU Assistant Secretary of Fossil Energy; U.S. Department of Energy [DE-AC03-76SF00098]; Chevron Energy Technology Company FX We gratefully acknowledge Don Sherlock, Russ Ewy, Rudy Wenk, Keith Katahara, Colin Sayers, and Michael Schoenberg for sharing their insights and expertise on clay-related anisotropy; Doug McCarty for performing the energy-dispersive X-ray spectroscopy and SEM; and Andrew Aplin for providing the X-ray goniometry measurements. We thank Chevron Deepwater Producing Operations for providing the Typhoon geotechnical core. We also thank the reviewers for improving the content and readability of this paper. This work was supported by the Assistant Secretary of Fossil Energy, U.S. Department of Energy under Contract No. DE-AC03-76SF00098, and the Chevron Energy Technology Company. NR 29 TC 1 Z9 1 U1 0 U2 10 PU SOC EXPLORATION GEOPHYSICISTS PI TULSA PA 8801 S YALE ST, TULSA, OK 74137 USA SN 0016-8033 J9 GEOPHYSICS JI Geophysics PD MAY-JUN PY 2011 VL 76 IS 3 BP WA113 EP WA123 DI 10.1190/1.3567160 PG 11 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 802PC UT WOS:000293522500044 ER PT J AU White, ER Mecklenburg, M Singer, SB Aloni, S Regan, BC AF White, Edward R. Mecklenburg, Matthew Singer, Scott B. Aloni, Shaul Regan, Brian Christopher TI Imaging Nanobubbles in Water with Scanning Transmission Electron Microscopy SO APPLIED PHYSICS EXPRESS LA English DT Article ID GROWTH; INTERFACE AB We present a technique based on scanning transmission electron microscopy (STEM) that is capable of probing nanobubble dynamics with nanometer spatial resolution. A vacuum-tight vessel holds a sub-micrometer layer of water between two electron-transparent dielectric membranes. Electrical current pulses passing through a platinum wire on one of the membranes inject sufficient heat locally to initiate single bubble formation. In the absence of power input, all bubbles are observed to be unstable against collapse, but the STEM beam alone can cause a shrinking bubble to grow. (C) 2011 The Japan Society of Applied Physics C1 [White, Edward R.; Mecklenburg, Matthew; Singer, Scott B.; Regan, Brian Christopher] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [White, Edward R.; Mecklenburg, Matthew; Singer, Scott B.; Regan, Brian Christopher] Univ Calif Los Angeles, Calif NanoSyst Inst, Los Angeles, CA 90095 USA. [Aloni, Shaul] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Mol Foundry, Berkeley, CA 94720 USA. RP White, ER (reprint author), Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. RI 骆, 庆群/C-3671-2012 FU NIH [1S10RR23057]; CNSI at UCLA; U.S. Department of Energy [DE-AC02-05CH11231]; The American Chemical Society; NSF [0748880] FX The authors acknowledge the Electron Imaging Center for NanoMachines supported by the NIH (1S10RR23057) and the CNSI at UCLA, and also the User Program at the Molecular Foundry of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Acknowledgment is made to the donors of The American Chemical Society Petroleum Research Fund for partial support of this research. This work was also supported in part by NSF CAREER grant No. 0748880. NR 18 TC 31 Z9 32 U1 5 U2 56 PU JAPAN SOC APPLIED PHYSICS PI TOKYO PA KUDAN-KITA BUILDING 5TH FLOOR, 1-12-3 KUDAN-KITA, CHIYODA-KU, TOKYO, 102-0073, JAPAN SN 1882-0778 J9 APPL PHYS EXPRESS JI Appl. Phys. Express PD MAY PY 2011 VL 4 IS 5 AR 055201 DI 10.1143/APEX.4.055201 PG 3 WC Physics, Applied SC Physics GA 802WP UT WOS:000293542000026 ER PT J AU Anagnostou, E Sherrell, RM Gagnon, A LaVigne, M Field, MP McDonough, WF AF Anagnostou, Eleni Sherrell, Robert M. Gagnon, Alex LaVigne, Michele Field, M. Paul McDonough, William F. TI Seawater nutrient and carbonate ion concentrations recorded as P/Ca, Ba/Ca, and U/Ca in the deep-sea coral Desmophyllum dianthus SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID ABLATION ICP-MS; PLASMA-MASS SPECTROMETRY; LASER-ABLATION; NORTH-ATLANTIC; ATMOSPHERIC-PRESSURE; CALCIUM-CARBONATE; SATURATION STATE; TRACE-ELEMENTS; SOUTHERN-OCEAN; WATER CORALS AB As paleoceanographic archives, deep sea coral skeletons offer the potential for high temporal resolution and precise absolute dating, but have not been fully investigated for geochemical reconstructions of past ocean conditions. Here we assess the utility of skeletal P/Ca, Ba/Ca and U/Ca in the deep sea coral D. dianthus as proxies of dissolved phosphate (remineralized at shallow depths), dissolved barium (trace element with silicate-type distribution) and carbonate ion concentrations, respectively. Measurements of these proxies in globally distributed D. dianthus specimens show clear dependence on corresponding seawater properties. Linear regression fits of mean coral Element/Ca ratios against seawater properties yield the equations: P/Ca(coral) (mu mol/mol) = (0.6 +/- 0.1) P/Ca(sw)(mu mol/mol) - (23 +/- 18), R(2) = 0.6, n = 16 and Ba/Ca(coral)(mu mol/mol) = (1.4 +/- 0.3) Ba/Ca(sw)(mu mol/mol) + (0 +/- 2), R(2) = 0.6, n = 17; no significant relationship is observed between the residuals of each regression and seawater temperature, salinity, pressure, pH or carbonate ion concentrations, suggesting that these variables were not significant secondary dependencies of these proxies. Four D. dianthus specimens growing at locations with Omega(arag) <= 0.6 displayed markedly depleted P/Ca compared to the regression based on the remaining samples, a behavior attributed to an undersaturation effect. These corals were excluded from the calibration. Coral U/Ca correlates with seawater carbonate ion: U/Ca(coral)(mu mol/mol) = (-0.016 +/- 0.003) [CO(3)(2-)] (mu mol/kg) + (3.2 +/- 0.3), R(2) = 0.6, n = 17. The residuals of the U/Ca calibration are not significantly related to temperature, salinity, or pressure. Scatter about the linear calibration lines is attributed to imperfect spatial-temporal matches between the selected globally distributed specimens and available water column chemical data, and potentially to unresolved additional effects. The uncertainties of these initial proxy calibration regressions predict that dissolved phosphate could be reconstructed to +/- 0.4 mu mol/kg (for 1.3-1.9 mu mol/kg phosphate), and dissolved Ba to +/- 19 nmol/kg (for 41-82 nmol/kg Ba(sw)). Carbonate ion concentration derived from U/Ca has an uncertainty of +/- 31 mu mol/kg (for 60-120 mu mol/kg CO(3)(2-)). The effect of microskeletal variability on P/Ca, Ba/Ca, and U/Ca was also assessed, with emphasis on centers of calcification, Fe-Mn phases, and external contaminants. Overall, the results show strong potential for reconstructing aspects of water mass mixing and biogeochemical processes in intermediate and deep waters using fossil deep-sea corals. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Anagnostou, Eleni; Sherrell, Robert M.; LaVigne, Michele; Field, M. Paul] Rutgers State Univ, Inst Marine & Coastal Sci, New Brunswick, NJ 08901 USA. [Sherrell, Robert M.] Rutgers State Univ, Dept Earth & Planetary Sci, Piscataway, NJ 08854 USA. [Gagnon, Alex] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [LaVigne, Michele] Univ Calif Davis, Bodega Marine Lab, Bodega Bay, CA 94923 USA. [McDonough, William F.] Univ Maryland, Dept Geol, College Pk, MD 20742 USA. RP Anagnostou, E (reprint author), Rutgers State Univ, Inst Marine & Coastal Sci, 71 Dudley Rd, New Brunswick, NJ 08901 USA. EM eleni@marine.rutgers.edu RI McDonough, William/C-4791-2009; McDonough, William/I-7720-2012; OI McDonough, William/0000-0001-9154-3673; McDonough, William/0000-0001-9154-3673; Anagnostou, Eleni/0000-0002-7200-4794 FU NSF [OCE 0752544, OCE 0962260] FX We thank Liz Sikes (Rutgers University) and Stephen Cairns (Smithsonian Institute) for providing corals for this work. Also we are indebted to Yair Rosenthal for extensive advice and Paolo Montagna for thoughtful discussions. We thank Associate Editor Anne Cohen and the anonymous reviewers for their significant help in improving this manuscript. This work was supported by Grants to RMS from NSF Chemical Oceanography (OCE 0752544) and Marine Geology and Geophysics (OCE 0962260). NR 93 TC 28 Z9 29 U1 5 U2 34 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD MAY 1 PY 2011 VL 75 IS 9 BP 2529 EP 2543 DI 10.1016/j.gca.2011.02.019 PG 15 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 796EK UT WOS:000293033300019 ER PT J AU Michael, JR AF Michael, Joseph R. TI High Resolution at Low Beam Energy in the SEM: Resolution Measurement of a Monochromated SEM SO SCANNING LA English DT Article DE SEM; resolution; monochromator; CTF ID SCANNING ELECTRON-MICROSCOPY AB The resolution of secondary electron low beam energy imaging of a scanning electron microscope equipped with a monochromator is quantitatively measured using the contrast transfer function (CTF) method. High-resolution images, with sub-nm resolutions, were produced using low beam energies. The use of a monochromator is shown to quantitatively improve the resolution of the SEM at low beam energies by limiting the chromatic aberration contribution to the electron probe size as demonstrated with calculations and images of suitable samples. Secondary electron image resolution at low beam energies is ultimately limited by noise in the images as shown by the CTFs. SCANNING 33: 147-154, 2011. (C) 2011 Wiley Periodicals, Inc. C1 Sandia Natl Labs, Mat Characterizat Dept, Albuquerque, NM 87185 USA. RP Michael, JR (reprint author), Sandia Natl Labs, Mat Characterizat Dept, POB 5800,MS 0886, Albuquerque, NM 87185 USA. EM jrmicha@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The author would first and very gratefully acknowledge the many enlightening discussions on topics in microscopy with David Joy over the past 30 years and for the calculations of the electron distributions in probes. The author has had many fruitful and engaging discussions on the topic of SEM performance with Brendan Griffin. Helpful discussions with Richard Young, Laurent Roussel, Sander Henstra and Ingo Gestmann of FEI are acknowledged. The expert maintenance of the SEM by Richard Grant is acknowledged. Thanks to Ronin Polsky for supplying the pyrolized photoresist samples. Sandia National Laboratories is a multi-program laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 21 TC 4 Z9 4 U1 0 U2 4 PU WILEY-BLACKWELL PI MALDEN PA COMMERCE PLACE, 350 MAIN ST, MALDEN 02148, MA USA SN 0161-0457 J9 SCANNING JI Scanning PD MAY-JUN PY 2011 VL 33 IS 3 SI SI BP 147 EP 154 DI 10.1002/sca.20254 PG 8 WC Instruments & Instrumentation; Microscopy SC Instruments & Instrumentation; Microscopy GA 801QK UT WOS:000293455100006 PM 21674539 ER PT J AU Mills, E AF Mills, Evan TI Building commissioning: a golden opportunity for reducing energy costs and greenhouse gas emissions in the United States SO ENERGY EFFICIENCY LA English DT Review DE Energy efficiency; Commissioning; Commercial buildings; Risk management; Quality assurance; Carbon reductions; Savings persistence AB Commissioning is arguably the single most cost-effective strategy for reducing energy, costs, and greenhouse gas emissions in buildings today. Although commissioning has earned increased recognition in recent years, it remains an enigmatic practice whose visibility severely lags its potential. The application of commissioning to new buildings ensures that they deliver or exceed the performance and energy savings promised by their design and intended operation. When applied to existing buildings, commissioning identifies deficiencies and the almost inevitable "drift" from intended performance over time, and carries out interventions to put the building back on course. More formally, commissioning is a systematic, forensic approach to quality assurance and performance risk management, rather than a technology per se. This article presents the world's largest compilation and meta-analysis of commissioning experience and the associated literature, comprising 643 non-residential buildings, 99 million ft(2) of floorspace, $43 million in commissioning expenditures, and the work of 37 commissioning providers. The median normalized cost to deliver commissioning is $0.30/ft(2) ($ 2009 currencies) for existing buildings and $ 1.16/ft(2) for new construction (or 0.4% of the overall construction cost). The one third of projects for which data are available reveal over 10,000 energy-related deficiencies, the correction of which resulted in 16% median whole-building energy savings in existing buildings and 13% in new construction, with payback times of 1.1 and 4.2 years, respectively. Because energy savings exceed commissioning costs, the associated reductions in greenhouse gas emissions come at a "negative" cost of -$110/tonne CO(2) for new buildings and -$25/tonne for new construction. Cases with comprehensive commissioning attained nearly twice the overall median level of savings and five times the savings of the least-thorough projects. Significant non-energy benefits such as improved indoor air quality are also achieved. Applying the median whole-building energy-saving values to the US non-residential buildings stock corresponds to an annual energy-saving potential of $30 billion (and 340 Mt of CO(2)) by the year 2030. C1 Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. RP Mills, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM emills@lbl.gov FU California Energy Commission through the US Department of Energy [DE-AC02-05CH11231] FX Sponsored by the California Energy Commission, Public Interest Energy Research Program (PIER), through the US Department of Energy under contract no. DE-AC02-05CH11231. This report would not have been possible without the support of my insightful and patient sponsors at PIER: Martha Brook and Norman Bourassa (Buildings) and Paul Roggensack and Pramod Kulkarni (Industry). This work expands significantly on a report originally published in 2004 with co-authors Hannah Friedman, Tehesia Powell, Norman Bourassa, David Claridge, Tudi Haasl, and Mary Ann Piette, who helped to build the original analysis framework and case-study database. Comments from two anonymous reviewers were appreciated. NR 54 TC 18 Z9 18 U1 5 U2 19 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1570-646X J9 ENERG EFFIC JI Energy Effic. PD MAY PY 2011 VL 4 IS 2 BP 145 EP 173 DI 10.1007/s12053-011-9116-8 PG 29 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Environmental Studies SC Science & Technology - Other Topics; Energy & Fuels; Environmental Sciences & Ecology GA 796RA UT WOS:000293068200002 ER PT J AU Babentsov, V Boiko, V Schepelskii, GA James, RB Franc, J Prochazka, J Hlidek, P AF Babentsov, V. Boiko, V. Schepelskii, G. A. James, R. B. Franc, J. Prochazka, J. Hlidek, P. TI Dislocation-induced electronic levels in semi-insulated CdTe SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 11th International Workshop on Radiation Imaging Detectors CY JUN 29-JUL 03, 2009 CL Czech Technical Univ, Inst Experimental & Applied Phys, Prague, CZECH REPUBLIC HO Czech Technical Univ, Inst Experimental & Applied Phys DE CdTe; Detectors; Dislocations ID CADMIUM ZINC TELLURIDE; SINGLE-CRYSTALS; CD0.96ZN0.04TE; RADIATION; PHOTOLUMINESCENCE; ABSORPTION; EMISSION; DEFECTS AB We studied deformation-induced defects in semi-insulating CdTe and CdZnTe by infrared photoluminescence (PL) and compared our data with earlier results. We confirmed the direct correlation between Y-emission and dislocation density in both compounds. The Y-band intensified near an indenter deformation or near a scribing line, but was barely visible in low-dislocation areas (etch pit density <2 x 10(5) cm(-2)). Plastic deformation also increased the concentrations of grown-in defects, namely, those of an important midgap level E(C)-0.74 eV in CdTe and Cd(1-x)Zn(x)Te (x < 0.1), the materials of choice in today's detector technology. Our findings demonstrate that dislocation-induced defects can degrade charge collection in radiation detectors. (C) 2010 Elsevier B.V. All rights reserved. C1 [Babentsov, V.; Boiko, V.; Schepelskii, G. A.] Natl Acad Sci, Inst Semicond Phys, UA-03028 Kiev, Ukraine. [James, R. B.] Brookhaven Natl Lab, Nonproliferat & Natl Secur Dept, Upton, NY 11973 USA. [Franc, J.; Prochazka, J.; Hlidek, P.] Charles Univ Prague, Inst Phys, Fac Math & Phys, CZ-12116 Prague, Czech Republic. RP Babentsov, V (reprint author), Natl Acad Sci, Inst Semicond Phys, UA-03028 Kiev, Ukraine. EM babentsov@isp.kiev.ua RI Franc, Jan/C-3802-2017 OI Franc, Jan/0000-0002-9493-3973 NR 15 TC 8 Z9 8 U1 1 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAY PY 2011 VL 633 SU 1 BP S81 EP S82 DI 10.1016/j.nima.2010.06.129 PG 2 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 792WZ UT WOS:000292782400024 ER PT J AU Hwang, O Kim, S Suh, J Cho, S Kim, K Hong, J Kim, S AF Hwang, OhHyeon Kim, SangSu Suh, JongHee Cho, ShinHang Kim, KiHyun Hong, JinKi Kim, SunUng TI Effect of thermal annealing of lead oxide film SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 11th International Workshop on Radiation Imaging Detectors CY JUN 29-JUL 03, 2009 CL Czech Technical Univ, Inst Experimental & Applied Phys, Prague, CZECH REPUBLIC HO Czech Technical Univ, Inst Experimental & Applied Phys DE Direct conversion; Lead oxide; PbO; X-ray detector ID MONOXIDE AB Oxygen partial pressure in a growth process of lead oxide determines chemical and physical properties as well as crystalline structure. In order to supply oxygen, two ring-shape suppliers have been installed in a growth chamber. Films have been deposited using vacuum thermal evaporation from a raw material of yellow lead oxide powder (5N). Growth rate is controlled to be about 400 angstrom/s, and film thickness more than 50 mu m has been achieved. After deposition, the film is annealed at various temperatures under an oxygen atmosphere. In this study, an optimum growth condition for a good X-ray detector has been achieved by fine control of oxygen flow-rate and by thermal treatment. An electrical resistivity of 4.5 x 10(12) Omega cm is measured, and is comparable with the best data of PbO. (C) 2010 Published by Elsevier B.V. C1 [Hwang, OhHyeon; Kim, SangSu; Suh, JongHee; Cho, ShinHang; Hong, JinKi; Kim, SunUng] Korea Univ, Dept Display & Semicond Phys, Chungnam 339700, South Korea. [Kim, KiHyun] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Kim, S (reprint author), Korea Univ, Dept Display & Semicond Phys, Chungnam 339700, South Korea. EM ksu45112@chollian.net; ksu45112@chollian.net NR 11 TC 3 Z9 4 U1 1 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAY PY 2011 VL 633 SU 1 BP S69 EP S71 DI 10.1016/j.nima.2010.06.125 PG 3 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 792WZ UT WOS:000292782400020 ER PT J AU Pinsky, LS Empl, A Gutierrez, A Jakubek, J Kitamura, H Miller, J Leroy, C Stoffle, N Pospisil, S Uchihori, Y Yasuda, N Zeitlin, C AF Pinsky, Lawrence S. Empl, Anton Gutierrez, Andrea Jakubek, Jan Kitamura, Hisashi Miller, Jack Leroy, Claude Stoffle, Nicholas Pospisil, Stanislav Uchihori, Yukio Yasuda, Nakahiro Zeitlin, Cary TI Penetrating heavy ion charge and velocity discrimination with a TimePix-based Si detector (for space radiation applications) SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 11th International Workshop on Radiation Imaging Detectors CY JUN 29-JUL 03, 2009 CL Czech Technical Univ, Inst Experimental & Applied Phys, Prague, CZECH REPUBLIC HO Czech Technical Univ, Inst Experimental & Applied Phys DE Charged particle detector; Pixel detector; Position sensitive detector; Medipix AB Exposures were made with Medipix2 TimePix-based Si detectors at the HIMAC facility in Japan to explore the potential for discrimination between tracks with differing charges and energies, but with very similar dE/dx values. Data were taken at 15 degrees increments for a number of different beams including 600 and 800 MeV/A Si, 180 MeV/A Ne and 100 MeV/A O. Data were also obtained for 400 MeV/A Si and 500 MeV/A Fe along with 290 and 180 MeV/A N. The TimePix chips have been calibrated to achieve the maximum resolution. Estimates for the angular resolution for these types of tracks are also possible from these data, which are essential in the development of a TimePix-based dosimetric device for use in a space radiation environment. One of the principal objectives of these data runs was to explore the resolution of TimePix-based Si detectors to discriminate between various ions with different energies and charges, but with similar dE/dx values in Si. Analysis of the images obtained shows the clear differences in the delta-ray halos for particles with similar dE/dx values but for differing charges and energies. These measurements are part of an ongoing program to explore the range of capabilities of the TimePix-based detector with respect to dosimetry uses in space. (C) 2010 Elsevier B.V. All rights reserved. C1 [Pinsky, Lawrence S.; Empl, Anton; Stoffle, Nicholas] Univ Houston, Houston, TX 77204 USA. [Gutierrez, Andrea; Leroy, Claude] Univ Montreal, Montreal, PQ H3T 1J4, Canada. [Jakubek, Jan; Pospisil, Stanislav] Czech Tech Univ, Inst Expt & Appl Phys, CZ-12800 Prague 2, Albertov, Czech Republic. [Kitamura, Hisashi; Uchihori, Yukio; Yasuda, Nakahiro] Natl Inst Radiol Sci, Inage Ku, Chiba 2638555, Japan. [Miller, Jack] Univ Calif Berkeley, Lawrence Berkeley Lab, Space Sci Lab, Berkeley, CA 94720 USA. [Zeitlin, Cary] SW Res Inst, San Antonio, TX 78238 USA. RP Pinsky, LS (reprint author), Univ Houston, 4800 Calhoun Blvd, Houston, TX 77204 USA. EM pinsky@uh.edu RI Jakubek, Jan/E-6530-2011 NR 4 TC 4 Z9 4 U1 2 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAY PY 2011 VL 633 SU 1 BP S190 EP S193 DI 10.1016/j.nima.2010.06.164 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 792WZ UT WOS:000292782400058 ER PT J AU Durso, AM Willson, JD Winne, CT AF Durso, Andrew M. Willson, John D. Winne, Christopher T. TI Needles in haystacks: Estimating detection probability and occupancy of rare and cryptic snakes SO BIOLOGICAL CONSERVATION LA English DT Article DE Aquatic snakes; Detectability estimates; Habitat use; Program PRESENCE; Site occupancy modeling; Wetland ID ESTIMATING SITE OCCUPANCY; SPECIES RICHNESS; PRESENCE-ABSENCE; ISOLATED WETLAND; DETECTABILITY; DISTRIBUTIONS; POPULATION; AMPHIBIANS; ABUNDANCE; SALAMANDERS AB The species most in need of conservation or management are often also the most difficult to monitor, because of their rarity, secretive habits, or both. To combat these challenges, presence/absence (site occupancy) models can be used to track species occupancy at landscape scales. However, quantitative knowledge of detection probability (which is almost always <1) is required to reliably estimate site occupancy. Here, we present a case study that combines detection probabilities and site occupancy modeling to monitor a notoriously secretive guild of animals, North American aquatic snakes. Specifically, we use program PRESENCE to estimate detection probability (p) and probability of site occupancy (psi) for seven snake species in relationship to site covariates, to understand the proximate and ultimate factors that influence habitat suitability. We were able to estimate p (3-46%) and psi (12-96%) for each species and calculate the amount of unsuccessful effort necessary to declare absence of each species with statistical confidence (5-63 visits: 150-1890 trap-nights). We documented considerable interspecific variation in p and psi; one species (Nerodia fasciata) was widespread and highly detectable, while another (Agkistrodon piscivorus) had low detectability despite its wide distribution. Five other species were secretive, or restricted to specific habitat types, or both, illustrating that complex and sometimes counterintuitive relationships exist between capture rate and occupancy. Incorporating p and psi is essential to the success of large-scale monitoring programs for elusive species. (C) 2011 Elsevier Ltd. All rights reserved. C1 Univ Georgia, Odum Sch Ecol, Athens, GA 30602 USA. Savannah River Ecol Lab, Aiken, SC 29802 USA. RP Durso, AM (reprint author), Eastern Illinois Univ, Dept Biol Sci, Charleston, IL 61920 USA. EM amdurso@gmail.com; willsonj@vt.edu; ctwinne@gmail.com RI Durso, Andrew/D-1657-2012; OI Durso, Andrew/0000-0002-3008-7763 FU National Science Foundation; Department of Energy [DE-FC09-96SR18546] FX We would like to acknowledge the faculty and staff at the Savannah River Ecology Lab, especially J. Whitfield Gibbons, Judy Greene, Deno Karapatakis and Lindy Steadman. We also thank the following individuals for their assistance with field work: Kevin P. Durso, Sandy Durso, Evan A. Eskew, Chad A. Jennison, Tom M. Luhring, Rebecca L Maska and Anna McKee; with data analysis: Greg Anderson, Robert J. Cooper, Mary C. Freeman, Scott J. Meiners and Todd Rasmussen: and for provisioning us with over a decade of hydrologic data: Evelyn Gaiser, Robert Lide and Ken McLeod. J.W. Gibbons, the Eastern Illinois University herpetology lab and one anonymous reviewer provided comments which improved the manuscript. This work was supported by the National Science Foundation through the Research Experiences for Undergraduates (REU) program to AMD and a Graduate Research Fellowship to JDW, and was supported by the Department of Energy under Award Number DE-FC09-96SR18546 to the University of Georgia Research Foundation. Animals were collected under South Carolina Department of Natural Resources scientific collection permits (G-06-04), and procedures used in the study were approved by the University of Georgia animal care and use committee (A2006-10069-0). NR 74 TC 31 Z9 34 U1 2 U2 54 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0006-3207 EI 1873-2917 J9 BIOL CONSERV JI Biol. Conserv. PD MAY PY 2011 VL 144 IS 5 BP 1508 EP 1515 DI 10.1016/j.biocon.2011.01.020 PG 8 WC Biodiversity Conservation; Ecology; Environmental Sciences SC Biodiversity & Conservation; Environmental Sciences & Ecology GA 791MB UT WOS:000292668200032 ER PT J AU Oh, JH Yoo, BG Choi, IC Santella, ML Jang, JI AF Oh, Jun-Hak Yoo, Byung-Gil Choi, In-Chul Santella, Michael L. Jang, Jae-il TI Influence of thermo-mechanical treatment on the precipitation strengthening behavior of Inconel 740, a Ni-based superalloy SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID PARTICLE HARDENING MECHANISMS; MICROSTRUCTURE; DISLOCATIONS; SIMULATIONS; STRESS; STEEL; TEMPERATURE; STABILITY; KINETICS; ALLOYS AB In this work, we have systematically explored the influence of thermo-mechanical treatment on the precipitation behavior and its strengthening in Inconel 740, a relatively new Ni-based superalloy, using specimens on which different levels of stresses were applied at 700 degrees C. With increasing applied stress, fraction of gamma prime precipitates increased (without significant size change) and nanoindentation hardness was enhanced. The stress effects were discussed in terms of the free energy barrier for heterogeneous nucleation and the prevailing mechanisms of precipitation strengthening. C1 [Oh, Jun-Hak; Yoo, Byung-Gil; Choi, In-Chul; Jang, Jae-il] Hanyang Univ, Div Mat Sci & Engn, Seoul 133791, South Korea. [Santella, Michael L.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Jang, JI (reprint author), Hanyang Univ, Div Mat Sci & Engn, Seoul 133791, South Korea. EM jijang@hanyang.ac.kr RI Jang, Jae-il/A-3486-2011; Choi, In-Chul/E-1499-2014 OI Jang, Jae-il/0000-0003-4526-5355; FU Korea government Ministry of Knowledge Economy [20101020300460] FX This work was supported by the Human Resources Development of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by the Korea government Ministry of Knowledge Economy (No. 20101020300460). NR 26 TC 11 Z9 13 U1 3 U2 13 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 J9 J MATER RES JI J. Mater. Res. PD MAY PY 2011 VL 26 IS 10 BP 1253 EP 1259 DI 10.1557/jmr.2011.70 PG 7 WC Materials Science, Multidisciplinary SC Materials Science GA 793NV UT WOS:000292831300009 ER PT J AU Bennett, CJC Kim, HS Varela, M Biegalski, MD Kim, DH Norton, DP Meyer, HM Christen, HM AF Bennett, Charlee J. C. Kim, Hyun Sik Varela, Maria Biegalski, Michael D. Kim, Dae Ho Norton, David P. Meyer, Harry M., III Christen, Hans M. TI Compositional tuning of the strain-induced structural phase transition and of ferromagnetism in Bi1-xBaxFeO3-delta SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID THIN-FILMS; BIFEO3; BAFEO3-X AB Recent studies by a number of research groups have shown that the structure of epitaxial BiFeO3 (BFO) films changes drastically as a function of substrate-induced biaxial compression, with the crystal structure changing from one being nearly rhombohedral (R-like) to one being nearly tetragonal (T-like), where the "T-like" structure is characterized by a highly enhanced c/a ratio of out-of-plane c to in-plane a lattice parameters. In this work, we show that the critical compressive strain sigma(c) necessary to induce this transition can be reduced significantly by substituting 10% Ba for Bi [Bi0.9Ba0.1FeO3-delta (BBFO)] and that the "T-like" phase in both BBFO and BFO is stable up to the decomposition temperatures of the films in air. Furthermore, our results show that the BBFO solid solution shows clear ferromagnetic properties in contrast to its undoped BFO counterpart. C1 [Bennett, Charlee J. C.; Kim, Hyun Sik; Varela, Maria; Kim, Dae Ho; Meyer, Harry M., III; Christen, Hans M.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Biegalski, Michael D.; Christen, Hans M.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Kim, Hyun Sik] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kim, Dae Ho] Tulane Univ, Dept Phys, New Orleans, LA 70118 USA. [Norton, David P.] Univ Florida, Dept Mat Sci & Engn, Gainesville, FL 32611 USA. RP Christen, HM (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM christenhm@ornl.gov RI Kim, Dae Ho/B-4670-2012; Varela, Maria/H-2648-2012; Christen, Hans/H-6551-2013; Varela, Maria/E-2472-2014 OI Christen, Hans/0000-0001-8187-7469; Varela, Maria/0000-0002-6582-7004 FU U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; Scientific User Facilities Division; Army Research Office; National Science Foundation [0704240] FX This research was supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division (C.J.C.B., H.S.K., M.V., H.M.M., and H.M.C.), and Scientific User Facilities Division (M.D.B.). D.P.N. acknowledges support by Army Research Office and National Science Foundation under Grant No. 0704240 (AFH). We thank J.T. Luck for specimen preparation. NR 28 TC 15 Z9 15 U1 1 U2 21 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 J9 J MATER RES JI J. Mater. Res. PD MAY PY 2011 VL 26 IS 10 BP 1326 EP 1331 DI 10.1557/jmr.2011.59 PG 6 WC Materials Science, Multidisciplinary SC Materials Science GA 793NV UT WOS:000292831300018 ER PT J AU Challa, SR Song, YJ Shelnutt, JA Miller, JE van Swol, F AF Challa, Sivakumar R. Song, Yujiang Shelnutt, John A. Miller, James E. van Swol, Frank TI Evolution of dendritic nanosheets into durable holey sheets: a lattice gas simulation study SO JOURNAL OF PORPHYRINS AND PHTHALOCYANINES LA English DT Article DE ripening; Monte Carlo simulations; platinum nanostructure; electrocatalyst ID PEM FUEL-CELLS; MONTE-CARLO; ISING-MODEL; PLATINUM; CATALYSTS; NANOCLUSTERS; DURABILITY; CATHODE; MICROSTRUCTURES; NANOSTRUCTURES AB Monte Carlo lattice gas simulations are performed to study sintering in a realistic dendritic platinum nanosheet. The morphological and topological transformations observed in the simulations are in good agreement with sintering experiments. Employing an intuitive method of quantifying surface area, the stability of the surface area of the dendritic nanosheets is analyzed. The surface area is found to have a double exponential decay, one decay corresponding to rapid coarsening of dendritic features into pores and the other decay corresponding to a slow disappearance of unstable pores. Long duration simulations indicate that the thickness of the dendritic nanosheet remains fairly stable. Stability simulations of a single model pore in a sheet establish that there exists a narrow range of sheet thickness and pore size combinations that produces stable holey sheets. Outside this parameter range pores either rapidly close or expand without bound. The thickness of the engineered dendritic platinum nanosheet and the size of the crevices between dendritic arms put the Pt sheet into this stable range, further corroborating the detailed simulations and explaining the persistence of pores observed in actual dendritic platinum nanosheets. C1 [Challa, Sivakumar R.; van Swol, Frank] Univ New Mexico, Dept Chem & Nucl Engn, Ctr Microengineered Mat, Albuquerque, NM 87131 USA. [Song, Yujiang; Shelnutt, John A.; Miller, James E.; van Swol, Frank] Sandia Natl Labs, Adv Mat Lab, Albuquerque, NM 87106 USA. RP van Swol, F (reprint author), Univ New Mexico, Dept Chem & Nucl Engn, Ctr Microengineered Mat, Albuquerque, NM 87131 USA. EM vanswol@unm.edu RI Miller, James/C-1128-2011; Song, Yujiang/A-8700-2009 OI Miller, James/0000-0001-6811-6948; FU UNM Center [2005006]; US DOE [DE-AC04-94AL85000] FX We thank Craig J. Medforth for helpful discussions, and acknowledge the computational support from the UNM Center for High Performance Computing under Grant No. 2005006. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed-Martin Company, for the US DOE under Contract No. DE-AC04-94AL85000. NR 33 TC 3 Z9 3 U1 1 U2 16 PU WORLD SCI PUBL CO INC PI HACKENSACK PA 27 WARREN ST, STE 401-402, HACKENSACK, NJ 07601 USA SN 1088-4246 J9 J PORPHYR PHTHALOCYA JI J. Porphyr. Phthalocyanines PD MAY-JUN PY 2011 VL 15 IS 5-6 BP 449 EP 458 DI 10.1142/S1088424611003409 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA 791EK UT WOS:000292646900016 ER PT J AU Airapetian, A Akopov, N Akopov, Z Aschenauer, EC Augustyniak, W Avakian, R Avetissian, A Avetisyan, E Belostotski, S Bianchi, N Blok, HP Borissov, A Bowles, J Bryzgalov, V Burns, J Capiluppi, M Capitani, GP Cisbani, E Ciullo, G Contalbrigo, M Dalpiaz, PF Deconinck, W De Leo, R De Nardo, L Sanctis, E Diefenthaler, M Di Nezza, P Duren, M Ehrenfried, M Elbakian, G Ellinghaus, F Fabbri, R Fantoni, A Felawka, L Frullani, S Gabbert, D Gapienko, G Gapienko, V Garibaldi, F Gavrilov, G Gharibyan, V Giordano, F Gliske, S Golembiovskaya, M Hadjidakis, C Hartig, M Hasch, D Hill, G Hillenbrand, A Hoek, M Holler, Y Hristova, I Imazu, Y Ivanilov, A Jackson, HE Jo, HS Joosten, S Kaiser, R Karyan, G Keri, T Kinney, E Kisselev, A Korotkov, V Kozlov, V Kravchenko, P Krivokhijine, VG Lagamba, L Lamb, R Lapikas, L Lehmann, I Lenisa, P Linden-Levy, LA Ruiz, AL Lorenzon, W Lu, XG Lu, XR Ma, BQ Mahon, D Makins, NCR Manaenkov, SI Manfre, L Mao, Y Marianski, B de la Ossa, AM Marukyan, H Miller, CA Miyachi, Y Movsisyan, A Muccifora, V Murray, M Mussgiller, A Nappi, E Naryshkin, Y Nass, A Negodaev, M Nowak, WD Pappalardo, LL Perez-Benito, R Pickert, N Raithel, M Reimer, PE Reolon, AR Riedl, C Rith, K Rosner, G Rostomyan, A Rubin, J Ryckbosch, D Salomatin, Y Sanftl, F Schafer, A Schnell, G Schuler, KP Seitz, B Shibata, TA Shutov, V Stancari, M Statera, M Steffens, E Steijger, JJM Stenzel, H Stewart, J Stinzing, F Taroian, S Trzcinski, A Tytgat, M Vandenbroucke, A Van Haarlem, Y Van Hulse, C Veretennikov, D Vikhrov, V Vilardi, I Vogel, C Wang, S Yaschenko, S Ye, H Ye, Z Yen, S Yu, W Zeiler, D Zihlmann, B Zupranski, P AF Airapetian, A. Akopov, N. Akopov, Z. Aschenauer, E. C. Augustyniak, W. Avakian, R. Avetissian, A. Avetisyan, E. Belostotski, S. Bianchi, N. Blok, H. P. Borissov, A. Bowles, J. Bryzgalov, V. Burns, J. Capiluppi, M. Capitani, G. P. Cisbani, E. Ciullo, G. Contalbrigo, M. Dalpiaz, P. F. Deconinck, W. De Leo, R. De Nardo, L. De Sanctis, E. Diefenthaler, M. Di Nezza, P. Dueren, M. Ehrenfried, M. Elbakian, G. Ellinghaus, F. Fabbri, R. Fantoni, A. Felawka, L. Frullani, S. Gabbert, D. Gapienko, G. Gapienko, V. Garibaldi, F. Gavrilov, G. Gharibyan, V. Giordano, F. Gliske, S. Golembiovskaya, M. Hadjidakis, C. Hartig, M. Hasch, D. Hill, G. Hillenbrand, A. Hoek, M. Holler, Y. Hristova, I. Imazu, Y. Ivanilov, A. Jackson, H. E. Jo, H. S. Joosten, S. Kaiser, R. Karyan, G. Keri, T. Kinney, E. Kisselev, A. Korotkov, V. Kozlov, V. Kravchenko, P. Krivokhijine, V. G. Lagamba, L. Lamb, R. Lapikas, L. Lehmann, I. Lenisa, P. Linden-Levy, L. A. Ruiz, A. Lopez Lorenzon, W. Lu, X. -G. Lu, X. -R. Ma, B. -Q. Mahon, D. Makins, N. C. R. Manaenkov, S. I. Manfre, L. Mao, Y. Marianski, B. de la Ossa, A. Martinez Marukyan, H. Miller, C. A. Miyachi, Y. Movsisyan, A. Muccifora, V. Murray, M. Mussgiller, A. Nappi, E. Naryshkin, Y. Nass, A. Negodaev, M. Nowak, W. -D. Pappalardo, L. L. Perez-Benito, R. Pickert, N. Raithel, M. Reimer, P. E. Reolon, A. R. Riedl, C. Rith, K. Rosner, G. Rostomyan, A. Rubin, J. Ryckbosch, D. Salomatin, Y. Sanftl, F. Schaefer, A. Schnell, G. Schueler, K. P. Seitz, B. Shibata, T. -A. Shutov, V. Stancari, M. Statera, M. Steffens, E. Steijger, J. J. M. Stenzel, H. Stewart, J. Stinzing, F. Taroian, S. Trzcinski, A. Tytgat, M. Vandenbroucke, A. Van Haarlem, Y. Van Hulse, C. Veretennikov, D. Vikhrov, V. Vilardi, I. Vogel, C. Wang, S. Yaschenko, S. Ye, H. Ye, Z. Yen, S. Yu, W. Zeiler, D. Zihlmann, B. Zupranski, P. CA HERMES Collaboration TI Inclusive measurements of inelastic electron and positron scattering from unpolarized hydrogen and deuterium targets SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Lepton-Nucleon Scattering ID CURRENT CROSS-SECTIONS; STRUCTURE-FUNCTION F-2; MUON SCATTERING; LOW Q(2); LOW-X; PROTON COLLISIONS; RATIO F2(N)/F2(P); E(+)P SCATTERING; QCD ANALYSIS; HERA AB Results of inclusive measurements of inelastic electron and positron scattering from unpolarized protons and deuterons at the HERMES experiment are presented. The structure functions F-2(p) and F-2(d) are determined using a parameterization of existing data for the longitudinal-to-transverse virtual-photon absorption cross-section ratio. The HERMES results provide data in the ranges 0.006 <= x <= 0.9 and 0.1 GeV2 <= Q(2) <= 20 GeV2, covering the transition region between the perturbative and the non-perturbative regimes of QCD in a so-far largely unexplored kinematic region. They are in agreement with existing world data in the region of overlap. The measured cross sections are used, in combination with data from other experiments, to perform fits to the photon-nucleon cross section using the functional form of the ALLM model. The deuteron-to-proton cross-section ratio is also determined. C1 [Jackson, H. E.; Reimer, P. E.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [De Leo, R.; Lagamba, L.; Nappi, E.; Vilardi, I.] Ist Nazl Fis Nucl, Sez Bari, I-70124 Bari, Italy. [Ma, B. -Q.; Mao, Y.; Wang, S.; Ye, H.] Peking Univ, Sch Phys, Beijing 100871, Peoples R China. [Ellinghaus, F.; Kinney, E.; de la Ossa, A. Martinez] Univ Colorado, Nucl Phys Lab, Boulder, CO 80309 USA. [Akopov, Z.; Avetisyan, E.; Borissov, A.; Deconinck, W.; De Nardo, L.; Gavrilov, G.; Giordano, F.; Hartig, M.; Holler, Y.; Mussgiller, A.; Rostomyan, A.; Schueler, K. P.; Ye, Z.; Zihlmann, B.] DESY, D-22603 Hamburg, Germany. [Aschenauer, E. C.; Fabbri, R.; Gabbert, D.; Golembiovskaya, M.; Hillenbrand, A.; Hristova, I.; Lu, X. -G.; Negodaev, M.; Nowak, W. -D.; Riedl, C.; Schnell, G.; Stewart, J.; Yaschenko, S.] DESY, D-15738 Zeuthen, Germany. [Krivokhijine, V. G.; Shutov, V.] Joint Inst Nucl Res, Dubna 141980, Russia. [Diefenthaler, M.; Kravchenko, P.; de la Ossa, A. Martinez; Mussgiller, A.; Nass, A.; Pickert, N.; Raithel, M.; Rith, K.; Steffens, E.; Stinzing, F.; Vogel, C.; Yaschenko, S.; Zeiler, D.] Univ Erlangen Nurnberg, Inst Phys, D-91058 Erlangen, Germany. [Capiluppi, M.; Ciullo, G.; Contalbrigo, M.; Dalpiaz, P. F.; Giordano, F.; Lenisa, P.; Pappalardo, L. L.; Stancari, M.; Statera, M.] Univ Ferrara, Ist Nazl Fis Nucl, Sez Ferrara, I-44100 Ferrara, Italy. [Capiluppi, M.; Ciullo, G.; Contalbrigo, M.; Dalpiaz, P. F.; Giordano, F.; Lenisa, P.; Pappalardo, L. L.; Stancari, M.; Statera, M.] Univ Ferrara, Dipartimento Fis, I-44100 Ferrara, Italy. [Bianchi, N.; Capitani, G. P.; De Sanctis, E.; Di Nezza, P.; Fantoni, A.; Hadjidakis, C.; Hasch, D.; Muccifora, V.; Reolon, A. R.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [De Nardo, L.; Jo, H. S.; Joosten, S.; Ruiz, A. Lopez; Ryckbosch, D.; Schnell, G.; Tytgat, M.; Vandenbroucke, A.; Van Haarlem, Y.; Van Hulse, C.] Univ Ghent, Dept Subat & Radiat Phys, B-9000 Ghent, Belgium. [Airapetian, A.; Dueren, M.; Ehrenfried, M.; Keri, T.; Perez-Benito, R.; Stenzel, H.; Yu, W.] Univ Giessen, Inst Phys, D-35392 Giessen, Germany. [Bowles, J.; Burns, J.; Hill, G.; Hoek, M.; Kaiser, R.; Keri, T.; Lehmann, I.; Mahon, D.; Murray, M.; Rosner, G.; Seitz, B.] Univ Glasgow, Dept Phys & Astron, Glasgow G12 8QQ, Lanark, Scotland. [Diefenthaler, M.; Joosten, S.; Lamb, R.; Linden-Levy, L. A.; Makins, N. C. R.; Rubin, J.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Airapetian, A.; Gliske, S.; Lorenzon, W.] Univ Michigan, Randall Lab Phys, Ann Arbor, MI 48109 USA. [Kozlov, V.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Blok, H. P.; Lapikas, L.; Steijger, J. J. M.] Natl Inst Subat Phys Nikhef, NL-1009 DB Amsterdam, Netherlands. [Belostotski, S.; Gavrilov, G.; Kisselev, A.; Kravchenko, P.; Manaenkov, S. I.; Naryshkin, Y.; Veretennikov, D.; Vikhrov, V.] Petersburg Nucl Phys Inst, Gatchina 188300, Leningrad Reg, Russia. [Bryzgalov, V.; Gapienko, G.; Gapienko, V.; Ivanilov, A.; Korotkov, V.; Salomatin, Y.] Inst High Energy Phys, Protvino 142281, Russia. [Sanftl, F.; Schaefer, A.] Univ Regensburg, Inst Theoret Phys, D-93040 Regensburg, Germany. [Cisbani, E.; Frullani, S.; Garibaldi, F.; Manfre, L.] Ist Nazl Fis Nucl, Sez Roma, Grp Collegato Sanita, I-00161 Rome, Italy. [Cisbani, E.; Frullani, S.; Garibaldi, F.; Manfre, L.] Ist Super Sanita, I-00161 Rome, Italy. [Felawka, L.; Gavrilov, G.; Miller, C. A.; Yen, S.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Imazu, Y.; Lu, X. -R.; Miyachi, Y.; Sanftl, F.; Shibata, T. -A.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [Blok, H. P.] Vrije Univ Amsterdam, Dept Phys, NL-1081 HV Amsterdam, Netherlands. [Augustyniak, W.; Marianski, B.; Trzcinski, A.; Zupranski, P.] Andrzej Soltan Inst Nucl Studies, PL-00689 Warsaw, Poland. [Akopov, N.; Avakian, R.; Avetissian, A.; Elbakian, G.; Gharibyan, V.; Karyan, G.; Marukyan, H.; Movsisyan, A.; Taroian, S.] Yerevan Phys Inst, Yerevan 375036, Armenia. RP Airapetian, A (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. EM klaus.rith@desy.de RI Gavrilov, Gennady/C-6260-2013; Reimer, Paul/E-2223-2013; Negodaev, Mikhail/A-7026-2014; Taroian, Sarkis/E-1668-2014; Kozlov, Valentin/M-8000-2015 FU DESY management; Ministry of Economy; Ministry of Education and Science of Armenia; FWO-Flanders and IWT, Belgium; Natural Sciences and Engineering Research Council of Canada; National Natural Science Foundation of China; Alexander von Humboldt Stiftung; German Bundesministerium fur Bildung und Forschung (BMBF); Deutsche Forschungsgemeinschaft (DFG); Italian Istituto Nazionale di Fisica Nucleare (INFN); MEXT; JSPS; G-COE of Japan; Dutch Foundation for Fundamenteel Onderzoek der Materie (FOM); Russian Academy of Science; Russian Federal Agency for Science and Innovations; U.K. Engineering and Physical Sciences Research Council; Science and Technology Facilities Council; Scottish Universities Physics Alliance; U.S. Department of Energy (DOE); National Science Foundation (NSF); Basque Foundation for Science (IKERBASQUE); European Community [227431] FX We gratefully acknowledge the DESY management for its support and the staff at DESY and the collaborating institutions for their significant effort. This work was supported by the Ministry of Economy and the Ministry of Education and Science of Armenia; the FWO-Flanders and IWT, Belgium; the Natural Sciences and Engineering Research Council of Canada; the National Natural Science Foundation of China; the Alexander von Humboldt Stiftung, the German Bundesministerium fur Bildung und Forschung (BMBF), and the Deutsche Forschungsgemeinschaft (DFG); the Italian Istituto Nazionale di Fisica Nucleare (INFN); the MEXT, JSPS, and G-COE of Japan; the Dutch Foundation for Fundamenteel Onderzoek der Materie (FOM); the Russian Academy of Science and the Russian Federal Agency for Science and Innovations; the U.K. Engineering and Physical Sciences Research Council, the Science and Technology Facilities Council, and the Scottish Universities Physics Alliance; the U.S. Department of Energy (DOE) and the National Science Foundation (NSF); the Basque Foundation for Science (IKERBASQUE); and the European Community Research Infrastructure Integrating Activity under the FP7 "Study of Strongly Interacting Matter (HadronPhysics2, Grant Agreement number 227431)". NR 53 TC 6 Z9 6 U1 1 U2 13 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY PY 2011 IS 5 AR 126 DI 10.1007/JHEP05(2011)126 PG 40 WC Physics, Particles & Fields SC Physics GA 774EN UT WOS:000291364500058 ER PT J AU Bustamante, M Gago, AM Perez, JJ AF Bustamante, M. Gago, A. M. Jones Perez, J. TI SUSY renormalization group effects in ultra high energy neutrinos SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Neutrino Physics; Supersymmetric Standard Model; Renormalization Group ID MASS OPERATOR RENORMALIZATION; FLAVOR RATIOS; MODELS; GAMMA; MSSM AB We have explored the question of whether the renormalization group running of the neutrino mixing parameters in the Minimal Supersymmetric Standard Model is detectable with ultra-high energy neutrinos from active galactic nuclei (AGN). We use as observables the ratios of neutrino fluxes produced at the AGN, focusing on four different neutrino production models: (Phi(0)(v epsilon+(v) over bar epsilon) : Phi(0)(v mu+(v) over bar mu) : Phi(0)(v tau+(v) over bar tau)) = (1 : 2 : 0), (0 : 1 : 0), (1 : 0 : 0), and (1 : 1 : 0). The prospects for observing deviations experimentally are taken into consideration, and we find out that it is necessary to impose a cut-off on the transferred momentum of Q(2) >= 10(7) GeV2. However, this condition, together with the expected low value of the diffuse AGN neutrino flux, yields a negligible event rate at a km-scale. Cerenkov detector such as IceCube. C1 [Bustamante, M.; Gago, A. M.] Pontificia Univ Catolica Peru, Dept Ciencias, Sec Fis, Lima, Peru. [Bustamante, M.] Fermilab Natl Accelerator Lab, Theoret Phys Dept, Batavia, IL 60510 USA. [Jones Perez, J.] Univ Valencia, Dept Fis Teor, CSIC, E-46100 Burjassot, Spain. [Jones Perez, J.] Univ Valencia, IFIC, CSIC, E-46100 Burjassot, Spain. [Jones Perez, J.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. RP Bustamante, M (reprint author), Pontificia Univ Catolica Peru, Dept Ciencias, Sec Fis, Apartado 1761, Lima, Peru. EM mbustamante@pucp.edu.pe; agago@pucp.edu.pe; joel.jones@lnf.infn.it OI Gago Medina, Alberto Martin/0000-0002-0019-9692; Jones-Perez, Joel/0000-0002-2037-6369; Bustamante, Mauricio/0000-0001-6923-0865 FU Vicerrectorado de Investigacion at PUCP [DGI-2010-0021]; Spanish MICINN; EC [FPA2008-02878]; ALFA-EC FX The work of M. B. and A. M. G. was supported by the Vicerrectorado de Investigacion at PUCP through Grant No. DGI-2010-0021. J. J. P. would like to thank Takashi Shimomura, Oscar Vives, Jose Bernabeu and particularly Arcadi Santamaria for fruitful discussions. He would also like to thank the Pontificia Universidad Catolica del Peru (PUCP) for its warm hospitality during his visit. The work of J. J. P. was partially supported by the Spanish MICINN and FEDER (EC) Grant No. FPA2008-02878. This work was made possible by the partial support of ALFA-EC funds in the framework of the HELEN Project. NR 60 TC 1 Z9 1 U1 0 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY PY 2011 IS 5 AR 133 DI 10.1007/JHEP05(2011)133 PG 26 WC Physics, Particles & Fields SC Physics GA 774EN UT WOS:000291364500065 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hammer, J Hansel, S Hoch, M Hormann, N Hrubec, J Jeitler, M Kasieczka, G Kiesenhofer, W Krammer, M Liko, D Mikulec, I Pernicka, M Rohringer, H Schofbeck, R Strauss, J Teischinger, F Wagner, P Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Benucci, L De Wolf, EA Janssen, X Maes, T Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Blekman, F Blyweert, S D'Hondt, J Devroede, O Suarez, RG Kalogeropoulos, A Maes, J Maes, M Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Charaf, O Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hammad, GH Hreus, T Marage, PE Thomas, L Velde, CV Vanlaer, P Adler, V Cimmino, A Costantini, S Grunewald, M Klein, B Lellouch, J Marinov, A Mccartin, J Ryckbosch, D Thyssen, F Tytgat, M Vanelderen, L Verwilligen, P Walsh, S Zaganidis, N Basegmez, S Bruno, G Caudron, J Ceard, L Gil, EC De Jeneret, JD Delaere, C Favart, D Giammanco, A Gregoire, G Hollar, J Lemaitre, V Liao, J Militaru, O Ovyn, S Pagano, D Pin, A Piotrzkowski, K Schul, N Beliy, N Caebergs, T Daubie, E Alves, GA Damiao, DD Pol, ME Souza, MHG Carvalho, W Da Costa, EM Martins, CD De Souza, SF Mundim, L Nogima, H Oguri, V Da Silva, WLP Santoro, A Do Amaral, SMS Sznajder, A De Araujo, FTD Dias, FA Tomei, TRFP Gregores, EM Lagana, C Marinho, F Mercadante, PG Novaes, SF Padula, SS Darmenov, N Dimitrov, L Genchev, V Iaydjiev, P Piperov, S Rodozov, M Stoykova, S Sultanov, G Tcholakov, V Trayanov, R Vankov, I Dimitrov, A Hadjiiska, R Karadzhinova, A Kozhuharov, V Litov, L Mateev, M Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, J Wang, J Wang, X Wang, Z Xiao, H Xu, M Zang, J Zhang, Z Ban, Y Guo, S Guo, Y Li, W Mao, Y Qian, SJ Teng, H Zhang, L Zhu, B Zou, W Cabrera, A Moreno, BG Rios, AAO Oliveros, AFO Sanabria, JC Godinovic, N Lelas, D Lelas, K Plestina, R Polic, D Puljak, I Antunovic, Z Dzelalija, M Brigljevic, V Duric, S Kadija, K Morovic, S Attikis, A Galanti, M Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Assran, Y Khalil, S Mahmoud, MA Hektor, A Kadastik, M Muntel, M Raidal, M Rebane, L Azzolini, V Eerola, P Fedi, G Czellar, S Harkonen, J Heikkinen, A Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Tuominen, E Tuominiemi, J Tuovinen, E Ungaro, D Wendland, L Banzuzi, K Korpela, A Tuuva, T Sillou, D Besancon, M Choudhury, S Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Gentit, FX Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Marionneau, M Millischer, L Rander, J Rosowsky, A Shreyber, I Titov, M Verrecchia, P Baffioni, S Beaudette, F Benhabib, L Bianchini, L Bluj, M Broutin, C Busson, P Charlot, C Dahms, T Dobrzynski, L Elgammal, S de Cassagnac, RG Haguenauer, M Mine, P Mironov, C Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Thiebaux, C Wyslouch, B Zabi, A Agram, JL Andrea, J Bloch, D Bodin, D Brom, JM Cardaci, M Chabert, EC Collard, C Conte, E Drouhin, F Ferro, C Fontaine, JC Gele, D Goerlach, U Greder, S Juillot, P Karim, M Le Bihan, AC Mikami, Y Van Hove, P Fassi, F Mercier, D Baty, C Beauceron, S Beaupere, N Bedjidian, M Bondu, O Boudoul, G Boumediene, D Brun, H Chierici, R Contardo, D Depasse, P El Mamouni, H Fay, J Gascon, S Ille, B Kurca, T Le Grand, T Lethuillier, M Mirabito, L Perries, S Sordini, V Tosi, S Tschudi, Y Verdier, P Lomidze, D Anagnostou, G Edelhoff, M Feld, L Heracleous, N Hindrichs, O Jussen, R Klein, K Merz, J Mohr, N Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Weber, M Wittmer, B Ata, M Bender, W Dietz-Laursonn, E Erdmann, M Frangenheim, J Hebbeker, 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Lungu, G. Malik, S. Mesropian, C. Yan, M. Atramentov, O. Barker, A. Duggan, D. Gershtein, Y. Gray, R. Halkiadakis, E. Hidas, D. Hits, D. Lath, A. Panwalkar, S. Patel, R. Richards, A. Rose, K. Schnetzer, S. Somalwar, S. Stone, R. Thomas, S. Cerizza, G. Hollingsworth, M. Spanier, S. Yang, Z. C. York, A. Asaadi, J. Eusebi, R. Gilmore, J. Gurrola, A. Kamon, T. Khotilovich, V. Montalvo, R. Nguyen, C. N. Osipenkov, I. Pakhotin, Y. Pivarski, J. Safonov, A. Sengupta, S. Tatarinov, A. Toback, D. Weinberger, M. Akchurin, N. Bardak, C. Damgov, J. Jeong, C. Kovitanggoon, K. Lee, S. W. Roh, Y. Sill, A. Volobouev, I. Wigmans, R. Yazgan, E. Appelt, E. Brownson, E. Engh, D. Florez, C. Gabella, W. Issah, M. Johns, W. Kurt, P. Maguire, C. Melo, A. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Balazs, M. Boutle, S. Cox, B. Francis, B. Hirosky, R. Ledovskoy, A. Lin, C. Neu, C. Yohay, R. Gollapinni, S. Harr, R. Karchin, P. E. Lamichhane, P. Mattson, M. Milstene, C. Sakharov, A. Anderson, M. Bachtis, M. Bellinger, J. N. Carlsmith, D. Dasu, S. Efron, J. Flood, K. Gray, L. Grogg, K. S. Grothe, M. Hall-Wilton, R. Herndon, M. Klabbers, P. Klukas, J. Lanaro, A. Lazaridis, C. Leonard, J. Loveless, R. Mohapatra, A. Palmonari, F. Reeder, D. Ross, I. Savin, A. Smith, W. H. Swanson, J. Weinberg, M. CA CMS Collaboration TI Search for resonances in the dilepton mass distribution in pp collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID FERMION-PAIR PRODUCTION; E(+)E(-) COLLISIONS; STANDARD MODEL; LEP; CONSTRAINTS; PHYSICS; HADRON AB A search for narrow resonances at high mass in the dimuon and dielectron channels has been performed by the CMS experiment at the CERN LHC, using pp collision data recorded at root s = 7 TeV. The event samples correspond to integrated luminosities of 40 pb(-1) in the dimuon channel and 35 pb(-1) in the dielectron channel. Heavy dilepton resonances are predicted in theoretical models with extra gauge bosons (Z') or as Kaluza-Klein graviton excitations (G(KK)) in the Randall-Sundrum model. Upper limits on the inclusive cross section of Z'(GKK) -> l + l(-) relative to Z -> l + l(-) are presented. These limits exclude at 95% confidence level a Z' with standard-model-like couplings below 1140 GeV, the superstring-inspired Z'(psi) below 887 GeV, and, for values of the coupling parameter k/(M) over bar (Pl) of 0.05 (0.1), Kaluza-Klein gravitons below 855 (1079) GeV. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hammer, J.; Haensel, S.; Hoch, M.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kasieczka, G.; Kiesenhofer, W.; Krammer, M.; Liko, D.; Mikulec, I.; Pernicka, M.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Teischinger, F.; Wagner, P.; Waltenberger, W.; Walzel, G.; Widl, E.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Benucci, L.; De Wolf, E. A.; Janssen, X.; Maes, T.; Mucibello, L.; Ochesanu, S.; Roland, B.; Rougny, R.; Selvaggi, M.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.] Univ Antwerp, B-2020 Antwerp, Belgium. [Blekman, F.; Blyweert, S.; D'Hondt, J.; Devroede, O.; Suarez, R. Gonzalez; Kalogeropoulos, A.; Maes, J.; Maes, M.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Villella, I.] Vrije Univ Brussel, Brussels, Belgium. [Charaf, O.; Clerbaux, B.; De Lentdecker, G.; Dero, V.; Gay, A. P. R.; Hammad, G. H.; Hreus, T.; Marage, P. E.; Thomas, L.; Velde, C. Vander; Vanlaer, P.] Univ Libre Bruxelles, Brussels, Belgium. [Adler, V.; Cimmino, A.; Costantini, S.; Grunewald, M.; Klein, B.; Lellouch, J.; Marinov, A.; Mccartin, J.; Ryckbosch, D.; Thyssen, F.; Tytgat, M.; Vanelderen, L.; Verwilligen, P.; Walsh, S.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Bruno, G.; Caudron, J.; Ceard, L.; Gil, E. Cortina; De Jeneret, J. De Favereau; Delaere, C.; Favart, D.; Giammanco, A.; Gregoire, G.; Hollar, J.; Lemaitre, V.; Liao, J.; Militaru, O.; Ovyn, S.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Schul, N.] Catholic Univ Louvain, B-1348 Louvain, Belgium. [Beliy, N.; Caebergs, T.; Daubie, E.] Univ Mons, B-7000 Mons, Belgium. [Alves, G. A.; De Jesus Damiao, D.; Pol, M. E.; Souza, M. H. G.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Carvalho, W.; Da Costa, E. M.; De Oliveira Martins, C.; Fonseca De Souza, S.; Mundim, L.; Nogima, H.; Oguri, V.; Prado Da Silva, W. L.; Santoro, A.; Silva Do Amaral, S. M.; Sznajder, A.; Torres Da Silva De Araujo, F.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Dias, F. A.; Fernandez Perez Tomei, T. R.; Gregores, E. M.; Lagana, C.; Marinho, F.; Mercadante, P. G.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Inst Fis Teor, BR-01405 Sao Paulo, Brazil. [Darmenov, N.; Dimitrov, L.; Genchev, V.; Iaydjiev, P.; Piperov, S.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Tcholakov, V.; Trayanov, R.; Vankov, I.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Dimitrov, A.; Hadjiiska, R.; Karadzhinova, A.; Kozhuharov, V.; Litov, L.; Mateev, M.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Bian, J. G.; Chen, G. M.; Chen, H. S.; Jiang, C. H.; Liang, D.; Liang, S.; Meng, X.; Tao, J.; Wang, J.; Wang, X.; Wang, Z.; Xiao, H.; Xu, M.; Zang, J.; Zhang, Z.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Ban, Y.; Guo, S.; Guo, Y.; Li, W.; Mao, Y.; Qian, S. J.; Teng, H.; Zhang, L.; Zhu, B.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Tech, Beijing 100871, Peoples R China. [Cabrera, A.; Gomez Moreno, B.; Ocampo Rios, A. A.; Osorio Oliveros, A. F.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Lelas, K.; Plestina, R.; Polic, D.; Puljak, I.] Tech Univ Split, Split, Croatia. [Antunovic, Z.; Dzelalija, M.] Univ Split, Split, Croatia. [Brigljevic, V.; Duric, S.; Kadija, K.; Morovic, S.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Galanti, M.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.] Univ Cyprus, Nicosia, Cyprus. [Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Assran, Y.; Khalil, S.; Mahmoud, M. A.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt. [Hektor, A.; Kadastik, M.; Muentel, M.; Raidal, M.; Rebane, L.] NICPB, Tallinn, Estonia. [Azzolini, V.; Eerola, P.; Fedi, G.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Czellar, S.; Harkonen, J.; Heikkinen, A.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Ungaro, D.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Banzuzi, K.; Korpela, A.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Sillou, D.] CNRS, IN2P3, Lab Annecy le Vieux Phys Particules, Annecy Le Vieux, France. [Besancon, M.; Choudhury, S.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Ferri, F.; Ganjour, S.; Gentit, F. X.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Marionneau, M.; Millischer, L.; Rander, J.; Rosowsky, A.; Shreyber, I.; Titov, M.; Verrecchia, P.] CEA Saclay, IRFU, DSM, F-91191 Gif Sur Yvette, France. [Plestina, R.; Baffioni, S.; Beaudette, F.; Benhabib, L.; Bianchini, L.; Bluj, M.; Broutin, C.; Busson, P.; Charlot, C.; Dahms, T.; Dobrzynski, L.; Elgammal, S.; de Cassagnac, R. Granier; Haguenauer, M.; Mine, P.; Mironov, C.; Ochando, C.; Paganini, P.; Sabes, D.; Salerno, R.; Sirois, Y.; Thiebaux, C.; Wyslouch, B.; Zabi, A.; Bernet, C.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Agram, J. -L.; Andrea, J.; Bloch, D.; Bodin, D.; Brom, J. -M.; Cardaci, M.; Chabert, E. C.; Collard, C.; Conte, E.; Drouhin, F.; Ferro, C.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Greder, S.; Juillot, P.; Karim, M.; Le Bihan, A. -C.; Mikami, Y.; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, CNRS, Inst Pluridisciplinaire Hubert Curien,IN2P3, Strasbourg, France. [Fassi, F.; Mercier, D.] IN2P3, Ctr Calcul, Villeurbanne, France. [Baty, C.; Beauceron, S.; Beaupere, N.; Bedjidian, M.; Bondu, O.; Boudoul, G.; Boumediene, D.; Brun, H.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fay, J.; Gascon, S.; Ille, B.; Kurca, T.; Le Grand, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Sordini, V.; Tosi, S.; Tschudi, Y.; Verdier, P.] Univ Lyon 1, CNRS, IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Lomidze, D.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Anagnostou, G.; Edelhoff, M.; Feld, L.; Heracleous, N.; Hindrichs, O.; Jussen, R.; Klein, K.; Merz, J.; Mohr, N.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Weber, M.; Wittmer, B.] Rhein Westfal TH Aachen, Phys Inst 1, Aachen, Germany. [Ata, M.; Bender, W.; Dietz-Laursonn, E.; Erdmann, M.; Frangenheim, J.; Hebbeker, T.; Hinzmann, A.; Hoepfner, K.; Klimkovich, T.; Klingebiel, D.; Kreuzer, P.; Lanske, D.; Magass, C.; Merschmeyer, M.; Meyer, A.; Papacz, P.; Pieta, H.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Steggemann, J.; Teyssier, D.; Tonutti, M.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Bontenackels, M.; Davids, M.; Duda, M.; Fluegge, G.; Geenen, H.; Giffels, M.; Ahmad, W. Haj; Heydhausen, D.; Kress, T.; Kuessel, Y.; Linn, A.; Nowack, A.; Perchalla, L.; Pooth, O.; Rennefeld, J.; Sauerland, P.; Stahl, A.; Thomas, M.; Tornier, D.; Zoeller, M. H.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Martin, M. Aldaya; Behrenhoff, W.; Behrens, U.; Bergholz, M.; Bethani, A.; Borras, K.; Cakir, A.; Campbell, A.; Castro, E.; Dammann, D.; Eckerlin, G.; Eckstein, D.; Flossdorf, A.; Flucke, G.; Geiser, A.; Hauk, J.; Jung, H.; Kasemann, M.; Katkov, I.; Katsas, P.; Kleinwort, C.; Kluge, H.; Knutsson, A.; Kraemer, M.; Kruecker, D.; Kuznetsova, E.; Lange, W.; Lohmann, W.; Mankel, R.; Marienfeld, M.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Olzem, J.; Pitzl, D.; Raspereza, A.; Raval, A.; Rosin, M.; Schmidt, R.; Schoerner-Sadenius, T.; Sen, N.; Spiridonov, A.; Stein, M.; Tomaszewska, J.; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Autermann, C.; Blobel, V.; Bobrovskyi, S.; Draeger, J.; Enderle, H.; Gebbert, U.; Kaschube, K.; Kaussen, G.; Klanner, R.; Lange, J.; Mura, B.; Naumann-Emme, S.; Nowak, F.; Pietsch, N.; Sander, C.; Schettler, H.; Schleper, P.; Schroeder, M.; Schum, T.; Schwandt, J.; Stadie, H.; Steinbrueck, G.; Thomsen, J.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Bauer, J.; Buege, V.; Chwalek, T.; De Boer, W.; Dierlamm, A.; Dirkes, G.; Feindt, M.; Gruschke, J.; Hackstein, C.; Hartmann, F.; Heinrich, M.; Held, H.; Hoffmann, K. H.; Honc, S.; Komaragiri, J. R.; Kuhr, T.; Martschei, D.; Mueller, S.; Mueller, Th.; Niegel, M.; Oberst, O.; Oehler, A.; Ott, J.; Peiffer, T.; Piparo, D.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Ratnikova, N.; Renz, M.; Saout, C.; Scheurer, A.; Schieferdecker, P.; Schilling, F. -P.; Schmanau, M.; Schott, G.; Simonis, H. J.; Stober, F. M.; Troendle, D.; Wagner-Kuhr, J.; Weiler, T.; Zeise, M.; Zhukov, V.; Ziebarth, E. B.] Univ Karlsruhe, Inst Expt Kernphys, D-7500 Karlsruhe, Germany. [Daskalakis, G.; Geralis, T.; Karafasoulis, K.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Manolakos, I.; Markou, A.; Markou, C.; Mavrommatis, C.; Ntomari, E.; Petrakou, E.] Inst Nucl Phys Demokritos, Aghia Paraskevi, Greece. [Gouskos, L.; Mertzimekis, T. J.; Panagiotou, A.; Stiliaris, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Evangelou, I.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Patras, V.; Triantis, F. A.] Univ Ioannina, GR-45110 Ioannina, Greece. [Aranyi, A.; Bencze, G.; Boldizsar, L.; Hajdu, C.; Hidas, P.; Horvath, D.; Kapusi, A.; Krajczar, K.; Sikler, F.; Veres, G. I.; Vesztergombi, G.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Molnar, J.; Palinkas, J.; Szillasi, Z.; Veszpremi, V.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Jindal, M.; Kaur, M.; Kohli, J. M.; Mehta, M. Z.; Nishu, N.; Saini, L. K.; Sharma, A.; Singh, A. P.; Singh, J. B.; Singh, S. P.] Panjab Univ, Chandigarh 160014, India. [Ahuja, S.; Bhattacharya, S.; Choudhary, B. C.; Gupta, P.; Jain, S.; Jain, S.; Kumar, A.; Ranjan, K.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Choudhury, R. K.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Guchait, M.; Gurtu, A.; Maity, M.; Majumder, D.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Saha, A.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res, EHEP, Bombay 400005, Maharashtra, India. [Guchait, M.; Banerjee, S.; Dugad, S.; Mondal, N. K.] Tata Inst Fundamental Res, HECR, Bombay 400005, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Hashemi, M.; Jafari, A.; Khakzad, M.; Mohammadi, A.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res & Fundamental Sci IPM, Tehran, Iran. [Abbrescia, M.; Barbone, L.; Calabria, C.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Lusito, L.; Maggi, G.; Maggi, M.; Manna, N.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pierro, G. A.; Pompili, A.; Pugliese, G.; Romano, F.; Roselli, G.; Selvaggi, G.; Silvestris, L.; Trentadue, R.; Tupputi, S.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; De Palma, M.; Lusito, L.; Manna, N.; Marangelli, B.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Roselli, G.; Selvaggi, G.; Tupputi, S.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.; Romano, F.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Giunta, M.; Marcellini, S.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Braibant-Giacomelli, S.; Capiluppi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Meneghelli, M.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Tricomi, A.] Univ Catania, Catania, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Tricomi, A.; Tuve, C.; Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Tricomi, A.; Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Lenzi, P.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Colafranceschi, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Ghezzi, A.; Malvezzi, S.; Martelli, A.; Massironi, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; Sala, S.; de Fatis, T. Tabarelli; Tancini, V.] Ist Nazl Fis Nucl, Sez Milano Biccoca, I-20133 Milan, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Ghezzi, A.; Martelli, A.; Massironi, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli; Tancini, V.] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Montoya, C. A. Carrillo; Cavallo, N.; De Cosa, A.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [De Cosa, A.; Merola, M.] Univ Naples Federico II, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bellan, P.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; De Mattia, M.; Dorigo, T.; Dosselli, U.; Fanzago, F.; Gasparini, F.; Gasparini, U.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Mazzucato, M.; Meneguzzo, A. T.; Nespolo, M.; Perrozzi, L.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, I-35100 Padua, Italy. [Bellan, P.; Bisello, D.; Carlin, R.; De Mattia, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Univ Padua, Padua, Italy. [Lazzizzera, I.] Univ Trento, Padua, Italy. [Baesso, P.; Berzano, U.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.; Viviani, C.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Baesso, P.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.; Viviani, C.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Caponeri, B.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Santocchia, A.; Taroni, S.; Valdata, M.; Pioppi, M.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Caponeri, B.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Taroni, S.; Valdata, M.; Pioppi, M.] Univ Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Segneri, G.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, I-56010 Pisa, Italy. [Bernardini, J.; Fiori, F.; Messineo, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Azzurri, P.; Broccolo, G.; D'Agnolo, R. T.; Foa, L.; Ligabue, F.; Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Di Marco, E.; Diemoz, M.; Franci, D.; Grassi, M.; Longo, E.; Nourbakhsh, S.; Organtini, G.; Pandolfi, F.; Paramatti, R.; Rahatlou, S.; Rovelli, C.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Colafranceschi, S.] Univ Roma La Sapienza, Fac Ingn, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Botta, C.; Cartiglia, N.; Castello, R.; Costa, M.; Demaria, N.; Graziano, A.; Mariotti, C.; Marone, M.; Maselli, S.; Migliore, E.; Mila, G.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Romero, A.; Ruspa, M.; Sacchi, R.; Sola, V.; Solano, A.; Staiano, A.; Pereira, A. Vilela] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Botta, C.; Castello, R.; Costa, M.; Graziano, A.; Marone, M.; Migliore, E.; Mila, G.; Monaco, V.; Musich, M.; Pelliccioni, M.; Romero, A.; Sacchi, R.; Sola, V.; Solano, A.; Pereira, A. Vilela] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Cossutti, F.; Della Ricca, G.; Gobboa, B.; Montanino, D.; Penzo, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Della Ricca, G.; Montanino, D.] Univ Trieste, Trieste, Italy. [Heo, S. G.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Chung, J.; Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Park, H.; Ro, S. R.; Son, D.; Son, D. C.; Son, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, Zero; Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Hong, B.; Jeong, M. S.; Jo, M.; Kim, H.; Kim, J. H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.; Rhee, H. B.; Seo, E.; Shin, S.; Sim, K. S.] Korea Univ, Seoul, South Korea. [Aranyi, A.; Choi, M.; Kang, S.; Kim, H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Martisiute, D.; Petrov, P.; Sabonis, T.] Vilnius Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Lopez-Fernandez, R.; Magana Villalba, R.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.; Tam, J.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ahmed, I.; Asghar, M. I.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Brona, G.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bluj, M.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Soltan Inst Nucl Studies, PL-00681 Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Musella, P.; Nayak, A.; Seixas, J.; Varela, J.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Belotelov, I.; Bunin, P.; Golutvin, I.; Kamenev, A.; Karjavin, V.; Kozlov, G.; Lanev, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Toropin, A.; Troitsky, S.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Kaftanov, V.; Kossov, M.; Krokhotin, A.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Katkov, I.; Zhukov, V.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Sarycheva, L.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Azhgirey, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Slabospitsky, S.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Arce, P.; Battilana, C.; Calvo, E.; Cepeda, M.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Diez Pardos, C.; Dominguez Vazquez, D.; Bedoya, C. Fernandez; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Jorda, C.; Lobelle Pardo, P.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Hammer, J.; Delaere, C.; Darmenov, N.; Genchev, V.; Jung, H.; Hajdu, C.; Sikler, F.; Mohanty, A. K.; De Filippis, N.; Tropiano, A.; De Guio, F.; Montoya, C. A. Carrillo; Iorio, A. O. M.; Nespolo, M.; Perrozzi, L.; Lucaroni, A.; Taroni, S.; Boccali, T.; Tonelli, G.; Venturi, A.; Grassi, M.; Pandolfi, F.; Botta, C.; Graziano, A.; Kossov, M.; Grishin, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Baillon, P.; Ball, A. H.; Barney, D.; Bell, A. J.; Benedetti, D.; Bernet, C.; Bialas, W.; Bloch, P.; Bocci, A.; Bolognesi, S.; Bona, M.; Breuker, H.; Bunkowski, K.; Camporesi, T.; Cerminara, G.; Perez, A. Coarasa; Cure, B.; D'Enterria, D.; De Roeck, A.; Di Guida, S.; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Gaddi, A.; Gennai, S.; Georgiou, G.; Gerwig, H.; Gigi, D.; Gill, K.; Giordano, D.; Glege, F.; Garrido, R. Gomez-Reino; Gouzevitch, M.; Govoni, P.; Gowdy, S.; Guiducci, L.; Hansen, M.; Hartl, C.; Harvey, J.; Hegeman, J.; Hegner, B.; Hoffmann, H. F.; Honma, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Lecoq, P.; Lourenco, C.; Maeki, T.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Maurisset, A.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Nesvold, E.; Nguyen, M.; Orimoto, T.; Orsini, L.; Perez, E.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Polese, G.; Racz, A.; Antunes, J. Rodrigues; Rolandi, G.; Rommerskirchen, T.; Rovelli, C.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Segoni, I.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiropulu, M.; Stoye, M.; Tropea, P.; Tsirou, A.; Vichoudis, P.; Voutilainen, M.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Starodumov, A.; Caminada, L.; Marchica, C.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bortignon, P.; Caminada, L.; Chanon, N.; Chen, Z.; Cittolin, S.; Dissertori, G.; Dittmar, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Herve, A.; Hintz, W.; Lecomte, P.; Lustermann, W.; Marchica, C.; Del Arbol, P. Martinez Ruiz; Meridiani, P.; Milenovic, P.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pape, L.; Pauss, F.; Punz, T.; Rizzi, A.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Sawley, M. -C.; Stieger, B.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, M.; Wehrli, L.; Weng, J.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Aguilo, E.; Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Otiougova, P.; Regenfus, C.; Robmann, P.; Schmidt, A.; Snoek, H.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Volpe, R.; Wu, J. H.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Topaksu, A. Kayis; Nart, A.; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Uzun, D.; Vergili, L. N.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Deliomeroglu, M.; Demir, D.; Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Levchuk, L.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Bostock, F.; Brooke, J. J.; Cheng, T. L.; Clement, E.; Cussans, D.; Frazier, R.; Goldstein, J.; Grimes, M.; Hansen, M.; Hartley, D.; Heath, G. P.; Heath, H. F.; Jackson, J.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Ward, S.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Camanzi, B.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.; Accomando, E.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Ballin, J.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Lyons, L.; MacEvoy, B. C.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rompotis, N.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Tourneur, S.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Wardrope, D.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Basso, L.; Belyaev, A.; Accomando, E.; King, S.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Barrett, M.; Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Martin, W.; Reid, I. D.; Teodorescu, L.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.] Baylor Univ, Waco, TX 76798 USA. [Bose, T.; Jarrin, E. Carrera; Fantasia, C.; Heister, A.; John, J. St.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Avetisyan, A.; Bhattacharya, S.; Chou, J. P.; Cutts, D.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Landsberg, G.; Narain, M.; Nguyen, D.; Segala, M.; Sinthuprasith, T.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Cox, P. T.; Dolen, J.; Erbacher, R.; Friis, E.; Ko, W.; Kopecky, A.; Lander, R.; Liu, H.; Maruyama, S.; Miceli, T.; Nikolic, M.; Pellett, D.; Robles, J.; Salur, S.; Schwarz, T.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez; Veelken, C.] Univ Calif Davis, Davis, CA 95616 USA. [Felcini, M.; Andreev, V.; Arisaka, K.; Cline, D.; Cousins, R.; Deisher, A.; Duris, J.; Erhan, S.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Tucker, J.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Chandra, A.; Clare, R.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Kao, S. C.; Liu, F.; Liu, H.; Long, O. R.; Luthra, A.; Nguyen, H.; Shen, B. C.; Stringer, R.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Belyaev, A.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Dusinberre, E.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pi, H.; Pieri, M.; Ranieri, R.; Sani, M.; Sharma, V.; Simon, S.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; Vlimant, J. R.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Gataullin, M.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Shin, K.; Timciuc, V.; Traczyk, P.; Veverka, J.; Wilkinson, R.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Akgun, B.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Jun, S. Y.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Dinardo, M. E.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Gaz, A.; Heyburn, B.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.; Zang, S. L.] Univ Colorado, Boulder, CO 80309 USA. [Agostino, L.; Alexander, J.; Cassel, D.; Chatterjee, A.; Das, S.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Kaufman, G. Nicolas; Patterson, J. R.; Puigh, D.; Ryd, A.; Salvati, E.; Shi, X.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Biselli, A.; Cirino, G.; Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Atac, M.; Bakken, J. A.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Borcherding, F.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Cooper, W.; Eartly, D. P.; Elvira, V. D.; Esen, S.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Green, D.; Gunthoti, K.; Gutsche, O.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jensen, H.; Johnson, M.; Joshi, U.; Khatiwada, R.; Klima, B.; Kousouris, K.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Limon, P.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Mason, D.; McBride, P.; Miao, T.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Pordes, R.; Prokofyev, O.; Saoulidou, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Tan, P.; Taylor, L.; Tkaczyk, S.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Piedra Gomez, J.; Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Matchev, K.; Mitselmakher, G.; Muniz, L.; Prescott, C.; Remington, R.; Schmitt, M.; Scurlock, B.; Sellers, P.; Skhirtladze, N.; Snowball, M.; Wang, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Ceron, C.; Gaultney, V.; Kramer, L.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Mesa, D.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bandurin, D.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Quertenmont, L.; Sekmen, S.; Veeraraghavan, V.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Guragain, S.; Hohlmann, M.; Kalakhety, H.; Ralich, R.; Vodopiyanov, I.] Florida Inst Technol, Melbourne, FL 32901 USA. [Belyaev, A.; Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Callner, J.; Cavanaugh, R.; Dragoiu, C.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kunde, G. J.; Lacroix, F.; Malek, M.; O'Brien, C.; Silvestre, C.; Smoron, A.; Strom, D.; Varelas, N.] UIC, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Duru, F.; Lae, C. K.; McCliment, E.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Olson, J.; Onel, Y.; Ozok, F.; Sen, S.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bonato, A.; Eskew, C.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Rappoccio, S.; Swartz, M.; Tran, N. V.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Belyaev, A.; Baringer, P.; Bean, A.; Benelli, G.; Grachov, O.; Iii, R. P. Kenny; Murray, M.; Noonan, D.; Sanders, S.; Wood, J. S.; Zhukova, V.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Bolton, T.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.; Wan, Z.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Boutemeur, M.; Eno, S. C.; Ferencek, D.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kirn, M.; Lu, Y.; Mignerey, A. C.; Rossato, K.; Rumerio, P.; Santanastasio, F.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.; Twedt, E.] Univ Maryland, College Pk, MD 20742 USA. [Wyslouch, B.; Alver, B.; Bauer, G.; Bendavid, J.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Everaerts, P.; Ceballos, G. Gomez; Goncharov, M.; Hahn, K. A.; Harris, P.; Kim, Y.; Klute, M.; Lee, Y. -J.; Li, W.; Loizides, C.; Luckey, P. 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Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bedoya, Cristina/0000-0001-8057-9152; Cerrada, Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Marinho, Franciole/0000-0002-7327-0349; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Dudko, Lev/0000-0002-4462-3192; Ruiz, Alberto/0000-0002-3639-0368; Stahl, Achim/0000-0002-8369-7506; Hektor, Andi/0000-0001-7873-8118; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Krammer, Manfred/0000-0003-2257-7751; Tinoco Mendes, Andre David/0000-0001-5854-7699; Katkov, Igor/0000-0003-3064-0466; Tomei, Thiago/0000-0002-1809-5226; Novaes, Sergio/0000-0003-0471-8549; Azzi, Patrizia/0000-0002-3129-828X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Montanari, Alessandro/0000-0003-2748-6373; Amapane, Nicola/0000-0001-9449-2509; Mundim, Luiz/0000-0001-9964-7805; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Ivanov, Andrew/0000-0002-9270-5643; Hill, Christopher/0000-0003-0059-0779; Troitsky, Sergey/0000-0001-6917-6600; Codispoti, Giuseppe/0000-0003-0217-7021 FU FMSR (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences (Estonia); NICPB (Estonia); Academy of Finland (Finland); ME (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Korea); WCU (Korea); LAS (Lithuania); CINVES-TAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MST (Russia); MAE (Russia); MSTD (Serbia); MICINN (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK (Turkey); TAEK (Turkey); STFC (United Kingdom); DOE (USA); NSF (USA) FX We wish to congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine. We thank the technical and administrative staff at CERN and other CMS institutes, and acknowledge support from: FMSR (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences and NICPB (Estonia); Academy of Finland, ME, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea); LAS (Lithuania); CINVES-TAV, CONACYT, SEP, and UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MST and MAE (Russia); MSTD (Serbia); MICINN and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK and TAEK (Turkey); STFC (United Kingdom); DOE and NSF (USA). NR 38 TC 34 Z9 34 U1 1 U2 44 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY PY 2011 IS 5 AR 093 DI 10.1007/JHEP05(2011)093 PG 35 WC Physics, Particles & Fields SC Physics GA 774EN UT WOS:000291364500025 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hammer, J Haensel, S Hoch, M Hormann, N Hrubec, J Jeitler, M Kasieczka, G Kiesenhofer, W Krammer, M Liko, D Mikulec, I Pernicka, M Rohringer, H Schofbeck, R Strauss, J Teischinger, F Wagner, P Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Benucci, L De Wolf, EA Janssen, X Maes, T Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Blekman, F Blyweert, S D'Hondt, J Devroede, O Suarez, RG Kalogeropoulos, A Maes, J Maes, M Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Charaf, O Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hammad, GH Hreus, T Marage, PE Thomas, L Velde, CV Vanlaer, P Adler, V Cimmino, A Costantini, S Grunewald, M Klein, B Lellouch, J Marinov, A Mccartin, J Ryckbosch, D Thyssen, F Tytgat, M Vanelderen, L Verwilligen, P Walsh, S Zaganidis, N Basegmez, S Bruno, G Caudron, J Ceard, L Gil, EC De Jeneret, JD Delaere, C Favart, D Giammanco, A Gregoire, G Hollar, J Lemaitre, V Liao, J Militaru, O Ovyn, S Pagano, D Pin, A Piotrzkowski, K Schul, N Beliy, N Caebergs, T Daubie, E Alves, GA Damiao, DD Pol, ME Souza, MHG Carvalho, W Da Costa, EM Martins, CD De Souza, SF Mundim, L Nogima, H Oguri, V Da Silva, WLP Santoro, A Do Amaral, SMS Sznajder, A De Araujo, FTD Dias, FA Tomei, TRFP Gregores, EM Lagana, C Marinho, F Mercadante, PG Novaes, SF Padula, SS Darmenov, N Dimitrov, L Genchev, V Iaydjiev, P Piperov, S Rodozov, M Stoykova, S Sultanov, G Tcholakov, V Trayanov, R Vankov, I Dimitrov, A Hadjiiska, R Karadzhinova, A Kozhuharov, V Litov, L Mateev, M Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, J Wang, J Wang, X Wang, Z Xiao, H 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Atramentov, O. Barker, A. Duggan, D. Gershtein, Y. Gray, R. Halkiadakis, E. Hidas, D. Hits, D. Lath, A. Panwalkar, S. Patel, R. Richards, A. Rose, K. Schnetzer, S. Somalwar, S. Stone, R. Thomas, S. Cerizza, G. Hollingsworth, M. Spanier, S. Yang, Z. C. York, A. Asaadi, J. Eusebi, R. Gilmore, J. Gurrola, A. Kamon, T. Khotilovich, V. Montalvo, R. Nguyen, C. N. Osipenkov, I. Pivarski, J. Safonov, A. Sengupta, S. Tatarinov, A. Toback, D. Weinberger, M. Akchurin, N. Bardak, C. Damgov, J. Jeong, C. Kovitanggoon, K. Lee, S. W. Roh, Y. Sill, A. Volobouev, I. Wigmans, R. Yazgan, E. Appelt, E. Brownson, E. Engh, D. Florez, C. Gabella, W. Issah, M. Johns, W. Kurt, P. Maguire, C. Melo, A. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Balazs, M. Boutle, S. Cox, B. Francis, B. Hirosky, R. Ledovskoy, A. Lin, C. Neu, C. Yohay, R. Gollapinni, S. Harr, R. Karchin, P. E. Lamichhane, P. Mattson, M. Milstene, C. Sakharov, A. Anderson, M. Bachtis, M. Bellinger, J. N. Carlsmith, D. Dasu, S. Efron, J. Flood, K. Gray, L. Grogg, K. S. Grothe, M. Hall-Wilton, R. Herndon, M. Klabbers, P. Klukas, J. Lanaro, A. Lazaridis, C. Leonard, J. Loveless, R. Mohapatra, A. Palmonari, F. Reeder, D. Ross, I. Savin, A. Smith, W. H. Swanson, J. Weinberg, M. CA CMS Collaboration TI Search for large extra dimensions in the diphoton final state at the Large Hadron Collider SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID PHOTON PAIR PRODUCTION; HIERARCHY; GRAVITY; SIGNALS AB A search for large extra spatial dimensions via virtual-graviton exchange in the diphoton channel has been carried out with the CMS detector at the LHC. No excess of events above the standard model expectations is found using a data sample collected in proton-proton collisions at root s = 7TeV and corresponding to an integrated luminosity of 36 pb(-1). 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T.; Nespolo, M.; Perrozzi, L.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bellan, P.; Bisello, D.; Carlin, R.; De Mattia, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Univ Padua, Padua, Italy. [Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Baesso, P.; Berzano, U.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.; Viviani, C.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Baesso, P.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.; Viviani, C.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Caponeri, B.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Santocchia, A.; Taroni, S.; Valdata, M.; Pioppi, M.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Caponeri, B.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Taroni, S.; Valdata, M.; Pioppi, M.] Univ Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Segneri, G.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bernardini, J.; Fiori, F.; Messineo, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Azzurri, P.; D'Agnolo, R. T.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Di Marco, E.; Diemoz, M.; Franci, D.; Grassi, M.; Longo, E.; Nourbakhsh, S.; Organtini, G.; Pandolfi, F.; Paramatti, R.; Rahatlou, S.] INFN Sez Roma, Rome, Italy. [Colafranceschi, S.] Univ Roma La Sapienza, Fac Ingn, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Botta, C.; Cartiglia, N.; Castello, R.; Costa, M.; Demaria, N.; Graziano, A.; Mariotti, C.; Marone, M.; Maselli, S.; Migliore, E.; Mila, G.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Romero, A.; Ruspa, M.; Sacchi, R.; Sola, V.; Solano, A.; Staiano, A.; Trocino, D.; Pereira, A. Vilela] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Botta, C.; Castello, R.; Costa, M.; Graziano, A.; Marone, M.; Migliore, E.; Mila, G.; Monaco, V.; Musich, M.; Pelliccioni, M.; Romero, A.; Sacchi, R.; Sola, V.; Solano, A.; Trocino, D.; Pereira, A. Vilela] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Montanino, D.; Penzo, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Della Ricca, G.; Montanino, D.] Univ Trieste, Trieste, Italy. [Heo, S. G.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Chung, J.; Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Park, H.; Ro, S. R.; Son, D. C.; Son, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, Zero; Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Hong, B.; Jeong, M. S.; Jo, M.; Kim, H.; Kim, J. H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.; Rhee, H. B.; Seo, E.; Shin, S.; Sim, K. S.] Korea Univ, Seoul, South Korea. [Choi, M.; Kang, S.; Kim, H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Martisiute, D.; Petrov, P.; Sabonis, T.] Vilnius Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] Ctr Invest & Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.; Tam, J.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ahmed, I.; Asghar, M. I.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bluj, M.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Soltan Inst Nucl Studies, PL-00681 Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Musella, P.; Nayak, A.; Seixas, J.; Varela, J.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Belotelov, I.; Bunin, P.; Golutvin, I.; Kamenev, A.; Karjavin, V.; Kozlov, G.; Lanev, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Toropin, A.; Troitsky, S.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Kaftanov, V.; Kossov, M.; Krokhotin, A.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Katkov, I.; Zhukov, V.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Sarycheva, L.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Azhgirey, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Slabospitsky, S.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Arce, P.; Battilana, C.; Calvo, E.; Cepeda, M.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Diez Pardos, C.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Jorda, C.; Lobelle Pardo, P.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Darmenov, N.; Genchev, V.; Iaydjiev, P.; Jung, H.; Hajdu, C.; Sikler, F.; Mohanty, A. K.; De Filippis, N.; Chiorboli, M.; Tropiano, A.; De Guio, F.; Montoya, C. A. Carrillo; Nespolo, M.; Perrozzi, L.; Lucaroni, A.; Taroni, S.; Boccali, T.; Tonelli, G.; Venturi, A.; Grassi, M.; Pandolfi, F.; Botta, C.; Graziano, A.; Kossov, M.; Grishin, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Baillon, P.; Ball, A. H.; Barney, D.; Bell, A. J.; Benedetti, D.; Bernet, C.; Bialas, W.; Bloch, P.; Bocci, A.; Bolognesi, S.; Bona, M.; Breuker, H.; Brona, G.; Bunkowski, K.; Camporesi, T.; Cerminara, G.; Perez, J. A. Coarasa; Cure, B.; D'Enterria, D.; De Roeck, A.; Di Guida, S.; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Gaddi, A.; Gennai, S.; Georgiou, G.; Gerwig, H.; Gigi, D.; Gill, K.; Giordano, D.; Glege, F.; Garrido, R. Gomez-Reino; Gouzevitch, M.; Govoni, P.; Gowdy, S.; Guiducci, L.; Hansen, M.; Hartl, C.; Harvey, J.; Hegeman, J.; Hegner, B.; Hoffmann, H. F.; Honma, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Lecoq, P.; Lourenco, C.; Maeki, T.; Malgeri, L.; Mannelli, M.; Masetti, L.; Maurisset, A.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Nesvold, E.; Nguyen, M.; Orimoto, T.; Orsini, L.; Perez, E.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Polese, G.; Racz, A.; Antunes, J. Rodrigues; Rolandi, G.; Rommerskirchen, T.; Rovelli, C.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Segoni, I.; Sharma, A.; Siegrist, P.; Simon, M.; Sphicas, P.; Spiropulu, M.; Stoye, M.; Tropea, P.; Tsirou, A.; Vichoudis, P.; Voutilainen, M.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Starodumov, A.; Caminada, L.; Marchica, C.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bortignon, P.; Caminada, L.; Chen, Z.; Cittolin, S.; Dissertori, G.; Dittmar, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Herve, A.; Hintz, W.; Lecomte, P.; Lustermann, W.; Marchica, C.; del Arbol, P. Martinez Ruiz; Meridiani, P.; Milenovic, P.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pape, L.; Pauss, F.; Punz, T.; Rizzi, A.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Sawley, M. -C.; Stieger, B.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, M.; Wehrli, L.; Weng, J.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aguilo, E.; Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Otiougova, P.; Regenfus, C.; Robmann, P.; Schmidt, A.; Snoek, H.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Volpe, R.; Wu, J. H.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Topaksu, A. Kayis; Nart, A.; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Uzun, D.; Vergili, L. N.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Deliomeroglu, M.; Demir, D.; Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Levchuk, L.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Bostock, F.; Brooke, J. J.; Cheng, T. L.; Clement, E.; Cussans, D.; Frazier, R.; Goldstein, J.; Grimes, M.; Hansen, M.; Hartley, D.; Heath, G. P.; Heath, H. F.; Jackson, J.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Ward, S.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Camanzi, B.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Ballin, J.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Lyons, L.; MacEvoy, B. C.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rompotis, N.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Tourneur, S.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Wardrope, D.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Barrett, M.; Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Martin, W.; Reid, I. D.; Teodorescu, L.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.] Baylor Univ, Waco, TX 76798 USA. [Bose, T.; Jarrin, E. Carrera; Fantasia, C.; Heister, A.; St John, J.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Avetisyan, A.; Bhattacharya, S.; Chou, J. P.; Cutts, D.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Landsberg, G.; Narain, M.; Nguyen, D.; Segala, M.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Cox, P. T.; Dolen, J.; Erbacher, R.; Friis, E.; Ko, W.; Kopecky, A.; Lander, R.; Liu, H.; Maruyama, S.; Miceli, T.; Nikolic, M.; Pellett, D.; Robles, J.; Salur, S.; Schwarz, T.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez; Veelken, C.] Univ Calif Davis, Davis, CA 95616 USA. [Andreev, V.; Arisaka, K.; Cline, D.; Cousins, R.; Deisher, A.; Duris, J.; Erhan, S.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Tucker, J.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Chandra, A.; Clare, R.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Kao, S. C.; Liu, F.; Liu, H.; Long, O. R.; Luthra, A.; Nguyen, H.; Shen, B. C.; Stringer, R.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Dusinberre, E.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pi, H.; Pieri, M.; Ranieri, R.; Sani, M.; Sharma, V.; Simon, S.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; Vlimant, J. R.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Spiropulu, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Gataullin, M.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Shin, K.; Timciuc, V.; Traczyk, P.; Veverka, J.; Wilkinson, R.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Akgun, B.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Jun, S. Y.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Dinardo, M. E.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Gaz, A.; Heyburn, B.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.; Zang, S. L.] Univ Colorado, Boulder, CO 80309 USA. [Agostino, L.; Alexander, J.; Cassel, D.; Chatterjee, A.; Das, S.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Kaufman, G. Nicolas; Patterson, J. R.; Puigh, D.; Ryd, A.; Shi, X.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Biselli, A.; Cirino, G.; Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Atac, M.; Bakken, J. A.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Borcherding, F.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Cooper, W.; Eartly, D. P.; Elvira, V. D.; Esen, S.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Green, D.; Gunthoti, K.; Gutsche, O.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jensen, H.; Johnson, M.; Joshi, U.; Khatiwada, R.; Klima, B.; Kousouris, K.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Limon, P.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Mason, D.; McBride, P.; Miao, T.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Pordes, R.; Prokofyev, O.; Saoulidou, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Tan, P.; Taylor, L.; Tkaczyk, S.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Matchev, K.; Mitselmakher, G.; Muniz, L.; Pakhotin, Y.; Prescott, C.; Remington, R.; Schmitt, M.; Scurlock, B.; Sellers, P.; Skhirtladze, N.; Snowball, M.; Wang, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Ceron, C.; Gaultney, V.; Kramer, L.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Mesa, D.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bandurin, D.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Quertenmont, L.; Sekmen, S.; Veeraraghavan, V.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Guragain, S.; Hohlmann, M.; Kalakhety, H.; Ralich, R.; Vodopiyanov, I.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Callner, J.; Cavanaugh, R.; Dragoiu, C.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kunde, G. J.; Lacroix, F.; Malek, M.; O'Brien, C.; Silvestre, C.; Smoron, A.; Strom, D.; Varelas, N.] UIC, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Duru, F.; Lae, C. K.; McCliment, E.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Olson, J.; Onel, Y.; Ozok, F.; Sen, S.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bonato, A.; Eskew, C.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Guo, Z. J.; Hu, G.; Maksimovic, P.; Rappoccio, S.; Swartz, M.; Tran, N. V.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Grachov, O.; Murray, M.; Noonan, D.; Sanders, S.; Wood, J. S.; Zhukova, V.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Bolton, T.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.; Wan, Z.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Boutemeur, M.; Eno, S. C.; Ferencek, D.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kirn, M.; Lu, Y.; Mignerey, A. C.; Rossato, K.; Rumerio, P.; Santanastasio, F.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.; Twedt, E.] Univ Maryland, College Pk, MD 20742 USA. [Wyslouch, B.; Alver, B.; Bauer, G.; Bendavid, J.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Everaerts, P.; Ceballos, G. Gomez; Goncharov, M.; Hahn, K. A.; Harris, P.; Kim, Y.; Klute, M.; Lee, Y. -J.; Li, W.; Loizides, C.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Rudolph, M.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Wenger, E. A.; Xie, S.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.] MIT, Cambridge, MA 02139 USA. [Cole, P.; Cooper, S. I.; Cushman, P.; Dahmes, B.; De Benedetti, A.; Dudero, P. R.; Franzoni, G.; Haupt, J.; Klapoetke, K.; Kubota, Y.; Mans, J.; Rekovic, V.; Rusack, R.; Sasseville, M.; Singovsky, A.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Godang, R.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, University, MS USA. [Bloom, K.; Bose, S.; Butt, J.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kelly, T.; Kravchenko, I.; Lazo-Flores, J.; Malbouisson, H.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Baur, U.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Shipkowski, S. P.; Smith, K.] SUNY Buffalo, Buffalo, NY 14260 USA. 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S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Acosta, J. G.; Huang, X. T.; Lopez, A.; Mendez, H.; Oliveros, S.; Vargas, J. E. Ramirez; Zatserklyaniy, A.] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Barnes, V. E.; Bolla, G.; Borrello, L.; Bortoletto, D.; Everett, A.; Garfinkel, A. F.; Gutay, L.; Hu, Z.; Jones, M.; Koybasi, O.; Kress, M.; Laasanen, A. T.; Leonardo, N.; Liu, C.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Jindal, P.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Boulahouache, C.; Cuplov, V.; Ecklund, K. M.; Geurts, F. J. M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Chung, Y. S.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Flacher, H.; Garcia-Bellido, A.; Goldenzweig, P.; Gotra, Y.; Han, J.; Harel, A.; Miner, D. 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W.; Roh, Y.; Sill, A.; Volobouev, I.; Wigmans, R.; Yazgan, E.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Brownson, E.; Engh, D.; Florez, C.; Gabella, W.; Issah, M.; Johns, W.; Kurt, P.; Maguire, C.; Melo, A.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN USA. [Arenton, M. W.; Balazs, M.; Boutle, S.; Cox, B.; Francis, B.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Yohay, R.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Lamichhane, P.; Mattson, M.; Milstene, C.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Anderson, M.; Bachtis, M.; Bellinger, J. N.; Carlsmith, D.; Dasu, S.; Efron, J.; Flood, K.; Gray, L.; Grogg, K. S.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Leonard, J.; Loveless, R.; Mohapatra, A.; Palmonari, F.; Reeder, D.; Ross, I.; Savin, A.; Smith, W. H.; Swanson, J.; Weinberg, M.] Univ Wisconsin, Madison, WI 53706 USA. [Gregores, E. 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RI Leonidov, Andrey/P-3197-2014; Russ, James/P-3092-2014; Dahms, Torsten/A-8453-2015; Ahmed, Ijaz/E-9144-2015; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; Bedoya, Cristina/K-8066-2014; Cerrada, Marcos/J-6934-2014; Calderon, Alicia/K-3658-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Marinho, Franciole/N-8101-2014; Ferguson, Thomas/O-3444-2014; Ragazzi, Stefano/D-2463-2009; Benussi, Luigi/O-9684-2014; Zalewski, Piotr/H-7335-2013; Cavallo, Nicola/F-8913-2012; Ivanov, Andrew/A-7982-2013; Hill, Christopher/B-5371-2012; Wimpenny, Stephen/K-8848-2013; Markina, Anastasia/E-3390-2012; Troitsky, Sergey/C-1377-2014; Marlow, Daniel/C-9132-2014; Janssen, Xavier/E-1915-2013; Oguri, Vitor/B-5403-2013; Codispoti, Giuseppe/F-6574-2014; Gribushin, Andrei/J-4225-2012; Montanari, Alessandro/J-2420-2012; Amapane, Nicola/J-3683-2012; tosi, mia/J-5777-2012; Petrushanko, Sergey/D-6880-2012; Raidal, Martti/F-4436-2012; Mercadante, Pedro/K-1918-2012; Della Ricca, Giuseppe/B-6826-2013; Kadastik, Mario/B-7559-2008; Mundim, Luiz/A-1291-2012; Santaolalla, Javier/C-3094-2013; Alves, Gilvan/C-4007-2013; Rolandi, Luigi (Gigi)/E-8563-2013; Katkov, Igor/E-2627-2012; Boos, Eduard/D-9748-2012; Snigirev, Alexander/D-8912-2012; Tomei, Thiago/E-7091-2012; Novaes, Sergio/D-3532-2012; Padula, Sandra /G-3560-2012; Fruhwirth, Rudolf/H-2529-2012; Azzi, Patrizia/H-5404-2012; Torassa, Ezio/I-1788-2012; Giacomelli, Paolo/B-8076-2009; Jeitler, Manfred/H-3106-2012; Venturi, Andrea/J-1877-2012; de Jesus Damiao, Dilson/G-6218-2012; Wulz, Claudia-Elisabeth/H-5657-2011; Chen, Jie/H-6210-2011; Bolton, Tim/A-7951-2012; Yang, Fan/B-2755-2012; Krammer, Manfred/A-6508-2010; Tinoco Mendes, Andre David/D-4314-2011; Lokhtin, Igor/D-7004-2012; Kodolova, Olga/D-7158-2012; Dudko, Lev/D-7127-2012; Perfilov, Maxim/E-1064-2012; Belyaev, Andrey/E-1540-2012; Stahl, Achim/E-8846-2011; Hektor, Andi/G-1804-2011; Ligabue, Franco/F-3432-2014; Azarkin, Maxim/N-2578-2015; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Sznajder, Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Gerbaudo, Davide/J-4536-2012; Matorras, Francisco/I-4983-2015; My, Salvatore/I-5160-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Arce, Pedro/L-1268-2014; Flix, Josep/G-5414-2012; Ozdemir, Kadri/P-8058-2014 OI Russ, James/0000-0001-9856-9155; Dahms, Torsten/0000-0003-4274-5476; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bedoya, Cristina/0000-0001-8057-9152; Cerrada, Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Marinho, Franciole/0000-0002-7327-0349; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Ivanov, Andrew/0000-0002-9270-5643; Hill, Christopher/0000-0003-0059-0779; Wimpenny, Stephen/0000-0003-0505-4908; Troitsky, Sergey/0000-0001-6917-6600; Codispoti, Giuseppe/0000-0003-0217-7021; Montanari, Alessandro/0000-0003-2748-6373; Amapane, Nicola/0000-0001-9449-2509; Della Ricca, Giuseppe/0000-0003-2831-6982; Mundim, Luiz/0000-0001-9964-7805; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Katkov, Igor/0000-0003-3064-0466; Tomei, Thiago/0000-0002-1809-5226; Novaes, Sergio/0000-0003-0471-8549; Azzi, Patrizia/0000-0002-3129-828X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Krammer, Manfred/0000-0003-2257-7751; Tinoco Mendes, Andre David/0000-0001-5854-7699; Dudko, Lev/0000-0002-4462-3192; Stahl, Achim/0000-0002-8369-7506; Hektor, Andi/0000-0001-7873-8118; Luukka, Panja/0000-0003-2340-4641; Goldstein, Joel/0000-0003-1591-6014; Heath, Helen/0000-0001-6576-9740; Grassi, Marco/0000-0003-2422-6736; Gutsche, Oliver/0000-0002-8015-9622; CHANG, PAO-TI/0000-0003-4064-388X; WANG, MIN-ZU/0000-0002-0979-8341; Martinez Ruiz del Arbol, Pablo/0000-0002-7737-5121; HSIUNG, YEE/0000-0003-4801-1238; Costa, Salvatore/0000-0001-9919-0569; Ligabue, Franco/0000-0002-1549-7107; Malik, Sudhir/0000-0002-6356-2655; Staiano, Amedeo/0000-0003-1803-624X; Tonelli, Guido Emilio/0000-0003-2606-9156; Abbiendi, Giovanni/0000-0003-4499-7562; Rizzi, Andrea/0000-0002-4543-2718; Gershtein, Yuri/0000-0002-4871-5449; Mrenna, Stephen/0000-0001-8731-160X; Kasemann, Matthias/0000-0002-0429-2448; Stober, Fred/0000-0003-2620-3159; Landsberg, Greg/0000-0002-4184-9380; Leonidopoulos, Christos/0000-0002-7241-2114; Blekman, Freya/0000-0002-7366-7098; Beuselinck, Raymond/0000-0003-2613-7446; Toback, David/0000-0003-3457-4144; Jun, Soon Yung/0000-0003-3370-6109; Giacomelli, Paolo/0000-0002-6368-7220; Arneodo, Michele/0000-0002-7790-7132; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Gerbaudo, Davide/0000-0002-4463-0878; Matorras, Francisco/0000-0003-4295-5668; My, Salvatore/0000-0002-9938-2680; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Arce, Pedro/0000-0003-3009-0484; Flix, Josep/0000-0003-2688-8047; Ozdemir, Kadri/0000-0002-0103-1488 FU FMSR (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences (Estonia); NICPB (Estonia); Academy of Finland (Finland); ME (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Korea); WCU (Korea); LAS (Lithuania); CINVES-TAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MST (Russia); MAE (Russia); MSTD (Serbia); MICINN (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK (Turkey); TAEK (Turkey); STFC (United Kingdom); DOE (U.S.A.); NSF (U.S.A.) FX We wish to congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine. We thank the technical and administrative staff at CERN and other CMS institutes, and acknowledge support from: FMSR (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences and NICPB (Estonia); Academy of Finland, ME, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea); LAS (Lithuania); CINVES-TAV, CONACYT, SEP, and UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MST and MAE (Russia); MSTD (Serbia); MICINN and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK and TAEK (Turkey); STFC (United Kingdom); DOE and NSF (U.S.A.). NR 26 TC 16 Z9 16 U1 1 U2 44 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY PY 2011 IS 5 AR 085 DI 10.1007/JHEP05(2011)085 PG 28 WC Physics, Particles & Fields SC Physics GA 774EN UT WOS:000291364500017 ER PT J AU Falkowski, A Ruderman, JT Volansky, T AF Falkowski, Adam Ruderman, Joshua T. Volansky, Tomer TI Asymmetric dark matter from leptogenesis SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Cosmology of Theories beyond the SM; Neutrino Physics ID STERILE NEUTRINOS; BARYOGENESIS; MASS AB We present a new realization of asymmetric dark matter in which the dark matter and lepton asymmetries are generated simultaneously through two-sector leptogenesis. The right-handed neutrinos couple both to the Standard Model and to a hidden sector where the dark matter resides. This framework explains the lepton asymmetry, dark matter abundance and neutrino masses all at once. In contrast to previous realizations of asymmetric dark matter, the model allows for a wide range of dark matter masses, from keV to 10 TeV. In particular, very light dark matter can be accommodated without violating experimental constraints. We discuss several variants of our model that highlight interesting phenomenological possibilities. In one, late decays repopulate the symmetric dark matter component, providing a new mechanism for generating a large annihilation rate at the present epoch and allowing for mixed warm/cold dark matter. In a second scenario, dark matter mixes with the active neutrinos, thus presenting a distinct method to populate sterile neutrino dark matter through leptogenesis. At late times, oscillations and dark matter decays lead to interesting indirect detection signals. C1 [Falkowski, Adam] Univ Paris 11, CNRS, Lab Phys Theor Orsay, UMR8627, F-91405 Orsay, France. [Ruderman, Joshua T.] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. [Volansky, Tomer] Univ Calif Berkeley, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. [Volansky, Tomer] Univ Calif Berkeley, Lawrence Berkeley Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Falkowski, A (reprint author), Univ Paris 11, CNRS, Lab Phys Theor Orsay, UMR8627, F-91405 Orsay, France. EM adam.falkowski@th.u-psud.fr; rudes@ias.edu; tomerv@post.tau.ac.il FU Office of Science, Office of High and Nuclear Physics, of the US Department of Energy [DE-AC02-05CH11231] FX We thank Ami Katz for collaboration in the early stages of this project. We also thank Cliff Cheung, Tim Cohen, Yanou Cui, Rouven Essig, Yuval Grossman, Marc Kamionkowski, Yasunori Nomura, Michele Papucci, Aaron Pierce, and Tracy Slatyer for useful conversations. work of T. V. was supported in part by the Director, Office of Science, Office of High and Nuclear Physics, of the US Department of Energy under Contract DE-AC02-05CH11231. NR 69 TC 86 Z9 86 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY PY 2011 IS 5 AR 106 DI 10.1007/JHEP05(2011)106 PG 32 WC Physics, Particles & Fields SC Physics GA 774EN UT WOS:000291364500038 ER PT J AU Heidenreich, B McAllister, L Torroba, G AF Heidenreich, Ben McAllister, Liam Torroba, Gonzalo TI Dynamic SU(2) structure from seven-branes SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Flux compactifications; Superstring Vacua; D-branes ID CALABI-YAU; SUPERSYMMETRY BREAKING; LARGE N; SUPERGRAVITY; STRINGS; FLUXES; BRANES AB We obtain a family of supersymmetric solutions of type IIB supergravity with dynamic SU(2) structure, which describe the local geometry near a stack of four D7-branes and one O7-plane wrapping a rigid four-cycle. The deformation to a generalized complex geometry is interpreted as a consequence of nonperturbative effects in the seven-brane gauge theory. We formulate the problem for seven-branes wrapping the base of an appropriate del Pezzo cone, and in the near-stack limit in which the four-cycle is flat, we obtain an exact solution in closed form. Our solutions serve to characterize the local geometry of nonperturbatively-stabilized flux compactifications. C1 [Heidenreich, Ben; McAllister, Liam] Cornell Univ, Dept Phys, Ithaca, NY 14853 USA. [Torroba, Gonzalo] Stanford Univ, SLAC, Stanford, CA 94309 USA. [Torroba, Gonzalo] Stanford Univ, Dept Phys, Stanford, CA 94309 USA. RP Heidenreich, B (reprint author), Cornell Univ, Dept Phys, Ithaca, NY 14853 USA. EM bjh77@cornell.edu; mcallister@cornell.edu; torrobag@slac.stanford.edu FU Alfred P. Sloan Foundation; NSF [PHY-0757868]; Cornell University; Swedish Foundation for International Cooperation in Research and Higher Education; US DOE at SLAC [DE-AC02-76SF00515] FX We are grateful to D. Baumann, M. Berg, P. Camara, A. Collinucci, F. Denef, A. Dymarsky, S. Franco, T. Grimm, S. Kachru, L. Martucci, G. Moore, E. Silverstein, T. Weigand, and T. Wrase for helpful discussions. We thank D. Baumann, S. Kachru, J. Liu, L. Martucci, and P. Szepietowski for useful comments on the manuscript. L.M. specially thanks T. Weigand for valuable discussions and correspondence. G.T. is particularly grateful to S. Kachru for many enlightening conversations. The research of L.M. was supported by the Alfred P. Sloan Foundation and by the NSF under grant PHY-0757868. The research of B.H. was supported in part by a Cornell University Olin Fellowship and by NSF grant PHY-0757868. B.H. and L.M. gratefully acknowledge support for this work by the Swedish Foundation for International Cooperation in Research and Higher Education. G.T. is supported by the US DOE under contract number DE-AC02-76SF00515 at SLAC. We thank the organizers of String Phenomenology 2010 for providing a stimulating environment for a portion of this work. G.T. would like to thank the KITP, where part of this work was done, for hospitality. NR 50 TC 13 Z9 13 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY PY 2011 IS 5 AR 110 DI 10.1007/JHEP05(2011)110 PG 47 WC Physics, Particles & Fields SC Physics GA 774EN UT WOS:000291364500042 ER PT J AU Lehner, C Bloch, J Hashimoto, S Wettig, T AF Lehner, Christoph Bloch, Jacques Hashimoto, Shoji Wettig, Tilo TI Geometry dependence of RMT-based methods to extract the low-energy constants Sigma and F SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Lattice QCD; Chiral Lagrangians; QCD ID CHIRAL PERTURBATION-THEORY; RANDOM-MATRIX THEORY; DIRAC OPERATOR; QCD; SYMMETRY; QUARK AB The lowest-order low-energy constants Sigma and F of chiral pertubation theory can be extracted from lattice data using methods based on the equivalence of random matrix theory (RMT) and QCD in the epsilon regime. We discuss how the choice of the lattice geometry affects such methods. In particular, we show how to minimize systematic deviations from RMT by an optimal choice of the lattice geometry in the case of two light quark flavors. We illustrate our findings by determining Sigma and F from lattice configurations with two dynamical overlap fermions generated by JLQCD, using two different lattice geometries. C1 [Lehner, Christoph; Bloch, Jacques; Wettig, Tilo] Univ Regensburg, Inst Theoret Phys, D-93040 Regensburg, Germany. [Lehner, Christoph] Brookhaven Natl Lab, RIKEN, BNL Res Ctr, Upton, NY 11973 USA. [Hashimoto, Shoji] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki 3050801, Japan. RP Lehner, C (reprint author), Univ Regensburg, Inst Theoret Phys, D-93040 Regensburg, Germany. EM clehner@quark.phy.bnl.gov; acques.bloch@physik.uni-regensburg.de; shoji.hashimoto@kek.jp; tilo.wettig@physik.uni-regensburg.de OI Lehner, Christoph/0000-0002-3584-4567 FU BayEFG; RIKEN FPR; Japanese Ministry of Education [21674002]; DFG [SFB-TR 55]; KEK fellowship; Large Scale Simulation Program [09/10-09] FX This work was supported in part by BayEFG and the RIKEN FPR program (CL), the Grant-in-Aid (No. 21674002) of the Japanese Ministry of Education (SH), DFG grant SFB-TR 55 (JB and TW), and a KEK fellowship (TW). The numerical calculations were carried out on the IBM System Blue Gene Solution at the High Energy Accelerator Research Organization under support of its Large Scale Simulation Program (No. 09/10-09). NR 25 TC 6 Z9 6 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY PY 2011 IS 5 AR 115 DI 10.1007/JHEP05(2011)115 PG 15 WC Physics, Particles & Fields SC Physics GA 774EN UT WOS:000291364500047 ER PT J AU Kobayashi, T Mao, K Wang, SG Lin, VSY Pruski, M AF Kobayashi, Takeshi Mao, Kanmi Wang, Shy-Guey Lin, Victor S. -Y. Pruski, Marek TI Molecular ordering of mixed surfactants in mesoporous silicas: A solid-state NMR study SO SOLID STATE NUCLEAR MAGNETIC RESONANCE LA English DT Article DE Solid-state NMR; Dipolar interactions; Fast MAS; HETCOR NMR; Mesoporous silica; Mixed surfactants; Heterogeneous catalysis ID PORE-SIZE; SPECTROSCOPY; MAS; TEMPLATES; BROMIDE; H-1-NMR; SYSTEM; MCM-41 AB The use of mixed surfactants in the synthesis of mesoporous silica nanoparticles (MSNs) is of importance in the context of adjusting pore structures, sizes and morphologies. In the present study, the arrangement of molecules in micelles produced from a mixture of two surfactants, cetyltrimethylammonium bromide (CTAB) and cetylpyridinium bromide (CPB) was detailed by solid-state NMR spectroscopy. Proximities of methyl protons in the trimethylammonium headgroup of CTAB and protons in the pyridinium headgroup of CPB were observed under fast magic angle spinning (MAS) by H-1-H-1 double quantum (DQ) MAS NMR and NOESY. This result suggested that CTAB and CPB co-exist in the pores without forming significant monocomponent domain structures. H-1-Si-29 heteronuclear correlation (HETCOR) NMR showed that protons in the headgroups of CTAB are in closer proximity to the silica surface than those in the CPB headgroups. The structural information obtained in this investigation leads to better understanding of the mechanisms of self-assembly and their role in determining the structure and morphology of mesoporous materials. (C) 2011 Elsevier Inc. All rights reserved. C1 [Kobayashi, Takeshi; Mao, Kanmi; Lin, Victor S. -Y.; Pruski, Marek] Iowa State Univ, US DOE Ames Lab, Ames, IA 50011 USA. [Wang, Shy-Guey; Lin, Victor S. -Y.; Pruski, Marek] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. RP Pruski, M (reprint author), Iowa State Univ, US DOE Ames Lab, Ames, IA 50011 USA. EM mpruski@iastate.edu FU U.S. Department of Energy, Office of Basic Energy Science at Ames Laboratory [DE-AC02-07CH11358] FX This research was supported at the Ames Laboratory by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-07CH11358. We thank Dr. Tommy Hung-ting Chen for helpful discussions. NR 29 TC 12 Z9 12 U1 2 U2 29 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0926-2040 EI 1527-3326 J9 SOLID STATE NUCL MAG JI Solid State Nucl. Magn. Reson. PD MAY-JUN PY 2011 VL 39 IS 3-4 SI SI BP 65 EP 71 DI 10.1016/j.ssnmr.2011.02.001 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical; Physics, Condensed Matter; Spectroscopy SC Chemistry; Physics; Spectroscopy GA 787FF UT WOS:000292361300005 PM 21392947 ER PT J AU Kim, D Kang, SH Slater, M Rood, S Vaughey, JT Karan, N Balasubramanian, M Johnson, CS AF Kim, Donghan Kang, Sun-Ho Slater, Michael Rood, Shawn Vaughey, John T. Karan, Naba Balasubramanian, Mahalingam Johnson, Christopher S. TI Enabling Sodium Batteries Using Lithium-Substituted Sodium Layered Transition Metal Oxide Cathodes SO ADVANCED ENERGY MATERIALS LA English DT Article ID ELECTRODES; LI; CELLS; NA; MN; NI C1 [Karan, Naba; Balasubramanian, Mahalingam] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Kim, Donghan; Kang, Sun-Ho; Slater, Michael; Rood, Shawn; Vaughey, John T.; Johnson, Christopher S.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Balasubramanian, M (reprint author), Argonne Natl Lab, Adv Photon Source, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM mali@aps.anl.gov; cjohnson@anl.gov RI Slater, Michael/D-5388-2012; Rood, Shawn/O-9843-2015; OI Rood, Shawn/0000-0002-5416-9894; Vaughey, John/0000-0002-2556-6129 FU Department of Energy (DOE) [DE-AC02 - 06CH11357]; US-DOE Basic Energy Sciences; NSERC-Canada; U.S. Department of Energy Office of Science laboratory [DE-AC02 - 06CH11357] FX Funding from the Department of Energy (DOE) under Contract DE-AC02 - 06CH11357 is gratefully acknowledged. Work at PNC/XSD facilities at the Advanced Photon Source, and research at these facilities, are supported by the US-DOE Basic Energy Sciences, NSERC-Canada and its founding institutions.; The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02 - 06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up, nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 20 TC 207 Z9 209 U1 21 U2 179 PU WILEY PERIODICALS, INC PI MALDEN PA COMMERCE PLACE, 350 MAIN STREET, MALDEN, MA 02148-529 USA SN 1614-6832 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD MAY PY 2011 VL 1 IS 3 BP 333 EP 336 DI 10.1002/aenm.201000061 PG 4 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA 778TH UT WOS:000291728400002 ER PT J AU Liu, B Chen, XB Dong, YL Mao, SS Cheng, MJ AF Liu, Bin Chen, Xiaobo Dong, Yonglai Mao, Samuel S. Cheng, Mojie TI A High-Performance, Nanostructured Ba0.5Sr0.5Co0.8Fe0.2O3-delta Cathode for Solid-Oxide Fuel Cells SO ADVANCED ENERGY MATERIALS LA English DT Article ID PULSED-LASER DEPOSITION; ELECTROLYTE; ANODE; PERMEATION; MEMBRANE; BEHAVIOR; SOFCS C1 [Liu, Bin; Chen, Xiaobo; Mao, Samuel S.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Liu, Bin; Dong, Yonglai; Cheng, Mojie] Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China. [Liu, Bin; Dong, Yonglai] Chinese Acad Sci, Grad Univ, Beijing 100039, Peoples R China. RP Mao, SS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. EM ssmao@newton.berkeley.edu; mjcheng@dicp.ac.cn FU Ministry of Science and Technology of China; Office of Energy Efficiency and Renewable Energy of the US Department of Energy; National Center for Electron Microscopy, Lawrence Berkeley National Laboratory by the US Department of Energy [DE-AC02 - 05CH11231] FX The authors acknowledge support from the Ministry of Science and Technology of China, the Office of Energy Efficiency and Renewable Energy of the US Department of Energy, and the National Center for Electron Microscopy, Lawrence Berkeley National Laboratory, which is supported by the US Department of Energy under Contract # DE-AC02 - 05CH11231. NR 19 TC 22 Z9 22 U1 0 U2 29 PU WILEY PERIODICALS, INC PI MALDEN PA COMMERCE PLACE, 350 MAIN STREET, MALDEN, MA 02148-529 USA SN 1614-6832 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD MAY PY 2011 VL 1 IS 3 BP 343 EP 346 DI 10.1002/aenm.201100042 PG 4 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA 778TH UT WOS:000291728400004 ER PT J AU Agakishiev, G Balanda, A Bannier, B Bassini, R Belver, D Belyaev, AV Blanco, A Bohmer, M Boyard, JL Cabanelas, P Castro, E Chernenko, S Christ, T Destefanis, M Diaz, J Dohrmann, F Dybczak, A Eberl, T Epple, E Fabbietti, L Fateev, OV Finocchiaro, P Fonte, P Friese, J Frohlich, I Galatyuk, T Garzon, JA Gernhauser, R Gil, A Gilardi, C Golubeva, M Gonzalez-Diaz, D Guber, F Gumberidze, M Heilmann, M Heinz, T Hennino, T Holzmann, R Huck, P Iori, I Ivashkin, A Jurkovic, M Kampfer, B Kanaki, K Karavicheva, T Kirschner, D Koenig, I Koenig, W Kolb, BW Kotte, R Krizek, F Krucken, R Kuhn, W Kugler, A Kurepin, A Lang, S Lange, JS Lapidus, K Liu, T Lopes, L Lorenz, M Maier, L Mangiarotti, A Markert, J Metag, V Michalska, B Michel, J Mishra, D Moriniere, E Mousa, J Muntz, C Naumann, L Otwinowski, J Pachmayer, YC Palka, M Parpottas, Y Pechenov, V Pechenova, O Cavalcanti, TP Pietraszko, J Przygoda, W Ramstein, B Reshetin, A Roy-Stephan, M Rustamov, A Sadovsky, A Sailer, B Salabura, P Schmah, A Schwab, E Siebenson, J Sobolev, YG Spataro, S Spruck, B Strobele, H Stroth, J Sturm, C Tarantola, A Teilab, K Tlusty, P Traxler, M Trebacz, R Tsertos, H Wagner, V Weber, M Wendisch, C Wisniowski, M Wojcik, T Wustenfeld, J Yurevich, S Zanevsky, YV Zhou, P Zumbruch, P AF Agakishiev, G. Balanda, A. Bannier, B. Bassini, R. Belver, D. Belyaev, A. V. Blanco, A. Boehmer, M. Boyard, J. L. Cabanelas, P. Castro, E. Chernenko, S. Christ, T. Destefanis, M. Diaz, J. Dohrmann, F. Dybczak, A. Eberl, T. Epple, E. Fabbietti, L. Fateev, O. V. Finocchiaro, P. Fonte, P. Friese, J. Froehlich, I. Galatyuk, T. Garzon, J. A. Gernhaeuser, R. Gil, A. Gilardi, C. Golubeva, M. Gonzalez-Diaz, D. Guber, F. Gumberidze, M. Heilmann, M. Heinz, T. Hennino, T. Holzmann, R. Huck, P. Iori, I. Ivashkin, A. Jurkovic, M. Kaempfer, B. Kanaki, K. Karavicheva, T. Kirschner, D. Koenig, I. Koenig, W. Kolb, B. W. Kotte, R. Krizek, F. Kruecken, R. Kuehn, W. Kugler, A. Kurepin, A. Lang, S. Lange, J. S. Lapidus, K. Liu, T. Lopes, L. Lorenz, M. Maier, L. Mangiarotti, A. Markert, J. Metag, V. Michalska, B. Michel, J. Mishra, D. Moriniere, E. Mousa, J. Muentz, C. Naumann, L. Otwinowski, J. Pachmayer, Y. C. Palka, M. Parpottas, Y. Pechenov, V. Pechenova, O. Cavalcanti, T. Perez Pietraszko, J. Przygoda, W. Ramstein, B. Reshetin, A. Roy-Stephan, M. Rustamov, A. Sadovsky, A. Sailer, B. Salabura, P. Schmah, A. Schwab, E. Siebenson, J. Sobolev, Yu. G. Spataro, S. Spruck, B. Stroebele, H. Stroth, J. Sturm, C. Tarantola, A. Teilab, K. Tlusty, P. Traxler, M. Trebacz, R. Tsertos, H. Wagner, V. Weber, M. Wendisch, C. Wisniowski, M. Wojcik, T. Wuestenfeld, J. Yurevich, S. Zanevsky, Y. V. Zhou, P. Zumbruch, P. TI pp and pi pi intensity interferometry in collisions of Ar+KCl at 1.76A GeV SO EUROPEAN PHYSICAL JOURNAL A LA English DT Article ID HEAVY-ION COLLISIONS; RELATIVISTIC NUCLEAR COLLISIONS; INTERMEDIATE-MASS FRAGMENTS; PROTON-PROTON CORRELATIONS; SMALL-ANGLE CORRELATIONS; VELOCITY CORRELATIONS; ENERGY; AU+AU; EMISSION; KCL AB Results on pp, pi(+) pi(+), and pi-pi-intensity interferometry are reported for collisions of Ar+KCl at 1.76A GeV beam energy, studied with the High Acceptance Di-Electron Spectrometer (HADES) at SIS18/GSI. The experimental correlation functions as a function of the relative momentum are compared to model calculations allowing the determination of the space-time extent of the corresponding emission sources. The pp source radii are found significantly larger than the pp emission radius. The present radii do well complement the beam-energy dependences of Gaussian source radii of the collision system of size A + A similar or equal to 40 + 40. The pp source radius at fixed beam energy is found to increase linearly with the cube root of the number of participants. From this trend, a lower limit of the pp correlation radius is deduced. C1 [Finocchiaro, P.] Ist Nazl Fis Nucl, Lab Nazl Sud, I-95125 Catania, Italy. [Blanco, A.; Fonte, P.; Lopes, L.; Mangiarotti, A.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-3004516 Coimbra, Portugal. [Balanda, A.; Dybczak, A.; Michalska, B.; Otwinowski, J.; Przygoda, W.; Salabura, P.; Trebacz, R.; Wisniowski, M.; Wojcik, T.] Jagiellonian Univ Cracow, Smoluchowski Inst Phys, PL-30059 Krakow, Poland. [Gonzalez-Diaz, D.; Heinz, T.; Holzmann, R.; Koenig, I.; Koenig, W.; Kolb, B. W.; Lang, S.; Palka, M.; Pechenov, V.; Pietraszko, J.; Rustamov, A.; Schwab, E.; Stroth, J.; Sturm, C.; Traxler, M.; Yurevich, S.; Zumbruch, P.] GSI Helmholtzzentrum Schwerionenforschung GmbH, D-64291 Darmstadt, Germany. [Bannier, B.; Dohrmann, F.; Kaempfer, B.; Kanaki, K.; Kotte, R.; Naumann, L.; Wendisch, C.; Wuestenfeld, J.; Zhou, P.] Helmholtz Zentrum Dresden Rossendorf, Inst Strahlenphys, D-01314 Dresden, Germany. [Belyaev, A. V.; Chernenko, S.; Fateev, O. V.; Zanevsky, Y. V.] Joint Inst Nucl Res, Dubna 141980, Russia. [Froehlich, I.; Galatyuk, T.; Heilmann, M.; Lorenz, M.; Markert, J.; Michel, J.; Muentz, C.; Pachmayer, Y. C.; Stroebele, H.; Stroth, J.; Tarantola, A.; Teilab, K.] Goethe Univ Frankfurt, Inst Kernphys, D-60438 Frankfurt, Germany. [Agakishiev, G.; Destefanis, M.; Gilardi, C.; Kirschner, D.; Kuehn, W.; Lange, J. S.; Metag, V.; Mishra, D.; Pechenova, O.; Cavalcanti, T. Perez; Spataro, S.; Spruck, B.] Justus Liebig Univ Giessen, Phys Inst 2, D-35392 Giessen, Germany. [Bassini, R.; Iori, I.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Golubeva, M.; Guber, F.; Ivashkin, A.; Karavicheva, T.; Kurepin, A.; Lapidus, K.; Reshetin, A.; Sadovsky, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Boehmer, M.; Christ, T.; Eberl, T.; Epple, E.; Fabbietti, L.; Friese, J.; Gernhaeuser, R.; Huck, P.; Jurkovic, M.; Kruecken, R.; Maier, L.; Sailer, B.; Schmah, A.; Siebenson, J.; Weber, M.] Tech Univ Munich, Phys Dept E12, D-85748 Munich, Germany. [Mousa, J.; Parpottas, Y.; Tsertos, H.] Univ Cyprus, Dept Phys, CY-1678 Nicosia, Cyprus. [Boyard, J. L.; Gumberidze, M.; Hennino, T.; Liu, T.; Moriniere, E.; Ramstein, B.; Roy-Stephan, M.] Univ Paris 11, Inst Phys Nucl, CNRS, UMR 8608,IN2P3, F-91406 Orsay, France. [Krizek, F.; Kugler, A.; Sobolev, Yu. G.; Tlusty, P.; Wagner, V.] Acad Sci Czech Republic, Inst Nucl Phys, Rez 25068, Czech Republic. [Belver, D.; Cabanelas, P.; Castro, E.; Garzon, J. A.] Univ Santiago Compostela, Dept Fis Particulas, Santiago De Compostela 15706, Spain. [Diaz, J.; Gil, A.] Univ Valencia, CSIC, Inst Fis Corpuscular, Valencia 46971, Spain. [Fabbietti, L.; Lapidus, K.] Tech Univ Munich, D-85748 Garching, Germany. [Fonte, P.] ISEC Coimbra, Coimbra, Portugal. [Iori, I.] Univ Milan, Dipartimento Fis, I-20133 Milan, Italy. [Kaempfer, B.] Tech Univ Dresden, D-01062 Dresden, Germany. [Schmah, A.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Spataro, S.] Univ Torino, Dipartimento Fis Gen, I-10125 Turin, Italy. RP Agakishiev, G (reprint author), Ist Nazl Fis Nucl, Lab Nazl Sud, I-95125 Catania, Italy. EM kotte@fzd.de RI Kurepin, Alexey/H-4852-2013; Eberl, Thomas/J-4826-2016; Kruecken, Reiner/A-1640-2013; Diaz, Jose/B-3454-2012; Spataro, Stefano/E-1305-2012; Finocchiaro, Paolo/G-5625-2010; Blanco, Alberto/L-2520-2014; Ivashkin, Alexander/B-9725-2014; Guber, Fedor/I-4271-2013; Gil Ortiz, Alejandro/M-1671-2014; Golubeva, Marina/C-6154-2014; Wagner, Vladimir/G-5650-2014; Krizek, Filip/G-8967-2014; Mangiarotti, Alessio/I-1072-2012; Gonzalez Diaz, Diego/K-7265-2014; Fonte, Paulo/B-1842-2008 OI Kurepin, Alexey/0000-0002-1851-4136; Eberl, Thomas/0000-0002-5301-9106; Kruecken, Reiner/0000-0002-2755-8042; Lopes, Luis/0000-0001-8571-0033; Destefanis, Marco Giovanni Maria/0000-0003-1997-6751; Diaz, Jose/0000-0002-7239-223X; Spataro, Stefano/0000-0001-9601-405X; Ivashkin, Alexander/0000-0003-4595-5866; Guber, Fedor/0000-0001-8790-3218; Gil Ortiz, Alejandro/0000-0002-0852-412X; Mangiarotti, Alessio/0000-0001-7837-6057; Gonzalez Diaz, Diego/0000-0002-6809-5996; Fonte, Paulo/0000-0002-2275-9099 FU BMBF [06DR9059D, 06FY171, 06MT238 T5, 06MT9156 TP5]; HGF [VH-NG-330]; DFG EClust [153]; GSI TMKRUE; Hessian LOEWE initiative through HIC for FAIR (Germany); MSMT [LC07050]; GA ASCR (Czech Rep.) [IAA100480803]; KBN (Poland) [1P03B 056 26]; CPAN (Spain) [CSD2007-00042]; Cyprus [UCY-10.3.11.12]; France [CNRS/IN2P3]; INFN (Italy); EU [RII3-CT-2005-515876, HP2 227431]; [FPA2006-09154] FX The HADES collaboration gratefully acknowledges the support by BMBF grants 06DR9059D, 06FY171, 06MT238 T5, and 06MT9156 TP5, by HGF VH-NG-330, by DFG EClust 153, by GSI TMKRUE, by the Hessian LOEWE initiative through HIC for FAIR (Germany), by grants MSMT LC07050 and GA ASCR IAA100480803 (Czech Rep.), by grant KBN 1P03B 056 26 (Poland), by grants FPA2006-09154 and CPAN: CSD2007-00042 (Spain), by grant UCY-10.3.11.12 (Cyprus), by CNRS/IN2P3 (France), by INFN (Italy), and by EU contracts RII3-CT-2005-515876 and HP2 227431. NR 44 TC 4 Z9 4 U1 0 U2 13 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 EI 1434-601X J9 EUR PHYS J A JI Eur. Phys. J. A PD MAY PY 2011 VL 47 IS 5 AR 63 DI 10.1140/epja/i2011-11063-x PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 777YA UT WOS:000291659900005 ER PT J AU Moazen, BH Matei, C Bardayan, DW Blackmon, JC Chae, KY Chipps, KA Hatarik, R Jones, KL Kozub, RL Matos, M Nesaraja, CD O'Malley, PD Pain, SD Pelham, T Peters, WA Pittman, ST Shriner, JF Smith, MS AF Moazen, B. H. Matei, C. Bardayan, D. W. Blackmon, J. C. Chae, K. Y. Chipps, K. A. Hatarik, R. Jones, K. L. Kozub, R. L. Matos, M. Nesaraja, C. D. O'Malley, P. D. Pain, S. D. Pelham, T. Peters, W. A. Pittman, S. T. Shriner, J. F., Jr. Smith, M. S. TI Direct studies of low-energy resonances in P-31(p, alpha)Si-28 and Cl-35(p, alpha)S-32 SO EUROPEAN PHYSICAL JOURNAL A LA English DT Article ID NOVA NUCLEOSYNTHESIS; PRESOLAR GRAINS; SCATTERING AB Low-energy resonances in P-31(p, alpha)Si-28 and Cl-35(p, alpha)(32) S were studied directly in order to gain a better understanding of reaction cycling in the Si-Ar region in novae. New resonance strengths at E-c.m. = 600 and 622 keV in P-31(p, alpha)Si-28 were measured (omega gamma(p,alpha) = (2.2 +/- 0.7) x 10(-2) eV and omega gamma(p,alpha) = (0.99 +/- 0.08) eV, respectively) as well as the E-c.m. = 610 keV resonance in Cl-35(p, alpha)S-32 [omega gamma(p,alpha) = (1.2 +/- 0.2) x 10(-2) eV], the lowest energy that any resonance in this reaction has been observed, directly or indirectly. The strengths of these resonances were found to be lower than previously determined, resulting in even weaker cycling in the Si-Ar region. C1 [Moazen, B. H.; Chae, K. Y.; Jones, K. L.; Nesaraja, C. D.; Pittman, S. T.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Matei, C.] Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. [Bardayan, D. W.; Chae, K. Y.; Nesaraja, C. D.; Smith, M. S.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Blackmon, J. C.] Louisiana State Univ, Dept Phys, Baton Rouge, LA 70803 USA. [Chipps, K. A.; Matos, M.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. [Hatarik, R.; O'Malley, P. D.; Pain, S. D.; Peters, W. A.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Kozub, R. L.; Shriner, J. F., Jr.] Tennessee Technol Univ, Dept Phys, Cookeville, TN 38505 USA. [Pelham, T.] Univ Surrey, Dept Phys, Guildford GU2 7XH, England. RP Moazen, BH (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. EM brianmoazen@gmail.com RI Pain, Steven/E-1188-2011; Jones, Katherine/B-8487-2011; Peters, William/B-3214-2012; Matos, Milan/G-6947-2012; OI Pain, Steven/0000-0003-3081-688X; Jones, Katherine/0000-0001-7335-1379; Peters, William/0000-0002-3022-4924; Matos, Milan/0000-0003-1722-9509; Chipps, Kelly/0000-0003-3050-1298 FU National Science Foundation [NSF-PHY-00-98800]; US Department of Energy [DE-FG02-96ER40983]; University of Tennessee [DE-FG02-96ER40955]; Tennessee Technological University [DE-AC05-00OR22725]; ORNL FX This work was supported in part by the National Science Foundation under contract No. NSF-PHY-00-98800, the US Department of Energy under contract numbers DE-FG02-96ER40983 with University of Tennessee, DE-FG02-96ER40955 with Tennessee Technological University, and DE-AC05-00OR22725 with ORNL. NR 16 TC 2 Z9 2 U1 0 U2 3 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 J9 EUR PHYS J A JI Eur. Phys. J. A PD MAY PY 2011 VL 47 IS 5 AR 66 DI 10.1140/epja/i2011-11066-7 PG 7 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 777YA UT WOS:000291659900008 ER PT J AU Flaud, JM Lafferty, WJ Devi, VM Sams, RL Benner, DC AF Flaud, J. -M. Lafferty, W. J. Devi, V. Malathy Sams, R. L. Benner, D. Chris TI Absolute line intensities and self-broadened half-width coefficients in the ethylene-1-C-13 bands in the 700-1190 cm(-1) region SO JOURNAL OF MOLECULAR SPECTROSCOPY LA English DT Article DE C-13-ethylene; Intensities; Self-broadening; Pressure-broadened width coefficients; Fourier transform spectra ID NU(7) BAND; C2H4; STRATOSPHERE; SPECTRA; PLUME AB Accurate individual line intensities have been measured for the five interacting bands nu(10), nu(g), nu(7), nu(4) and nu(6) of ethylene-1-C-13 using a multispectrum nonlinear least squares fitting technique. The measured intensities have been very satisfactorily fit leading to the determination of precise vibrational transition moments. A calculated spectrum accounting for the various rovibrational interactions has been generated. Such a spectrum should be useful for the planetary atmosphere modeling-community. Lorentz self-broadened half-width coefficients have also been measured for nearly 300 transitions in the strongest nu(7) band. Published by Elsevier Inc. C1 [Lafferty, W. J.] NIST, Opt Technol Div, Gaithersburg, MD 20899 USA. [Flaud, J. -M.] Univ Paris Est, UMR CNRS 7583, LISA, IPSL, F-94010 Creteil, France. [Flaud, J. -M.] Univ Paris Diderot, LISA, UMR CNRS 7583, IPSL, F-94010 Creteil, France. [Devi, V. Malathy; Benner, D. Chris] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. [Sams, R. L.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Lafferty, WJ (reprint author), NIST, Opt Technol Div, Gaithersburg, MD 20899 USA. EM Walter.Lafferty@NIST.gov FU Department of Energy's Office of Biological and Environmental Research, Pacific Northwest National Laboratory (PNNL); Battelle Memorial Institute [DE-AC05-76RLO1830]; NASA FX All the experimental spectra for the present study were recorded at the W.R. Wiley Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at the Pacific Northwest National Laboratory (PNNL). PNNL is operated for the United States Department of Energy by the Battelle Memorial Institute under Contract DE-AC05-76RLO1830. The research at the College of William and Mary was performed under grants with NASA. The portion of this study carried out at NIST was supported by the Upper Atmospheric Research Program of NASA. One of the authors (J.M.F.) thanks the Optical Technology Division for support during his stay at NIST. Over many years, both Philip Bunker and Robert McKellar have contributed greatly to the advancement of molecular spectroscopy. NR 25 TC 10 Z9 10 U1 0 U2 8 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0022-2852 J9 J MOL SPECTROSC JI J. Mol. Spectrosc. PD MAY-JUN PY 2011 VL 267 IS 1-2 SI SI BP 3 EP 12 DI 10.1016/j.jms.2011.01.002 PG 10 WC Physics, Atomic, Molecular & Chemical; Spectroscopy SC Physics; Spectroscopy GA 778PE UT WOS:000291715800002 ER PT J AU Chang, CH Wang, Z Hall, GE Sears, TJ Xin, J AF Chang, Chih-Hsuan Wang, Zhong Hall, Gregory E. Sears, Trevor J. Xin, Ju TI Transient laser absorption spectroscopy of CH2 near 780 nm SO JOURNAL OF MOLECULAR SPECTROSCOPY LA English DT Article DE Spectra; Rotationally resolved; Vibronic; Near-infrared ID ORBITAL ANGULAR-MOMENTUM; MAGNETIC-ROTATION SPECTROSCOPY; RENNER-TELLER; SINGLET CH2; VIBRATIONAL RESONANCES; TRIATOMIC-MOLECULES; VISIBLE ABSORPTION; 1A1 STATE; SPECTRUM; TRANSITION AB Bands in the CH2 (b) over tilde B-1(1)-(a) over tilde (1)A(1) transition between 12500 and 13000 cm(-1) were recorded at Doppler-limited resolution using a transient frequency-modulation (FM) laser absorption spectrometer. Rotational levels in seven upper vibronic states: (a) over tilde (0, 11, 0)(1,3), (a) over tilde (2, 6, 0)(1), (b) over tilde (0, 2, 0)(4), (b) over tilde (1 1, 0)(1,2), and (b) over tilde (0, 3, 0)(1) were assigned with the assistance of optical-optical double resonance (OODR) and ground state combination differences. Perturbations due to rotation-vibration coupling, anharmonic couplings, e-resonance, as well as the Renner-Teller effect are discussed as sources of the irregular rotational patterns observed in the (b) over tilde (0, 3, 0)(1), (b) over tilde (1, 1, 0)(1), and (a) over tilde (0, 11, 0)(3) vibronic levels. (C) 2011 Elsevier Inc. All rights reserved. C1 [Chang, Chih-Hsuan; Hall, Gregory E.; Sears, Trevor J.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Wang, Zhong] Suffolk Cty Community Coll, Math & Sci Dept, Riverhead, NY 11901 USA. [Sears, Trevor J.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Xin, Ju] Bloomsburg Univ, Dept Phys, Bloomsburg, PA 17815 USA. RP Sears, TJ (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM sears@bnl.gov RI Hall, Gregory/D-4883-2013; Sears, Trevor/B-5990-2013 OI Hall, Gregory/0000-0002-8534-9783; Sears, Trevor/0000-0002-5559-0154 FU Brookhaven National Laboratory [DE-AC02-98CH10886]; US Department of Energy, Office of Science [DE-AC02-98CH10886]; Division of Chemical Sciences, Geosciences, and Biosciences within the Office of Basic Energy Sciences FX This work was carried out at Brookhaven National Laboratory under Contract No. DE-AC02-98CH10886 with the US Department of Energy, Office of Science, and supported by its Division of Chemical Sciences, Geosciences, and Biosciences within the Office of Basic Energy Sciences. J. Xin thanks the Educational Programs Office at Brookhaven National Laboratory for support from a Faculty and Teams summer program. NR 25 TC 1 Z9 1 U1 2 U2 8 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0022-2852 EI 1096-083X J9 J MOL SPECTROSC JI J. Mol. Spectrosc. PD MAY-JUN PY 2011 VL 267 IS 1-2 SI SI BP 50 EP 57 DI 10.1016/j.jms.2011.02.004 PG 8 WC Physics, Atomic, Molecular & Chemical; Spectroscopy SC Physics; Spectroscopy GA 778PE UT WOS:000291715800008 ER PT J AU Rosenbloom, MH Alkalay, A Agarwal, N Baker, SL O'Neil, JP Janabi, M Yen, IV Growdon, M Jang, J Madison, C Mormino, EC Rosen, HJ Gorno-Tempini, ML Weiner, MW Miller, BL Jagust, WJ Rabinovici, GD AF Rosenbloom, M. H. Alkalay, A. Agarwal, N. Baker, S. L. O'Neil, J. P. Janabi, M. Yen, I. V. Growdon, M. Jang, J. Madison, C. Mormino, E. C. Rosen, H. J. Gorno-Tempini, M. L. Weiner, M. W. Miller, B. L. Jagust, W. J. Rabinovici, G. D. TI Distinct clinical and metabolic deficits in PCA and AD are not related to amyloid distribution SO NEUROLOGY LA English DT Article ID POSTERIOR CORTICAL ATROPHY; PITTSBURGH COMPOUND-B; PRIMARY-PROGRESSIVE-APHASIA; ONSET ALZHEIMERS-DISEASE; GLUCOSE-METABOLISM; 3 VARIANTS; PET; BRAIN; DEMENTIA; COGNITION AB Background/Objective: Patients with posterior cortical atrophy (PCA) often have Alzheimer disease (AD) at autopsy, yet are cognitively and anatomically distinct from patients with clinical AD. We sought to compare the distribution of beta-amyloid and glucose metabolism in PCA and AD in vivo using Pittsburgh compound B (PiB) and FDG-PET. Methods: Patients with PCA (n = 12, age 57.5 +/- 7.4, Mini-Mental State Examination [MMSE] 22.2 +/- 5.1), AD (n = 14, age 58.8 +/- 9.6, MMSE 23.8 +/- 6.7), and cognitively normal controls (NC, n = 30, age 73.6 +/- 6.4) underwent PiB and FDG-PET. Group differences in PiB distribution volume ratios (DVR, cerebellar reference) and FDG uptake (pons-averaged) were assessed on a voxel-wise basis and by comparing binding in regions of interest (ROIs). Results: Compared to NC, both patients with AD and patients with PCA showed diffuse PiB uptake throughout frontal, temporoparietal, and occipital cortex (p < 0.0001). There were no regional differences in PiB binding between PCA and AD even after correcting for atrophy. FDG patterns in PCA and AD were distinct: while both groups showed hypometabolism compared to NC in temporoparietal cortex and precuneus/posterior cingulate, patients with PCA further showed hypometabolism in inferior occipitotemporal cortex compared to both NC and patients with AD (p < 0.05). Patients with AD did not show areas of relative hypometabolism compared to PCA. Conclusions: Fibrillar amyloid deposition in PCA is diffuse and similar to AD, while glucose hypometabolism extends more posteriorly into occipital cortex. Further studies are needed to determine the mechanisms of selective network degeneration in focal variants of AD. Neurology (R) 2011;76:1789-1796 C1 [Rosenbloom, M. H.; Alkalay, A.; Growdon, M.; Jang, J.; Rosen, H. J.; Gorno-Tempini, M. L.; Miller, B. L.; Jagust, W. J.; Rabinovici, G. D.] Univ Calif San Francisco, Memory & Aging Ctr, San Francisco, CA 94143 USA. [Rosenbloom, M. H.; Alkalay, A.; Growdon, M.; Jang, J.; Rosen, H. J.; Gorno-Tempini, M. L.; Miller, B. L.; Jagust, W. J.; Rabinovici, G. D.] Univ Calif San Francisco, Dept Neurol, San Francisco, CA 94143 USA. [Alkalay, A.; Agarwal, N.; Madison, C.; Mormino, E. C.; Jagust, W. J.; Rabinovici, G. D.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Baker, S. L.; O'Neil, J. P.; Janabi, M.; Yen, I. V.; Jagust, W. J.; Rabinovici, G. D.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Weiner, M. W.] Dept Vet Affairs Med Ctr, Ctr Imaging Neurodegenerat Dis, San Francisco, CA USA. RP Rosenbloom, MH (reprint author), HealthPartner Specialty Ctr, Ctr Dementia & Alzheimers Care, 401 Phalen Blvd,Mail Stop 41104C, St Paul, MN 55130 USA. EM Michael.H.Rosenbloom@HealthPartners.com RI Gorno-Tempini, Maria Luisa/E-7203-2012 FU NIH/NIA [K23-AG031861, R01-AG027859, P01-AG1972403, P50 AG023501]; Alzheimer's Association [NIRG-07-59422, ZEN-08-87090]; John Douglas French Alzheimer's Foundation; State of California DHS-ADRC [04-33516] FX Supported by the NIH/NIA K23-AG031861, R01-AG027859, P01-AG1972403, P50 AG023501, Alzheimer's Association NIRG-07-59422, ZEN-08-87090, John Douglas French Alzheimer's Foundation, and State of California DHS-ADRC 04-33516. NR 40 TC 55 Z9 57 U1 0 U2 5 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA 530 WALNUT ST, PHILADELPHIA, PA 19106-3621 USA SN 0028-3878 J9 NEUROLOGY JI Neurology PD MAY PY 2011 VL 76 IS 21 BP 1789 EP 1796 PG 8 WC Clinical Neurology SC Neurosciences & Neurology GA 768AY UT WOS:000290904800006 PM 21525424 ER PT J AU Thorn, DB Gumberidze, A Trotsenko, S Banas, D Beyer, H Bostock, CJ Bray, I Chen, W DuBois, R Fontes, CJ Fritzsche, S Fursa, DV Grisenti, R Geyer, S Hagmann, S Hess, S Hegewald, M Kozhuharov, C Martin, R Orban, I Petridis, N Reuschl, R Simon, A Spillmann, U Surzhykov, A Trassinelli, M Weber, G Winters, DFA Winters, N Zhang, HL Stohlker, T AF Thorn, D. B. Gumberidze, A. Trotsenko, S. Banas, D. Beyer, H. Bostock, C. J. Bray, I. Chen, W. DuBois, R. Fontes, C. J. Fritzsche, S. Fursa, D. V. Grisenti, R. Geyer, S. Hagmann, S. Hess, S. Hegewald, M. Kozhuharov, C. Maertin, R. Orban, I. Petridis, N. Reuschl, R. Simon, A. Spillmann, U. Surzhykov, A. Trassinelli, M. Weber, G. Winters, D. F. A. Winters, N. Zhang, H. L. Stoehlker, Th. TI Polarization and anisotropic emission of K-shell radiation from heavy few electron ions SO CANADIAN JOURNAL OF PHYSICS LA English DT Article ID GENERALIZED BREIT INTERACTION; HE-LIKE; EXCITATION; SUBLEVELS; CAPTURE; URANIUM; IMPACT; TARGET AB The population of magnetic sublevels in hydrogen-like uranium ions has been investigated in relativistic ion-atom collisions by observing the subsequent X-ray emission. Using the gas target at the experimental storage ring facility we observed the angular emission of Lyman-alpha radiation from hydrogen-like uranium ions. The alignment parameter for three different interaction energies was measured and found to agree well with theory. In addition, the use of different gas targets allowed for the electron-impact excitation process to be observed. C1 [Thorn, D. B.; Gumberidze, A.] GSI Helmholtzzentrum Schwerionenforsch, Div Res, EMMI, D-64291 Darmstadt, Germany. [Thorn, D. B.; Gumberidze, A.; Fritzsche, S.; Maertin, R.; Winters, N.] FIAS, D-60438 Frankfurt, Germany. [Trotsenko, S.; Weber, G.] Helmholtz Inst Jena, D-07743 Jena, Germany. [Banas, D.] Jan Kochanowski Univ Humanities & Sci, PL-25314 Kielce, Poland. [Bostock, C. J.; Bray, I.; Fursa, D. V.] Curtin Univ, Perth, WA, Australia. [DuBois, R.] Univ Missouri, Rolla, MO 65409 USA. [Fontes, C. J.; Zhang, H. L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Fritzsche, S.] Univ Oulu, Dept Phys Sci, Oulu 90014, Finland. [Grisenti, R.; Geyer, S.; Hagmann, S.; Hegewald, M.; Petridis, N.] Goethe Univ Frankfurt, Inst Kernphys, D-60438 Frankfurt, Germany. [Maertin, R.; Surzhykov, A.; Winters, D. F. A.; Winters, N.; Stoehlker, Th.] Univ Heidelberg, Inst Phys, D-69120 Heidelberg, Germany. [Orban, I.] Stockholms Univ, S-10691 Stockholm, Sweden. [Reuschl, R.; Trassinelli, M.] Inst NanoSci Paris, F-75005 Paris, France. [Simon, A.] Jagiellonian Univ, PL-31007 Krakow, Poland. [Stoehlker, Th.] Helmholtz Inst Jena, D-07743 Jena, Germany. RP Thorn, DB (reprint author), GSI Helmholtzzentrum Schwerionenforsch, Div Res, EMMI, D-64291 Darmstadt, Germany. EM dbthorn@gsi.de RI Fursa, Dmitry/C-2301-2009; Bray, Igor/B-8586-2009; Winters, Danyal/A-2933-2013; Bostock, Christopher/B-2413-2013; Banas, Dariusz/F-5025-2011; Trassinelli, Martino/M-5326-2016 OI Fursa, Dmitry/0000-0002-3951-9016; Bray, Igor/0000-0001-7554-8044; Bostock, Christopher/0000-0001-7141-5252; Banas, Dariusz/0000-0003-1566-5446; Trassinelli, Martino/0000-0003-4414-1801 FU Helmholtz Association [HA216/EMMI, VH-NG-421]; Polish Ministry of Education and Science [N N202 463539] FX We would like to thank U. Popp for help in running the gas jet target and W. Enders in the setup of the experiment. This work was supported in part by the Alliance Program of the Helmholtz Association (HA216/EMMI). DB acknowledges the support by the Polish Ministry of Education and Science under Grant No. N N202 463539. AS acknowledges support from the Helmholtz Association under the Project No. VH-NG-421. NR 16 TC 3 Z9 3 U1 0 U2 8 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 1200 MONTREAL ROAD, BUILDING M-55, OTTAWA, ON K1A 0R6, CANADA SN 0008-4204 J9 CAN J PHYS JI Can. J. Phys. PD MAY PY 2011 VL 89 IS 5 BP 513 EP 519 DI 10.1139/P11-033 PG 7 WC Physics, Multidisciplinary SC Physics GA 775QH UT WOS:000291476700005 ER PT J AU Csanak, G Fontes, CJ Kilcrease, DP Fursa, DV AF Csanak, G. Fontes, C. J. Kilcrease, D. P. Fursa, D. V. TI Creation, destruction, and transfer of atomic multipole moments by electron scattering: relativistic treatment SO CANADIAN JOURNAL OF PHYSICS LA English DT Article ID POLARIZATION; FOUNDATIONS; SYSTEMS; HELIUM; PLASMA; STATES; BODY; SPIN AB We have obtained expressions for the creation, destruction, and transfer of atomic multipole moments by electron scattering under relativistic conditions. More specifically, we have obtained separate expressions for different-level processes (inelastic scattering) and for same-level processes (elastic and inelastic scattering). The cross sections for different-level processes are expressed in terms of inelastic magnetic sublevel cross sections, except for the coherence transfer cross section, which is expressed in terms of an angular integral of a product of inelastic magnetic sublevel amplitudes. The same-level cross sections are expressed in terms of the imaginary part of the elastic forward scattering amplitude and in terms of elastic scattering magnetic sublevel cross sections, except for the coherence transfer cross section, which is expressed in terms of the (complex) forward elastic scattering amplitudes and an angular integral of a product of elastic scattering magnetic sublevel amplitudes. If the collisional model supports the optical theorem, then the same-level cross sections can be rewritten in such a form that they are broken up into two parts: an elastic scattering part and an inelastic scattering part. In carrying out this work, we have used the density matrix formalism of Fano and Blum in combination with the electron scattering formalism of Gell-Mann and Goldberger. C1 [Fontes, C. J.] Los Alamos Natl Lab, Computat Phys Div, Los Alamos, NM 87545 USA. [Csanak, G.; Kilcrease, D. P.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Fursa, D. V.] Curtin Univ Technol, ARC Ctr Antimatter Matter Studies, Perth, WA 6845, Australia. RP Fontes, CJ (reprint author), Los Alamos Natl Lab, Computat Phys Div, POB 1663, Los Alamos, NM 87545 USA. EM cjf@lanl.gov RI Fursa, Dmitry/C-2301-2009; OI Fursa, Dmitry/0000-0002-3951-9016; Kilcrease, David/0000-0002-2319-5934 FU U. S. Department of Energy; Australian Research Council FX The authors want to thank to Dr. Peter Hakel from the University of Nevada, Reno for helpful comments on the original manuscript. This work was supported by the the U. S. Department of Energy and the Australian Research Council. NR 41 TC 3 Z9 3 U1 0 U2 1 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 1200 MONTREAL ROAD, BUILDING M-55, OTTAWA, ON K1A 0R6, CANADA SN 0008-4204 J9 CAN J PHYS JI Can. J. Phys. PD MAY PY 2011 VL 89 IS 5 BP 521 EP 531 DI 10.1139/P11-029 PG 11 WC Physics, Multidisciplinary SC Physics GA 775QH UT WOS:000291476700006 ER PT J AU Clementson, J Beiersdorfer, P Brown, GV Gu, MF Lundberg, H Podpaly, Y Trabert, E AF Clementson, J. Beiersdorfer, P. Brown, G. V. Gu, M. F. Lundberg, H. Podpaly, Y. Traebert, E. TI Tungsten spectroscopy at the Livermore electron beam ion trap facility SO CANADIAN JOURNAL OF PHYSICS LA English DT Review ID SOFT-X-RAY; HIGHLY IONIZED TUNGSTEN; EBIT CALORIMETER SPECTROMETER; MANY-BODY CALCULATIONS; LASER-PRODUCED PLASMAS; ENERGY-LEVEL SCHEME; NI-LIKE IONS; TRANSITION-PROBABILITIES; EXTREME-ULTRAVIOLET; RESONANCE LINES AB The utilization of tungsten spectroscopy for diagnostics of magnetically confined fusion plasmas requires the radiative properties of tungsten ions to be accurately known. At the Lawrence Livermore National Laboratory, a program to gather spectroscopic data on tungsten ions has been initiated with the purpose to study spectral signatures and identify candidate fusion plasma diagnostics. In this paper, an overview of recent results from the Livermore WOLFRAM spectroscopy project is presented, which includes experimental investigations at the EBIT-I and SuperEBIT electron beam ion traps. In particular, the spectra of highly charged M-and L-shell tungsten ions have been studied. These investigations cover energy measurements of n = 2 to n = 2, 3 transitions in Ne-like W64+ through Li-like W71+ ions and soft X-ray measurements of n = 3 to n = 3, 4 transitions in M-shell ions with emphasis on the Ni-like W46+ and Si-like W60+ through Na-like W63+ ions. The measurements are complemented by atomic-structure calculations and spectral modeling using the Flexible Atomic Code (FAC). C1 [Clementson, J.; Beiersdorfer, P.; Brown, G. V.; Traebert, E.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Gu, M. F.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Lundberg, H.] Lund Univ, SE-22100 Lund, Sweden. [Podpaly, Y.] MIT Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. RP Clementson, J (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM clementson@llnl.gov FU United States Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA-27344]; LDRD [09-ERD-016] FX This work was performed under the auspices of the United States Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA-27344 and supported by LDRD project 09-ERD-016. The authors would like to acknowledge technical support from Ed Magee and helpful input from Dr. Alexander Kramida. Joel Clementson would like to acknowledge support from Professor Sune Svanberg, Dr. Sven Huldt, Dr. Christoph Biedermann, Professor Roger Hutton, Professor Claes-Goran Wahlstrom, and the late Professor Sveneric Johansson. NR 90 TC 30 Z9 31 U1 0 U2 11 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 1200 MONTREAL ROAD, BUILDING M-55, OTTAWA, ON K1A 0R6, CANADA SN 0008-4204 J9 CAN J PHYS JI Can. J. Phys. PD MAY PY 2011 VL 89 IS 5 BP 571 EP 580 DI 10.1139/P11-028 PG 10 WC Physics, Multidisciplinary SC Physics GA 775QH UT WOS:000291476700009 ER PT J AU Safronova, UI Safronova, AS Beiersdorfer, P AF Safronova, U. I. Safronova, A. S. Beiersdorfer, P. TI Dielectronic recombination and satellite line spectra of highly charged tungsten ions SO CANADIAN JOURNAL OF PHYSICS LA English DT Article ID MANY-BODY CALCULATIONS; AR-LIKE TUNGSTEN; GA-LIKE IONS; TRANSITION-PROBABILITIES; X-RAY; RATE COEFFICIENTS; EXCITED-STATES; NI; WAVELENGTHS; RATES AB We present our recent progress on theoretical studies that involve auto-ionizing states of highly charged tungsten ions. Such auto-ionizing states have two channels for decay, which requires that both radiative and auto-ionization atomic data be calculated and combined in a detailed study of the dielectronic recombination (DR). Three atomic codes are used to produce relativistic atomic data (energy levels, radiative transition probabilities, and auto-ionization rates). These are the relativistic many-body perturbation theory (RMBPT) code, the multiconfiguration relativistic Hebrew University Lawrence Livermore atomic code (HULLAC), and the Hartree-Fock relativistic (Cowan) code. Branching ratios relative to the first threshold and intensity factors are calculated for satellite lines, and DR rate coefficients are determined for the excited states. The total DR rate coefficient is derived as a function of electron temperature, and it is shown that the contribution of the highly excited states is very important for the calculation of the total DR rates. Synthetic dielectronic satellite spectra are constructed, and the atomic properties specific to the relevant tungsten ions are highlighted. First, we will consider the results for Na-like tungsten (W(63+)) and Mg-like tungsten (W(62+)) using all three codes. Then, we move to even higher ionization states and present the results in Li-like W (W(71+)). For this we use the RMBPT code as well as the quasi-relativistic many-body perturbation theory (MZ) code. The inclusion of the DR process is essential for correct identification of the lines in impurity spectra and for understanding the main contributions to the total radiation losses. C1 [Safronova, U. I.; Safronova, A. S.] Univ Nevada, Dept Phys, Reno, NV 89557 USA. [Beiersdorfer, P.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. RP Safronova, UI (reprint author), Univ Nevada, Dept Phys, Reno, NV 89557 USA. EM ulyanas@unr.edu FU DOE under OFES [DE-FG02-08ER54951]; DOE under NNSA [DE-FC52-06NA27588]; DOE [DE-AC52-07NA2344] FX This research was sponsored by DOE under OFES grant DE-FG02-08ER54951 and in part under the NNSA Cooperative agreement DE-FC52-06NA27588. Work at the Lawrence Livermore National Laboratory was performed under auspices of the DOE under contract DE-AC52-07NA2344. NR 57 TC 7 Z9 8 U1 1 U2 5 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 1200 MONTREAL ROAD, BUILDING M-55, OTTAWA, ON K1A 0R6, CANADA SN 0008-4204 J9 CAN J PHYS JI Can. J. Phys. PD MAY PY 2011 VL 89 IS 5 BP 581 EP 589 DI 10.1139/P10-114 PG 9 WC Physics, Multidisciplinary SC Physics GA 775QH UT WOS:000291476700010 ER PT J AU Podpaly, YA Rice, JE Beiersdorfer, P Reinke, ML Clementson, J Barnard, HS AF Podpaly, Y. A. Rice, J. E. Beiersdorfer, P. Reinke, M. L. Clementson, J. Barnard, H. S. TI Tungsten measurement on Alcator C-Mod and EBIT for future fusion reactors SO CANADIAN JOURNAL OF PHYSICS LA English DT Article ID SPECTRA; PLASMAS; RADIATION AB Tungsten will be an important element in nearly all future fusion reactors because of its presence in plasma facing components. This makes tungsten a good candidate for a diagnostic element for ion temperature and toroidal velocity measurement, and it makes understanding tungsten emissions important for tokamak power balance. The effect of tungsten on tokamak plasmas is investigated at the Alcator C-Mod tokamak using VUV, bolometry, and soft X-ray spectroscopy. Tungsten was present in Alcator C-Mod as a plasma facing component and through laser blow-off impurity injection. Quasi-continuum emission previously seen at other tokamaks has been identified. Theoretical predictions are presented of tungsten emission that could be expected in future Alcator C-Mod measurements. Furthermore, spectra of highly charged tungsten ions have been studied at the SuperEBIT electron beam ion trap. This emission could prove useful for spectroscopic diagnostics of future high-temperature fusion reactor plasmas. C1 [Podpaly, Y. A.; Rice, J. E.; Reinke, M. L.; Barnard, H. S.] MIT Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. [Beiersdorfer, P.; Clementson, J.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. RP Podpaly, YA (reprint author), MIT Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. EM ypodpaly@mit.edu FU US Department of Energy; Oak Ridge Associated Universities; Department of Energy [DE-AC52-07NA-27344, DE-FC02-99ER54512]; Laboratory Directed Research and Development [09-ERD-016] FX The authors would like to thank M. F. Gu, G. V. Brown, E. W. Magee, A. Bader, C. Gao, L. Delgado-Aparicio, M. Bitter, K. Hill, and E. Marmar for their help with this work. This work was supported by Fusion Energy Sciences Program, administered by Oak Ridge Institute for Science and Education under a contract between the US Department of Energy and the Oak Ridge Associated Universities, the Department of Energy under Contract No. DE-AC52-07NA-27344 and the Laboratory Directed Research and Development program under Project No. 09-ERD-016, and the Department of Energy under Contract No. DE-FC02-99ER54512. NR 30 TC 8 Z9 8 U1 0 U2 9 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 1200 MONTREAL ROAD, BUILDING M-55, OTTAWA, ON K1A 0R6, CANADA SN 0008-4204 J9 CAN J PHYS JI Can. J. Phys. PD MAY PY 2011 VL 89 IS 5 BP 591 EP 597 DI 10.1139/P11-038 PG 7 WC Physics, Multidisciplinary SC Physics GA 775QH UT WOS:000291476700011 ER PT J AU Osborne, GC Safronova, AS Kantsyrev, VL Safronova, UI Beiersdorfer, P Williamson, KM Weller, ME Shrestha, I AF Osborne, G. C. Safronova, A. S. Kantsyrev, V. L. Safronova, U. I. Beiersdorfer, P. Williamson, K. M. Weller, M. E. Shrestha, I. TI Spectroscopic analysis and modeling of tungsten EBIT and Z-pinch plasma experiments SO CANADIAN JOURNAL OF PHYSICS LA English DT Article ID LASER-PRODUCED PLASMAS; X-RAY-SPECTRA; IONS; CLASSIFICATION; TRANSITIONS; RATES; ATOMS; RE; TM AB Spectral tungsten data taken on an electron beam ion trap (EBIT) at Lawrence Livermore National Laboratory are analyzed between 3 and 8 angstrom for electron beam energies between 2.5 and 4.1 keV. The advantage of using charge state balancing with the experimental EBIT spectra for the identification of lines is employed and discussed. Theoretical Hebrew University Lawrence Livermore Atomic Code (HULLAC) modeling is then benchmarked against the experimental EBIT results. In particular, Co-, Ni-, Zn-, Cu-, Ga-, and Ge-like transitions were modeled independently using HULLAC to aid in charge state balancing. This model is then compared with Z-pinch plasma data collected on Zebra, the 1.6 MA pulse power generator located in the Nevada Terawatt Facility at the University of Nevada, Reno. The model is used to calculate charge balance and average ionization levels of these experimental plasma results, with particular focus on planar tungsten arrays. C1 [Osborne, G. C.; Safronova, A. S.; Kantsyrev, V. L.; Safronova, U. I.; Williamson, K. M.; Weller, M. E.; Shrestha, I.] Univ Nevada, Dept Phys, Reno, NV 89557 USA. [Beiersdorfer, P.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Osborne, GC (reprint author), Univ Nevada, Dept Phys, Reno, NV 89557 USA. EM Osborne@physics.unr.edu FU DOE [DE-FG02-08ER54951, DE-AC52-07NA-27344]; NNSA [DE-FC52-06NA27588, DE-FC52-06NA27586]; LORD [09-ERD-016] FX A special acknowledgement is extended to Dr. Kramida for his many suggestions and aid in development of this paper. This work was supported by the DOE under Grant No. DE-FG02-08ER54951 and in part under NNSA Cooperative Agreements DE-FC52-06NA27588 and DE-FC52-06NA27586. Work at LLNL was performed under the auspices of the DOE under contract DE-AC52-07NA-27344 and supported under LORD project 09-ERD-016. NR 21 TC 11 Z9 11 U1 1 U2 4 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 1200 MONTREAL ROAD, BUILDING M-55, OTTAWA, ON K1A 0R6, CANADA SN 0008-4204 J9 CAN J PHYS JI Can. J. Phys. PD MAY PY 2011 VL 89 IS 5 BP 599 EP 608 DI 10.1139/P11-026 PG 10 WC Physics, Multidisciplinary SC Physics GA 775QH UT WOS:000291476700012 ER PT J AU Graf, AT May, MJ Beiersdorfer, P AF Graf, A. T. May, M. J. Beiersdorfer, P. TI A visible spectral survey from the Alcator C-Mod tokamak SO CANADIAN JOURNAL OF PHYSICS LA English DT Article ID SCRAPE-OFF-LAYER; PROFILE MEASUREMENTS; DIVERTOR; RECOMBINATION; EMISSION; EDGE; TURBULENCE; PLASMA; BEAM; TFTR AB A visible spectral survey (3675-6744 angstrom) from the Alcator C-Mod tokamak has been performed using a high-resolution visible spectrometer constructed at the Lawrence Livermore National Laboratory. The Alcator C-Mod deuterium plasma is shown to have visible emission from numerous atomic species and low charge state ions including, D I, B II-III, B V, C II-III, N II-III, O II-IV, F II-III, Ne I, Na X, Al II-III, Si I-II, Cl II-III, Ar I-III, Ar X, Ti I and III, Fe I-III, Cu I, and III, Mo I, and W I. Nearly all of the emission is thought to come from the cooler edge of the plasma including the scrape-off layer, outside of the last closed magnetic flux surface. However, there is at least one example, included here, where intrinsic visible emission persists deeper into the plasma. C1 [Graf, A. T.; May, M. J.; Beiersdorfer, P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Graf, AT (reprint author), Lawrence Livermore Natl Lab, L-490,7000 East Ave, Livermore, CA 94550 USA. EM graf2@llnl.gov FU US Department of Energy by Lawrence Livermore National Laboratory [DEAC52-07NA27344] FX Thanks are extended to the Alcator C-Mod team for excellent operation of the tokamak. Also much appreciation is given to Jim Terry for his help in the integration of this spectrometer into the C-Mod diagnostic suite. This work was performed under the auspices of the US Department of Energy by the Lawrence Livermore National Laboratory under Contract No. DEAC52-07NA27344. NR 36 TC 2 Z9 2 U1 0 U2 3 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 1200 MONTREAL ROAD, BUILDING M-55, OTTAWA, ON K1A 0R6, CANADA SN 0008-4204 J9 CAN J PHYS JI Can. J. Phys. PD MAY PY 2011 VL 89 IS 5 BP 615 EP 626 DI 10.1139/P11-005 PG 12 WC Physics, Multidisciplinary SC Physics GA 775QH UT WOS:000291476700014 ER PT J AU Hansen, SB AF Hansen, S. B. TI Configuration interaction in statistically complete hybrid-structure atomic models SO CANADIAN JOURNAL OF PHYSICS LA English DT Article ID TRANSITION ARRAYS; SPECTRA; IONS AB Configuration interaction can have significant effects on the transition energies and strengths of diagnostically important X-ray emission lines and features. However, including full configuration interaction (CI) effects by computing extensive collections of fine structure (LS term) levels may be computationally prohibitive for complex ions. In this paper, we show that CI effects in a simple ion vary little with the configuration of spectator electrons, and that CI effects in complex ions are fairly consistent from one ionization stage to the next, particularly for highly charged ions. Therefore, we argue that the CI effects within an ion can be approximated by extending the CI effects computed from a small subset of configurations in that ion to all transitions of the type (nlj)-(nlj)' in that ion, regardless of the spectator electron. This approach to CI enforces consistency between the fine structure and averaged states in hybrid-structure atomic models, which are designed to provide a computationally efficient balance of spectroscopic accuracy and statistical completeness. C1 Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Hansen, SB (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM sbhanse@sandia.gov FU United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The author thanks Jacqes Bauche and Claire Bauche-Arnoult for their many contributions to the ideas underlying this approach to hybrid-structure modeling, and C. Fontes, H. Scott, B. Wilson, and M. F. Gu for valuable discussions. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 16 TC 11 Z9 11 U1 0 U2 6 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 1200 MONTREAL ROAD, BUILDING M-55, OTTAWA, ON K1A 0R6, CANADA SN 0008-4204 J9 CAN J PHYS JI Can. J. Phys. PD MAY PY 2011 VL 89 IS 5 BP 633 EP 638 DI 10.1139/P11-006 PG 6 WC Physics, Multidisciplinary SC Physics GA 775QH UT WOS:000291476700016 ER PT J AU Trabert, E Clementson, J Beiersdorfer, P Santana, JA Ishikawa, Y AF Traebert, Elmar Clementson, Joel Beiersdorfer, Peter Santana, Juan A. Ishikawa, Yasuyuki TI Measurements and calculations of Zn-like heavy ions: an update SO CANADIAN JOURNAL OF PHYSICS LA English DT Article ID SOFT-X-RAY; CU-LIKE IONS; ENERGY-LEVELS; ISOELECTRONIC SEQUENCE; SPECTRAL-LINES; ATOMIC DATA; NA-LIKE; TRAP; TRANSITIONS; WAVELENGTHS AB Previous observations of Zn-like ions of elements Yb (Z = 70) through U (Z = 92) in an electron beam ion trap differed (by value and by isoelectronic trend) from the (less precise) results of laser-produced plasma experiments and highlighted the need for much better calculations of ions with more than one electron in the valence shell. We review the progress since achieved and present new calculations for ions in the above range as well as EBIT observations of Zn-like Pt(48+) ions (Z = 78). We identify accurate ab initio calculations that agree with the EBIT data as well as recent calculations that clearly fall short. C1 [Traebert, Elmar; Clementson, Joel; Beiersdorfer, Peter] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. [Traebert, Elmar] Ruhr Univ Bochum, Fak Phys & Astron, Astron Inst, D-44780 Bochum, Germany. [Santana, Juan A.; Ishikawa, Yasuyuki] Univ Puerto Rico, Dept Chem, Rio Piedras, PR 00931 USA. RP Trabert, E (reprint author), Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. EM traebert@astro.rub.de RI Santana, Juan A./G-4329-2011 OI Santana, Juan A./0000-0003-2349-6312 FU Deutsche Forschungsgemeinschaft (DFG); US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX ET acknowledges support by the Deutsche Forschungsgemeinschaft (DFG). Some of this work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 52 TC 3 Z9 3 U1 1 U2 5 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 1200 MONTREAL ROAD, BUILDING M-55, OTTAWA, ON K1A 0R6, CANADA SN 0008-4204 J9 CAN J PHYS JI Can. J. Phys. PD MAY PY 2011 VL 89 IS 5 BP 639 EP 645 DI 10.1139/P10-116 PG 7 WC Physics, Multidisciplinary SC Physics GA 775QH UT WOS:000291476700017 ER PT J AU Zulick, C Dollar, F Chen, H Falk, K Gregori, G Hazi, A Murphy, CD Park, J Seely, J Szabo, CI Tommasini, R Shepherd, R Krushelnick, K AF Zulick, C. Dollar, F. Chen, H. Falk, K. Gregori, G. Hazi, A. Murphy, C. D. Park, J. Seely, J. Szabo, C. I. Tommasini, R. Shepherd, R. Krushelnick, K. TI K-shell spectroscopy of Au plasma generated with a short-pulse laser SO CANADIAN JOURNAL OF PHYSICS LA English DT Article AB The production of X-rays from electron transitions into K-shell vacancies (K(alpha,beta)) emission) is a well-known process in atomic physics and has been extensively studied as a plasma diagnostic in low-and mid-Z materials. However, X-ray spectra from near neutral high-Z ions are very complex, and their interpretation requires the use of state-of-the-art atomic calculations. In this experiment, the Titan laser system at Lawrence Livermore National Laboratory was used to deliver an approximately 350 J laser pulse, with a 10 ps duration and a wavelength of 1054 nm, to a gold (Au) target. A transparent bent quartz crystal spectrometer with a hard X-ray energy window, ranging from 17 to 102 keV, was used to measure the emission spectrum. K(alpha 1,alpha 2) and K(beta 1,gamma 1) transitions were observed over a range of target sizes. Additionally, a series of shots were conducted with a pre-ionizing long pulse (3 ns, 1-10 J, 527 nm) on the backside of the target. FLYCHK, an atomic non-LTE code, designed to provide ionization and population distributions, was used to model the experiment. K(alpha)/K(beta) ratios were found to be in good agreement with the predicted value for room temperature Au targets. C1 [Zulick, C.; Dollar, F.; Krushelnick, K.] Univ Michigan, Ctr Ultrafast Opt Sci, Ann Arbor, MI 48109 USA. [Chen, H.; Hazi, A.; Park, J.; Tommasini, R.; Shepherd, R.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Falk, K.; Gregori, G.; Murphy, C. D.] Univ Oxford, Clarendon Lab, Oxford OX1 3PU, England. [Seely, J.; Szabo, C. I.] USN, Div Space Sci, Res Lab, Washington, DC 20375 USA. RP Zulick, C (reprint author), Univ Michigan, Ctr Ultrafast Opt Sci, Ann Arbor, MI 48109 USA. EM czulick@umich.edu RI Dollar, Franklin/C-9214-2013; Tommasini, Riccardo/A-8214-2009; Falk, Katerina/D-2369-2017 OI Dollar, Franklin/0000-0003-3346-5763; Tommasini, Riccardo/0000-0002-1070-3565; Falk, Katerina/0000-0001-5975-776X FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; [LDRD-09-LW-080] FX Part of this work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344, as part of a project funded by LDRD-09-LW-080. NR 10 TC 2 Z9 2 U1 2 U2 10 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 1200 MONTREAL ROAD, BUILDING M-55, OTTAWA, ON K1A 0R6, CANADA SN 0008-4204 J9 CAN J PHYS JI Can. J. Phys. PD MAY PY 2011 VL 89 IS 5 BP 647 EP 651 DI 10.1139/P11-034 PG 5 WC Physics, Multidisciplinary SC Physics GA 775QH UT WOS:000291476700018 ER PT J AU Beiersdorfer, P Brown, GV Kamp, JB Magee, EW Lepson, JK Podpaly, Y Reinke, ML AF Beiersdorfer, P. Brown, G. V. Kamp, J. B. Magee, E. W. Lepson, J. K. Podpaly, Y. Reinke, M. L. TI Measuring plasma impurities in Alcator C-Mod as a function of time in the extreme ultraviolet SO CANADIAN JOURNAL OF PHYSICS LA English DT Article ID TRANSMISSION GRATING SPECTROMETER; X-RAY REGION; SPECTROSCOPY; ASTROPHYSICS; EMISSION; CAPELLA; SPECTRA; FE AB A flat-field grazing-incidence grating spectrometer has been installed on the MIT Alcator C-MOD tokamak, following the installation of such a spectrometer on the Livermore electron beam ion trap facility and on the National Spherical Torus Experiment at Princeton. The spectrometer employs a variable space grating with an average spacing of 2400 lines/mm and covers the 10-70 angstrom wavelength band. It is being used to monitor the presence of impurity ions such as boron, oxygen, fluorine, argon, calcium, iron, molybdenum, and tungsten, and to calibrate spectral diagnostics of astrophysical plasmas. The Alcator instrument provides spectral emission data in a density regime that is one to three orders of magnitude higher than that covered by the other two instruments and thus produces complementary data. C1 [Beiersdorfer, P.; Brown, G. V.; Kamp, J. B.; Magee, E. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Lepson, J. K.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Podpaly, Y.; Reinke, M. L.] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. RP Beiersdorfer, P (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM beiersdorfer1@llnl.gov FU US Department of Energy by the Massachusetts Institute of Technology [DE-FC0299ER54512]; US Department of Energy by the Lawrence Livermore National Laboratory [DE-AC52-07NA-27344]; Office of Fusion Energy Sciences (FES) Basic and Applied Plasma Science Initiative FX This work was performed under the auspices of the US Department of Energy under Contact number DE-FC0299ER54512 by the Massachusetts Institute of Technology and DE-AC52-07NA-27344 by the Lawrence Livermore National Laboratory. Support from the Office of Fusion Energy Sciences (FES) Basic and Applied Plasma Science Initiative is gratefully acknowledged. Additional support was provided from FES Education Program at LLNL and the Cal-Poly SLO Center for Excellence in Science and Mathematics Education STAR Program. NR 18 TC 6 Z9 6 U1 0 U2 4 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 1200 MONTREAL ROAD, BUILDING M-55, OTTAWA, ON K1A 0R6, CANADA SN 0008-4204 J9 CAN J PHYS JI Can. J. Phys. PD MAY PY 2011 VL 89 IS 5 BP 653 EP 656 DI 10.1139/P10-102 PG 4 WC Physics, Multidisciplinary SC Physics GA 775QH UT WOS:000291476700019 ER PT J AU Wang, JH Zhou, Z Botterud, A AF Wang, Jianhui Zhou, Zhi Botterud, Audun TI An evolutionary game approach to analyzing bidding strategies in electricity markets with elastic demand SO ENERGY LA English DT Article DE Evolutionary game; Game theory; Coevolutionary algorithm; Bidding strategies; Strategy selection; Agent based-modeling ID INCOMPLETE INFORMATION; COMPETITION; PRODUCERS; ALGORITHM AB In this paper we propose an evolutionary imperfect information game approach to analyzing bidding strategies in electricity markets with price-elastic demand. In previous research, opponent generation companies' (GENCOs') bidding strategies were assumed to be fixed or subject to a fixed probability distribution. In contrast, the adaptive and learning agents in the presented model can dynamically update their beliefs about opponents' bidding strategies during the simulation. GENCOs are represented as different. species in the coevolutionary algorithm to search the equilibrium. By modeling the evolutionary gaming behavior of GENCOs, the simulation can capture the dynamics of GENCOs' strategy change. This is important for analyzing transitory behavior of agents in the market in addition to the long-run equilibrium state. Simulations show that due to the adaptive learning, the bidding evolution is different from the one in the traditional game. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Wang, Jianhui; Zhou, Zhi; Botterud, Audun] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA. RP Wang, JH (reprint author), Argonne Natl Lab, Decis & Informat Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jianhui.wang@anl.gov RI Zhou, Zhi/D-2168-2009 NR 37 TC 21 Z9 24 U1 1 U2 17 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-5442 J9 ENERGY JI Energy PD MAY PY 2011 VL 36 IS 5 BP 3459 EP 3467 DI 10.1016/j.energy.2011.03.050 PG 9 WC Thermodynamics; Energy & Fuels SC Thermodynamics; Energy & Fuels GA 774UF UT WOS:000291411400121 ER PT J AU Aad, G Abbott, B Abdallah, J Abdelalim, AA Abdesselam, A Abdinov, O Abi, B Abolins, M Abramowicz, H Abreu, H Acerbia, E Acharya, BS Adams, DL Addy, TN Adelman, J Aderholz, M Adomeit, S Adragna, P Adye, T Aefsky, S Aguilar-Saavedrab, JA Aharrouche, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akdogan, T Akesson, TP Akimoto, G Akimov, AV Alam, MS Alam, MA Albrand, S Aleksa, M Aleksandrov, IN Aleppo, M Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Aliyev, M Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alviggi, MG Amako, K Amaral, P Amelung, C Ammosov, VV Amorim, A Amoros, G Amram, N Anastopoulos, C Andeen, T Anders, CF Anderson, KJ Andreazza, A Andrei, V Andrieux, ML Anduaga, XS Angerami, A Anghinolfi, F Anjos, N Annovi, A Antonaki, A Antonelli, M Antonelli, S Antos, J Anulli, F Aoun, S Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Archambault, JP Arfaoui, S Arguin, JF Arik, E Arik, M Armbruster, AJ Arnaez, O Arnault, C Artamonov, A Artoni, G Arutinov, D Asai, S Asfandiyarov, R Ask, S Asman, B Asquith, L Assamagan, K Astbury, A Astvatsatourov, A Atoian, G Aubert, B Auerbach, B Auge, E Augsten, K Aurousseau, M Austin, N Avramidou, R Axen, D Ay, C Azuelos, G Azuma, Y Baak, MA Baccaglioni, G Bacci, C Bach, AM Bachacou, H Bachas, K Bachy, G Backes, M Backhaus, M Badescu, E Bagnaia, P Bahinipati, S Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, MD Baker, S Pedrosa, FBD Banas, E Banerjee, P Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L 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Wildauer, A. Wildt, M. A. Wilhelm, I. Wilkens, H. G. Will, J. Z. Williams, E. Williams, H. H. Willis, W. Willocq, S. Wilson, J. A. Wilson, M. G. Wilson, A. Wingerter-Seez, I. Winkelmann, S. Winklmeier, F. Wittgen, M. Wolter, M. W. Wolters, H. Wooden, G. Wosiek, B. K. Wotschack, J. Woudstr, M. J. Wraight, K. Wright, C. Wrona, B. Wu, S. L. Wu, X. Wu, Y. Wulf, E. Wunstorf, R. Wynne, B. M. Xaplanteris, L. Xella, S. Xie, S. Xie, Y. Xu, C. Xu, D. Xu, G. Yabsley, B. Yamada, M. Yamamoto, A. Yamamoto, K. Yamamoto, S. Yamamura, T. Yamaoka, J. Yamazaki, T. Yamazaki, Y. Yan, Z. Yang, H. Yang, U. K. Yang, Y. Yang, Y. Yang, Z. Yanush, S. Yao, W. -M. Yao, Y. Yasu, Y. Ye, J. Ye, S. Yilmaz, M. Yoosoofmiya, R. Yorita, K. Yoshida, R. Young, C. Youssef, S. Yu, D. Yu, J. Yu, J. Yuan, L. Yurkewicz, A. Zaets, V. G. Zaidan, R. Zaitsev, A. M. Zajacova, Z. Zalite, Yo K. Zanello, L. Zarzhitsky, P. Zaytsev, A. Zeitnitz, C. Zeller, M. Zema, P. F. Zemla, A. Zendler, C. Zenin, A. V. Zenin, O. Zenis, T. Zenonos, Z. Zenz, S. Zerwas, D. della Porta, G. Zevi Zhan, Z. Zhang, D. Zhang, H. Zhang, J. Zhang, X. Zhang, Z. Zhao, L. Zhao, T. Zhao, Z. Zhemchugov, A. Zheng, S. Zhong, J. Zhou, B. Zhou, N. Zhou, Y. Zhu, C. G. Zhu, H. Zhu, Y. Zhuang, X. Zhuravlov, V. Zieminska, D. Zilka, B. Zimmermann, R. Zimmermann, S. Zimmermann, S. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zmouchko, V. V. Zobernig, G. Zoccoli, A. Zolnierowski, Y. Zsenei, A. zur Nedden, M. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Measurements of underlying-event properties using neutral and charged particles in pp collisions at root s=900 GeV and root s=7 TeV with the ATLAS detector at the LHC SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID CALORIMETER; DISTRIBUTIONS; JETS; HERA AB We present first measurements of charged and neutral particle-flow correlations in pp collisions using the ATLAS calorimeters. Data were collected in 2009 and 2010 at centre-of-mass energies of 900 GeV and 7 TeV. Events were selected using a minimum-bias trigger which required a charged particle in scintillation counters on either side of the interaction point. Particle flows, sensitive to the underlying event, are measured using clusters of energy in the ATLAS calorimeters, taking advantage of their fine granularity. No Monte Carlo generator used in this analysis can accurately describe the measurements. The results are independent of those based on charged particles measured by the ATLAS tracking systems and can be used to constrain the parameters of Monte Carlo generators. C1 [Aleksa, M.; Amaral, P.; Anghinolfi, F.; Arfaoui, S.; Asai, S.; Baak, M. A.; Bachas, K.; Bachy, G.; Pedrosa, F. Baltasar Dos Santos; Banfi, D.; Battistin, M.; Bellina, F.; Beltramello, O.; Berge, D.; Bertinelli, F.; Bianchi, R. M.; Blanchot, G.; Bogaerts, J. A.; Boyd, J.; Braem, A.; Bremer, J.; Burckhart, H.; Butin, F.; Campana, S.; Garrido, M. D. M. 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K.; Ciftci, R.; Persembe, S.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Yildiz, H. Duran] Dumlupinar Univ, Dept Phys, Kutahya, Turkey. [Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Cakir, I. Turk] Turkish Atom Energy Commiss, Ankara, Turkey. [Bella, L. Aperio; Aubert, B.; Aurousseau, M.; Berger, N.; Colas, J.; Di Ciaccio, L.; Doan, T. K. O.; El Kacimi, M.; Elles, S.; Ghez, P.; Gouanere, M.; Goy, C.; Guillemin, T.; Helary, L.; Hiller, K. H.; Hryn'ova, T.; Iengo, P.; Ionescu, G.; Jeremie, A.; Jezequel, S.; Kataoka, M.; Labbe, J.; Lafaye, R.; Massol, N.; Perrodo, P.; Przysiezniak, H.; Sauvage, G.; Todorov, T.; Tsionou, D.; Wingerter-Seez, I.; Zitoun, R.; Zolnierowski, Y.] CNRS, IN2P3, LAPP, Annecy Le Vieux, France. [Bella, L. Aperio; Aubert, B.; Aurousseau, M.; Berger, N.; Colas, J.; Di Ciaccio, L.; Doan, T. K. 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W.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Brandt, A.; De, K.; Farbin, A.; Kim, H.; Nilsson, P.; Ozturk, N.; Pravahan, R.; Sarkisyan-Grinbaum, E.; Sosebee, M.; Spurlock, B.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Antonaki, A.; Fassouliotis, D.; Giakoumopoulou, V.; Giokaris, N.; Ioannou, P.; Kourkoumelis, C.; Manousakis-Katsikakis, A.; Tzanakos, G.; Vellidis, C.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Avramidou, R.; Dris, M.; Filippas, A.; Fokitis, M.; Gazis, E. N.; Iakovidis, G.; Katsoufis, E.; Leontsinis, S.; Maltezos, S.; Mountricha, E.; Panagiotopoulou, E.; Papadopoulou, Th D.; Savva, P.; Tsipolitis, G.; Vlachos, S.; Xaplanteris, L.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Abdinov, O.; Aliyev, M.; Khalil-zada, F.; Rzaeva, S.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Abdallah, J.; Bosman, M.; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Demirkoz, B.; Dosil, M.; Espinal Curull, X.; Fiorini, L.; Grinstein, S.; Helsens, C.; Korolkov, I.; Martinez, M.; Meoni, E.; Mir, L. M.; Miralles Verge, L.; Nadal, J.; Osuna, C.; Pacheco Pages, A.; Padilla Aranda, C.; Perez Codina, E.; Riu, I.; Rossetti, V.; Segura, E.; Sushkov, S.; Vaque, F. Vives; Volpi, M.; Vorwerk, V.] Univ Autonoma Barcelona, E-08193 Barcelona, Spain. [Abdallah, J.; Bosman, M.; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Demirkoz, B.; Dosil, M.; Espinal Curull, X.; Fiorini, L.; Grinstein, S.; Helsens, C.; Korolkov, I.; Martinez, M.; Meoni, E.; Mir, L. M.; Miralles Verge, L.; Nadal, J.; Osuna, C.; Pacheco Pages, A.; Padilla Aranda, C.; Perez Codina, E.; Riu, I.; Rossetti, V.; Segura, E.; Sushkov, S.; Vaque, F. Vives; Volpi, M.; Vorwerk, V.] Inst Fis Altes Energies, Barcelona, Spain. [Abdallah, J.; Bosman, M.; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Demirkoz, B.; Dosil, M.; Espinal Curull, X.; Fiorini, L.; Grinstein, S.; Helsens, C.; Korolkov, I.; Martinez, M.; Meoni, E.; Mir, L. M.; Miralles Verge, L.; Nadal, J.; Osuna, C.; Pacheco Pages, A.; Padilla Aranda, C.; Perez Codina, E.; Riu, I.; Rossetti, V.; Segura, E.; Sushkov, S.; Vaque, F. Vives; Volpi, M.; Vorwerk, V.] ICREA, Barcelona, Spain. [Borjanovic, I.; Krstic, J.; Popovic, D. S.; Reljic, D.; Sijacki, Dj; Simic, Lj; Vranjes, N.; Milosavljevic, M. Vranjes] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Bozovic-Jelisavcic, I.; Mamuzic, J.; Mudrinic, M.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Buanes, T.; Burgess, T.; Eigen, G.; Johansen, L. G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Mohn, B.; Oye, O. K.; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Stugu, B.; Tonoyan, A.; Ugland, M.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Arguin, J-F.; Bach, A. M.; Galtieri, A. Barbaro; Barnett, R. M.; Beringer, J.; Biesiada, J.; Calafiura, P.; Ciocio, A.; Cooke, M.; Dube, S.; Einsweiler, K.; Ely, R.; Gaponenko, A.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Heinemann, B.; Hinchliffe, I.; Hsu, S. -C.; Hurwitz, M.; Joseph, J.; Korn, A.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Lys, J.; Madaras, R. J.; Quarrie, D. R.; Ruwiedel, C.; Scherzer, M. I.; Shapiro, M.; Siegrist, J.; Skinnari, L. A.; Stavropoulos, G.; Tatarkhanov, M.; Tompkins, L.; Vahsen, S.; Varouchas, D.; Virzi, J.; Yao, W. -M.; Yao, Y.; Zenz, S.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Phys, Berkeley, CA 94720 USA. [Aliev, M.; Brandt, G.; Giorgi, F. M.; Grancagnolo, S.; Herrberg, R.; Kind, O.; Kolanoski, H.; Kwee, R.; Lacker, H.; Leyton, M.; Lohse, T.; Mandrysch, R.; Nikiforov, A.; Garcia, Y. Rodriguez; Schulz, H.; Sidoti, A.; zur Nedden, M.] Humboldt Univ, Dept Phys, Berlin, Germany. [Battaglia, A.; Beck, H. P.; Borer, C.; Ereditato, A.; Martin, T. Fonseca; Gallo, V.; Haug, S.; Kabana, S.; Pretzl, K.; Topfel, C.; Venturi, N.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Battaglia, A.; Beck, H. P.; Borer, C.; Ereditato, A.; Martin, T. Fonseca; Gallo, V.; Haug, S.; Kabana, S.; Pretzl, K.; Topfel, C.; Venturi, N.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Bansil, H. S.; Bracinik, J.; Bright-Thomas, P. G.; Charlton, D. G.; Collins, N. J.; Curtis, C. J.; Dowell, J. D.; Garvey, J.; Hadley, D. R.; Harrison, K.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Lilley, J. N.; Mahout, G.; Martin, T. A.; Mclaughlan, T.; Newman, P. R.; O'Neale, S. W.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Typaldos, D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Akdogan, T.; Arik, E.; Arik, M.; Dogan, O. B.; Istin, S.; Ozcan, V. E.; Rador, T.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Div Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.; Diblen, F.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. Istanbul Tech Univ, Dept Phys, TR-80626 Istanbul, Turkey. [Antonelli, S.; Bellagamba, L.; Bertin, A.; Bindi, M.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Ciocca, C.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Giacobbe, B.; Giusti, P.; Jha, M. K.; Massa, I.; Mengarelli, A.; Monzani, S.; Negri, A.; Piccinini, M.; Polini, A.; Rinaldi, L.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Spighi, R.; Valentinetti, S.; Villa, M.; Vitale, A.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Antonelli, S.; Bertin, A.; Bindi, M.; Caforio, D.; Ciocca, C.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Massa, I.; Mengarelli, A.; Monzani, S.; Negri, A.; Piccinini, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Valentinetti, S.; Villa, M.; Vitale, A.; Zoccoli, A.] Univ Bologna, Dipartimento Fis, Bologna, Italy. [Alhroob, M.; Anders, C. F.; Arutinov, D.; Backhaus, M.; Barbero, M.; Bartsch, D.; Brock, I.; Cammin, J.; Cristinziani, M.; Desch, K.; Dingfelder, J.; Fischer, P.; Gaycken, G.; Geich-Gimbel, Ch; Gonella, L.; Havranek, M.; Hillert, S.; Huegging, F.; Ince, T.; Janus, M.; Khoriauli, G.; Koevesarki, P.; Kokott, T.; Kostyukhin, V. V.; Kroseberg, J.; Krueger, H.; Kruth, A.; Lapoire, C.; Lehmacher, M.; Loddenkoetter, T.; Mathes, M.; Mazur, M.; Meuser, S.; Moeser, N.; Mueller, K.; Nanava, G.; Nattermann, T.; Nuncio-Quiroz, A. -E.; Hanninger, G. Nunes; Peric, I.; Poghosyan, T.; Psoroulas, S.; Radics, B.; Rottlaender, I.; Runolfsson, O.; Schmieden, K.; Schmitz, M.; Schumacher, J. W.; Stillings, J. A.; Stockmanns, T.; Therhaag, J.; Treis, J.; Tsung, J. -W.; Uchida, K.; Uhlenbrock, M.; Vlasov, N.; Vogel, A.; von Toerne, E.; Wermes, N.; Wienemann, P.; Zendler, C.; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, D-5300 Bonn, Germany. [Ahlen, S. P.; Black, K. M.; Butler, J. M.; Harrington, R. D.; Hazen, E.; Lewandowska, M.; Love, J.; Marin, A.; Nation, N. R.; Posch, C.; Shank, J. T.; Whitaker, S. P.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Aefsky, S.; Amelung, C.; Bensinger, J. R.; Blocker, C.; Kirsch, L. E.; Pomeroy, D.; Skvorodnev, N.; Wellenstein, H.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Caloba, L. P.; Cerqueira, A. S.; Coura Torres, R.; Da Rocha Gesualdi Mello, A.; Da Silva, P. V. M.; do Vale, M. A. B.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Perantoni, M.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE, EE, IF, BR-21945 Rio De Janeiro, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Baker, M. D.; Begel, M.; Bernius, C.; Chen, H.; Chernyatin, V.; Salgado, P. E. De Castro Faria; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Greenwood, Z. D.; Hackenburg, R.; Klimentov, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Majewski, S.; Nevski, P.; Nikolopoulos, K.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Park, W.; Pleier, M. -A.; Poblaguev, A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Rahm, C.; Rajagopalan, S.; Redlinger, G.; Sawyer, L.; Snyder, S.; Sondericker, J.; Steinberg, P.; Stumer, I.; Takai, H.; Tamsett, M. C.; Tarrade, F.; Trivedi, A.; Undrus, A.; Wenaus, T.; White, S.; Ye, S.; Yu, D.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Caramarcu, C.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Micu, L.; Pantea, D.; Popeneciu, G. A.; Rotaru, M.; Stoicea, G.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. W Univ Timisoara, Timisoara, Romania. [Gonzalez Silva, M. L.; Otero y Garzon, G.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barber, T.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cowden, C.; French, S. T.; Frost, J. A.; Hill, J. C.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Parker, M. A.; Phillips, A. W.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Archambault, J. P.; Cojocaru, C. D.; Gillberg, D.; Heelan, L.; Khakzad, M.; Liu, C.; McCarthy, T. G.; Oakham, F. G.; Randrianarivony, K.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aad, G.; Ahles, F.; Beckingham, M.; Bernhard, R.; Bitenc, U.; Bruneliere, R.; Caron, S.; Carpentieri, C.; Christov, A.; Dahlhoff, A.; Dietrich, J.; Eckert, S.; Fehling-Kaschek, M.; Flechl, M.; Glatzer, J.; Hartert, J.; Heldmann, M.; Herten, G.; Horner, S.; Jakobs, K.; Ketterer, C.; Koenig, S.; Kollefrath, M.; Kononov, A. I.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Lumb, D.; Mahboubi, K.; Meinhardt, J.; Mohr, W.; Nilsen, H.; Parzefall, U.; Bueso, X. Portell; Rammensee, M.; Runge, K.; Rurikova, Z.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tobias, J.; Tsiskaridze, V.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Wiik, L. A. M.; Winkelmann, S.; Xie, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Freiburg, Germany. [Anderson, K. J.; Boveia, A.; Brubaker, E.; Canelli, F.; Choudalakis, G.; Costin, T.; Feng, E. J.; Fiascaris, M.; Gardner, R. W.; Gupta, A.; Plante, I. Jen-La; Kapliy, A.; Melachrinos, C.; Onyisi, P. U. E.; Oreglia, M. J.; Pilcher, J. E.; Shochet, M. J.; Tuggle, J. M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Diaz, M. A.; Panes, B.; Quinonez, F.; Romero Maltrana, D.; Urrejola, P.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Oyarzun, A.; Pezoa, R.; Prokoshin, F.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Cheng, S.; Han, H.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Tong, G.; Xie, Y.; Xu, G.; Yang, Y.; Yuan, L.; Zheng, S.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Jiang, Y.; Jin, G.; Li, S.; Liu, M.; Liu, Y.; Wu, Y.; Xu, C.; Zhang, D.; Zhao, Z.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Chen, T.; Ping, J.; Yu, J.; Zhong, J.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; He, M.; Liu, D.; Meng, Z.; Miao, J.; Wang, J.; Zhan, Z.; Zhang, X.; Zhu, C. G.] Shandong Univ, High Energy Phys Grp, Jinan, Shandong, Peoples R China. [Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Febbraro, R.; Ghodbane, N.; Gris, P. L. Y.; Guicheney, C.; Pallin, D.; Podlyski, F.; Santoni, C.; Says, L. P.; Vazeille, F.; Viret, S.] CNRS, IN2P3, Aubiere, France. [Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Febbraro, R.; Ghodbane, N.; Gris, P. L. Y.; Guicheney, C.; Pallin, D.; Podlyski, F.; Santoni, C.; Says, L. P.; Vazeille, F.; Viret, S.] Univ Clermont Ferrand, Aubiere, France. [Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Febbraro, R.; Ghodbane, N.; Gris, P. L. Y.; Guicheney, C.; Pallin, D.; Podlyski, F.; Santoni, C.; Says, L. P.; Vazeille, F.; Viret, S.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Aubiere, France. [Andeen, T.; Angerami, A.; Brooijmans, G.; Copic, K.; Dodd, J.; Grau, N.; Gray, H. M.; Guo, J.; Hughes, E. W.; Leltchouk, M.; Marshall, Z.; Parsons, J. A.; Penson, A.; Perez, K.; Reale, V. Perez; Spano, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Boelaert, N.; Dam, M.; Driouichi, C.; Facius, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Jez, P.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Lundquist, J.; Mackeprang, R.; Mehlhase, S.; Petersen, T. C.; Rensch, B.; Simonyan, M.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Mastroberardino, A.; Morello, G.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Mastroberardino, A.; Morello, G.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Ciba, K.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Idzik, M.; Jelen, K.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Rulikowska-Zarebska, E.; Toczek, B.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa; Malecki, P.; Olszewski, A.; Olszowska, J.; Richter-Was, E.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Daya, R. K.; Yagci, K. Dindar; Firan, A.; Goldin, D.; Hadavand, H. K.; Hoffman, J.; Ilchenko, Y.; Ishmukhametov, R.; Joffe, D.; Kama, S.; Kasmi, A.; Kehoe, R.; Liang, Z.; Lu, L.; Renkel, P.; Rios, R. R.; Stroynowski, R.; Ye, J.; Zarzhitsky, P.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Galyaev, E.; Izen, J. M.; Lou, X.; Reeves, K.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bechtle, P.; Kuutmann, E. Bergeaas; Boehler, M.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Gosdzik, B.; Gregor, I. M.; Hiller, K. H.; Hristova, I.; Husemann, U.; Belenguer, M. Jimenez; Johnert, S.; Karnevskiy, M.; Katzy, J.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Mijovic, L.; Moenig, K.; Naumann, T.; Nozicka, M.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Placakyte, R.; Qin, Z.; Rubinskiy, I.; Stelzer, H. J.; Terwort, M.; Vankov, P.; Viti, M.; Wildt, M. A.; Zhu, H.] DESY, D-2000 Hamburg, Germany. [Bechtle, P.; Kuutmann, E. Bergeaas; Boehler, M.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Gosdzik, B.; Gregor, I. M.; Hiller, K. H.; Hristova, I.; Husemann, U.; Belenguer, M. Jimenez; Johnert, S.; Karnevskiy, M.; Katzy, J.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Mijovic, L.; Moenig, K.; Naumann, T.; Nozicka, M.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Placakyte, R.; Qin, Z.; Rubinskiy, I.; Stelzer, H. J.; Terwort, M.; Vankov, P.; Viti, M.; Wildt, M. A.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Dobos, D.; Goessling, C.; Hirsch, F.; Klaiber-Lodewigs, J.; Klingenberg, R.; Krasel, O.; Mass, M.; Muenstermann, D.; Rajek, S.; Reisinger, I.; Walbersloh, J.; Weber, J.; Wunstorf, R.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Goepfert, T.; Kar, D.; Kobel, M.; Leonhardt, K.; Ludwig, A.; Mader, W. F.; Prudent, X.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Ebenstein, W. L.; Fowler, A. J.; Ko, B. R.; Oh, S. H.; Wang, C.; Yamaoka, J.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; O'Brien, B. J.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Asai, S.; Griesmayer, E.] Fachhochsch Wiener Neustadt, Wiener Neustadt, Austria. [Annovi, A.; Antonelli, M.; Bilokon, H.; Cerutti, F.; Curatolo, M.; Esposito, B.; Ferrer, M. L.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Wen, M.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Bell, P. J.; Bell, W. H.; Berglund, E.; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Efthymiopoulos, I.; Ferrere, D.; Gadomski, S.; Navarro, J. E. Garcia; Gaumer, O.; Gonzalez-Sevilla, S.; Goulette, M. P.; Hamilton, A.; Leger, A.; Lister, A.; Macina, D.; Latour, B. Martin Dit; Mikulec, B.; Moneta, L.; Herrera, C. Mora; Morone, M-C.; Nektarijevic, S.; Orellana, F.; Pasztor, G.; Pohl, M.; Robichaud-Veronneau, A.; Rosselet, L.; Urquijo, P.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Coccaro, A.; Cornelissen, T.; Cuneo, S.; Dameri, M.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Morettini, P.; Olcese, M.; Osculati, B.; Parodi, F.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Caso, C.; Coccaro, A.; Cornelissen, T.; Cuneo, S.; Dameri, M.; Parodi, A. Ferretto; Gagliardi, G.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Chikovani, L.; Djobava, T.; Khubua, J.; Magradze, E.; Mchedlidze, G.; Mosidze, M.; Tskhadadze, E. G.] Georgian Acad Sci, Inst Phys, GE-380077 Tbilisi, Rep of Georgia. [Chikovani, L.; Djobava, T.; Khubua, J.; Magradze, E.; Mchedlidze, G.; Mosidze, M.; Tskhadadze, E. G.] HEP Inst, GE-380060 Tbilisi, Rep of Georgia. [Chikovani, L.; Djobava, T.; Khubua, J.; Magradze, E.; Mchedlidze, G.; Mosidze, M.; Tskhadadze, E. G.] Tbilisi State Univ, GE-380086 Tbilisi, Rep of Georgia. [Astvatsatourov, A.; Dueren, M.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-6300 Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Gemmell, A.; Kenyon, M.; McGlone, H.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Pickford, A.; Robson, A.; Saxon, D. H.; Shaw, C.; Smith, K. M.; St Denis, R. D.; Steele, G.; Stewart, G. A.; Thompson, A. S.; Wraight, K.; Wright, C.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Asai, S.; Ay, C.; Blumenschein, U.; Brandt, O.; Erdmann, J.; Evangelakou, D.; Grosse-Knetter, J.; Guindon, S.; Haller, J.; Henrichs, A.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Mann, A.; Meyer, J.; Morel, J.; Quadt, A.; Roe, A.; Shabalina, E.; Uhrmacher, M.; Weber, P.; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Andrieux, M-L; Clement, B.; Collot, J.; Crepe-Renaudin, S.; de Saintignon, P.; Delsart, P. A.; Donini, J.; Dzahini, D.; Hostachy, J. -Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Martin, Ph; Polci, F.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Andrieux, M-L; Clement, B.; Collot, J.; Crepe-Renaudin, S.; de Saintignon, P.; Delsart, P. 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A.; Foehlisch, F.; Geweniger, C.; Hanke, P.; Henke, M.; Khomicha, A.; Kluge, E. -E.; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Radescu, V.; Schaetzel, S.; Schoening, A.] Heidelberg Univ, Inst Phys, D-6900 Heidelberg, Germany. [Kugel, A.; Maenner, R.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Heidelberg, Germany. [Ohsugi, T.] Hiroshima Univ, Fac Sci, Hiroshima 730, Japan. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Jain, V.; Luehring, F.; Marino, C. P.; Ogren, H.; Penwell, J.; Price, D.; Rust, D. R.; Whittington, D.; Yang, Y.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Epp, B.; Jussel, P.; Kneringer, E.; Kuhn, D.; Rudolph, G.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Behera, P. K.; Limper, M.; Mallik, U.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Cochran, J.; Dudziak, F.; Lebedev, A.; Mete, A. S.; Meyer, W. T.; Nelson, A.; Prell, S.; Rosenberg, E. I.; Ruiz-Martinez, A.; Triplett, N.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Barashkou, A.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chepurnov, V. F.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Gusakov, Y.; Kalinovskaya, L. V.; Kazarinov, M. Y.; Kekelidze, G. D.; Kharchenko, D.; Khovanskiy, N.; Khramov, E.; Kolesnikov, V.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Lazarev, A. B.; Malyukov, S.; Manjavidze, I. D.; Minashvili, I. A.; Mineev, M.; Nikolaev, K.; Olchevski, A. G.; Peshekhonov, V. D.; Romanov, V. M.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. 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F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Brodbeck, T. J.; Catmore, J. R.; Cheatham, S.; Chilingarov, A.; Davidson, R.; De Mora, L.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Ratoff, P. N.; Sloan, T. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Brambilla, E.; Cataldi, G.; Cazzato, A.; Chiodini, G.; Coluccia, R.; Crupi, R.; Gorini, E.; Grancagnolo, F.; Guida, A.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Bianco, M.; Brambilla, E.; Cazzato, A.; Coluccia, R.; Crupi, R.; Gorini, E.; Guida, A.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Fis, Lecce, Italy. [Allport, P. P.; Austin, N.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Houlden, M. A.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Maxfield, S. J.; Mehta, A.; Migas, S.; Prichard, P. M.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wiglesworth, C.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Landon, M. P. J.; Lloyd, S. L.; Morin, J.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Stevenson, K.; Castanheira, M. Teixeira Dias; Traynor, D.] Queen Mary Univ London, Dept Phys, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Boorman, G.; Cooper-Smith, N. J.; Cowan, G.; Edwards, C. A.; George, S.; Goncalo, R.; Hayden, D.; Kilvington, G.; Misiejuk, A.; Rose, M.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Boeser, S.; Butterworth, J. M.; Byatt, T.; Campanelli, M.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dean, S.; Drohan, J. G.; Jansen, E.; Jones, T. W.; Konstantinidis, N.; Monk, J.; Nash, M.; Nurse, E.; Prabhu, R.; Richards, A.; Robinson, J. E. M.; Sherwood, P.; Simmons, B.; Taylor, C.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Beau, T.; Bordoni, S.; Calderini, G.; Camard, A.; Cavalleri, P.; Chareyre, E.; De Cecco, S.; Derue, F.; Imbault, D.; Krasny, M. 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G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Siragusa, G.; Tapprogge, S.; Anh, T. Vu] Johannes Gutenberg Univ Mainz, Inst Phys, D-6500 Mainz, Germany. [Almond, J.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Foster, J. M.; Howarth, J.; Hughes-Jones, R. E.; Ibbotson, M.; Jones, G.; Keates, J. R.; Kelly, M.; Kolya, S. D.; Lane, J. L.; Loebinger, F. K.; Marshall, R.; Martyniuk, A. C.; Marx, M.; Masik, J.; Miyagawa, P. S.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Plano, W. G.; Schwanenberger, C.; Snow, S. W.; Tevlin, C. M.; Watts, S.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aoun, S.; Arfaoui, S.; Bee, C.; Benchouk, C.; Bernardet, K.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Delpierre, P.; Djama, F.; Etienne, F.; Feligioni, L.; Henry-Couannier, F.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Kuna, M.; Le Guirriec, E.; Leveque, J.; Li, B.; Monnier, E.; Odier, J.; Petit, E.; Pralavorio, P.; Qian, Z.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aoun, S.; Arfaoui, S.; Bee, C.; Benchouk, C.; Bernardet, K.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Delpierre, P.; Djama, F.; Etienne, F.; Feligioni, L.; Henry-Couannier, F.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Kuna, M.; Le Guirriec, E.; Leveque, J.; Li, B.; Monnier, E.; Odier, J.; Petit, E.; Pralavorio, P.; Qian, Z.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Thompson, E. N.; van Eldik, N.; Willocq, S.; Woudstr, M. J.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Chapleau, B.; Dobbs, M.; Dufour, M. -A.; Guler, H.; Klemetti, M.; Potter, C. T.; Robertson, S. H.; Rios, C. Santamarina; Schram, M.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Davey, W.; Davidson, N.; Felzmann, C. U.; Kazi, S. I.; Limosani, A.; Moorhead, G. F.; Phan, A.; Sevior, M. E.; Shao, Q. T.; Taylor, G. N.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Eppig, A.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, H.; Liu, J. B.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Purdham, J.; Qian, J.; Scheirich, D.; Strandberg, J.; Thun, R. P.; Walch, S.; Wilson, A.; Yang, H.; Zhou, B.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Comune, G.; Di Mattia, A.; Fedorko, W.; Hauser, R.; Heim, S.; Holzbauer, J. L.; Huston, J.; Koll, J.; Kraus, J.; Linnemann, J. T.; Mangeard, P. S.; Martin, B.; Miller, R. J.; Pope, B. G.; Ryan, P.; Schwienhorst, R.; Tollefson, K.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Acerbia, E.; Aleppo, M.; Alessandria, F.; Alimonti, G.; Andreazza, A.; Baccaglioni, G.; Battistoni, G.; Bellomo, G.; Besana, M. I.; Broggi, F.; Caccia, M.; Carminati, L.; Cavalli, D.; Costa, G.; Dell'Asta, L.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Lazzaro, A.; Lombardo, V. P.; Mandelli, L.; Mazzanti, M.; Meroni, C.; Montesano, S.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Rossi, L.; Sorbi, M.; Tartarelli, G. F.; Troncon, C.; Vegni, G.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Acerbia, E.; Aleppo, M.; Andreazza, A.; Bellomo, G.; Besana, M. I.; Caccia, M.; Carminati, L.; Dell'Asta, L.; Fanti, M.; Favareto, A.; Lazzaro, A.; Montesano, S.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Rossi, L.; Sorbi, M.; Vegni, G.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Gilewsky, V.; Kuzhir, P.; Rumiantsev, V.; Starovoitov, P.; Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Azuelos, G.; Banerjee, P.; Bouchami, J.; Davies, M.; Ferland, J.; Guler, H.; Gutierrez, A.; Lebel, C.; Leroy, C.; Goia, J. A. Macana; Martin, J. P.; Mehdiyev, R.; Scallon, O.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Belotskiy, K.; Bondarenko, V. G.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Morozov, S. 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[Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Cevenini, F.; Chiefari, G.; della Volpe, D.; Giordano, R.; Merola, L.; Musto, E.; Patricelli, S.; Rossi, E.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Metcalfe, J.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Aloisio, A.; Consonni, M.; De Groot, N.; Filthaut, F.; Klok, P. F.; Konig, A. C.; Koetsveld, F.; Magrath, C. A.; Ordonez, G.; Raas, M.; Timmermans, C. J. W. P.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Bentvelsen, S.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Buis, E. J.; Colijn, A. P.; Dankers, R.; Daum, C.; de Jong, P.; De Nooij, L.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. 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P.; Peters, O.; Reichold, A.; Rijpstra, M.; Ruckstuhl, N.; Salamanna, G.; Sandstroem, R.; Snuverink, J.; Ta, D.; Tsiakiris, M.; Turlay, E.; van der Graaf, H.; van der Kraaij, E.; Van Der Leeuw, R.; van der Poel, E.; Van Eijk, B.; van Kesteren, Z.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; de Lima, J. G. Rocha; Suhr, C.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Beloborodova, O.; Bobrovnikov, V. B.; Bogdanchikov, A.; Kazanin, V. A.; Kolachev, G. M.; Korol, A.; Malyshev, V.; Maslennikov, A. L.; Maximov, D. A.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.; Zaytsev, A.] BINP, Novosibirsk, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; Djilkibaev, R.; van Huysduynen, L. Hooft; Konoplich, R.; Krasznahorkay, A.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.; Shibata, A.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA. [Fernando, W.; Fisher, M. J.; Gan, K. K.; Kagan, H.; Kass, R. D.; Moss, J.; Rahimi, A. M.; Strang, M.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Huang, G. S.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Kocnar, A.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Ptacek, E.; Reinsch, A.; Robinson, M.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abreu, H.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Blanchard, J. -B.; Bourdarios, C.; Breton, D.; Collard, C.; De La Taille, C.; De Regie, J. B. De Vivie; Diglio, S.; Duflot, L.; Escalier, M.; Falou, A. C.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Heller, M.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lounis, A.; Makovec, N.; Matricon, P.; Nakahama, Y.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Veillet, J. J.; Vukotic, I.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Abreu, H.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Blanchard, J. -B.; Bourdarios, C.; Breton, D.; Collard, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Falou, A. 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[Alison, J.; Degenhardt, J.; Donega, M.; Dressnandt, N.; Fratina, S.; Hance, M.; Hines, E.; Jackson, B.; Kroll, J.; Kunkle, J.; LeGeyt, B. C.; Lipeles, E.; Martin, F. F.; Olivito, D.; Ospanov, R.; Reece, R.; Stahlman, J.; Thomson, E.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Nesterov, S. Y.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Zalite, Yo K.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dottia, A.; Francavilla, P.; Giangiobbe, V.; Lupi, A.; Mazzoni, E.; Roda, C.; Sarri, F.; Zenonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dottia, A.; Francavilla, P.; Giangiobbe, V.; Lupi, A.; Mazzoni, E.; Roda, C.; Sarri, F.; Zenonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Boudreau, J.; Boulahouache, C.; Cleland, W.; Kittelmann, T.; Mueller, J.; Paolone, V.; Prieur, D.; Savinov, V.; Tsulaia, V.; Wendler, S.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedrab, J. A.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Do Valle Wemans, A.; Fernandes, B.; Fiolhais, M. C. N.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Magalhaes Martins, P. J.; Maio, A.; Maneira, J.; Morais, A.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Rossi, L. P.; Santos, H.; Saraiva, J. G.; Silva, J.; Soares, M.; Veloso, F.; Wolters, H.; Zhong, J.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedrab, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedrab, J. A.] Univ Granada, CAFPE, Granada, Spain. [Chudoba, J.; Gallus, P.; Gunther, J.; Hruska, I.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Kvasnicka, O.; Lipinsky, L.; Lokajicek, M.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Panuskova, M.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Tic, T.; Valenta, J.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Davidek, T.; Dolejsi, J.; Dolezal, Z.; Drasal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Tasevsky, M.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Asai, S.; Augsten, K.; Holy, T.; Horazdovsky, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Ammosov, V. V.; Asai, S.; Borisov, A.; Bozhko, N. I.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Gapienko, V. A.; Golovnia, S. N.; Gorokhov, S. A.; Goryachev, V. N.; Gushchin, V. N.; Ivashin, A. V.; Kabachenko, V. V.; Karyukhin, A. N.; Kholodenko, A. G.; Kiver, A. M.; Kopikov, S. V.; Koreshev, V.; Korotkov, V. A.; Kozhin, A. S.; Lapin, V. V.; Larionov, A. V.; Levitski, M. S.; Minaenko, A. A.; Mitrofanov, G. Y.; Moisseev, A. M.; Myagkov, A. G.; Nikolaenko, V.; Pleskach, A. V.; Ryadovikov, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Sviridov, Yu M.; Vorobiev, A. P.; Vovenko, A. S.; Zaets, V. G.; Zaitsev, A. M.; Zenin, A. V.; Zenin, O.; Zmouchko, V. V.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Botterill, D.; Burke, S.; Clifft, R. W.; Dallison, S. J.; Dewhurst, A.; Emeliyanov, D.; Fisher, S. M.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Greenfield, D.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Strube, J.; Tyndel, M.; Weber, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.; Ju, X.; Ming, Y.; Ortega, E. O.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagnaia, P.; Biglietti, M.; Bini, C.; Borroni, S.; Caloi, R.; Cavallari, A.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; Dionisi, C.; Falciano, S.; Gentile, S.; Giagu, S.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Maiani, C.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Tehrani, F. Safai; Camillocci, E. Solfaroli; Spila, F.; Valente, P.; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma 1, Rome, Italy. [Artoni, G.; Bagnaia, P.; Biglietti, M.; Bini, C.; Borroni, S.; Caloi, R.; Cavallari, A.; Ciapetti, G.; D'Orazio, A.; Dionisi, C.; Gentile, S.; Giagu, S.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Maiani, C.; Tehrani, F. Safai; Camillocci, E. Solfaroli; Spila, F.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Nardo, R.; Di Simone, A.; Liberti, B.; Marchese, F.; Paoloni, A.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Nardo, R.; Di Simone, A.; Marchese, F.; Paoloni, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncellia, A.; Branchini, P.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Ruggieri, F.; Spiriti, E.; Stanescu, C.; Tonazzo, A.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Ruggieri, F.; Tonazzo, A.] Univ Roma Tre, Dipartimento Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Goujdami, D.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [Derkaoui, J. E.; Ouchrif, M.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Ghazlane, H.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Boonekamp, M.; Chevalier, L.; Chevallier, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Lancon, E.; Laporte, J. F.; Le Menedeu, E.; Legendre, M.; Lenzi, B.; Mansoulie, B.; Meyer, J-P.; Morange, N.; Ouraou, A.; Pomarede, D. M.; Resende, B.; Royon, C. R.; Schwindling, J.; Simard, O.; Virchaux, M.] CEA, CEA Saclay, Inst Rech Lois Fondament Univers, DSM,IRFU, Gif Sur Yvette, France. [Bangert, A.; Chouridou, S.; Damiani, D. S.; Dubbs, T.; Fowler, K.; Grillo, A. A.; Hare, G. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Forbush, D. A.; Goussiou, A. G.; Griffiths, J.; Harris, O. M.; Kuykendall, W.; Lubatti, H. J.; Mockett, P.; Policicchio, A.; Rosati, S.; Rothberg, J.; Ventura, D.; Verducci, M.; Wang, J. C.; Watts, G.; Zhao, T.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Booth, C. N.; Booth, P.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Duxfield, R.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mayne, A.; Mcfayden, J. A.; Nicolas, L.; Owen, S.; Paganis, E.; Sutton, M. R.; Tovey, D. R.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Ohshita, H.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Sipica, V.; Stahl, T.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-5900 Siegen, Germany. [Dawe, E.; Godfrey, J.; Komaragiri, J. R.; O'Neil, D. C.; Petteni, M.; Schouten, D.; Stelzer, B.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Coan, J. G.; Gao, Y. S.; Grenier, P.; Haas, A.; Hansson, P.; Horn, C.; Jackson, P.; Kim, P. C.; Kocian, M.; Koi, T.; Lowe, A. J.; Miller, D. 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T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Meng, Z.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhong, J.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Harpaz, S. Behar; Ben Ami, S.; Bressler, S.; Hershenhorn, A. D.; Kajomovitz, E.; Landsman, H.; Lifshitz, R.; Rozen, Y.; Tarem, S.; Tennenbaum-Katan, Y. D.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Brodet, E.; Etzion, E.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hod, N.; Kreisel, A.; Mahalalel, Y.; Munwes, Y.; Oren, Y.; Reinherz-Aronis, E.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.; Urkovsky, E.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Azuma, Y.; Dohmae, T.; Imori, M.; Isobe, T.; Kanaya, N.; Kaneda, M.; Kataoka, Y.; Kawamoto, T.; Kessoku, K.; Kobayashi, T.; Kubota, T.; Mashimo, T.; Masubuchi, T.; Matsumoto, H.; Matsunaga, H.; Nakamura, K.; Ninomiya, Y.; Nomoto, H.; Oda, S.; Okuyama, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamamura, T.; Yamazaki, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Azuma, Y.; Dohmae, T.; Imori, M.; Isobe, T.; Kanaya, N.; Kaneda, M.; Kataoka, Y.; Kawamoto, T.; Kessoku, K.; Kobayashi, T.; Kubota, T.; Mashimo, T.; Masubuchi, T.; Matsumoto, H.; Matsunaga, H.; Nakamura, K.; Ninomiya, Y.; Nomoto, H.; Oda, S.; Okuyama, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamamura, T.; Yamazaki, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Jinnouchi, O.; Kanno, T.; Kuze, M.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [Asai, S.; Bailey, D. C.; Bain, T.; Beare, B.; Brelier, B.; Cheung, S. L.; Deviveiros, P. O.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Jankowski, E.; Krieger, P.; Le Maner, C.; Martens, F. K.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Sandhu, P.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.] Univ Toronto, Dept Phys, Toronto, ON M5S 1A1, Canada. [Azuelos, G.; Canepa, A.; Caron, B.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Losty, M. J.; Nugent, I. M.; Oakham, F. G.; Oram, C. J.; Savard, P.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Kim, S. H.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Inst Pure & Appl Sci, Ibaraki, Japan. [Hamilton, S.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.] Tufts Univ, Ctr Sci & Technol, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Rodriguez, D.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Benedict, B. H.; Bold, T.; Ciobotaru, M. D.; Deng, J.; Dobson, M.; Eschrich, I. Gough; Grabowska-Bold, I.; Hawkins, D.; Lankford, A. J.; Okawa, H.; Porter, R.; Scannicchio, D. A.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Wheeler-Ellis, S. J.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Cauz, D.; Cobal, M.; De Lotto, B.; De Sanctis, U.; Del Papa, C.; Pinamonti, M.; Shaw, K.; Suruliz, K.] Ist Nazl Fis Nucl, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Suruliz, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. 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A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, Inst Fis Corpuscular, Valencia, Spain. [Amoros, G.; Cabrera Urban, S.; Gimenez, V. Castillo; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Amoros, G.; Cabrera Urban, S.; Gimenez, V. Castillo; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Amoros, G.; Cabrera Urban, S.; Gimenez, V. Castillo; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, IMB, CNM, Valencia, Spain. [Amoros, G.; Cabrera Urban, S.; Gimenez, V. Castillo; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] CSIC, Valencia, Spain. [Axen, D.; Gay, C.; Loh, C. W.; Mills, W. J.; Muir, A.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Asai, S.; Astbury, A.; Banerjee, Sw; Bansal, V.; Berghaus, F.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; McPherson, R. A.; Plamondon, M.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Kimura, N.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Duchovni, E.; Frank, T.; Gabizon, O.; Gross, E.; Klier, A.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Asfandiyarov, R.; Montoya, G. D. Carrillo; Hernandez, A. M. Castaneda; Castaneda-Miranda, E.; Chen, X.; Dos Anjos, A.; Fang, Y.; Fasching, D.; Castillo, L. R. Flores; Gonzalez, S.; Gutzwiller, O.; Ji, H.; Kashif, L.; Cheong, A. Leung Fook; Li, H.; Ma, L. L.; Garcia, B. R. Mellado; Pan, Y. B.; Pataraia, S.; Morales, M. I. Pedraza; Peng, H.; Poveda, J.; Quayle, W. B.; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Zhu, Y.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Meyer, J.; Redelbach, A.; Stroehmer, R.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, Wurzburg, Germany. [Barisonzi, M.; Becks, K. H.; Boek, J.; Braun, H. M.; Dopke, J.; Drees, J.; Fleischmann, S.; Flick, T.; Gerlach, P.; Glitza, K. W.; Gorfine, G.; Grah, C.; Hamacher, K.; Harenberg, T.; Henss, T.; Hirschbuehl, D.; Imhaeuser, M.; Kalinin, S.; Kersten, S.; Kootz, A.; Kuhl, T.; Lenz, T.; Lenzen, G.; Maettig, P.; Mechtel, M.; Sandhoff, M.; Sandvoss, S.; Sartisohn, G.; Schultes, J.; Siebel, A.; Sturm, P.; Thadome, J.; Voss, T. T.; Wagner, W.; Wahlen, H.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Atoian, G.; Auerbach, B.; Baker, O. K.; Almenar, C. Cuenca; Demers, S.; Garberson, F.; Golling, T.; Guest, D.; Hsu, P. J.; Kaplan, B.; Lee, L.; Lockwitz, S.; Loginov, A.; Martin, A. J.; Schmidt, M. 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RI Smirnov, Sergei/F-1014-2011; Gladilin, Leonid/B-5226-2011; Kramarenko, Victor/E-1781-2012; Alexa, Calin/F-6345-2010; Moorhead, Gareth/B-6634-2009; Petrucci, Fabrizio/G-8348-2012; Wemans, Andre/A-6738-2012; Fabbri, Laura/H-3442-2012; Kurashige, Hisaya/H-4916-2012; Kuzhir, Polina/H-8653-2012; Delmastro, Marco/I-5599-2012; Weigell, Philipp/I-9356-2012; Veneziano, Stefano/J-1610-2012; collins-tooth, christopher/A-9201-2012; Perrino, Roberto/B-4633-2010; De Cecco, Sandro/B-1016-2012; branchini, paolo/A-4857-2011; Wolter, Marcin/A-7412-2012; McKee, Shawn/B-6435-2012; Rotaru, Marina/A-3097-2011; Buttar, Craig/D-3706-2011; Takai, Helio/C-3301-2012; St.Denis, Richard/C-8997-2012; Britton, David/F-2602-2010; Li, Xuefei/C-3861-2012; Smirnova, Lidia/D-8089-2012; valente, paolo/A-6640-2010; Fazio, Salvatore /G-5156-2010; Bauer, Florian/G-8816-2011; Gutierrez, Phillip/C-1161-2011; Ferrando, James/A-9192-2012; Doyle, Anthony/C-5889-2009; Jakubek, Jan/E-6530-2011; Marti-Garcia, Salvador/F-3085-2011; 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Morozov, Sergey/C-1396-2014; Villa, Mauro/C-9883-2009; Nemecek, Stanislav/G-5931-2014; Staroba, Pavel/G-8850-2014; Lokajicek, Milos/G-7800-2014; Kupco, Alexander/G-9713-2014; Marcisovsky, Michal/H-1533-2014; Mikestikova, Marcela/H-1996-2014; Snesarev, Andrey/H-5090-2013; Chudoba, Jiri/G-7737-2014; Peleganchuk, Sergey/J-6722-2014; Santamarina Rios, Cibran/K-4686-2014; Bosman, Martine/J-9917-2014; Grinstein, Sebastian/N-3988-2014; Lei, Xiaowen/O-4348-2014; Demirkoz, Bilge/C-8179-2014; Ventura, Andrea/A-9544-2015; Villaplana Perez, Miguel/B-2717-2015; Livan, Michele/D-7531-2012; Mitsou, Vasiliki/D-1967-2009; CARPENTIERI, CARMELA/E-2137-2015; Joergensen, Morten/E-6847-2015; Martins, Paulo/M-1844-2014; Mir, Lluisa-Maria/G-7212-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Cavalli-Sforza, Matteo/H-7102-2015; Ferrer, Antonio/H-2942-2015; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; Tikhomirov, Vladimir/M-6194-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Akimov, Andrey/N-1769-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Carvalho, Joao/M-4060-2013; Booth, Christopher/B-5263-2016; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Smirnova, Oxana/A-4401-2013; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Samset, Bjorn H./B-9248-2012; Olshevskiy, Alexander/I-1580-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Morone, Maria Cristina/P-4407-2016; Goncalo, Ricardo/M-3153-2016; Canelli, Florencia/O-9693-2016; Idzik, Marek/A-2487-2017; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017 OI Smirnov, Sergei/0000-0002-6778-073X; Gladilin, Leonid/0000-0001-9422-8636; Moorhead, Gareth/0000-0002-9299-9549; Petrucci, Fabrizio/0000-0002-5278-2206; Wemans, Andre/0000-0002-9669-9500; Fabbri, Laura/0000-0002-4002-8353; Kuzhir, Polina/0000-0003-3689-0837; Delmastro, Marco/0000-0003-2992-3805; Veneziano, Stefano/0000-0002-2598-2659; Perrino, Roberto/0000-0002-5764-7337; McKee, Shawn/0000-0002-4551-4502; Rotaru, Marina/0000-0003-3303-5683; Takai, Helio/0000-0001-9253-8307; Britton, David/0000-0001-9998-4342; valente, paolo/0000-0002-5413-0068; Ferrando, James/0000-0002-1007-7816; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Stoicea, Gabriel/0000-0002-7511-4614; Brooks, William/0000-0001-6161-3570; Pina, Joao /0000-0001-8959-5044; Vanyashin, Aleksandr/0000-0002-0367-5666; La Rosa, Alessandro/0000-0001-6291-2142; Moraes, Arthur/0000-0002-5157-5686; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Wolters, Helmut/0000-0002-9588-1773; spagnolo, stefania/0000-0001-7482-6348; Andreazza, Attilio/0000-0001-5161-5759; Della Pietra, Massimo/0000-0003-4446-3368; Cascella, Michele/0000-0003-2091-2501; Orlov, Ilya/0000-0003-4073-0326; Annovi, Alberto/0000-0002-4649-4398; Warburton, Andreas/0000-0002-2298-7315; De, Kaushik/0000-0002-5647-4489; O'Shea, Val/0000-0001-7183-1205; Lee, Jason/0000-0002-2153-1519; Morozov, Sergey/0000-0002-6748-7277; Villa, Mauro/0000-0002-9181-8048; Mikestikova, Marcela/0000-0003-1277-2596; Peleganchuk, Sergey/0000-0003-0907-7592; Santamarina Rios, Cibran/0000-0002-9810-1816; Bosman, Martine/0000-0002-7290-643X; Grinstein, Sebastian/0000-0002-6460-8694; Lei, Xiaowen/0000-0002-2564-8351; Ventura, Andrea/0000-0002-3368-3413; Villaplana Perez, Miguel/0000-0002-0048-4602; Livan, Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886; CARPENTIERI, CARMELA/0000-0002-2994-0317; Joergensen, Morten/0000-0002-6790-9361; Martins, Paulo/0000-0003-3753-3751; Mir, Lluisa-Maria/0000-0002-4276-715X; Riu, Imma/0000-0002-3742-4582; Ferrer, Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543; Grancagnolo, Sergio/0000-0001-8490-8304; Tikhomirov, Vladimir/0000-0002-9634-0581; Camarri, Paolo/0000-0002-5732-5645; Gorelov, Igor/0000-0001-5570-0133; Carvalho, Joao/0000-0002-3015-7821; Booth, Christopher/0000-0002-6051-2847; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Smirnova, Oxana/0000-0003-2517-531X; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Samset, Bjorn H./0000-0001-8013-1833; Olshevskiy, Alexander/0000-0002-8902-1793; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Morone, Maria Cristina/0000-0002-0200-0632; Goncalo, Ricardo/0000-0002-3826-3442; Canelli, Florencia/0000-0001-6361-2117; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; ARTEMIS, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNAS, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia; ROSATOM, Russian Federation; JINR, Serbia; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society and Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; ARTEMIS, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNAS, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 33 TC 14 Z9 14 U1 4 U2 52 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAY PY 2011 VL 71 IS 5 AR 1636 DI 10.1140/epjc/s10052-011-1636-z PG 24 WC Physics, Particles & Fields SC Physics GA 772QJ UT WOS:000291249300022 ER PT J AU Abramowicz, H Abt, I Adamczyk, L Adamus, M Aggarwal, R Antonelli, S Antonioli, P Antonov, A Arneodo, M Aushev, V Aushev, Y Bachynska, O Bamberger, A Barakbaev, AN Barbagli, G Bari, G Barreiro, F Bartosik, N Bartsch, D Basile, M Behnke, O Behr, J Behrens, U Bellagamba, L Bertolin, A Bhadra, S Bindi, M Blohm, C Bokhonov, V Bold, T Bolilyi, O Bondarenko, K Boos, EG Borras, K Boscherini, D Bot, D Brock, I Brownson, E Brugnera, R Brummer, N Bruni, A Bruni, G Brzozowska, B Bussey, PJ Bylsma, B Caldwell, A Capua, M Carlin, R Catterall, CD Chekanov, S Chwastowski, J Ciborowski, J Ciesielski, R Cifarelli, L Cindolo, F Contin, A Cooper-Sarkar, AM Coppola, N Corradi, M Corriveau, F Costa, M D'Agostini, G Dal Corso, F del Peso, J Dementiev, RK De Pasquale, S Derrick, M Devenish, RCE Dobur, D Dolgoshein, BA Dolinska, G Doyle, AT Drugakov, V Durkin, LS Dusini, S Eisenberg, Y Ermolov, PF Eskreys, A Fang, S Fazio, S Ferrando, J Ferrero, MI Figiel, J Forrest, M Foster, B Fourletov, S Gach, G Galas, A Gallo, E Garfagnini, A Geiser, A Gialas, I Gladilin, LK Gladkov, D Glasman, C Gogota, O Golubkov, YA Gottlicher, P Grabowska-Bold, I Grebenyuk, J Gregor, I Grigorescu, G Grzelak, G Gueta, O Gwenlan, C Haas, T Hain, W Hamatsu, R Hart, JC Hartmann, H Hartner, G Hilger, E Hochman, D Hori, R Horton, K Huttmann, A Ibrahim, ZA Iga, Y Ingbir, R Ishitsuka, M Jakob, HP Januschek, F Jimenez, M Jones, TW Jungst, M Kadenko, I Kahle, B Kamaluddin, B Kananov, S Kanno, T Karshon, U Karstens, F Katkov, II Kaur, M Kaur, P Keramidas, A Khein, LA Kim, JY Kisielewska, D Kitamura, S Klanner, R Klein, U Koffeman, E Kooijman, P Korol, I Korzhavina, IA Kotanski, A Kotz, U Kowalski, H Kulinski, P Kuprash, O Kuze, M Lee, A Levchenko, BB Levy, A Libov, V Limentani, S Ling, TY Lisovyi, M Lobodzinska, E Lohmann, W Lohr, B Lohrmann, E Long, KR Longhin, A Lontkovskyi, D Lukina, OY Luzniak, P Maeda, J Magill, S Makarenko, I Malka, J Mankel, R Margotti, A Marini, G Martin, JF Mastroberardino, A Mattingly, MCK Melzer-Pellmann, IA Mergelmeyer, S Miglioranzi, S Idris, FM Monaco, V Montanari, A Morris, JD Mujkic, K Musgrave, B Nagano, K Namsoo, T Nania, R Nicholass, D Nigro, A Ning, Y Nobe, T Noor, U Notz, D Nowak, RJ Nuncio-Quiroz, AE Oh, BY Okazaki, N Oliver, K Olkiewicz, K Onishchuk, Y Papageorgiu, K Parenti, A Paul, E Pawlak, JM Pawlik, B Pelfer, PG Pellegrino, A Perlanski, W Perrey, H Piotrzkowski, K Plucinski, P Pokrovskiy, NS Polini, A Proskuryakov, AS Przybycien, M Raval, A Reeder, DD Reisert, B Ren, Z Repond, J Ri, YD Robertson, A Roloff, P Ron, E Rubinsky, I Ruspa, M Sacchi, R Salii, A Samson, U Sartorelli, G Savin, AA Saxon, DH Schioppa, M Schlenstedt, S Schleper, P Schmidke, WB Schneekloth, U Schonberg, V Schorner-Sadenius, T Schwartz, J Sciulli, F Shcheglova, LM Shehzadi, R Shimizu, S Singh, I Skillicorn, IO Slominski, W Smith, WH Sola, V Solano, A Son, D Sosnovtsev, V Spiridonov, A Stadie, H Stanco, L Stern, A Stewart, TP Stifutkin, A Stopa, P Suchkov, S Susinno, G Suszycki, L Sztuk-Dambietz, J Szuba, D Szuba, J Tapper, AD Tassi, E Terron, J Theedt, T Tiecke, H Tokushuku, K Tomalak, O Tomaszewska, J Tsurugai, T Turcato, M Tymieniecka, T Uribe-Estrada, C Vazquez, M Verbytskyi, A Viazlo, O Vlasov, NN Volynets, O Walczak, R Abdullah, WATW Whitmore, JJ Whyte, J Wiggers, L Wing, M Wlasenko, M Wolf, G Wolfe, H Wrona, K Yagues-Molina, AG Yamada, S Yamazaki, Y Yoshida, R Youngman, C Zarnecki, AF Zawiejski, L Zenaiev, O Zeuner, W Zhautykov, BO Zhmak, N Zhou, C Zichichi, A Zolko, M Zotkin, DS Zulkapli, Z AF Abramowicz, H. Abt, I. Adamczyk, L. Adamus, M. Aggarwal, R. Antonelli, S. Antonioli, P. Antonov, A. Arneodo, M. Aushev, V. Aushev, Y. Bachynska, O. Bamberger, A. Barakbaev, A. N. Barbagli, G. Bari, G. Barreiro, F. Bartosik, N. Bartsch, D. Basile, M. Behnke, O. Behr, J. Behrens, U. Bellagamba, L. Bertolin, A. Bhadra, S. Bindi, M. Blohm, C. Bokhonov, V. Bold, T. Bolilyi, O. Bondarenko, K. Boos, E. G. Borras, K. Boscherini, D. Bot, D. Brock, I. Brownson, E. Brugnera, R. Bruemmer, N. Bruni, A. Bruni, G. Brzozowska, B. Bussey, P. J. Bylsma, B. Caldwell, A. Capua, M. Carlin, R. Catterall, C. D. Chekanov, S. Chwastowski, J. Ciborowski, J. Ciesielski, R. Cifarelli, L. Cindolo, F. Contin, A. Cooper-Sarkar, A. M. Coppola, N. Corradi, M. Corriveau, F. Costa, M. D'Agostini, G. Dal Corso, F. del Peso, J. Dementiev, R. K. De Pasquale, S. Derrick, M. Devenish, R. C. E. Dobur, D. Dolgoshein, B. A. Dolinska, G. Doyle, A. T. Drugakov, V. Durkin, L. S. Dusini, S. Eisenberg, Y. Ermolov, P. F. Eskreys, A. Fang, S. Fazio, S. Ferrando, J. Ferrero, M. I. Figiel, J. Forrest, M. Foster, B. Fourletov, S. Gach, G. Galas, A. Gallo, E. Garfagnini, A. Geiser, A. Gialas, I. Gladilin, L. K. Gladkov, D. Glasman, C. Gogota, O. Golubkov, Yu A. Goettlicher, P. Grabowska-Bold, I. Grebenyuk, J. Gregor, I. Grigorescu, G. Grzelak, G. Gueta, O. Gwenlan, C. Haas, T. Hain, W. Hamatsu, R. Hart, J. C. Hartmann, H. Hartner, G. Hilger, E. Hochman, D. Hori, R. Horton, K. Huettmann, A. Ibrahim, Z. A. Iga, Y. Ingbir, R. Ishitsuka, M. Jakob, H. -P. Januschek, F. Jimenez, M. Jones, T. W. Juengst, M. Kadenko, I. Kahle, B. Kamaluddin, B. Kananov, S. Kanno, T. Karshon, U. Karstens, F. Katkov, I. I. Kaur, M. Kaur, P. Keramidas, A. Khein, L. A. Kim, J. Y. Kisielewska, D. Kitamura, S. Klanner, R. Klein, U. Koffeman, E. Kooijman, P. Korol, I. Korzhavina, I. A. Kotanski, A. Koetz, U. Kowalski, H. Kulinski, P. Kuprash, O. Kuze, M. Lee, A. Levchenko, B. B. Levy, A. Libov, V. Limentani, S. Ling, T. Y. Lisovyi, M. Lobodzinska, E. Lohmann, W. Loehr, B. Lohrmann, E. Long, K. R. Longhin, A. Lontkovskyi, D. Lukina, O. Yu Luzniak, P. Maeda, J. Magill, S. Makarenko, I. Malka, J. Mankel, R. Margotti, A. Marini, G. Martin, J. F. Mastroberardino, A. Mattingly, M. C. K. Melzer-Pellmann, I. -A. Mergelmeyer, S. Miglioranzi, S. Idris, F. Mohamad Monaco, V. Montanari, A. Morris, J. D. Mujkic, K. Musgrave, B. Nagano, K. Namsoo, T. Nania, R. Nicholass, D. Nigro, A. Ning, Y. Nobe, T. Noor, U. Notz, D. Nowak, R. J. Nuncio-Quiroz, A. E. Oh, B. Y. Okazaki, N. Oliver, K. Olkiewicz, K. Onishchuk, Yu Papageorgiu, K. Parenti, A. Paul, E. Pawlak, J. M. Pawlik, B. Pelfer, P. G. Pellegrino, A. Perlanski, W. Perrey, H. Piotrzkowski, K. Plucinski, P. Pokrovskiy, N. S. Polini, A. Proskuryakov, A. S. Przybycien, M. Raval, A. Reeder, D. D. Reisert, B. Ren, Z. Repond, J. Ri, Y. D. Robertson, A. Roloff, P. Ron, E. Rubinsky, I. Ruspa, M. Sacchi, R. Salii, A. Samson, U. Sartorelli, G. Savin, A. A. Saxon, D. H. Schioppa, M. Schlenstedt, S. Schleper, P. Schmidke, W. B. Schneekloth, U. Schoenberg, V. Schoerner-Sadenius, T. Schwartz, J. Sciulli, F. Shcheglova, L. M. Shehzadi, R. Shimizu, S. Singh, I. Skillicorn, I. O. Slominski, W. Smith, W. H. Sola, V. Solano, A. Son, D. Sosnovtsev, V. Spiridonov, A. Stadie, H. Stanco, L. Stern, A. Stewart, T. P. Stifutkin, A. Stopa, P. Suchkov, S. Susinno, G. Suszycki, L. Sztuk-Dambietz, J. Szuba, D. Szuba, J. Tapper, A. D. Tassi, E. Terron, J. Theedt, T. Tiecke, H. Tokushuku, K. Tomalak, O. Tomaszewska, J. Tsurugai, T. Turcato, M. Tymieniecka, T. Uribe-Estrada, C. Vazquez, M. Verbytskyi, A. Viazlo, O. Vlasov, N. N. Volynets, O. Walczak, R. Abdullah, W. A. T. Wan Whitmore, J. J. Whyte, J. Wiggers, L. Wing, M. Wlasenko, M. Wolf, G. Wolfe, H. Wrona, K. Yaguees-Molina, A. G. Yamada, S. Yamazaki, Y. Yoshida, R. Youngman, C. Zarnecki, A. F. Zawiejski, L. Zenaiev, O. Zeuner, W. Zhautykov, B. O. Zhmak, N. Zhou, C. Zichichi, A. Zolko, M. Zotkin, D. S. Zulkapli, Z. CA ZEUS Collaboration TI Measurement of heavy-quark jet photoproduction at HERA SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID CENTRAL TRACKING DETECTOR; ZEUS BARREL CALORIMETER; OPEN BEAUTY PRODUCTION; DIJET CROSS-SECTIONS; PARTON DISTRIBUTIONS; HADRON-COLLISIONS; FLAVOR PRODUCTION; VERTEX DETECTOR; DESIGN; CHARM AB Photoproduction of beauty and charm quarks in events with at least two jets has been measured with the ZEUS detector at HERA using an integrated luminosity of 133 pb(-1). The fractions of jets containing b and c quarks were extracted using the invariant mass of charged tracks associated with secondary vertices and the decay-length significance of these vertices. Differential cross sections as a function of jet transverse momentum, p(T)(jet) T, and pseudora-pidity, eta(jet), were measured. The data are compared with previous measurements and are well described by next-to-leading-order QCD predictions. C1 [Chekanov, S.; Derrick, M.; Magill, S.; Musgrave, B.; Nicholass, D.; Repond, J.; Yoshida, R.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mattingly, M. C. K.] Andrews Univ, Berrien Springs, MI 49104 USA. [Bari, G.; Basile, M.; Bellagamba, L.; Bindi, M.; Boscherini, D.; Bruni, A.; Bruni, G.; Cifarelli, L.; Cindolo, F.; Contin, A.; Corradi, M.; De Pasquale, S.; Margotti, A.; Nania, R.; Polini, A.; Sartorelli, G.; Zichichi, A.] Ist Nazl Fis Nucl, I-40126 Bologna, Italy. [Basile, M.; Bindi, M.; Cifarelli, L.; Contin, A.; De Pasquale, S.; Sartorelli, G.; Zichichi, A.] Univ Bologna, Bologna, Italy. [Bartsch, D.; Brock, I.; Hartmann, H.; Hilger, E.; Jakob, H. -P.; Juengst, M.; Mergelmeyer, S.; Nuncio-Quiroz, A. E.; Paul, E.; Samson, U.; Schoenberg, V.; Shehzadi, R.; Wlasenko, M.] Univ Bonn, Inst Phys, D-5300 Bonn, Germany. [Morris, J. D.] Univ Bristol, HH Wills Phys Lab, Bristol BS8 1TL, Avon, England. [Kaur, M.; Kaur, P.] Panjab Univ, Dept Phys, Chandigarh 160014, India. [Capua, M.; Fazio, S.; Mastroberardino, A.; Schioppa, M.; Susinno, G.] Univ Calabria, Dept Phys, I-87036 Cosenza, Italy. [Capua, M.; Fazio, S.; Mastroberardino, A.; Schioppa, M.; Susinno, G.] Univ Calabria, Ist Nazl Fis Nucl, I-87036 Cosenza, Italy. [Kim, J. Y.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Ibrahim, Z. A.; Kamaluddin, B.; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Zulkapli, Z.] Univ Malaya, Kuala Lumpur 50603, Malaysia. [Ning, Y.; Ren, Z.; Sciulli, F.] Columbia Univ, Nevis Labs, Irvington, NY 10027 USA. [Chwastowski, J.; Eskreys, A.; Figiel, J.; Galas, A.; Olkiewicz, K.; Pawlik, B.; Stopa, P.; Zawiejski, L.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Adamczyk, L.; Bold, T.; Gach, G.; Grabowska-Bold, I.; Kisielewska, D.; Przybycien, M.; Suszycki, L.; Szuba, J.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Kotanski, A.; Slominski, W.] Jagiellonian Univ, Dept Phys, Krakow, Poland. [Bachynska, O.; Behnke, O.; Behr, J.; Behrens, U.; Blohm, C.; Borras, K.; Bot, D.; Ciesielski, R.; Coppola, N.; Fang, S.; Geiser, A.; Goettlicher, P.; Grebenyuk, J.; Gregor, I.; Haas, T.; Hain, W.; Huettmann, A.; Januschek, F.; Kahle, B.; Katkov, I. I.; Klein, U.; Koetz, U.; Kowalski, H.; Libov, V.; Lisovyi, M.; Lobodzinska, E.; Loehr, B.; Mankel, R.; Melzer-Pellmann, I. -A.; Miglioranzi, S.; Montanari, A.; Mujkic, K.; Namsoo, T.; Notz, D.; Parenti, A.; Raval, A.; Roloff, P.; Rubinsky, I.; Schneekloth, U.; Schoerner-Sadenius, T.; Spiridonov, A.; Szuba, D.; Szuba, J.; Theedt, T.; Tomaszewska, J.; Verbytskyi, A.; Wolf, G.; Wrona, K.; Yaguees-Molina, A. G.; Youngman, C.; Zeuner, W.] DESY, D-2000 Hamburg, Germany. [Drugakov, V.; Lohmann, W.; Schlenstedt, S.] DESY, Zeuthen, Germany. [Barbagli, G.; Gallo, E.; Pelfer, P. G.] Ist Nazl Fis Nucl, I-50125 Florence, Italy. [Pelfer, P. G.] Univ Florence, Florence, Italy. [Bamberger, A.; Dobur, D.; Karstens, F.; Vlasov, N. N.] Univ Freiburg, Fak Phys, D-7800 Freiburg, Germany. [Bussey, P. J.; Doyle, A. T.; Forrest, M.; Saxon, D. H.; Skillicorn, I. O.] Univ Glasgow, Sch Phys & Astron, Glasgow, Lanark, Scotland. [Gialas, I.; Papageorgiu, K.] Univ Aegean, Dept Engn Management & Finance, Chios, Greece. [Klanner, R.; Lohrmann, E.; Perrey, H.; Schleper, P.; Stadie, H.; Sztuk-Dambietz, J.; Tassi, E.; Turcato, M.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Long, K. R.; Tapper, A. D.] Univ London Imperial Coll Sci Technol & Med, High Energy Nucl Phys Grp, London, England. [Nagano, K.; Tokushuku, K.; Yamada, S.; Yamazaki, Y.] Natl Lab High Energy Phys, KEK, Inst Particle & Nucl Studies, Tsukuba, Ibaraki 305, Japan. [Barakbaev, A. N.; Boos, E. G.; Pokrovskiy, N. S.; Zhautykov, B. O.] Minist Educ & Sci Kazakhstan, Inst Phys & Technol, Alma Ata, Kazakhstan. [Aushev, V.; Bokhonov, V.; Dolinska, G.; Gogota, O.; Korol, I.; Viazlo, O.; Zhmak, N.] Natl Acad Sci Ukraine, Inst Nucl Res, Kiev, Ukraine. [Aushev, V.; Aushev, Y.; Bartosik, N.; Bolilyi, O.; Bondarenko, K.; Dolinska, G.; Gogota, O.; Kadenko, I.; Korol, I.; Kuprash, O.; Lontkovskyi, D.; Makarenko, I.; Onishchuk, Yu; Salii, A.; Tomalak, O.; Volynets, O.; Zenaiev, O.; Zolko, M.] Natl Taras Shevchenko Univ Kyiv, Dept Nucl Phys, Kiev, Ukraine. [Son, D.] Kyungpook Natl Univ, Ctr High Energy Phys, Taegu, South Korea. [Piotrzkowski, K.] Catholic Univ Louvain, Inst Phys Nucl, B-1348 Louvain, Belgium. [Barreiro, F.; del Peso, J.; Glasman, C.; Jimenez, M.; Ron, E.; Terron, J.; Uribe-Estrada, C.] Univ Autonoma Madrid, Dept Fis Teor, Madrid, Spain. [Corriveau, F.; Schwartz, J.; Zhou, C.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Tsurugai, T.] Meiji Gakuin Univ, Fac Gen Educ, Yokohama, Kanagawa, Japan. [Antonov, A.; Dolgoshein, B. A.; Gladkov, D.; Sosnovtsev, V.; Stifutkin, A.; Suchkov, S.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Dementiev, R. K.; Ermolov, P. F.; Gladilin, L. K.; Golubkov, Yu A.; Khein, L. A.; Korzhavina, I. A.; Levchenko, B. B.; Lukina, O. Yu; Proskuryakov, A. S.; Shcheglova, L. M.; Zotkin, D. S.] Moscow MV Lomonosov State Univ, Inst Nucl Phys, Moscow, Russia. [Abt, I.; Caldwell, A.; Reisert, B.; Schmidke, W. B.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Grigorescu, G.; Keramidas, A.; Koffeman, E.; Kooijman, P.; Pellegrino, A.; Tiecke, H.; Vazquez, M.; Wiggers, L.] Univ Amsterdam, Amsterdam, Netherlands. [Grigorescu, G.; Keramidas, A.; Koffeman, E.; Kooijman, P.; Pellegrino, A.; Tiecke, H.; Vazquez, M.; Wiggers, L.] NIKHEF, Amsterdam, Netherlands. [Bruemmer, N.; Bylsma, B.; Durkin, L. S.; Lee, A.; Ling, T. Y.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Cooper-Sarkar, A. M.; Devenish, R. C. E.; Ferrando, J.; Foster, B.; Gwenlan, C.; Horton, K.; Oliver, K.; Robertson, A.; Walczak, R.] Univ Oxford, Dept Phys, Oxford, England. [Bertolin, A.; Brugnera, R.; Carlin, R.; Dal Corso, F.; Dusini, S.; Garfagnini, A.; Limentani, S.; Longhin, A.; Stanco, L.] Ist Nazl Fis Nucl, Padua, Italy. [Brugnera, R.; Carlin, R.; Garfagnini, A.; Limentani, S.] Univ Padua, Dipartimento Fis, Padua, Italy. [Oh, B. Y.; Whitmore, J. J.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Iga, Y.] Polytech Univ, Sagamihara, Kanagawa, Japan. [D'Agostini, G.; Marini, G.; Nigro, A.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [D'Agostini, G.; Marini, G.; Nigro, A.] Ist Nazl Fis Nucl, Rome, Italy. [Hart, J. C.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Abramowicz, H.; Gueta, O.; Ingbir, R.; Kananov, S.; Levy, A.; Stern, A.] Tel Aviv Univ, Sch Phys, Raymond & Beverly Sackler Fac Exact Sci, Tel Aviv, Israel. [Ishitsuka, M.; Kanno, T.; Kuze, M.; Maeda, J.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [Hori, R.; Okazaki, N.; Shimizu, S.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Hamatsu, R.; Kitamura, S.; Ri, Y. D.] Tokyo Metropolitan Univ, Dept Phys, Tokyo, Japan. [Arneodo, M.; Costa, M.; Ferrero, M. I.; Monaco, V.; Ruspa, M.; Sacchi, R.; Sola, V.; Solano, A.] Ist Nazl Fis Nucl, I-10125 Turin, Italy. [Costa, M.; Ferrero, M. I.; Monaco, V.; Sacchi, R.; Sola, V.; Solano, A.] Univ Turin, Turin, Italy. [Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Turin, Italy. [Fourletov, S.; Martin, J. F.; Stewart, T. P.] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada. [Jones, T. W.; Wing, M.] UCL, Dept Phys & Astron, London, England. [Brzozowska, B.; Ciborowski, J.; Grzelak, G.; Kulinski, P.; Luzniak, P.; Malka, J.; Nowak, R. J.; Pawlak, J. M.; Perlanski, W.; Zarnecki, A. F.] Univ Warsaw, Fac Phys, Warsaw, Poland. [Adamus, M.; Plucinski, P.; Tymieniecka, T.] Inst Nucl Studies, PL-00681 Warsaw, Poland. [Eisenberg, Y.; Hochman, D.; Karshon, U.] Weizmann Inst Sci, Dept Particle Phys & Astrophys, Rehovot, Israel. [Brownson, E.; Reeder, D. D.; Savin, A. A.; Smith, W. H.; Wolfe, H.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Bhadra, S.; Catterall, C. D.; Hartner, G.; Noor, U.; Whyte, J.] York Univ, Dept Phys, N York, ON M3J 1P3, Canada. [Chwastowski, J.] Cracow Univ Technol, Fac Phys Math & Appl Comp Sci, Krakow, Poland. [Spiridonov, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Szuba, D.] INP, Krakow, Poland. [Gialas, I.] DESY, Hamburg, Germany. [Ciborowski, J.] Univ Lodz, PL-90131 Lodz, Poland. [Tymieniecka, T.] Univ Podlasie, Siedlce, Poland. EM levy@alzt.tau.ac.il RI Suchkov, Sergey/M-6671-2015; De Pasquale, Salvatore/B-9165-2008; dusini, stefano/J-3686-2012; Dementiev, Roman/K-7201-2012; Korzhavina, Irina/D-6848-2012; Wiggers, Leo/B-5218-2015; Fazio, Salvatore /G-5156-2010; Doyle, Anthony/C-5889-2009; IBRAHIM, ZAINOL ABIDIN/C-1121-2010; Ferrando, James/A-9192-2012; Gladilin, Leonid/B-5226-2011; Katkov, Igor/E-2627-2012; Levchenko, B./D-9752-2012; Proskuryakov, Alexander/J-6166-2012 OI De Pasquale, Salvatore/0000-0001-9236-0748; dusini, stefano/0000-0002-1128-0664; Chwastowski, Janusz/0000-0002-6190-8376; Wiggers, Leo/0000-0003-1060-0520; Doyle, Anthony/0000-0001-6322-6195; Ferrando, James/0000-0002-1007-7816; Gladilin, Leonid/0000-0001-9422-8636; Katkov, Igor/0000-0003-3064-0466; FU US Department of Energy; Italian National Institute for Nuclear Physics (INFN); German Federal Ministry for Education and Research (BMBF) [05 H09PDF, 05h09GUF]; Science and Technology Facilities Council, UK; Malaysian government; US National Science Foundation; Polish Ministry of Science and Higher Education [DPN/N188/DESY/2009]; Deutsche Forschungsgemeinschaft (DFG) [SFB 676]; Japanese Ministry of Education, Culture, Sports, Science and Technology (MEXT); Korean Ministry of Education; Korea Science and Engineering Foundation; FNRS; IISN; FRIA; Inter-University subsidised by the Belgian Federal Science Policy Office; Spanish Ministry of Education and Science through CICYT; Natural Sciences and Engineering Research Council of Canada (NSERC); RF [N 41-42.2010.2]; Russian Ministry of Education and Science; Netherlands Foundation for Research on Matter (FOM); Israel Science Foundation; Max Planck Institute for Physics, Munich, Germany; Warsaw University, Poland; DESY, Germany; Bogolyubov Institute for Theoretical Physics of the National Academy of Sciences, Ukraine; National Science Foundation; [1 P03B 04529] FX Supported by the US Department of Energy.; Supported by the Italian National Institute for Nuclear Physics (INFN).; Supported by the German Federal Ministry for Education and Research (BMBF), under contract No. 05 H09PDF.; Supported by the Science and Technology Facilities Council, UK.; Supported by an FRGS grant from the Malaysian government.; Supported by the US National Science Foundation. Any opinion, findings and conclusions or recommendations expressed in this material are those of the authors and do not necessarily reflect the views of the National Science Foundation.; Supported by the Polish Ministry of Science and Higher Education as a scientific project No. DPN/N188/DESY/2009.; Supported by the German Federal Ministry for Education and Research (BMBF), under contract No. 05h09GUF, and the SFB 676 of the Deutsche Forschungsgemeinschaft (DFG).; Supported by the Japanese Ministry of Education, Culture, Sports, Science and Technology (MEXT) and its grants for Scientific Research.; Supported by the Korean Ministry of Education and Korea Science and Engineering Foundation.; Supported by FNRS and its associated funds (IISN and FRIA) and by an Inter-University Attraction Poles Programme subsidised by the Belgian Federal Science Policy Office.; Supported by the Spanish Ministry of Education and Science through funds provided by CICYT.; Supported by the Natural Sciences and Engineering Research Council of Canada (NSERC).; Supported by RF Presidential grant N 41-42.2010.2 for the Leading Scientific Schools and by the Russian Ministry of Education and Science through its grant for Scientific Research on High Energy Physics.; Supported by the Netherlands Foundation for Research on Matter (FOM).; Supported by the Israel Science Foundation.; Also funded by Max Planck Institute for Physics, Munich, Germany; Supported by the research grant No. 1 P03B 04529 (2005-2008).; Partially supported by Warsaw University, Poland.; Supported by DESY, Germany.; Supported by the Bogolyubov Institute for Theoretical Physics of the National Academy of Sciences, Ukraine.; This material was based on work supported by the National Science Foundation, while working at the Foundation. NR 54 TC 11 Z9 11 U1 1 U2 16 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAY PY 2011 VL 71 IS 5 AR 1659 DI 10.1140/epjc/s10052-011-1659-5 PG 16 WC Physics, Particles & Fields SC Physics GA 772QJ UT WOS:000291249300007 ER PT J AU Buchmueller, O Cavanaugh, R Colling, D De Roeck, A Dolan, MJ Ellis, JR Flacher, H Heinemeyer, S Isidori, G Olive, K Rogerson, S Ronga, F Weiglein, G AF Buchmueller, O. Cavanaugh, R. Colling, D. De Roeck, A. Dolan, M. J. Ellis, J. R. Flaecher, H. Heinemeyer, S. Isidori, G. Olive, K. Rogerson, S. Ronga, F. Weiglein, G. TI Implications of initial LHC searches for supersymmetry SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID NEUTRALINO DARK-MATTER; LIGHTEST HIGGS-BOSON; LARGE TAN-BETA; ONE-LOOP CORRECTIONS; STANDARD MODEL; RELIC DENSITY; RADIATIVE-CORRECTIONS; MINIMAL SUPERGRAVITY; MASSES; MSSM AB The CMS and ATLAS Collaborations have recently published the results of initial direct LHC searches for supersymmetry analyzing similar to 35/pb of data taken at 7 TeV in the centre of mass. We incorporate these results into a frequentist analysis of the probable ranges of parameters of simple versions of the minimal supersymmetric extension of the Standard Model (MSSM), namely the constrained MSSM (CMSSM), a model with common non-universal Higgs masses (NUHM1), the very constrained MSSM (VCMSSM) and minimal supergravity (mSUGRA). We present updated predictions for the gluino mass, m((g) over tilde), the light-Higgs boson mass, M(h), BR(B(s) -> mu(+)mu(-)) and the spin-independent dark matter scattering cross section, sigma(SI)(p). The CMS and ATLAS data make inroads into the CMSSM, NUHM1 and VCMSSM (but not mSUGRA) parameter spaces, thereby strengthening previous lower limits on sparticle masses and upper limits on sigma(SI)(p) in the CMSSM and VCMSSM. The favoured ranges of BR(B(s) -> mu(+)mu(-)) in the CMSSM, VCMSSM and mSUGRA are close to the Standard Model, but considerably larger values of BR(B(s) -> mu(+)mu(-)) are possible in the NUHM1. Applying the CMS and ATLAS constraints improves the consistency of the model predictions for M(h) with the LEP exclusion limits. C1 [Buchmueller, O.; Colling, D.; Rogerson, S.] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, High Energy Phys Grp, London SW7 2AZ, England. [Cavanaugh, R.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Cavanaugh, R.] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [De Roeck, A.; Ellis, J. R.] CERN, CH-1211 Geneva 23, Switzerland. [De Roeck, A.] Univ Antwerp, B-2610 Antwerp, Belgium. [Dolan, M. J.] Univ Durham, Inst Particle Phys Phenomenol, Durham DH1 3LE, England. [Ellis, J. R.] Kings Coll London, Dept Phys, Theoret Phys & Cosmol Grp, London WC2R 2LS, England. [Flaecher, H.] Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA. [Heinemeyer, S.] Inst Fis Cantabria CSIC UC, Santander 39005, Spain. [Isidori, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Olive, K.] Univ Minnesota, William I Fine Theoret Phys Inst, Minneapolis, MN 55455 USA. [Ronga, F.] ETH, Inst Particle Phys, CH-8093 Zurich, Switzerland. [Weiglein, G.] DESY, D-22607 Hamburg, Germany. RP Buchmueller, O (reprint author), Univ London Imperial Coll Sci Technol & Med, Blackett Lab, High Energy Phys Grp, Prince Consort Rd, London SW7 2AZ, England. EM olive@physics.umn.edu RI Ellis, John/J-2222-2012; OI Ellis, John/0000-0002-7399-0813; DOLAN, MATTHEW/0000-0003-3420-8718 FU European Community's Marie-Curie Research Training Network [MRTN-CT-2006-035505, MRTN-CT-2006-035482]; Spanish MEC [FPA2005-01678]; CICYT [FPA 2007-66387, FPA 2010-22163-C02-01]; DOE, University of Minnesota [DE-FG02-94ER-40823]; DOE [DE-AC02-76SF00515] FX This work was supported in part by the European Community's Marie-Curie Research Training Network under contracts MRTN-CT-2006-035505 'Tools and Precision Calculations for Physics Discoveries at Colliders' and MRTN-CT-2006-035482 'FLAVIAnet', and by the Spanish MEC and FEDER under grant FPA2005-01678. The work of S.H. was supported in part by CICYT (grant FPA 2007-66387 and FPA 2010-22163-C02-01), and the work of K.A.O. was supported in part by DOE grant DE-FG02-94ER-40823 at the University of Minnesota. K.A.O. also thanks SLAC (supported by the DOE under contract number DE-AC02-76SF00515) and the Stanford Institute for Theoretical Physics for their hospitality and support while this work was being finished. NR 127 TC 45 Z9 45 U1 0 U2 3 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAY PY 2011 VL 71 IS 5 AR 1634 DI 10.1140/epjc/s10052-011-1634-1 PG 13 WC Physics, Particles & Fields SC Physics GA 772QJ UT WOS:000291249300028 ER PT J AU Zholents, A Zolotorev, M AF Zholents, A. Zolotorev, M. TI Comment on "Proposal for Raman X-ray free electron laser" SO EUROPEAN PHYSICAL JOURNAL D LA English DT Editorial Material C1 [Zholents, A.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Zolotorev, M.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. RP Zholents, A (reprint author), Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Argonne, IL 60439 USA. EM azholents@aps.anl.gov NR 0 TC 1 Z9 1 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6060 J9 EUR PHYS J D JI Eur. Phys. J. D PD MAY PY 2011 VL 62 IS 3 BP 457 EP 457 DI 10.1140/epjd/e2011-10511-0 PG 1 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 775VM UT WOS:000291491500016 ER PT J AU Gonzalez, J Casas, M Gimenez, J Moreto, M Ramirez, A Labarta, J Valero, M AF Gonzalez, Juan Casas, Marc Gimenez, Judit Moreto, Miquel Ramirez, Alex Labarta, Jesus Valero, Mateo TI SIMULATING WHOLE SUPERCOMPUTER APPLICATIONS SO IEEE MICRO LA English DT Article AB Detailed simulations of large scale message-passing interface parallel applications are extremely time consuming and resource intensive. A new methodology that combines signal processing and data mining techniques plus a multilevel simulation reduces the simulated data by various orders of magnitude. This reduction makes possible detailed software performance analysis and accurate performance predictions in a reasonable time. C1 [Gonzalez, Juan] Univ Politecn Cataluna, Barcelona Supercomp Ctr, Barcelona, Spain. [Casas, Marc] Lawrence Livermore Natl Lab, Livermore, CA USA. [Moreto, Miquel] Univ Politecn Cataluna, Comp Architecture Dept, Girona, Spain. RP Gonzalez, J (reprint author), Campus Nord UPC-C6,Bldg Off 002,C Jordi Girona 1-, Barcelona 08034, Spain. EM juan.gonzalez@bsc.es RI Valero, Mateo/L-5709-2014; Labarta, Jesus/G-5256-2015; Moreto Planas, Miquel/C-1823-2016; OI Valero, Mateo/0000-0003-2917-2482; Labarta, Jesus/0000-0002-7489-4727; Moreto Planas, Miquel/0000-0002-9848-8758; Casas, Marc/0000-0003-4564-2093 FU Ministry of Science and Technology of Spain [TIN2007-60625]; HiPEAC European Network of Excellence; IBM/BSC MareIncognito Project FX This work has been supported by the Ministry of Science and Technology of Spain under contract TIN2007-60625, by the HiPEAC European Network of Excellence, and by the IBM/BSC MareIncognito Project. NR 15 TC 8 Z9 8 U1 0 U2 0 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 0272-1732 J9 IEEE MICRO JI IEEE Micro PD MAY-JUN PY 2011 VL 31 IS 3 BP 32 EP 45 PG 14 WC Computer Science, Hardware & Architecture; Computer Science, Software Engineering SC Computer Science GA 775GB UT WOS:000291445700004 ER PT J AU Gray, G Warren, G AF Gray, George Rusty Warren, Garry TI TMS Changes for Good with Enhanced Volunteerism Program SO JOM LA English DT Article C1 [Gray, George Rusty] Los Alamos Natl Lab, Dynam Mat Properties Sect, Los Alamos, NM USA. [Warren, Garry] Univ Alabama, Dept Met & Mat Engn, Tuscaloosa, AL 35487 USA. RP Los Alamos Natl Lab, Dynam Mat Properties Sect, Los Alamos, NM USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1047-4838 J9 JOM-US JI JOM PD MAY PY 2011 VL 63 IS 5 BP 21 EP 22 PG 2 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering; Mineralogy; Mining & Mineral Processing SC Materials Science; Metallurgy & Metallurgical Engineering; Mineralogy; Mining & Mineral Processing GA 777IY UT WOS:000291610300001 ER PT J AU Blazek, J McQuinn, M Seljak, U AF Blazek, Jonathan McQuinn, Matthew Seljak, Uros TI Testing the tidal alignment model of galaxy intrinsic alignment SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE galaxy formation; weak gravitational lensing; galaxy morphology; cosmological parameters from LSS ID LARGE-SCALE STRUCTURE; WEAK-LENSING SURVEYS; DIGITAL SKY SURVEY; RADIAL ORBIT INSTABILITY; LUMINOUS RED GALAXIES; ELLIPTICITY CORRELATION; SPIN CORRELATIONS; HALO ELLIPTICITY; DISTANT GALAXIES; POWER SPECTRA AB Weak gravitational lensing has become a powerful probe of large-scale structure and cosmological parameters. Precision weak lensing measurements require an understanding of the intrinsic alignment of galaxy ellipticities, which can in turn inform models of galaxy format ion. It is hypothesized that elliptical galaxies align with the background tidal field and that this alignment mechanism dominates the correlation between ellipticities on cosmological scales (in the absence of lensing). We use recent large-scale structure measurements from the Sloan Digital Sky Survey to test this picture with several statistics: (1) the correlation between ellipticity and galaxy overdensity, w(g+); (2) the intrinsic alignment auto-correlation functions; (3) the correlation functions of curl-free. E. and divergence-free, B, modes, the latter of which is zero in the linear tidal alignment theory; (4) the alignment correlation function, w(g)(r(p), theta), a recently developed statistic that generalizes the galaxy correlation function to account for the angle between the galaxy separation vector and the principle axis of ellipticity. We show that recent measurements are largely consistent with the tidal alignment model and discuss dependence on galaxy luminosity. In addition, we show that at linear order the tidal alignment model predicts that the angular dependence of w(g)(r(p), theta) is simply w(g+)(r(p)) COS(2 theta) and that this dependence is consistent with recent measurements. We also study how stochastic nonlinear contributions to galaxy ellipticity impact these statistics. We find that a significant fraction of the observed LEG ellipticity can be explained by alignment with the tidal field on scales greater than or similar to 10 h(-1)Mpc. These considerations are relevant to galaxy formation and evolution. C1 [Blazek, Jonathan; Seljak, Uros] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Blazek, Jonathan; Seljak, Uros] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [McQuinn, Matthew; Seljak, Uros] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Seljak, Uros] Univ Zurich, Inst Theoret Phys, CH-8057 Zurich, Switzerland. [Seljak, Uros] Ewha Womans Univ, Inst Early Universe, Seoul 120750, South Korea. RP Blazek, J (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM blazek@berkeley.edu; mmcquinn@berkeley.edu; useljak@berkeley.edu FU DOE; Swiss National Foundation [200021-116696/1]; WCU [R32-2009-000-10130-0]; NSF; NASA FX We thank Teppei Okumura for several useful discussions and Rachel Mandelbaum for comments on the manuscript. We also thank Cheng Li and Andreas Faltenbacher for sharing their measurements and Michael Schneider for helpful discussion. Finally, we are grateful for comments from an anonymous referee. This work is supported by the DOE, the Swiss National Foundation under contract 200021-116696/1, WCU grant R32-2009-000-10130-0, and an NSF Graduate Research Fellowship. M.M. is supported by a NASA Einstein Fellowship. NR 57 TC 42 Z9 42 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD MAY PY 2011 IS 5 AR 010 DI 10.1088/1475-7516/2011/05/010 PG 22 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 772UY UT WOS:000291264100010 ER PT J AU Jiao, L Zhang, JL Balakirev, FF Chen, GF Luo, JL Wang, NL Yuan, HQ AF Jiao, L. Zhang, J. L. Balakirev, F. F. Chen, G. F. Luo, J. L. Wang, N. L. Yuan, H. Q. TI Upper critical field of the 122-type iron pnictide superconductors SO JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS LA English DT Article; Proceedings Paper CT International Conference on Spectroscopies in Novel Superconductors (SNS2010) CY MAY 23-28, 2010 CL Shanghai, PEOPLES R CHINA DE Superconductor; Critical phenomena; Transport properties ID GAPS AB The upper critical fields (H-c2) of the single crystals (Sr,Na)Fe2As2 and Ba0.55K0.45Fe2As2 were determined by means of measuring the electrical resistivity, rho(xx)(mu H-0), using the facilities of pulsed magnetic field at Los Alamos. In general, these compounds possess a very large upper critical field (H-c2(0)) with a weak anisotropic effect. The detailed curvature of H-c2(T-c) may depend on the magnetic field orientation and the sample compositions. We argue that such a difference mainly results from the multi-band effect, which might be modified via doping. (C) 2010 Elsevier Ltd. All rights reserved. C1 [Jiao, L.; Zhang, J. L.; Yuan, H. Q.] Zhejiang Univ, Dept Phys, Hangzhou 310027, Zhejiang, Peoples R China. [Balakirev, F. F.] Los Alamos Natl Lab, NHMFL, Los Alamos, NM 87545 USA. [Chen, G. F.; Luo, J. L.; Wang, N. L.] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100080, Peoples R China. RP Yuan, HQ (reprint author), Zhejiang Univ, Dept Phys, Hangzhou 310027, Zhejiang, Peoples R China. EM hqyuan@zju.edu.cn NR 21 TC 3 Z9 3 U1 2 U2 12 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-3697 J9 J PHYS CHEM SOLIDS JI J. Phys. Chem. Solids PD MAY PY 2011 VL 72 IS 5 SI SI BP 423 EP 425 DI 10.1016/j.jpcs.2010.10.070 PG 3 WC Chemistry, Multidisciplinary; Physics, Condensed Matter SC Chemistry; Physics GA 776EU UT WOS:000291518100030 ER PT J AU Yoshida, T Nishi, I Fujimori, A Yi, M Moore, RG Luc, DH Shen, ZX Kihou, K Shirage, PM Kito, H Lee, CH Iyo, A Eisaki, H Harima, H AF Yoshida, T. Nishi, I. Fujimori, A. Yi, M. Moore, R. G. Luc, D. -H. Shen, Z. -X. Kihou, K. Shirage, P. M. Kito, H. Lee, C. H. Iyo, A. Eisaki, H. Harima, H. TI Fermi surfaces and quasi-particle band dispersions of the iron pnictides superconductor KFe2As2 observed by angle-resolved photoemission spectroscopy SO JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS LA English DT Article; Proceedings Paper CT International Conference on Spectroscopies in Novel Superconductors (SNS2010) CY MAY 23-28, 2010 CL Shanghai, PEOPLES R CHINA DE Electronic structure AB We have performed an angle-resolved photoemission study of the iron pnictide superconductor KFe2As2 with T-c similar to 4 K. Most of the observed Fermi surfaces show almost two-dimensional shapes, while one of the quasi-particle bands near the Fermi level has a strong dispersion along the k(z) direction, consistent with the result of a band-structure calculation. However, hole Fermi surfaces alpha and zeta are smaller than those predicted by the calculation while other Fermi surfaces are larger. These observations are consistent with the result of a de Haas-van Alphen study and a theoretical prediction on inter-band scattering, possibly indicating many body effects on the electronic structure. (C) 2010 Elsevier Ltd. All rights reserved. C1 [Yoshida, T.; Nishi, I.; Fujimori, A.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Yoshida, T.; Fujimori, A.; Kihou, K.; Shirage, P. M.; Kito, H.; Lee, C. H.; Iyo, A.; Eisaki, H.; Harima, H.] Transformat Res Project Iron Pnictides TRIP, JST, Chiyoda Ku, Tokyo 1020075, Japan. [Yi, M.; Moore, R. G.; Luc, D. -H.; Shen, Z. -X.] Stanford Univ, Stanford Synchrotron Radiat Lab, Stanford, CA 94305 USA. [Yi, M.; Moore, R. G.; Luc, D. -H.; Shen, Z. -X.] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. [Kihou, K.; Shirage, P. M.; Kito, H.; Lee, C. H.; Iyo, A.; Eisaki, H.] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058562, Japan. [Harima, H.] Kobe Univ, Dept Phys, Kobe, Hyogo 6578561, Japan. RP Yoshida, T (reprint author), Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. EM yoshida@wyvern.phys.s.u-tokyo.ac.jp RI Yi, Ming/E-3145-2010 NR 11 TC 33 Z9 34 U1 1 U2 19 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-3697 J9 J PHYS CHEM SOLIDS JI J. Phys. Chem. Solids PD MAY PY 2011 VL 72 IS 5 SI SI BP 465 EP 468 DI 10.1016/j.jpcs.2010.10.064 PG 4 WC Chemistry, Multidisciplinary; Physics, Condensed Matter SC Chemistry; Physics GA 776EU UT WOS:000291518100041 ER PT J AU Homes, CC Akrap, A Wen, JS Xu, ZJ Lin, ZW Li, Q Gu, GD AF Homes, Christopher C. Akrap, Ana Wen, Jinsheng Xu, Zhijun Lin, Zhi Wei Li, Qiang Gu, Genda TI Optical properties of the iron-chalcogenide superconductor FeTe0.55Se0.45 SO JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS LA English DT Article; Proceedings Paper CT International Conference on Spectroscopies in Novel Superconductors (SNS2010) CY MAY 23-28, 2010 CL Shanghai, PEOPLES R CHINA DE Chalcogenides; Infrared spectroscopy; Optical properties; Superconductivity ID HIGH-TEMPERATURE SUPERCONDUCTORS; T-C SUPERCONDUCTORS; PHASE-DIAGRAM; SUM-RULE; CONDUCTIVITY; STATE; BORON; MGB2 AB The complex optical properties of the iron-chalcogenide superconductor FeTe0.55Se0.45 with T-c=14 K have been examined over a wide frequency range for light polarized in the Fe-Te(Se) planes above and below T. At room temperature the optical response may be described by a weakly interacting Fermi liquid; however, just above T-c this picture breaks down and the scattering rate takes on a linear frequency dependence. Below Tc there is evidence for two gap features in the optical conductivity at Delta(1) similar or equal to 2.5 meV and Delta(2) similar or equal to 5.1 meV. Less than 20% of the free carriers collapse into the condensate for T << T-c, and this material is observed to fall on the universal scaling line for a BCS dirty-limit superconductor in the weak-coupling limit. (C) 2010 Elsevier Ltd. All rights reserved. C1 [Homes, Christopher C.; Akrap, Ana; Wen, Jinsheng; Xu, Zhijun; Lin, Zhi Wei; Li, Qiang; Gu, Genda] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Homes, CC (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM homes@bnl.gov RI Wen, Jinsheng/F-4209-2010; xu, zhijun/A-3264-2013; Akrap, Ana/G-1409-2013 OI Wen, Jinsheng/0000-0001-5864-1466; xu, zhijun/0000-0001-7486-2015; Akrap, Ana/0000-0003-4493-5273 NR 85 TC 7 Z9 7 U1 0 U2 16 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-3697 J9 J PHYS CHEM SOLIDS JI J. Phys. Chem. Solids PD MAY PY 2011 VL 72 IS 5 SI SI BP 505 EP 510 DI 10.1016/j.jpcs.2010.10.014 PG 6 WC Chemistry, Multidisciplinary; Physics, Condensed Matter SC Chemistry; Physics GA 776EU UT WOS:000291518100050 ER PT J AU Le Tacon, M Forrest, TR Ruegg, C Bosak, A Noffsinger, J Walters, AC Toulemonde, P Palenzona, A Zhigadlo, ND Karpinski, J Hill, JP Krisch, M McMorrow, DF AF Le Tacon, Mathieu Forrest, T. R. Rueegg, Ch Bosak, A. Noffsinger, J. Walters, A. C. Toulemonde, P. Palenzona, A. Zhigadlo, N. D. Karpinski, J. Hill, J. P. Krisch, M. McMorrow, D. F. TI Inelastic X-ray scattering investigations of lattice dynamics in SmFeAsO1-xFy superconductors SO JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS LA English DT Article; Proceedings Paper CT International Conference on Spectroscopies in Novel Superconductors (SNS2010) CY MAY 23-28, 2010 CL Shanghai, PEOPLES R CHINA DE Superconductors; Lattice dynamics; Phonons ID IRON; COMPOUND AB We report measurements of the phonon density of states as probed with inelastic X-ray scattering in SmFeAsO1-xFy powders. An unexpected strong renormalization of phonon branches around 23 meV is observed as fluorine is substituted for oxygen. Phonon dispersion measurements on SmFeAsO1-xFy single crystals allow us to identify the 21 meV A(1g) in-phase (Sm,As) and the 26 meV B-1g (Fe,O) modes to be responsible for this renormalization, and may reveal unusual electron-phonon coupling through the spin channel in iron-based superconductors. (C) 2010 Elsevier Ltd. All rights reserved. C1 [Le Tacon, Mathieu] Max Planck Inst Festkorperforsch, D-70569 Stuttgart, Germany. [Forrest, T. R.; Rueegg, Ch; Walters, A. C.; McMorrow, D. F.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Forrest, T. R.; Rueegg, Ch; Walters, A. C.; McMorrow, D. F.] UCL, London Ctr Nanotechnol, London WC1E 6BT, England. [Forrest, T. R.; Noffsinger, J.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bosak, A.; Walters, A. C.; Krisch, M.] European Synchrotron Radiat Facil, F-38043 Grenoble, France. [Noffsinger, J.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Toulemonde, P.] CNRS UJF, Inst Neel, Grenoble, France. [Palenzona, A.] CNR INFM LAMIA Artificial & Innovat Mat Lab, I-16152 Genoa, Italy. [Palenzona, A.] Univ Genoa, Dept Chem & Ind Chem, I-16146 Genoa, Italy. [Zhigadlo, N. D.; Karpinski, J.] ETH, Solid State Phys Lab, CH-8093 Zurich, Switzerland. [Hill, J. P.] Brookhaven Natl Lab, Dept Condensed Matter Phys & Mat Sci, Upton, NY 11973 USA. RP Le Tacon, M (reprint author), Max Planck Inst Festkorperforsch, Heisenbergstr 1, D-70569 Stuttgart, Germany. EM m.letacon@fkf.mpg.de RI Le Tacon, Mathieu/D-8023-2011; Hill, John/F-6549-2011; Ruegg, Christian/A-3476-2012; BOSAK, Alexei/J-7895-2013; McMorrow, Desmond/C-2655-2008 OI Le Tacon, Mathieu/0000-0002-5838-3724; Ruegg, Christian/0000-0003-0139-7786; McMorrow, Desmond/0000-0002-4947-7788 NR 28 TC 3 Z9 3 U1 0 U2 8 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-3697 J9 J PHYS CHEM SOLIDS JI J. Phys. Chem. Solids PD MAY PY 2011 VL 72 IS 5 SI SI BP 523 EP 526 DI 10.1016/j.jpcs.2010.10.006 PG 4 WC Chemistry, Multidisciplinary; Physics, Condensed Matter SC Chemistry; Physics GA 776EU UT WOS:000291518100054 ER PT J AU Song, DJ Kyung, WS Park, SR Leem, CS Kim, C Kim, YK Choi, SK Jung, WS Koh, YY Choi, HY Han, G Yoshida, Y Eisaki, H Lu, DH Shen, ZX Kim, C AF Song, D. J. Kyung, W. S. Park, S. R. Leem, C. S. Kim, Chul Kim, Y. K. Choi, S. K. Jung, W. S. Koh, Y. Y. Choi, H. Y. Han, Garam Yoshida, Yoshiyuki Eisaki, Hirosh Lu, D. H. Shen, Z. -X. Kim, C. TI Photoemission studies on electron doped cuprate Pr0.85LaCe0.15CuO4: Revisiting the chemical pressure effect SO JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS LA English DT Article; Proceedings Paper CT International Conference on Spectroscopies in Novel Superconductors (SNS2010) CY MAY 23-28, 2010 CL Shanghai, PEOPLES R CHINA DE Cuprate; Electron doped compound; Antiferromagnetic materials; Electronic structure; Photoemission and photoelectron spectra ID TEMPERATURE SUPERCONDUCTOR; STATE; GAP AB We performed angle resolved photoemission spectroscopy (ARPES) experiments on electron doped cuprates Pr0.85LaCe0.15CuO4 (PLCCO) and Nd1.85Ce0.15CuO4 (NCCO). Critical temperatures (T-c) of PLCCO and NCCO are similar but PLCCO has weaker Fermi surface curvature than NCCO. As the ionic radius of Pr and La is larger than that of Nd, this result is inconsistent with the earlier view that chemical pressure determines the Fermi surface curvature. On the other hand, anti-ferromagnetic (AFM) band renormalization effect in PLCCO is larger than that in NCCO, which implies AFM is stronger in PLCCO. This is consistent not only with the view that AFM is correlated with t'/t but also with recent inelastic neutron scattering results. Therefore, we suggest that the chemical pressure effect is not the only factor that determines the Fermi surface topology. (C) 2010 Elsevier Ltd. All rights reserved. C1 [Song, D. J.; Kyung, W. S.; Park, S. R.; Leem, C. S.; Kim, Chul; Kim, Y. K.; Choi, S. K.; Jung, W. S.; Koh, Y. Y.; Choi, H. Y.; Han, Garam; Kim, C.] Yonsei Univ, Inst Phys & Appl Phys, Seoul 120749, South Korea. [Yoshida, Yoshiyuki; Eisaki, Hirosh] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058568, Japan. [Lu, D. H.; Shen, Z. -X.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Lu, D. H.; Shen, Z. -X.] Stanford Univ, Stanford Synchrotron Radiat Lab, Stanford, CA 94305 USA. RP Kim, C (reprint author), Yonsei Univ, Inst Phys & Appl Phys, Seoul 120749, South Korea. EM changyoung@yonsei.ac.kr; changyoung@yonsei.ac.kr RI Kim, Yeong Kwan/L-8207-2016 NR 18 TC 0 Z9 0 U1 2 U2 6 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-3697 J9 J PHYS CHEM SOLIDS JI J. Phys. Chem. Solids PD MAY PY 2011 VL 72 IS 5 SI SI BP 533 EP 535 DI 10.1016/j.jpcs.2010.10.069 PG 3 WC Chemistry, Multidisciplinary; Physics, Condensed Matter SC Chemistry; Physics GA 776EU UT WOS:000291518100057 ER PT J AU Kim, C Kyung, WS Park, SR Leem, CS Song, DJ Kim, YK Choi, SK Jung, WS Koh, YY Choi, HY Yoshida, Y Moore, RG Shen, ZX Kim, C AF Kim, Chul Kyung, W. S. Park, S. R. Leem, C. S. Song, D. J. Kim, Y. K. Choi, S. K. Jung, W. S. Koh, Y. Y. Choi, H. Y. Yoshida, Yoshiyuki Moore, R. G. Shen, Z. -X Kim, C. TI Self-energy analysis of multiple-bosonic mode coupling in Sr2RuO4 SO JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS LA English DT Article; Proceedings Paper CT International Conference on Spectroscopies in Novel Superconductors (SNS2010) CY MAY 23-28, 2010 CL Shanghai, PEOPLES R CHINA DE Oxides; Photoelectron spectroscopy; Electronic structure ID SUPERCONDUCTOR SR2RUO4; LAYERED PEROVSKITE AB We report angle-resolved photoemission spectroscopy studies on Sr2RuO4. We observe multiple-bosonic mode coupling in the alpha and beta band dispersions. To extract the self-energy from the data for which the usual fitting methods do not work well, we propose a scheme that exploits the relation between the spectral intensity and self-energy, termed as relative self-energy. The relative self-energy obtained in that way contains important features of the self-energy. We observe not only the features that can be obtained from the band dispersions but also additional features that were not seen. (C) 2010 Elsevier Ltd. All rights reserved. C1 [Kim, Chul; Kyung, W. S.; Park, S. R.; Leem, C. S.; Song, D. J.; Kim, Y. K.; Choi, S. K.; Jung, W. S.; Koh, Y. Y.; Choi, H. Y.; Kim, C.] Yonsei Univ, Inst Phys & Appl Phys, Seoul 120749, South Korea. [Yoshida, Yoshiyuki] Natl Inst Adv Ind Sci & Technol, Nanoelect Res Inst, Tsukuba, Ibaraki 3058568, Japan. [Moore, R. G.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Shen, Z. -X] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Shen, Z. -X] Stanford Univ, Stanford Synchrotron Radiat Lab, Stanford, CA 94305 USA. RP Kim, C (reprint author), Yonsei Univ, Inst Phys & Appl Phys, Seoul 120749, South Korea. EM changyoung@yonsei.ac.kr; changyoung@yonsei.ac.kr RI Kim, Yeong Kwan/L-8207-2016 NR 20 TC 2 Z9 2 U1 1 U2 5 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-3697 J9 J PHYS CHEM SOLIDS JI J. Phys. Chem. Solids PD MAY PY 2011 VL 72 IS 5 SI SI BP 556 EP 558 DI 10.1016/j.jpcs.2010.10.068 PG 3 WC Chemistry, Multidisciplinary; Physics, Condensed Matter SC Chemistry; Physics GA 776EU UT WOS:000291518100063 ER PT J AU Yuan, HQ Chen, J Singleton, J Akutagawa, S Akimitsu, J AF Yuan, H. Q. Chen, J. Singleton, J. Akutagawa, S. Akimitsu, J. TI Large upper critical field in non-centrosymmetric superconductor Y2C3 SO JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS LA English DT Article; Proceedings Paper CT International Conference on Spectroscopies in Novel Superconductors (SNS2010) CY MAY 23-28, 2010 CL Shanghai, PEOPLES R CHINA DE Superconductor; Critical phenomena; Thermodynamic properties ID YTTRIUM SESQUICARBIDE SYSTEM; 18 K AB We determine the upper critical field mu H-0(c2)(T-c) of non-centrosymmetric superconductor Y2C3 using two distinct methods: the bulk magnetization M(T) and the tunnel-diode oscillator (TDO) based impedance measurements. It is found that the upper critical field reaches a value of 30 Tat zero temperature which is above the weak-coupling Pauli paramagnetic limit. We argue that the observation of such a large mu H-0(c2)(0) in Y2C3 could be attributed to the admixture of spin-singlet and spin-triplet pairing states as a result of broken inversion symmetry. (C) 2010 Elsevier Ltd. All rights reserved. C1 [Yuan, H. Q.; Chen, J.] Zhejiang Univ, Dept Phys, Hangzhou 310027, Peoples R China. [Singleton, J.] Los Alamos Natl Lab, NHMFL, Los Alamos, NM 87545 USA. [Akutagawa, S.; Akimitsu, J.] Aoyama Gakuin Univ, Dept Math & Phys, Kanagawa 2298558, Japan. RP Yuan, HQ (reprint author), Zhejiang Univ, Dept Phys, Hangzhou 310027, Peoples R China. EM hqyuan@zju.edu.cn NR 30 TC 3 Z9 3 U1 3 U2 14 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-3697 J9 J PHYS CHEM SOLIDS JI J. Phys. Chem. Solids PD MAY PY 2011 VL 72 IS 5 SI SI BP 577 EP 579 DI 10.1016/j.jpcs.2010.10.072 PG 3 WC Chemistry, Multidisciplinary; Physics, Condensed Matter SC Chemistry; Physics GA 776EU UT WOS:000291518100069 ER PT J AU Homer, C Cooper, L Gonzalez, A AF Homer, Christina Cooper, Laura Gonzalez, Ana TI Energy dependence of site-specific radiation damage in protein crystals SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE specific radiation damage; disulphide bridges; methionine sulphur; cystein suphur; X-ray energy ID X-RAY DATA; DATA-COLLECTION; MACROMOLECULAR CRYSTALLOGRAPHY; SYNCHROTRON-RADIATION; CRYOGENIC TEMPERATURES; BIOLOGICAL SAMPLES; DATA QUALITY; WAVELENGTH; SCAVENGERS; CHOICE AB It is important to consider radiation damage to crystals caused by data collection when solving structures and critical when determining protein function, which can often depend on very subtle structural characteristics. In this study the rate of damage to specific sites in protein crystals cooled at 100 K is found to depend on the energy of the incident X-ray beam. Several lysozyme crystals were each subjected to 3-26 MGy of cumulative X-ray exposure by collecting multiple data sets from each crystal at either 9 keV or 14 keV. The integrated electron density surrounding each S atom in the structure was calculated for each data set and the change in electron density was evaluated as a function of dose at the two energies. The rate of electron density decrease per cubic A per MGy was determined to be greater at 14 keV than at 9 keV for cysteine sulfurs involved in disulphide bridges; no statistically significant differences in the decay rates were found for methionine sulfurs. These preliminary results imply that it might be possible to minimize certain types of specific radiation damage by an appropriate choice of energy. Further experiments studying a variety of photolabile sites over a wider range of energies are needed to confirm this conclusion. C1 [Homer, Christina; Cooper, Laura; Gonzalez, Ana] SSRL, Menlo Pk, CA 94025 USA. RP Gonzalez, A (reprint author), SSRL, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. EM ana@slac.stanford.edu FU Department of Energy, Office of Biological and Environmental Research; National Institutes of Health; National Center for Research Resources; Biomedical Technology Program; National Institute of General Medical Sciences; Science Teacher and Researcher (STAR) program; National Center for Research Resources, a component of the National Institutes of Health [P41 RR001209] FX This research was carried out at the Stanford Synchrotron Radiation Lightsource, a national user facility operated by Stanford University on behalf of the US Department of Energy, Office of Basic Energy Sciences. The SSRL Structural Molecular Biology Program is supported by the Department of Energy, Office of Biological and Environmental Research, and by the National Institutes of Health, National Center for Research Resources, Biomedical Technology Program, and the National Institute of General Medical Sciences. LC was supported by the Science Teacher and Researcher (STAR) program. The authors thank the SSRL Molecular Crystallography group for their support and, in particular, Irimpan Mathews for the help preparing the crystals used in the experiment. The project described was supported by Award Number P41 RR001209 from the National Center for Research Resources, a component of the National Institutes of Health, and its contents are solely the responsibility of the authors and do not necessarily represent the official view of NCRR or NIH. NR 46 TC 8 Z9 8 U1 1 U2 6 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0909-0495 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD MAY PY 2011 VL 18 BP 338 EP 345 DI 10.1107/S0909049511005504 PN 3 PG 8 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA 774QT UT WOS:000291401900004 PM 21525641 ER PT J AU Orville, AM Buono, R Cowan, M Heroux, A Shea-McCarthy, G Schneider, DK Skinner, JM Skinner, MJ Stoner-Ma, D Sweet, RM AF Orville, Allen M. Buono, Richard Cowan, Matt Heroux, Annie Shea-McCarthy, Grace Schneider, Dieter K. Skinner, John M. Skinner, Michael J. Stoner-Ma, Deborah Sweet, Robert M. TI Correlated single-crystal electronic absorption spectroscopy and X-ray crystallography at NSLS beamline X26-C SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE metalloenzymes; cofactors; electronic absorption spectroscopy; Raman spectroscopy ID PHOTOACTIVE YELLOW PROTEIN; UV-VIS SPECTROSCOPY; MACROMOLECULAR CRYSTALLOGRAPHY; RAMAN-SPECTROSCOPY; INTEGRATED SOFTWARE; BIOLOGICAL CRYSTALS; FLUORESCENT PROTEIN; SIGNAL-TRANSDUCTION; STRUCTURAL-ANALYSIS; CATALYTIC PATHWAY AB The research philosophy and new capabilities installed at NSLS beamline X26-C to support electronic absorption and Raman spectroscopies coupled with X-ray diffraction are reviewed. This beamline is dedicated full time to multidisciplinary studies with goals that include revealing the relationship between the electronic and atomic structures in macromolecules. The beamline instrumentation has been fully integrated such that optical absorption spectra and X-ray diffraction images are interlaced. Therefore, optical changes induced by X-ray exposure can be correlated with X-ray diffraction data collection. The installation of Raman spectroscopy into the beamline is also briefly reviewed. Data are now routinely generated almost simultaneously from three complementary types of experiments from the same sample. The beamline is available now to the NSLS general user population. C1 [Orville, Allen M.; Buono, Richard; Cowan, Matt; Heroux, Annie; Shea-McCarthy, Grace; Schneider, Dieter K.; Skinner, John M.; Skinner, Michael J.; Stoner-Ma, Deborah; Sweet, Robert M.] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. RP Orville, AM (reprint author), Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. EM amorv@bnl.gov FU Office of Biological and Environmental Research, US Department of Energy [FWP BO-70]; National Center for Research Resources of the National Institutes of Health [2-P41-RR012408]; US Department of Energy Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by the Office of Biological and Environmental Research, US Department of Energy (FWP BO-70), and the National Center for Research Resources (2-P41-RR012408) of the National Institutes of Health. Data for this review were measured, in part, at beamline X26-C of the National Synchrotron Light Source (NSLS) at the Brookhaven National Laboratory. Use of the NSLS was supported by the US Department of Energy Office of Basic Energy Sciences, under Contract DE-AC02-98CH10886. We are grateful to the many users who collaborate with us as we continue to improve our capabilities at beamline X26-C. We also thank the entire PXRR staff and the many beamline scientists at ESRF, SLS, Diamond and Soliel for their kind openness and for sharing their insights from developing similar capabilities in Europe. NR 63 TC 19 Z9 19 U1 0 U2 6 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0909-0495 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD MAY PY 2011 VL 18 BP 358 EP 366 DI 10.1107/S0909049511006315 PN 3 PG 9 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA 774QT UT WOS:000291401900006 PM 21525643 ER PT J AU Titarenko, S Titarenko, V Kyrieleis, A Withers, PJ De Carlo, F AF Titarenko, Sofya Titarenko, Valeriy Kyrieleis, Albrecht Withers, Philip J. De Carlo, Francesco TI Suppression of ring artefacts when tomographing anisotropically attenuating samples SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE X-ray absorption computerized tomography; laterally extended objects; ring artefacts; filtered back-projection; inverse problem; laminography ID MICROTOMOGRAPHY; DETECTORS; IMAGES AB There are many objects for which the attenuation varies significantly as they are rotated during computerized X-ray tomography, for example plate samples. This can lead to significant ring artefacts in the subsequent tomographic reconstructions. In this paper a new method is presented that can successfully suppress such ring artefacts and is applicable to both parallel and cone-beam geometries. Rapid correction is achieved via an analytical formula which involves only a matrix-vector multiplication, for which the matrix is known and depends on a regularization parameter. The efficacy of the method is demonstrated for a paleontological sample (calcified shark cartilage) and a carbon-carbon composite/Ti-SiC metal matrix composite test sample. C1 [Titarenko, Valeriy; Kyrieleis, Albrecht; Withers, Philip J.] Univ Manchester, Sch Mat, Henry Moseley Xray Imaging Facil, Manchester M1 7HS, Lancs, England. [Titarenko, Sofya] Moscow MV Lomonosov State Univ, Dept Math, Fac Phys, Moscow 119991, Russia. [De Carlo, Francesco] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Titarenko, V (reprint author), Univ Manchester, Sch Mat, Henry Moseley Xray Imaging Facil, Grosvenor St, Manchester M1 7HS, Lancs, England. EM valeriy.titarenko@manchester.ac.uk RI Withers, Philip/A-6760-2009 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; EPSRC; STFC FX The authors would like to thank the Diamond Light Source for use of the X-ray light source. The use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The piece of shark cartilage was provided by Professor Michael Coates (University of Chicago) and scanned by Mason Dean (Max Planck Institute). ST is grateful to EPSRC for funds through the 'Collaborating for Success' grant. VT and AK are grateful to STFC for funding the project. NR 32 TC 15 Z9 15 U1 1 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0909-0495 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD MAY PY 2011 VL 18 BP 427 EP 435 DI 10.1107/S0909049511006005 PN 3 PG 9 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA 774QT UT WOS:000291401900014 PM 21525651 ER PT J AU Kelly, ST Trenkle, JC Koerner, LJ Barron, SC Walker, N Pouliquen, PO Tate, MW Gruner, SM Dufresne, EM Weihs, TP Hufnagel, TC AF Kelly, Stephen T. Trenkle, Jonathan C. Koerner, Lucas J. Barron, Sara C. Walker, Noeel Pouliquen, Philippe O. Tate, Mark W. Gruner, Sol M. Dufresne, Eric M. Weihs, Timothy P. Hufnagel, Todd C. TI Fast X-ray microdiffraction techniques for studying irreversible transformations in materials SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE X-ray diffraction; phase transformations ID PIXEL-ARRAY DETECTOR; SYNCHROTRON-RADIATION; DIFFRACTION; SCATTERING; LASER; SHUTTER; OPTICS AB A pair of techniques have been developed for performing time-resolved X-ray microdiffraction on irreversible phase transformations. In one technique capillary optics are used to focus a high-flux broad-spectrum X-ray beam to a 60 mu m spot size and a fast pixel array detector is used to achieve temporal resolution of 55 mu s. In the second technique the X-rays are focused with Kirkpatrick-Baez mirrors to achieve a spatial resolution better than 10 mu m and a fast shutter is used to provide temporal resolution better than 20 mu s while recording the diffraction pattern on a (relatively slow) X-ray CCD camera. Example data from experiments are presented where these techniques are used to study self-propagating high-temperature synthesis reactions in metal laminate foils. C1 [Kelly, Stephen T.; Trenkle, Jonathan C.; Barron, Sara C.; Walker, Noeel; Weihs, Timothy P.; Hufnagel, Todd C.] Johns Hopkins Univ, Dept Mat Sci & Engn, Baltimore, MD 21218 USA. [Koerner, Lucas J.; Tate, Mark W.; Gruner, Sol M.] Cornell Univ, Dept Phys, Ithaca, NY 14853 USA. [Pouliquen, Philippe O.] Johns Hopkins Univ, Dept Elect & Comp Engn, Baltimore, MD 21218 USA. [Gruner, Sol M.] Cornell Univ, Cornell High Energy Synchrotron Source, Ithaca, NY 14853 USA. [Dufresne, Eric M.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Hufnagel, TC (reprint author), Johns Hopkins Univ, Dept Mat Sci & Engn, Baltimore, MD 21218 USA. EM hufnagel@jhu.edu RI Weihs, Timothy/A-3313-2010; Gruner, Sol/G-2924-2010; Hufnagel, Todd/A-3309-2010 OI Gruner, Sol/0000-0002-1171-4426; Hufnagel, Todd/0000-0002-6373-9377 FU National Science Foundation [DMI-0300396]; Department of Energy [FG02-97ER62443, DE-FG02-09ER46648]; Office of Naval Research [N000014-07-1-0740]; National Science Foundation; National Institutes of Health/National Institutes of General Medical Sciences [DMR-0225180]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We gratefully acknowledge Alexander Kazimirov, Darol Chamberlain, Daniel Schuette, Darren Southworth and Harish Nathani for their assistance with the experiments at CHESS, and Sterling Cornaby and Don Bilderback for providing the X-ray capillary. We also acknowledge Kurt Goetze and Ulrich Lienert for their help developing the fast X-ray shutter used in the APS experiments. This work proceeded in stages over several years, with two rounds of experiments at CHESS and three at APS. Financial support was provided by the National Science Foundation (grant No. DMI-0300396, with Howmet Research Corporation as the industrial partner) for JCT, TPW and TCH for the experiments at CHESS; the Department of Energy (grant No. FG02-97ER62443) for LJK, MWT and SMG for the experiments at CHESS; the Office of Naval Research (grant No. N000014-07-1-0740) for NW, TPW and TCH for the first round and SCB for the second round of experiments at APS; and the Department of Energy (grant No. DE-FG02-09ER46648) for STK, SCB, TPW and TCH for the third round of experiments at APS. Portions of this research were conducted at the Cornell High Energy Synchrotron Source (CHESS), which is supported by the National Science Foundation and the National Institutes of Health/National Institutes of General Medical Sciences under award DMR-0225180. Use of the Advanced Photon Source (APS) was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 37 TC 10 Z9 10 U1 1 U2 15 PU WILEY-BLACKWELL PI MALDEN PA COMMERCE PLACE, 350 MAIN ST, MALDEN 02148, MA USA SN 0909-0495 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD MAY PY 2011 VL 18 BP 464 EP 474 DI 10.1107/S0909049511002640 PN 3 PG 11 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA 774QT UT WOS:000291401900019 PM 21525656 ER PT J AU Said, AH Sinn, H Divan, R AF Said, Ayman H. Sinn, Harald Divan, Ralu TI New developments in fabrication of high-energy-resolution analyzers for inelastic X-ray spectroscopy SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE high-energy-resolution analyzers; inelastic X-ray scattering spectroscopy ID SCATTERING; MONOCHROMATOR AB In this work new improvements related to the fabrication of spherical bent analyzers for 1 meV energy-resolution inelastic X-ray scattering spectroscopy are presented. The new method includes the use of a two-dimensional bender to achieve the required radius of curvature for X-ray analyzers. The advantage of this method is the ability to monitor the focus during bending, which leads to higher-efficiency analyzers. C1 [Said, Ayman H.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Sinn, Harald] European XFEL, D-22607 Hamburg, Germany. [Divan, Ralu] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Said, AH (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. EM said@aps.anl.gov FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; NSF [DMR-0115852] FX We would like to thank Dr Bran Brajuskovic for providing some of the engineering drawings. Also, we would like to thank Ruben Khachatryan and Michael Wiezorek for their help during cutting, orienting and etching of the crystals. We would like to thank Tim Roberts for his help with setting up the tables used to mount the laser and bender. Use of the Advanced Photon Source and Center for Nanoscale Materials at Argonne National Laboratory was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The construction of HERIX was partially supported by the NSF under Grant No. DMR-0115852. NR 15 TC 28 Z9 28 U1 0 U2 8 PU WILEY-BLACKWELL PI MALDEN PA COMMERCE PLACE, 350 MAIN ST, MALDEN 02148, MA USA SN 0909-0495 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD MAY PY 2011 VL 18 BP 492 EP 496 DI 10.1107/S0909049511001828 PN 3 PG 5 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA 774QT UT WOS:000291401900022 PM 21525659 ER PT J AU Yang, X Tsang, T Murphy, J Shen, Y Wang, XJ AF Yang, X. Tsang, T. Murphy, J. Shen, Y. Wang, X. J. TI Electron bunch length monitors using spatially encoded electro-optical technique SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT International Workshop on Ultra-short Electron & Photon Beams - Techniques and Applications CY SEP 07-11, 2009 CL Xian, PEOPLES R CHINA DE Photoinjector; Bunch length monitor ID BEAM AB A single-shot, nondestructive, electro-optical, electron bunch length monitor is experimentally verified by encoding the Coulomb field of the bunch profile on the spatial intensity distribution of an unchirped femtosecond laser pulse in an orthogonal geometry (hence, a temporal-to-spatial transformation). This electron bunch measurement scheme can simultaneously measure large timing jitter (similar to ps) with a wide measurement timespan covering picosecond to subpicosecond ranges. Published by Elsevier B.V. C1 [Yang, X.; Murphy, J.; Shen, Y.; Wang, X. J.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Tsang, T.; Murphy, J.; Shen, Y.; Wang, X. J.] Brookhaven Natl Lab, Instrumentat Div, Upton, NY 11973 USA. RP Yang, X (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. EM xiyang@bnl.gov FU Office of Naval Research (ONR); High Energy Laser Joint Technology Office (JTO); US Department of Energy (DOE) [DE-AC02-98CH1-886] FX This work is supported in part by the Office of Naval Research (ONR), the High Energy Laser Joint Technology Office (JTO), and the US Department of Energy (DOE) under contract No. DE-AC02-98CH1-886. NR 10 TC 0 Z9 0 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAY 1 PY 2011 VL 637 SU 1 BP S20 EP S23 DI 10.1016/j.nima.2010.02.013 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 774WD UT WOS:000291416600006 ER PT J AU Kovtun, IV Johnson, KO McMurray, CT AF Kovtun, Irina V. Johnson, Kurt O. McMurray, Cynthia T. TI Cockayne Syndrome B protein antagonizes OGG1 in modulating CAG repeat length in vivo SO AGING-US LA English DT Article DE CSB; transcription coupled repair; CAG expansion; base excision DNA repair; Huntington's Disease ID BASE EXCISION-REPAIR; TRANSGENIC MICE; TRINUCLEOTIDE EXPANSION; OXIDATIVE DAMAGE; COUPLING FACTOR; DNA; TRANSCRIPTION; INSTABILITY; CELLS; DISEASE AB OGG1 and MSH2/MSH3 promote CAG repeat expansion at Huntington(1)s disease (HD) locus in vivo during removal of oxidized bases from DNA. CSB, a transcription-coupled repair (TCR) protein, facilitates repair of some of the same oxidative lesions. In vitro, a knock down CSB results in a reduction of transcription-induced deletions at CAG repeat tract. To test the role of CSB in vivo, we measured intergenerational and somatic expansion of CAG tracts in HD mice lacking CSB, OGG1, or both. We provide evidence that CSB protects CAG repeats from expansion by either active reduction of the tract length during parent-child transmission, or by antagonizing the action of OGG1, which tends to promote expansion in somatic cells. These results raise a possibility that actions of transcription-coupled and base excision repair pathways lead to different outcomes at CAG tracts in vivo. C1 [Kovtun, Irina V.; Johnson, Kurt O.; McMurray, Cynthia T.] Mayo Clin & Mayo Fdn, Dept Pharmacol & Expt Therapeut, Rochester, MN 55905 USA. [McMurray, Cynthia T.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Kovtun, IV (reprint author), Mayo Clin & Mayo Fdn, Dept Pharmacol & Expt Therapeut, Rochester, MN 55905 USA. EM kovtun.irina@mayo.edu; CTMcMurray@lbl.gov FU National Institutes of Health [NS40738, GM 066359, NS062384, CA092584, NS061998] FX The authors wish to acknowledge support from the National Institutes of Health NS40738 (to CTM), GM 066359 (to CTM), NS062384 (to CTM), CA092584 (to CTM), and NS061998 (to IVK). NR 41 TC 25 Z9 25 U1 1 U2 3 PU IMPACT JOURNALS LLC PI ALBANY PA 6211 TIPTON HOUSE, STE 6, ALBANY, NY 12203 USA SN 1945-4589 J9 AGING-US JI Aging-US PD MAY PY 2011 VL 3 IS 5 BP 509 EP 514 PG 6 WC Cell Biology SC Cell Biology GA 774CP UT WOS:000291359200008 PM 21566259 ER PT J AU McNamara, LK Brunzelle, JS Schavocky, JP Watterson, DM Grum-Tokars, V AF McNamara, Laurie K. Brunzelle, Joseph S. Schavocky, James P. Watterson, D. Martin Grum-Tokars, Valerie TI Site-directed mutagenesis of the glycine-rich loop of death associated protein kinase (DAPK) identifies it as a key structure for catalytic activity SO BIOCHIMICA ET BIOPHYSICA ACTA-MOLECULAR CELL RESEARCH LA English DT Article DE Death associated protein kinase; Calmodulin; Glycine-rich region; Neurodegeneration; Central nervous system; Phosphorylation; Protein kinase inhibitor ID ATP-BINDING-SITE; TUMOR SUPPRESSION; APOPTOSIS; ISCHEMIA; INJURY; MODEL AB Death associated protein kinase (DAPK) is a calmodulin (CaM)-regulated protein kinase that is a therapeutic target for central nervous system (CNS) disorders. We report here the results of studies that test the hypothesis of McNamara et al. (2009) that conformational selection in DAPK's glycine-rich region is key for catalytic activity. The hypothesis was tested by site-directed mutagenesis of glutamine-23 (Q23) in the middle of this loop. The glycine-rich loop exhibits localized differences in structure among DAPK conformations that correlate with different stages of the catalytic cycle. Changing the Q23 to a Valine (V23), found at the corresponding position in another CaM regulated protein kinase, results in a reduced catalytic efficiency. High resolution X-ray crystal structures of various conformations of the Q23V mutant DAPK and their superimposition with the corresponding conformations from wild type catalytic domain reveal localized changes in the glycine-rich region. The effect of the mutation on DAPK catalytic activity and the finding of only localized changes in the DAPK structure provide experimental evidence implicating conformational selection in this domain with activity. This article is part of a Special Issue entitled: 11th European Symposium on Calcium. (C) 2010 Elsevier B.V. All rights reserved. C1 [McNamara, Laurie K.; Schavocky, James P.; Watterson, D. Martin; Grum-Tokars, Valerie] Northwestern Univ, Feinberg Sch Med, Dept Mol Pharmacol & Biol Chem, Chicago, IL 60611 USA. [Brunzelle, Joseph S.] Argonne Natl Lab, Adv Photon Source, Life Sci Collaborat Access Team, Argonne, IL 60439 USA. RP Grum-Tokars, V (reprint author), Northwestern Univ, Feinberg Sch Med, Dept Mol Pharmacol & Biol Chem, Chicago, IL 60611 USA. EM v-tokars@northwestern.edu OI Watterson, Daniel/0000-0001-7605-5866 FU NIA NIH HHS [AG031311, R01 AG031311, R01 AG031311-01A1]; NINDS NIH HHS [NS056051, R01 NS056051, R01 NS056051-01A2] NR 20 TC 1 Z9 1 U1 0 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-4889 J9 BBA-MOL CELL RES JI Biochim. Biophys. Acta-Mol. Cell Res. PD MAY PY 2011 VL 1813 IS 5 BP 1068 EP 1073 DI 10.1016/j.bbamcr.2010.11.011 PG 6 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA 770YV UT WOS:000291125300043 PM 21126544 ER PT J AU Qian, F He, Z Thelen, MP Li, Y AF Qian, Fang He, Zhen Thelen, Michael P. Li, Yat TI A microfluidic microbial fuel cell fabricated by soft lithography SO BIORESOURCE TECHNOLOGY LA English DT Article DE Microliter-scale; Shewanella oneidensis MR-1; Polydimethylsiloxane; Power density ID ELECTRICITY-GENERATION; ELECTRON-TRANSFER; POWER-DENSITY; SHEWANELLA; CHAMBER; MR-1; IMPROVEMENT AB Here we report a new microfluidic microbial fuel cell (MFC) platform built by soft-lithography techniques. The MFC design includes a unique sub-5 mu L polydimethylsiloxane soft chamber featuring carbon cloth electrodes and microfluidic delivery of electrolytes. Bioelectricity was generated using Shewanella oneidensis MR-1 cultivated on either complex organic substrates or lactate-based minimal medium. These micro-MFCs exhibited fast start-ups, reproducible current generation, and enhanced power densities up to 62.5 W m(-3) that represents the best result for sub-100 mu L MFCs. Systematic comparisons of custom-made MFC reactors having different chamber sizes indicate volumetric power density is inversely correlated with chamber size in our systems: i.e., the smaller the chamber, the higher the power density is achieved. Published by Elsevier Ltd. C1 [Qian, Fang; Li, Yat] Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. [Qian, Fang; Thelen, Michael P.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94551 USA. [He, Zhen] Univ Wisconsin, Dept Civil Engn & Mech, Milwaukee, WI 53211 USA. RP Qian, F (reprint author), Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. EM fqian@lifesci.ucsb.edu; yli@chemis-try.ucsc.edu RI Thelen, Michael/C-6834-2008; He, Zhen/D-1275-2009; Zong, Xu/B-7149-2013; Thelen, Michael/G-2032-2014; OI Thelen, Michael/0000-0002-2479-5480; He, Zhen/0000-0001-6302-6556; Thelen, Michael/0000-0002-2479-5480; Li, Yat/0000-0002-8058-2084 FU NSF [CBET 1034222]; UCSC; LDRD [11-LW-054]; US. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We thank Prof. Daniel E. Morse for discussion and offering part of the fabrication facilities. We thank Jim Velzy for assistance in cell incubation and Ningning Feng for help in silicon mold design and fabrication. YL acknowledges the financial support in part from the NSF (CBET 1034222) and the UCSC new faculty startup fund. FQ and MPT acknowledge support from LDRD Project 11-LW-054, performed under the auspices of the US. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 32 TC 51 Z9 52 U1 5 U2 52 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD MAY PY 2011 VL 102 IS 10 BP 5836 EP 5840 DI 10.1016/j.biortech.2011.02.095 PG 5 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA 770ZA UT WOS:000291125800039 PM 21421307 ER PT J AU Park, JI Kent, MS Datta, S Holmes, BM Huang, ZH Simmons, BA Sale, KL Sapra, R AF Park, Joshua I. Kent, Michael S. Datta, Supratim Holmes, Bradley M. Huang, Zhaohua Simmons, Blake A. Sale, Kenneth L. Sapra, Rajat TI Enzymatic hydrolysis of cellulose by the cellobiohydrolase domain of CelB from the hyperthermophilic bacterium Caldicellulosiruptor saccharolyticus SO BIORESOURCE TECHNOLOGY LA English DT Article DE Caldicellulosiruptor saccharolyticus; Cellulase; Cellobiohydrolase; Carbohydrate binding module; Hyperthermophile ID THERMOPHILE CALDOCELLUM-SACCHAROLYTICUM; CARBOHYDRATE-BINDING MODULES; GLYCOSIDE HYDROLASES; BIOMASS; MULTIDOMAIN AB The celB gene of Caldicellulosiruptor saccharolyticus was cloned and expressed in Escherichia coli to create a recombinant biocatalyst for hydrolyzing lignocellulosic biomass at high temperature. The GH5 domain of CelB hydrolyzed 4-nitrophenyl-beta-D-cellobioside and carboxymethyl cellulose with optimum activity at pH 4.7-5.5 and 80 degrees C. The recombinant GH5 and CBM3-GH5 constructs were both stable at 80 degrees C with half-lives of 23 h and 39 h, respectively, and retained > 94% activity after 48 h at 70 degrees C. Enzymatic hydrolysis of corn stover and cellulose pretreated with the ionic liquid 1-ethyl-3-methylimidazolium acetate showed that GH5 and CBM3-GH5 primarily produce cellobiose, with product yields for CBM3-GH5 being 1.2- to 2-fold higher than those for GH5. Confocal microscopy of bound protein on cellulose confirmed tighter binding of CBM3-GH5 to cellulose than GH5, indicating that the enhancement of enzymatic activity on solid substrates may be due to the substrate binding activity of CBM3 domain. Published by Elsevier Ltd. C1 [Park, Joshua I.; Kent, Michael S.; Datta, Supratim; Holmes, Bradley M.; Simmons, Blake A.; Sale, Kenneth L.; Sapra, Rajat] Joint BioEnergy Inst, Deconstruct Div, Emeryville, CA 94608 USA. [Park, Joshua I.; Datta, Supratim; Holmes, Bradley M.; Simmons, Blake A.; Sapra, Rajat] Sandia Natl Labs, Dept Biomass Sci & Convers Technol, Livermore, CA 94551 USA. [Sale, Kenneth L.] Sandia Natl Labs, Biosyst R&D Dept, Livermore, CA 94551 USA. [Kent, Michael S.] Sandia Natl Labs, Albuquerque, NM 87123 USA. [Huang, Zhaohua] Univ Calif San Francisco, Dept Bioengn, San Francisco, CA 94143 USA. [Huang, Zhaohua] Univ Calif San Francisco, Dept Therapeut Sci, San Francisco, CA 94143 USA. [Huang, Zhaohua] Univ Calif San Francisco, Dept Pharmaceut Chem, San Francisco, CA 94143 USA. RP Sapra, R (reprint author), 5885 Hollis St,4th Floor, Emeryville, CA 94608 USA. EM rajatsapra@gmail.com OI Simmons, Blake/0000-0002-1332-1810 FU Office of Science, Office of Biological and Environmental Research, of the US Department of Energy [DE-AC02-05CH11231] FX We thank Professor Bruce Dale at Michigan State University for providing corn stover, Professor Francis C. Szoka Jr., at the University of California, San Francisco for DSC, and Sophia S. Evans for technical assistance. This work conducted by the Joint BioEnergy Institute was supported by the Office of Science, Office of Biological and Environmental Research, of the US Department of Energy under Contract No, DE-AC02-05CH11231. NR 25 TC 16 Z9 18 U1 0 U2 13 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 EI 1873-2976 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD MAY PY 2011 VL 102 IS 10 BP 5988 EP 5994 DI 10.1016/j.biortech.2011.02.036 PG 7 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA 770ZA UT WOS:000291125800060 PM 21421309 ER PT J AU Pa, A Bi, XTT Sokhansanj, S AF Pa, Ann Bi, Xiaotao T. Sokhansanj, Shahab TI A life cycle evaluation of wood pellet gasification for district heating in British Columbia SO BIORESOURCE TECHNOLOGY LA English DT Article DE Life cycle analysis (LCA); Wood pellets; British Columbia; District heating; Gasification ID COMBUSTION; EMISSIONS; PARTICLES AB The replacement of natural gas combustion for district heating by wood waste and wood pellets gasification systems with or without emission control has been investigated by a streamlined LCA. While stack emissions from controlled gasification systems are lower than the applicable regulations, compared to the current base case, 12% and 133% increases are expected in the overall human health impacts for wood pellets and wood waste, respectively. With controlled gasification, external costs and GHG emission can be reduced by 35% and 82% on average, respectively. Between wood pellets and wood waste, wood pellets appear to be the better choice as it requires less primary energy and has a much lower impact on the local air quality. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Pa, Ann; Bi, Xiaotao T.; Sokhansanj, Shahab] Univ British Columbia, Clean Energy Res Ctr, Vancouver, BC V6T 1Z3, Canada. [Sokhansanj, Shahab] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Bi, XTT (reprint author), Univ British Columbia, Clean Energy Res Ctr, 2360 East Mall, Vancouver, BC V6T 1Z3, Canada. EM xbi@chbe.ubc.ca FU Agriculture Canada; UBC FX The authors would like to thank UBC Sustainability office, UBC Utility, and Dr. Anthony Lau for providing the air emission data for the existing natural gas district heating facility. The authors are also grateful to the financial support from Agriculture Canada's ABIN program and the UBC Graduate Fellowship (UGF) program. NR 49 TC 24 Z9 25 U1 1 U2 16 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD MAY PY 2011 VL 102 IS 10 BP 6167 EP 6177 DI 10.1016/j.biortech.2011.02.009 PG 11 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA 770ZA UT WOS:000291125800084 PM 21377867 ER PT J AU Lei, HW Ren, SJ Wang, L Bu, Q Julson, J Holladay, J Ruan, R AF Lei, Hanwu Ren, Shoujie Wang, Lu Bu, Quan Julson, James Holladay, John Ruan, Roger TI Microwave pyrolysis of distillers dried grain with solubles (DDGS) for biofuel production SO BIORESOURCE TECHNOLOGY LA English DT Article DE Microwave pyrolysis; DDGS; Hydrocarbon; GC/MS ID BIOMASS; CORN; TEMPERATURE; ETHANOL; ENERGY; OIL AB Microwave pyrolysis of distillers dried grain with solubles (DDGS) was investigated to determine the effects of pyrolytic conditions on the yields of bio-oil, syngas, and biochar. Pyrolysis process variables included reaction temperature, time, and power input. Microwave pyrolysis of DOGS was analyzed using response surface methodology to find out the effect of process variables on the biofuel (bio-oil and syngas) conversion yield and establish prediction models. Bio-oil recovery was in the range of 26.5-50.3 wt.% of the biomass. Biochar yields were 23.5-62.2% depending on the pyrolysis conditions. The energy content of DOGS bio-oils was 28 MJ/kg obtained at the 650 degrees C and 8 min, which was about 66.7% of the heating value of gasoline. GC/MS analysis indicated that the biooil contained a series of important and useful chemical compounds: aliphatic and aromatic hydrocarbons. At least 13% of DOGS bio-oil was the same hydrocarbon compounds found in regular unleaded gasoline. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Lei, Hanwu; Ren, Shoujie; Wang, Lu; Bu, Quan] Washington State Univ, Dept Biol Syst Engn, Sci & Engn Lab, Richland, WA 99354 USA. [Julson, James] S Dakota State Univ, Dept Agr & Biol Engn, Brookings, SD 57006 USA. [Holladay, John] Pacific NW Natl Lab, Richland, WA 99354 USA. [Ruan, Roger] Univ Minnesota, Dept Bioprod & Biosyst Engn, St Paul, MN 55108 USA. RP Lei, HW (reprint author), Washington State Univ, Dept Biol Syst Engn, Sci & Engn Lab, Richland, WA 99354 USA. EM hlei@tricity.wsu.edu RI ren, shoujie/P-1384-2014; OI Ruan, Roger/0000-0001-8835-2649 FU South Dakota Corn Utilization Council; US USDA/Sun Grant Initiative FX This work was supported in part by grants from the South Dakota Corn Utilization Council, and US USDA/Sun Grant Initiative. The authors also wish to thank Dr. Linhong Jing from SDSU Core Campus Mass Spectrometry Facility. NR 33 TC 34 Z9 35 U1 2 U2 28 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD MAY PY 2011 VL 102 IS 10 BP 6208 EP 6213 DI 10.1016/j.biortech.2011.02.050 PG 6 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA 770ZA UT WOS:000291125800089 PM 21377870 ER PT J AU Wang, SZ Bianco, R Hynes, JT AF Wang, Shuzhi Bianco, Roberto Hynes, James T. TI An atmospherically relevant acid: HNO3 SO COMPUTATIONAL AND THEORETICAL CHEMISTRY LA English DT Article DE Nitric acid; Proton transfer; Hydrogen bonds; Heterogeneous reactions; Atmospheric chemistry ID INITIO MOLECULAR-DYNAMICS; SUM-FREQUENCY GENERATION; MODEL AQUEOUS SURFACE; DENSITY-FUNCTIONAL THEORY; PROTON-TRANSFER REACTIONS; FREE-ENERGY RELATIONS; AB-INITIO; NITRIC-ACID; WATER CLUSTERS; SULFURIC-ACID AB Here we briefly review our theoretical work on nitric acid dissociation at an aqueous interface, an issue important in a wide range of atmospheric contexts, employing both quantum chemical methods and Car-Parrinello molecular dynamics simulations. A first aspect concerns whether or not this dissociation, via proton transfer to a neighboring water molecule, occurs as a function of the acid's location atop and at various depths below the surface. Further aspects concern the molecular level details of the mechanism, i.e. which motions are important, of the first proton transfer to form a contact ion pair, and of the subsequent proton transfer to produce a solvent-separated ion pair from that contact ion pair. (C) 2011 Elsevier B.V. All rights reserved. C1 [Wang, Shuzhi; Bianco, Roberto; Hynes, James T.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Hynes, James T.] Ecole Normale Super, Dept Chem, F-75005 Paris, France. [Hynes, James T.] CNRS UMR Pasteur, Paris, France. RP Wang, SZ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, MS 66,1 Cyclotron Rd, Berkeley, CA 94720 USA. EM swang2@lbl.gov; Roberto.Bianco@Colorado.EDU; James.Hynes@Colorado.EDU FU NSF [CHE-0417570, CHE-0750477]; National Center for Supercomputing Applications [TG-CHE070039, TG-CHE070033N]; ANR [NT05-4-43154] FX This work was supported in part by NSF Grants CHE-0417570 and CHE-0750477 and by the National Center for Supercomputing Applications under TG-CHE070039 and TG-CHE070033N and utilized the systems TUNGSTEN and ABE. J.T.H. also acknowledges support via an ANR Grant (NT05-4-43154). NR 100 TC 12 Z9 12 U1 2 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2210-271X EI 1872-7999 J9 COMPUT THEOR CHEM JI Comput. Theor. Chem. PD MAY PY 2011 VL 965 IS 2-3 SI SI BP 340 EP 345 DI 10.1016/j.comptc.2011.01.027 PG 6 WC Chemistry, Physical SC Chemistry GA 773RI UT WOS:000291326400014 ER PT J AU Gonzalez-Delgado, AM Shukla, MK Ulery, AL Bawazir, AS Brady, PV AF Gonzalez-Delgado, Amir M. Shukla, Manoj K. Ulery, April L. Bawazir, A. Salim Brady, Patrick V. TI Saturated hydraulic conductivity of self-sealing lining materials for desalination evaporation ponds SO DESALINATION AND WATER TREATMENT LA English DT Article DE Saturated hydraulic conductivity; Bulk density; Lining material; Electrical conductivity; X-ray diffraction; Evaporation pond ID TRANSPORT; JAROSITE; CLAY AB Evaporation ponds are used in the disposal of saline waste produced by desalination plants. An increase in concentration of saline wastewater by evaporation reduces the resistance of clay-based lining material commonly used in evaporation ponds and increases the risk of groundwater pollution. Self-sealing lining materials can add resistance to the lining system against advective flow through their capacity of reacting with the saline waste, unlike other liners. The objectives of this research were to quantify the effect of electrical conductivity (EC) of solution, duration of ponding of solution, bulk density of lining material and porous media, and wet-dry cycles on the saturated hydraulic conductivity (K(s)) of porous media through laboratory experiments. The Alamogordo variant very fine sandy loam (Tularosa soil) and #1 dry-silica sand/SIL-CO-SIL 125-silica (synthetic soil) were the two soils used in this study. Sodium silicate, calcium hydroxide and magnesium hydroxide, were the lining materials used in this study because of their expected ability to form transport-limiting solids. The lining materials were packed as either a homogenized mixture of 5-10 g of lining material and 60 g of soil or as layering the lining material between 50 and 10 g of soil. A stock solution of 0.25 M of calcium chloride, magnesium chloride, sodium carbonate and sodium sulfate was diluted using DI water to prepare different solutions of EC 30, 20, 10, 5 and 2 dS/m. The K(s) was determined by the constant head method in each soil column for different EC-solutions. Mostly, the layer of lining material produced lower K(s) of porous media than the homogenized mixture. The K(s) decreased with increasing EC, duration of ponding (1-14 d), and bulk density in columns packed with calcium hydroxide. X-ray diffraction results showed that calcium hydroxide reacted with the saline solution to form precipitates such as calcite and gypsum. The inverse relationship between K(s) bulk density and amount of lining material showed that in order to achieve the EPA-recommended K(s), the porous media including the layer of lining material must be compacted to higher bulk density using greater amounts of lining material. This study demonstrated that calcium hydroxide could be used as a lining material with self-sealing capacity for desalination evaporation ponds. C1 [Gonzalez-Delgado, Amir M.; Shukla, Manoj K.; Ulery, April L.] New Mexico State Univ, Plant & Environm Sci Dept, Las Cruces, NM 88003 USA. [Bawazir, A. Salim] New Mexico State Univ, Civil & Geol Engn Dept, Las Cruces, NM 88003 USA. [Brady, Patrick V.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Gonzalez-Delgado, AM (reprint author), New Mexico State Univ, Plant & Environm Sci Dept, MSC-3Q,POB 30003, Las Cruces, NM 88003 USA. EM amgonz4@nmsu.edu FU Sandia University FX Authors thank New Mexico State University Agricultural Experiment Station, Las Cruces, NM, USA for the support. Authors also thank Dr. H. Curtis Monger and Dr. Peter Cooke from New Mexico State University for help in conducting XRD and SEM analyses. We also thank Dr. David Smith for useful suggestions and Ms. Amy Smith for editorial assistance. This study was partially funded by Sandia University Research Partnership (SURP). NR 24 TC 1 Z9 1 U1 3 U2 14 PU DESALINATION PUBL PI HOPKINTON PA 36 WALCOTT VALLEY DRIVE,, HOPKINTON, MA 01748 USA SN 1944-3994 J9 DESALIN WATER TREAT JI Desalin. Water Treat. PD MAY PY 2011 VL 29 IS 1-3 BP 187 EP 195 DI 10.5004/dwt.2011.2024 PG 9 WC Engineering, Chemical; Water Resources SC Engineering; Water Resources GA 773NQ UT WOS:000291314400022 ER EF