FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Halverson, JD Lee, WB Grest, GS Grosberg, AY Kremer, K AF Halverson, Jonathan D. Lee, Won Bo Grest, Gary S. Grosberg, Alexander Y. Kremer, Kurt TI Molecular dynamics simulation study of nonconcatenated ring polymers in a melt. I. Statics SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID ARM STAR POLYMERS; CHROMOSOME TERRITORIES; TOPOLOGICAL CONSTRAINTS; COMPUTER-SIMULATION; ENTANGLEMENT LENGTH; CYCLIC POLYSTYRENE; FIXED OBSTACLES; MODEL; CHAIN; CONFORMATION AB Molecular dynamics simulations were conducted to investigate the structural properties of melts of nonconcatenated ring polymers and compared to melts of linear polymers. The longest rings were composed of N = 1600 monomers per chain which corresponds to roughly 57 entanglement lengths for comparable linear polymers. For the rings, the radius of gyration squared, < R-g(2)>, was found to scale as N-4/5 for an intermediate regime and N-2/3 for the larger rings indicating an overall conformation of a crumpled globule. However, almost all beads of the rings are "surface beads" interacting with beads of other rings, a result also in agreement with a primitive path analysis performed in the next paper [J. D. Halverson, W. Lee, G. S. Grest, A. Y. Grosberg, and K. Kremer, J. Chem. Phys. 134, 204905 (2011)]. Details of the internal conformational properties of the ring and linear polymers as well as their packing are analyzed and compared to current theoretical models. (C) 2011 American Institute of Physics. [doi:10.1063/1.3587137] C1 [Halverson, Jonathan D.; Lee, Won Bo; Kremer, Kurt] Max Planck Inst Polymer Res, D-55128 Mainz, Germany. [Lee, Won Bo] Sogang Univ, Dept Chem & Biomol Engn, Seoul, South Korea. [Grest, Gary S.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Grosberg, Alexander Y.] NYU, Dept Phys, New York, NY 10003 USA. RP Kremer, K (reprint author), Max Planck Inst Polymer Res, Ackermannweg 10, D-55128 Mainz, Germany. EM kremer@mpip-mainz.mpg.de RI Kremer, Kurt/G-5652-2011; MPIP, Theory/I-9884-2014; Grosberg, Alexander/O-2122-2015; OI Grosberg, Alexander/0000-0002-4230-8690; Lee, Won Bo/0000-0001-7801-083X FU Alexander von Humboldt Foundation; Ministry of Education, Science and Technology [2010-0007886]; Multiscale Materials Modeling (MMM) initiative of the Max Planck Society; Sandia National Laboratories; United States Department of Energy [DE-AC04-94AL85000] FX The authors are grateful to T. Vilgis, T. Vettorel, and V. Harmandaris for their comments on an early version of the manuscript. The ESPResSo development team is acknowledged for optimizing the simulation software on the IBM Blue Gene/P at the Rechenzentrum Garching in Munich, Germany. We thank Donghui Zhang for discussions and references relating to experimental studies on cyclic polymers. This project was in part funded by the Alexander von Humboldt Foundation through a research grant awarded to A.Y.G. A.Y.G. also acknowledges the hospitality of the Aspen Center for Physics where part of this work was done. W. B. L. acknowledges financial support from the Alexander von Humboldt Foundation and the Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science and Technology (2010-0007886). Additional funding was provided by the Multiscale Materials Modeling (MMM) initiative of the Max Planck Society. We thank the New Mexico Computing Application Center (NMCAC) for a generous allocation of computer time. This work is supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract No. DE-AC04-94AL85000. NR 77 TC 91 Z9 92 U1 6 U2 53 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 28 PY 2011 VL 134 IS 20 AR 204904 DI 10.1063/1.3587137 PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 770SD UT WOS:000291107900063 PM 21639474 ER PT J AU Meredith, NP Horne, RB Lam, MM Denton, MH Borovsky, JE Green, JC AF Meredith, Nigel P. Horne, Richard B. Lam, Mai Mai Denton, Michael H. Borovsky, Joseph E. Green, Janet C. TI Energetic electron precipitation during high-speed solar wind stream driven storms SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article ID COROTATING INTERACTION REGIONS; RECURRENT GEOMAGNETIC STORMS; OUTER RADIATION BELT; MAGNETIC STORMS; RELATIVISTIC ELECTRONS; PARTICLE-PRECIPITATION; PLASMASPHERIC HISS; CHORUS EMISSIONS; PLASMA SHEET; ACCELERATION AB Electron precipitation from the Earth's inner magnetosphere transmits solar variability to the Earth's upper atmosphere and may affect surface level climate. Here we conduct a superposed epoch analysis of energetic electrons observed by the NOAA POES spacecraft during 42 high-speed solar wind stream (HSS) driven geomagnetic storms to determine the temporal evolution and global distribution of the precipitating flux. The flux of trapped and precipitating E > 30 keV electrons increases immediately following storm onset and remains elevated during the passage of the HSS. In contrast, the trapped and precipitating relativistic electrons (E > 1 MeV) drop out following storm onset and subsequently increase during the recovery phase to levels which eventually exceed the prestorm levels. There is no evidence for enhanced precipitation of relativistic electrons during the MeV flux drop out, suggesting that flux drop outs during the main phase of HSS-driven storms are not due to precipitation to the atmosphere. On average, the flux of precipitating E > 30 keV electrons is enhanced by a factor of similar to 10 during the passage of the high-speed stream at all geographic longitudes. In contrast, the precipitating relativistic electron count rate is observed to peak in the region poleward of the South Atlantic Anomaly. During the passage of the high-speed stream, the flux of precipitating E > 30 keV electrons peaks in the region from 2100 to 1200 magnetic local time at low L (4 < L < 7) and in the prenoon sector at high L (7 < L < 9), suggesting that chorus waves are responsible for the precipitation of E > 30 keV electrons in both regions. C1 [Meredith, Nigel P.; Horne, Richard B.] British Antarctic Survey, NERC, Cambridge CB3 0ET, England. [Lam, Mai Mai] Univ Leicester, Dept Phys & Astron, Leicester LE1 7RH, Leics, England. [Denton, Michael H.] Univ Lancaster, Dept Phys, Lancaster LA1 4YW, England. [Borovsky, Joseph E.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Green, Janet C.] NOAA, Space Weather Predict Ctr, Boulder, CO 80305 USA. RP Meredith, NP (reprint author), British Antarctic Survey, NERC, Madingley Rd, Cambridge CB3 0ET, England. EM nmer@bas.ac.uk; r.horne@bas.ac.uk; mml9@ion.le.ac.uk; m.denton@lancaster.ac.uk; jborovsky@lanl.gov; janet.green@noaa.gov OI Horne, Richard/0000-0002-0412-6407; Meredith, Nigel/0000-0001-5032-3463; Denton, Michael/0000-0002-1748-3710 FU Natural Environment Research Council; STFC [ST/G002401/1/] FX We thank the NSSDC Omniweb for providing the geomagnetic indices and solar wind parameters used in this study. This work was supported, in part, by the Natural Environment Research Council. J.E.B. and M. H. D. would like to thank all at BAS for their hospitality during their visit in Spring 2010. Work at Lancaster was supported by STFC grant ST/G002401/1/. NR 84 TC 53 Z9 53 U1 0 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAY 28 PY 2011 VL 116 AR A05223 DI 10.1029/2010JA016293 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 770RX UT WOS:000291107300004 ER PT J AU Mishra, PK Neuman, SP AF Mishra, Phoolendra Kumar Neuman, Shlomo P. TI Saturated-unsaturated flow to a well with storage in a compressible unconfined aquifer SO WATER RESOURCES RESEARCH LA English DT Article ID HYDRAULIC CONDUCTIVITY; NUMERICAL INVERSION; PARTIAL PENETRATION; LAPLACE TRANSFORMS; DRAINAGE; WATER; MODEL; DIAMETER AB Mishra and Neuman (2010) developed an analytical solution for flow to a partially penetrating well of zero radius in a compressible unconfined aquifer that allows inferring its saturated and unsaturated hydraulic properties from responses recorded in the saturated and/or unsaturated zones. Their solution accounts for horizontal as well as vertical flows in each zone. It represents unsaturated zone constitutive properties in a manner that is at once mathematically tractable and sufficiently flexible to provide much improved fits to standard constitutive models. In this paper we extend the solution of Mishra and Neuman [2010] to the case of a finite diameter pumping well with storage; investigate the effects of storage in the pumping well and delayed piezometer response on drawdowns in the saturated and unsaturated zones as functions of position and time; validate our solution against numerical simulations of drawdown in a synthetic aquifer having unsaturated properties described by the van Genuchten [1980]-Mualem [1976] model; use our solution to analyze 11 transducer-measured drawdown records from a seven-day pumping test conducted by University of Waterloo researchers at the Canadian Forces Base Borden in Ontario, Canada; validate our parameter estimates against manually-measured drawdown records in 14 other piezometers at Borden; and compare (a) our estimates of aquifer parameters with those obtained on the basis of all these records by Moench [2008], (b) on the basis of 11 transducer-measured drawdown records by Endres et al. [2007], (c) our estimates of van Genuchten-Mualem parameters with those obtained on the basis of laboratory drainage data from the site by Akindunni and Gillham [1992], and (d) our corresponding prediction of how effective saturation varies with elevation above the initial water table under static conditions with a profile based on water contents measured in a neutron access tube at a radial distance of about 5 m from the center of the pumping well. We also use our solution to analyze 11 transducer-measured drawdown records from a 7 day pumping test conducted by University of Waterloo researchers at the Canadian Forces Base Borden in Ontario, Canada. We validate our parameter estimates against manually measured drawdown records in 14 other piezometers at Borden. We compare our estimates of aquifer parameters with those obtained on the basis of all these records by Moench (2008) and on the basis of 11 transducer-measured drawdown records by Endres et al. (2007), and we compare our estimates of van Genuchten-Mualem parameters with those obtained on the basis of laboratory drainage data from the site by Akindunni and Gillham (1992); finally, we compare our corresponding prediction of how effective saturation varies with elevation above the initial water table under static conditions with a profile based on water contents measured in a neutron access tube at a radial distance of about 5 m from the center of the pumping well. C1 [Mishra, Phoolendra Kumar; Neuman, Shlomo P.] Univ Arizona, Dept Hydrol & Water Resources, Tucson, AZ 85721 USA. RP Mishra, PK (reprint author), Los Alamos Natl Lab, Hydrol Geochem & Geol Grp, MS T003, Los Alamos, NM 87545 USA. EM neuman@hwr.arizona.edu RI Mishra, Phoolendra/A-1927-2012 FU Vanderbilt University under the Consortium of Risk Evaluation with Stakeholder Participation (CRESP) III; U.S. Department of Energy FX This research was supported in part through a contract with Vanderbilt University under the Consortium of Risk Evaluation with Stakeholder Participation (CRESP) III, funded by the U.S. Department of Energy. NR 29 TC 15 Z9 15 U1 2 U2 17 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 J9 WATER RESOUR RES JI Water Resour. Res. PD MAY 28 PY 2011 VL 47 AR W05553 DI 10.1029/2010WR010177 PG 15 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA 770TJ UT WOS:000291111100017 ER PT J AU Pindzola, MS Ludlow, JA Ballance, CP Robicheaux, F Colgan, J AF Pindzola, M. S. Ludlow, J. A. Ballance, C. P. Robicheaux, F. Colgan, J. TI Electron-impact double ionization of B+ SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article ID CROSS-SECTIONS; HELIUM; IONS AB Time-dependent close-coupling and time-independent distorted-wave methods are used to calculate the electron-impact double-ionization cross section for the 1s(2)2s(2) ground configuration of the B+ atomic ion. The direct double-ionization cross section is calculated using the non-perturbative close-coupling method between the direct double-ionization threshold of 63.1 eV and the 1s ionization threshold of 218.4 eV. The indirect single ionization-autoionization cross section is calculated using the perturbative distorted-wave method between the 1s ionization threshold of 218.4 and 750 eV. The double-ionization cross section calculated using the two methods is compared with a crossed-beam experiment over the entire energy range. C1 [Pindzola, M. S.; Ludlow, J. A.; Ballance, C. P.; Robicheaux, F.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Colgan, J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. RP Pindzola, MS (reprint author), Auburn Univ, Dept Phys, Auburn, AL 36849 USA. RI Robicheaux, Francis/F-4343-2014; OI Robicheaux, Francis/0000-0002-8054-6040; Colgan, James/0000-0003-1045-3858 FU US Department of Energy; US National Science Foundation FX We would like to thank Professor Alfred Muller of the University of Giessen for sending us the experimental data for the electron-impact double ionization of B+. This work was supported in part by grants from the US Department of Energy and the US National Science Foundation. Computational work was carried out at the National Energy Research Scientific Computing Center in Oakland, CA, and at the National Institute for Computational Sciences in Oak Ridge, TN. NR 12 TC 9 Z9 9 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD MAY 28 PY 2011 VL 44 IS 10 AR 105202 DI 10.1088/0953-4075/44/10/105202 PG 4 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 762DQ UT WOS:000290452900013 ER PT J AU Keeling, RF Manning, AC Dubey, MK AF Keeling, Ralph F. Manning, Andrew C. Dubey, Manvendra K. TI The atmospheric signature of carbon capture and storage SO PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES LA English DT Article DE carbon capture and storage; geosequestration; leak detection; atmospheric oxygen; carbon-13; carbon-14 ID GENERAL-CIRCULATION MODEL; BOX-DIFFUSION; CO2; DIOXIDE; OXYGEN; SINKS; O-2; VERIFICATION; GAS; AIR AB Compared with other industrial processes, carbon capture and storage (CCS) will have an unusual impact on atmospheric composition by reducing the CO2 released from fossil-fuel combustion plants, but not reducing the associated O-2 loss. CO2 that leaks into the air from below-ground CCS sites will also be unusual in lacking the O-2 deficit normally associated with typical land CO2 sources, such as from combustion or ecosystem exchanges. CCS may also produce distinct isotopic changes in atmospheric CO2. Using simple models and calculations, we estimate the impact of CCS or leakage on regional atmospheric composition. We also estimate the possible impact on global atmospheric composition, assuming that the technology is widely adopted. Because of its unique signature, CCS may be especially amenable to monitoring, both regionally and globally, using atmospheric observing systems. Measurements of the O-2/N-2 ratio and the CO2 concentration in the proximity of a CCS site may allow detection of point leaks of the order of 1000 ton CO2 yr(-1) from a CCS reservoir up to 1km from the source. Measurements of O-2/N-2 and CO2 in background air from a global network may allow quantification of global and hemispheric capture rates from CCS to the order of +/- 0.4 PgCyr(-1). C1 [Keeling, Ralph F.] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA. [Manning, Andrew C.] Univ E Anglia, Sch Environm Sci, Norwich NR4 7TJ, Norfolk, England. [Dubey, Manvendra K.] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. RP Keeling, RF (reprint author), Univ Calif San Diego, Scripps Inst Oceanog, 9500 Gilman Dr, La Jolla, CA 92093 USA. EM rkeeling@ucsd.edu RI Dubey, Manvendra/E-3949-2010; Manning, Andrew/D-4416-2011 OI Dubey, Manvendra/0000-0002-3492-790X; Manning, Andrew/0000-0001-6952-7773 FU UK NERC/QUEST [NE/C002504/1]; US NSF [ATM-0632770, ATM-0651834]; DoE [DE-FG02-07ER64362]; NOAA [2007-2000636] FX We thank David Bowling (University of Utah) and Elena Kozlova (University of East Anglia) for providing data shown in figures 2 and 3, respectively. We thank David Etheridge for providing access to the Otway modelling results and other helpful comments. A. C. M. is supported by a UK NERC/QUEST Advanced Fellowship (ref. no. NE/C002504/1). R. F. K. has been supported under grants from the US NSF (ATM-0632770, ATM-0651834), DoE (DE-FG02-07ER64362) and NOAA (2007-2000636). M. K. D. thanks LANL's Laboratory Directed Research and Development Program for nurturing his work in direct air capture of CO2 and CCS. NR 47 TC 10 Z9 10 U1 0 U2 26 PU ROYAL SOC PI LONDON PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND SN 1364-503X EI 1471-2962 J9 PHILOS T R SOC A JI Philos. Trans. R. Soc. A-Math. Phys. Eng. Sci. PD MAY 28 PY 2011 VL 369 IS 1943 BP 2113 EP 2132 DI 10.1098/rsta.2011.0016 PG 20 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 751LK UT WOS:000289619100016 PM 21502179 ER PT J AU Avci, S Chmaissem, O Goremychkin, EA Rosenkranz, S Castellan, JP Chung, DY Todorov, IS Schlueter, JA Claus, H Kanatzidis, MG Daoud-Aladine, A Khalyavin, D Osborn, R AF Avci, S. Chmaissem, O. Goremychkin, E. A. Rosenkranz, S. Castellan, J-P. Chung, D. Y. Todorov, I. S. Schlueter, J. A. Claus, H. Kanatzidis, M. G. Daoud-Aladine, A. Khalyavin, D. Osborn, R. TI Magnetoelastic coupling in the phase diagram of Ba1-xKxFe2As2 as seen via neutron diffraction SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC ORDER; SUPERCONDUCTIVITY; COEXISTENCE AB We report a high resolution neutron diffraction investigation of the coupling of structural and magnetic transitions in Ba1-xKxFe2As2. The tetragonal-orthorhombic and antiferromagnetic transitions are suppressed with potassium doping, falling to zero at x less than or similar to 0.24. However, unlike Ba(Fe1-xCox)(2)As-2, the two transitions are first order and coincident over the entire phase diagram, with a biquadratic coupling of the two order parameters. The phase diagram is refined showing that the onset of superconductivity is at x = 0.133 with all three phases coexisting until x <= 0.24. C1 [Avci, S.; Chmaissem, O.; Goremychkin, E. A.; Rosenkranz, S.; Castellan, J-P.; Chung, D. Y.; Todorov, I. S.; Schlueter, J. A.; Claus, H.; Kanatzidis, M. G.; Osborn, R.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Chmaissem, O.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Kanatzidis, M. G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Daoud-Aladine, A.; Khalyavin, D.] Rutherford Appleton Lab, ISIS Pulsed Neutron & Muon Facil, Didcot OX11 0QX, Oxon, England. RP Avci, S (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RI Osborn, Raymond/E-8676-2011; Rosenkranz, Stephan/E-4672-2011; Khalyavin, Dmitry/E-4335-2017 OI Osborn, Raymond/0000-0001-9565-3140; Rosenkranz, Stephan/0000-0002-5659-0383; Khalyavin, Dmitry/0000-0002-6724-7695 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We acknowledge valuable discussions with I. Paul and A. Cano. Work supported by US Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract No. DE-AC02-06CH11357. NR 30 TC 60 Z9 60 U1 1 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 27 PY 2011 VL 83 IS 17 AR 172503 DI 10.1103/PhysRevB.83.172503 PG 4 WC Physics, Condensed Matter SC Physics GA 769LP UT WOS:000291015400002 ER PT J AU Gates, JM Dullmann, CE Schadel, M Yakushev, A Turler, A Eberhardt, K Kratz, JV Ackermann, D Andersson, LL Block, M Bruchle, W Dvorak, J Essel, HG Ellison, PA Even, J Forsberg, U Gellanki, J Gorshkov, A Graeger, R Gregorich, KE Hartmann, W Herzberg, RD Hessberger, FP Hild, D Hubner, A Jager, E Khuyagbaatar, J Kindler, B Krier, J Kurz, N Lahiri, S Liebe, D Lommel, B Maiti, M Nitsche, H Omtvedt, JP Parr, E Rudolph, D Runke, J Schaffner, H Schausten, B Schimpf, E Semchenkov, A Steiner, J Thorle-Pospiech, P Uusitalo, J Wegrzecki, M Wiehl, N AF Gates, J. M. Duellmann, Ch E. Schaedel, M. Yakushev, A. Tuerler, A. Eberhardt, K. Kratz, J. V. Ackermann, D. Andersson, L. -L. Block, M. Bruechle, W. Dvorak, J. Essel, H. G. Ellison, P. A. Even, J. Forsberg, U. Gellanki, J. Gorshkov, A. Graeger, R. Gregorich, K. E. Hartmann, W. Herzberg, R. -D. Hessberger, F. P. Hild, D. Huebner, A. Jaeger, E. Khuyagbaatar, J. Kindler, B. Krier, J. Kurz, N. Lahiri, S. Liebe, D. Lommel, B. Maiti, M. Nitsche, H. Omtvedt, J. P. Parr, E. Rudolph, D. Runke, J. Schaffner, H. Schausten, B. Schimpf, E. Semchenkov, A. Steiner, J. Thoerle-Pospiech, P. Uusitalo, J. Wegrzecki, M. Wiehl, N. TI First superheavy element experiments at the GSI recoil separator TASCA: The production and decay of element 114 in the Pu-244(Ca-48,3-4n) reaction SO PHYSICAL REVIEW C LA English DT Article ID SPONTANEOUS-FISSION DECAY; CROSS-SECTIONS; MASS-DRIFT; NUCLEI; ISOTOPES; HEAVY; SYSTEMATICS; ISOMERS; TARGETS; NO-252 AB Experiments with the new recoil separator, Transactinide Separator and Chemistry Apparatus (TASCA), at the GSI were performed by using beams of Ca-48 to irradiate targets of Pb206-208, which led to the production of No252-254 isotopes. These studies allowed for evaluation of the performance of TASCA when coupled to a new detector and electronics system. By following these studies, the isotopes of element 114 ((288-291)114) were produced in irradiations of Pu-244 targets with Ca-48 beams at compound nucleus excitation energies around 41.7 and 37.5 MeV, demonstrating TASCA's ability to perform experiments with picobarn-level cross sections. A total of 15 decay chains were observed and were assigned to the decay of 288-291114. A new a-decay branch in (281)Ds was observed, leading to the new nucleus (277)Hs. C1 [Gates, J. M.; Duellmann, Ch E.; Schaedel, M.; Ackermann, D.; Block, M.; Bruechle, W.; Essel, H. G.; Hartmann, W.; Hessberger, F. P.; Huebner, A.; Jaeger, E.; Khuyagbaatar, J.; Kindler, B.; Krier, J.; Kurz, N.; Lommel, B.; Schaffner, H.; Schausten, B.; Schimpf, E.; Steiner, J.] GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany. [Gates, J. M.; Yakushev, A.; Tuerler, A.; Gorshkov, A.; Graeger, R.] Tech Univ Munich, D-85748 Garching, Germany. [Gates, J. M.; Dvorak, J.; Ellison, P. A.; Gregorich, K. E.; Nitsche, H.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Duellmann, Ch E.; Eberhardt, K.; Kratz, J. V.; Hild, D.; Liebe, D.; Runke, J.; Thoerle-Pospiech, P.; Wiehl, N.] Johannes Gutenberg Univ Mainz, D-55099 Mainz, Germany. [Duellmann, Ch E.] Helmholtz Inst Mainz, D-55099 Mainz, Germany. [Andersson, L. -L.; Herzberg, R. -D.; Parr, E.] Univ Liverpool, Liverpool L69 7ZE, Merseyside, England. [Forsberg, U.; Gellanki, J.; Rudolph, D.] Lund Univ, SE-22100 Lund, Sweden. [Lahiri, S.; Maiti, M.] Saha Inst Nucl Phys, Kolkata 700064, India. [Omtvedt, J. P.; Semchenkov, A.] Univ Oslo, NO-0315 Oslo, Norway. [Uusitalo, J.] Univ Jyvaskyla, FI-40014 Jyvaskyla, Finland. [Wegrzecki, M.] Inst Electr Mat Technol, PL-02668 Warsaw, Poland. RP Gates, JM (reprint author), GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany. EM jmgates@lbl.gov RI Rudolph, Dirk/D-4259-2009; Herzberg, Rolf-Dietmar/E-1558-2011; Omtvedt, Jon Petter/C-8194-2011; Block, Michael/I-2782-2015; Even, Julia/K-1186-2016; Turler, Andreas/D-3913-2014 OI Rudolph, Dirk/0000-0003-1199-3055; Omtvedt, Jon Petter/0000-0002-1822-7348; Block, Michael/0000-0001-9282-8347; Even, Julia/0000-0002-6314-9094; Turler, Andreas/0000-0002-4274-1056 FU German BMBF [06MT247I, 06MT248, 06MZ223I]; Research Center Elementary Forces and Mathematical Foundations (EMG); Swedish Science Council; U.S. D.O.E [DE-AC02-05CH11231]; NNSA [DE-FC52-08NA28752]; Norwegian Research Council [177538]; Government of India FX We thank the ECR ion source and UNILAC staffs for providing excellent and stable 48Ca beams. H. Brand and the GSI Experimental Electronics Department, H. Grosslhuber, G. Matheis, and R. Buhnemann from the machine shop at the Institute of Radiochemistry, TU Munich as well as V. Gorshkov, who provided technical support. L. Stavsetra provided preliminary BGS results for the 48Ca + 242Pu reaction prior to publication, which we gratefully acknowledge. This work was financially supported by the German BMBF (Grants No. 06MT247I, No. 06MT248, and No. 06MZ223I); the Research Center Elementary Forces and Mathematical Foundations (EMG); the GSI-F& E (MT/TUR, MZJVKR); the Swedish Science Council; the U.S. D.O.E. under Contract No. DE-AC02-05CH11231 and the NNSA under Contract No. DE-FC52-08NA28752; the Norwegian Research Council (Project No. 177538); and the Government of India-XIth 5-year plan project TADDS. NR 59 TC 69 Z9 71 U1 0 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAY 27 PY 2011 VL 83 IS 5 AR 054618 DI 10.1103/PhysRevC.83.054618 PG 17 WC Physics, Nuclear SC Physics GA 769LX UT WOS:000291016300005 ER PT J AU Song, HC Bass, SA Heinz, U AF Song, Huichao Bass, Steffen A. Heinz, Ulrich TI Elliptic flow in root s=200 GeV Au+Au collisions and root s=2.76 TeV Pb+Pb collisions: Insights from viscous hydrodynamics plus hadron cascade hybrid model SO PHYSICAL REVIEW C LA English DT Article ID HEAVY-ION COLLISIONS; QUARK-GLUON PLASMA; PB-PB COLLISIONS; ECCENTRICITY FLUCTUATIONS; NUCLEAR COLLISIONS; SUPPRESSION AB Using the newly developed hybrid model VISHNU, which connects viscous hydrodynamics with a hadron cascade model, we study the differential and integrated elliptic flow v(2) at different centrality bins for 200 A GeV Au + Au collisions and 2.76 A TeV Pb + Pb collisions. We find that the average quark-gluon plasma (QGP)-specific shear viscosity eta/s slightly increases from Relativistic Heavy Ion Collider to Large Hadron Collider (LHC) energies. However, a further study assuming different temperature dependencies for (eta/s)(QGP) shows that one cannot uniquely constrain the form of (eta/s)(QGP) (T) by fitting the spectra and v(2) alone. Based on our current understanding, the question whether the QGP fluid is more viscous or more perfect in the temperature regime reached by LHC energies is still open. C1 [Song, Huichao] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Bass, Steffen A.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Heinz, Ulrich] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. RP Song, HC (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM hsong@lbl.gov FU US Department of Energy [DE-AC02-05CH11231, DE-FG02-05ER41367, DE-SC0004286, DE-SC0004104] FX We gratefully acknowledge fruitful discussions with T. Hirano, P. Huovinen, H. Masui, H. Niemi, A. Poskanzer, C. Shen, R. Snellings, and X.-N. Wang. We especially thank T. Hirano for providing the new initial conditions at LHC energies, R. Snellings for the experimental data shown in Figs. 2 and 3, and H. Buesching for the ALICE data show in Fig. 1(a). This work was supported by the US Department of Energy under Grant Nos. DE-AC02-05CH11231, DE-FG02-05ER41367, DE-SC0004286, and (within the framework of the Jet Collaboration) DE-SC0004104. We gratefully acknowledge extensive computing resources provided to us by the Ohio Supercomputer Center. NR 66 TC 84 Z9 84 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAY 27 PY 2011 VL 83 IS 5 AR 054912 DI 10.1103/PhysRevC.83.054912 PG 6 WC Physics, Nuclear SC Physics GA 769LX UT WOS:000291016300006 ER PT J AU Bott, SC Haas, DM Madden, RE Ueda, U Eshaq, Y Collins, G Gunasekera, K Mariscal, D Peebles, J Beg, FN Mazarakis, M Struve, K Sharpe, R AF Bott, S. C. Haas, D. M. Madden, R. E. Ueda, U. Eshaq, Y. Collins, G. Gunasekera, K. Mariscal, D. Peebles, J. Beg, F. N. Mazarakis, M. Struve, K. Sharpe, R. TI 250 kA compact linear transformer driver for wire array z-pinch loads SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article AB We present the application of a short rise (similar to 150 ns) 250 kA linear transformer driver (LTD) to wire array z-pinch loads for the first time. The generator is a modification of a previous driver in which a new conical power feed provides a low inductance coupling to wire loads. Performance of the new design using both short circuit and plasma loads is presented and discussed. The final design delivers similar to 200 kA to a wire array load which is in good agreement with SCREAMER calculations using a simplified representative circuit. Example results demonstrate successful experiments using cylindrical, conical, and inverse wire arrays as well as previously published work on x-pinch loads. C1 [Bott, S. C.; Haas, D. M.; Madden, R. E.; Ueda, U.; Eshaq, Y.; Collins, G.; Gunasekera, K.; Mariscal, D.; Peebles, J.; Beg, F. N.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Mazarakis, M.; Struve, K.; Sharpe, R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Bott, SC (reprint author), Univ Calif San Diego, La Jolla, CA 92093 USA. FU Department of Energy [DE-SC-0001063] FX The UC San Diego team is grateful to Sandia National Laboratories and to Dr. Chris Deeney for both the loan of the generator and the technical support in completing its installation. The UCSD authors also thank Mr. Sean McGraw (Ashland University, Ohio) who helped with some of the laboratory testing during his National Undergraduate Fellowship (NUF) placement. This work was supported by the Department of Energy under Contract No. DE-SC-0001063. NR 26 TC 10 Z9 10 U1 1 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD MAY 27 PY 2011 VL 14 IS 5 AR 050401 DI 10.1103/PhysRevSTAB.14.050401 PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 769MO UT WOS:000291018200001 ER PT J AU Liu, XJ Lu, WC Wang, CZ Ho, KM AF Liu, Xiaojie Lu, Wen-Cai Wang, C. Z. Ho, K. M. TI Energetic and fragmentation stability of water clusters (H2O)(n), n=2-30 SO CHEMICAL PHYSICS LETTERS LA English DT Article ID HEXAMER CLUSTERS; AB-INITIO; BINDING-ENERGIES; SPECTRA; SPECTROSCOPY; FORM AB Ab initio calculations have been performed to study the structural trend, energetic stability, and fragmentation behavior of water clusters (H2O)(2-30). We show that as size increases, the cluster structures evolve from a mono-ring motif to multi-ring and ring-stacking motifs, and then to stuffed cage structures. We also show that losing water molecules one-by-one is the most favorable fragmentation channel with a dissociation energy of similar to 11.53 kcal/mol. Small water clusters such as water dimer, trimer, and tetramer, can also be observed in the fragmentation products since they often appear in the second best fragmentation channel. (C) 2011 Elsevier B. V. All rights reserved. C1 [Liu, Xiaojie; Lu, Wen-Cai] Jilin Univ, Inst Theoret Chem, State Key Lab Theoret & Computat Chem, Changchun 130021, Jilin, Peoples R China. [Lu, Wen-Cai] Qingdao Univ, Growing Base State Key Lab, Lab Fiber Mat & Modern Text, Qingdao 266071, Shandong, Peoples R China. [Lu, Wen-Cai] Qingdao Univ, Coll Phys, Qingdao 266071, Shandong, Peoples R China. [Liu, Xiaojie; Wang, C. Z.; Ho, K. M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Liu, Xiaojie; Wang, C. Z.; Ho, K. M.] US DOE, Ames Lab, Ames, IA 50011 USA. RP Lu, WC (reprint author), Jilin Univ, Inst Theoret Chem, State Key Lab Theoret & Computat Chem, Changchun 130021, Jilin, Peoples R China. EM wencailu@jlu.edu.cn FU National Natural Science Foundation of China [21043001, 20773047]; U.S. Department of Energy by Iowa State University [DE-AC02-07CH11358]; Office of Basic Energy Sciences, Division of Material Science and Engineering; China Scholarship Council [2009617104] FX This work was supported by the National Natural Science Foundation of China (Nos. 21043001 and 20773047). Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. This work was also supported by the Director for Energy Research, Office of Basic Energy Sciences, Division of Material Science and Engineering including a grant for computer time at the National Energy Research Supercomputing Center (NERSC) in Berkeley, CA. Xiaojie Liu acknowledges the support from China Scholarship Council (File No. 2009617104). NR 28 TC 15 Z9 15 U1 1 U2 18 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD MAY 27 PY 2011 VL 508 IS 4-6 BP 270 EP 275 DI 10.1016/j.cplett.2011.04.055 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 766AK UT WOS:000290750400017 ER PT J AU He, J Scott, JL Heroux, A Roy, S Lenoir, M Overduin, M Stahelin, RV Kutateladze, TG AF He, Ju Scott, Jordan L. Heroux, Annie Roy, Siddhartha Lenoir, Marc Overduin, Michael Stahelin, Robert V. Kutateladze, Tatiana G. TI Molecular Basis of Phosphatidylinositol 4-Phosphate and ARF1 GTPase Recognition by the FAPP1 Pleckstrin Homology (PH) Domain SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID STRUCTURAL BASIS; FYVE DOMAIN; MEMBRANE; BINDING; PROTEINS; ACIDIFICATION; PTDINS(4)P; MECHANISM; APOPTOSIS; SOFTWARE AB Four-phosphate-adaptor protein 1 (FAPP1) regulates secretory transport from the trans-Golgi network (TGN) to the plasma membrane. FAPP1 is recruited to the Golgi through binding of its pleckstrin homology (PH) domain to phosphatidylinositol 4-phosphate (PtdIns(4) P) and a small GTPase ADP-ribosylation factor 1 (ARF1). Despite the critical role of FAPP1 in membrane trafficking, the molecular basis of its dual function remains unclear. Here, we report a 1.9 angstrom resolution crystal structure of the FAPP1 PH domain and detail the molecular mechanisms of the PtdIns(4) P and ARF1 recognition. The FAPP1 PH domain folds into a seven-stranded beta-barrel capped by an beta-helix at one edge, whereas the opposite edge is flanked by three loops and the beta 4 and beta 7 strands that form a lipid-binding pocket within the beta-barrel. The ARF1-binding site is located on the outer side of the beta-barrel as determined by NMR resonance perturbation analysis, mutagenesis, and measurements of binding affinities. The two binding sites have little overlap, allowing FAPP1 PH to associate with both ligands simultaneously and independently. Binding to PtdIns(4) P is enhanced in an acidic environment and is required for membrane penetration and tubulation activity of FAPP1, whereas the GTP-bound conformation of the GTPase is necessary for the interaction with ARF1. Together, these findings provide structural and biochemical insight into the multivalent membrane anchoring by the PH domain that may augment affinity and selectivity of FAPP1 toward the TGN membranes enriched in both PtdIns(4) P and GTP-bound ARF1. C1 [Scott, Jordan L.; Stahelin, Robert V.] Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA. [He, Ju; Roy, Siddhartha; Kutateladze, Tatiana G.] Univ Colorado, Sch Med, Dept Pharmacol, Aurora, CO 80045 USA. [Scott, Jordan L.; Stahelin, Robert V.] Univ Notre Dame, Walther Ctr Canc Res, Notre Dame, IN 46556 USA. [Stahelin, Robert V.] Indiana Univ Sch Med, Dept Biochem & Mol Biol, South Bend, IN 46617 USA. [Heroux, Annie] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. [Lenoir, Marc; Overduin, Michael] Univ Birmingham, Sch Canc Sci, Birmingham B15 2TT, W Midlands, England. RP Stahelin, RV (reprint author), Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA. EM rstaheli@iupui.edu; Tatiana.Kutateladze@ucdenver.edu OI Overduin, Michael/0000-0002-3114-6585 FU National Institutes of Health [GM071424, CA95144]; American Heart Association; Indiana University Biomedical Research; American Cancer Society; Cancer Research UK; Offices of Biological and Environmental Research and of Basic Energy Sciences of the United States Department of Energy; National Center for Research Resources of the National Institutes of Health [P41RR012408] FX This work was supported, in whole or in part, by National Institutes of Health Grants GM071424 and CA95144 and the American Heart Association (to T. G. K.). This work was also supported by grants from Indiana University Biomedical Research and the American Cancer Society (to R. V. S.) and Cancer Research UK (to M. O.).; We thank Y. Gedle, M. Lemmon, C. Musselman, E. Odintsova, and R. Zhao for discussions and helping with experiments and R. Prekeris and S. Wakatsuki for providing cDNAs of wild type and ARF1 Q71L. X-ray crystallographic data were collected at beamline X25 of the NSLS. Financial support for NSLS comes from the Offices of Biological and Environmental Research and of Basic Energy Sciences of the United States Department of Energy and from the National Center for Research Resources of the National Institutes of Health (Grant P41RR012408). NR 38 TC 41 Z9 43 U1 0 U2 7 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 J9 J BIOL CHEM JI J. Biol. Chem. PD MAY 27 PY 2011 VL 286 IS 21 BP 18650 EP 18657 DI 10.1074/jbc.M111.233015 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 766ME UT WOS:000290785700037 PM 21454700 ER PT J AU Schushan, M Landau, M Padan, E Ben-Tal, N AF Schushan, Maya Landau, Meytal Padan, Etana Ben-Tal, Nir TI Two Conflicting NHE1 Model Structures: Compatibility with Experimental Data and Implications for the Transport Mechanism SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Letter ID ANTIPORTER C1 [Schushan, Maya; Ben-Tal, Nir] Tel Aviv Univ, George S Wise Fac Life Sci, Dept Biochem & Mol Biol, IL-69978 Ramat Aviv, Israel. [Landau, Meytal] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90024 USA. [Landau, Meytal] Univ Calif Los Angeles, UCLA DOE Inst Genom & Prote, Los Angeles, CA USA. [Padan, Etana] Hebrew Univ Jerusalem, Dept Biol Chem, Alexander Silberman Inst Life Sci, IL-91904 Jerusalem, Israel. RP Schushan, M (reprint author), Tel Aviv Univ, George S Wise Fac Life Sci, Dept Biochem & Mol Biol, IL-69978 Ramat Aviv, Israel. EM NirB@tauex.tau.ac.il RI landau, Meytal/J-3075-2012 NR 5 TC 5 Z9 5 U1 0 U2 1 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 J9 J BIOL CHEM JI J. Biol. Chem. PD MAY 27 PY 2011 VL 286 IS 21 AR le9 DI 10.1074/jbc.L110.159202 PG 1 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 766ME UT WOS:000290785700003 ER PT J AU Mendes, R Kruijt, M de Bruijn, I Dekkers, E van der Voort, M Schneider, JHM Piceno, YM DeSantis, TZ Andersen, GL Bakker, PAHM Raaijmakers, JM AF Mendes, Rodrigo Kruijt, Marco de Bruijn, Irene Dekkers, Ester van der Voort, Menno Schneider, Johannes H. M. Piceno, Yvette M. DeSantis, Todd Z. Andersen, Gary L. Bakker, Peter A. H. M. Raaijmakers, Jos M. TI Deciphering the Rhizosphere Microbiome for Disease-Suppressive Bacteria SO SCIENCE LA English DT Article ID PATHOGENS AB Disease-suppressive soils are exceptional ecosystems in which crop plants suffer less from specific soil-borne pathogens than expected owing to the activities of other soil microorganisms. For most disease-suppressive soils, the microbes and mechanisms involved in pathogen control are unknown. By coupling PhyloChip-based metagenomics of the rhizosphere microbiome with culture-dependent functional analyses, we identified key bacterial taxa and genes involved in suppression of a fungal root pathogen. More than 33,000 bacterial and archaeal species were detected, with Proteobacteria, Firmicutes, and Actinobacteria consistently associated with disease suppression. Members of the gamma-Proteobacteria were shown to have disease-suppressive activity governed by nonribosomal peptide synthetases. Our data indicate that upon attack by a fungal root pathogen, plants can exploit microbial consortia from soil for protection against infections. C1 [Mendes, Rodrigo; Kruijt, Marco; de Bruijn, Irene; Dekkers, Ester; van der Voort, Menno; Raaijmakers, Jos M.] Wageningen Univ, Phytopathol Lab, NL-6700 EE Wageningen, Netherlands. [Schneider, Johannes H. M.] Inst Sugar Beet Res, NL-4611 HL Bergen Op Zoom, Netherlands. [Piceno, Yvette M.; DeSantis, Todd Z.; Andersen, Gary L.] Lawrence Berkeley Natl Lab, Dept Ecol, Berkeley, CA 94720 USA. [DeSantis, Todd Z.] Second Genome Inc, San Francisco, CA 94158 USA. [Bakker, Peter A. H. M.] Univ Utrecht, Dept Biol, NL-3584 CH Utrecht, Netherlands. RP Raaijmakers, JM (reprint author), Wageningen Univ, Phytopathol Lab, Droevendaalsesteeg 1, NL-6700 EE Wageningen, Netherlands. EM jos.raaijmakers@wur.nl RI Bakker, Peter/B-9355-2011; Utrecht Univ., PMI/G-9549-2011; de Bruijn, Irene/A-7437-2014; Raaijmakers, Jos/D-1574-2014; Mendes, Rodrigo/F-1534-2010; Andersen, Gary/G-2792-2015; Piceno, Yvette/I-6738-2016 OI de Bruijn, Irene/0000-0002-4889-3253; Raaijmakers, Jos/0000-0003-1608-6614; Mendes, Rodrigo/0000-0002-9817-4118; Andersen, Gary/0000-0002-1618-9827; Piceno, Yvette/0000-0002-7915-4699 FU Netherlands Science Organisation (NWO) [838.06.101]; Netherlands Genomics Initiative-Ecogenomics, Netherlands; Lawrence Berkeley National Laboratory (LBNL) [DE-AC02-05CH11231]; U.S. Department of Energy FX We thank T. Bisseling for critical reading and valuable suggestions. We acknowledge assistance by L. Sibbel-Wagemakers, N. Pangesti, M. de Milliano, N. Sharma, R. de Vries, P. M. S. van Oorschot, A. H. L. Schoone, and Y. Bakker. This work was financially supported by grants from Netherlands Science Organisation (NWO)-ERGO (#838.06.101) and Netherlands Genomics Initiative-Ecogenomics, Netherlands. Additional work was performed at Lawrence Berkeley National Laboratory (LBNL) (contract DE-AC02-05CH11231 with the U.S. Department of Energy). The 16S rDNA sequences are available on GenBank under accessions HQ848634 to HQ848643, and the thaABCD sequences under accession HQ888764. LBNL has a patent on the PhyloChip assay and Second Genome has licensed this assay from LBNL. Although the G3 PhyloChip is under patent (and under exclusive license to Second Genome), the data generated from the use of the chip are not patented or restricted. T.Z.dS. owns stock in Second Genome valued at under $10,000. NR 14 TC 381 Z9 410 U1 58 U2 432 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 J9 SCIENCE JI Science PD MAY 27 PY 2011 VL 332 IS 6033 BP 1097 EP 1100 DI 10.1126/science.1203980 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 769FN UT WOS:000290996700048 PM 21551032 ER PT J AU Hwang, GS Kaviany, M Gostick, JT Kientiz, B Weber, AZ Kim, MH AF Hwang, Gi Suk Kaviany, Massoud Gostick, Jeffrey T. Kientiz, Brian Weber, Adam Z. Kim, Moo Hwan TI Role of water states on water uptake and proton transport in Nafion using molecular simulations and bimodal network SO POLYMER LA English DT Article DE Water uptake; Proton conductivity; Water diffusivity ID POLYMER-ELECTROLYTE MEMBRANES; FUEL-CELL MEMBRANES; EXCHANGE MEMBRANES; SCHROEDERS-PARADOX; X-RAY; MODEL; DIFFUSION; ACID; CONDUCTIVITY; HYDRATION AB Using molecular simulations and a bimodal-domain network, the role of water state on Nafion water uptake and water and proton transport is investigated. Although the smaller domains provide moderate transport pathways, their effectiveness remains low due to strong, resistive water molecules/domain surface interactions. The water occupancy of the larger domains yields bulk-like water, and causes the observed transition in the water uptake and significant increases in transport properties. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Hwang, Gi Suk; Kaviany, Massoud] Univ Michigan, Dept Mech Engn, Ann Arbor, MI 48109 USA. [Gostick, Jeffrey T.; Kientiz, Brian; Weber, Adam Z.] Univ Calif Berkeley, Lawrence Berkeley Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Kim, Moo Hwan] Pohang Univ Sci & Technol, Dept Mech Engn, Pohang 790874, Kyungbuk, South Korea. RP Kaviany, M (reprint author), Univ Michigan, Dept Mech Engn, Ann Arbor, MI 48109 USA. EM kaviany@umich.edu OI Weber, Adam/0000-0002-7749-1624 FU Ministry of Science and Technology, South Korea; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Fuel Cell Technologies; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX We are thankful for the sponsorship of Global Partnership Program ("Ministry of Science and Technology, South Korea), assistance by Drs. Alexander Hexemer and Cheng Wang (Lawrence Berkeley National Laboratory) on the SAXS measurements, and discussions with Professor Reinhard Hentschke (University of Wuppertal, Germany) on the GCMD-MC simulation. This work was partially supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Fuel Cell Technologies, and the Director, Office of Science, Office of Basic Energy Sciences (for support of the Advanced Light Source), of the U.S. Department of Energy under contract number DE-AC02-05CH11231. NR 74 TC 25 Z9 25 U1 0 U2 21 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 EI 1873-2291 J9 POLYMER JI Polymer PD MAY 26 PY 2011 VL 52 IS 12 BP 2584 EP 2593 DI 10.1016/j.polymer.2011.03.056 PG 10 WC Polymer Science SC Polymer Science GA 771BY UT WOS:000291133400017 ER PT J AU Kim, E Ahn, H Lee, H Lee, B Ryu, DY AF Kim, Eunhye Ahn, Hyungju Lee, Hoyeon Lee, Byeongdu Ryu, Du Yeol TI Ordering and microdomain orientation in block copolymer films by thermal deprotection SO POLYMER LA English DT Article DE Ordering; Microdomain orientation; Block copolymer films ID X-RAY-SCATTERING; THIN-FILMS; TRANSITION; SURFACES; CYLINDER; ARRAYS; TEMPLATES; SUBSTRATE; BEHAVIOR; DOMAINS AB Ordering and microdomain orientation for the films of symmetric polystyrene-b-poly(tert-butyl methacrylate)s (PS-b-PtBMAs) was investigated by in-situ grazing incidence small-angle X-ray scattering (GISAXS) and the electron microscopy. During thermal deprotection at higher temperature (200 degrees C), functional tert-butyl ester units in the PtBMA block component are integrated into inter- or intra-molecular anhydride linkages. It was observed that this process causes an increase in the Flory -Huggins interaction parameter (chi) between the two block components for disordered PS-b-PtBMA film, leading to a modulated nonequilibrium structure. Interestingly, for lamella-forming PS-b-PtBMA film, a significant chain stretching in lateral direction during thermal deprotection resulted in a characteristic strain-induced perpendicular orientation in the middle of the film confined between two parallel orientations of lamellar microdomains. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Kim, Eunhye; Ahn, Hyungju; Lee, Hoyeon; Ryu, Du Yeol] Yonsei Univ, Dept Chem & Biomol Engn, Seoul 120749, South Korea. [Lee, Byeongdu] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. RP Ryu, DY (reprint author), Yonsei Univ, Dept Chem & Biomol Engn, 262 Seongsanno, Seoul 120749, South Korea. EM dyryu@yonsei.ac.kr RI Ryu, Du Yeol/G-8278-2012; OI Lee, Byeongdu/0000-0003-2514-8805 FU Ministry of Education, Science & Technology (MEST), Korea [2009-0067295, 2010K001430, R11-2007-050-00000] FX This work was supported by NRF grants (2009-0067295), Converging Research Center Program (2010K001430), and APCPI ERC program (R11-2007-050-00000), which are funded by the Ministry of Education, Science & Technology (MEST), Korea. NR 39 TC 3 Z9 3 U1 0 U2 17 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 J9 POLYMER JI Polymer PD MAY 26 PY 2011 VL 52 IS 12 BP 2677 EP 2684 DI 10.1016/j.polymer.2011.04.031 PG 8 WC Polymer Science SC Polymer Science GA 771BY UT WOS:000291133400027 ER PT J AU Liu, C Lee, Y Kondo, T Mun, ED Caudle, M Harmon, BN Bud'ko, SL Canfield, PC Kaminski, A AF Liu, Chang Lee, Yongbin Kondo, Takeshi Mun, Eun Deok Caudle, Malinda Harmon, B. N. Bud'ko, Sergey L. Canfield, Paul C. Kaminski, Adam TI Metallic surface electronic state in half-Heusler compounds RPtBi (R = Lu, Dy, Gd) SO PHYSICAL REVIEW B LA English DT Article ID HGTE QUANTUM-WELLS; TOPOLOGICAL INSULATORS; TERNARY COMPOUNDS; TRANSPORT; TRANSITION; BI2TE3; PHASE AB Rare-earth platinum bismuth (RPtBi) has been proposed recently as a potential topological insulator. In this paper, we present measurements of the metallic surface electronic structure in three members of this family, using angle-resolved photoemission spectroscopy (ARPES). Our data show clear spin-orbit splitting of the surface bands and the Kramers' degeneracy of spins at the (Gamma) over bar and (M) over bar points, which is reproduced nicely with our full-potential linearized augmented plane wave calculation for a surface electronic state. Topologically nontrivial behavior is signified by band inversion in the calculated bulk electronic structures, yet no direct indication of such behavior is detected by ARPES except for a weak Fermi crossing detected in close proximity to the (Gamma) over bar point, making the total number of Fermi crossings odd. In the surface band calculation, however, this crossing is explained by a Kramers pair of bands that are very close to each other. The classification of this family of materials as topological insulators remains an open question. C1 [Liu, Chang; Lee, Yongbin; Kondo, Takeshi; Mun, Eun Deok; Caudle, Malinda; Harmon, B. N.; Bud'ko, Sergey L.; Canfield, Paul C.; Kaminski, Adam] Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. [Liu, Chang; Kondo, Takeshi; Mun, Eun Deok; Caudle, Malinda; Harmon, B. N.; Bud'ko, Sergey L.; Canfield, Paul C.; Kaminski, Adam] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Liu, C (reprint author), Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. RI Canfield, Paul/H-2698-2014; Kondo, Takeshi/H-2680-2016 FU Department of Energy-Basic Energy Sciences [DE-AC02-07CH11358]; US DOE [DE-AC03-76SF00098] FX We thank S.-C. Zhang and J. Schmalian for instructive discussions as well as Sung-Kwan Mo for grateful instrumental support at the ALS. Ames Laboratory was supported by the Department of Energy-Basic Energy Sciences under Contract No. DE-AC02-07CH11358. ALS is operated by the US DOE under Contract No. DE-AC03-76SF00098. NR 27 TC 37 Z9 37 U1 4 U2 49 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 26 PY 2011 VL 83 IS 20 AR 205133 DI 10.1103/PhysRevB.83.205133 PG 5 WC Physics, Condensed Matter SC Physics GA 769IH UT WOS:000291005600002 ER PT J AU Rahman, R Verduijn, J Kharche, N Lansbergen, GP Klimeck, G Hollenberg, LCL Rogge, S AF Rahman, R. Verduijn, J. Kharche, N. Lansbergen, G. P. Klimeck, G. Hollenberg, L. C. L. Rogge, S. TI Engineered valley-orbit splittings in quantum-confined nanostructures in silicon SO PHYSICAL REVIEW B LA English DT Article ID NEMO 3-D; SIMULATION; TRANSPORT; ATOM; DOTS AB An important challenge in silicon quantum electronics in the few electron regime is the potentially small energy gap between the ground and excited orbital states in 3D quantum confined nanostructures due to the multiple valley degeneracies of the conduction band present in silicon. Understanding the "valley-orbit" (VO) gap is essential for silicon qubits, as a large VO gap prevents leakage of the qubit states into a higher dimensional Hilbert space. The VO gap varies considerably depending on quantum confinement, and can be engineered by external electric fields. In this work we investigate VO splitting experimentally and theoretically in a range of confinement regimes. We report measurements of the VO splitting in silicon quantum dot and donor devices through excited state transport spectroscopy. These results are underpinned by large-scale atomistic tight-binding calculations involving over 1 million atoms to compute VO splittings as functions of electric fields, donor depths, and surface disorder. The results provide a comprehensive picture of the range of VO splittings that can be achieved through quantum engineering. C1 [Rahman, R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Verduijn, J.; Lansbergen, G. P.; Rogge, S.] Delft Univ Technol, Kavli Inst Nanosci, NL-2628 CJ Delft, Netherlands. [Verduijn, J.; Rogge, S.] Univ New S Wales, Sch Phys, Ctr Quantum Computat & Commun Technol, Sydney, NSW 2052, Australia. [Kharche, N.] Rensselaer Polytech Inst, Dept Phys, Computat Ctr Nanotechnol Innovat, Troy, NY 12180 USA. [Klimeck, G.] Purdue Univ, Network Computat Nanotechnol, W Lafayette, IN 47907 USA. [Hollenberg, L. C. L.] Univ Melbourne, Sch Phys, Ctr Quantum Computat & Commun Technol, Melbourne, Vic 3010, Australia. RP Rahman, R (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM rrahman@sandia.gov RI Lansbergen, Gabriel/A-7895-2011; Kharche, Neerav/F-4331-2015; Klimeck, Gerhard/A-1414-2012; Rogge, Sven/G-3709-2010; OI Kharche, Neerav/0000-0003-1014-6022; Klimeck, Gerhard/0000-0001-7128-773X; Rahman, Rajib/0000-0003-1649-823X FU United States Department of Energy [DEAC04-94AL85000]; NASA; Australian Research Council Centre of Excellence for Quantum Computation and Communication Technology [CE110001029]; NSA; ARO [W911NF-08-1-0527] FX Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Corporation, for the United States Department of Energy under Contract No. DEAC04-94AL85000. NEMO-3D was initially developed at JPL, Caltech under a contract with NASA. NCN/nanohub.org computational resources were used. This research was conducted by the Australian Research Council Centre of Excellence for Quantum Computation and Communication Technology (Project No. CE110001029), NSA and ARO Contract No. W911NF-08-1-0527). NR 32 TC 22 Z9 22 U1 2 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 26 PY 2011 VL 83 IS 19 AR 195323 DI 10.1103/PhysRevB.83.195323 PG 5 WC Physics, Condensed Matter SC Physics GA 769IG UT WOS:000291005500005 ER PT J AU Armijo, J Barnard, JJ AF Armijo, J. Barnard, J. J. TI Droplet evolution in expanding flow of warm dense matter SO PHYSICAL REVIEW E LA English DT Article ID MOLECULAR-DYNAMICS; LASER-ABLATION; LIQUID; EVAPORATION; SIMULATION; EQUATION; FRAGMENTATION; TEMPERATURE; EXPANSION; FACILITY AB We propose a simple, self-consistent kinetic model for the evolution of a mixture of droplets and vapor expanding adiabatically in vacuum after rapid, almost isochoric heating. We study the evolution of the two-phase fluid at intermediate times between the molecular and the hydrodynamic scales, focusing on out-of-equilibrium and surface effects. We use the van der Waals equation of state as a test bed to implement our model and study the phenomenology of the upcoming second neutralized drift compression experiment (NDCX-II) at Lawrence Berkeley National Laboratory (LBNL) that uses ion beams for target heating. We find an approximate expression for the temperature difference between the droplets and the expanding gas and we check it with numerical calculations. The formula provides a useful criterion to distinguish the thermalized and nonthermalized regimes of expansion. In the thermalized case, the liquid fraction grows in a proportion that we estimate analytically, whereas, in case of too rapid expansion, a strict limit for the evaporation of droplets is derived. The range of experimental situations is discussed. C1 [Armijo, J.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Barnard, J. J.] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Armijo, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. EM julienarmijo@gmail.com RI Armijo, Julien/I-5413-2013 FU Ecole Normale Superieure, France; US Department of Energy under University of California at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; US Department of Energy under University of California at Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We wish to thank R. M. More, F. M. Bieniosek, P. A. Seidl, B. G. Logan, and I. D. Kaganovich for helpful discussions. One of us (J.A.) was partially supported by Ecole Normale Superieure, France. Work performed under the auspices of the US Department of Energy under University of California Contract No. DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory and Contract No. DE-AC52-07NA27344 at Lawrence Livermore National Laboratory. NR 44 TC 3 Z9 3 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 J9 PHYS REV E JI Phys. Rev. E PD MAY 26 PY 2011 VL 83 IS 5 AR 051507 DI 10.1103/PhysRevE.83.051507 PN 1 PG 11 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 769IR UT WOS:000291006600002 PM 21728540 ER PT J AU Carlsten, BE Bishofberger, KA Duffy, LD Russell, SJ Ryne, RD Yampolsky, NA Dragt, AJ AF Carlsten, Bruce E. Bishofberger, Kip A. Duffy, Leanne D. Russell, Steven J. Ryne, Robert D. Yampolsky, Nikolai A. Dragt, Alex J. TI Arbitrary emittance partitioning between any two dimensions for electron beams SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID OPERATION AB The flat-beam transform (FBT) for round symmetric beams can be extended using the concept of eigenemittances. By tailoring the initial beam conditions at the cathode, including adding arbitrary correlations between any two dimensions, this extension can be used to provide greater freedom in controlling the beam's final emittances. In principle, this technique can be used to generate extraordinarily transversely bright electron beams. Examples are provided where an equivalent FBT is established between the horizontal and the longitudinal beam dimensions. C1 [Carlsten, Bruce E.; Bishofberger, Kip A.; Duffy, Leanne D.; Russell, Steven J.; Yampolsky, Nikolai A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Ryne, Robert D.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Dragt, Alex J.] Univ Maryland, College Pk, MD 20742 USA. RP Carlsten, BE (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RI Yampolsky, Nikolai/A-7521-2011; OI Duffy, Leanne/0000-0002-0123-6723; Carlsten, Bruce/0000-0001-5619-907X NR 22 TC 10 Z9 10 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD MAY 26 PY 2011 VL 14 IS 5 AR 050706 DI 10.1103/PhysRevSTAB.14.050706 PG 16 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 769IY UT WOS:000291007300001 ER PT J AU Hamidi, H Gustafason, D Pellegrini, M Gasson, J AF Hamidi, Habib Gustafason, Derek Pellegrini, Matteo Gasson, Judith TI Identification of Novel Targets of CSL-Dependent Notch Signaling in Hematopoiesis SO PLOS ONE LA English DT Article ID EMBRYONIC STEM-CELLS; ACUTE LYMPHOBLASTIC-LEUKEMIA; IN-VITRO DIFFERENTIATION; FACTOR-BINDING SITES; MODEL-BASED ANALYSIS; ZONE B-CELLS; RBP-J-KAPPA; T-CELLS; TRANSCRIPTION FACTORS; GENE-EXPRESSION AB Somatic activating mutations in the Notch1 receptor result in the overexpression of activated Notch1, which can be tumorigenic. The goal of this study is to understand the molecular mechanisms underlying the phenotypic changes caused by the overexpression of ligand independent Notch 1 by using a tetracycline inducible promoter in an in vitro embryonic stem (ES) cells/OP9 stromal cells coculture system, recapitulating normal hematopoiesis. First, an in silico analysis of the promoters of Notch regulated genes (previously determined by microarray analysis) revealed that the motifs recognized by regulatory proteins known to mediate hematopoiesis were overrepresented. Notch 1 does not bind DNA but instead binds the CSL transcription factor to regulate gene expression. The in silico analysis also showed that there were putative CSL binding sites observed in the promoters of 28 out of 148 genes. A custom ChIP-chip array was used to assess the occupancy of CSL in the promoter regions of the Notch1 regulated genes in vivo and showed that 61 genes were bound by activated Notch responsive CSL. Then, comprehensive mapping of the CSL binding sites genome-wide using ChIP-seq analysis revealed that over 10,000 genes were bound within 10 kb of the TSS (transcription start site). The majority of the targets discovered by ChIP-seq belong to pathways that have been shown by others to crosstalk with Notch signaling. Finally, 83 miRNAs were significantly differentially expressed by greater than 1.5-fold during the course of in vitro hematopoiesis. Thirty one miRNA were up-regulated and fifty two were down-regulated. Overexpression of Notch1 altered this pattern of expression of microRNA: six miRNAs were up-regulated and four were down regulated as a result of activated Notch1 overexpression during the course of hematopoiesis. Time course analysis of hematopoietic development revealed that cells with Notch 1 overexpression mimic miRNA expression of cells in a less mature stage, which is consistent with our previous biological characterization. C1 [Hamidi, Habib; Gasson, Judith] Univ Calif Los Angeles, David Geffen Sch Med, Dept Biol Chem, Los Angeles, CA 90095 USA. [Gustafason, Derek; Pellegrini, Matteo] Univ Calif Los Angeles, DOE Inst Genom & Prote, Los Angeles, CA USA. [Pellegrini, Matteo] Univ Calif Los Angeles, Dept Mol Cell & Dev Biol, Los Angeles, CA USA. [Gasson, Judith] Univ Calif Los Angeles, David Geffen Sch Med, Dept Med, Div Hematol Oncol, Los Angeles, CA 90095 USA. [Gasson, Judith] Univ Calif Los Angeles, David Geffen Sch Med, Dept Biol Chem, Los Angeles, CA 90095 USA. [Gasson, Judith] Univ Calif Los Angeles, David Geffen Sch Med, Jonsson Comprehens Canc Ctr, Los Angeles, CA 90095 USA. RP Hamidi, H (reprint author), Univ Calif Los Angeles, David Geffen Sch Med, Dept Biol Chem, Los Angeles, CA 90095 USA. EM jgasson@mednet.ucla.edu NR 118 TC 22 Z9 23 U1 0 U2 6 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 185 BERRY ST, STE 1300, SAN FRANCISCO, CA 94107 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 26 PY 2011 VL 6 IS 5 AR e20022 DI 10.1371/journal.pone.0020022 PG 19 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 769XS UT WOS:000291052200027 PM 21637838 ER PT J AU Weyman, PD Vargas, WA Tong, YK Yu, JP Maness, PC Smith, HO Xu, Q AF Weyman, Philip D. Vargas, Walter A. Tong, Yingkai Yu, Jianping Maness, Pin-Ching Smith, Hamilton O. Xu, Qing TI Heterologous Expression of Alteromonas macleodii and Thiocapsa roseopersicina [NiFe] Hydrogenases in Synechococcus elongatus SO PLOS ONE LA English DT Article ID BIDIRECTIONAL HYDROGENASE; ACCESSORY GENES; MUTAGENESIS; MATURATION; OXIDATION; CLONING; BBS; CYANOBACTERIA; BIOSYNTHESIS; ALCALIGENES AB Oxygen-tolerant [NiFe] hydrogenases may be used in future photobiological hydrogen production systems once the enzymes can be heterologously expressed in host organisms of interest. To achieve heterologous expression of [NiFe] hydrogenases in cyanobacteria, the two hydrogenase structural genes from Alteromonas macleodii Deep ecotype (AltDE), hynS and hynL, along with the surrounding genes in the gene operon of HynSL were cloned in a vector with an IPTG-inducible promoter and introduced into Synechococcus elongatus PCC7942. The hydrogenase protein was expressed at the correct size upon induction with IPTG. The heterologously-expressed HynSL hydrogenase was active when tested by in vitro H-2 evolution assay, indicating the correct assembly of the catalytic center in the cyanobacterial host. Using a similar expression system, the hydrogenase structural genes from Thiocapsa roseopersicina (hynSL) and the entire set of known accessory genes were transferred to S. elongatus. A protein of the correct size was expressed but had no activity. However, when the 11 accessory genes from AltDE were co-expressed with hynSL, the T. roseopersicina hydrogenase was found to be active by in vitro assay. This is the first report of active, heterologously-expressed [NiFe] hydrogenases in cyanobacteria. C1 [Weyman, Philip D.; Vargas, Walter A.; Tong, Yingkai; Smith, Hamilton O.; Xu, Qing] J Craig Venter Inst, Dept Synthet Biol & Bioenergy, Rockville, MD USA. [Yu, Jianping; Maness, Pin-Ching] Natl Renewable Energy Lab, Golden, CO USA. RP Weyman, PD (reprint author), J Craig Venter Inst, Dept Synthet Biol & Bioenergy, Rockville, MD USA. EM qxu2019@gmail.com OI Weyman, Philip/0000-0001-5787-0291 FU U.S. Department of Energy [DE-FG36-05GO15027] FX This work was supported by the U.S. Department of Energy, the Hydrogen, Fuel Cells, and Infrastructure Technology Program (DE-FG36-05GO15027). The funder had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 39 TC 16 Z9 16 U1 0 U2 18 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 26 PY 2011 VL 6 IS 5 AR e20126 DI 10.1371/journal.pone.0020126 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 769XS UT WOS:000291052200035 PM 21637846 ER PT J AU Li, HY Sivapalan, M AF Li, Hongyi Sivapalan, Murugesu TI Effect of spatial heterogeneity of runoff generation mechanisms on the scaling behavior of event runoff responses in a natural river basin SO WATER RESOURCES RESEARCH LA English DT Article ID ELEMENTARY WATERSHED APPROACH; FLOOD FREQUENCY; GEOMORPHOLOGICAL DISPERSION; KINEMATIC DISPERSION; HYDROLOGIC RESPONSE; CATCHMENT-SCALE; RESIDENCE TIME; COLD REGIONS; MODEL; NETWORK AB This paper presents a theoretical investigation of the effects of spatial heterogeneity of runoff generation on the scaling behavior of runoff timing responses. A previous modeling study on the Illinois River Basin in Oklahoma had revealed a systematic spatial trend in the relative dominance of different runoff generation mechanisms, attributable to corresponding systematic trends in landscape properties. Considering the differences in the timing of hillslope responses between the different runoff mechanisms, this paper explores their impacts on the catchment-scale runoff routing responses, including how they change with spatial scale. For this purpose we utilize a distributed, physically based hydrological model, with a fully hydraulic stream network routing component. The model is used to generate instantaneous response functions (IRF) for nested catchments of a range of sizes along the river network and quantitative measures of their shape, e. g., peak and time to peak. In order to separate the effects of soil heterogeneity from those due to basin geomorphology, the model simulations are carried out for three hypothetical cases that make assumptions regarding landscape properties (uniform, a systematic trend, and heterogeneity plus the trend), repeating these simulations under wet and dry antecedent conditions. The simulations produced expected and also surprising results. The power law relationship between the peak of the IRF and drainage area is shown to be flatter under wet conditions than under dry conditions, even though the (faster) saturation excess mechanism is more dominant under wet conditions. This result appears to be caused by partial area runoff generation: under wet conditions, the fraction of saturation area is about 30%, while under dry conditions it is less than 10% for the same input of rainfall. This means travel times associated with overland flow (which mostly contributes to the peak and time to peak) are, in fact, longer during wet conditions than during dry conditions. The power law relationship between peak and drainage area also exhibits a scaling break at around 1000 km(2), which can be shown to be related to the peculiar geomorphology of the catchment. C1 [Li, Hongyi; Sivapalan, Murugesu] Univ Illinois, Dept Civil & Environm Engn, Urbana, IL 61801 USA. [Sivapalan, Murugesu] Univ Illinois, Dept Geog, Urbana, IL 61801 USA. [Sivapalan, Murugesu] Delft Univ Technol, Dept Water Management, Fac Civil Engn & Geosci, Delft, Netherlands. RP Li, HY (reprint author), Pacific NW Natl Lab, Hydrol Tech Grp, POB 999, Richland, WA 99352 USA. EM hongyi.li@pnl.gov RI Sivapalan, Murugesu/A-3538-2008; Li, Hong-Yi/C-9143-2014 OI Sivapalan, Murugesu/0000-0003-3004-3530; Li, Hong-Yi/0000-0001-5690-3610 FU DMIP2 team at the National Weather Service, NOAA; University of Illinois; National Science Foundation [NSF EFRI-0835982] FX We are grateful to the DMIP2 team at the National Weather Service, NOAA, for providing most of the data used in this study and for providing financial support to attend DMIP2 meetings. The research was partly funded by financial support provided by the University of Illinois through the AESIS project (Barbara Minsker, PI) and by the National Science Foundation (NSF EFRI-0835982, Ximing Cai, PI). This support is gratefully acknowledged. We dedicate this paper to Steve Burges for his significant and diverse contributions to hydrology over an illustrious 40 year career. NR 30 TC 17 Z9 17 U1 2 U2 15 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 J9 WATER RESOUR RES JI Water Resour. Res. PD MAY 26 PY 2011 VL 47 AR W00H08 DI 10.1029/2010WR009712 PG 20 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA 770TH UT WOS:000291110900003 ER PT J AU Xiao, HY Weber, WJ AF Xiao, H. Y. Weber, W. J. TI Oxygen Vacancy Formation and Migration in CexTh1-xO2 Solid Solution SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID DENSITY-FUNCTIONAL CALCULATION; GROUND-STATE PROPERTIES; ELECTRONIC-STRUCTURE; 1ST PRINCIPLES; ACTINIDE DIOXIDES; THORIUM-DIOXIDE; CERIUM DIOXIDE; CEO2 SURFACES; BULK MODULUS; THO2 AB A local-density approximation with the Hubbard U correction (LDA+U) method has been employed to investigate oxygen vacancy formation and migration in CexTh1-xO2. The addition of CeO2 into ThO2 significantly decreases the oxygen vacancy formation and migration energies. ThO2 containing 50% CeO2 exhibits the lowest calculated formation energy, 3.7 eV, and the lowest calculated migration energy, 0.2 eV, occurs for a CeO2 content of 75%, suggesting that introducing CeO2 into ThO2 promotes the formation of mobile oxygen vacancies. If the ceria content is less than about 35%, the reduced CexTh1-xO2 becomes antiferromagnetic (AFM), whereas the ferromagnetic (FM) state dominates for x values above about 35%, which may allow the tailoring of magnetic properties by varying the CeO2 content. C1 [Xiao, H. Y.; Weber, W. J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Weber, W. J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Xiao, HY (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RI Xiao, Haiyan/A-1450-2012; Weber, William/A-4177-2008 OI Weber, William/0000-0002-9017-7365 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX This work was supported as part of the Materials Science of Actinides, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. The theoretical calculations were performed using the supercomputer resources at the Environmental Molecular Sciences Laboratory located at Pacific Northwest National Laboratory, and the National Energy Research Scientific Computing Center located at Lawrence Berkeley National Laboratory. NR 78 TC 29 Z9 29 U1 4 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 26 PY 2011 VL 115 IS 20 BP 6524 EP 6533 DI 10.1021/jp202016s PG 10 WC Chemistry, Physical SC Chemistry GA 764SE UT WOS:000290652100016 PM 21542655 ER PT J AU Han, SP van Duin, ACT Goddard, WA Strachan, A AF Han, Si-ping van Duin, Adri C. T. Goddard, William A., III Strachan, Alejandro TI Thermal Decomposition of Condensed-Phase Nitromethane from Molecular Dynamics from ReaxFF Reactive Dynamics SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID FORCE-FIELD; LIQUID NITROMETHANE; AB-INITIO; SIMULATIONS; DETONATION; MECHANISM; PRESSURE; HYDROCARBONS; KINETICS; OXIDE AB We studied the thermal decomposition and subsequent reaction of the energetic material nitromethane (CH3NO2) using molecular dynamics with ReaxFF, a first principles-based reactive force field. We characterize the chemistry of liquid and solid nitromethane at high temperatures (2000-3000 K) and density 1.97 g/cm(3) for times up to 200 ps. At T = 3000 K the first reaction in the decomposition of nitromethane is an intermolecular proton transfer leading to CH3NOOH and CH2NO2. For lower temperatures (T = 2500 and 2000 K) the first reaction during decomposition is often an isomerization reaction involving the scission of the C-N bond the formation of a C-O bond to form methyl nitrate (CH3ONO). Also at very early times we observe intramolecular proton transfer events. The main product of these reactions is H2O which starts forming following those initiation steps. The appearance of H2O marks the beginning of the exothermic chemistry. Recent quantum-mechanics-based molecular dynamics simulations on the chemical reactions and time scales for decomposition of a crystalline sample heated to T = 3000 K for a few picoseconds are in excellent agreement with our results, providing an important, direct validation of ReaxFF. C1 [Strachan, Alejandro] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. [Han, Si-ping] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Han, Si-ping; van Duin, Adri C. T.; Goddard, William A., III] CALTECH, Mat & Proc Simulat Ctr, Beckman Inst 139 74, Pasadena, CA 91125 USA. RP Strachan, A (reprint author), Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. EM strachan@purdue.edu FU Seaborg Institute; ASC Materials and Physics modeling project; DARPA; ONR [N00014-09-1-0634]; LANL [65287-001-08] FX S.H. would like to thank the Seaborg Institute for a summer fellowship, Jason Keith for preparation of the ReaxFF training set, and P.W.K. Rothemund for help in formatting the manuscript. Work at Los Alamos was supported by the ASC Materials and Physics modeling project and DARPA (program manager Carey Schwatz). Work at Caltech is supported by ONR (N00014-09-1-0634, program manager Cliff Bedford), LANL (65287-001-08, program manager Ed Kober), and DARPA (program manager Carey Schwatz). NR 31 TC 43 Z9 52 U1 6 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 26 PY 2011 VL 115 IS 20 BP 6534 EP 6540 DI 10.1021/jp1104054 PG 7 WC Chemistry, Physical SC Chemistry GA 764SE UT WOS:000290652100017 PM 21542572 ER PT J AU White, CE Provis, JL Proffen, T van Deventer, JSJ AF White, Claire E. Provis, John L. Proffen, Thomas van Deventer, Jannie S. J. TI Quantitative Mechanistic Modeling of Silica Solubility and Precipitation during the Initial Period of Zeolite Synthesis SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID MONTE-CARLO-SIMULATION; PRECURSOR NANOPARTICLES; HYDROTHERMAL SYNTHESIS; ALKALINE-SOLUTIONS; NETWORK FORMATION; DISSOLUTION; DIFFUSION; SYSTEM; CRYSTALLIZATION; CYCLIZATION AB The mechanistic details of the structural changes occurring during the initial stages of silica polymerization to form gels or zeolites remain largely unknown due mainly to the complexity of sol gel synthesis processes. Previous simulation studies have applied simple lattice models to qualitatively replicate spontaneous silica nanoparticle formation using fitted interaction energy parameters to replicate the behavior of real systems. This study moves for the first time to the use of quantum chemical-based interaction (dimerization) energies, determined through density functional theory computations, in a coarse-grained Monte Carlo simulation of the initial stages of gel/cluster formation in sodium silicate systems across a range of concentrations. The use of accurate dimerization energies as model inputs enables setniquantitatively accurate results to be obtained, as determined by comparisons with Si-29 nuclear magnetic resonance data. The most concentrated system simulated (9.36 m silica concentration) undergoes Ostwald ripening, whereby a single large cluster forms, indicative of colloidal silica formation. Furthermore, as the extent of the reaction progresses, this initial nonequilibrated cluster (known as the primary amorphous phase in the zeolite synthesis literature) is progressively transformed to the secondary amorphous phase via structural rearrangements, without significant changes in the overall size of the cluster. These results are in good agreement with previous experimental studies on the nature of the amorphous phase (s) present during silicate gelation and prior to zeolite crystallintion. Hence, this investigation demonstrates for the first time the successful application of multiscale simulation methodology to the coarse-grained Monte Carlo approach of a sot gel process, revealing important quantitative mechanistic information regarding complex silicate reaction processes. C1 [White, Claire E.; Provis, John L.; van Deventer, Jannie S. J.] Univ Melbourne, Dept Chem & Biomol Engn, Melbourne, Vic 3010, Australia. [White, Claire E.; Proffen, Thomas] Los Alamos Natl Lab, Lujan Neutron Scattering Ctr, Los Alamos, NM 87545 USA. RP Provis, JL (reprint author), Univ Melbourne, Dept Chem & Biomol Engn, Melbourne, Vic 3010, Australia. EM jprovis@unimelb.edu.au RI White, Claire/A-1722-2011; Lujan Center, LANL/G-4896-2012; Provis, John/A-7631-2008; Proffen, Thomas/B-3585-2009 OI White, Claire/0000-0002-4800-7960; Provis, John/0000-0003-3372-8922; Proffen, Thomas/0000-0002-1408-6031 FU Australian Research Council (ARC) via the Particulate Fluids Processing Centre, a Special Research Centre; Centre for Sustainable Resource Processing via the Geopolymer Alliance FX The authors would like to thank Dr. Daniel Riley, University of Melbourne/Australian Nuclear Science and Technology Organisation, for computational hardware support and insightful discussions. This work was funded in part by the Australian Research Council (ARC) (including some funding via the Particulate Fluids Processing Centre, a Special Research Centre of the ARC), and in part by a studentship paid to Claire White by the Centre for Sustainable Resource Processing via the Geopolymer Alliance. NR 44 TC 15 Z9 15 U1 4 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2011 VL 115 IS 20 BP 9879 EP 9888 DI 10.1021/jp2006217 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 764SF UT WOS:000290652200007 ER PT J AU Sasaki, K Kuttiyiel, KA Barrio, L Su, D Frenkel, AI Marinkovic, N Mahajan, D Adzic, RR AF Sasaki, Kotaro Kuttiyiel, Kurian A. Barrio, Laura Su, Dong Frenkel, Anatoly I. Marinkovic, Nebojsa Mahajan, Devinder Adzic, Radoslav R. TI Carbon-Supported IrNi Core-Shell Nanoparticles: Synthesis, Characterization, and Catalytic Activity SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; PLATINUM MONOLAYER; SURFACE SEGREGATION; ELECTROCATALYSTS; REDUCTION; EXAFS; TRANSITION; STABILITY; ALLOYS; GROWTH AB We synthesized carbon-supported IrNi core- shell nanoparticles by chemical reduction and subsequent thermal annealing in H(2), and verified the formation of Ir shells on IrNi solid solution alloy cores by various experimental methods. The EXAFS analysis is consistent with the model wherein the IrNi nanoparticles are composed of two-layer Ir shells and IrNi alloy cores. In situ XAS revealed that the Ir shells completely protect Ni atoms in the cores from oxidation or dissolution in an acid electrolyte under elevated potentials. The formation of Ir shell during annealing due to thermal segregation is monitored by time-resolved synchrotron XRD measurements, coupled with Rietveld refinement analyses. The H(2) oxidation activity of the IrNi nanoparticles was found to be higher than that of a commercial Pt/C catalyst. This is predominantly due to Ni-core-induced Ir shell contraction that makes the surface less reactive for IrOH formation, and the resulting more metallic Ir surface becomes more active for H(2) oxidation. This new class of core shell nanopartides appears promising for application as hydrogen anode fuel cell electrocatalysts. C1 [Sasaki, Kotaro; Kuttiyiel, Kurian A.; Barrio, Laura; Adzic, Radoslav R.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Mahajan, Devinder] Brookhaven Natl Lab, Dept Energy Sci, Upton, NY 11973 USA. [Frenkel, Anatoly I.] Yeshiva Univ, Dept Phys, New York, NY 10016 USA. [Marinkovic, Nebojsa] Univ Delaware, Dept Chem Engn, Newark, DE 19716 USA. RP Sasaki, K (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM ksasaki@bnl.gov RI Frenkel, Anatoly/D-3311-2011; Barrio, Laura/A-9509-2008; Su, Dong/A-8233-2013; Marinkovic, Nebojsa/A-1137-2016; OI Frenkel, Anatoly/0000-0002-5451-1207; Barrio, Laura/0000-0003-3496-4329; Su, Dong/0000-0002-1921-6683; Marinkovic, Nebojsa/0000-0003-3579-3453; Barrio, Laura/0000-0002-6919-6414 FU U.S. Department of Energy, Divisions of Chemical and Material Sciences [DE-AC02-98CH10886]; DOE BES [DE-FG02-03ER15476]; Synchrotron Catalysis Consortium, U.S. Department of Energy [DE-FG02-05ER15688] FX This work is supported by U.S. Department of Energy, Divisions of Chemical and Material Sciences under the Contract No. DE-AC02-98CH10886. A.I.F. acknowledges support by DOE BES Grant DE-FG02-03ER15476. Beamlines X19A and X18B at the NSLS are supported in part by the Synchrotron Catalysis Consortium, U.S. Department of Energy Grant No DE-FG02-05ER15688. NR 45 TC 17 Z9 17 U1 3 U2 54 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2011 VL 115 IS 20 BP 9894 EP 9902 DI 10.1021/jp200746j PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 764SF UT WOS:000290652200009 ER PT J AU Moon, HG Shim, YS Su, D Park, HH Yoon, SJ Jang, HW AF Moon, Hi Gyu Shim, Young-Seok Su, Dong Park, Hyung-Ho Yoon, Seok-Jin Jang, Ho Won TI Embossed TiO2 Thin Films with Tailored Links between Hollow Hemispheres: Synthesis and Gas-Sensing Properties SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SENSOR APPLICATIONS; HYDROGEN SENSOR; METAL-OXIDES; TEMPLATES; NANOBELTS; NANOWIRES; NANOSTRUCTURES; PERFORMANCE; FABRICATION; NANOFIBERS AB Embossed TiO2 thin films with high surface areas were achieved using soft templates composed of monolayer polystyrene beads. The structure of links between beads in the templates could be controlled by varying O-2 plasma etching time, resulting in a variety of templates with close-linked, nanolinked, or isolated beads. Room-temperature deposition of TiO2 on the plasma-treated templates and calcination at 550 degrees C resulted in embossed films with tailored links between anatase TiO2 hollow hemispheres. Although all embossed TiO2 films displayed a similar increase in the surface-to-volume ratio compared with a plain TiO2 thin film, the response of embossed TiO2 films with nanolinked hollow hemispheres to CO or ethanol gases was much higher than the response of films with close-linked or isolated. hollow hemispheres. The strong correlation between gas sensitivity and the structure of links between the TiO2 hollow hemispheres revealed the critical importance of tailoring links between individual oxide nanostructures for enhancing gas-sensing properties of the ensemble of the individual nanostructures. The facile and large-scale synthesis of embossed TiO2 films with nanolinked hollow hemispheres on Si substrates and the high sensitivity that is achieved without the aid of additives provide a sustainable competitive advantage over other methods for fabricating highly sensitive metal oxide gas sensors. C1 [Moon, Hi Gyu; Shim, Young-Seok; Yoon, Seok-Jin; Jang, Ho Won] Korea Inst Sci & Technol, Ctr Elect Mat, Seoul 136791, South Korea. [Moon, Hi Gyu; Park, Hyung-Ho] Yonsei Univ, Dept Mat Sci & Engn, Seoul 120749, South Korea. [Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Jang, HW (reprint author), Korea Inst Sci & Technol, Ctr Elect Mat, Seoul 136791, South Korea. EM hwjang@kist.re.kr RI Su, Dong/A-8233-2013; Jang, Ho Won/D-9866-2011 OI Su, Dong/0000-0002-1921-6683; Jang, Ho Won/0000-0002-6952-7359 FU Korea Ministry of Intelligence and Economy [K0004114]; KIST [2E22121]; U.S. Department of Energy, Office of Basic Energy Science [DE-AC02-98CH10886] FX This work was financially supported by the Core Technology of Materials Research and Development Program of the Korea Ministry of Intelligence and Economy (grant no. K0004114) and a KIST research program (grant no. 2E22121). We thank Mr. Kisslinger for his help with TEM sample preparation. The work of D.S. was supported by the U.S. Department of Energy, Office of Basic Energy Science, under contract no. DE-AC02-98CH10886. NR 43 TC 28 Z9 28 U1 2 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2011 VL 115 IS 20 BP 9993 EP 9999 DI 10.1021/jp2020325 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 764SF UT WOS:000290652200021 ER PT J AU Dolocan, A Acharya, DP Zahl, P Sutter, P Camillone, N AF Dolocan, A. Acharya, D. P. Zahl, P. Sutter, P. Camillone, N., III TI Two-Color Ultrafast Photoexcited Scanning Tunneling Microscopy SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RESOLVED 2-PHOTON PHOTOEMISSION; PHOTOELECTRON EMISSION; ELECTRON DYNAMICS; THERMAL-EXPANSION; PROBE MICROSCOPY; RESOLUTION; SURFACES; PULSE; RELAXATION; CU(110) AB We report on two-color two-photon photoexcitation of a metal surface driven by ultrafast laser pulses and detected with a scanning tunneling microscope (STM) tip as a proximate anode. Results are presented for two cases: (i) where the tip is retracted from the surface far enough to prohibit tunneling, and (ii) where the tip is within tunneling range of the surface. A delay-modulation technique is implemented to isolate the two-color photoemission from concurrent one-color two-photon photoemission and provide subpicosecond time-resolved detection. When applied with the tip in tunneling range, this approach effectively isolates the two-photon photoexcited current signal from the conventional tunneling current and enables subpicosecond time-resolved detection of the photoexcited surface electrons. The advantage of the two-color approach is highlighted by comparison with the one-color case where optical interference causes thermal modulation of the STM tip length, resulting in tunneling current modulations that are orders of magnitude larger than the current due to photoexcitation of surface electrons. By completely eliminating this interference, and thereby avoiding thermal modulation of the STM tip length, the two-color approach represents an important step toward the ultimate goal of simultaneous subnanometer and subpicosecond measurements of surface electron dynamics by ultrafast-laser-excited STM. C1 [Dolocan, A.; Camillone, N., III] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Acharya, D. P.; Zahl, P.; Sutter, P.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Camillone, N (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM nicholas@bnl.gov RI Zahl, Percy/B-1244-2008 OI Zahl, Percy/0000-0002-6629-7500 FU Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences [DE-AC02-98CH10886] FX We gratefully acknowledge M. G. White and J. Zhou for their help with frequency doubling. We also thank G. Hall and A. Harris for helpful discussions. The experiments were carried out at the Center for Functional Nanomaterials, a Nanoscale Science Research Center supported by the Office of Basic Energy Sciences, U.S. Department of Energy. The research was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, under Contract No. DE-AC02-98CH10886 as part of a Chemical Imaging initiative within the Catalysis Science Program. NR 43 TC 14 Z9 14 U1 3 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2011 VL 115 IS 20 BP 10033 EP 10043 DI 10.1021/jp111875f PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 764SF UT WOS:000290652200027 ER PT J AU Pan, YX Mei, DH Liu, CJ Ge, QF AF Pan, Yun-xiang Mei, Donghai Liu, Chang-jun Ge, Qingfeng TI Hydrogen Adsorption on Ga2O3 Surface: A Combined Experimental and Computational Study SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID GAMMA-ALUMINA SURFACES; AUGMENTED-WAVE METHOD; GALLIUM OXIDE; OXYGEN VACANCY; BETA-GA2O3; PHOTOCATALYST; POLYMORPHS; CO2; DECOMPOSITION; GAMMA-GA2O3 AB In the present work, hydrogen adsorption on the Ga2O3 surfaces was investigated using Fourier transform infrared spectroscopy (FTIR) measurements and periodic density functional theory (DFT) calculations. Both the FTIR and DFT studies suggest that H-2 dissociates on the Ga2O3 surfaces, producing OH and GaH species. The FTIR bands at 3730, 3700, 3630, and 3600 cm(-1) are attributed to the vibration of the OH species whereas those at 2070 and 1990 cm(-1) to the GaH species. The structures of the species detected in experiments are established through a comparison with the DFT calculated stretching frequencies. The O atom of the experimentally detected OH species is believed to originate from the three-coordinated surface O atom. However, the H adatom that binds the coordinately unsaturated Ga atom results in the experimentally detected GaH species. Dissociative adsorption of H-2 on the perfect Ga2O3 surface, with the formation of both OH and GaH species, is endothermic and has an energy barrier of 0.90 eV. In contrast, dissociative adsorption of H-2 on the defective Ga2O3 surface with oxygen vacancies, which mainly produces GaH species, is exothermic, with an energy barrier of 0.61 eV. Accordingly, presence of the oxygen vacancies promotes H-2 dissociation and production of GaH species on the Ga2O3 surfaces. Higher temperatures are expected to favor oxygen vacancy creation on the Ga2O3 surfaces and thereby benefit the production of GaH species. This analysis is consistent with the FTIR results that the bands assigned to GaH species become stronger at higher temperatures. C1 [Pan, Yun-xiang; Liu, Chang-jun] Tianjin Univ, Sch Chem Engn, Adv Nano Technol Ctr, Tianjin 300072, Peoples R China. [Mei, Donghai] Pacific NW Natl Lab, Inst Interfacial Catalysis, Richland, WA 99352 USA. [Ge, Qingfeng] So Illinois Univ, Dept Chem & Biochem, Carbondale, IL 62901 USA. RP Liu, CJ (reprint author), Tianjin Univ, Sch Chem Engn, Adv Nano Technol Ctr, Tianjin 300072, Peoples R China. EM ughg_cjl@yahoo.com; qge@chem.siu.edu RI Mei, Donghai/D-3251-2011; Ge, Qingfeng/A-8498-2009; Mei, Donghai/A-2115-2012; Pan, Yun-xiang/G-6904-2015; OI Ge, Qingfeng/0000-0001-6026-6693; Mei, Donghai/0000-0002-0286-4182; Liu, Chang-jun/0000-0001-9918-1638 FU National Natural Science Foundation of China [20990223]; Pacific Northwest National Laboratory (PNNL); National Energy Research Scientific Computing Center (NERSC) [752] FX We gratefully acknowledge the support from the National Natural Science Foundation of China (#20990223). D. Mei was supported by a Laboratory Directed Research and Development (LDRD) project at Pacific Northwest National Laboratory (PNNL). The computations were performed using the Molecular Science Computing Facility in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), which is a U.S. Department of Energy national scientific user facility located at PNNL in Richland, Washington. Part of the computing time was also granted by the National Energy Research Scientific Computing Center (NERSC) under project No. 752. NR 36 TC 18 Z9 19 U1 4 U2 62 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2011 VL 115 IS 20 BP 10140 EP 10146 DI 10.1021/jp2014226 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 764SF UT WOS:000290652200039 ER PT J AU Priyadarshini, D Kondratyuk, P Picard, YN Morreale, BD Gellman, AJ Miller, JB AF Priyadarshini, Deepika Kondratyuk, Petro Picard, Yoosuf N. Morreale, Bryan D. Gellman, Andrew J. Miller, James B. TI High-Throughput Characterization of Surface Segregation in CuxPd1-x Alloys SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID POLYCRYSTALLINE PD70CU30 ALLOY; SINGLE-CRYSTAL ALLOY; CU-PD SYSTEM; AG-AU ALLOYS; HYDROGEN SEPARATION; ELEVATED-TEMPERATURES; COMPOSITE MEMBRANES; COMPOSITION SPREADS; TERNARY ALLOYS; BINARY-ALLOYS AB A high throughput methodology for the study of surface segregation in alloys has been developed and applied to the CuxPd1-x system. A novel offset-filament deposition tool was used to prepare CuxPd1-x composition spread alloy films (CSAFs), high throughput sample libraries with continuous lateral composition variation spanning the range x = 0.05-0.95. Spatially resolved low energy ion scattering spectroscopy (LEISS) and X-ray photoelectron spectroscopy (XPS) were used to characterize the films' top-surface and near-surface compositions, respectively, as functions of alloy composition, x, and temperature. Electron backscatter diffraction (EBSD) was used to identify the bulk phases in the CSAF as a function of alloy composition, x. Films equilibrated by annealing at temperatures >= 700 K displayed preferential segregation of Cu to their top-surfaces at all bulk compositions; segregation patterns did not, however, depend on local structure. The Langmuir-McLean thermodynamic model was applied to segregation measurements made in the temperature range 700-900 K in order to estimate the enthalpy (Delta H-seg) and entropy (Delta S-seg) of segregation as a function of bulk CuxPd1-x composition. Segregation measurements at x = 0.30 on the CSAF compare well with results previously reported for a bulk, polycrystalline Cu0.30Pd0.70 alloy, demonstrating the utility of the CSAF as a high throughput library for study of segregation. C1 [Priyadarshini, Deepika; Kondratyuk, Petro; Morreale, Bryan D.; Gellman, Andrew J.; Miller, James B.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Priyadarshini, Deepika; Kondratyuk, Petro; Gellman, Andrew J.; Miller, James B.] Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA. [Picard, Yoosuf N.] Carnegie Mellon Univ, Dept Mat Sci & Engn, Pittsburgh, PA 15213 USA. RP Miller, JB (reprint author), US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. EM jbmiller@andrew.cmu.edu RI Gellman, Andrew/M-2487-2014; OI Gellman, Andrew/0000-0001-6618-7427; Picard, Yoosuf/0000-0002-2853-5213 FU National Energy Technology Laboratory's ongoing research in Computational and Basic Sciences under RDS [DE-AC26-04NT41817]; RDS [DE-FE0004000] FX This technical effort was performed in support of the National Energy Technology Laboratory's ongoing research in Computational and Basic Sciences under RDS Contract DE-AC26-04NT41817 and RDS contract DE-FE0004000. NR 72 TC 19 Z9 19 U1 5 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2011 VL 115 IS 20 BP 10155 EP 10163 DI 10.1021/jp201793d PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 764SF UT WOS:000290652200041 ER PT J AU Presiado, I Lal, J Mamontov, E Kolesnikov, AI Huppert, D AF Presiado, Itay Lal, Jyotsana Mamontov, Eugene Kolesnikov, Alexander I. Huppert, Dan TI Fast Proton Hopping Detection in Ice I-h by Quasi-Elastic Neutron Scattering SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DOPED ICE; HYDROCHLORIC-ACID; ISOTOPIC EXCHANGE; ELEMENTARY STEPS; LIQUID WATER; DIFFUSION; DYNAMICS; CONDUCTIVITY; MECHANISM; MOBILITY AB Quasi-elastic neutron scattering was employed on samples of HCl-doped polycrystalline ice I-h. The analysis of the scattering signal provides the excess proton hopping time, tau(hop), in the temperature range of 140-195 K. The hopping time strongly depends on the temperature of the sample, and the activation energy of a hopping step is 17 kJ/mol. The values of tau(hop) of the current experiment are in good agreement with calculated values derived from previous photochemical experiments,(1) in which we found that the proton hopping time at T > 242 K is on the order of 200 fs, roughly 10 times shorter than in liquid water at room temperature. C1 [Presiado, Itay; Huppert, Dan] Tel Aviv Univ, Raymond & Beverly Sackler Fac Exact Sci, Sch Chem, IL-69978 Tel Aviv, Israel. [Lal, Jyotsana] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Mamontov, Eugene; Kolesnikov, Alexander I.] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. RP Huppert, D (reprint author), Tel Aviv Univ, Raymond & Beverly Sackler Fac Exact Sci, Sch Chem, IL-69978 Tel Aviv, Israel. EM huppert@tulip.tau.ac.il RI Kolesnikov, Alexander/I-9015-2012; Mamontov, Eugene/Q-1003-2015 OI Kolesnikov, Alexander/0000-0003-1940-4649; Mamontov, Eugene/0000-0002-5684-2675 FU Israel Science Foundation; James-Franck German-Israeli Program; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy [DE-AC0500OR22725]; US DOE-BES [DE-AC02-06CH11357] FX This work was supported by grants from the Israel Science Foundation and from the James-Franck German-Israeli Program in Laser-Matter Interaction. The experiment at Oak Ridge National Laboratory's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; ORNL is managed by UT-Batelle, LLC, under contract DE-AC0500OR22725 for the U.S. Department of Energy. Work at ANL was performed under the auspices of the US DOE-BES under contract DE-AC02-06CH11357. NR 43 TC 17 Z9 17 U1 0 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2011 VL 115 IS 20 BP 10245 EP 10251 DI 10.1021/jp2008094 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 764SF UT WOS:000290652200052 ER PT J AU DiMaio, F Terwilliger, TC Read, RJ Wlodawer, A Oberdorfer, G Wagner, U Valkov, E Alon, A Fass, D Axelrod, HL Das, D Vorobiev, SM Iwai, H Pokkuluri, PR Baker, D AF DiMaio, Frank Terwilliger, Thomas C. Read, Randy J. Wlodawer, Alexander Oberdorfer, Gustav Wagner, Ulrike Valkov, Eugene Alon, Assaf Fass, Deborah Axelrod, Herbert L. Das, Debanu Vorobiev, Sergey M. Iwai, Hideo Pokkuluri, P. Raj Baker, David TI Improved molecular replacement by density- and energy-guided protein structure optimization SO NATURE LA English DT Article ID LOW-RESOLUTION; CRYSTALLOGRAPHIC REFINEMENT; SOFTWARE; PREDICTION; ACCURACY; ROSETTA AB Molecular replacement(1-4) procedures, which search for placements of a starting model within the crystallographic unit cell that best account for the measured diffraction amplitudes, followed by automatic chain tracing methods(5-8), have allowed the rapid solution of large numbers of protein crystal structures. Despite extensive work(9-14), molecular replacement or the subsequent rebuilding usually fail with more divergent starting models based on remote homologues with less than 30% sequence identity. Here we show that this limitation can be substantially reduced by combining algorithms for protein structure modelling with those developed for crystallographic structure determination. An approach integrating Rosetta structure modelling with Autobuild chain tracing yielded high-resolution structures for 8 of 13 X-ray diffraction data sets that could not be solved in the laboratories of expert crystallographers and that remained unsolved after application of an extensive array of alternative approaches. We estimate that the new method should allow rapid structure determination without experimental phase information for over half the cases where current methods fail, given diffraction data sets of better than 3.2 angstrom resolution, four or fewer copies in the asymmetric unit, and the availability of structures of homologous proteins with >20% sequence identity. C1 [Terwilliger, Thomas C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [DiMaio, Frank; Baker, David] Univ Washington, Dept Biochem, Seattle, WA 98195 USA. [DiMaio, Frank; Baker, David] Univ Washington, Howard Hughes Med Inst, Seattle, WA 98195 USA. [Read, Randy J.] Univ Cambridge, Dept Haematol, Cambridge Inst Med Res, Cambridge CB2 0XY, England. [Wlodawer, Alexander] NCI, Macromol Crystallog Lab, Frederick, MD 21702 USA. [Oberdorfer, Gustav; Wagner, Ulrike] Graz Univ, Inst Mol Biosci, A-8010 Graz, Austria. [Valkov, Eugene] Univ Cambridge, Dept Biochem, Cambridge CB2 1GA, England. [Alon, Assaf; Fass, Deborah] Weizmann Inst Sci, Dept Biol Struct, IL-76100 Rehovot, Israel. [Axelrod, Herbert L.; Das, Debanu] SLAC Natl Accelerator Lab, Joint Ctr Struct Genom, Menlo Pk, CA 94025 USA. [Axelrod, Herbert L.; Das, Debanu] SLAC Natl Accelerator Lab, SSRL, Menlo Pk, CA 94025 USA. [Vorobiev, Sergey M.] Columbia Univ, NE Struct Genom Consortium, New York, NY 10027 USA. [Iwai, Hideo] Univ Helsinki, Inst Biotechnol, FI-00014 Helsinki, Finland. [Pokkuluri, P. Raj] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. RP Terwilliger, TC (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM terwilliger@lanl.gov; dabaker@u.washington.edu RI Iwai, Hideo/A-6416-2009; Valkov, Eugene/C-1554-2010; Read, Randy/L-1418-2013; Terwilliger, Thomas/K-4109-2012; Baker, David/K-8941-2012 OI Iwai, Hideo/0000-0001-7376-5264; Read, Randy/0000-0001-8273-0047; Terwilliger, Thomas/0000-0001-6384-0320; Baker, David/0000-0001-7896-6217 FU NIH [5R01GM092802, P41RR002250]; Wellcome Trust; HHMI; Israel Science Foundation; DK Molecular Enzymology [W901]; Austrian Science Fund [P19858]; NIH, National Cancer Institute, Center for Cancer Research; academy of Finland [1131413]; Protein Structure Initiative of National Institute of General Medical Sciences [U54 GM074958]; US Department of Energy's Office of Science, Biological and Environmental Research [DE-AC02-06CH11357]; NIH, National Institutes of General Medical Sciences, Protein Structure Initiative [U54 GM094586, GM074898] FX R.J.R., T.C.T. and D.B. thank the NIH (5R01GM092802), the Wellcome Trust (R.J.R.), and HHMI (D.B.) for funding this research. F.D. acknowledges the NIH (P41RR002250) and HHMI. D.F. and A.A. acknowledge support from the Israel Science Foundation. G.O. thanks DK Molecular Enzymology (FWF-project W901) and the Austrian Science Fund (FWF-project P19858). The work of A.W. was supported by the Intramural Research Program of the NIH, National Cancer Institute, Center for Cancer Research. H.I. acknowledges support from the academy of Finland (1131413). S.M.V. was supported by a grant from the Protein Structure Initiative of National Institute of General Medical Sciences (U54 GM074958). The work of P.R.P. at Argonne National Laboratory was supported by the US Department of Energy's Office of Science, Biological and Environmental Research GTL programme under contract DE-AC02-06CH11357. We thank all members of the JCSG for their general contributions to the protein production and structural work. The JCSG is supported by the NIH, National Institutes of General Medical Sciences, Protein Structure Initiative (U54 GM094586 and GM074898). NR 29 TC 123 Z9 124 U1 2 U2 34 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAY 26 PY 2011 VL 473 IS 7348 BP 540 EP U149 DI 10.1038/nature09964 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 768QM UT WOS:000290951300047 PM 21532589 ER PT J AU Ilie, C Freese, K Spolyar, D AF Ilie, Cosmin Freese, Katherine Spolyar, Douglas TI Dark stars and boosted dark matter annihilation rates SO NEW JOURNAL OF PHYSICS LA English DT Article ID 1ST STARS; FERMI LAT; PAMELA; HALOS; EVOLUTION; POSITRON; MASS; UNIVERSE; TELESCOPE; OPACITIES AB Dark stars (DSs) may constitute the first phase of stellar evolution, powered by dark matter (DM) annihilation. We investigate here the properties of DSs, assuming that the DM particle has the properties required for explaining the excess positron and electron signals in the cosmic rays detected by the PAMELA and FERMI satellites. Any possible DM interpretation of these signals will require exotic DM candidates, with annihilation cross-sections a few orders of magnitude higher than the canonical value required for correct thermal relic abundance for weakly interacting DM candidates; additionally, in most models, the annihilation must be preferentially to leptons. Secondly, we study the dependence of DS properties on the concentration parameter of the initial DM density profile of the halos where the first stars are formed. We restrict our study to the DM in the star due to simple (versus extended) adiabatic contraction and minimal (versus extended) capture; this simple study is sufficient to illustrate dependence on the cross-section and concentration parameter. Our basic results are that the final stellar properties, once the star enters the main sequence, are always roughly the same, regardless of the value of the boosted annihilation or concentration parameter in the range between c = 2 and c = 5: stellar mass similar to 1000M(circle dot), luminosity similar to 10(7)L(circle dot) and lifetime similar to 10(6) years (for the minimal DM models considered here; additional DM would lead to more massive DSs). However, the lifetime, final mass and final luminosity of the DSs show some dependence on the boost factor and concentration parameter, as discussed in this paper. C1 [Ilie, Cosmin; Freese, Katherine] Univ Michigan, Dept Phys, Michigan Ctr Theoret Phys, Ann Arbor, MI 48109 USA. [Spolyar, Douglas] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA. RP Ilie, C (reprint author), Univ Michigan, Dept Phys, Michigan Ctr Theoret Phys, Ann Arbor, MI 48109 USA. EM cilie@umich.edu FU DOE; Michigan Center for Theoretical Physics at the University of Michigan; DOE at Fermilab FX We acknowledge support from the DOE and the Michigan Center for Theoretical Physics at the University of Michigan (to CI and KF) and the DOE at Fermilab (to DS). We thank Pearl Sandick for helpful conversations and the anonymous referees for helpful suggestions for the improvement of the manuscript. NR 123 TC 4 Z9 4 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD MAY 26 PY 2011 VL 13 AR 053050 DI 10.1088/1367-2630/13/5/053050 PG 27 WC Physics, Multidisciplinary SC Physics GA 782IW UT WOS:000292002700001 ER PT J AU Yu, XH Rawat, R Shanklin, J AF Yu, Xiao-Hong Rawat, Richa Shanklin, John TI Characterization and analysis of the cotton cyclopropane fatty acid synthase family and their contribution to cyclopropane fatty acid synthesis SO BMC PLANT BIOLOGY LA English DT Article ID ADENOSYLMETHIONINE-DEPENDENT METHYLTRANSFERASES; AGROBACTERIUM-MEDIATED TRANSFORMATION; MYCOBACTERIUM-TUBERCULOSIS; MYCOLIC ACIDS; STEARIC-ACID; SEED OIL; STERCULIA-FOETIDA; LIPID-COMPOSITION; SEQUENCE MOTIFS; HEN LIVER AB Background: Cyclopropane fatty acids (CPA) have been found in certain gymnosperms, Malvales, Litchi and other Sapindales. The presence of their unique strained ring structures confers physical and chemical properties characteristic of unsaturated fatty acids with the oxidative stability displayed by saturated fatty acids making them of considerable industrial interest. While cyclopropenoid fatty acids (CPE) are well-known inhibitors of fatty acid desaturation in animals, CPE can also inhibit the stearoyl-CoA desaturase and interfere with the maturation and reproduction of some insect species suggesting that in addition to their traditional role as storage lipids, CPE can contribute to the protection of plants from herbivory. Results: Three genes encoding cyclopropane synthase homologues GhCPS1, GhCPS2 and GhCPS3 were identified in cotton. Determination of gene transcript abundance revealed differences among the expression of GhCPS1, 2 and 3 showing high, intermediate and low levels, respectively, of transcripts in roots and stems; whereas GhCPS1 and 2 are both expressed at low levels in seeds. Analyses of fatty acid composition in different tissues indicate that the expression patterns of GhCPS1 and 2 correlate with cyclic fatty acid (CFA) distribution. Deletion of the N-terminal oxidase domain lowered GhCPS's ability to produce cyclopropane fatty acid by approximately 70%. GhCPS1 and 2, but not 3 resulted in the production of cyclopropane fatty acids upon heterologous expression in yeast, tobacco BY2 cell and Arabidopsis seed. Conclusions: In cotton GhCPS1 and 2 gene expression correlates with the total CFA content in roots, stems and seeds. That GhCPS1 and 2 are expressed at a similar level in seed suggests both of them can be considered potential targets for gene silencing to reduce undesirable seed CPE accumulation. Because GhCPS1 is more active in yeast than the published Sterculia CPS and shows similar activity when expressed in model plant systems, it represents a strong candidate gene for CFA accumulation via heterologous expression in production plants. C1 [Yu, Xiao-Hong; Rawat, Richa; Shanklin, John] SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA. [Shanklin, John] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. RP Shanklin, J (reprint author), SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA. EM shanklin@bnl.gov FU Office of Basic Energy Sciences of the U.S. Department of Energy; National Science Foundation [DBI 0701919] FX We thank Dr. Carl Andre at Brookhaven National Laboratory for critical reading of our manuscript, Prof. John Ohlorogge at Michigan State University for SfCPS gene, Prof. Kent Chapman at the University of North Texas for providing us with the cotton seeds, and Mr. Kevin Lutke from Donald Danforth Plant Science Center who helped with the BY2 transformation. This work was supported by the Office of Basic Energy Sciences of the U.S. Department of Energy (JS), and by the National Science Foundation (Grant DBI 0701919) (RR and X-HY). NR 48 TC 13 Z9 14 U1 1 U2 32 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2229 J9 BMC PLANT BIOL JI BMC Plant Biol. PD MAY 25 PY 2011 VL 11 AR 97 DI 10.1186/1471-2229-11-97 PG 10 WC Plant Sciences SC Plant Sciences GA 789ZN UT WOS:000292558400001 PM 21612656 ER PT J AU Hin, C Lepinoux, J Neaton, JB Dresselhaus, M AF Hin, Celine Lepinoux, Joel Neaton, Jeffrey B. Dresselhaus, Mildred TI From the interface energy to the solubility limit of aluminium in nickel from first-principles and Kinetic Monte Carlo calculations SO MATERIALS SCIENCE AND ENGINEERING B-ADVANCED FUNCTIONAL SOLID-STATE MATERIALS LA English DT Article DE Phase diagrams; First-principles calculations; Interface energy ID WAVE BASIS-SET; AL-NI SYSTEM; COHESIVE ENERGY; SURFACE-TENSION; BINARY-ALLOYS; METALS; PHASE; NI3AL; BOUNDARIES; MODEL AB We developed a way to predict the solubility limit of solute atoms in a binary alloy using a Kinetic Monte Carlo algorithm. The idea is to use the interface energies calculated by first-principles calculations to parameterize the pair interaction energies used in the Kinetic Monte Carlo algorithm. In order to validate this method, it was tested on a very well known case: the Ni-Al alloy. We found that the calculations are in very good agreement with the previously calculated phase diagrams. (C) 2011 Elsevier B.V. All rights reserved. C1 [Hin, Celine] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Lepinoux, Joel] UJF, CNRS, Grenoble INP, SIMaP, F-38402 St Martin Dheres, France. [Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Lab, Mol Foundry, Berkeley, CA 94720 USA. [Dresselhaus, Mildred] MIT, Dept Phys, Cambridge, MA 02139 USA. RP Hin, C (reprint author), MIT, Dept Mech Engn, Cambridge, MA 02139 USA. EM celine_hin@yahoo.fr RI Neaton, Jeffrey/F-8578-2015 OI Neaton, Jeffrey/0000-0001-7585-6135 FU Department of Energy [DE-FG02-08ER46516] FX We gratefully acknowledge useful and stimulating discussions with Professor W.C. Carter. The authors gratefully acknowledge the financial support of the Department of Energy under Grant DE-FG02-08ER46516. NR 45 TC 3 Z9 3 U1 3 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-5107 J9 MATER SCI ENG B-ADV JI Mater. Sci. Eng. B-Adv. Funct. Solid-State Mater. PD MAY 25 PY 2011 VL 176 IS 9 BP 767 EP 771 DI 10.1016/j.mseb.2011.02.023 PG 5 WC Materials Science, Multidisciplinary; Physics, Condensed Matter SC Materials Science; Physics GA 779DE UT WOS:000291757500014 ER PT J AU Li, ADQ Zhan, CL Hu, DH Wan, W Yao, JN AF Li, Alexander D. Q. Zhan, Chuanlang Hu, Dehong Wan, Wei Yao, Jiannian TI Photoswitchable Nanoprobes Offer Unlimited Brightness in Frequency-Domain Imaging SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID FLUORESCENCE; NANOPARTICLES; RECOVERY AB A single probe has limited brightness in time-domain imaging and such limitation frequently renders individual molecules undetectable in the presence of interference or complex cellular structures. However, a single photoswitchable probe produces a signal, which can be separated from interference or noise using photoswitching-enabled Fourier transformation (PFT). As a result, the light-modulated probes can be made super bright in the frequency domain simply by acquiring more cycles in the time domain. C1 [Li, Alexander D. Q.; Wan, Wei] Washington State Univ, Dept Chem, Pullman, WA 99164 USA. [Li, Alexander D. Q.; Wan, Wei] Washington State Univ, Ctr Mat Res, Pullman, WA 99164 USA. [Zhan, Chuanlang; Yao, Jiannian] Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China. [Hu, Dehong] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Li, ADQ (reprint author), Washington State Univ, Dept Chem, Pullman, WA 99164 USA. EM dequan@wsu.edu RI Zhan, Chuanlang/F-5247-2011; Yao, Jiannian/A-9773-2012; Hu, Dehong/B-4650-2010 OI Zhan, Chuanlang/0000-0001-5127-0973; Hu, Dehong/0000-0002-3974-2963 FU National Science Foundation [CHE-0805547] FX We acknowledge the support of National Science Foundation (CHE-0805547). A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 15 TC 23 Z9 23 U1 3 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 25 PY 2011 VL 133 IS 20 BP 7628 EP 7631 DI 10.1021/ja1108479 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 776ZN UT WOS:000291580400003 PM 21539363 ER PT J AU Bhandari, D Kravchenko, II Lavrik, NV Sepaniak, MJ AF Bhandari, Deepak Kravchenko, Ivan I. Lavrik, Nickolay V. Sepaniak, Michael J. TI Nanotransfer Printing Using Plasma Etched Silicon Stamps and Mediated by in Situ Deposited Fluoropolymer SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ELECTRICAL CONTACTS; FILMS; LITHOGRAPHY; NANOFABRICATION; FABRICATION; THIN AB This communication describes a simple method that uses a thin film of octafluorocyclobutane (OFCB) polymer for efficient nanoscale transfer printing (nTP). Plasma polymerization of OFCB produces a Teflon-like fluoropolymer which strongly adheres and conformally covers a 3-D inorganic stamp. The inherently low surface energy of in situ deposited OFCB polymer on nanoscale silicon features is demonstrated as a unique nanocomposite stamp to fabricate various test structures with improved nTP feature resolution down to sub-100 nm. C1 [Bhandari, Deepak; Sepaniak, Michael J.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Kravchenko, Ivan I.; Lavrik, Nickolay V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Sepaniak, MJ (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM msepaniak@utk.edu RI Kravchenko, Ivan/K-3022-2015; Lavrik, Nickolay/B-5268-2011 OI Kravchenko, Ivan/0000-0003-4999-5822; Lavrik, Nickolay/0000-0002-9543-5634 FU Scientific User Facilities Division, U.S. Department of Energy at Oak Ridge National Laboratory FX A portion of this research was conducted at the Center for Nanophase Materials Sciences (CNMS) and Shared Research Equipment (SHaRE) User Facility, which are sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, U.S. Department of Energy. We thank Dr. H. M. Meyer III for assistance with X-ray photoelectron spectroscopy. NR 20 TC 6 Z9 6 U1 1 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 25 PY 2011 VL 133 IS 20 BP 7722 EP 7724 DI 10.1021/ja201497a PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 776ZN UT WOS:000291580400027 PM 21526774 ER PT J AU Wu, HP Pan, SL Poeppelmeier, KR Li, HY Jia, DZ Chen, ZH Fan, XY Yang, Y Rondinelli, JM Luo, HS AF Wu, Hongping Pan, Shilie Poeppelmeier, Kenneth R. Li, Hongyi Jia, Dianzeng Chen, Zhaohui Fan, Xiaoyun Yang, Yun Rondinelli, James M. Luo, Haosu TI K3B6O10Cl: A New Structure Analogous to Perovskite with a Large Second Harmonic Generation Response and Deep UV Absorption Edge SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID NONLINEAR-OPTICAL CRYSTAL; AUGMENTED-WAVE METHOD; K2AL2B2O7 CRYSTALS; BORATE CRYSTALS; SINGLE-CRYSTALS; KBBF CRYSTAL; GROWTH; RB; POLAR; BI2ZNOB2O6 AB Introduction of the Cl anion in the borate systems generates a new perovskite-like phase, K3B6O10Cl, which exhibits a large second harmonic response, about four times that of KH2PO4 (KDP), and is transparent from the deep UV (180 nm) to middle-IR region. K3B6O10Cl crystallizes in the noncentrosymmetric and rhombohedral space group R3m. The structure consists of the A-site hexaborate [B6O10] groups and the BX3 Cl-centered octahedral [ClK6] groups linked together through vertices to form the perovskite framework represented by ABX(3). C1 [Wu, Hongping; Pan, Shilie; Li, Hongyi; Chen, Zhaohui; Fan, Xiaoyun; Yang, Yun] Chinese Acad Sci, Xinjiang Key Lab Elect Informat Mat & Devices, Xinjiang Tech Inst Phys & Chem, Urumqi 830011, Peoples R China. [Wu, Hongping; Jia, Dianzeng] Xinjiang Univ, Coll Chem & Chem Engn, Urumqi 830046, Peoples R China. [Poeppelmeier, Kenneth R.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Rondinelli, James M.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Luo, Haosu] Chinese Acad Sci, State Key Lab High Performance Ceram & Superfine, Shanghai Inst Ceram, Shanghai 201800, Peoples R China. RP Pan, SL (reprint author), Chinese Acad Sci, Xinjiang Key Lab Elect Informat Mat & Devices, Xinjiang Tech Inst Phys & Chem, 40-1 S Beijing Rd, Urumqi 830011, Peoples R China. EM slpan@ms.xjb.ac.cn; krp@northwestern.edu RI Rondinelli, James/A-2071-2009 OI Rondinelli, James/0000-0003-0508-2175 FU Chinese Academy of Sciences [KJCX2-EW-H03-03]; National Natural Science Foundation of China [50802110, 21001114]; "One Hundred Talents Project Foundation" of Chinese Academy of Sciences; "Western Light Joint Scholar Foundation" of Chinese Academy of Sciences; "High Technology Research and Development Program" of Xinjiang Uygur Autonomous Region of China [200816120]; Scientific Research Program of Urumqi of China [G09212001]; National Science Foundation [DMR-1005827]; U.S. DOE, Office of Science [DE-AC02-06CH11357] FX This work is supported by Main Direction Program of Knowledge Innovation of Chinese Academy of Sciences (Grant No. KJCX2-EW-H03-03), the "National Natural Science Foundation of China" (Grant Nos. 50802110, 21001114), the "One Hundred Talents Project Foundation Program" of Chinese Academy of Sciences, the "Western Light Joint Scholar Foundation" Program of Chinese Academy of Sciences, the "High Technology Research and Development Program" of Xinjiang Uygur Autonomous Region of China (Grant No. 200816120), and Scientific Research Program of Urumqi of China (Grant No. G09212001). K.R.P. acknowledges the National Science Foundation Solid State Chemistry Award No. DMR-1005827. J.M.R. was supported by the U.S. DOE, Office of Science, under Contract No. DE-AC02-06CH11357. Computations were carried out at the Laboratory Computing Resource Center (LCRC) at Argonne National Laboratory. NR 67 TC 224 Z9 228 U1 8 U2 109 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 25 PY 2011 VL 133 IS 20 BP 7786 EP 7790 DI 10.1021/ja111083x PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 776ZN UT WOS:000291580400034 PM 21534555 ER PT J AU Shi, X Yang, J Salvador, JR Chi, MF Cho, JY Wang, H Bai, SQ Yang, JH Zhang, WQ Chen, LD AF Shi, Xun Yang, Jiong Salvador, James R. Chi, Miaofang Cho, Jung Y. Wang, Hsin Bai, Shengqiang Yang, Jihui Zhang, Wenqing Chen, Lidong TI Multiple-Filled Skutterudites: High Thermoelectric Figure of Merit through Separately Optimizing Electrical and Thermal Transports SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID FILLING FRACTION; BULK MATERIALS; COSB3; PERFORMANCE; CONDUCTIVITY; CRYSTALS; DEVICES; BARIUM AB Skutterudites CoSb(3) with multiple cofillers Ba, La, and Yb were synthesized and very high thermoelectric figure of merit ZT = 1.7 at 850 K was realized. X-ray diffraction of the densified multiple-filled bulk samples reveals all samples are phase pure. High-resolution scanning transmission electron microscopy (STEM) and energy dispersive X-ray spectroscopy (EDS) analysis confirm that multiple guest fillers occupy the nanoscale-cages in the skutterudites. The fillers are further shown to be uniformly distributed and the Co-Sb skutterudite framework is virtually unperturbed from atomic scale to a few micrometers. Our results firmly show that high power factors can be realized by adjusting the total filling fraction of fillers with different charge states to reach the optimum carrier density, at the same time, lattice thermal conductivity can also be significantly reduced, to values near the glass limit of these materials, through combining filler species of different rattling frequencies to achieve broad-frequency phonon scattering. Therefore, partially filled skutterudites with multiple fillers of different chemical nature render unique structural characteristics for optimizing electrical and thermal transports in a relatively independent way, leading to continually enhanced ZT values from single- to double-, and finally to multiple-filled skutterudites. The idea of combining multiple fillers with different charge states and rattling frequencies for performance optimization is also expected to be valid for other caged TE compounds. C1 [Yang, Jihui] Gen Motors R&D Ctr, Electrochem Energy Res Lab, Warren, MI 48090 USA. [Shi, Xun; Yang, Jiong; Zhang, Wenqing] Chinese Acad Sci, State Key Lab High Performance Ceram & Superfine, Shanghai Inst Ceram, Shanghai 200050, Peoples R China. [Shi, Xun; Salvador, James R.; Cho, Jung Y.] Gen Motors R&D Ctr, Chem Sci & Mat Syst Lab, Warren, MI 48090 USA. [Chi, Miaofang; Wang, Hsin] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Bai, Shengqiang; Chen, Lidong] Chinese Acad Sci, CAS Key Lab Mat Energy Convers, Shanghai Inst Ceram, Shanghai 200050, Peoples R China. RP Yang, JH (reprint author), Gen Motors R&D Ctr, Electrochem Energy Res Lab, Warren, MI 48090 USA. EM jihui.yang@gm.com; wqzhang@mail.sic.ac.cn; dd@mail.sic.ac.cn RI shi, xun/B-4499-2009; Yang, Jihui/A-3109-2009; Chen, Lidong/F-2705-2010; Zhang, Wenqing/K-1236-2012; Yang, Jiong/K-6330-2014; Chi, Miaofang/Q-2489-2015; Wang, Hsin/A-1942-2013 OI shi, xun/0000-0002-3806-0303; Yang, Jiong/0000-0002-5862-5981; Chi, Miaofang/0000-0003-0764-1567; Wang, Hsin/0000-0003-2426-9867 FU GM; DOE [DE-FC26-04NT42278, DEAC05000OR22725]; National Basic Research Program of China (973-program) [2007CB607503]; NSFC [50825205, 50672118, 50821004, 50820145203, 10634070]; Office of BES, U.S. DOE FX This work is supported by GM and by DOE under corporate agreement DE-FC26-04NT42278, by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Transportation Technologies as part of the High Temperature Materials Laboratory User Program at Oak Ridge National Laboratory managed by the UT-Battelle LLC, for the Department of Energy under contract DEAC05000OR22725, and by National Basic Research Program of China (973-program) under Project No. 2007CB607503 and NSFC projects (50825205, 50672118, 50821004, 50820145203, and 10634070). Microscopy research is supported by ORNL's Shared Research Equipment (SHaRE) User Facility, which is sponsored by the Office of BES, U.S. DOE. NR 57 TC 454 Z9 462 U1 71 U2 398 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 25 PY 2011 VL 133 IS 20 BP 7837 EP 7846 DI 10.1021/ja111199y PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA 776ZN UT WOS:000291580400040 PM 21524125 ER PT J AU Liu, QQ Yu, XH Wang, XC Deng, Z Lv, YX Zhu, JL Zhang, SJ Liu, HZ Yang, WG Wang, L Mao, HW Shen, GY Lu, ZY Ren, Y Chen, ZQ Lin, ZJ Zhao, YS Jin, CQ AF Liu, Qingqing Yu, Xiaohui Wang, Xiancheng Deng, Zheng Lv, Yuxi Zhu, Jinlong Zhang, Sijia Liu, Haozhe Yang, Wenge Wang, Lin Mao, Hokwang Shen, Guoyin Lu, Zhong-Yi Ren, Yang Chen, Zhiqiang Lin, Zhijun Zhao, Yusheng Jin, Changqing TI Pressure-Induced Isostructural Phase Transition and Correlation of FeAs Coordination with the Superconducting Properties of 111-Type Na1-xFeAs SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID IRON ARSENIDE SUPERCONDUCTOR; 43 K; T-C; LIFEAS; COMPOUND AB The effect of pressure on the crystalline structure and superconducting transition temperature (T-c) of the 111-type Na1-xFeAs system using in situ high-pressure synchrotron X-ray powder diffraction and diamond anvil cell techniques is studied. A pressure-induced tetragonal to tetragonal isostructural phase transition was found. The systematic evolution of the FeAs4 tetrahedron as a function of pressure based on Rietveld refinements on the powder X-ray diffraction patterns was obtained. The nonmonotonic T-c(P) behavior of Na1-xFeAs is found to correlate with the anomalies of the distance between the anion (As) and the iron layer as well as the bond angle of As-Fe-As for the two tetragonal phases. This behavior provides the key structural information in understanding the origin of the pressure dependence of T-c for 111-type iron pnictide superconductors. A pressure-induced structural phase transition is also observed at 20 GPa. C1 [Liu, Qingqing; Yu, Xiaohui; Wang, Xiancheng; Deng, Zheng; Lv, Yuxi; Zhu, Jinlong; Zhang, Sijia; Jin, Changqing] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Yu, Xiaohui; Lin, Zhijun; Zhao, Yusheng] Los Alamos Natl Lab, Los Alamos Neutron Sci Ctr LANSCE, Los Alamos, NM 87545 USA. [Liu, Haozhe] Harbin Inst Technol, Nat Sci Res Ctr, Harbin 150080, Peoples R China. [Yang, Wenge; Wang, Lin; Shen, Guoyin] Carnegie Inst Sci, HPSynC, Argonne, IL 60439 USA. [Yang, Wenge; Wang, Lin; Shen, Guoyin] Carnegie Inst Sci, HPCAT, Geophys Lab, Argonne, IL 60439 USA. [Mao, Hokwang] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. [Lu, Zhong-Yi] Renmin Univ China, Dept Phys, Beijing 100872, Peoples R China. [Ren, Yang] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Chen, Zhiqiang] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Jin, CQ (reprint author), Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. EM Jin@iphy.ac.cn RI Liu, Haozhe/E-6169-2011; 石, 源/D-5929-2012; 上官, 敏慧/E-8964-2012; ruc, phy/E-4170-2012; Lujan Center, LANL/G-4896-2012; Yang, Wenge/H-2740-2012; chen, zhiqiang/C-9134-2013; WANG, LIN/G-7884-2012; Chen, Zonghai/K-8745-2013; Lin, Zhijun/A-5543-2010 FU National Science Foundation (NSF); Ministry of Science and Technology of China (MOST); U.S. Department of Energy (DOE) [DE-SC0001057]; DOE Office of Basic Energy Sciences; DOE National Nuclear Security Administration FX This work was supported by the National Science Foundation (NSF) and the Ministry of Science and Technology of China (MOST) through research projects. HPSynC is supported as part of EFree, an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE) under Award DE-SC0001057. HPCAT is supported by the DOE Office of Basic Energy Sciences, DOE National Nuclear Security Administration, and NSF. NR 42 TC 31 Z9 32 U1 8 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 25 PY 2011 VL 133 IS 20 BP 7892 EP 7896 DI 10.1021/ja2009949 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 776ZN UT WOS:000291580400046 PM 21528857 ER PT J AU Szigethy, G Raymond, KN AF Szigethy, Geza Raymond, Kenneth N. TI Hexadentate Terephthalamide(bis-hydroxypyridinone) Ligands for Uranyl Chelation: Structural and Thermodynamic Consequences of Ligand Variation SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID STEREOGNOSTIC COORDINATION CHEMISTRY; CATION-CATION COMPLEXES; SEQUESTERING AGENTS; CRYSTAL-STRUCTURE; SCHIFF-BASE; UO22+ COMPLEXES; METAL-COMPLEXES; IRON CHELATORS; ACTINIDES; ION AB Several linear, hexa- and tetradentate ligands incorporating a combination of 2,3-dihydroxy-terephthalamide (TAM) and hydroxypyridinone-amide (HOPO) moieties have been developed as uranyl chelating agents. Crystallographic analysis of several {UO2[TAM(HOPO)(2)]}(2-) complexes revealed a variable and crowded coordination geometry about the uranyl center. The TAM moiety dominates the bonding in hexadenate complexes, with linker rigidity dictating the equality of equatorial U-O bonding. Hexadentate TAM-(HOPO)(2) ligands demonstrated slow binding kinetics with uranyl affinities on average 6 orders of magnitude greater than those of similarly linked bis-HOPO ligands. Study of tetradentate TAM(HOPO) ligands revealed that the high uranyl affinity stems primarily from the presence of the TAM moiety and only marginally from increased ligand denticity. Uranyl affinities of TAM(HOPO)(2) ligands were within experimental error, with TAM-(o-phen-1,2-HOPO)(2) exhibiting the most consistent uranyl affinity at variable pH. C1 [Raymond, Kenneth N.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Lab, Div Chem Sci, Glenn T Seaborg Ctr, Berkeley, CA 94720 USA. RP Raymond, KN (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM raymond@socrates.berkeley.edu FU Office of Science, Office of Basic Energy Sciences; Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231] FX We thank Drs. Rebecca Abergel and Trisha Hoette for assistance with the titration measurements and data treatment. This research is supported by the Director, Office of Science, Office of Basic Energy Sciences, and the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. NR 76 TC 22 Z9 22 U1 6 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 25 PY 2011 VL 133 IS 20 BP 7942 EP 7956 DI 10.1021/ja201511u PG 15 WC Chemistry, Multidisciplinary SC Chemistry GA 776ZN UT WOS:000291580400051 PM 21542587 ER PT J AU Klug, DD Tse, JS Zhao, JY Sturhahn, W Alp, EE Tulk, CA AF Klug, D. D. Tse, J. S. Zhao, J. Y. Sturhahn, W. Alp, E. E. Tulk, C. A. TI Dynamics of Kr in dense clathrate hydrates SO PHYSICAL REVIEW B LA English DT Article ID SYNCHROTRON-RADIATION; THERMAL-CONDUCTIVITY; SCATTERING; NUCLEAR; DEPENDENCE; HYDROGEN; KRYPTON; MOTIONS; XENON AB The dynamics of Kr atoms as guests in dense clathrate hydrate structures are investigated using site specific (83)Kr nuclear resonant inelastic x-ray scattering (NRIXS) spectroscopy in combination with molecular dynamics simulations. The dense structure H hydrate and filled-ice structures are studied at high pressures in a diamond anvil high-pressure cell. The dynamics of Kr in the structure H clathrate hydrate quench recovered at 77 K is also investigated. The Kr phonon density of states obtained from the experimental NRIXS data are compared with molecular dynamics simulations. The temperature and pressure dependence of the phonon spectra provide details of the Kr dynamics in the clathrate hydrate cages. Comparison with the dynamics of Kr atoms in the low-pressure structure II obtained previously was made. The Lamb-Mossbauer factor obtained from NRIXS experiments and molecular dynamics calculations are in excellent agreement and are shown to yield unique information on the strength and temperature dependence of guest-host interactions. C1 [Klug, D. D.] Natl Res Council Canada, Steacie Inst Mol Sci, Ottawa, ON K1A 0R6, Canada. [Tse, J. S.] Univ Saskatchewan, Dept Phys & Engn Phys, Saskatoon, SK S7N 5E2, Canada. [Zhao, J. Y.; Sturhahn, W.; Alp, E. E.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Tulk, C. A.] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. RP Klug, DD (reprint author), Natl Res Council Canada, Steacie Inst Mol Sci, 100 Sussex Dr, Ottawa, ON K1A 0R6, Canada. RI Tulk, Chris/R-6088-2016 OI Tulk, Chris/0000-0003-3400-3878 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX A portion of this Research at Oak Ridge National Laboratory's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 24 TC 4 Z9 4 U1 3 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 25 PY 2011 VL 83 IS 18 AR 184116 DI 10.1103/PhysRevB.83.184116 PG 6 WC Physics, Condensed Matter SC Physics GA 768NP UT WOS:000290942100003 ER PT J AU Miura, M Maiorov, B Baily, SA Haberkorn, N Willis, JO Marken, K Izumi, T Shiohara, Y Civale, L AF Miura, M. Maiorov, B. Baily, S. A. Haberkorn, N. Willis, J. O. Marken, K. Izumi, T. Shiohara, Y. Civale, L. TI Mixed pinning landscape in nanoparticle-introduced YGdBa2Cu3Oy films grown by metal organic deposition SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTORS; IRREVERSIBILITY LINE; COATED CONDUCTORS; CRITICAL CURRENTS; COLUMNAR DEFECTS; FLUX-CREEP; YBA2CU3O7; WIRES; CRYSTALS AB We study the field (H) and temperature (T) dependence of the critical current density (J(c)) and irreversibility field (H-irr) at different field orientations in Y0.77Gd0.23Ba2Cu3Oy with randomly distributed BaZrO3 nanoparticles (YGdBCO + BZO) and YBa2Cu3Oy (YBCO) films. Both MOD films have large RE2Cu2O5 (225) nanoparticles (similar to 80 nm in diameter) and a high density of twin boundaries (TB). In addition, YGdBCO + BZO films have a high density of BZO nanoparticles (similar to 25 nm in diameter). At high temperatures (T > 40 K), the superconducting properties, such as J(c), H-irr, and flux creep rates, are greatly affected by the BZO nanoparticles, while at low temperatures the superconducting properties of both the YBCO and YGdBCO + BZO films show similar field and temperature dependencies. In particular, while the J(c) of YBCO films follow a power-law dependence (proportional to H-alpha) at all measured T, this dependence is only followed at low T for YGdBCO + BZO films. As a function of T, the YGdBCO + BZO film shows J(c) (T, 0.01T) similar to [1 -(T/T-c)(2)](n) with n similar to 1.24 +/- 0.05, which points to "delta T-c pinning." We analyze the role of different types of defects in the different temperature regimes and find that the strong pinning of the BZO nanoparticles yields a higher H-irr and improved J(c) along the c axis and at intermediate orientations at high T. The mixed pinning landscapes due to the presence of disorder of various dimensionalities have an important role in the improvement of in-field properties. C1 [Miura, M.; Maiorov, B.; Baily, S. A.; Haberkorn, N.; Willis, J. O.; Marken, K.; Civale, L.] Los Alamos Natl Lab, Superconduct Technol Ctr, Los Alamos, NM 87545 USA. [Baily, S. A.] Los Alamos Natl Lab, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA. [Izumi, T.; Shiohara, Y.] Int Superconduct Technol Ctr, Superconduct Res Lab, Koto Ku, Tokyo 1350062, Japan. RP Miura, M (reprint author), Los Alamos Natl Lab, Superconduct Technol Ctr, POB 1663, Los Alamos, NM 87545 USA. EM miura38ktgaj@gmail.com OI Maiorov, Boris/0000-0003-1885-0436; Civale, Leonardo/0000-0003-0806-3113 FU Los Alamos National Laboratory; by the US DOE, Office of Basic Energy Sciences (Division of Materials Sciences and Engineering); NHMFL-UCGP; State of Florida; US NSF; NEDO as a Collaborative Research FX We thank T. Kato for assistance with TEM observations. This work was supported by the Laboratory Directed Research and Development program at Los Alamos National Laboratory; by the US DOE, Office of Basic Energy Sciences (Division of Materials Sciences and Engineering); by NHMFL-UCGP, the State of Florida, and by the US NSF. Work at ISTEC-SRL was supported by NEDO as a Collaborative Research. NR 41 TC 55 Z9 55 U1 3 U2 36 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 25 PY 2011 VL 83 IS 18 AR 184519 DI 10.1103/PhysRevB.83.184519 PG 8 WC Physics, Condensed Matter SC Physics GA 768NP UT WOS:000290942100009 ER PT J AU Knorowski, C Burleigh, S Travesset, A AF Knorowski, C. Burleigh, S. Travesset, A. TI Dynamics and Statics of DNA-Programmable Nanoparticle Self-Assembly and Crystallization SO PHYSICAL REVIEW LETTERS LA English DT Article ID COLLOIDS AB DNA linker mediated self-assembly is emerging as a very general strategy for designing new materials. In this Letter, we characterize both the dynamics and thermodynamics of nanoparticle-DNA self-assembly by molecular dynamics simulations from a new coarse-grained model. We establish the general phase diagram and discuss the stability of a previously overlooked crystalline phase (D-bcc). We also characterize universal properties about the dynamics of crystallization. We point out the connection to f-star polymer systems and discuss the implications for ongoing experiments as well as for the general field of DNA mediated self-assembly. C1 [Knorowski, C.; Travesset, A.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Knorowski, C.; Travesset, A.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Burleigh, S.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. RP Knorowski, C (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. FU DOE through the Ames Lab [DE-AC02-07CH11358] FX We acknowledge discussions with J. Anderson, O. Gang, D. Nykypanchuk, and C. Philips. S. B. acknowledges a DOE SULI internship at the Ames Lab. This work is funded by DOE through the Ames Lab under Contract No. DE-AC02-07CH11358. NR 26 TC 59 Z9 60 U1 4 U2 68 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 25 PY 2011 VL 106 IS 21 AR 215501 DI 10.1103/PhysRevLett.106.215501 PG 4 WC Physics, Multidisciplinary SC Physics GA 768MY UT WOS:000290940200009 PM 21699312 ER PT J AU Anderson, I Scheuner, C Goker, M Mavromatis, K Hooper, SD Porat, I Klenk, HP Ivanova, N Kyrpides, N AF Anderson, Iain Scheuner, Carmen Goeker, Markus Mavromatis, Kostas Hooper, Sean D. Porat, Iris Klenk, Hans-Peter Ivanova, Natalia Kyrpides, Nikos TI Novel Insights into the Diversity of Catabolic Metabolism from Ten Haloarchaeal Genomes SO PLOS ONE LA English DT Article ID ENTNER-DOUDOROFF PATHWAY; EXTREMELY HALOPHILIC ARCHAEA; UNIVERSAL STRESS-PROTEIN; SP-NOV; HALOQUADRATUM-WALSBYI; HALORHABDUS-UTAHENSIS; HALOFERAX-VOLCANII; GEN. NOV.; DEAD-SEA; HALOARCULA-MARISMORTUI AB Background: The extremely halophilic archaea are present worldwide in saline environments and have important biotechnological applications. Ten complete genomes of haloarchaea are now available, providing an opportunity for comparative analysis. Methodology/Principal Findings: We report here the comparative analysis of five newly sequenced haloarchaeal genomes with five previously published ones. Whole genome trees based on protein sequences provide strong support for deep relationships between the ten organisms. Using a soft clustering approach, we identified 887 protein clusters present in all halophiles. Of these core clusters, 112 are not found in any other archaea and therefore constitute the haloarchaeal signature. Four of the halophiles were isolated from water, and four were isolated from soil or sediment. Although there are few habitat-specific clusters, the soil/sediment halophiles tend to have greater capacity for polysaccharide degradation, siderophore synthesis, and cell wall modification. Halorhabdus utahensis and Haloterrigena turkmenica encode over forty glycosyl hydrolases each, and may be capable of breaking down naturally occurring complex carbohydrates. H. utahensis is specialized for growth on carbohydrates and has few amino acid degradation pathways. It uses the non-oxidative pentose phosphate pathway instead of the oxidative pathway, giving it more flexibility in the metabolism of pentoses. Conclusions: These new genomes expand our understanding of haloarchaeal catabolic pathways, providing a basis for further experimental analysis, especially with regard to carbohydrate metabolism. Halophilic glycosyl hydrolases for use in biofuel production are more likely to be found in halophiles isolated from soil or sediment. C1 [Anderson, Iain; Mavromatis, Kostas; Hooper, Sean D.; Ivanova, Natalia; Kyrpides, Nikos] US DOE, Genome Biol Program, Joint Genome Inst, Walnut Creek, CA USA. [Scheuner, Carmen; Goeker, Markus; Klenk, Hans-Peter] Deutsch Sammlung Mikroorganismen & Zellkulturen, D-3300 Braunschweig, Germany. [Porat, Iris] INEOS Bio, Fayetteville, AR USA. RP Anderson, I (reprint author), US DOE, Genome Biol Program, Joint Genome Inst, Walnut Creek, CA USA. EM IJAnderson@lbl.gov RI Kyrpides, Nikos/A-6305-2014 OI Kyrpides, Nikos/0000-0002-6131-0462 FU Office of Science of the United States Department of Energy [DE-AC02-05CH112] FX This work was supported by the Office of Science of the United States Department of Energy (http://www.er.doe.gov/) under Contract No. DE-AC02-05CH112. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 90 TC 35 Z9 35 U1 2 U2 29 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 25 PY 2011 VL 6 IS 5 AR e20237 DI 10.1371/journal.pone.0020237 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 769IQ UT WOS:000291006500046 PM 21633497 ER PT J AU Voolstra, CR Sunagawa, S Matz, MV Bayer, T Aranda, M Buschiazzo, E DeSalvo, MK Lindquist, E Szmant, AM Coffroth, MA Medina, M AF Voolstra, Christian R. Sunagawa, Shinichi Matz, Mikhail V. Bayer, Till Aranda, Manuel Buschiazzo, Emmanuel DeSalvo, Michael K. Lindquist, Erika Szmant, Alina M. Coffroth, Mary Alice Medina, Monica TI Rapid Evolution of Coral Proteins Responsible for Interaction with the Environment SO PLOS ONE LA English DT Article ID ANEMONE AIPTASIA-PALLIDA; SYMBIOTIC SEA-ANEMONE; REEF-BUILDING CORALS; GENE-EXPRESSION; MONTASTRAEA-FAVEOLATA; DINOFLAGELLATE MUTUALISM; NUCLEOTIDE SUBSTITUTION; FLUORESCENT PROTEINS; POSITIVE SELECTION; ACROPORA-PALMATA AB Background: Corals worldwide are in decline due to climate change effects (e. g., rising seawater temperatures), pollution, and exploitation. The ability of corals to cope with these stressors in the long run depends on the evolvability of the underlying genetic networks and proteins, which remain largely unknown. A genome-wide scan for positively selected genes between related coral species can help to narrow down the search space considerably. Methodology/Principal Findings: We screened a set of 2,604 putative orthologs from EST-based sequence datasets of the coral species Acropora millepora and Acropora palmata to determine the fraction and identity of proteins that may experience adaptive evolution. 7% of the orthologs show elevated rates of evolution. Taxonomically-restricted (i.e. lineage-specific) genes show a positive selection signature more frequently than genes that are found across many animal phyla. The class of proteins that displayed elevated evolutionary rates was significantly enriched for proteins involved in immunity and defense, reproduction, and sensory perception. We also found elevated rates of evolution in several other functional groups such as management of membrane vesicles, transmembrane transport of ions and organic molecules, cell adhesion, and oxidative stress response. Proteins in these processes might be related to the endosymbiotic relationship corals maintain with dinoflagellates in the genus Symbiodinium. Conclusion/Relevance: This study provides a birds-eye view of the processes potentially underlying coral adaptation, which will serve as a foundation for future work to elucidate the rates, patterns, and mechanisms of corals' evolutionary response to global climate change. C1 [Voolstra, Christian R.; Bayer, Till; Aranda, Manuel] King Abdullah Univ Sci & Technol, Red Sea Res Ctr, Thuwal, Saudi Arabia. [Sunagawa, Shinichi] European Mol Biol Lab, Heidelberg, Germany. [Matz, Mikhail V.] Univ Texas Austin, Sch Biol Sci, Sect Integrat Biol, Austin, TX 78712 USA. [Buschiazzo, Emmanuel; Medina, Monica] Univ Calif Merced, Sch Nat Sci, Merced, CA USA. [DeSalvo, Michael K.] Univ Calif San Francisco, Dept Anesthesia, UCSF Sch Med, San Francisco, CA 94143 USA. [Lindquist, Erika] Joint Genome Inst, Dept Energy, Walnut Creek, CA USA. [Szmant, Alina M.] Univ N Carolina, Ctr Marine Sci, Wilmington, NC 28401 USA. [Coffroth, Mary Alice] SUNY Buffalo, Grad Program Evolut Ecol & Behav, Buffalo, NY 14260 USA. [Coffroth, Mary Alice] SUNY Buffalo, Dept Geol, Buffalo, NY 14260 USA. RP Voolstra, CR (reprint author), King Abdullah Univ Sci & Technol, Red Sea Res Ctr, Thuwal, Saudi Arabia. EM christian.voolstra@kaust.edu.sa; mmedina@ucmerced.edu RI Aranda Lastra, Manuel/D-9530-2011; Sunagawa, Shinichi/D-9715-2011; Buschiazzo, Emmanuel/B-5126-2011; Voolstra, Christian/H-7158-2014; Bayer, Till/H-6826-2016; OI Aranda Lastra, Manuel/0000-0001-6673-016X; Sunagawa, Shinichi/0000-0003-3065-0314; Voolstra, Christian/0000-0003-4555-3795; Bayer, Till/0000-0002-4704-2449; Matz, Mikhail/0000-0001-5453-9819 FU National Science Foundation [IOS-0644438, OCE-0313708]; Collaborative Travel Fund; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; [DEB-1054766] FX This work was supported by DEB-1054766 to M. V. M. and National Science Foundation grants IOS-0644438 and OCE-0313708 to M. M., and by a Collaborative Travel Fund to C. R. V. made by King Abdullah University of Science and Technology (KAUST). The work conducted by the U.S. Department of Energy Joint Genome Institute is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 79 TC 28 Z9 28 U1 3 U2 43 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 185 BERRY ST, STE 1300, SAN FRANCISCO, CA 94107 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 25 PY 2011 VL 6 IS 5 AR e20392 DI 10.1371/journal.pone.0020392 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 769IQ UT WOS:000291006500059 PM 21633702 ER PT J AU Volkow, ND Tomasi, D Vaska, P AF Volkow, Nora D. Tomasi, Dardo Vaska, Paul TI Cell Phone Activation and Brain Glucose Metabolism Reply SO JAMA-JOURNAL OF THE AMERICAN MEDICAL ASSOCIATION LA English DT Letter C1 [Volkow, Nora D.] NIDA, Bethesda, MD 20892 USA. [Tomasi, Dardo] NIAAA, Bethesda, MD USA. [Vaska, Paul] Brookhaven Natl Lab, Dept Med, Upton, NY 11973 USA. RP Volkow, ND (reprint author), NIDA, Bethesda, MD 20892 USA. EM nvolkow@nida.nih.gov RI Tomasi, Dardo/J-2127-2015 NR 3 TC 0 Z9 0 U1 0 U2 1 PU AMER MEDICAL ASSOC PI CHICAGO PA 330 N WABASH AVE, STE 39300, CHICAGO, IL 60611-5885 USA SN 0098-7484 EI 1538-3598 J9 JAMA-J AM MED ASSOC JI JAMA-J. Am. Med. Assoc. PD MAY 25 PY 2011 VL 305 IS 20 BP 2067 EP 2068 DI 10.1001/jama.2011.672 PG 2 WC Medicine, General & Internal SC General & Internal Medicine GA 768AC UT WOS:000290901700014 ER PT J AU Song, HC Bass, SA Heinz, U Hirano, T Shen, C AF Song, Huichao Bass, Steffen A. Heinz, Ulrich Hirano, Tetsufumi Shen, Chun TI Hadron spectra and elliptic flow for 200 A GeV Au plus Au collisions from viscous hydrodynamics coupled to a Boltzmann cascade SO PHYSICAL REVIEW C LA English DT Article ID ECCENTRICITY FLUCTUATIONS; NUCLEAR COLLISIONS AB It is shown that the recently developed hybrid code VISHNU, which couples a relativistic viscous fluid dynamical description of the quark-gluon plasma (QGP) with a microscopic Boltzmann cascade for the late hadronic rescattering stage, yields an excellent description of charged and identified hadron spectra and elliptic flow measured in 200 A GeV Au + Au collisions at the Relativistic Heavy-Ion Collider (RHIC). Using initial conditions that incorporate event-by-event fluctuations in the initial shape and orientation of the collision fireball and values eta/s for the specific shear viscosity of the quark-gluon plasma that were recently extracted from the measured centrality dependence of the eccentricity-scaled, p(T)-integrated charged hadron elliptic flow v(2,ch)/epsilon, we obtain universally good agreement between theory and experiment for the p(T) spectra and differential elliptic flow v(2)(p(T)) for both pions and protons at all collision centralities. C1 [Song, Huichao; Hirano, Tetsufumi] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Bass, Steffen A.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Heinz, Ulrich; Shen, Chun] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Hirano, Tetsufumi] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. RP Song, HC (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. FU US Department of Energy [DE-AC02-05CH11231, DE-FG02-05ER41367, DE-SC0004286, DE-SC0004104]; Japan Society for the Promotion of Science [22740151, 213383] FX We gratefully acknowledge fruitful discussions with P. Huovinen, H. Masui, A. Poskanzer, S. Voloshin, and A. Tang. We specifically thank A. Poskanzer for computing for us the a values listed in Table I and R. Snellings for providing some of the data shown in Fig. 6. This work was supported by the US Department of Energy under Grants No. DE-AC02-05CH11231, No. DE-FG02-05ER41367, No. DE-SC0004286, and (within the framework of the JET Collaboration) No. DE-SC0004104. T. H. acknowledges support through Grant-in-Aid for Scientific Research No. 22740151 and through the Excellent Young Researchers Oversea Visit Program (No. 213383) of the Japan Society for the Promotion of Science. We gratefully acknowledge extensive computing resources provided to us by the Ohio Supercomputer Center. NR 51 TC 77 Z9 77 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 J9 PHYS REV C JI Phys. Rev. C PD MAY 25 PY 2011 VL 83 IS 5 AR 054910 DI 10.1103/PhysRevC.83.054910 PG 12 WC Physics, Nuclear SC Physics GA 768OM UT WOS:000290944500001 ER PT J AU Musch, BU Hagler, P Negele, JW Schafer, A AF Musch, B. U. Haegler, Ph. Negele, J. W. Schaefer, A. TI Exploring quark transverse momentum distributions with lattice QCD SO PHYSICAL REVIEW D LA English DT Article ID GENERALIZED PARTON DISTRIBUTIONS; FINAL-STATE INTERACTIONS; DEEP-INELASTIC SCATTERING; GAUGE-THEORY; DRELL-YAN; FRAGMENTATION FUNCTIONS; SPIN ASYMMETRIES; HADRON STRUCTURE; PHASE-FACTORS; SINGLE-SPIN AB We discuss in detail a method to study transverse momentum dependent parton distribution functions (TMDs) using lattice QCD. To develop the formalism and to obtain first numerical results, we directly implement a bilocal quark-quark operator connected by a straight Wilson line, allowing us to study T-even, "process-independent'' TMDs. Beyond results for x-integrated TMDs and quark densities, we present a study of correlations in x and k(perpendicular to). Our calculations are based on domain wall valence quark propagators by the LHP Collaboration calculated on top of gauge configurations provided by the MILC Collaboration with N-f = 2 + 1 asqtad-improved staggered sea quarks. C1 [Musch, B. U.] Jefferson Lab, Ctr Theory, Newport News, VA 23606 USA. [Haegler, Ph.] Tech Univ Munich, Inst Theoret Phys T39, Dept Phys, D-85747 Garching, Germany. [Haegler, Ph.; Schaefer, A.] Univ Regensburg, Inst Theoret Phys, D-93040 Regensburg, Germany. [Negele, J. W.] MIT, Ctr Theoret Phys, Cambridge, MA 02139 USA. RP Musch, BU (reprint author), Jefferson Lab, Ctr Theory, Newport News, VA 23606 USA. EM bmusch@jlab.org; phaegler@ph.tum.de NR 107 TC 49 Z9 49 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 25 PY 2011 VL 83 IS 9 AR 094507 DI 10.1103/PhysRevD.83.094507 PG 37 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 768OR UT WOS:000290945000001 ER PT J AU Berry, JW Hendrickson, B LaViolette, RA Phillips, CA AF Berry, Jonathan W. Hendrickson, Bruce LaViolette, Randall A. Phillips, Cynthia A. TI Tolerating the community detection resolution limit with edge weighting SO PHYSICAL REVIEW E LA English DT Article ID NETWORKS AB Communities of vertices within a giant network such as the World Wide Web are likely to be vastly smaller than the network itself. However, Fortunato and Barthelemy have proved that modularity maximization algorithms for community detection may fail to resolve communities with fewer than root L/2 edges, where L is the number of edges in the entire network. This resolution limit leads modularity maximization algorithms to have notoriously poor accuracy on many real networks. Fortunato and Barthelemy's argument can be extended to networks with weighted edges as well, and we derive this corollary argument. We conclude that weighted modularity algorithms may fail to resolve communities with less than root W is an element of/2 total edge weight, where W is the total edge weight in the network and is an element of is the maximum weight of an intercommunity edge. If is an element of is small, then small communities can be resolved. Given a weighted or unweighted network, we describe how to derive new edge weights in order to achieve a low is an element of, we modify the Clauset, Newman, and Moore (CNM) community detection algorithm to maximize weighted modularity, and we show that the resulting algorithm has greatly improved accuracy. In experiments with an emerging community standard benchmark, we find that our simple CNM variant is competitive with the most accurate community detection methods yet proposed. C1 [Berry, Jonathan W.; Hendrickson, Bruce; LaViolette, Randall A.; Phillips, Cynthia A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Berry, JW (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM jberry@sandia.gov; bahendr@sandia.gov; randall.laviolette@science.doe.gov; caphill@sandia.gov FU Laboratory Directed Research and Development program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We thank Santo Fortunato (ISI), Joseph McCloskey (DoD), Cris Moore (UNM), Tamara Kolda (Sandia), Dan Nordman (Iowa State), and Alyson Wilson (Iowa State) for helpful discussions and comments. This work was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 30 TC 42 Z9 43 U1 0 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD MAY 25 PY 2011 VL 83 IS 5 AR 056119 DI 10.1103/PhysRevE.83.056119 PN 2 PG 9 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 768PH UT WOS:000290946900001 PM 21728617 ER PT J AU Webb, S Wang, G Litvinenko, V AF Webb, Stephen Wang, Gang Litvinenko, Vladimir TI Three-dimensional model of small signal free-electron lasers SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID GAIN AB Coherent electron cooling is an ultrahigh-bandwidth form of stochastic cooling which utilizes the charge perturbation from Debye screening as a seed for a free-electron laser. The amplified and frequency-modulated signal that results from the free-electron laser process is then used to give an energy-dependent kick on the hadrons in a bunch. In this paper, we present a theoretical description of a high-gain free-electron laser with applications to a complete theoretical description of coherent electron cooling. C1 [Webb, Stephen] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Webb, Stephen; Wang, Gang; Litvinenko, Vladimir] Brookhaven Natl Lab, Collider Accelerator Dept, Upton, NY 11973 USA. RP Webb, S (reprint author), SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. EM swebb@grad.physics.sunysb.edu; gawang@bnl.gov; vl@bnl.gov FU Brookhaven Science Associates, LLC, U.S. Department of Energy [DE-AC02-98CH10886] FX The authors would like to thank Michael Blaskiewicz and Evgeny Saldin for helpful discussion. This work was supported by Brookhaven Science Associates, LLC under Contract No. DE-AC02-98CH10886 with the U.S. Department of Energy. NR 18 TC 4 Z9 4 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD MAY 25 PY 2011 VL 14 IS 5 AR 051003 DI 10.1103/PhysRevSTAB.14.051003 PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 768PK UT WOS:000290947200001 ER PT J AU Hou, C Xiong, YJ Fu, N Jacquot, CC Squier, TC Cao, HS AF Hou, Chen Xiong, Yijia Fu, Na Jacquot, Caitlin C. Squier, Thomas C. Cao, Haishi TI Turn-on ratiometric fluorescent sensor for Pb2+ detection SO TETRAHEDRON LETTERS LA English DT Article DE Pb2+; Sensor; Pyrene ID EXCIMER FORMATION; IONS; PB(II); LEAD; CHEMOSENSORS; DERIVATIVES; PYRENE; SENSITIVITY; SELECTIVITY; PROBES AB We report a ratiometric lead fluorescent sensor (LFS-1) with high affinity to Pb2+ that shows considerable selectivity over 12 other physiological related metal cations in aqueous media. Binding induces excimer formation, providing a highly sensitive ratiometric measure of lead concentrations. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Hou, Chen; Jacquot, Caitlin C.; Cao, Haishi] Univ Nebraska, Dept Chem, Kearney, NE 68849 USA. [Xiong, Yijia; Fu, Na; Squier, Thomas C.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99354 USA. RP Cao, HS (reprint author), Univ Nebraska, Dept Chem, Kearney, NE 68849 USA. EM caoh1@unk.edu RI Fu, Na/C-8662-2011; Xiong, Yijia/C-1341-2011 FU University Research and Creative Activity in the University of Nebraska at Kearney FX This research is supported by Mini-Grant, Undergraduate Research Fellows Program, and University Research and Creative Activity in the University of Nebraska at Kearney. Authors would also like to acknowledge Sara Basiaga in University of Nebraska at Lincoln for her assistance in collecting fluorescence spectra. NR 46 TC 12 Z9 12 U1 3 U2 30 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0040-4039 J9 TETRAHEDRON LETT JI Tetrahedron Lett. PD MAY 25 PY 2011 VL 52 IS 21 BP 2692 EP 2696 DI 10.1016/j.tetlet.2011.03.075 PG 5 WC Chemistry, Organic SC Chemistry GA 764AZ UT WOS:000290602100020 ER PT J AU Huang, GY Wirth, BD AF Huang, Gui-Yang Wirth, Brian D. TI First-principles study of diffusion of interstitial and vacancy in alpha U-Zr SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID AUGMENTED-WAVE METHOD; GAS BUBBLES; URANIUM; METALS; ALLOYS; STRESS; SYSTEM; PHASE AB Metallic uranium-zirconium alloys are of interest for a variety of fast reactor designs, and there is substantial experience with the behavior of metallic fuels. Yet, there remain a number of questions regarding the mechanisms controlling fission-gas-driven swelling in these alloys. Here we present results of ab initio calculations of the diffusion behavior of interstitial and vacancy point defects in alpha U-Zr alloys. The formation energy and migration barrier of vacancy and interstitial defects, and the influence of Zr on these values, is obtained and compared with experimental results. Our results confirm that self-diffusion in pure alpha U is via a simple vacancy mechanism, and shows anisotropic character. The calculated values of activation energy are consistent with the experimental results in the literature. For interstitial diffusion, the kick-out mechanism was found to have the smallest energy barrier. The calculations of point defects, and later Xe, in U-Zr alloys will provide a foundation for computational modeling of fission gas bubble nucleation and growth. C1 [Huang, Gui-Yang; Wirth, Brian D.] Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA. [Wirth, Brian D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Huang, GY (reprint author), Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA. EM huangguiyang@gmail.com; bdwirth@utk.edu RI Huang, Guiyang/E-7746-2012; Wirth, Brian/O-4878-2015 OI Huang, Guiyang/0000-0003-0144-7376; Wirth, Brian/0000-0002-0395-0285 FU US Department of Energy, Office of Nuclear Energy through Nuclear Energy University [00091204, CFDA 81.049] FX This research has been funded by the US Department of Energy, Office of Nuclear Energy through the Nuclear Energy University Program, administered by Battelle Energy Alliance, LLC, subcontract no. 00091204, CFDA#81.049. NR 43 TC 13 Z9 13 U1 5 U2 18 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAY 25 PY 2011 VL 23 IS 20 AR 205402 DI 10.1088/0953-8984/23/20/205402 PG 9 WC Physics, Condensed Matter SC Physics GA 759AQ UT WOS:000290212300011 PM 21540501 ER PT J AU Spencer, EC Ross, NL Parker, SF Woodfield, BF Boerio-Goates, J Smith, SJ Olsen, RE Kolesnikov, AI Navrotsky, A Ma, C AF Spencer, E. C. Ross, N. L. Parker, S. F. Woodfield, B. F. Boerio-Goates, J. Smith, S. J. Olsen, R. E. Kolesnikov, A. I. Navrotsky, A. Ma, C. TI Determination of the magnetic contribution to the heat capacity of cobalt oxide nanoparticles and the thermodynamic properties of the hydration layers SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID INELASTIC NEUTRON-SCATTERING; COO NANOPARTICLES; METAL-OXIDES; TRANSITION; CO3O4; WATER; OXIDATION; EXCITATIONS; ICE AB We present low temperature (11 K) inelastic neutron scattering (INS) data on four hydrated nanoparticle systems: 10 nm CoO center dot 0.10H(2)O (1), 16 nmCo(3)O(4)center dot 0.40H(2)O (2), 25 nm Co3O4 center dot 0.30H(2)O (3) and 40 nmCo(3)O4 center dot 0.026H(2)O (4). The vibrational densities of states were obtained for all samples and from these the isochoric heat capacity and vibrational energy for the hydration layers confined to the surfaces of these nanoparticle systems have been elucidated. The results show that water on the surface of CoO nanoparticles is more tightly bound than water confined to the surface of Co3O4, and this is reflected in the reduced heat capacity and vibrational entropy for water on CoO relative to water on Co3O4 nanoparticles. This supports the trend, seen previously, for water to be more tightly bound in materials with higher surface energies. The INS spectra for the antiferromagnetic Co3O4 particles (2-4) also show sharp and intense magnetic excitation peaks at 5 meV, and from this the magnetic contribution to the heat capacity of Co3O4 nanoparticles has been calculated; this represents the first example of use of INS data for determining the magnetic contribution to the heat capacity of any magnetic nanoparticle system. C1 [Spencer, E. C.; Ross, N. L.] Virginia Tech, Dept Geosci, Blacksburg, VA 24061 USA. [Parker, S. F.] STFC Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Woodfield, B. F.; Boerio-Goates, J.; Smith, S. J.; Olsen, R. E.] Brigham Young Univ, Dept Chem & Biochem, Provo, UT 84602 USA. [Kolesnikov, A. I.] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. [Navrotsky, A.; Ma, C.] Univ Calif Davis, Peter A Rock Thermochem Lab, Davis, CA 95616 USA. [Navrotsky, A.; Ma, C.] Univ Calif Davis, NEAT ORU, Davis, CA 95616 USA. RP Ross, NL (reprint author), Virginia Tech, Dept Geosci, Blacksburg, VA 24061 USA. RI davidson, anne/A-5160-2012; Kolesnikov, Alexander/I-9015-2012; OI Kolesnikov, Alexander/0000-0003-1940-4649; Parker, Stewart/0000-0002-3228-2570 FU US Department of Energy, Office of Basic Energy Sciences (DOE-BES) [DE FG03 01ER15237]; DOE [DE-AC05-00OR22725] FX N L Ross, E C Spencer, and A Navrotsky acknowledge support from the US Department of Energy, Office of Basic Energy Sciences (DOE-BES), grant DE FG03 01ER15237. A I Kolesnikov wishes to acknowledge ORNL/SNS at Oak Ridge National Laboratory that is managed by UT-Battelle, LLC, for DOE under contract DE-AC05-00OR22725. The STFC Rutherford Appleton Laboratory is thanked for access to neutron beam facilities. NR 33 TC 7 Z9 7 U1 1 U2 29 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAY 25 PY 2011 VL 23 IS 20 AR 205303 DI 10.1088/0953-8984/23/20/205303 PG 6 WC Physics, Condensed Matter SC Physics GA 759AQ UT WOS:000290212300007 PM 21540512 ER PT J AU Zhang, J Lu, WC Zang, QJ Zhao, LZ Wang, CZ Ho, KM AF Zhang, Jing Lu, Wen-Cai Zang, Qing-Jun Zhao, Li-Zhen Wang, C. Z. Ho, K. M. TI An ab initio calculation study of silicon and carbon binary clusters C7Sin (n=1-7) SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID MOLECULAR-ORBITAL CALCULATIONS; STABILITY; SPECTRA; FRAGMENTATION; ENERGETICS; SI AB Binary C7Sin (n = 1-7) clusters are studied using density functional calculations at the level of B3LYP/6-311G(d). Lowest-energy structures have been determined theoretically and their properties such as binding energies, second differences in energy and highest-occupied and lowest-unoccupied molecular orbital gaps have been analyzed. It is found that the lowest-energy structures of the C7Sin (n = 1-7) clusters change from linear to planar when n >= 3, and in the planar structures C atoms prefer to form five-and six-membered rings surrounded by extra Si atoms in the form of the C2Si units. C1 [Zhang, Jing; Lu, Wen-Cai] Jilin Univ, Inst Theoret Chem, State Key Lab Theoret & Computat Chem, Changchun 130021, Jilin, Peoples R China. [Lu, Wen-Cai; Zang, Qing-Jun; Zhao, Li-Zhen] Qingdao Univ, Growing Base State Key Lab, Lab Fiber Mat & Modern Text, Qingdao 266071, Shandong, Peoples R China. [Lu, Wen-Cai; Zang, Qing-Jun; Zhao, Li-Zhen] Qingdao Univ, Growing Base State Key Lab, Coll Phys, Qingdao 266071, Shandong, Peoples R China. [Wang, C. Z.; Ho, K. M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Wang, C. Z.; Ho, K. M.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. RP Lu, WC (reprint author), Jilin Univ, Inst Theoret Chem, State Key Lab Theoret & Computat Chem, Changchun 130021, Jilin, Peoples R China. EM wencailu@jlu.edu.cn FU National Natural Science Foundation of China [20773047, 21043001]; US Department of Energy by Iowa State University [DE-AC02-07CH11358] FX This work was supported by the National Natural Science Foundation of China under grant nos. 20773047 and 21043001. Ames Laboratory is operated for the US Department of Energy by Iowa State University under contract no. DE-AC02-07CH11358. This work was also supported by the Director for Energy Research, Office of Basic Energy Sciences including a grant of computer time at the National Energy Research Supercomputing Center (NERSC) in Berkeley. NR 28 TC 2 Z9 2 U1 1 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAY 25 PY 2011 VL 23 IS 20 AR 205305 DI 10.1088/0953-8984/23/20/205305 PG 7 WC Physics, Condensed Matter SC Physics GA 759AQ UT WOS:000290212300009 PM 21540510 ER PT J AU Ku, SY Liman, CD Cochran, JE Toney, MF Chabinyc, ML Hawker, CJ AF Ku, Sung-Yu Liman, Christopher D. Cochran, Justin E. Toney, Michael F. Chabinyc, Michael L. Hawker, Craig J. TI Solution-Processed Nanostructured Benzoporphyrin with Polycarbonate Binder for Photovoltaics SO ADVANCED MATERIALS LA English DT Article ID ORGANIC SOLAR-CELLS; CARBON-DIOXIDE; EFFICIENT; POLYMERS; FILMS AB A new method to aid large-area solution processing of organic small molecule semiconductors is reported. A thermally degradable poly(propylene carbonate) (PC) binder is added to a solution of soluble precursor to a tetrabenzoporphyrin to increase its viscosity, allowing for the use of large-area methods such as inkjet printing, slot coating, or blade coating. This method is used to make bulk heterojunction solar cells with a p-i-n type structure. C1 [Ku, Sung-Yu; Liman, Christopher D.; Chabinyc, Michael L.; Hawker, Craig J.] Univ Calif Santa Barbara, Mat Res Lab, Dept Mat, Mitsubishi Chem Ctr Adv Mat, Santa Barbara, CA 93106 USA. [Cochran, Justin E.] Univ Calif Santa Barbara, Dept Chem & Biochem, Santa Barbara, CA 93106 USA. [Toney, Michael F.] Stanford Synchrotron Radiat Lab, Stanford, CA 94305 USA. RP Chabinyc, ML (reprint author), Univ Calif Santa Barbara, Mat Res Lab, Dept Mat, Mitsubishi Chem Ctr Adv Mat, Santa Barbara, CA 93106 USA. EM mchabinyc@engineering.ucsb.edu; hawker@mrl.ucsb.edu RI Chabinyc, Michael/E-2387-2011; Hawker, Craig/G-4971-2011 OI Hawker, Craig/0000-0001-9951-851X FU NSF [CHE-1035292]; Mitsubsihi Chemicals Center for Advanced Materials; UCSB MRSEC under NSF [DMR05-20415] FX We thank M. Guide, N. Treat, M. Burkhardt, J. Heo, and M. Dimitriou for their insights, N. Eisenmenger and C. Shuttle for assistance with OPV testing, and Eric Verploegen for assistance with the in-situ annealing. We thank the Mitsubishi Chemical Group Science and Technology Research Center, Inc. for sharing their insights and provision of CP and analytical data. Software for analyzing GIWAXS data was written by Stefan Mannsfeld (SSRL) and R. Joseph Kline (NIST). Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a national user facility operated by Stanford University on behalf of the U. S. Department of Energy, Office of Basic Energy Sciences. This work was supported by the NSF SOLAR program (CHE-1035292), Mitsubsihi Chemicals Center for Advanced Materials and the UCSB MRSEC Program under NSF award DMR05-20415. This article is part of the Special Issue on Materials Research at the University of California, Santa Barbara. NR 24 TC 25 Z9 25 U1 3 U2 43 PU WILEY-BLACKWELL PI MALDEN PA COMMERCE PLACE, 350 MAIN ST, MALDEN 02148, MA USA SN 0935-9648 J9 ADV MATER JI Adv. Mater. PD MAY 24 PY 2011 VL 23 IS 20 SI SI BP 2289 EP + DI 10.1002/adma.201100028 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 776OZ UT WOS:000291547600006 PM 21520461 ER PT J AU Feldman, DR Algieri, CA Ong, JR Collins, WD AF Feldman, Daniel R. Algieri, Chris A. Ong, Jonathan R. Collins, William D. TI CLARREO shortwave observing system simulation experiments of the twenty-first century: Simulator design and implementation SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID GENERAL-CIRCULATION MODELS; CLIMATE SYSTEM; RADIATIVE-TRANSFER; BIDIRECTIONAL REFLECTANCE; ATMOSPHERIC CORRECTION; FEEDBACK PROCESSES; OPTICAL-PROPERTIES; VERSION-3 CCSM3; SURFACE ALBEDO; CLOUD FEEDBACK AB Projected changes in the Earth system will likely be manifested in changes in reflected solar radiation. This paper introduces an operational Observational System Simulation Experiment (OSSE) to calculate the signals of future climate forcings and feedbacks in top-of-atmosphere reflectance spectra. The OSSE combines simulations from the Intergovernmental Panel on Climate Change (IPCC) Fourth Assessment Report for the NCAR Community Climate System Model (CCSM) with the MODTRAN radiative transfer code to calculate reflectance spectra for simulations of current and future climatic conditions over the 21st century. The OSSE produces narrowband reflectances and broadband fluxes, the latter of which have been extensively validated against archived CCSM results. The shortwave reflectance spectra contain atmospheric features including signals from water vapor, liquid and ice clouds, and aerosols. The spectra are also strongly influenced by the surface bidirectional reflectance properties of predicted snow and sea ice and the climatological seasonal cycles of vegetation. By comparing and contrasting simulated reflectance spectra based on emissions scenarios with increasing projected and fixed present-day greenhouse gas and aerosol concentrations, we find that prescribed forcings from increases in anthropogenic sulfate and carbonaceous aerosols are detectable and are spatially confined to lower latitudes. Also, changes in the intertropical convergence zone and poleward shifts in the subsidence zones and the storm tracks are all detectable along with large changes in snow cover and sea ice fraction. These findings suggest that the proposed NASA Climate Absolute Radiance and Refractivity Observatory (CLARREO) mission to measure shortwave reflectance spectra may help elucidate climate forcings, responses, and feedbacks. C1 [Feldman, Daniel R.; Collins, William D.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Algieri, Chris A.; Collins, William D.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Earth Sci, Climate Sci Dept, Berkeley, CA 94720 USA. [Ong, Jonathan R.] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. RP Feldman, DR (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, 307 McCone Hall,MC 4767, Berkeley, CA 94720 USA. EM daniel_r_feldman@berkeley.edu RI Feldman, Daniel/N-8703-2013; Collins, William/J-3147-2014; Richards, Amber/K-8203-2015 OI Feldman, Daniel/0000-0003-3365-5233; Collins, William/0000-0002-4463-9848; FU NASA [NNX08AT80G, NAS2-03144, NNX10AK27G, SMD-08-0999, SMD-09-1397, SMD-10-1799]; Contractor Supporting Research (CSR); Office of Science, of the U.S. Department of Energy [DE-AC02-05CH11231] FX Funding for this research was supported by the following NASA grants: NNX08AT80G, NAS2-03144, and NNX10AK27G. This work was also supported by Contractor Supporting Research (CSR) funding from Berkeley Laboratory, provided by the Director, Office of Science, of the U.S. Department of Energy under contract DE-AC02-05CH11231. Additionally, NASA High-End Computing grants SMD-08-0999, SMD-09-1397, and SMD-10-1799 provided computational resources produce the simulations. The following individuals also provided considerable assistance with this research: Don Anderson of NASA Headquarters; Tsengdar Lee of the NASA Science Mission Directorate; Gail Anderson of AFRL; Vincent Ross of Aerex Corp.; Lex Berk of Spectral Sciences, Inc.; David Young, Bruce Wielicki, Zhonghai Jin, and Rosemary Baize of NASA Langley Research Center; Crystal Schaaf and Zhousen Wang of Boston University; and the entire NASA High-End Computing technical support team of NASA User Services. We also wish to thank the three reviewers for their insightful comments and suggestions. NR 66 TC 14 Z9 14 U1 2 U2 12 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAY 24 PY 2011 VL 116 AR D10107 DI 10.1029/2010JD015350 PG 15 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 770PW UT WOS:000291102000005 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hammer, J Hansel, S Hoch, M Hormann, N Hrubec, J Jeitler, M Kasieczka, G Kiesenhofer, W Krammer, M Liko, D Mikulec, I Pernicka, M Rohringer, H Schofbeck, R Strauss, J Teischinger, F Wagner, P Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Benucci, L De Wolf, EA Janssen, X Maes, T Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Blekman, F Blyweert, S D'Hondt, J Devroede, O Suarez, RG Kalogeropoulos, A Maes, J Maes, M Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Charaf, O Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hammad, GH Hreus, T Marage, E Thomas, L Velde, CV Vanlaer, P Adler, V Cimmino, A Costantini, S Grunewald, M Klein, B Lellouch, J Marinov, A Mccartin, J Ryckbosch, D Thyssen, F Tytgat, M Vanelderen, L Verwilligen, P Walsh, S Zaganidis, N Basegmez, S Bruno, G Caudron, J Ceard, L Gil, EC De Jeneret, JD Delaere, C Favart, D Giammanco, A Gregoire, G Hollar, J Lemaitre, V Liao, J Militaru, O Ovyn, S Pagano, D Pin, A Piotrzkowski, K Schul, N Beliy, N Caebergs, T Daubie, E Alves, GA Damiao, DD Pol, ME Souza, MHG Carvalho, W Da Costa, EM Martins, CD De Souza, SF Mundim, L Nogima, H Oguri, V Da Silva, WLP Santoro, A Do Amaral, SMS Sznajder, A De Araujo, FTD Dias, FA Tomei, TRFP Gregores, EM Lagana, C Marinho, F Mercadante, PG Novaes, SF Padula, SS Darmenov, N Dimitrov, L Genchev, V Iaydjiev, P Piperov, S Rodozov, M Stoykova, S Sultanov, G Tcholakov, V Trayanov, R Vankov, I Dimitrov, A Hadjiiska, R Karadzhinova, A Kozhuharov, V Litov, L Mateev, M Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, J Wang, J Wang, X Wang, Z Xiao, H Xu, M Zang, J Zhang, Z Ban, Y Guo, S Guo, Y Li, W Mao, Y Qian, SJ Teng, H Zhang, L Zhu, B Zou, W Cabrera, A Moreno, BG Rios, AAO Oliveros, AFO Sanabria, JC Godinovic, N Lelas, D Lelas, K Plestina, R Polic, D Puljak, I Antunovic, Z Dzelalija, M Brigljevic, V Duric, S Kadija, K Morovic, S Attikis, A Galanti, M Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Assran, Y Khalil, S Mahmoud, MA Hektor, A Kadastik, M Muntel, M Raidal, M Rebane, L Azzolini, V Eerola, P Fedi, G Czellar, S Harkonen, J Heikkinen, A Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Tuominen, E Tuominiemi, J Tuovinen, E Ungaro, D Wendland, L Banzuzi, K Korpela, A Tuuva, T Sillou, D Besancon, M Choudhury, S Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Gentit, FX Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Marionneau, M Millischer, L Rander, J Rosowsky, A Shreyber, I Titov, 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Lungu, G. Malik, S. Mesropian, C. Yan, M. Atramentov, O. Barker, A. Duggan, D. Gershtein, Y. Gray, R. Halkiadakis, E. Hidas, D. Hits, D. Lath, A. Panwalkar, S. Patel, R. Richards, A. Rose, K. Schnetzer, S. Somalwar, S. Stone, R. Thomas, S. Cerizza, G. Hollingsworth, M. Spanier, S. Yang, Z. C. York, A. Asaadi, J. Eusebi, R. Gilmore, J. Gurrola, A. Kamon, T. Khotilovich, V. Montalvo, R. Nguyen, C. N. Osipenkov, I. Pakhotin, Y. Pivarski, J. Safonov, A. Sengupta, S. Tatarinov, A. Toback, D. Weinberger, M. Akchurin, N. Bardak, C. Damgov, J. Jeong, C. Kovitanggoon, K. Lee, S. W. Roh, Y. Sill, A. Volobouev, I. Wigmans, R. Yazgan, E. Appelt, E. Brownson, E. Engh, D. Florez, C. Gabella, W. Issah, M. Johns, W. Kurt, P. Maguire, C. Sheldon, A. Melo P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Balazs, M. Boutle, S. Cox, B. Francis, B. Hirosky, R. Ledovskoy, A. Lin, C. Neu, C. Yohay, R. Gollapinni, S. Harr, R. Karchin, P. E. Lamichhane, P. Mattson, M. Ne, C. Milste Sakharov, A. Anderson, M. Bachtis, M. Bellinger, J. N. Carlsmith, D. Dasu, S. Efron, J. Flood, K. Gray, L. Grogg, K. S. Grothe, M. Hall-Wilton, R. Herndon, M. Klabbers, P. Klukas, J. Lanaro, A. Lazaridis, C. Leonard, J. Loveless, R. Mohapatra, A. Palmonari, F. Reeder, D. Ross, I. Savin, A. Smith, W. H. Swanson, J. Weinberg, M. CA CMS Collaboration TI Search for Supersymmetry in pp Collisions at root s=7 TeV in Events with Two Photons and Missing Transverse Energy SO PHYSICAL REVIEW LETTERS LA English DT Article ID OF-MASS ENERGIES; E(+)E(-) COLLISIONS; BREAKING TOPOLOGIES; GRAVITINO; LEP AB A search for supersymmetry in the context of general gauge-mediated breaking with the lightest neutralino as the next-to-lightest supersymmetric particle and the gravitino as the lightest is presented. The data sample corresponds to an integrated luminosity of 36 pb(-1) recorded by the CMS experiment at the LHC. The search is performed by using events containing two or more isolated photons, at least one hadronic jet, and significant missing transverse energy. No excess of events at high missing transverse energy is observed. Upper limits on the signal cross section for general gauge-mediated supersymmetry between 0.3 and 1.1 pb at the 95% confidence level are determined for a range of squark, gluino, and neutralino masses, excluding supersymmetry parameter space that was inaccessible to previous experiments. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.; Zhukov, V.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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[Adler, V.; Cimmino, A.; Costantini, S.; Grunewald, M.; Klein, B.; Lellouch, J.; Marinov, A.; Mccartin, J.; Ryckbosch, D.; Thyssen, F.; Tytgat, M.; Vanelderen, L.; Verwilligen, P.; Walsh, S.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Charaf, O.; Clerbaux, B.; De Lentdecker, G.; Dero, V.; Gay, A. P. R.; Hammad, G. H.; Hreus, T.; Marage, E.; Thomas, L.; Velde, C. Vander; Vanlaer, P.] Univ Libre Brussels, Brussels, Belgium. [Basegmez, S.; Bruno, G.; Caudron, J.; Ceard, L.; Gil, E. Cortina; De Jeneret, J. De Favereau; Delaere, C.; Favart, D.; Giammanco, A.; Gregoire, G.; Hollar, J.; Lemaitre, V.; Liao, J.; Militaru, O.; Ovyn, S.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Schul, N.] Catholic Univ Louvain, B-1348 Louvain, Belgium. [Beliy, N.; Caebergs, T.; Daubie, E.] Univ Mons, B-7000 Mons, Belgium. [Alves, G. A.; De Jesus Damiao, D.; Pol, M. E.; Souza, M. H. G.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Carvalho, W.; Da Costa, E. 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[Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Della Ricca, G.; Montanino, D.] Univ Trieste, Trieste, Italy. [Belforte, S.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Montanino, D.; Penzo, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Heo, S. G.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Chung, J.; Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Park, H.; Ro, S. R.; Son, D.; Son, D. C.; Son, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, Zero; Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Hong, B.; Jeong, M. S.; Jo, M.; Kim, H.; Kim, J. H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.; Rhee, H. B.; Seo, E.; Shin, S.; Sim, K. S.] Korea Univ, Seoul, South Korea. [Choi, M.; Kang, S.; Kim, H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. 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A.; Khurshid, T.; Qazi, S.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Brona, G.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bluj, M.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Soltan Inst Nucl Studies, PL-00681 Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Musella, P.; Nayak, A.; Seixas, J.; Varela, J.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Belotelov, I.; Bunin, P.; Golutvin, I.; Kamenev, A.; Karjavin, V.; Kozlov, G.; Lanev, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Toropin, A.; Troitsky, S.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Kaftanov, V.; Kossov, M.; Krokhotin, A.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Katkov, I.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Sarycheva, L.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Azhgirey, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Slabospitsky, S.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.; Adzic, P.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Djordjevic, M.; Krpic, D.; Milosevic, J.; Aguilar-Benitez, M.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Djordjevic, M.; Krpic, D.; Milosevic, J.; Aguilar-Benitez, M.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Arce, P.; Battilana, C.; Calvo, E.; Cepeda, M.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Diez Pardos, C.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.] Univ Oviedo, Oviedo, Spain. [Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Vizan Garcia, J. M.; Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Jorda, C.; Lobelle Pardo, P.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Gomez, J. Piedra; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Hammer, J.; Delaere, C.; Darmenov, N.; Genchev, V.; Iaydjiev, P.; Jung, H.; Hajdu, C.; Sikler, F.; Mohanty, A. K.; Chiorboli, M.; De Guio, F.; Montoya, C. A. Carrillo; Iorio, A. O. M.; Lucaroni, A.; Taroni, S.; Boccali, T.; Tonelli, G.; Grassi, M.; Pandolfi, F.; Botta, C.; Graziano, A.; Kossov, M.; Grishin, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Baillon, P.; Ball, A. H.; Barney, D.; Bell, A. J.; Benedetti, D.; Bernet, C.; Bialas, W.; Bloch, P.; Bocci, A.; Bolognesi, S.; Bona, M.; Breuker, H.; Bunkowski, K.; Camporesi, T.; Cerminara, G.; Coarasa Perez, J. A.; Cure, B.; D'Enterria, D.; De Roeck, A.; Di Guida, S.; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Gaddi, A.; Gennai, S.; Georgiou, G.; Gerwig, H.; Gigi, D.; Gill, K.; Giordano, D.; Glege, F.; Gomez-Reino Garrido, R.; Gouzevitch, M.; Govoni, P.; Gowdy, S.; Guiducci, L.; Hansen, M.; Hartl, C.; Harvey, J.; Hegeman, J.; Hegner, B.; Hoffmann, H. F.; Honma, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Lecoq, P.; Lourenco, C.; Maeki, T.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Maurisset, A.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Nesvold, E.; Nguyen, M.; Orimoto, T.; Orsini, L.; Perez, E.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Polese, G.; Racz, A.; Rodrigues Antunes, J.; Rolandi, G.; Rommerskirchen, T.; Rovelli, C.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Segoni, I.; Sharma, A.; Siegrist, P.; Simon, M.; Sphicas, P.; Spiropulu, M.; Stoye, M.; Tropea, P.; Tsirou, A.; Vichoudis, P.; Voutilainen, M.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Starodumov, A.; Bortignon, P.; Caminada, L.; Marchica, C.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Caminada, L.; Chanon, N.; Chen, Z.; Cittolin, S.; Dissertori, G.; Dittmar, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Herve, A.; Hintz, W.; Lecomte, P.; Lustermann, W.; Marchica, C.; del Arbol, P. Martinez Ruiz; Meridiani, P.; Milenovic, P.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pape, L.; Pauss, F.; Punz, T.; Rizzi, A.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Sawley, M. -C.; Stieger, B.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, M.; Wehrli, L.; Weng, J.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aguilo, E.; Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Otiougova, P.; Regenfus, C.; Robmann, P.; Schmidt, A.; Snoek, H.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Volpe, R.; Wu, J. H.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Topaksu, A. Kayis; Nart, A.; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Uzun, D.; Vergili, L. N.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Deliomeroglu, M.; Demir, D.; Lmez, E. Gu; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Levchuk, L.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Bostock, F.; Brooke, J. J.; Cheng, T. L.; Clement, E.; Cussans, D.; Frazier, R.; Goldstein, J.; Grimes, M.; Hansen, M.; Hartley, D.; Heath, G. P.; Heath, H. F.; Jackson, J.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Ward, S.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Camanzi, B.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Ballin, J.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Lyons, L.; MacEvoy, B. C.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rompotis, N.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Tourneur, S.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Wardrope, D.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Barrett, M.; Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Martin, W.; Reid, I. D.; Teodorescu, L.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.] Baylor Univ, Waco, TX 76798 USA. [Bose, T.; Jarrin, E. Carrera; Fantasia, C.; Heister, A.; John, J. St.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Avetisyan, A.; Bhattacharya, S.; Chou, J. P.; Cutts, D.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Landsberg, G.; Narain, M.; Nguyen, D.; Segala, M.; Sinthuprasith, T.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Cox, P. T.; Dolen, J.; Erbacher, R.; Friis, E.; Ko, W.; Kopecky, A.; Lander, R.; Liu, H.; Maruyama, S.; Miceli, T.; Nikolic, M.; Pellett, D.; Robles, J.; Salur, S.; Schwarz, T.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez; Veelken, C.] Univ Calif Davis, Davis, CA 95616 USA. [Brochero Cifuentes, J. A.; Andreev, V.; Arisaka, K.; Cline, D.; Cousins, R.; Deisher, A.; Duris, J.; Erhan, S.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Tucker, J.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Chandra, A.; Clare, R.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Kao, S. C.; Liu, F.; Liu, H.; Long, O. R.; Luthra, A.; Nguyen, H.; Shen, B. C.; Stringer, R.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Dusinberre, E.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pi, H.; Pieri, M.; Ranieri, R.; Sani, M.; Sharma, V.; Simon, S.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; Vlimant, J. R.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Spiropulu, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Gataullin, M.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Shin, K.; Timciuc, V.; Traczyk, P.; Veverka, J.; Wilkinson, R.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Akgun, B.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Jun, S. Y.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Dinardo, M. E.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Gaz, A.; Heyburn, B.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.; Zang, S. L.] Univ Colorado, Boulder, CO 80309 USA. [Agostino, L.; Alexander, J.; Cassel, D.; Chatterjee, A.; Das, S.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Kaufman, G. Nicolas; Patterson, J. R.; Puigh, D.; Ryd, A.; Salvati, E.; Shi, X.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Biselli, A.; Cirino, G.; Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Atac, M.; Bakken, J. A.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Borcherding, F.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Cooper, W.; Eartly, D. P.; Elvira, V. D.; Esen, S.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Green, D.; Gunthoti, K.; Gutsche, O.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jensen, H.; Johnson, M.; Joshi, U.; Khatiwada, R.; Klima, B.; Kousouris, K.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Limon, P.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Mason, D.; McBride, P.; Miao, T.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Pordes, R.; Prokofyev, O.; Saoulidou, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Tan, P.; Taylor, L.; Tkaczyk, S.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Gomez, J. Piedra; Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Matchev, K.; Mitselmakher, G.; Muniz, L.; Prescott, C.; Remington, R.; Schmitt, M.; Scurlock, B.; Sellers, P.; Skhirtladze, N.; Snowball, M.; Wang, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Ceron, C.; Gaultney, V.; Kramer, L.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Mesa, D.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bandurin, D.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Quertenmont, L.; Sekmen, S.; Veeraraghavan, V.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Guragain, S.; Hohlmann, M.; Kalakhety, H.; Ralich, R.; Vodopiyanov, I.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Callner, J.; Cavanaugh, R.; Dragoiu, C.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kunde, G. J.; Lacroix, F.; Malek, M.; O'Brien, C.; Silvestre, C.; Smoron, A.; Strom, D.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Duru, F.; Lae, C. K.; McCliment, E.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Olson, J.; Onel, Y.; Ozok, F.; Sen, S.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bonato, A.; Eskew, C.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Rappoccio, S.; Swartz, M.; Tran, N. V.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Grachov, O.; Iii, R. P. Kenny; Murray, M.; Noonan, D.; Sanders, S.; Wood, J. S.; Zhukova, V.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Bolton, T.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.; Wan, Z.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Boutemeur, M.; Eno, S. C.; Ferencek, D.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kirn, M.; Lu, Y.; Mignerey, A. C.; Rossato, K.; Rumerio, P.; Santanastasio, F.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.; Twedt, E.] Univ Maryland, College Pk, MD 20742 USA. [Wyslouch, B.; Alver, B.; Bauer, G.; Bendavid, J.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Everaerts, P.; Ceballos, G. Gomez; Goncharov, M.; Hahn, K. A.; Harris, P.; Kim, Y.; Klute, M.; Lee, Y. -J.; Li, W.; Loizides, C.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Rudolph, M.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Wenger, E. A.; Xie, S.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.] MIT, Cambridge, MA 02139 USA. [Cooper, S. I.; Cushman, P.; Dahmes, B.; De Benedetti, A.; Dudero, P. R.; Franzoni, G.; Haupt, J.; Klapoetke, K.; Kubota, Y.; Mans, J.; Rekovic, V.; Rusack, R.; Sasseville, M.; Singovsky, A.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Godang, R.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, University, MS 38677 USA. [Bloom, K.; Bose, S.; Butt, J.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kelly, T.; Kravchenko, I.; Lazo-Flores, J.; Malbouisson, H.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Baur, U.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Shipkowski, S. P.; Smith, K.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Boeriu, O.; Chasco, M.; Reucroft, S.; Swain, J.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Kubik, A.; Odell, N.; Ofierzynski, R. 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JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MST (Russia); MAE (Russia); MSTD (Serbia); MICINN (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK (Turkey); TAEK (Turkey); STFC (United Kingdom); DOE (USA); NSF (USA) FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine. We thank the technical and administrative staff at CERN and other CMS institutes and acknowledge support from: FMSR (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences and NICPB (Estonia); Academy of Finland, ME, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MST and MAE (Russia); MSTD (Serbia); MICINN and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK and TAEK (Turkey); STFC (United Kingdom); DOE and NSF (USA). NR 30 TC 43 Z9 43 U1 1 U2 46 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 24 PY 2011 VL 106 IS 21 AR 211802 DI 10.1103/PhysRevLett.106.211802 PG 15 WC Physics, Multidisciplinary SC Physics GA 767YE UT WOS:000290895300002 PM 21699288 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hammer, J Hansel, S Hartl, C Hoch, M Hormann, N Hrubec, J Jeitler, M Kasieczka, G Kiesenhofer, W Krammer, M Liko, D Mikulec, I Pernicka, M Rohringer, H Schofbeck, R Strauss, J Teischinger, F Wagner, P Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Benucci, L De Wolf, EA Janssen, X Maes, T Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Blekman, F Blyweert, S D'Hondt, J Devroede, O Suarez, RG Kalogeropoulos, A Maes, J Maes, M Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Charaf, O Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hammad, GH Hreus, T Marage, PE Thomas, L Vander 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CA CMS Collaboration TI Study of Z Boson Production in PbPb Collisions at root s(NN)=2.76 TeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID HEAVY-ION COLLISIONS; LHC AB A search for Z bosons in the mu(+)mu(-) decay channel has been performed in PbPb collisions at root s(NN) = 2.76 TeV with the CMS detector at the LHC, in a 7.2 mu b(-1) data sample. The number of opposite-sign muon pairs observed in the 60-120 GeV/c(2) invariant mass range is 39, corresponding to a yield per unit of rapidity (y) and per minimum bias event of [33.8 +/- 5.5(stat) +/- 4.4(syst)] x 10(-8), in the vertical bar y vertical bar < 2.0 range. Rapidity, transverse momentum, and centrality dependencies are also measured. The results agree with next-to-leading order QCD calculations, scaled by the number of incoherent nucleon-nucleon collisions. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. 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M.; Caponeri, B.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Menichelli, M.; Nappi, A.; Santocchia, A.; Taroni, S.; Valdata, M.; Volpe, R.; Pioppi, M.] Univ Perugia, Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Palmonari, F.; Segneri, G.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bernardini, J.; Boccali, T.; Fiori, F.; Messineo, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Azzurri, P.; Broccolo, G.; D'Agnolo, R. T.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. 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[Amapane, N.; Argiro, S.; Botta, C.; Castello, R.; Costa, M.; Graziano, A.; Marone, M.; Migliore, E.; Mila, G.; Monaco, V.; Musich, M.; Pelliccioni, M.; Romero, A.; Sacchi, R.; Sola, V.; Solano, A.; Trocino, D.; Pereira, A. Vilela] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Montanino, D.; Penzo, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Della Ricca, G.; Montanino, D.] Univ Trieste, Trieste, Italy. [Heo, S. G.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Chung, J.; Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Park, H.; Ro, S. R.; Son, D.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, Zero; Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Hong, B.; Jeong, M. S.; Jo, M.; Kim, H.; Kim, J. H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.; Rhee, H. B.; Seo, E.; Shin, S.; Sim, K. S.] Korea Univ, Seoul, South Korea. [Choi, M.; Kang, S.; Kim, H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Martisiute, D.; Petrov, P.; Sabonis, T.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ahmed, I.; Asghar, M. I.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Qazi, S.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bluj, M.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Soltan Inst Nucl Studies, PL-00681 Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Musella, P.; Nayak, A.; Seixas, J.; Varela, J.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Belotelov, I.; Bunin, P.; Golutvin, I.; Kamenev, A.; Karjavin, V.; Kozlov, G.; Lanev, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Toropin, A.; Troitsky, S.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Kaftanov, V.; Kossov, M.; Krokhotin, A.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Zhukov, V.; Boos, E.; Demiyanov, A.; Ershov, A.; Gribushin, A.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Sarycheva, L.; Savrin, V.; Snigirev, A.; Vardanyan, I.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Azhgirey, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Slabospitsky, S.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Maestre, J. Alcaraz; Arce, P.; Battilana, C.; Calvo, E.; Cepeda, M.; Cerrada, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Diez Pardos, C.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Redondo, I.; Romero, L.; Santaolalla, J.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chamizo Llatas, M.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Jorda, C.; Lobelle Pardo, P.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria, E-39005 Santander, Spain. [Hammer, J.; Darmenov, N.; Genchev, V.; Iaydjiev, P.; Hajdu, C.; Mohanty, A. K.; Lusito, L.; Chiorboli, M.; Ghezzi, A.; Malberti, M.; Lucaroni, A.; Tonelli, G.; Venturi, A.; Pandolfi, F.; Botta, C.; Graziano, A.; Pelliccioni, M.; Pereira, A. Vilela; Kossov, M.; Grishin, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Baillon, P.; Ball, A. H.; Barney, D.; Bell, A. J.; Benedetti, D.; Bernet, C.; Bialas, W.; Bloch, P.; Bocci, A.; Bolognesi, S.; Bona, M.; Breuker, H.; Brona, G.; Bunkowski, K.; Camporesi, T.; Cerminara, G.; Perez, J. A. Coarasa; Cure, B.; D'Enterria, D.; De Roeck, A.; Di Guida, S.; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Gaddi, A.; Gennai, S.; Georgiou, G.; Gerwig, H.; Gigi, D.; Gill, K.; Giordano, D.; Glege, F.; Garrido, R. Gomez-Reino; Gouzevitch, M.; Govoni, P.; Gowdy, S.; Guiducci, L.; Hansen, M.; Harvey, J.; Hegeman, J.; Hegner, B.; Hoffmann, H. F.; Honma, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Lecoq, P.; Lourenco, C.; Maeki, T.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Nesvold, E.; Nguyen, M.; Orimoto, T.; Orsini, L.; Perez, E.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Polese, G.; Racz, A.; Antunes, J. Rodrigues; Rolandi, G.; Rommerskirchen, T.; Rovelli, C.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Segoni, I.; Sharma, A.; Siegrist, P.; Simon, M.; Sphicas, P.; Spiropulu, M.; Stoeckli, F.; Stoye, M.; Tropea, P.; Tsirou, A.; Vichoudis, P.; Voutilainen, M.; Zeuner, W. D.; Sharma, V.; Hall-Wilton, R.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Starodumov, A.; Caminada, L.; Marchica, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bortignon, P.; Caminada, L.; Chen, Z.; Cittolin, S.; Dissertori, G.; Dittmar, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Herve, A.; Hintz, W.; Lecomte, P.; Lustermann, W.; Marchica, C.; del Arbol, P. Martinez Ruiz; Meridiani, P.; Milenovic, P.; Moortgat, F.; Nef, P.; Nessi-Tedaldi, F.; Pape, L.; Pauss, F.; Punz, T.; Rizzi, A.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Sawley, M. -C.; Stieger, B.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, M.; Wehrli, L.; Weng, J.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aguilo, E.; Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Regenfus, C.; Robmann, P.; Schmidt, A.; Snoek, H.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, E. A.; Chen, K. H.; Chen, W. T.; Dutta, S.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, M. H.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Wu, J. H.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Demir, Z.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Topaksu, A. Kayis; Nart, A.; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Uzun, D.; Vergili, L. N.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Deliomeroglu, M.; Demir, D.; Guelmez, E.; Halu, A.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Levchuk, L.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Bell, P.; Bostock, F.; Brooke, J. J.; Cheng, T. L.; Clement, E.; Cussans, D.; Frazier, R.; Goldstein, J.; Grimes, M.; Hansen, M.; Hartley, D.; Heath, G. P.; Heath, H. F.; Huckvale, B.; Jackson, J.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Ward, S.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Camanzi, B.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Ballin, J.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Davies, G.; Della Negra, M.; Fulcher, J.; Futyan, D.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Karapostoli, G.; MacEvoy, B. C.; Magnan, A. -M.; Marrouche, J.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rompotis, N.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Barrett, M.; Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Martin, W.; Reid, I. D.; Teodorescu, L.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.] Baylor Univ, Waco, TX 76798 USA. [Bose, T.; Jarrin, E. Carrera; Fantasia, C.; Heister, A.; John, J. St.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Avetisyan, A.; Bhattacharya, S.; Chou, J. P.; Cutts, D.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Landsberg, G.; Narain, M.; Nguyen, D.; Segala, M.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Cox, P. T.; Dolen, J.; Erbacher, R.; Friis, E.; Ko, W.; Kopecky, A.; Lander, R.; Liu, H.; Maruyama, S.; Miceli, T.; Nikolic, M.; Pellett, D.; Robles, J.; Salur, S.; Schwarz, T.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez; Veelken, C.] Univ Calif Davis, Davis, CA 95616 USA. [Felcini, M.; Andreev, V.; Arisaka, K.; Cline, D.; Cousins, R.; Deisher, A.; Duris, J.; Erhan, S.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Tucker, J.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Chandra, A.; Clare, R.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Kao, S. C.; Liu, F.; Liu, H.; Long, O. R.; Luthra, A.; Nguyen, H.; Shen, B. C.; Stringer, R.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Dusinberre, E.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pi, H.; Pieri, M.; Ranieri, R.; Sani, M.; Sharma, V.; Simon, S.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Rthwein, F. Wu; Yagil, A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; Vlimant, J. R.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Spiropulu, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Gataullin, M.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Timciuc, V.; Traczyk, P.; Veverka, J.; Wilkinson, R.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Akgun, B.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Jun, S. Y.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Dinardo, M. E.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Gaz, A.; Heyburn, B.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.; Zang, S. L.] Univ Colorado, Boulder, CO 80309 USA. [Agostino, L.; Alexander, J.; Cassel, D.; Chatterjee, A.; Das, S.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Kaufman, G. Nicolas; Patterson, J. R.; Puigh, D.; Ryd, A.; Shi, X.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Biselli, A.; Cirino, G.; Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Atac, M.; Bakken, J. A.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Borcherding, F.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Cooper, W.; Eartly, D. P.; Elvira, V. D.; Esen, S.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Green, D.; Gunthoti, K.; Gutsche, O.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jensen, H.; Johnson, M.; Joshi, U.; Khatiwada, R.; Klima, B.; Kousouris, K.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Limon, P.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Mason, D.; McBride, P.; Miao, T.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Pordes, R.; Prokofyev, O.; Saoulidou, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Tan, P.; Taylor, L.; Tkaczyk, S.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Piedra Gomez, J.; Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Goldberg, S.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Matchev, K.; Mitselmakher, G.; Muniz, L.; Pakhotin, Y.; Prescott, C.; Remington, R.; Schmitt, M.; Scurlock, B.; Sellers, P.; Skhirtladze, N.; Wang, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Ceron, C.; Gaultney, V.; Kramer, L.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bandurin, D.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Quertenmont, L.; Sekmen, S.; Veeraraghavan, V.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Guragain, S.; Hohlmann, M.; Kalakhety, H.; Ralich, R.; Vodopiyanov, I.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Callner, J.; Cavanaugh, R.; Dragoiu, C.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kunde, G. J.; Lacroix, F.; Malek, M.; O'Brien, C.; Silvestre, C.; Smoron, A.; Strom, D.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Duru, F.; Lae, C. K.; McCliment, E.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Olson, J.; Onel, Y.; Ozok, F.; Sen, S.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bonato, A.; Eskew, C.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Rappoccio, S.; Swartz, M.; Tran, N. V.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. 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MST (Russia); MAE (Russia); MSTD (Serbia); MICINN (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK (Turkey); TAEK (Turkey); STFC (United Kingdom); DOE (USA); NSF (USA) FX We thank Bryon Neufeld, Hannu Paukkunen, Carlos Salgado, Ivan Vitev, and Ramona Vogt for fruitful theoretical inputs on the nuclear effects involved in Z production. We wish to congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine in 2010. We thank the technical and administrative staff at CERN and other CMS institutes, and acknowledge support from FMSR (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); Academy of Sciences and NICPB (Estonia); Academy of Finland, ME, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); PAEC (Pakistan); SCSR (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MST and MAE (Russia); MSTD (Serbia); MICINN and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK and TAEK (Turkey); STFC (United Kingdom); DOE and NSF (USA). NR 22 TC 63 Z9 63 U1 1 U2 47 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 24 PY 2011 VL 106 IS 21 AR 212301 DI 10.1103/PhysRevLett.106.212301 PG 14 WC Physics, Multidisciplinary SC Physics GA 767YE UT WOS:000290895300004 PM 21699291 ER PT J AU Nicholson, A Ge, WH Zhang, XT Riera, J Daghofer, M Oles, AM Martins, GB Moreo, A Dagotto, E AF Nicholson, Andrew Ge, Weihao Zhang, Xiaotian Riera, Jose Daghofer, Maria Oles, Andrzej M. Martins, George B. Moreo, Adriana Dagotto, Elbio TI Competing Pairing Symmetries in a Generalized Two-Orbital Model for the Pnictide Superconductors SO PHYSICAL REVIEW LETTERS LA English DT Article ID ELECTRONS AB We introduce and study an extended "t-U-J'' two-orbital model for the pnictides that includes Heisenberg terms deduced from the strong coupling expansion. Including these J terms explicitly allows us to enhance the strength of the (pi, 0)-(0, pi) spin order which favors the presence of tightly bound pairing states even in the small clusters that are here exactly diagonalized. The A(1g) and B-2g pairing symmetries are found to compete in the realistic spin-ordered and metallic regime. The dynamical pairing susceptibility additionally unveils low-lying B-1g states, suggesting that small changes in parameters may render any of the three channels stable. C1 [Nicholson, Andrew; Ge, Weihao; Zhang, Xiaotian; Moreo, Adriana; Dagotto, Elbio] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Nicholson, Andrew; Ge, Weihao; Zhang, Xiaotian; Moreo, Adriana; Dagotto, Elbio] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Riera, Jose] Univ Nacl Rosario, Inst Fis Rosario, RA-2000 Rosario, Santa Fe, Argentina. [Daghofer, Maria] IFW Dresden, D-01171 Dresden, Germany. [Oles, Andrzej M.] Max Planck Inst Festkorperforsch, D-70569 Stuttgart, Germany. [Oles, Andrzej M.] Jagiellonian Univ, M Smoluchowski Inst Phys, PL-30059 Krakow, Poland. [Martins, George B.] Oakland Univ, Dept Phys, Rochester, MI 48309 USA. RP Nicholson, A (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RI Daghofer, Maria/C-5762-2008; Riera, Jose/A-1234-2008; Martins, George/C-9756-2012 OI Daghofer, Maria/0000-0001-9434-8937; Riera, Jose/0000-0003-4546-1137; Martins, George/0000-0001-7846-708X FU U.S. DOE, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; CONICET, Argentina; DFG; Foundation for Polish Science (FNP); Polish government [N202 069639] FX This work was supported by the U.S. DOE, Office of Basic Energy Sciences, Materials Sciences and Engineering Division (A. N., W. G., X. Z., G. M., A. M., E. D.), CONICET, Argentina (J. R.), the DFG under the Emmy-Noether program (M. D.), and by the Foundation for Polish Science (FNP) and the Polish government Project N202 069639 (A. M. O.). Conversations with D.X. Yao and Thomas Prestel are acknowledged. NR 28 TC 40 Z9 40 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 24 PY 2011 VL 106 IS 21 AR 217002 DI 10.1103/PhysRevLett.106.217002 PG 4 WC Physics, Multidisciplinary SC Physics GA 767YE UT WOS:000290895300011 PM 21699330 ER PT J AU Ren, X Bray, I Fursa, DV Colgan, J Pindzola, MS Pfluger, T Senftleben, A Xu, S Dorn, A Ullrich, J AF Ren, X. Bray, I. Fursa, D. V. Colgan, J. Pindzola, M. S. Pflueger, T. Senftleben, A. Xu, S. Dorn, A. Ullrich, J. TI Electron-impact ionization of helium: A comprehensive experiment benchmarks theory SO PHYSICAL REVIEW A LA English DT Article ID DIFFERENTIAL CROSS-SECTIONS; ENERGY; HE AB Single ionization of helium by 70.6-eV electron impact is studied in a comprehensive experiment covering a major part of the entire collision kinematics and the full 4 pi solid angle for the emitted electron. The absolutely normalized triple-differential experimental cross sections are compared with results from the convergent close-coupling (CCC) and the time-dependent close-coupling (TDCC) theories. Whereas excellent agreement with the TDCC prediction is only found for equal energy sharing, the CCC calculations are in excellent agreement with essentially all experimentally observed dynamical features, including the absolute magnitude of the cross sections. C1 [Ren, X.; Pflueger, T.; Senftleben, A.; Xu, S.; Dorn, A.; Ullrich, J.] Max Planck Inst Nucl Phys, DE-69117 Heidelberg, Germany. [Bray, I.; Fursa, D. V.] Curtin Univ, ARC Ctr Antimatter Matter Studies, Perth, WA, Australia. [Colgan, J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Pindzola, M. S.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. RP Ren, X (reprint author), Max Planck Inst Nucl Phys, DE-69117 Heidelberg, Germany. EM Alexander.Dorn@mpi-hd.mpg.de RI Fursa, Dmitry/C-2301-2009; Bray, Igor/B-8586-2009; Xu, Shenyue/G-3907-2015; OI Fursa, Dmitry/0000-0002-3951-9016; Bray, Igor/0000-0001-7554-8044; Xu, Shenyue/0000-0001-9872-2244; Colgan, James/0000-0003-1045-3858; Senftleben, Arne/0000-0003-0932-9892 FU DFG [RE 2966/1-1]; Australian Research Council; Australian National Computational Infrastructure Facility and its Western Australian node iVEC; US Department of Energy [DE-AC5206NA25396]; DOE; NSF FX X.R. is grateful for support from DFG Project No. RE 2966/1-1. I.B. and D.V.F. are grateful for the support of the Australian Research Council and the Australian National Computational Infrastructure Facility and its Western Australian node iVEC. The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the National Nuclear Security Administration of the US Department of Energy under Contract No. DE-AC5206NA25396. A portion of this work was performed through DOE and NSF grants to Auburn University. NR 21 TC 26 Z9 26 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 J9 PHYS REV A JI Phys. Rev. A PD MAY 24 PY 2011 VL 83 IS 5 AR 052711 DI 10.1103/PhysRevA.83.052711 PG 6 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 767YF UT WOS:000290895400010 ER PT J AU Adekola, AS Bardayan, DW Blackmon, JC Brune, CR Chae, KY Domizioli, C Greife, U Heinen, Z Hornish, MJ Jones, KL Kozub, RL Livesay, RJ Ma, Z Massey, TN Moazen, B Nesaraja, CD Pain, SD Shriner, JF Smith, ND Smith, MS Thomas, JS Visser, DW Voinov, AV AF Adekola, A. S. Bardayan, D. W. Blackmon, J. C. Brune, C. R. Chae, K. Y. Domizioli, C. Greife, U. Heinen, Z. Hornish, M. J. Jones, K. L. Kozub, R. L. Livesay, R. J. Ma, Z. Massey, T. N. Moazen, B. Nesaraja, C. D. Pain, S. D. Shriner, J. F., Jr. Smith, N. D. Smith, M. S. Thomas, J. S. Visser, D. W. Voinov, A. V. TI First proton-transfer study of F-18 + p resonances relevant for novae SO PHYSICAL REVIEW C LA English DT Article ID GAMMA-RAY EMISSION; REACTION-RATES; NOVA; CYGNI AB The F-18(p, alpha)O-15 reaction is the predominant destruction mechanism in novae of the radionuclide F-18, a target of gamma-ray observatories. Thus, its rate is important for understanding F-18 production in novae. We have studied resonances in the F-18 + p system by making a measurement of a proton-transfer reaction F-18(d, n). We have observed 15 Ne-19 levels, 5 of which are below the proton threshold, including a subthreshold state, which has significant l(p) = 0 strength. Our data provide a direct determination of the spectroscopic strength of these states and new constraints on their spins and parities, thereby resolving a controversy, which involves the 8- and 38-keV resonances. The F-18(p, alpha)O-15 reaction rate is reevaluated, which takes the subthreshold resonance and other new information determined in this experiment into account. C1 [Adekola, A. S.; Brune, C. R.; Heinen, Z.; Hornish, M. J.; Massey, T. N.; Voinov, A. V.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Adekola, A. S.; Jones, K. L.; Pain, S. D.; Thomas, J. S.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Bardayan, D. W.; Blackmon, J. C.; Nesaraja, C. D.; Smith, M. S.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Chae, K. Y.; Domizioli, C.; Ma, Z.; Moazen, B.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Greife, U.; Livesay, R. J.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. [Kozub, R. L.; Shriner, J. F., Jr.; Smith, N. D.] Tennessee Technol Univ, Dept Phys, Cookeville, TN 38505 USA. [Visser, D. W.] Univ N Carolina, Dept Phys & Astron, Chapel Hill, NC 27599 USA. RP Adekola, AS (reprint author), Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. EM aadekola@physics.rutgers.edu RI Jones, Katherine/B-8487-2011; Pain, Steven/E-1188-2011; OI Jones, Katherine/0000-0001-7335-1379; Pain, Steven/0000-0003-3081-688X; Nesaraja, Caroline/0000-0001-5571-8341 FU U.S. Department of Energy [DE-FG02-88ER40387, DE-FG02-93ER40789, DE-FG02-96ER40990, DE-FG02-96ER40955]; National Nuclear Security Administration through the U.S. Department of Energy [DE-FG52-08NA28552]; National Nuclear Security Administration through the National Science Foundation FX We thank the staff of the HRIBF for making this experiment possible. This work was supported, in part, by the U.S. Department of Energy under Grants No. DE-FG02-88ER40387 (OU), No. DE-FG02-93ER40789 (CSM), No. DE-FG02-96ER40990, and No. DE-FG02-96ER40955 (TTU) and the National Nuclear Security Administration under the Stewardship Science Academic Alliances program through the U.S. Department of Energy Cooperative Agreement No. DE-FG52-08NA28552 and the National Science Foundation (RUTGERS). NR 29 TC 18 Z9 18 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 J9 PHYS REV C JI Phys. Rev. C PD MAY 24 PY 2011 VL 83 IS 5 AR 052801 DI 10.1103/PhysRevC.83.052801 PG 5 WC Physics, Nuclear SC Physics GA 767YM UT WOS:000290896300001 ER PT J AU Ichikawa, T Kanada-En'yo, Y Moller, P AF Ichikawa, Takatoshi Kanada-En'yo, Yoshiko Moeller, Peter TI Cluster formations in deformed states for Si-28 and S-32 SO PHYSICAL REVIEW C LA English DT Article ID HIGH-SPIN STATES; Z NUCLEI; FISSION-BARRIERS; UNSTABLE NUCLEI; MEAN-FIELD; SHELL; HEAVY; BANDS; DEFORMATIONS; SCATTERING AB We study cluster formation in strongly deformed states for Si-28 and S-32 using a macroscopic-microscopic model. The study is based on calculated total-energy surfaces, which are the sums of deformation-dependent macroscopic-microscopic potential-energy surfaces and rotational-energy contributions. We analyze the angular-momentum-dependent total-energy surfaces and identify the normal-and superdeformed states in Si-28 and S-32. We show that at sufficiently high angular momenta strongly deformed minima appear. The corresponding microscopic density distributions show cluster structures that closely resemble the O-16 + C-12 and O-16 + O-16 configurations. At still higher deformations, beyond the minima, valleys develop in the calculated surfaces. These valleys lead to mass divisions that correspond to the target-projectile configurations for which molecular resonance states have been observed. We discuss the relation between the one-body deformed minima and the two-body molecular-resonance states. C1 [Ichikawa, Takatoshi] Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan. [Kanada-En'yo, Yoshiko] Kyoto Univ, Dept Phys, Kyoto 6068502, Japan. [Moeller, Peter] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Ichikawa, T (reprint author), Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan. FU MEXT of Japan; JPSJ Kakenhi [22540275]; National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; University of Tennessee [DE-FG02-06ER41407] FX This work was done under the Yukawa International Project for Quark-Hadron Sciences (YIPQS) and was partly supported by the GCOE program "The Next Generation of Physics, Spun from Universality and Emergence" under MEXT of Japan. The work of Y.K.-E. was supported by JPSJ Kakenhi (Grant No. 22540275). P. M. acknowledges that this work was carried out under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396 and was also supported by a travel grant to the Japan-US Theory Institute for Physics with Exotic Nuclei (JUSTIPEN) under Grant No. DE-FG02-06ER41407 (University of Tennessee). The numerical calculations were carried out on Altix3700 BX2 at YITP at the Kyoto University. NR 42 TC 13 Z9 13 U1 0 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 J9 PHYS REV C JI Phys. Rev. C PD MAY 24 PY 2011 VL 83 IS 5 AR 054319 DI 10.1103/PhysRevC.83.054319 PG 7 WC Physics, Nuclear SC Physics GA 767YM UT WOS:000290896300003 ER PT J AU Abbasi, R Abdou, Y Abu-Zayyad, T Adams, J Aguilar, JA Ahlers, M Andeen, K Auffenberg, J Bai, X Baker, M Barwick, SW Bay, R Alba, JLB Beattie, K Beatty, JJ Bechet, S Becker, JK Becker, KH Benabderrahmane, ML BenZvi, S Berdermann, J Berghaus, P Berley, D Bernardini, E Bertrand, D Besson, DZ Bindig, D Bissok, M Blaufuss, E Blumenthal, J Boersma, DJ Bohm, C Bose, D Boser, S Botner, O Braun, J Brown, AM Buitink, S Carson, M Chirkin, D Christy, B Clem, J Clevermann, F Cohen, S Colnard, C Cowen, DF D'Agostino, MV Danninger, M Daughhetee, J Davis, JC De Clercq, C Demirors, L Denger, T Depaepe, O Descamps, F Desiati, P de Vries-Uiterweerd, G DeYoung, T Diaz-Velez, JC Dierckxsens, M Dreyer, J Dumm, JP Ehrlich, R Eisch, J Ellsworth, RW Engdegard, O Euler, S Evenson, PA Fadiran, O Fazely, AR Fedynitch, A Feusels, T Filimonov, K Finley, C Fischer-Wasels, T Foerster, MM Fox, BD Franckowiak, A Franke, R Gaisser, TK Gallagher, J Geisler, M Gerhardt, L Gladstone, L Glusenkamp, T Goldschmidt, A Goodman, JA Gora, D Grant, D Griesel, T Gross, A Grullon, S Gurtner, M Ha, C Hallgren, A Halzen, F Han, K Hanson, K Heinen, D Helbing, K Herquet, P Hickford, S Hill, GC Hoffman, KD Homeier, A Hoshina, K Hubert, D Huelsnitz, W Hulss, JP Hulth, PO Hultqvist, K Hussain, S Ishihara, A Jacobsen, J Japaridze, GS Johansson, H Joseph, JM Kampert, KH Kappes, A Karg, T Karle, A Kelley, JL Kenny, P Kiryluk, J Kislat, F Klein, SR Kohne, JH Kohnen, G Kolanoski, H Kopke, L Kopper, S Koskinen, DJ Kowalski, M Kowarik, T Krasberg, M Krings, T Kroll, G Kuwabara, T Labare, M Lafebre, S Laihem, K Landsman, H Larson, MJ Lauer, R Lunemann, J Madsen, J Majumdar, P Marotta, A Maruyama, R Mase, K Matis, HS Meagher, K Merck, M Meszaros, P Meures, T Middell, E Milke, N Miller, J Montaruli, T Morse, R Movit, SM Nahnhauer, R Nam, JW Naumann, U Niessen, P Nygren, DR Odrowski, S Olivas, A Olivo, M O'Murchadha, A Ono, M Panknin, S Paul, L Heros, CPD Petrovic, J Piegsa, A Pieloth, D Porrata, R Posselt, J Price, PB Przybylski, GT Rawlins, K Redl, P Resconi, E Rhode, W Ribordy, M Rizzo, A Rodrigues, JP Roth, P Rothmaier, F Rott, C Ruhe, T Rutledge, D Ruzybayev, B Ryckbosch, D Sander, HG Santander, M Sarkar, S Schatto, K Schmidt, T Schonwald, A Schukraft, A Schultes, A Schulz, O Schunck, M Seckel, D Semburg, B Seo, SH Sestayo, Y Seunarine, S Silvestri, A Slipak, A Spiczak, GM Spiering, C Stamatikos, M Stanev, T Stephens, G Stezelberger, T Stokstad, RG Stossl, A Stoyanov, S Strahler, EA Straszheim, T Stur, M Sullivan, GW Swillens, Q Taavola, H Taboada, I Tamburro, A Tepe, A Ter-Antonyan, S Tilav, S Toale, PA Toscano, S Tosi, D Turcan, D van Eijndhoven, N Vandenbroucke, J Van Overloop, A van Santen, J Vehring, M Voge, M Walck, C Waldenmaier, T Wallraff, M Walter, M Weaver, C Wendt, C Westerhoff, S Whitehorn, N Wiebe, K Wiebusch, CH Williams, DR Wischnewski, R Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, C Xu, XW Yodh, G Yoshida, S Zarzhitsky, P AF Abbasi, R. Abdou, Y. Abu-Zayyad, T. Adams, J. Aguilar, J. A. Ahlers, M. Andeen, K. Auffenberg, J. Bai, X. Baker, M. Barwick, S. W. Bay, R. Alba, J. L. Bazo Beattie, K. Beatty, J. J. Bechet, S. Becker, J. K. Becker, K. -H. Benabderrahmane, M. L. BenZvi, S. Berdermann, J. Berghaus, P. Berley, D. Bernardini, E. Bertrand, D. Besson, D. Z. Bindig, D. Bissok, M. Blaufuss, E. Blumenthal, J. Boersma, D. J. Bohm, C. Bose, D. Boeser, S. Botner, O. Braun, J. Brown, A. M. Buitink, S. Carson, M. Chirkin, D. Christy, B. Clem, J. Clevermann, F. Cohen, S. Colnard, C. Cowen, D. F. D'Agostino, M. V. Danninger, M. Daughhetee, J. Davis, J. C. De Clercq, C. Demiroers, L. Denger, T. Depaepe, O. Descamps, F. Desiati, P. de Vries-Uiterweerd, G. DeYoung, T. Diaz-Velez, J. C. Dierckxsens, M. Dreyer, J. Dumm, J. P. Ehrlich, R. Eisch, J. Ellsworth, R. W. Engdegard, O. Euler, S. Evenson, P. A. Fadiran, O. Fazely, A. R. Fedynitch, A. Feusels, T. Filimonov, K. Finley, C. Fischer-Wasels, T. Foerster, M. M. Fox, B. D. Franckowiak, A. Franke, R. Gaisser, T. K. Gallagher, J. Geisler, M. Gerhardt, L. Gladstone, L. Gluesenkamp, T. Goldschmidt, A. Goodman, J. A. Gora, D. Grant, D. Griesel, T. Gross, A. Grullon, S. Gurtner, M. Ha, C. Hallgren, A. Halzen, F. Han, K. Hanson, K. Heinen, D. Helbing, K. Herquet, P. Hickford, S. Hill, G. C. Hoffman, K. D. Homeier, A. Hoshina, K. Hubert, D. Huelsnitz, W. Huelss, J. -P. Hulth, P. O. Hultqvist, K. Hussain, S. Ishihara, A. Jacobsen, J. Japaridze, G. S. Johansson, H. Joseph, J. M. Kampert, K. -H. Kappes, A. Karg, T. Karle, A. Kelley, J. L. Kenny, P. Kiryluk, J. Kislat, F. Klein, S. R. Koehne, J. -H. Kohnen, G. Kolanoski, H. Koepke, L. Kopper, S. Koskinen, D. J. Kowalski, M. Kowarik, T. Krasberg, M. Krings, T. Kroll, G. Kuwabara, T. Labare, M. Lafebre, S. Laihem, K. Landsman, H. Larson, M. J. Lauer, R. Luenemann, J. Madsen, J. Majumdar, P. Marotta, A. Maruyama, R. Mase, K. Matis, H. S. Meagher, K. Merck, M. Meszaros, P. Meures, T. Middell, E. Milke, N. Miller, J. Montaruli, T. Morse, R. Movit, S. M. Nahnhauer, R. Nam, J. W. Naumann, U. Niessen, P. Nygren, D. R. Odrowski, S. Olivas, A. Olivo, M. O'Murchadha, A. Ono, M. Panknin, S. Paul, L. de los Heros, C. Perez Petrovic, J. Piegsa, A. Pieloth, D. Porrata, R. Posselt, J. Price, P. B. Przybylski, G. T. Rawlins, K. Redl, P. Resconi, E. Rhode, W. Ribordy, M. Rizzo, A. Rodrigues, J. P. Roth, P. Rothmaier, F. Rott, C. Ruhe, T. Rutledge, D. Ruzybayev, B. Ryckbosch, D. Sander, H. -G. Santander, M. Sarkar, S. Schatto, K. Schmidt, T. Schoenwald, A. Schukraft, A. Schultes, A. Schulz, O. Schunck, M. Seckel, D. Semburg, B. Seo, S. H. Sestayo, Y. Seunarine, S. Silvestri, A. Slipak, A. Spiczak, G. M. Spiering, C. Stamatikos, M. Stanev, T. Stephens, G. Stezelberger, T. Stokstad, R. G. Stoessl, A. Stoyanov, S. Strahler, E. A. Straszheim, T. Stuer, M. Sullivan, G. W. Swillens, Q. Taavola, H. Taboada, I. Tamburro, A. Tepe, A. Ter-Antonyan, S. Tilav, S. Toale, P. A. Toscano, S. Tosi, D. Turcan, D. van Eijndhoven, N. Vandenbroucke, J. Van Overloop, A. van Santen, J. Vehring, M. Voge, M. Walck, C. Waldenmaier, T. Wallraff, M. Walter, M. Weaver, Ch. Wendt, C. Westerhoff, S. Whitehorn, N. Wiebe, K. Wiebusch, C. H. Williams, D. R. Wischnewski, R. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, C. Xu, X. W. Yodh, G. Yoshida, S. Zarzhitsky, P. CA IceCube Collaboration TI Constraints on the extremely-high energy cosmic neutrino flux with the IceCube 2008-2009 data SO PHYSICAL REVIEW D LA English DT Article ID RAYS; SPECTRUM AB We report on a search for extremely-high energy neutrinos with energies greater than 10(6) GeV using the data taken with the IceCube detector at the South Pole. The data was collected between April 2008 and May 2009 with the half-completed IceCube array. The absence of signal candidate events in the sample of 333.5 days of live time significantly improves model-independent limits from previous searches and allows to place a limit on the diffuse flux of cosmic neutrinos with an E-2 spectrum in the energy range 2.0 x 10(6) - 6.3 x 10(9) GeV to a level of E-2 phi <= 3.6 x 10(-8) GeV cm(-2) sec(-1) sr(-1). C1 [Ishihara, A.; Mase, K.; Ono, M.; Yoshida, S.] Chiba Univ, Dept Phys, Chiba 2638522, Japan. [Bissok, M.; Blumenthal, J.; Boersma, D. J.; Euler, S.; Geisler, M.; Gluesenkamp, T.; Heinen, D.; Huelss, J. -P.; Krings, T.; Laihem, K.; Meures, T.; Paul, L.; Schukraft, A.; Schunck, M.; Vehring, M.; Wallraff, M.; Wiebusch, C. H.] Rhein Westfal TH Aachen, Inst Phys 3, D-52056 Aachen, Germany. [Toale, P. A.; Williams, D. R.; Zarzhitsky, P.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Rawlins, K.] Univ Alaska Anchorage, Dept Phys & Astron, Anchorage, AK 99508 USA. [Fadiran, O.; Japaridze, G. S.] USA Clark Atlanta Univ, CTSPS, Atlanta, GA 30314 USA. [Daughhetee, J.; Taboada, I.; Tepe, A.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Daughhetee, J.; Taboada, I.; Tepe, A.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Fazely, A. R.; Ter-Antonyan, S.; Xu, X. W.] Southern Univ, Dept Phys, Baton Rouge, LA 70813 USA. [Bay, R.; D'Agostino, M. V.; Filimonov, K.; Gerhardt, L.; Kiryluk, J.; Klein, S. R.; Porrata, R.; Price, P. B.; Vandenbroucke, J.; Woschnagg, K.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Beattie, K.; Buitink, S.; Gerhardt, L.; Goldschmidt, A.; Joseph, J. M.; Kiryluk, J.; Klein, S. R.; Matis, H. S.; Nygren, D. R.; Przybylski, G. T.; Stezelberger, T.; Stokstad, R. G.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Kappes, A.; Kolanoski, H.; Waldenmaier, T.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Becker, J. K.; Dreyer, J.; Fedynitch, A.; Olivo, M.] Ruhr Univ Bochum, Fac Phys & Astron, D-44780 Bochum, Germany. [Boeser, S.; Denger, T.; Franckowiak, A.; Homeier, A.; Kowalski, M.; Panknin, S.; Stuer, M.; Voge, M.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Seunarine, S.] Univ W Indies, Dept Phys, BB-11000 Bridgetown, Barbados. [Bechet, S.; Bertrand, D.; Dierckxsens, M.; Hanson, K.; Marotta, A.; Petrovic, J.; Swillens, Q.] Univ Libre Bruxelles, Fac Sci, B-1050 Brussels, Belgium. [Bose, D.; De Clercq, C.; Depaepe, O.; Hubert, D.; Labare, M.; Rizzo, A.; Strahler, E. A.; van Eijndhoven, N.] Vrije Univ Brussel, Dienst ELEM, B-1050 Brussels, Belgium. [Adams, J.; Brown, A. M.; Gross, A.; Hickford, S.] Univ Canterbury, Dept Phys & Astron, Christchurch 1, New Zealand. [Berley, D.; Blaufuss, E.; Christy, B.; Ehrlich, R.; Ellsworth, R. W.; Goodman, J. A.; Hoffman, K. D.; Huelsnitz, W.; Meagher, K.; Olivas, A.; Redl, P.; Roth, P.; Schmidt, T.; Straszheim, T.; Sullivan, G. W.; Turcan, D.; Wissing, H.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Beatty, J. J.; Davis, J. C.; Rott, C.; Stamatikos, M.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Beatty, J. J.; Davis, J. C.; Rott, C.; Stamatikos, M.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Beatty, J. J.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Clevermann, F.; Koehne, J. -H.; Milke, N.; Pieloth, D.; Rhode, W.; Ruhe, T.] TU Dortmund Univ, Dept Phys, D-44221 Dortmund, Germany. [Grant, D.; Wood, T. R.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2G7, Canada. [Abdou, Y.; Carson, M.; Descamps, F.; de Vries-Uiterweerd, G.; Feusels, T.; Ryckbosch, D.; Van Overloop, A.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [Colnard, C.; Gross, A.; Odrowski, S.; Resconi, E.; Schulz, O.; Sestayo, Y.; Wolf, M.] Max Planck Inst Kernphys, D-69177 Heidelberg, Germany. [Barwick, S. W.; Nam, J. W.; Silvestri, A.; Yodh, G.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Cohen, S.; Demiroers, L.; Ribordy, M.] Ecole Polytech Fed Lausanne, High Energy Phys Lab, CH-1015 Lausanne, Switzerland. [Besson, D. Z.; Kenny, P.] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. [Gallagher, J.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Abbasi, R.; Aguilar, J. A.; Andeen, K.; Baker, M.; BenZvi, S.; Berghaus, P.; Braun, J.; Chirkin, D.; Desiati, P.; Diaz-Velez, J. C.; Dumm, J. P.; Eisch, J.; Gladstone, L.; Grullon, S.; Halzen, F.; Hanson, K.; Hill, G. C.; Hoshina, K.; Jacobsen, J.; Karle, A.; Kelley, J. L.; Krasberg, M.; Landsman, H.; Maruyama, R.; Merck, M.; Montaruli, T.; Morse, R.; O'Murchadha, A.; Rodrigues, J. P.; Santander, M.; Toscano, S.; van Santen, J.; Weaver, Ch.; Wendt, C.; Westerhoff, S.; Whitehorn, N.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Griesel, T.; Koepke, L.; Kowarik, T.; Kroll, G.; Luenemann, J.; Piegsa, A.; Rothmaier, F.; Sander, H. -G.; Schatto, K.; Wiebe, K.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55099 Mainz, Germany. [Herquet, P.; Kohnen, G.] Univ Mons, B-7000 Mons, Belgium. [Bai, X.; Clem, J.; Evenson, P. A.; Gaisser, T. K.; Hussain, S.; Kuwabara, T.; Niessen, P.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Stoyanov, S.; Tilav, S.; Xu, C.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Bai, X.; Clem, J.; Evenson, P. A.; Gaisser, T. K.; Hussain, S.; Kuwabara, T.; Niessen, P.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Stoyanov, S.; Tilav, S.; Xu, C.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Ahlers, M.; Sarkar, S.] Univ Oxford, Dept Phys, Oxford OX1 3NP, England. [Abu-Zayyad, T.; Madsen, J.; Spiczak, G. M.; Tamburro, A.] Univ Wisconsin, Dept Phys, River Falls, WI 54022 USA. [Bohm, C.; Danninger, M.; Finley, C.; Hulth, P. O.; Hultqvist, K.; Johansson, H.; Seo, S. H.; Walck, C.] Stockholm Univ, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Bohm, C.; Danninger, M.; Finley, C.; Hulth, P. O.; Hultqvist, K.; Johansson, H.; Seo, S. H.; Walck, C.] Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden. [Cowen, D. F.; Meszaros, P.; Movit, S. M.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Cowen, D. F.; DeYoung, T.; Foerster, M. M.; Fox, B. D.; Ha, C.; Koskinen, D. J.; Lafebre, S.; Larson, M. J.; Meszaros, P.; Rutledge, D.; Slipak, A.; Stephens, G.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Botner, O.; Engdegard, O.; Hallgren, A.; Miller, J.; de los Heros, C. Perez; Taavola, H.] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden. [Auffenberg, J.; Becker, K. -H.; Bindig, D.; Fischer-Wasels, T.; Gurtner, M.; Helbing, K.; Kampert, K. -H.; Karg, T.; Kopper, S.; Naumann, U.; Posselt, J.; Schultes, A.; Semburg, B.] Univ Wuppertal, Dept Phys, D-42119 Wuppertal, Germany. [Alba, J. L. Bazo; Benabderrahmane, M. L.; Berdermann, J.; Bernardini, E.; Franke, R.; Gora, D.; Han, K.; Kislat, F.; Lauer, R.; Majumdar, P.; Middell, E.; Nahnhauer, R.; Schoenwald, A.; Spiering, C.; Stoessl, A.; Tosi, D.; Walter, M.; Wischnewski, R.] DESY, D-15735 Zeuthen, Germany. [Montaruli, T.] Univ Bari, I-70126 Bari, Italy. [Montaruli, T.] Sezione Ist Nazl Fis Nucl, Dipartimento Fis, I-70126 Bari, Italy. RP Ishihara, A (reprint author), Chiba Univ, Dept Phys, Chiba 2638522, Japan. EM aya@hepburn.s.chiba-u.ac.jp RI Taavola, Henric/B-4497-2011; Aguilar Sanchez, Juan Antonio/H-4467-2015; HAN, KyoungHoon/D-4588-2011; Wiebusch, Christopher/G-6490-2012; Maruyama, Reina/A-1064-2013; Kowalski, Marek/G-5546-2012; Sarkar, Subir/G-5978-2011; Beatty, James/D-9310-2011; Tamburro, Alessio/A-5703-2013; Botner, Olga/A-9110-2013; Hallgren, Allan/A-8963-2013; Tjus, Julia/G-8145-2012; Auffenberg, Jan/D-3954-2014; Koskinen, David/G-3236-2014 OI Ter-Antonyan, Samvel/0000-0002-5788-1369; Schukraft, Anne/0000-0002-9112-5479; Perez de los Heros, Carlos/0000-0002-2084-5866; Taavola, Henric/0000-0002-2604-2810; Buitink, Stijn/0000-0002-6177-497X; Carson, Michael/0000-0003-0400-7819; Hubert, Daan/0000-0002-4365-865X; Benabderrahmane, Mohamed Lotfi/0000-0003-4410-5886; Aguilar Sanchez, Juan Antonio/0000-0003-2252-9514; Wiebusch, Christopher/0000-0002-6418-3008; Maruyama, Reina/0000-0003-2794-512X; Sarkar, Subir/0000-0002-3542-858X; Beatty, James/0000-0003-0481-4952; Auffenberg, Jan/0000-0002-1185-9094; Koskinen, David/0000-0002-0514-5917 FU U.S. National Science Foundation-Office of Polar Programs; U.S. National Science Foundation-Physics Division; University of Wisconsin Almni Research Foundation; Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin Madison; Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy; National Energy Research Scientific Computing Center; Louisiana Optical Network Initiative (LONI) grid computing resources; National Science and Engineering Research Council of Canada; Swedish Research Council; Swedish Polar Research Secretariat; Swedish National Infrastructure for Computing (SNIC); Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF); Deutsche Forschungsgemeinschaft (DFG); Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO); FWO Odysseus programme; Flanders Institute to encourage scientific and technological research in industry (IWT); Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Japan Society for Promotion of Science (JSPS); Swiss National Science Foundation (SNSF), Switzerland; EU; Capes Foundation, Ministry of Education of Brazil FX We acknowledge the support from the following agencies: U.S. National Science Foundation-Office of Polar Programs, U.S. National Science Foundation-Physics Division, University of Wisconsin Almni Research Foundation, the Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin Madison, the Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy, and National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI) grid computing resources; National Science and Engineering Research Council of Canada; Swedish Research Council, Swedish Polar Research Secretariat, Swedish National Infrastructure for Computing (SNIC), and Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Deutsche Forschungsgemeinschaft (DFG), Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO), FWO Odysseus programme, Flanders Institute to encourage scientific and technological research in industry (IWT), Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Japan Society for Promotion of Science (JSPS); the Swiss National Science Foundation (SNSF), Switzerland; A. Gross acknowledges support by the EU Marie Curie OIF Program; J. P. Rodrigues acknowledges support by the Capes Foundation, Ministry of Education of Brazil. NR 41 TC 72 Z9 72 U1 1 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 24 PY 2011 VL 83 IS 9 AR 092003 DI 10.1103/PhysRevD.83.092003 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 767YS UT WOS:000290897000001 ER PT J AU Pauzauskie, PJ Crowhurst, JC Worsley, MA Laurence, TA Kilcoyne, ALD Wang, YM Willey, TM Visbeck, KS Fakra, SC Evans, WJ Zaug, JM Satcher, JH AF Pauzauskie, Peter J. Crowhurst, Jonathan C. Worsley, Marcus A. Laurence, Ted A. Kilcoyne, A. L. David Wang, Yinmin Willey, Trevor M. Visbeck, Kenneth S. Fakra, Sirine C. Evans, William J. Zaug, Joseph M. Satcher, Joe H., Jr. TI Synthesis and characterization of a nanocrystalline diamond aerogel SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE gigapascal; nanomaterials; phase transition; photonics; qubit ID MESOPOROUS COESITE; COHERENT DYNAMICS; CARBON; PRESSURE; SPIN; TEMPERATURE; COMPLEX; SILICA; PHASE AB Aerogel materials have myriad scientific and technological applications due to their large intrinsic surface areas and ultralow densities. However, creating a nanodiamond aerogel matrix has remained an outstanding and intriguing challenge. Here we report the high-pressure, high-temperature synthesis of a diamond aerogel from an amorphous carbon aerogel precursor using a laser-heated diamond anvil cell. Neon is used as a chemically inert, near-hydrostatic pressure medium that prevents collapse of the aerogel under pressure by conformally filling the aerogel's void volume. Electron and X-ray spectromicroscopy confirm the aerogel morphology and composition of the nanodiamond matrix. Time-resolved photoluminescence measurements of recovered material reveal the formation of both nitrogen- and silicon-vacancy point-defects, suggesting a broad range of applications for this nanocrystalline diamond aerogel. C1 [Pauzauskie, Peter J.; Crowhurst, Jonathan C.; Worsley, Marcus A.; Laurence, Ted A.; Wang, Yinmin; Willey, Trevor M.; Visbeck, Kenneth S.; Evans, William J.; Zaug, Joseph M.; Satcher, Joe H., Jr.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94551 USA. [Kilcoyne, A. L. David; Fakra, Sirine C.] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Pauzauskie, PJ (reprint author), Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA. EM peterpz@uw.edu RI Laurence, Ted/E-4791-2011; Willey, Trevor/A-8778-2011; Pauzauskie, Peter/A-1316-2014; Worsley, Marcus/G-2382-2014; Kilcoyne, David/I-1465-2013; Wang, Yinmin (Morris)/F-2249-2010 OI Laurence, Ted/0000-0003-1474-779X; Willey, Trevor/0000-0002-9667-8830; Worsley, Marcus/0000-0002-8012-7727; Wang, Yinmin (Morris)/0000-0002-7161-2034 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-05CH11231]; US Department of Energy by the Lawrence Livermore National Laboratory (LLNL) [DE-AC52-07NA27344]; LLNL FX The authors thank A. Goncharov for assistance in determining LHDAC temperatures from thermal emission data, as well as L. Hrubesh, L. Fried, D. Awschalom, M. Armstrong, C. Grant, T. Baumann, P. Weber, J. Bradley, I. Hutcheon, W. Goldstein, and G. Fox for valuable comments, and I. Hutcheon for access to SEM facilities. Use of the Advanced Light Source is supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-05CH11231. This work performed under the auspices of the US Department of Energy by the Lawrence Livermore National Laboratory (LLNL) under Contract DE-AC52-07NA27344. P.J.P. gratefully acknowledges funding from an E.O. Lawrence Fellowship at the LLNL. NR 33 TC 14 Z9 14 U1 3 U2 56 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 24 PY 2011 VL 108 IS 21 BP 8550 EP 8553 DI 10.1073/pnas.1010600108 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 768CB UT WOS:000290908000013 PM 21555550 ER PT J AU Lucks, JB Qi, L Mutalik, VK Wang, D Arkin, AP AF Lucks, Julius B. Qi, Lei Mutalik, Vivek K. Wang, Denise Arkin, Adam P. TI Versatile RNA-sensing transcriptional regulators for engineering genetic networks SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE gene networks; regulatory systems; orthogonal regulators ID ANTISENSE RNA; SYNTHETIC BIOLOGY; ESCHERICHIA-COLI; PLASMID PT181; IN-VIVO; EXPRESSION; RIBOREGULATORS; ATTENUATION; REPLICATION; ELEMENTS AB The widespread natural ability of RNA to sense small molecules and regulate genes has become an important tool for synthetic biology in applications as diverse as environmental sensing and metabolic engineering. Previous work in RNA synthetic biology has engineered RNA mechanisms that independently regulate multiple targets and integrate regulatory signals. However, intracellular regulatory networks built with these systems have required proteins to propagate regulatory signals. In this work, we remove this requirement and expand the RNA synthetic biology toolkit by engineering three unique features of the plasmid pT181 antisense-RNA-mediated transcription attenuation mechanism. First, because the antisense RNA mechanism relies on RNA-RNA interactions, we show how the specificity of the natural system can be engineered to create variants that independently regulate multiple targets in the same cell. Second, because the pT181 mechanism controls transcription, we show how independently acting variants can be configured in tandem to integrate regulatory signals and perform genetic logic. Finally, because both the input and output of the attenuator is RNA, we show how these variants can be configured to directly propagate RNA regulatory signals by constructing an RNA-meditated transcriptional cascade. The combination of these three features within a single RNA-based regulatory mechanism has the potential to simplify the design and construction of genetic networks by directly propagating signals as RNA molecules. C1 [Lucks, Julius B.; Qi, Lei; Wang, Denise; Arkin, Adam P.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Lucks, Julius B.] Miller Inst Basic Res Sci, Berkeley, CA 94720 USA. [Mutalik, Vivek K.; Arkin, Adam P.] Univ Calif Berkeley, Lawrence Berkeley Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Arkin, Adam P.] Calif Inst Quantitat Sci QB3, Berkeley, CA 94720 USA. RP Arkin, AP (reprint author), EO Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,MS Stanley 922, Berkeley, CA 94720 USA. EM aparkin@lbl.gov RI Arkin, Adam/A-6751-2008; Lucks, Julius/L-2801-2016; OI Arkin, Adam/0000-0002-4999-2931; Qi, Lei S/0000-0002-3965-3223; Mutalik, Vivek/0000-0001-7934-0400 FU Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231]; Synthetic Biology Engineering Research Center under National Science Foundation [04-570/0540879]; Miller Institute for Basic Research in Science FX The authors thank Richard Novick (Department of Microbiology, New York University School of Medicine, New York) for donating plasmid pT181; Ron Breaker, Blake Wiedenheft, and Vincent Rouilly for comments; Weston Whitaker and Jeff Skerker for discussions; and Richard Shan and Quintara Biosciences for assistance in plasmid sequencing. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract DE-AC02-05CH11231. This work was supported by the Synthetic Biology Engineering Research Center under National Science Foundation Grant 04-570/0540879. J.B.L. acknowledges the financial support of the Miller Institute for Basic Research in Science. NR 39 TC 106 Z9 106 U1 1 U2 27 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 24 PY 2011 VL 108 IS 21 BP 8617 EP 8622 DI 10.1073/pnas.1015741108 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 768CB UT WOS:000290908000025 PM 21555549 ER PT J AU Cipriano, R Kan, CE Graham, J Danielpour, D Stampfer, M Jackson, MW AF Cipriano, Rocky Kan, Charlene E. Graham, James Danielpour, David Stampfer, Martha Jackson, Mark W. TI TGF-beta signaling engages an ATM-CHK2-p53-independent RAS-induced senescence and prevents malignant transformation in human mammary epithelial cells SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE breast cancer; tumor suppressor ID ONCOGENE-INDUCED SENESCENCE; DNA-DAMAGE RESPONSE; BREAST-CANCER CELLS; GROWTH-FACTOR-BETA; C-MYC; CELLULAR-TRANSFORMATION; P16 INACTIVATION; P53; TUMORIGENESIS; ACTIVATION AB Oncogene-induced senescence (OIS), the proliferative arrest engaged in response to persistent oncogene activation, serves as an important tumor-suppressive barrier. We show here that finite lifespan human mammary epithelial cells (HMEC) undergo a p16/RB- and p53-independent OIS in response to oncogenic RAS that requires TGF-beta signaling. Suppression of TGF-beta signaling by expression of a dominant-negative TGF-beta type II receptor, use of a TGF-beta type I receptor inhibitor, or ectopic expression of MYC permitted continued proliferation upon RAS expression. Surprisingly, unlike fibroblasts, shRNA-mediated knockdown of ATM or CHK2 was unable to prevent RAS-mediated OIS, arguing that the DNA damage response is not required for OIS in HMEC. Abrogation of TGF-beta signaling not only allowed HMEC lacking p53 to tolerate oncogenic RAS but also conferred the capacity for anchorage-independent growth. Thus, the OIS engaged after dysregulated RAS expression provides an early barrier to malignant progression and is mediated by TGF-beta receptor activation in HMEC. Understanding the mechanisms that initiate and maintain OIS in epithelial cells may provide a foundation for future therapies aimed at reengaging this proliferative barrier as a cancer therapy. C1 [Cipriano, Rocky; Graham, James; Jackson, Mark W.] Case Western Reserve Univ, Dept Pathol, Cleveland, OH 44106 USA. [Kan, Charlene E.] Case Western Reserve Univ, Dept Genet, Cleveland, OH 44106 USA. [Danielpour, David; Jackson, Mark W.] Case Western Reserve Univ, Case Comprehens Canc Ctr, Cleveland, OH 44106 USA. [Stampfer, Martha] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Jackson, MW (reprint author), Case Western Reserve Univ, Dept Pathol, Cleveland, OH 44106 USA. EM mwj7@case.edu FU National Institutes of Health [T32CA059366]; Department of Defense [BC074072] FX This work was supported by National Institutes of Health Grant T32CA059366 (to R. C.) and Department of Defense Breast Cancer Research Program Grant BC074072 (to M.W.J). NR 42 TC 41 Z9 43 U1 3 U2 5 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 24 PY 2011 VL 108 IS 21 BP 8668 EP 8673 DI 10.1073/pnas.1015022108 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 768CB UT WOS:000290908000034 PM 21555587 ER PT J AU Schaefer, JK Rocks, SS Zheng, W Liang, LY Gu, BH Morel, FMM AF Schaefer, Jeffra K. Rocks, Sara S. Zheng, Wang Liang, Liyuan Gu, Baohua Morel, Francois M. M. TI Active transport, substrate specificity, and methylation of Hg(II) in anaerobic bacteria SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE mercury bioavailability; mercury detoxification ID SULFATE-REDUCING BACTERIA; HEAVY-METAL RESISTANCE; FRESH-WATER SEDIMENTS; MERCURY METHYLATION; ESCHERICHIA-COLI; DEGRADATION; ECOSYSTEMS; TOXICOLOGY; SALINITY; SAMPLES AB The formation of methylmercury (MeHg), which is biomagnified in aquatic food chains and poses a risk to human health, is effected by some iron-and sulfate-reducing bacteria (FeRB and SRB) in anaerobic environments. However, very little is known regarding the mechanism of uptake of inorganic Hg by these organisms, in part because of the inherent difficulty in measuring the intracellular Hg concentration. By using the FeRB Geobacter sulfurreducens and the SRB Desulfovibrio desulfuricans ND132 as model organisms, we demonstrate that Hg(II) uptake occurs by active transport. We also establish that Hg(II) uptake by G. sulfurreducens is highly dependent on the characteristics of the thiols that bind Hg(II) in the external medium, with some thiols promoting uptake and methylation and others inhibiting both. The Hg(II) uptake system of D. desulfuricans has a higher affinity than that of G. sulfurreducens and promotes Hg methylation in the presence of stronger complexing thiols. We observed a tight coupling between Hg methylation and MeHg export from the cell, suggesting that these two processes may serve to avoid the build up and toxicity of cellular Hg. Our results bring up the question of whether cellular Hg uptake is specific for Hg(II) or accidental, occurring via some essential metal importer. Our data also point at Hg(II) complexation by thiols as an important factor controlling Hg methylation in anaerobic environments. C1 [Schaefer, Jeffra K.; Rocks, Sara S.; Morel, Francois M. M.] Princeton Univ, Dept Geosci, Princeton, NJ 08544 USA. [Zheng, Wang; Liang, Liyuan; Gu, Baohua] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Morel, FMM (reprint author), Princeton Univ, Dept Geosci, Princeton, NJ 08544 USA. EM morel@princeton.edu RI Gu, Baohua/B-9511-2012; Liang, Liyuan/O-7213-2014 OI Gu, Baohua/0000-0002-7299-2956; Liang, Liyuan/0000-0003-1338-0324 FU Office of Biological and Environmental Research, Office of Science, US Department of Energy; US Department of Energy [DE-AC05-00OR22725] FX We thank C. Cobb-Adams for the analysis of Hg and MeHg at Princeton University. We also thank J. Jay and T. Barkay for helpful comments in review of this manuscript. This research was supported in part by the Office of Biological and Environmental Research, Office of Science, US Department of Energy, as part of the Mercury Science Focus Area Program at Oak Ridge National Laboratory, which is managed by UT-Battelle, LLC, for the US Department of Energy under contract DE-AC05-00OR22725. NR 33 TC 82 Z9 88 U1 5 U2 110 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 24 PY 2011 VL 108 IS 21 BP 8714 EP 8719 DI 10.1073/pnas.1105781108 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 768CB UT WOS:000290908000042 PM 21555571 ER PT J AU Kakar, S Sturms, R Tiffany, A Nix, JC DiSpirito, AA Hargrove, MS AF Kakar, Smita Sturms, Ryan Tiffany, Andrea Nix, Jay C. DiSpirito, Alan A. Hargrove, Mark S. TI Crystal Structures of Parasponia and Trema Hemoglobins: Differential Heme Coordination Is Linked to Quaternary Structure SO BIOCHEMISTRY LA English DT Article ID PLANT HEMOGLOBIN; HEXACOORDINATE HEMOGLOBINS; RESPIRATION; ADAPTATION; EXPRESSION; CYTOGLOBIN; EVOLUTION; HYPOXIA; SURFACE; NO AB Hemoglobins from the plants Parasponia andersonii (ParaHb) and Trema tomentosa (TremaHb) are 93% identical in primary structure but differ in oxygen binding constants in accordance with their distinct physiological functions. Additionally, these proteins are dimeric, and ParaHb exhibits the unusual property of having different heme redox potentials for each subunit. To investigate how these hemoglobins could differ in function despite their shared sequence identity and to determine the cause of subunit heterogeneity in ParaHb, we have measured their crystal structures in the ferric oxidation state. Furthermore, we have made a monomeric ParaHb mutant protein (I43N) and measured its ferrous/ferric heme redox potential to test the hypothesized link between quaternary structure and heme heterogeneity in wild-type ParaHb. Our results demonstrate that TremaHb is a symmetric dimeric hemoglobin similar to other class 1 nonsymbiotic plant hemoglobins but that ParaHb has structurally distinct heme coordination in each of its two subunits that is absent in the monomeric I43N mutant protein. A mechanism for achieving structural heterogeneity in ParaHb in which the Ile(101(F4)) side chain contacts the proximal His(105(F8)) in one subunit but not the other is proposed. These results are discussed in the context of the evolution of plant oxygen transport hemoglobins, and other potential functions of plant hemoglobins. C1 [Kakar, Smita; Sturms, Ryan; Tiffany, Andrea; DiSpirito, Alan A.; Hargrove, Mark S.] Iowa State Univ, Dept Biochem Biophys & Mol Biol, Ames, IA 50011 USA. [Nix, Jay C.] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Hargrove, MS (reprint author), Iowa State Univ, Dept Biochem Biophys & Mol Biol, Ames, IA 50011 USA. EM msh@iastate.edu NR 36 TC 7 Z9 7 U1 0 U2 4 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD MAY 24 PY 2011 VL 50 IS 20 BP 4273 EP 4280 DI 10.1021/bi2002423 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 763XW UT WOS:000290594000006 PM 21491905 ER PT J AU Harper, JC Lopez, DM Larkin, EC Economides, MK McIntyre, SK Alam, TM Tartis, MS Werner-Washburne, M Brinker, CJ Brozik, SM Wheeler, DR AF Harper, Jason C. Lopez, DeAnna M. Larkin, Elizabeth C. Economides, Megan K. McIntyre, Sarah K. Alam, Todd M. Tartis, Michaelann S. Werner-Washburne, Margaret Brinker, C. Jeffrey Brozik, Susan M. Wheeler, David R. TI Encapsulation of S. cerevisiae in Poly(glycerol) Silicate Derived Matrices: Effect of Matrix Additives and Cell Metabolic Phase on Long-Term Viability and Rate of Gene Expression SO CHEMISTRY OF MATERIALS LA English DT Article DE living hybrid biomaterials; bioencapsulation; glycerol modified silanes; cell viability; cell metabolic phase; whole-cell based biosensors ID RECOMBINANT ESCHERICHIA-COLI; SOL-GEL ENCAPSULATION; SACCHAROMYCES-CEREVISIAE; LIVING BACTERIA; SI-29 NMR; BIOSENSOR; YEAST; PERSPECTIVES; BIOMOLECULES; SELECTIVITY AB Bioencapsulation of living cells into silica materials derived from the sol gel process has resulted in novel hybrid living materials with exciting functionalities. Despite the many successes in this field, long-term viability and activity of the encapsulated cells remain a significant obstacle to producing practical and robust devices,.e.g., whole-cell-based biosensors. We report the first study on the effects of various media additives and the metabolic phase of encapsulated cells on long-term viability and the rate of inducible gene expression. Saccharomyces cerevisiae (S. cerevisiae) cells, genetically engineered to produce yellow fluorescent protein (YFP) in response to galactose, were encapsulated in poly(glycerol) silicate derived matrices. Surprisingly, we find that addition of media components to the glycerol-silica matrix adversely impacted long-term viability in all cases studied, with a 1.3, 1.4, or 5.4 fold decrease in viability after only 9 days of storage in matrices containing yeast peptone dextrose (YPD), yeast peptone (YP, no glucose), or Synthetic Complete (SC) +2% glucose media, respectively. These findings are attributed to the media components inducing exit of the cells from the more robust quiescent state, and the metabolic production of toxic byproducts. Encapsulated cells from exponential culture exhibited inducible reporter gene expression rates approximately 33% higher than cells from stationary cultures. Addition of media components to the silica matrix increased gene expression rates under certain conditions. These results further elaborate on other silica matrix encapsulated living cell studies, and provide important design parameters for developing effective living cell-based biosensors for case-specific detection applications. C1 [Harper, Jason C.; Economides, Megan K.; Brinker, C. Jeffrey; Brozik, Susan M.] Univ New Mexico, Dept Chem & Nucl Engn, Albuquerque, NM 87131 USA. [Werner-Washburne, Margaret; Brinker, C. Jeffrey] Univ New Mexico, Dept Mol Genet & Microbiol, Albuquerque, NM 87131 USA. [Larkin, Elizabeth C.; Tartis, Michaelann S.] New Mexico Inst Min & Technol, Dept Chem Engn, Socorro, NM 87801 USA. [Harper, Jason C.; Lopez, DeAnna M.; McIntyre, Sarah K.; Alam, Todd M.; Brinker, C. Jeffrey; Brozik, Susan M.; Wheeler, David R.] Sandia Natl Labs, Albuquerque, NM 87106 USA. RP Brinker, CJ (reprint author), Univ New Mexico, Dept Chem & Nucl Engn, Albuquerque, NM 87131 USA. EM cjbrink@sandia.gov; smbrozi@sandia.gov; drwheel@sandia.gov FU Defense Treat Reduction Agency (DTRA) [B0844671]; DoE NNSA Office for Nonproliferation Research and Development [NA-22]; Sandia Lab Directed Research and Development program; Air Force Office of Scientific Research [FA 9550-10-1-0054]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was funded by the Defense Treat Reduction Agency (DTRA) Chem. Bio. Basic Research Program grant B0844671, the DoE NNSA Office for Nonproliferation Research and Development (NA-22), and the Sandia Lab Directed Research and Development program. CJB acknowledges funding from the Air Force Office of Scientific Research grant FA 9550-10-1-0054, and the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 53 TC 16 Z9 16 U1 2 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 J9 CHEM MATER JI Chem. Mat. PD MAY 24 PY 2011 VL 23 IS 10 BP 2555 EP 2564 DI 10.1021/cm103525u PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 763YD UT WOS:000290594700009 ER PT J AU Babu, GS Valant, M Page, K Llobet, A Kolodiazhnyi, T Axelsson, AK AF Babu, Gunda Santosh Valant, Matjaz Page, Katharine Llobet, Anna Kolodiazhnyi, Taras Axelsson, Anna-Karin TI New (Bi1.88Fe0.12)(Fe1.42Te0.58)O-6.87 Pyrochlore with Spin-Glass Transition SO CHEMISTRY OF MATERIALS LA English DT Article DE Bi-pyrochlore; displacive disorder; Raman spectra; dielectric relaxation; spin glass ID X-RAY-DIFFRACTION; DIELECTRIC-PROPERTIES; DISPLACIVE DISORDER; CRYSTAL-CHEMISTRY; OXIDE PYROCHLORES; PHASE-FORMATION; RELAXATION; SPECTRA AB The synthesized (Bi1.88Fe0.12)(Fe1.42Te0.58)O-6.87 is characterized with so far the highest Fe content among pyrochlores. Consequently, it exhibits a strong spin-glass magnetic transition at around 20 K The dielectric relaxation in the same temperature range originates from multiwall hopping of the displaced ions on A and O' sites. The displacement was confirmed with the structural analysis of the pyrochlore using Rietveld refinement on joint neutron and X-ray diffraction data. At room temperature, the pyrochlore exhibits a cubic Fd (3) over barm symmetry (a = 10.38804 (13) angstrom) with Fe3+ ions sharing A and B structural sites. The refined results indicate on a displacive disorder with A-site positioned at 96g and O' positioned at 32e. The lattice vibrational analysis using Raman spectra is in agreement with the displacive disorder of the pyrochlore. C1 [Babu, Gunda Santosh; Valant, Matjaz] Univ Nova Gorica, Mat Res Lab, Nova Gorica 5000, Slovenia. [Page, Katharine; Llobet, Anna] Los Alamos Natl Lab, Lujan Neutron Scattering Ctr, Los Alamos, NM 87545 USA. [Kolodiazhnyi, Taras] Natl Inst Mat Sci, Tsukuba, Ibaraki 3050044, Japan. [Axelsson, Anna-Karin] Univ London Imperial Coll Sci Technol & Med, Dept Mat, London SW7 2AZ, England. RP Valant, M (reprint author), Univ Nova Gorica, Mat Res Lab, Vipavska 13, Nova Gorica 5000, Slovenia. EM matjaz.valant@ung.si RI gunda, santosh babu/B-1499-2010; Page, Katharine/C-9726-2009; Llobet, Anna/B-1672-2010; KOLODIAZHNYI, Taras/H-2860-2011; Lujan Center, LANL/G-4896-2012; axelsson, anna-karin/E-6884-2013; OI Page, Katharine/0000-0002-9071-3383; Valant, Matjaz/0000-0003-4842-5676; Kolodiazhnyi, Taras/0000-0002-9630-9461 FU DOE Office of Basic Energy Sciences; DOE [DE-AC52-06NA25396] FX The authors thank Hiroya Sakurai for valuable comments on spin-glass properties. This work has benefited from the use of HIPD at the Lujan Center at Los Alamos Neutron Science Center, funded by DOE Office of Basic Energy Sciences. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE Contract DE-AC52-06NA25396. NR 49 TC 14 Z9 14 U1 2 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAY 24 PY 2011 VL 23 IS 10 BP 2619 EP 2625 DI 10.1021/cm200281z PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 763YD UT WOS:000290594700017 ER PT J AU Schutz-Sikma, EA Joshi, HM Ma, Q MacRenaris, KW Eckermann, AL Dravid, VP Meade, TJ AF Schutz-Sikma, Elise A. Joshi, Hrushikesh M. Ma, Qing MacRenaris, Keith W. Eckermann, Amanda L. Dravid, Vinayak P. Meade, Thomas J. TI Probing the Chemical Stability of Mixed Ferrites: Implications for Magnetic Resonance Contrast Agent Design SO CHEMISTRY OF MATERIALS LA English DT Article DE MRI; ferrite; nanoparticle; leaching; magnetic properties ID IRON-OXIDE NANOPARTICLES; ABSORPTION FINE-STRUCTURE; MRI CONTRAST; BIOMEDICAL APPLICATIONS; MFE2O4 M; COBALT; SPINEL; SIZE; NANOCRYSTALS; MN AB Nanomaterials with mixed composition, in particular magnetic spinel ferrites, are emerging as efficient contrast agents for magnetic resonance imaging. Many factors, including size, composition, atomic structure, and surface properties, are crucial in the design of such nanoparticle-based probes because of their influence on the magnetic properties. Silica-coated iron oxide (IO-SiO(2)) and cobalt ferrite (CoIO-SiO(2)) nanoparticles were synthesized using standard high-temperature thermal decomposition and base-catalyzed water-in-oil microemulsion techniques. Under neutral aqueous conditions, it was found that 50-75% of the cobalt content in the CoIO-SiO(2) nanoparticles leached out the core structure. Leaching caused a 7.2-fold increase in the longitudinal relaxivity and an increase in the saturation magnetization from similar to 48 to similar to 65 emu/g of the core. X-ray absorption fine structure studies confirmed that the atomic structure of the ferrite core was altered following leaching, while transmission electron microscopy and dynamic light scattering confirmed that the morphology and size of the nanoparticle remained unchanged. The CoIO-SiO(2) nanoparticles converted from a partially inverted spinel cation arrangement (unleached state) to an inverse spine arrangement (leached state). The control IO-SiO(2) nanoparticles remained stable with no change in the structure and negligible changes in the magnetic behavior. This detailed analysis highlights how important understanding the properties of nanomaterials is in the development of reliable agents for diagnostic and therapeutic applications. C1 [Schutz-Sikma, Elise A.; MacRenaris, Keith W.; Eckermann, Amanda L.; Meade, Thomas J.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Joshi, Hrushikesh M.; Dravid, Vinayak P.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Ma, Qing] Northwestern Univ, Argonne Natl Lab, Synchrotron Res Ctr, DND CAT, Argonne, IL 60439 USA. RP Meade, TJ (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM tmeade@northwestern.edu RI Dravid, Vinayak/B-6688-2009; Eckermann, Amanda/A-3224-2013 FU Center for Cancer Nanotechnology Excellence (CCNE) initiative of the National Institutes of Health's National Cancer Institute [U54CA119341]; National Institute of Biomedical Imaging and Bioengineering [1RO1EB005866-01]; E. I. DuPont de Nemours Co.; Dow Chemical Co.; State of Illinois; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The work performed at Northwestern University was supported by the Center for Cancer Nanotechnology Excellence (CCNE) initiative of the National Institutes of Health's National Cancer Institute under Award U54CA119341 and the National Institute of Biomedical Imaging and Bioengineering under Award 1RO1EB005866-01. The DND-CAT located at the Advanced Photon Source (APS) is supported by E. I. DuPont de Nemours & Co., The Dow Chemical Co., and the State of Illinois. Use of the APS was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. The SQUID measurements were performed by Oleksandr Chernyashevskyy in the Magnetic and Physical Properties Measurement Facility at Northwestern University. TEM analysis was performed in the EPIC/NIFTI facility of the NUANCE Center at Northwestern University. Special thanks go to Collin Morris in the Chemistry Department at Northwestern University for help with the ferrite crystallographic models. NR 59 TC 29 Z9 29 U1 3 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 J9 CHEM MATER JI Chem. Mat. PD MAY 24 PY 2011 VL 23 IS 10 BP 2657 EP 2664 DI 10.1021/cm200509g PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 763YD UT WOS:000290594700022 PM 21603070 ER PT J AU Aad, G Abbott, B Abdallah, J Abdelalim, AA Abdesselam, A Abdinov, O Abi, B Abolins, M Abramowicz, H Abreu, H Acerbi, E Acharya, BS Adams, DL Addy, TN Adelman, J Aderholz, M Adomeit, S Adragna, P Adye, T Aefsky, S Aguilar-Saavedra, A Aharrouche, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akdogan, T Akesson, TP Akimoto, G Akimov, AV Akiyama, A Alam, MS Alam, MA Albrand, S Aleksa, M Aleksandrov, IN Aleppo, M Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Aliyev, M Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alviggi, MG Amako, K Amaral, P Amelung, C Ammosov, VV Amorim, A Amoros, G Amram, N Anastopoulos, C Andeen, T Anders, CF Anderson, KJ Andreazza, A Andrei, V Andrieux, ML Anduaga, XS Angerami, A Anghinolfi, F Anjos, N Annovi, A Antonaki, A Antonelli, M Antonelli, S Antonov, A Antos, J Anulli, F Aoun, S Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Archambault, JP Arfaoui, S Arguin, JF Arik, E Arik, M Armbruster, AJ Arnaez, O Arnault, C Artamonov, A Artoni, G Arutinov, D Asai, S Asfandiyarov, R Ask, S Asman, B Asquith, L Assamagan, K Astbury, A Astvatsatourov, A Atoian, G Aubert, B Auerbach, B Auge, E Augsten, K Aurousseau, M Austin, N Avramidou, R Axen, D Ay, C Azuelos, G Azuma, Y Baak, MA Baccaglioni, G Bacci, C Bach, AM Bachacou, H Bachas, K Bachy, G Backes, M Backhaus, M Badescu, E Bagnaia, P Bahinipati, S Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, MD Baker, S Pedrosa, FBD Banas, E Banerjee, P Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Barashkou, A Galtieri, AB Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barr, AJ Barreiro, F da Costa, JBG Barrillon, P Bartoldus, R Barton, AE Bartsch, D Bartsch, V Bates, RL Batkova, L Batley, JR Battaglia, A Battistin, M Battistoni, G Bauer, F Bawa, HS Beare, B Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Beckingham, M Becks, KH Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Begel, M Harpaz, SB Behera, PK Beimforde, M Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellina, F Bellomo, G Bellomo, M Belloni, A Beloborodova, O Belotskiy, K Beltramello, O Ben Ami, S Benary, O Benchekroun, D Benchouk, C Bendel, M Benedict, BH Benekos, N Benhammou, Y Benjamin, DP Benoit, M Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernardet, K Bernat, P Bernhard, R Bernius, C Berry, T Bertin, A Bertinelli, F Bertolucci, F Besana, MI Besson, N Bethke, S Bhimji, W Bianchi, RM Bianco, M Biebel, O Bieniek, SP Biesiada, J Biglietti, M Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biscarat, C Bitenc, U Black, KM Blair, RE Blanchard, JB Blanchot, G Blocker, C Blocki, J Blondel, A Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VB Bocci, A Boddy, CR Boehler, M Boek, J Boelaert, N Boser, S Bogaerts, JA Bogdanchikov, A Bogouch, A Bohm, C Boisvert, V Bold, T Boldea, V Bona, M Bondarenko, VG Boonekamp, M Boorman, G Booth, CN Booth, P Bordoni, S Borer, C Borisov, A Borissov, G Borjanovic, I Borroni, S Bos, K Boscherini, D Bosman, M Boterenbrood, H Botterill, D Bouchami, J Boudreau, J Bouhova-Thacker, EV Boulahouache, C Bourdarios, C Bousson, N Boveia, A Boyd, J Boyko, IR Bozhko, NI Bozovic-Jelisavcic, I Bracinik, J Braem, A Brambilla, E Branchini, P Brandenburg, GW Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brelier, B Bremer, J Brenner, R Bressler, S Breton, D Brett, ND Bright-Thomas, PG Britton, D Brochu, FM Brock, I Brock, R Brodbeck, TJ Brodet, E Broggi, F Bromberg, C Brooijmans, G Brooksb, WK Brown, G Brubaker, E de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Buanes, T Bucci, F Buchanan, J Buchanan, NJ Buchholz, P Buckingham, RM Buckley, AG Buda, SI Budagov, IA Budick, B Buescher, V Bugge, L Buira-Clark, D Buis, EJ Bulekov, O Bunse, M Buran, T Burckhart, H Burdin, S Burgess, T Burke, S Busato, E Bussey, P Buszello, CP Butin, F Butler, B Butler, JM Buttar, CM Butterworth, JM Buttinger, W Byatt, T Urban, SC Caccia, M Caforio, D Cakir, O Calafiura, P Calderini, G Calfayan, P Calkins, R Caloba, LP Caloi, R Calvet, D Calvet, S Toro, RC Camard, A Camarri, P Cambiaghi, M Cameron, D Cammin, J Campana, S Campanelli, M Canale, V Canelli, F Canepa, A Cantero, J Capasso, L Garrido, MDMC Caprini, I Caprini, M Capriotti, D Capua, M Caputo, R Caramarcu, C Cardarelli, R Carli, T Carlino, G Carminati, L Caron, B Caron, S Carpentieri, C Montoya, GDC Carter, AA Carter, JR Carvalho, J Casadei, D Casado, MP Cascella, M Caso, C Hernandez, AMC Castaneda-Miranda, E Gimenez, VC Castro, NF Cataldi, G Cataneo, F Catinaccio, A Catmore, JR Cattai, A Cattani, G Caughron, S Cauz, D Cavallari, A Cavalleri, P Cavalli, D Cavalli-Sforza, M Cavasinni, V Cazzato, A Ceradini, F Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cetin, SA Cevenini, F Chafaq, A Chakraborty, D Chan, K Chapleau, B Chapman, JD Chapman, JW Chareyre, E Charlton, DG Chavda, V Cheatham, S Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, L Chen, S Chen, T Chen, X Cheng, S Cheplakov, A Chepurnov, VF El Moursli, RC Chernyatin, V Cheu, E Cheung, SL Chevalier, L Chevallier, F Chiefari, G Chikovani, L Childers, JT Chilingarov, A Chiodini, G Chizhov, MV Choudalakis, G Chouridou, S Christidi, IA Christov, A Chromek-Burckhart, D Chu, ML Chudoba, J Ciapetti, G Ciba, K Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciobotaru, MD Ciocca, C Ciocio, A Cirilli, M Ciubancan, M Clark, A Clark, PJ Cleland, W Clemens, JC Clement, B Clement, C Clifft, RW Coadou, Y Cobal, M Coccaro, A Cochran, J Coe, P Cogan, JG Coggeshall, J Cogneras, E Cojocaru, CD Colas, J Colijn, AP Collard, C Collins, NJ Collins-Tooth, C Collot, J Colon, G Coluccia, R Comune, G Muino, PC Coniavitis, E Conidi, MC Consonni, M Constantinescu, S Conta, C Conventi, F Cook, J Cooke, M Cooper, BD Cooper-Sarkar, AM Cooper-Smith, NJ Copic, K Cornelissen, T Corradi, M Corriveau, F Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Costin, T Cote, D Torres, RC Courneyea, L Cowan, G Cowden, C Cox, BE Cranmer, K Crescioli, F Cristinziani, M Crosetti, G Crupi, R Crepe-Renaudin, S Almenar, CC Donszelmann, TC Cuneo, S Curatolo, M Curtis, CJ Cwetanski, P Czirr, H Czyczula, Z D'Auria, S D'Onofrio, M D'Orazio, A Mello, ADG Da Silva, PVM Da Via, C Dabrowski, W Dahlhoff, A Dai, T Dallapiccola, C Dallison, SJ Dam, M Dameri, M Damiani, DS Danielsson, HO Dankers, R Dannheim, D Dao, V Darbo, G Darlea, GL Daum, C Dauvergne, JP Davey, W Davidek, T Davidson, N Davidson, R Davies, M Davison, AR Dawe, E Dawson, I Dawson, JW Daya, RK De, K de Asmundis, R De Castro, S Salgado, PEDF De Cecco, S de Graat, J De Groot, N de Jong, P De La Taille, C De la Torre, H De Lotto, B De Mora, L De Nooij, L Branco, MD De Pedis, D De Saintignon, P De Salvo, A De Sanctis, U De Santo, A De Regie, JBD Dean, S Dedovich, DV Degenhardt, J Dehchar, M Deile, M Del Papa, C Del Peso, J Del Prete, T Dell'Acqua, A Dell'Asta, L Della Pietra, M Della Volpe, D Delmastro, M Delpierre, P Delruelle, N Delsart, PA Deluca, C Demers, S Demichev, M Demirkoz, B Deng, J Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Devetak, E Deviveiros, PO Dewhurst, A DeWilde, B Dhaliwal, S Dhullipudi, R Di Ciaccio, A Di Ciaccio, L Di Girolamo, A Di Girolamo, B Di Luise, S Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Diaz, MA Diblen, F Diehl, EB Dietl, H Dietrich, J Dietzsch, TA Diglio, S Yagci, KD Dingfelder, J Dionisi, C Dita, P Dita, S Dittus, F Djama, F Djilkibaev, R Djobava, T do Vale, B Wemans, ADV Doan, TKO Dobbs, M Dobinson, R Dobos, D Dobson, E Dobson, M 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Evangelakou, D Evans, H Fabbri, L Fabre, C Facius, K Fakhrutdinov, RM Falciano, S Falou, AC Fang, Y Fanti, M Farbin, A Farilla, A Farley, J Farooque, T Farrington, SM Farthouat, P Fasching, D Fassnacht, P Fassouliotis, D Fatholahzadeh, B Favareto, A Fayard, L Fazio, S Febbraro, R Federic, P Fedin, OL Fedorko, I Fedorko, W Fehling-Kaschek, M Feligioni, L Fellmann, D Felzmann, CU Feng, C Feng, EJ Fenyuk, AB Ferencei, J Ferland, J Fernandes, B Fernando, W Ferrag, S Ferrando, J Ferrara, V Ferrari, A Ferrari, P Ferrari, R Ferrer, A Ferrer, ML Ferrere, D Ferretti, C Parodi, AF Fiascaris, M Fiedler, F Filipcic, A Filippas, A Filthaut, F Fincke-Keeler, M Fiolhais, MCN Fiorini, L Firan, A Fischer, G Fischer, P Fisher, MJ Fisher, SM Flammer, J Flechl, M Fleck, I Fleckner, J Fleischmann, P Fleischmann, S Flick, T Castillo, LRF Flowerdew, MJ Fohlisch, F Fokitis, M Martin, TF Forbush, DA Formica, A Forti, A Fortin, D Foster, JM Fournier, D Foussat, A Fowler, AJ Fowler, K Fox, H Francavilla, P 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CA ATLAS Collaboration TI A search for new physics in dijet mass and angular distributions in pp collisions at root s=7 TeV measured with the ATLAS detector SO NEW JOURNAL OF PHYSICS LA English DT Article ID PARTON DISTRIBUTIONS; HADRON COLLIDERS; CHIRAL COLOR; QCD; QUARK AB A search for new interactions and resonances produced in LHC proton-proton (pp) collisions at a centre-of-mass energy root s = 7 TeV was performed with the ATLAS detector. Using a dataset with an integrated luminosity of 36 pb(-1), dijet mass and angular distributions were measured up to dijet masses of similar to 3.5 TeV and were found to be in good agreement with Standard Model predictions. This analysis sets limits at 95% CL on various models for new physics: an excited quark is excluded for mass between 0.60 and 2.64 TeV, an axigluon hypothesis is excluded for axigluon masses between 0.60 and 2.10 TeV and quantum black holes are excluded in models with six extra space-time dimensions for quantum gravity scales between 0.75 and 3.67 TeV. Production cross section limits as a function of dijet mass are set using a simplified Gaussian signal model to facilitate comparisons with other hypotheses. Analysis of the dijet angular distribution using a novel technique simultaneously employing the dijet mass excludes quark contact interactions with a compositeness scale 3 below 9.5 TeV. 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P.; Vazeille, F.; Viret, S.] Clermont Univ, Lab Phys Corpusculaire, Aubiere, France. [Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Febbraro, R.; Ghodbane, N.; Gris, P. L. Y.; Guicheney, C.; Pallin, D.; Podlyski, F.; Santoni, C.; Says, L. P.; Vazeille, F.; Viret, S.] Univ Clermont Ferrand, Aubiere, France. [Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Febbraro, R.; Ghodbane, N.; Gris, P. L. Y.; Guicheney, C.; Pallin, D.; Podlyski, F.; Santoni, C.; Says, L. P.; Vazeille, F.; Viret, S.] IN2P3, CNRS, Aubiere, France. [Angerami, A.; Brooijmans, G.; Dodd, J.; Guo, J.; Hughes, E. W.; Mateos, D. Lopez; Parsons, J. A.; Penson, A.; Spano, F.; Urbaniec, D.; Williams, E.; Wulf, E.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Dam, M.; Driouichi, C.; Facius, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Klinkby, E. B.; Lundquist, J.; Rensch, B.; Simonyan, M.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Mastroberardino, A.; Morello, G.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Cosenza, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Morello, G.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Bold, T.; Ciba, K.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Idzik, M.; Jelen, K.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Rulikowska-Zarebska, E.; Toczek, B.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa; Malecki, P.; Olszewski, A.; Olszowska, J.; Richter-Was, E.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Daya, R. 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F.; Prudent, X.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Ebenstein, W. L.; Fowler, A. J.; Ko, B. R.; Oh, S. H.; Wang, C.; Yamaoka, J.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; O'Brien, B. J.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Griesmayer, E.] Fachhsch Wiener Neustadt, Wiener Neustadt, Austria. [Annovi, A.; Antonelli, M.; Bilokon, H.; Cerutti, F.; Curatolo, M.; Esposito, B.; Ferrer, M. L.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.; Wen, M.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Bell, P. J.; Bell, W. H.; Berglund, E.; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Efthymiopoulos, I.; Ferrere, D.; Gadomski, S.; Navarro, J. E. 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G.] Georgian Acad Sci, Inst Phys, GE-380077 Tbilisi, Rep of Georgia. [Chikovani, L.; Djobava, T.; Khubua, J.; Magradze, E.; Mchedlidze, G.; Mosidze, M.; Tskhadadze, E. G.] Georgian Acad Sci, HEP Inst, GE-380060 Tbilisi, Rep of Georgia. [Chikovani, L.; Djobava, T.; Khubua, J.; Magradze, E.; Mchedlidze, G.; Mosidze, M.; Tskhadadze, E. G.] Tbilisi State Univ, GE-380086 Tbilisi, Rep of Georgia. [Astvatsatourov, A.; Dueren, M.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-6300 Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Gemmell, A.; Kenyon, M.; McGlone, H.; Moraes, A.; O'Shea, V.; Barrer, C. Oropeza; Pickford, A.; Robson, A.; Saxon, D. H.; Shaw, C.; Smith, K. M.; St Denis, R. D.; Steele, G.; Stewart, G. A.; Thompson, A. S.; Wraight, K.; Wright, C.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Ay, C.; Blumenschein, U.; Brandt, O.; Erdmann, J.; Evangelakou, D.; George, M.; Grosse-Knetter, J.; Guindon, S.; Haller, J.; Henrichs, A.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Mann, A.; Meyer, J.; Quadt, A.; Roe, A.; Shabalina, E.; Uhrmacher, M.; Weber, P.; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Andrieux, M-L; Clement, B.; Collot, J.; Crepe-Renaudin, S.; de Saintignon, P.; Delsart, P. A.; Donini, J.; Dzahini, D.; Hostachy, J-Y; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Martin, Ph; Polci, F.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Andrieux, M-L; Clement, B.; Collot, J.; Crepe-Renaudin, S.; de Saintignon, P.; Delsart, P. A.; Donini, J.; Dzahini, D.; Hostachy, J-Y; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Martin, Ph; Polci, F.; Stark, J.; Sun, X.; Trocme, B.] IN2P3, CNRS, Grenoble, France. [Albrand, S.; Andrieux, M-L; Clement, B.; Collot, J.; Crepe-Renaudin, S.; de Saintignon, P.; Delsart, P. A.; Donini, J.; Dzahini, D.; Hostachy, J-Y; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Martin, Ph; Polci, F.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Brandenburg, G. W.; Franklin, M.; Hurst, P.; Huth, J.; Jeanty, L.; Kagan, M.; Outschoorn, V. Martinez; Mercurio, K. M.; Mills, C.; Moed, S.; Morii, M.; Prasad, S.; Smith, B. C.; Zevi della Porta, G.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Childers, J. T.; Dietzsch, T. A.; Foehlisch, F.; Geweniger, C.; Hanke, P.; Henke, M.; Khomich, A.; Kluge, E-E; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H-C; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Radescu, V.; Schaetzel, S.; Schoening, A.] Heidelberg Univ, Inst Phys, D-6900 Heidelberg, Germany. [Abdesselam, A.; Kugel, A.; Maenner, R.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, D-6800 Mannheim, Germany. [Ohsugi, T.] Hiroshima Univ, Fac Sci, Hiroshima 730, Japan. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Jain, V.; Luehring, F.; Marino, C. P.; Ogren, H.; Penwell, J.; Price, D.; Rust, D. R.; Whittington, D.; Yang, Y.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Epp, B.; Jussel, P.; Kneringer, E.; Kuhn, D.; Rudolph, G.] Leopold Franzens Univ, Inst Astro Teilchenphys, Innsbruck, Austria. [Behera, P. K.; Limper, M.; Mallik, U.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; Dudziak, F.; Lebedev, A.; Mete, A. S.; Meyer, W. T.; Nelson, A.; Prell, S.; Rosenberg, E. I.; Ruiz-Martinez, A.; Triplett, N.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Barashkou, A.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chepurnov, V. F.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Gusakov, Y.; Huseynov, N.; Kalinovskaya, L. V.; Kazarinov, M. Y.; Kekelidze, G. D.; Kharchenko, D.; Khovanskiy, N.; Khramov, E.; Kolesnikov, V.; Kotov, Vm; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Lazarev, A. B.; Malyukov, S.; Manjavidze, I. D.; Minashvili, I. A.; Mineev, M.; Nikolaev, K.; Olchevski, A. G.; Peshekhonov, V. D.; Romanov, V. M.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Ishii, K.; Ishino, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Manabe, A.; Mitsui, S.; Morita, Y.; Murakami, K.; Nagano, K.; Nozaki, M.; Odaka, S.; Ohska, T. K.; Sasaki, O.; Sasaki, T.; Suzuki, Y.; Tanaka, S.; Terada, S.; Tojo, J.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Akiyama, A.; Hayakawa, T.; Homma, Y.; Ichimiya, R.; Ishikawa, A.; Kawagoe, K.; King, M.; Kiyamura, H.; Kurashige, H.; Matsushita, T.; Miyazaki, K.; Nishiyama, T.; Ochi, A.; Okada, S.; Omachi, C.; Suita, K.; Takeda, H.; Tani, K.; Tokunaga, K.; Yamazaki, Y.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Sasao, N.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Brodbeck, T. J.; Catmore, J. R.; Cheatham, S.; Chilingarov, A.; Davidson, R.; De Mora, L.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Ratoff, P. N.; Sloan, T. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Brambilla, E.; Cazzato, A.; Chiodini, G.; Coluccia, R.; Crupi, R.; Gorini, E.; Grancagnolo, F.; Guida, A.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Bianco, M.; Brambilla, E.; Cazzato, A.; Coluccia, R.; Crupi, R.; Gorini, E.; Guida, A.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Fis, Lecce, Italy. [Allport, P. P.; Austin, N.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Houlden, M. A.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Maxfield, S. J.; Mehta, A.; Migas, S.; Prichard, P. M.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wiglesworth, C.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Landon, M. P. J.; Lloyd, S. L.; Morin, J.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Stevenson, K.; Castanheira, M. Teixeira Dias; Traynor, D.] Queen Mary Univ London, Dept Phys, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Boorman, G.; Cooper-Smith, N. J.; Cowan, G.; Edwards, C. A.; George, S.; Goncalo, R.; Hayden, D.; Kilvington, G.; Misiejuk, A.; Rose, M.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Boeser, S.; Butterworth, J. M.; Byatt, T.; Campanelli, M.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dean, S.; Drohan, J. G.; Jansen, E.; Jones, T. W.; Konstantinidis, N.; Monk, J.; Nash, M.; Nurse, E.; Prabhu, R.; Richards, A.; Robinson, J. E. M.; Sherwood, P.; Simmons, B.; Taylor, C.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Beauchemin, P. H.; Bordoni, S.; Calderini, G.; Camard, A.; Cavalleri, P.; Chareyre, E.; De Cecco, S.; Derue, F.; Imbault, D.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lellouch, J.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph; Theveneaux-Pelzer, T.; Trincaz-Duvoid, S.; Trinh, T. N.; Vannucci, F.; Yuan, L.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beauchemin, P. H.; Bordoni, S.; Calderini, G.; Camard, A.; Cavalleri, P.; Chareyre, E.; De Cecco, S.; Derue, F.; Imbault, D.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lellouch, J.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph; Theveneaux-Pelzer, T.; Trincaz-Duvoid, S.; Trinh, T. N.; Vannucci, F.; Yuan, L.] Univ Paris Diderot, Paris, France. [Beauchemin, P. H.; Bordoni, S.; Calderini, G.; Camard, A.; Cavalleri, P.; Chareyre, E.; De Cecco, S.; Derue, F.; Imbault, D.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lellouch, J.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph; Theveneaux-Pelzer, T.; Trincaz-Duvoid, S.; Trinh, T. N.; Vannucci, F.; Yuan, L.] IN2P3, CNRS, Paris, France. [Akesson, T. P.; Alonso, A.; Groth-Jensen, J.; Hedberg, V.; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.] Lund Univ, Inst Fys, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Lagouri, T.; March, L.; Nebot, E.; Rodier, S.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Aharrouche, M.; Arnaez, O.; Bendel, M.; Blum, W.; Buescher, V.; Eckweiler, S.; Edmonds, K.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Ji, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Meyer, C.; Moreno, D.; Neusiedl, A.; Rieke, S.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Siragusa, G.; Tapprogge, S.; Anh, T. Vu] Johannes Gutenberg Univ Mainz, Inst Phys, D-6500 Mainz, Germany. [Almond, J.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Foster, J. M.; Howarth, J.; Hughes-Jones, R. E.; Ibbotson, M.; Jones, G.; Keates, J. R.; Kelly, M.; Kolya, S. D.; Lane, J. L.; Loebinger, F. K.; Marshall, R.; Martyniuk, A. C.; Marx, M.; Masik, J.; Miyagawa, P. S.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Plano, W. G.; Schwanenberger, C.; Snow, S. W.; Tevlin, C. M.; Watts, S.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aoun, S.; Arfaoui, S.; Bee, C. P.; Benchouk, C.; Bernardet, K.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Delpierre, P.; Djama, F.; Etienne, F.; Feligioni, L.; Henry-Couannier, F.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Monnier, E.; Odier, J.; Petit, E.; Pralavorio, P.; Qian, Z.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aoun, S.; Arfaoui, S.; Bee, C. P.; Benchouk, C.; Bernardet, K.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Delpierre, P.; Djama, F.; Etienne, F.; Feligioni, L.; Henry-Couannier, F.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Monnier, E.; Odier, J.; Petit, E.; Pralavorio, P.; Qian, Z.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] IN2P3, CNRS, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Thompson, E. N.; van Eldik, N.; Willocq, S.; Woudstra, M. J.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Chapleau, B.; Corriveau, F.; Dobbs, M.; Dufour, M-A; Guler, H.; Klemetti, M.; Robertson, S. H.; Schram, M.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Davey, W.; Davidson, N.; Felzmann, C. U.; Kazi, S. I.; Limosani, A.; Moorhead, G. F.; Phan, A.; Sevior, M. E.; Shao, Q. T.; Taylor, G. N.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Eppig, A.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, H.; Liu, J. B.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Purdham, J.; Qian, J.; Scheirich, D.; Strandberg, J.; Thun, R. P.; Walch, S.; Wilson, A.; Yang, H.; Zhou, B.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Comune, G.; Di Mattia, A.; Fedorko, W.; Hauser, R.; Heim, S.; Holzbauer, J. L.; Huston, J.; Koll, J.; Kraus, J.; Linnemann, J. T.; Mangeard, P. S.; Martin, B.; Miller, R. J.; Pope, B. G.; Ryan, P.; Schwienhorst, R.; Tollefson, K.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Acerbi, E.; Aleppo, M.; Alessandria, F.; Alimonti, G.; Andreazza, A.; Baccaglioni, G.; Battistoni, G.; Bellomo, G.; Besana, M. I.; Broggi, F.; Caccia, M.; Carminati, L.; Cavalli, D.; Dell'Asta, L.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Lazzaro, A.; Lombardo, V. P.; Mandelli, L.; Mazzanti, M.; Meroni, C.; Montesano, S.; Perini, L.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Rossi, L.; Sorbi, M.; Tartarellia, G. F.; Troncon, C.; Turra, R.; Vegni, G.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Acerbi, E.; Aleppo, M.; Andreazza, A.; Bellomo, G.; Besana, M. I.; Caccia, M.; Carminati, L.; Dell'Asta, L.; Fanti, M.; Favareto, A.; Lazzaro, A.; Montesano, S.; Perini, L.; Ragusa, F.; Rivoltella, G.; Rossi, L.; Sorbi, M.; Turra, R.; Vegni, G.] Univ Milan, Dipartimento Fis, Milan, Italy. [Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Gilewsky, V.; Kuzhir, P.; Rumiantsev, V.; Starovoitov, P.; Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Azuelos, G.; Banerjee, P.; Bouchami, J.; Davies, M.; Ferland, J.; Guler, H.; Gutierrez, A.; Lebel, C.; Leroy, C.; Goia, J. A. Macana; Martin, J. P.; Mehdiyev, R.; Scallon, O.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bondarenko, V. G.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Morozov, S. V.; Romaniouk, A.; Smirnov, S. Yu; Soldatov, E.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu; Smirnova, L. N.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Biebel, O.; Calfayan, P.; de Graat, J.; Deile, M.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Genest, M. H.; Hertenberger, R.; Kennedy, J.; Kummer, C.; Legger, F.; Lichtnecker, M.; Mameghani, R.; Mueller, T. A.; Nunnemann, T.; Rauscher, F.; Reznicek, P.; Ruckert, B.; Sanders, M. P.; Schaile, D.; Schieck, J.; Serfon, C.; Staude, A.; Walker, R.; Will, J. Z.; Zhuang, X.] Univ Munich, Fak Phys, Munich, Germany. [Aderholz, M.; Barillari, T.; Beimforde, M.; Bethke, S.; Capriotti, D.; Cortiana, G.; Dannheim, D.; Dietl, H.; Dubbert, J.; Ehrich, T.; Flowerdew, M. J.; Giovannini, P.; Goettfert, T.; Groh, M.; Haefner, P.; Hauff, D.; Hott, T.; Jantsch, A.; Kaiser, S.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Lutz, G.; Macchiolo, A.; Manz, A.; Menke, S.; Mohrdieck-Moeck, S.; Moser, H. G.; Nisius, R.; Oberlack, H.; Pospelov, G. E.; Potrap, I. N.; Rauter, E.; Richter, R.; Salihagic, D.; Schacht, P.; Seuster, R.; Stonjek, S.; Valderanis, C.; von der Schmitt, H.; von Loeben, J.; Weigell, P.; Zhuravlov, V.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.; Tanaka, Y.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Itoh, Y.; Ohshima, T.; Okumura, Y.; Sugimoto, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Cevenini, F.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Della Volpe, D.; Doria, A.; Giordano, R.; Iacobucci, G.; Izzo, V.; Merola, L.; Musto, E.; Patricelli, S.; Rossi, E.; Sekhniaidze, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Cevenini, F.; Chiefari, G.; Della Volpe, D.; Giordano, R.; Merola, L.; Musto, E.; Patricelli, S.; Rossi, E.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Metcalfe, J.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Chelstowska, M. A.; Consonni, M.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Koetsveld, F.; Magrath, A.; Ordonez, G.; Raas, M.; Timmermans, C. J. W. P.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Bentvelsen, S.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Buis, E. J.; Colijn, A. P.; Dankers, R.; Daum, C.; de Jong, P.; De Nooij, L.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Koutsman, A.; Lee, H.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Muijs, A.; Mussche, I.; Ottersbach, J. P.; Peters, O.; Reichold, A.; Rijpstra, M.; Ruckstuhl, N.; Salamanna, G.; Sandstroem, R.; Snuverink, J.; Ta, D.; Tsiakiris, M.; Turlay, E.; van der Graaf, H.; van der Kraaij, E.; van der Leeuw, R.; van der Poel, E.; Van Eijk, B.; van Kesteren, Z.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Bentvelsen, S.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Buis, E. J.; Colijn, A. P.; Dankers, R.; Daum, C.; de Jong, P.; De Nooij, L.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Koutsman, A.; Lee, H.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Muijs, A.; Mussche, I.; Ottersbach, J. P.; Peters, O.; Reichold, A.; Rijpstra, M.; Ruckstuhl, N.; Salamanna, G.; Sandstroem, R.; Snuverink, J.; Ta, D.; Tsiakiris, M.; Turlay, E.; van der Graaf, H.; van der Kraaij, E.; van der Leeuw, R.; van der Poel, E.; Van Eijk, B.; van Kesteren, Z.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; de Lima, J. G. Rocha; Suhr, C.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Beloborodova, O.; Bobrovnikov, V. B.; Bogdanchikov, A.; Kazanin, V. A.; Kolachev, G. M.; Korol, A.; Malyshev, V.; Maslennikov, A. L.; Maximov, D. A.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.; Zaytsev, A.] Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; Djilkibaev, R.; van Huysduynen, L. Hooft; Konoplich, R.; Krasznahorkay, A.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.; Shibata, A.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA. [Fernando, W.; Fisher, M. J.; Gan, K. K.; Kagan, H.; Kass, R. D.; Moss, J.; Rahimi, A. M.; Strang, M.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Huang, G. S.; Issever, C.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Kocnar, A.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Potter, C. T.; Ptacek, E.; Reinsch, A.; Robinson, M.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abreu, H.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Blanchard, J-B; Bourdarios, C.; Breton, D.; Collard, C.; De La Taille, C.; De Regie, J. B. De Vivie; Diglio, S.; Duflot, L.; Escalier, M.; Falou, A. C.; Fayard, L.; Fournier, D.; Grivaz, J-F; Heller, M.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lounis, A.; Makovec, N.; Matricon, P.; Nakahama, Y.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Veillet, J. J.; Vukotic, I.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Abreu, H.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Blanchard, J-B; Bourdarios, C.; Breton, D.; Collard, C.; De La Taille, C.; De Regie, J. B. De Vivie; Diglio, S.; Duflot, L.; Escalier, M.; Falou, A. C.; Fayard, L.; Fournier, D.; Grivaz, J-F; Heller, M.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lounis, A.; Makovec, N.; Matricon, P.; Nakahama, Y.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Veillet, J. J.; Vukotic, I.; Wicek, F.; Zerwas, D.; Zhang, Z.] IN2P3, CNRS, Orsay, France. [Hanagaki, K.; Hirose, M.; Meguro, T.; Nomachi, M.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Czyczula, Z.; Gjelsten, B. K.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Pylypchenko, Y.; Read, A. L.; Rohne, O.; Samset, B. H.; Stapnes, S.; Strandlie, A.; Taga, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Abdesselam, A.; Apolle, R.; Barr, A. J.; Boddy, C. R.; Brett, N. D.; Buchanan, J.; Buckingham, R. M.; Buira-Clark, D.; Coe, P.; Coniavitis, E.; Cooper-Sarkar, A. M.; Dehchar, M.; Doglioni, C.; Farrington, S. M.; Ferrando, J.; Gallas, E. J.; Gilbert, L. M.; Gwenlan, C.; Hawes, B. M.; Holmes, A.; Horton, K.; Howell, D. F.; Huffman, T. B.; Issever, C.; Karagoz, M.; King, R. S. B.; Kirsch, G. P.; Kundu, N.; Larner, A.; Lau, W.; Lavorato, A.; Liang, Z.; Livermore, S. S. A.; Loken, J.; Mattravers, C.; Mermod, P.; Nickerson, R. B.; Pinder, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Wooden, G.] Univ Oxford, Dept Phys, Oxford, England. [Bellomo, M.; Cambiaghi, M.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudioa, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Cambiaghi, M.; Conta, C.; Franchino, S.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.] Univ Pavia, Dipartimento Fis Nucl & Teor, I-27100 Pavia, Italy. [Alison, J.; Degenhardt, J.; Donega, M.; Dressnandt, N.; Fratina, S.; Hance, M.; Hines, E.; Jackson, B.; Kroll, J.; Kunkle, J.; LeGeyt, C.; Lipeles, E.; Martin, F. F.; Olivito, D.; Ospanov, R.; Reece, R.; Stahlman, J.; Thomson, E.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Nesterov, S. Y.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Zalite, Yo K.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Francavilla, P.; Giangiobbe, V.; Lupi, A.; Mazzoni, E.; Roda, C.; Sarri, F.; Zenonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Francavilla, P.; Giangiobbe, V.; Lupi, A.; Mazzoni, E.; Roda, C.; Sarri, F.; Zenonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Boudreau, J.; Boulahouache, C.; Cleland, W.; Kittelmann, T.; Mueller, J.; Paolone, V.; Prieur, D.; Savinov, V.; Tsulaia, V.; Wendler, S.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, A.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Wemans, A. Do Valle; Fernandes, B.; Fiolhais, M. C. N.; Gomes, A.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Magalhaes Martins, P. J.; Maio, A.; Maneira, J.; Morais, A.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Soares, M.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedra, A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, A.] Univ Granada, CAFPE, Granada, Spain. [Chudoba, J.; Gallus, P.; Gunther, J.; Hruska, I.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Kvasnicka, O.; Lipinsky, L.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Panuskova, M.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Davidek, T.; Dolejsi, J.; Dolezal, Z.; Drasal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Augsten, K.; Holy, T.; Horazdovsky, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Bozhko, N. I.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Gapienko, V. A.; Golovnia, S. N.; Gorokhov, S. A.; Goryachev, V. N.; Gushchin, V. N.; Ivashin, A. V.; Kabachenko, V. V.; Karyukhin, N.; Kholodenko, A. G.; Kiver, A. M.; Kopikov, S. V.; Koreshev, V.; Korotkov, V. A.; Kozhin, A. S.; Lapin, V. V.; Larionov, A. V.; Levitski, M. S.; Lokajicek, M.; Minaenko, A. A.; Mitrofanov, G. Y.; Moisseev, A. M.; Myagkov, A. G.; Nikolaenko, V.; Pleskach, A. V.; Ryadovikov, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Sviridov, Yu M.; Vorobiev, A. P.; Vovenko, A. S.; Zaets, V. G.; Zaitsev, A. M.; Zenin, A. V.; Zenin, O.; Zmouchko, V. V.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Botterill, D.; Burke, S.; Clifft, R. W.; Dallison, S. J.; Dewhurst, A.; Emeliyanov, D.; Fisher, S. M.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Greenfield, D.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Strube, J.; Tyndel, M.; Weber, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.; Ju, X.; Ming, Y.; Ortega, E. O.; Smit, G. V. Ybeles] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagnaia, P.; Bini, C.; Borroni, S.; Caloi, R.; Cavallari, A.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; Dionisi, C.; Falciano, S.; Gentile, S.; Giagu, S.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Maiani, C.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Spila, F.; Valente, P.; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma I, Rome, Italy. [Artoni, G.; Bagnaia, P.; Bini, C.; Borroni, S.; Caloi, R.; Cavallari, A.; Ciapetti, G.; D'Orazio, A.; Dionisi, C.; Gentile, S.; Giagu, S.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Maiani, C.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Spila, F.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Nardo, R.; Di Simone, A.; Liberti, B.; Marchese, F.; Paoloni, A.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Nardo, R.; Di Simone, A.; Marchese, F.; Paoloni, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Ruggieri, F.; Spiriti, E.; Stanescu, C.; Tonazzo, A.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Biglietti, M.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.; Ruggieri, F.; Tonazzo, A.] Univ Roma Tre, Dipartimento Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Goujdami, D.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Fac Sci Ain Chock, Reseau Univ Phys Hautes Energies, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. Univ Cadi Ayyad, Fac Sci, Semlalia Dept Phys, Marrakech 40000, Morocco. [Derkaoui, J. E.; Ouchrif, M.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Boonekamp, M.; Chevalier, L.; Chevallier, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Le Menedeu, E.; Legendre, M.; Lenzi, B.; Mansoulie, B.; Meyer, J-P; Morange, N.; Nicolaidou, R.; Ouraou, A.; Pomarede, D. M.; Resende, B.; Royon, C. R.; Schune, Ph; Schwindling, J.; Simard, O.; Virchaux, M.; Yu, J.] CEA, CEA Saclay, DSM, IRFU Inst Rech Lois Fondament Univers, Gif Sur Yvette, France. [Bangert, A.; Chouridou, S.; Damiani, D. S.; Dubbs, T.; Fowler, K.; Grillo, A. A.; Hare, G. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Forbush, D. A.; Goussiou, A. G.; Griffiths, J.; Harris, O. M.; Kuykendall, W.; Lubatti, H. J.; Mockett, P.; Policicchio, A.; Rothberg, J.; Ventura, D.; Verducci, M.; Wang, J. C.; Watts, G.; Zhao, T.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Abdesselam, A.; Anastopoulos, C.; Booth, C. N.; Booth, P.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Duxfield, R.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mayne, A.; Mcfayden, J. A.; Nicolas, L.; Owen, S.; Paganis, E.; Sutton, M. R.; Tovey, D. R.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Ohshita, H.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Sipica, V.; Stahl, T.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-5900 Siegen, Germany. [Dawe, E.; Gao, Y. S.; Godfrey, J.; Komaragiri, J. R.; O'Neil, D. C.; Petteni, M.; Schouten, D.; Stelzer, B.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Grenier, P.; Haas, A.; Hansson, P.; Horn, C.; Jackson, P.; Kenney, C. J.; Kim, P. C.; Kocian, M.; Koi, T.; Lowe, A. J.; Miller, D. W.; Mount, R.; Nelson, S.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Wilson, M. G.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Batkova, L.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.; Zilka, B.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Aurousseau, M.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Leney, C.; Vickey, T.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Asman, B.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Hidvegi, A.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Lesser, J.; Lundberg, J.; Milstead, D. A.; Moa, T.; Nordkvist, B.; Ohm, C. C.; Papadelis, A.; Ramstedt, M.; Sellden, B.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Asman, B.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Lundberg, J.; Milstead, D. A.; Moa, T.; Nordkvist, B.; Ohm, C. C.; Ramstedt, M.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Grahn, K-J; Lund-Jensen, B.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Caputo, R.; Deluca, C.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Khodinov, A.; McCarthy, L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.; Yurkewicz, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Potter, C. J.; Salvatore, F.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Lee, J. S. H.; Patel, N.; Saavedra, A. F.; Varvell, K. E.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Harpaz, S. Behar; Ben Ami, S.; Bressler, S.; Kajomovitz, E.; Landsman, H.; Lifshitz, R.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Brodet, E.; Etzion, E.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hershenhorn, A. D.; Hod, N.; Kreisel, A.; Mahalalel, Y.; Munwes, Y.; Oren, Y.; Reinherz-Aronis, E.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.; Urkovsky, E.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Imori, M.; Kanaya, N.; Kaneda, M.; Kataoka, Y.; Kawamoto, T.; Kessoku, K.; Kobayashi, T.; Kubota, T.; Mashimo, T.; Masubuchi, T.; Matsumoto, H.; Matsunaga, H.; Nakamura, K.; Ninomiya, Y.; Nomoto, H.; Oda, S.; Okuyama, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamamura, T.; Yamazaki, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Imori, M.; Kanaya, N.; Kaneda, M.; Kataoka, Y.; Kawamoto, T.; Kessoku, K.; Kobayashi, T.; Kubota, T.; Mashimo, T.; Masubuchi, T.; Matsumoto, H.; Matsunaga, H.; Nakamura, K.; Ninomiya, Y.; Nomoto, H.; Oda, S.; Okuyama, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamamura, T.; Yamazaki, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Jinnouchi, O.; Kanno, T.; Kuze, M.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [Bailey, D. C.; Bain, T.; Beau, T.; Brelier, B.; Cheung, S. L.; Deviveiros, P. O.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Jankowski, E.; Krieger, P.; Le Maner, C.; Martens, F. K.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Sandhu, P.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Caron, B.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Losty, M. J.; Nugent, I. M.; Oakham, F. G.; Oram, C. J.; Savard, P.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Hara, K.; Kim, S. H.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Inst Pure & Appl Sci, Ibaraki, Japan. [Hamilton, S.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.] Tufts Univ, Ctr Sci & Technol, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Rodriguez, D.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Benedict, B. H.; Bold, T.; Ciobotaru, M. D.; Deng, J.; Dobson, M.; Eschrich, I. Gough; Grabowska-Bold, I.; Hawkins, D.; Lankford, A. J.; Okawa, H.; Porter, R.; Scannicchio, D. A.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Wheeler-Ellis, S. J.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Cauz, D.; Cobal, M.; De Lotto, B.; De Sanctis, U.; Del Papa, C.; Pinamonti, M.; Shaw, K.; Suruliz, K.] Ist Nazl Fis Nucl, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Suruliz, K.] ICTP, Udine, Italy. [Cauz, D.; Cobal, M.; De Lotto, B.; De Sanctis, U.; Del Papa, C.; Pinamonti, M.; Shaw, K.] Univ Udine, Dipartimento Fis, I-33100 Udine, Italy. [Benekos, N.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Khandanyan, H.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Belanger-Champagne, C.; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Hansen, C. J.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Amoros, G.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Amoros, G.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, Dept Fis Atom, Valencia, Spain. [Amoros, G.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, IMB, CNM, Valencia, Spain. [Amoros, G.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] CSIC, Valencia, Spain. [Axen, D.; Gay, C.; Loh, C. W.; Mills, W. J.; Muir, A.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Astbury, A.; Banerjee, Sw; Bansal, V.; Berghaus, F.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R; McPherson, A.; Plamondon, M.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Kimura, N.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Duchovni, E.; Frank, T.; Gabizon, O.; Gross, E.; Klier, A.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Asfandiyarov, R.; Montoya, G. D. Carrillo; Hernandez, A. M. Castaneda; Castaneda-Miranda, E.; Chen, X.; Dos Anjos, A.; Fang, Y.; Fasching, D.; Castillo, L. R. Flores; Gonzalez, S.; Gutzwiller, O.; Ji, H.; Kashif, L.; Cheong, A. Leung Fook; Li, H.; Ma, L. L.; Mellado Garcia, B. R.; Pan, Y. B.; Pataraia, S.; Morales, M. I. Pedraza; Peng, H.; Poveda, J.; Quayle, W. B.; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Zhu, Y.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Meyer, J.; Redelbach, A.; Stroehmer, R.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, Wurzburg, Germany. [Barisonzi, M.; Becks, K. H.; Boek, J.; Braun, H. M.; Drees, J.; Fleischmann, S.; Flick, T.; Gerlach, P.; Glitza, K. W.; Gorfine, G.; Grah, C.; Hamacher, K.; Harenberg, T.; Henss, T.; Hirschbuehl, D.; Imhaeuser, M.; Kalinin, S.; Kersten, S.; Kootz, A.; Kuhl, T.; Lenz, T.; Lenzen, G.; Maettig, P.; Mechtel, M.; Sandhoff, M.; Sandvoss, S.; Sartisohn, G.; Schultes, J.; Siebel, A.; Sturm, P.; Thadome, J.; Voss, T. T.; Wagner, W.; Wahlen, H.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Atoian, G.; Auerbach, B.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Demers, S.; Garberson, F.; Golling, T.; Guest, D.; Hsu, P. J.; Kaplan, B.; Lee, L.; Lockwitz, S.; Loginov, A.; Martin, A. J.; Schmidt, M. P.; Sherman, D.; Thioye, M.; Tipton, P.; Wall, R.; Zeller, M.] Yale Univ, Dept Phys, New Haven, CT USA. [Grabski, V.; Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Biscarat, C.; Cogneras, E.; Rahal, G.] IN2P3, Ctr Calcul CNRS, Villeurbanne, France. [Amorim, A.; Fernandes, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Maio, A.; Morais, A.; Palma, A.; Pina, J.; Pinto, B.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amorim, A.; Fernandes, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Maio, A.; Morais, A.; Palma, A.; Pina, J.; Pinto, B.; Saraiva, J. G.; Silva, J.] Univ Lisbon, CFNUL, P-1699 Lisbon, Portugal. [Beare, B.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Carvalho, J.; Fiolhais, M. C. N.; Magalhaes Martins, P. J.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Kono, T.; Terwort, M.; Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mateos, D. Lopez; Marshall, Z.; Perez, K.] CALTECH, Pasadena, CA 91125 USA. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Park, W.; Purohit, M.; Trivedi, A.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Pasztor, G.; Toth, J.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Richter-Was, E.] Jagiellonian Univ, Inst Phys, Krakow, Poland. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Freiburg, Germany. RI valente, paolo/A-6640-2010; Fazio, Salvatore /G-5156-2010; Doyle, Anthony/C-5889-2009; Jakubek, Jan/E-6530-2011; Marti-Garcia, Salvador/F-3085-2011; Conde Muino, Patricia/F-7696-2011; collins-tooth, christopher/A-9201-2012; Stoicea, Gabriel/B-6717-2011; Robson, Aidan/G-1087-2011; Losada, Marta/B-2261-2010; Gutierrez, Phillip/C-1161-2011; Ferrando, James/A-9192-2012; Perrino, Roberto/B-4633-2010; De Cecco, Sandro/B-1016-2012; branchini, paolo/A-4857-2011; Wolter, Marcin/A-7412-2012; McKee, Shawn/B-6435-2012; Rotaru, Marina/A-3097-2011; Nemecek, Stanislav/C-3487-2012; Buttar, Craig/D-3706-2011; Takai, Helio/C-3301-2012; St.Denis, Richard/C-8997-2012; Britton, David/F-2602-2010; Li, Xuefei/C-3861-2012; Smirnova, Lidia/D-8089-2012; Smirnov, Sergei/F-1014-2011; Gladilin, Leonid/B-5226-2011; Kramarenko, Victor/E-1781-2012; Alexa, Calin/F-6345-2010; Moorhead, Gareth/B-6634-2009; Petrucci, Fabrizio/G-8348-2012; Wemans, Andre/A-6738-2012; Fabbri, Laura/H-3442-2012; Kurashige, Hisaya/H-4916-2012; Kuzhir, Polina/H-8653-2012; Delmastro, Marco/I-5599-2012; Weigell, Philipp/I-9356-2012; Veneziano, Stefano/J-1610-2012; Di Micco, Biagio/J-1755-2012; spagnolo, stefania/A-6359-2012; Andreazza, Attilio/E-5642-2011; Di Nardo, Roberto/J-4993-2012; Della Pietra, Massimo/J-5008-2012; Bergeaas Kuutmann, Elin/A-5204-2013; Cascella, Michele/B-6156-2013; messina, andrea/C-2753-2013; de Groot, Nicolo/A-2675-2009; Amorim, Antonio/C-8460-2013; Orlov, Ilya/E-6611-2012; Annovi, Alberto/G-6028-2012; Pina, Joao /C-4391-2012; Vanyashin, Aleksandr/H-7796-2013; La Rosa, Alessandro/I-1856-2013; Casadei, Diego/I-1785-2013; Moraes, Arthur/F-6478-2010; Boyko, Igor/J-3659-2013; Kuleshov, Sergey/D-9940-2013; Anjos, Nuno/I-3918-2013; Kartvelishvili, Vakhtang/K-2312-2013; Dawson, Ian/K-6090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Castro, Nuno/D-5260-2011; Wolters, Helmut/M-4154-2013; Warburton, Andreas/N-8028-2013; De, Kaushik/N-1953-2013; Sukharev, Andrey/A-6470-2014; O'Shea, Val/G-1279-2010; Lee, Jason/B-9701-2014; Morozov, Sergey/C-1396-2014; Villa, Mauro/C-9883-2009; Nemecek, Stanislav/G-5931-2014; Staroba, Pavel/G-8850-2014; Lokajicek, Milos/G-7800-2014; Kupco, Alexander/G-9713-2014; Marcisovsky, Michal/H-1533-2014; Mikestikova, Marcela/H-1996-2014; Snesarev, Andrey/H-5090-2013; Chudoba, Jiri/G-7737-2014; Peleganchuk, Sergey/J-6722-2014; Santamarina Rios, Cibran/K-4686-2014; Bosman, Martine/J-9917-2014; Lei, Xiaowen/O-4348-2014; Demirkoz, Bilge/C-8179-2014; Ventura, Andrea/A-9544-2015; Villaplana Perez, Miguel/B-2717-2015; Livan, Michele/D-7531-2012; Mitsou, Vasiliki/D-1967-2009; CARPENTIERI, CARMELA/E-2137-2015; Joergensen, Morten/E-6847-2015; Martins, Paulo/M-1844-2014; Mir, Lluisa-Maria/G-7212-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Cavalli-Sforza, Matteo/H-7102-2015; Ferrer, Antonio/H-2942-2015; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; Tikhomirov, Vladimir/M-6194-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Jones, Roger/H-5578-2011; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Carvalho, Joao/M-4060-2013; Booth, Christopher/B-5263-2016; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Smirnova, Oxana/A-4401-2013; Leyton, Michael/G-2214-2016; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Olshevskiy, Alexander/I-1580-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Morone, Maria Cristina/P-4407-2016; Goncalo, Ricardo/M-3153-2016; Canelli, Florencia/O-9693-2016; Battistoni, Giuseppe/B-5264-2012; Idzik, Marek/A-2487-2017; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; la rotonda, laura/B-4028-2016; OI valente, paolo/0000-0002-5413-0068; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Stoicea, Gabriel/0000-0002-7511-4614; Ferrando, James/0000-0002-1007-7816; Perrino, Roberto/0000-0002-5764-7337; McKee, Shawn/0000-0002-4551-4502; Rotaru, Marina/0000-0003-3303-5683; Takai, Helio/0000-0001-9253-8307; Britton, David/0000-0001-9998-4342; Smirnov, Sergei/0000-0002-6778-073X; Gladilin, Leonid/0000-0001-9422-8636; Moorhead, Gareth/0000-0002-9299-9549; Petrucci, Fabrizio/0000-0002-5278-2206; Wemans, Andre/0000-0002-9669-9500; Fabbri, Laura/0000-0002-4002-8353; Kuzhir, Polina/0000-0003-3689-0837; Delmastro, Marco/0000-0003-2992-3805; Veneziano, Stefano/0000-0002-2598-2659; spagnolo, stefania/0000-0001-7482-6348; Andreazza, Attilio/0000-0001-5161-5759; Della Pietra, Massimo/0000-0003-4446-3368; Cascella, Michele/0000-0003-2091-2501; Orlov, Ilya/0000-0003-4073-0326; Annovi, Alberto/0000-0002-4649-4398; Pina, Joao /0000-0001-8959-5044; Vanyashin, Aleksandr/0000-0002-0367-5666; La Rosa, Alessandro/0000-0001-6291-2142; Moraes, Arthur/0000-0002-5157-5686; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Castro, Nuno/0000-0001-8491-4376; Wolters, Helmut/0000-0002-9588-1773; Warburton, Andreas/0000-0002-2298-7315; De, Kaushik/0000-0002-5647-4489; O'Shea, Val/0000-0001-7183-1205; Lee, Jason/0000-0002-2153-1519; Morozov, Sergey/0000-0002-6748-7277; Villa, Mauro/0000-0002-9181-8048; Mikestikova, Marcela/0000-0003-1277-2596; Peleganchuk, Sergey/0000-0003-0907-7592; Santamarina Rios, Cibran/0000-0002-9810-1816; Bosman, Martine/0000-0002-7290-643X; Lei, Xiaowen/0000-0002-2564-8351; Ventura, Andrea/0000-0002-3368-3413; Villaplana Perez, Miguel/0000-0002-0048-4602; Livan, Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886; CARPENTIERI, CARMELA/0000-0002-2994-0317; Joergensen, Morten/0000-0002-6790-9361; Martins, Paulo/0000-0003-3753-3751; Mir, Lluisa-Maria/0000-0002-4276-715X; Riu, Imma/0000-0002-3742-4582; Ferrer, Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543; Grancagnolo, Sergio/0000-0001-8490-8304; Tikhomirov, Vladimir/0000-0002-9634-0581; Camarri, Paolo/0000-0002-5732-5645; Jones, Roger/0000-0002-6427-3513; Gorelov, Igor/0000-0001-5570-0133; Carvalho, Joao/0000-0002-3015-7821; Booth, Christopher/0000-0002-6051-2847; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Smirnova, Oxana/0000-0003-2517-531X; Leyton, Michael/0000-0002-0727-8107; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Olshevskiy, Alexander/0000-0002-8902-1793; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Morone, Maria Cristina/0000-0002-0200-0632; Goncalo, Ricardo/0000-0002-3826-3442; Canelli, Florencia/0000-0001-6361-2117; Battistoni, Giuseppe/0000-0003-3484-1724; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Maio, Amelia/0000-0001-9099-0009; Fiolhais, Miguel/0000-0001-9035-0335; Karyukhin, Andrey/0000-0001-9087-4315; Anjos, Nuno/0000-0002-0018-0633; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; Veloso, Filipe/0000-0002-5956-4244; Gomes, Agostinho/0000-0002-5940-9893; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Santos, Helena/0000-0003-1710-9291; Coccaro, Andrea/0000-0003-2368-4559; De Lotto, Barbara/0000-0003-3624-4480 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; ARTEMIS; European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNAS, Greece; ISF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, UK; Royal Society, UK; Leverhulme Trust, UK; DOE, USA; NSF, USA FX We thank CERN for the highly successful operation of the LHC and we also thank the support staff from our institutions without whom ATLAS could not have been operated efficiently. We acknowledge support from ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; ARTEMIS, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNAS, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, UK; DOE and NSF, USA. The crucial computing support from all WLCG partners is also acknowledged, in particular from CERN and not only the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway and Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) but also the Tier-2 facilities worldwide. NR 50 TC 62 Z9 62 U1 3 U2 71 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD MAY 24 PY 2011 VL 13 AR 053044 DI 10.1088/1367-2630/13/5/053044 PG 44 WC Physics, Multidisciplinary SC Physics GA 782IT UT WOS:000292002400004 ER PT J AU Ni, S Wang, YB Liao, XZ Figueiredo, RB Li, HQ Zhao, YH Lavernia, EJ Ringer, SP Langdon, TG Zhu, YT AF Ni, S. Wang, Y. B. Liao, X. Z. Figueiredo, R. B. Li, H. Q. Zhao, Y. H. Lavernia, E. J. Ringer, S. P. Langdon, T. G. Zhu, Y. T. TI Strain softening in nanocrystalline Ni-Fe alloy induced by large HPT revolutions SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Severe plastic deformation; Nanocrystalline materials; Strain softening; Dislocation density; Lomer-Cottrell locks ID HIGH-PRESSURE TORSION; MOLECULAR-DYNAMICS SIMULATION; GRAIN-GROWTH; MICROSTRUCTURAL EVOLUTION; PLASTIC-DEFORMATION; FCC METALS; DISLOCATION JUNCTIONS; STRENGTH; NICKEL; COPPER AB The influence of strain on the hardness of an electrochemically deposited nanocrystalline Ni-20 wt.% Fe alloy processed by high-pressure torsion (HFT) for 20 and 30 revolutions was investigated. Strain softening followed by a stable hardness value was observed. Structural investigations revealed that, while dislocation density was important, continuous grain growth played a major role in the strain softening. The stable hardness indicates that an equilibrium structure was achieved, supporting a dynamic balance between deformation-induced grain growth and grain refinement and between deformation-induced dislocation generation and dislocation annihilation. (C) 2011 Elsevier B.V. All rights reserved. C1 [Ni, S.; Wang, Y. B.; Liao, X. Z.] Univ Sydney, Sch Aerosp Mech & Mechatron Engn, Sydney, NSW 2006, Australia. [Figueiredo, R. B.] Univ Fed Minas Gerais, Dept Met & Mat Engn, BR-31270901 Belo Horizonte, MG, Brazil. [Li, H. Q.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Zhao, Y. H.; Lavernia, E. J.] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [Ringer, S. P.] Univ Sydney, Australian Ctr Microscopy & Microanal, Sydney, NSW 2006, Australia. [Langdon, T. G.] Univ So Calif, Dept Aerosp & Mech Engn, Los Angeles, CA 90089 USA. [Langdon, T. G.] Univ So Calif, Dept Mat Sci, Los Angeles, CA 90089 USA. [Langdon, T. G.] Univ Southampton, Sch Engn Sci, Mat Res Grp, Southampton SO17 1BJ, Hants, England. [Zhu, Y. T.] N Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27659 USA. RP Liao, XZ (reprint author), Univ Sydney, Sch Aerosp Mech & Mechatron Engn, Sydney, NSW 2006, Australia. EM xiaozhou.liao@sydney.edu.au RI Liao, Xiaozhou/B-3168-2009; Wang, Yanbo/B-3175-2009; Ni, Song/E-9484-2011; Figueiredo, Roberto/F-3451-2012; Lavernia, Enrique/I-6472-2013; Li, Hongqi/B-6993-2008; Zhu, Yuntian/B-3021-2008; Langdon, Terence/B-1487-2008; Zhao, Yonghao/A-8521-2009; Ringer, Simon/E-3487-2012; Lujan Center, LANL/G-4896-2012 OI Liao, Xiaozhou/0000-0001-8565-1758; Lavernia, Enrique/0000-0003-2124-8964; Zhu, Yuntian/0000-0002-5961-7422; Ringer, Simon/0000-0002-1559-330X; FU Australian Microscopy & Microanalysis Research Facility node at the University of Sydney; Australian Research Council [DP0772880]; Los Alamos National Laboratory; Office of Naval Research [N00014-08-1-0405]; National Science Foundation of the United States [DMR-0855009]; U.S. Army Research Office and Army Research Laboratory; China Scholarship Council FX The authors are grateful for scientific and technical input and support from the Australian Microscopy & Microanalysis Research Facility node at the University of Sydney. This project is supported by the Australian Research Council [Grant No. DP0772880 (S.N., Y.B.W., and X.Z.L.)], the LDRD program of Los Alamos National Laboratory (H.Q.L.), the Office of Naval Research [Grant No. N00014-08-1-0405 (Y.H.Z. and E.J.L.)], the National Science Foundation of the United States (Grant No. DMR-0855009, T.G.L.) and the U.S. Army Research Office and Army Research Laboratory (Y.T.Z.). S.N. also appreciates support from the China Scholarship Council. NR 42 TC 10 Z9 11 U1 1 U2 26 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD MAY 24 PY 2011 VL 528 IS 13-14 BP 4807 EP 4811 DI 10.1016/j.msea.2011.03.007 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA 756IF UT WOS:000290004200070 ER PT J AU Belof, JL Cioce, CR Xu, X Zhang, XP Space, B Woodcock, HL AF Belof, Jonathan L. Cioce, Christian R. Xu, Xue Zhang, X. Peter Space, Brian Woodcock, H. Lee TI Characterization of Tunable Radical Metal-Carbenes: Key Intermediates in Catalytic Cyclopropanation SO ORGANOMETALLICS LA English DT Article ID HIGHLY ENANTIOSELECTIVE CYCLOPROPANATION; RUTHENIUM PORPHYRIN COMPLEXES; DENSITY-FUNCTIONAL THEORY; ASYMMETRIC CYCLOPROPANATION; CHIRAL PORPHYRIN; INTRAMOLECULAR CYCLOPROPANATIONS; BENZODIAZEPINE-RECEPTOR; OLEFIN AZIRIDINATION; MOLECULAR-ORBITALS; AMINOBUTYRIC-ACID AB A new class of radical metal-carbene complex has been characterized as having Fischer-like orbital interactions and adjacent pi acceptor stabilization. Density functional theory along with natural bond orbital analysis and charge decomposition analysis has given insight into the electronics of this catalytic intermediate in an open-shell cobalt-porphyrin, [Co(Por)], system. The complex has a single bond from the metal to the carbene and has radical character with localized spin density on the carbene carbon. In addition, the carbene carbon is found to be nucleophilic and "tunable" through the introduction of different alpha-carbon substituents. Finally, based on these findings, rational design strategies are proposed that should lead to the enhancement of catalytic activity. C1 [Belof, Jonathan L.; Cioce, Christian R.; Xu, Xue; Zhang, X. Peter; Space, Brian; Woodcock, H. Lee] Univ S Florida, Dept Chem, Tampa, FL 33620 USA. [Belof, Jonathan L.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Woodcock, HL (reprint author), Univ S Florida, Dept Chem, 4202 Fowler Ave,CHE205, Tampa, FL 33620 USA. EM hlw@mail.usf.edu RI Zhang, Peter/B-7976-2011; Cioce, Christian/E-2875-2013; OI Zhang, Peter/0000-0001-7574-8409; Woodcock, Henry/0000-0003-3539-273X FU NIH [1K22HL088341-01A1]; University of South Florida; NCSA [TG-DMR090028]; NSF [CHE-0722887, CHE-0711024]; U.S. Department of Energy [DE0GG02-07ER46470]; U.S. Department of Defense [HDTRA1-08-C-0035]; Draper Laboratory [URAD2010187] FX H.L.W. would like to acknowledge NIH (1K22HL088341-01A1) and the University of South Florida (start-up) for funding. Computations were performed on the NCSA Cobalt supercomputer under a Teragrid Grant (Grant No. TG-DMR090028) to B.S., and also at the USF Research Computing Center, where NSF-funded computational resources (under Grant No. CHE-0722887) were greatly appreciated. B.S. and X.P.Z. acknowledge funding from the U.S. Department of Energy (Grant No. DE0GG02-07ER46470), the U.S. Department of Defense (Grant No. HDTRA1-08-C-0035), the National Science Foundation (Grant No. CHE-0711024), and Draper Laboratory (Grant No. URAD2010187). The authors also thank the Space Foundation (Basic and Applied Research) for partial support. NR 83 TC 32 Z9 32 U1 4 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 J9 ORGANOMETALLICS JI Organometallics PD MAY 23 PY 2011 VL 30 IS 10 BP 2739 EP 2746 DI 10.1021/om2001348 PG 8 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA 799TA UT WOS:000293307800015 PM 21643517 ER PT J AU Lavrik, NV Taylor, LT Sepaniak, MJ AF Lavrik, N. V. Taylor, L. T. Sepaniak, M. J. TI Nanotechnology and chip level systems for pressure driven liquid chromatography and emerging analytical separation techniques: A review SO ANALYTICA CHIMICA ACTA LA English DT Review DE Microfluidic; Pressure driven separation; HPLC; Pillar arrays; Liquid chromatography; Nanocolumns ID PILLAR-ARRAY COLUMNS; DETERMINISTIC LATERAL DISPLACEMENT; ELECTROSPRAY MASS-SPECTROMETRY; ENHANCED RAMAN-SCATTERING; HIGH-ASPECT-RATIO; ON-A-CHIP; CAPILLARY-ELECTROPHORESIS DEVICES; MONOLITHIC SILICA COLUMN; MICROFLUIDIC DEVICES; HPLC-CHIP AB Pressure driven liquid chromatography (LC) is a powerful and versatile separation technique particularly suitable for differentiating species present in extremely small quantities. This paper briefly reviews main historical trends and focuses on more recently developed technological approaches in miniaturization and on-chip integration of LC columns. The review emphasizes enabling technologies as well as main technological challenges specific to pressure driven separations and highlights emerging concepts that could ultimately overcome fundamental limitations of conventional LC columns. (C) 2011 Elsevier B.V. All rights reserved. C1 [Taylor, L. T.; Sepaniak, M. J.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Lavrik, N. V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37830 USA. RP Sepaniak, MJ (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM msepaniak@utk.edu RI Lavrik, Nickolay/B-5268-2011 OI Lavrik, Nickolay/0000-0002-9543-5634 FU Office of Basic Energy Sciences, U.S. Department of Energy; Office of Basic Energy Sciences; US Environmental Protection Agency [EPA-83274001]; University of Tennessee FX A portion of this work was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Office of Basic Energy Sciences, U.S. Department of Energy. NVL acknowledges support by the Office of Basic Energy Sciences. This research was also supported by the US Environmental Protection Agency STAR Program under grant EPA-83274001 with the University of Tennessee. NR 163 TC 36 Z9 37 U1 2 U2 77 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0003-2670 J9 ANAL CHIM ACTA JI Anal. Chim. Acta PD MAY 23 PY 2011 VL 694 IS 1-2 BP 6 EP 20 DI 10.1016/j.aca.2011.03.059 PG 15 WC Chemistry, Analytical SC Chemistry GA 772MZ UT WOS:000291239300002 PM 21565297 ER PT J AU Arnaldi, R Banicz, K Castor, J Chaurand, B Chen, W Cicalo, C Colla, A Cortese, P Damjanovic, S David, A de Falco, A Devaux, A Ducroux, L En'yo, H Fargeix, J Ferretti, A Floris, M Forster, A Force, P Guettet, N Guichard, A Gulkanian, H Heuser, JM Keil, M Li, Z Lourenco, C Lozano, J Manso, F Martins, P Masoni, A Neves, A Ohnishi, H Oppedisano, C Parracho, P Pillot, P Poghosyan, T Puddu, G Radermacher, E Ramalhete, P Rosinsky, P Scomparin, E Seixas, J Serci, S Shahoyan, R Sonderegger, P Specht, HJ Tieulent, R Uras, A Usai, G Veenhof, R Wohri, HK AF Arnaldi, R. Banicz, K. Castor, J. Chaurand, B. Chen, W. Cicalo, C. Colla, A. Cortese, P. Damjanovic, S. David, A. de Falco, A. Devaux, A. Ducroux, L. En'yo, H. Fargeix, J. Ferretti, A. Floris, M. Foerster, A. Force, P. Guettet, N. Guichard, A. Gulkanian, H. Heuser, J. M. Keil, M. Li, Z. Lourenco, C. Lozano, J. Manso, F. Martins, P. Masoni, A. Neves, A. Ohnishi, H. Oppedisano, C. Parracho, P. Pillot, P. Poghosyan, T. Puddu, G. Radermacher, E. Ramalhete, P. Rosinsky, P. Scomparin, E. Seixas, J. Serci, S. Shahoyan, R. Sonderegger, P. Specht, H. J. Tieulent, R. Uras, A. Usai, G. Veenhof, R. Woehri, H. K. CA NA60 Collaboration TI A comparative measurement of phi -> K+K- and phi -> mu(+)mu(-) in In-In collisions at the CERN SPS SO PHYSICS LETTERS B LA English DT Article DE Heavy ion collisions; phi puzzle ID HEAVY-ION COLLISIONS; MESON PRODUCTION; DECAYS; MATTER AB The NA60 experiment at the CERN SPS has studied phi meson production in In-In collisions at 158 AGeV via both the K+K- and the mu(+)mu(-) decay channels. The yields and inverse slope parameters of the m(T) spectra observed in the two channels are compatible within errors, different from the large discrepancies seen in Pb-Pb collisions between the hadronic (NA49) and dimuon (NA50) decay channels. Possible physics implications are discussed. (C) 2011 Elsevier B.V. All rights reserved. C1 [de Falco, A.; Floris, M.; Puddu, G.; Serci, S.; Uras, A.; Usai, G.; Woehri, H. K.] Univ Cagliari, Cagliari, Italy. [Arnaldi, R.; Oppedisano, C.; Scomparin, E.] Ist Nazl Fis Nucl, Sez Torino, Cagliari, Italy. [Banicz, K.; Damjanovic, S.; David, A.; Foerster, A.; Guettet, N.; Keil, M.; Lourenco, C.; Martins, P.; Parracho, P.; Radermacher, E.; Ramalhete, P.; Rosinsky, P.; Shahoyan, R.; Veenhof, R.] CERN, CH-1211 Geneva 23, Switzerland. [Banicz, K.; Damjanovic, S.; Specht, H. J.] Heidelberg Univ, Inst Phys, D-6900 Heidelberg, Germany. [Castor, J.; Devaux, A.; Fargeix, J.; Force, P.; Manso, F.] Univ Blaise Pascal, LPC, Clermont Ferrand, France. [Castor, J.; Devaux, A.; Force, P.; Guettet, N.] Univ Clermont Ferrand 2, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Chaurand, B.] Ecole Polytech, LLR, Palaiseau, France. [Chaurand, B.] CNRS, IN2P3, Palaiseau, France. [Chen, W.; Li, Z.] BNL, Upton, NY USA. [Cicalo, C.; Masoni, A.] Ist Nazl Fis Nucl, Sez Cagliari, Cagliari, Italy. [Colla, A.; Cortese, P.; Ferretti, A.] Univ Turin, I-10124 Turin, Italy. [David, A.; Keil, M.; Lozano, J.; Martins, P.; Neves, A.; Parracho, P.; Seixas, J.; Shahoyan, R.; Sonderegger, P.; Woehri, H. K.] Inst Super Tecn, Lisbon, Portugal. [Ducroux, L.; Guichard, A.; Pillot, P.; Tieulent, R.] Univ Lyon 1, IPN Lyon, F-69365 Lyon, France. [Ducroux, L.; Guichard, A.; Pillot, P.; Tieulent, R.] CNRS, IN2P3, Lyon, France. [En'yo, H.; Heuser, J. M.; Ohnishi, H.] RIKEN, Wako, Saitama, Japan. [Gulkanian, H.; Poghosyan, T.] Yerevan Phys Inst, Yerevan 375036, Armenia. RP de Falco, A (reprint author), Univ Cagliari, Cagliari, Italy. EM alessandro.de.falco@ca.infn.it RI En'yo, Hideto/B-2440-2015; Usai, Gianluca/E-9604-2015; Lozano-Bahilo, Julio/F-4881-2016; Ferretti, Alessandro/F-4856-2013; Tinoco Mendes, Andre David/D-4314-2011; Cortese, Pietro/G-6754-2012; Colla, Alberto/J-4694-2012 OI Usai, Gianluca/0000-0002-8659-8378; Lozano-Bahilo, Julio/0000-0003-0613-140X; Ferretti, Alessandro/0000-0001-9084-5784; Tinoco Mendes, Andre David/0000-0001-5854-7699; NR 18 TC 6 Z9 6 U1 0 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAY 23 PY 2011 VL 699 IS 5 BP 325 EP 329 DI 10.1016/j.physletb.2011.04.028 PG 5 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 771CK UT WOS:000291134600003 ER PT J AU Griggio, F Jesse, S Kumar, A Marincel, DM Tinberg, DS Kalinin, SV Trolier-McKinstry, S AF Griggio, F. Jesse, S. Kumar, A. Marincel, D. M. Tinberg, D. S. Kalinin, S. V. Trolier-McKinstry, S. TI Mapping piezoelectric nonlinearity in the Rayleigh regime using band excitation piezoresponse force microscopy SO APPLIED PHYSICS LETTERS LA English DT Article ID FERROELECTRIC THIN-FILMS; DYNAMICS AB Band excitation piezoresponse force microscopy enables local investigation of the nonlinear piezoelectric behavior of ferroelectric thin films. However, the presence of additional nonlinearity associated with the dynamic resonant response of the tip-surface junction can complicate the study of a material's nonlinearity. Here, the relative importance of the two nonlinearity sources was examined as a function of the excitation function. It was found that in order to minimize the effects of nonlinear tip-surface interactions but achieve good signal to noise level, an optimal excitation function must be used. (C) 2011 American Institute of Physics. [doi: 10.1063/1.3593138] C1 [Griggio, F.; Marincel, D. M.; Tinberg, D. S.; Trolier-McKinstry, S.] Penn State Univ, Dept Mat Sci & Engn, Mat Res Inst, Mat Res Lab, University Pk, PA 16802 USA. [Jesse, S.; Kumar, A.; Kalinin, S. V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Jesse, S.; Kumar, A.; Kalinin, S. V.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Trolier-McKinstry, S (reprint author), Penn State Univ, Dept Mat Sci & Engn, Mat Res Inst, Mat Res Lab, University Pk, PA 16802 USA. EM fxg14@psu.edu; stmckinstry@psu.edu RI Kumar, Amit/C-9662-2012; Kalinin, Sergei/I-9096-2012; Jesse, Stephen/D-3975-2016; OI Kumar, Amit/0000-0002-1194-5531; Kalinin, Sergei/0000-0001-5354-6152; Jesse, Stephen/0000-0002-1168-8483; Trolier-McKinstry, Susan/0000-0002-7267-9281 FU National Security Science and Engineering Faculty Fellowship; CNMS [CNMS2010-090]; Oak Ridge National Laboratory by the Office of Basic Energy Sciences, U. S. Department of Energy [DE-AC05-00OR22725] FX Support for this work was provided in part by the National Security Science and Engineering Faculty Fellowship and by CNMS user Proposal No. CNMS2010-090 (F. G. and S. T. M.). A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Office of Basic Energy Sciences, U. S. Department of Energy under contract DE-AC05-00OR22725. Thanks to Oleg Ovchinnikov for useful discussions on MATLAB coding. NR 14 TC 17 Z9 17 U1 1 U2 24 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 23 PY 2011 VL 98 IS 21 AR 212901 DI 10.1063/1.3593138 PG 3 WC Physics, Applied SC Physics GA 769TQ UT WOS:000291041600056 ER PT J AU Klaer, P Jenkins, CA Alijani, V Winterlik, J Balke, B Felser, C Elmers, HJ AF Klaer, P. Jenkins, C. A. Alijani, V. Winterlik, J. Balke, B. Felser, C. Elmers, H. J. TI Disentangling the Mn moments on different sublattices in the half-metallic ferrimagnet Mn3-xCoxGa SO APPLIED PHYSICS LETTERS LA English DT Article ID RAY CIRCULAR-DICHROISM AB Ferrimagnetic Mn3-xCoxGa compounds have been investigated by magnetic circular dichroism in x-ray absorption (XMCD). Compounds with x>0.5 crystallize in the CuHg2Ti structure. A tetragonal distortion of the cubic structure occurs for x <= 0.5. For the cubic phase, magnetometry reveals a linearly increasing magnetization of 2x Bohr magnetons per formula unit obeying the generalized Slater-Pauling rule. XMCD confirms the ferrimagnetic character with Mn atoms occupying two different sublattices with antiparallel spin orientation and different degrees of spin localization and identifies the region 0.6omega > I(2)) regime. We show that the energy spacing Delta E = E(1) - E(2) between the two emitted electrons provides the key parameter that controls both the energy and the angular distribution and reveals the universal features present in both the nonsequential and sequential regime. This universality, i.e., independence of (h) over bar omega, is a manifestation of the continuity across the threshold for sequential double ionization. For all photon energies considered, the energy distribution can be described by a universal shape function that contains only the spectral and temporal information entering second-order time-dependent perturbation theory. Angular correlations and distributions are found to be more sensitive to the value of (h) over bar omega. In particular, shake-up interferences have a large effect on the angular distribution. Energy spectra, angular distributions parametrized by the anisotropy parameters beta(j), and total cross sections presented in this paper are obtained by fully correlated time-dependent ab initio calculations. C1 [Pazourek, R.; Feist, J.; Nagele, S.; Persson, E.; Burgdoerfer, J.] Vienna Univ Technol, Inst Theoret Phys, A-1040 Vienna, Austria. [Feist, J.] Harvard Smithsonian Ctr Astrophys, ITAMP, Cambridge, MA 02138 USA. [Schneider, B. I.] Natl Sci Fdn, Div Phys, Off Cyberinfrastruct, Arlington, VA 22230 USA. [Collins, L. A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Pazourek, R (reprint author), Vienna Univ Technol, Inst Theoret Phys, A-1040 Vienna, Austria. EM renate.pazourek@tuwien.ac.at RI Nagele, Stefan/E-6938-2011; Feist, Johannes/J-7394-2012 OI Nagele, Stefan/0000-0003-1213-0294; Feist, Johannes/0000-0002-7972-0646 FU FWF-Austria [SFB016, P21141-N16]; NSF [TG-PHY090031]; US Department of Energy [DE-AC52-06NA25396] FX We thank I. Ivanov for sending us results in numerical form. R.P., J.F., S.N., E.P., and J.B. acknowledge support by the FWF-Austria, Grants No. SFB016 and No. P21141-N16. J.F. acknowledges support by the NSF through a grant to ITAMP. This research was supported in part by the National Science Foundation through TeraGrid resources provided by NICS and TACC under Grant No. TG-PHY090031. Additional computational time was provided by the Vienna Scientific Cluster (VSC) and under Institutional Computing at Los Alamos National Laboratory. The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the National Nuclear Security Administration of the US Department of Energy under Contract No. DE-AC52-06NA25396. NR 54 TC 29 Z9 30 U1 0 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 J9 PHYS REV A JI Phys. Rev. A PD MAY 20 PY 2011 VL 83 IS 5 AR 053418 DI 10.1103/PhysRevA.83.053418 PG 11 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 767MF UT WOS:000290860000009 ER PT J AU Koretsune, T Saito, S Cohen, ML AF Koretsune, Takashi Saito, Susumu Cohen, Marvin L. TI One-dimensional alkali-doped C-60 chains encapsulated in BN nanotubes SO PHYSICAL REVIEW B LA English DT Article ID BORON-NITRIDE NANOTUBES; ELECTRON-PHONON INTERACTIONS; CARBON NANOTUBE; SUPERCONDUCTIVITY; MICROTUBULES AB We study the energetics, electronic structures, and electron-phonon couplings of a one-dimensional potassium-doped C-60 chain encapsulated in a boron nitride nanotube using the framework of the density-functional theory. We demonstrate that the reaction of potassium doping is exothermic and the resulting material is one-dimensional metal where conducting electrons are only in the C-60 chain. Interestingly, the Fermi-level density of states has a peculiar pressure dependence and can be larger than those in the three-dimensional alkali-doped fullerene compounds, indicating the possibility of various phase transitions. We also discuss the electron-phonon couplings and the possibility of superconductivity. C1 [Koretsune, Takashi; Saito, Susumu] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan. [Cohen, Marvin L.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Cohen, Marvin L.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Koretsune, T (reprint author), Tokyo Inst Technol, Dept Phys, Meguro Ku, 2-12-1 Oh Okayama, Tokyo 1528551, Japan. RI Koretsune, Takashi/D-3209-2017 OI Koretsune, Takashi/0000-0002-5334-0792 FU National Science Foundation [DMR07-05941]; Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy [DE-AC02-05CH11231]; MEXT Japan [22740252, 22013005, 19054005]; Ishikawa Carbon Foundation; MEXT Japan through the Tokyo Institute of Technology FX We would like to thank J. Noffsinger for useful discussions. Numerical calculations were performed on TSUB-AME Grid Cluster at Global Scientific Information and Computing Center of the Tokyo Institute of Technology. This work was partially supported by National Science Foundation Grant No. DMR07-05941, by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy under Contract No. DE-AC02-05CH11231, by a Grant-in-Aid for Scientific Research (Contracts No. 22740252, No. 22013005, and No. 19054005) and Elements Science and Technology Project from MEXT Japan, by Ishikawa Carbon Foundation, and by the Global Center of Excellence Program by MEXT Japan through the "Nanoscience and Quantum Physics" Project of the Tokyo Institute of Technology. NR 31 TC 1 Z9 1 U1 1 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD MAY 20 PY 2011 VL 83 IS 19 AR 193406 DI 10.1103/PhysRevB.83.193406 PG 4 WC Physics, Condensed Matter SC Physics GA 767OC UT WOS:000290864900001 ER PT J AU Zaki, N Knox, K Johnson, PD Fujii, J Vobornik, I Panaccione, G Osgood, RM AF Zaki, N. Knox, K. Johnson, P. D. Fujii, J. Vobornik, I. Panaccione, G. Osgood, R. M. TI Surface states on vicinal Cu(775): STM and photoemission study SO PHYSICAL REVIEW B LA English DT Article ID STEP MODULATION; WAVE-FUNCTION; TERRACE AB We report angle-resolved photoemission spectroscopy (ARPES) and a set of in situ scanning tunneling microscopy (STM) measurements on a narrow-terrace-width vicinal Cu(111) crystal surface, Cu(775), whose vicinal cut lies close to the transition between terrace and step modulation. These measurements show sharp zone-folding (or umklapp) features with a periodicity in k(parallel to), indicating that the predominant reference plane is that of Cu(775), i.e., that the surface is predominately step-modulated. Our measurements also show variation in umklapp intensity with photon energy, which is consistent with prior ARPES experiments on other vicinal Cu(111) surfaces and in agreement with our designation of the state as being step-modulated. The measurements also show a weak terrace-modulated state, which, based on several characteristics, we attribute to the presence of terrace widths larger than the ideal terrace width. By measuring the intensity ratio of the two distinct surface-state modulations from photoemission and the terrace-width distribution from STM, we derive a value for the terrace width at which the surface state switches between the two modulations. C1 [Zaki, N.; Knox, K.; Osgood, R. M.] Columbia Univ, New York, NY 10027 USA. [Johnson, P. D.] Brookhaven Natl Lab, New York, NY 11973 USA. [Fujii, J.; Vobornik, I.; Panaccione, G.] Lab TASC, Ist Officina Mat Consiglio Nazl Ric IOM CNR, I-34149 Trieste, Italy. RP Zaki, N (reprint author), Columbia Univ, New York, NY 10027 USA. RI Vobornik, Ivana/B-9463-2015; Vobornik, Ivana/A-7461-2011; OI Vobornik, Ivana/0000-0001-9957-3535; Jun, Fujii/0000-0003-3208-802X FU Department of Energy [DE-FG 02-04-ER-46157, DE-AC02-98CH10886] FX This research was supported by the Department of Energy Contract No. DE-FG 02-04-ER-46157. Work at Brookhaven National Laboratory was supported by the Department of Energy under Contract No. DE-AC02-98CH10886. We thank Jerry Dadap, Mehmet Yilmaz, and Manolis Antonoyiannak for several useful comments and suggestions. We thank Peter Lucak for writing some of the step-width analysis code. NR 24 TC 7 Z9 7 U1 2 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAY 20 PY 2011 VL 83 IS 20 AR 205420 DI 10.1103/PhysRevB.83.205420 PG 7 WC Physics, Condensed Matter SC Physics GA 767OV UT WOS:000290866800007 ER PT J AU Yeoh, EY Zhu, SJ Hamilton, JH Li, K Ramayya, AV Liu, YX Hwang, JK Liu, SH Wang, JG Sun, Y Sheikh, JA Bhat, GH Luo, YX Rasmussen, JO Lee, IY Ding, HB Gu, L Xu, Q Xiao, ZG Ma, WC AF Yeoh, E. Y. Zhu, S. J. Hamilton, J. H. Li, K. Ramayya, A. V. Liu, Y. X. Hwang, J. K. Liu, S. H. Wang, J. G. Sun, Y. Sheikh, J. A. Bhat, G. H. Luo, Y. X. Rasmussen, J. O. Lee, I. Y. Ding, H. B. Gu, L. Xu, Q. Xiao, Z. G. Ma, W. C. TI High-spin structure and multiphonon gamma vibrations in very neutron-rich Ru-114 SO PHYSICAL REVIEW C LA English DT Article ID PROJECTED SHELL-MODEL; IDENTICAL BANDS; PARITY BANDS; RU-108,RU-110,RU-112; NUCLEI; ISOTOPES; STATES AB High-spin levels of the neutron-rich Ru-114 have been investigated by measuring the prompt. rays in the spontaneous fission of Cf-252. The ground-state band and one-phonon gamma-vibrational band have been extended up to 14(+) and 9(+), respectively. Two levels are proposed as the members of a two-phonon gamma-vibrational band. A back bending (band crossing) has been observed in the ground-state band at (h) over bar omega approximate to 0.40 MeV. Using the triaxial deformation parameters, the cranked shell model calculations indicate that this back bending in Ru-114 should originate from the alignment of a pair of h(11/2) neutrons. Triaxial projected shell model calculations for the gamma-vibrational band structures of Ru-114 are in good agreement with the experimental data. However, when using the oblate deformation parameters, both of the above-calculated results are not in agreement with the experimental data. C1 [Yeoh, E. Y.; Zhu, S. J.; Wang, J. G.; Ding, H. B.; Gu, L.; Xu, Q.; Xiao, Z. G.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Zhu, S. J.; Hamilton, J. H.; Li, K.; Ramayya, A. V.; Hwang, J. K.; Liu, S. H.; Luo, Y. X.] Vanderbilt Univ, Dept Phys, Nashville, TN 37235 USA. [Liu, Y. X.] Huzhou Teachers Coll, Sch Sci, Huzhou 313000, Peoples R China. [Liu, S. H.] UNIRIB Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. [Sun, Y.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200240, Peoples R China. [Sheikh, J. A.; Bhat, G. H.] Univ Kashmir, Dept Phys, Srinagar 190006, Jammu & Kashmir, India. [Luo, Y. X.; Rasmussen, J. O.; Lee, I. Y.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Ma, W. C.] Mississippi State Univ, Dept Phys, Mississippi State, MS 39762 USA. RP Yeoh, EY (reprint author), Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. EM zhushj@mail.tsinghua.edu.cn RI XIAO, Zhigang/C-3788-2015; Sun, Yang/P-2417-2015 FU National Natural Science Foundation of China [10975082, 10875077, 10975051, 11075103]; Major State Basic Research Development Program [2007CB815005]; Higher Education Science Foundation [20100002110077]; US Department of Energ [DE-FG05-88ER40407]; [DE-AC03-76SF00098] FX The work at Tsinghua University, Shanghai Jiao Tong University, and Huzhou Teachers College was supported by the National Natural Science Foundation of China under Grants No. 10975082, No. 10875077, No. 10975051, and No. 11075103, the Major State Basic Research Development Program under Grant No. 2007CB815005, and the Special Program of Higher Education Science Foundation under Grant No. 20100002110077, respectively. The work at Vanderbilt University and LBNL was supported by the US Department of Energy under Grant No. DE-FG05-88ER40407 and Contract No. DE-AC03-76SF00098, respectively. NR 28 TC 11 Z9 13 U1 0 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 J9 PHYS REV C JI Phys. Rev. C PD MAY 20 PY 2011 VL 83 IS 5 AR 054317 DI 10.1103/PhysRevC.83.054317 PG 6 WC Physics, Nuclear SC Physics GA 767RX UT WOS:000290874800001 ER PT J AU An, YQ Taylor, AJ Conradson, SD Trugman, SA Durakiewicz, T Rodriguez, G AF An, Yong Q. Taylor, Antoinette J. Conradson, Steven D. Trugman, Stuart A. Durakiewicz, Tomasz Rodriguez, George TI Ultrafast Hopping Dynamics of 5f Electrons in the Mott Insulator UO2 Studied by Femtosecond Pump-Probe Spectroscopy SO PHYSICAL REVIEW LETTERS LA English DT Article ID URANIUM-DIOXIDE; POLARON; CRYSTAL; PHONONS; ENERGY AB We describe a femtosecond pump-probe study of ultrafast hopping dynamics of 5f electrons in the Mott insulator UO2 following Mott-gap excitation at temperatures of 5-300 K. Hopping-induced response of the lattice and electrons is probed by transient reflectivity at mid- and above-gap photon energies, respectively. These measurements show an instantaneous hop, subsequent picosecond lattice deformation, followed by acoustic phonon emission and microsecond relaxation. Temperature-dependent studies indicate that the slow relaxation results from Hubbard excitons formed by U3+ - U5+ pairs. C1 [An, Yong Q.; Taylor, Antoinette J.; Conradson, Steven D.; Trugman, Stuart A.; Durakiewicz, Tomasz; Rodriguez, George] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP An, YQ (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM yqan@lanl.gov RI An, Yong/N-7479-2013; Rodriguez, George/G-7571-2012; OI Rodriguez, George/0000-0002-6044-9462; Durakiewicz, Tomasz/0000-0002-1980-1874; Trugman, Stuart/0000-0002-6688-7228 FU LDRD; BES FX We thank R. L. Martin, J. Demsar, Y.-S. Park, and M. T. Paffett for helpful contributions. This work was performed, in part, at CINT and supported by LDRD and BES core materials program. NR 23 TC 16 Z9 16 U1 3 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 207402 DI 10.1103/PhysRevLett.106.207402 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200025 PM 21668262 ER PT J AU Banerjee, P Haxton, WC Qian, YZ AF Banerjee, Projjwal Haxton, W. C. Qian, Yong-Zhong TI Long, Cold, Early r Process? Neutrino-Induced Nucleosynthesis in He Shells Revisited SO PHYSICAL REVIEW LETTERS LA English DT Article ID BLACK-HOLE FORMATION; STAR MERGERS; HELIUM SHELL; EARLY GALAXY; SUPERNOVAE; EVOLUTION; ELEMENTS; ABUNDANCES; DEPENDENCE; DYNAMICS AB We revisit a nu-driven r-process mechanism in the He shell of a core-collapse supernova, finding that it could succeed in early stars of metallicity Z less than or similar to 10(-3)Z(circle dot), at relatively low temperatures and neutron densities, producing A similar to 130 and 195 abundance peaks over similar to 10-20 s. The mechanism is sensitive to the nu emission model and to nu oscillations. We discuss the implications of an r process that could alter interpretations of abundance data from metal-poor stars, and point out the need for further calculations that include effects of the supernova shock. C1 [Banerjee, Projjwal; Qian, Yong-Zhong] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Haxton, W. C.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Haxton, W. C.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Banerjee, P (reprint author), Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. EM banerjee@physics.umn.edu; haxton@berkeley.edu; qian@physics.umn.edu FU U.S. DOE at UMN [DE-FG02-87ER40328]; U.S. DOE at Berkeley [DE-SC00046548] FX We thank Alexander Heger for discussions of massive stars and Frank Timmes and Rob Hoffman for help with the torch network. This work was supported in part by the U.S. DOE under DE-FG02-87ER40328 at UMN and DE-SC00046548 at Berkeley. NR 28 TC 35 Z9 35 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 201104 DI 10.1103/PhysRevLett.106.201104 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200007 PM 21668217 ER PT J AU Drut, JE Lahde, TA Ten, T AF Drut, Joaquin E. Lahde, Timo A. Ten, Timour TI Momentum Distribution and Contact of the Unitary Fermi Gas SO PHYSICAL REVIEW LETTERS LA English DT Article ID PHYSICS; MATTER; ATOMS AB We calculate the momentum distribution n(k) of the unitary Fermi gas by using quantum Monte Carlo calculations at finite temperature T/epsilon(F) as well as in the ground state. At large momenta k/k(F), we find that n(k) falls off as C/k(4), in agreement with the Tan relations. From the asymptotics of n(k), we determine the contact C as a function of T/epsilon(F) and present a comparison with theory. At low T/epsilon(F), we find that C increases with temperature, and we tentatively identify a maximum around T/epsilon(F) similar or equal to 0.4. Our calculations are performed on lattices of spatial extent up to N(x) = 14 with a particle number per unit volume of similar or equal to 0.03-0.07. C1 [Drut, Joaquin E.; Ten, Timour] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Drut, Joaquin E.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Lahde, Timo A.] Aalto Univ, Helsinki Inst Phys, FI-00076 Espoo, Finland. [Lahde, Timo A.] Aalto Univ, Dept Appl Phys, FI-00076 Espoo, Finland. [Ten, Timour] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. RP Drut, JE (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. FU U.S. DOE [DE-FG02-00ER41132, DE-AC02-05CH11231]; UNEDF SciDAC Collaboration [DE-FC02-09ER41586]; NSF [PHY-0653312]; Academy of Finland; Vilho, Yrjo, and Kalle Vaisala Foundation of the Finnish Academy of Science and Letters; Waldemar von Frenckell Foundation of the Finnish Society of Sciences and Letters; Magnus Ehrnrooth Foundation of the Finnish Society of Sciences and Letters FX We thank R. J. Furnstahl for encouragement and A. Bulgac, J. Carlson, S. Gandolfi, A. Gezerlis, and K. Schmidt for instructive discussions and comments. We are also grateful to T. Enss, H. Hu, and F. Palestini for giving us access to their respective results. We acknowledge support under U.S. DOE Grants No. DE-FG02-00ER41132 and No. DE-AC02-05CH11231, UNEDF SciDAC Collaboration Grant No. DE-FC02-09ER41586, and NSF Grant No. PHY-0653312. This study was supported, in part, by the Academy of Finland through its Centers of Excellence Program (2006-2011), the Vilho, Yrjo, and Kalle Vaisala Foundation of the Finnish Academy of Science and Letters, and the Waldemar von Frenckell and Magnus Ehrnrooth Foundations of the Finnish Society of Sciences and Letters. Part of this work was performed by using an allocation of computing time from the Ohio Supercomputer Center. NR 59 TC 38 Z9 38 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 205302 DI 10.1103/PhysRevLett.106.205302 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200016 PM 21668239 ER PT J AU Harvey-Thompson, AJ Lebedev, SV Burdiak, G Waisman, EM Hall, GN Suzuki-Vidal, F Bland, SN Chittenden, JP De Grouchy, P Khoory, E Pickworth, L Skidmore, J Swadling, G AF Harvey-Thompson, A. J. Lebedev, S. V. Burdiak, G. Waisman, E. M. Hall, G. N. Suzuki-Vidal, F. Bland, S. N. Chittenden, J. P. De Grouchy, P. Khoory, E. Pickworth, L. Skidmore, J. Swadling, G. TI Suppression of the Ablation Phase in Wire Array Z Pinches Using a Tailored Current Prepulse SO PHYSICAL REVIEW LETTERS LA English DT Article ID ENHANCEMENT; IMPLOSION; POWER AB A new wire array configuration has been used to create thin shell-like implosions in a cylindrical array. The setup introduces a similar to 5 kA, similar to 25 ns current prepulse followed by a similar to 140 ns current-free interval before the application of the main (similar to 1 MA) current pulse. The prepulse volumetrically heats the wires which expand to similar to 1 mm diameter leaving no dense wire core and without development of instabilities. The main current pulse then ionizes all the array mass resulting in suppression of the ablation phase, an accelerating implosion, and no trailing mass. Rayleigh-Taylor instability growth in the imploding plasma is inferred to be seeded by mu m-scale perturbations on the surface of the wires. The absence of wire cores is found to be the critical factor in altering the implosion dynamics. C1 [Harvey-Thompson, A. J.; Lebedev, S. V.; Burdiak, G.; Hall, G. N.; Suzuki-Vidal, F.; Bland, S. N.; Chittenden, J. P.; De Grouchy, P.; Khoory, E.; Pickworth, L.; Skidmore, J.; Swadling, G.] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, London SW7 2BW, England. [Waisman, E. M.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Harvey-Thompson, AJ (reprint author), Univ London Imperial Coll Sci Technol & Med, Blackett Lab, London SW7 2BW, England. RI Hall, Gareth/C-4179-2015; Swadling, George/S-5980-2016 OI Swadling, George/0000-0001-8370-8837 FU Sandia National Laboratories Albuquerque; NNSA under DOE [DE-F03-02NA00057] FX The authors are grateful to Dr. M. E. Cuneo and Dr. R. B. Spielman for many useful discussions. This research was sponsored by Sandia National Laboratories Albuquerque and the NNSA under DOE Cooperative Agreement No. DE-F03-02NA00057. NR 13 TC 26 Z9 28 U1 1 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 205002 DI 10.1103/PhysRevLett.106.205002 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200014 PM 21668237 ER PT J AU Lo, CC Lang, V George, RE Morton, JJL Tyryshkin, AM Lyon, SA Bokor, J Schenkel, T AF Lo, C. C. Lang, V. George, R. E. Morton, J. J. L. Tyryshkin, A. M. Lyon, S. A. Bokor, J. Schenkel, T. TI Electrically Detected Magnetic Resonance of Neutral Donors Interacting with a Two-Dimensional Electron Gas SO PHYSICAL REVIEW LETTERS LA English DT Article ID SPIN-RESONANCE; SILICON; SCATTERING AB We have measured the electrically detected magnetic resonance of donor-doped silicon field-effect transistors in resonant X- (9.7 GHz) and W-band (94 GHz) microwave cavities. The two-dimensional electron gas resonance signal increases by 2 orders of magnitude from X to W band, while the donor resonance signals are enhanced by over 1 order of magnitude. Bolometric effects and spin-dependent scattering are inconsistent with the observations. We propose that polarization transfer from the donor to the two-dimensional electron gas is the main mechanism giving rise to the spin resonance signals. C1 [Lo, C. C.; Bokor, J.] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Lang, V.; Morton, J. J. L.] Univ Oxford, Dept Mat, Oxford OX1 3PH, England. [George, R. E.; Morton, J. J. L.] Univ Oxford, Dept Phys, Clarendon Lab, CAESR, Oxford OX1 3PU, England. [Tyryshkin, A. M.; Lyon, S. A.] Princeton Univ, Dept Elect Engn, Princeton, NJ 08544 USA. [Schenkel, T.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Accelerator & Fus Res, Berkeley, CA 94720 USA. RP Lo, CC (reprint author), Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. EM cclo@eecs.berkeley.edu; volker.lang@materials.ox.ac.uk RI Morton, John/I-3515-2013; Bokor, Jeffrey/A-2683-2011 FU U.S. National Security Agency [100000080295]; DOE [DE-AC02-05CH11231 (LBNL)]; EPSRC [EP/D048559/1 (Oxford)]; NSF [DMR-0213706 (Princeton)]; Konrad-Adenauer-Stiftung e.V; Royal Society; St. John's College, Oxford FX We thank A. Ardavan, R. de Sousa, and T. Last for useful discussions, and the UC Berkeley Microlab staff for technical support in device fabrication. This work was supported by the U.S. National Security Agency under 100000080295. Additional support by the DOE under Contract No. DE-AC02-05CH11231 (LBNL), EPSRC through CAESR EP/D048559/1 (Oxford), and NSF through the Princeton MRSEC under Grant No. DMR-0213706 (Princeton) are also acknowledged. V. L. is supported by Konrad-Adenauer-Stiftung e.V. and EPSRC DTA. J.J.L.M. is supported by The Royal Society and St. John's College, Oxford. NR 31 TC 21 Z9 21 U1 1 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 207601 DI 10.1103/PhysRevLett.106.207601 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200026 PM 21668263 ER PT J AU Maris, P Vary, JP Navratil, P Ormand, WE Nam, H Dean, DJ AF Maris, P. Vary, J. P. Navratil, P. Ormand, W. E. Nam, H. Dean, D. J. TI Origin of the Anomalous Long Lifetime of C-14 SO PHYSICAL REVIEW LETTERS LA English DT Article ID EFFECTIVE-FIELD THEORY; MODEL-OPERATOR APPROACH; CHIRAL LAGRANGIANS; NUCLEAR-FORCES; SYSTEMS AB We report the microscopic origins of the anomalously suppressed beta decay of C-14 to N-14 using the ab initio no-core shell model with the Hamiltonian from the chiral effective field theory including three-nucleon force terms. The three-nucleon force induces unexpectedly large cancellations within the p shell between contributions to beta decay, which reduce the traditionally large contributions from the nucleon-nucleon interactions by an order of magnitude, leading to the long lifetime of C-14. C1 [Maris, P.; Vary, J. P.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Navratil, P.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Navratil, P.; Ormand, W. E.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Ormand, W. E.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Nam, H.; Dean, D. J.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Maris, P (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. FU U.S. DOE (UNEDF SciDAC Collaboration) [DE-FC02-09ER41582, DE-FG02-87ER40371]; DOE Office of Science [DE-AC05-00OR22725]; U.S. DOE [DE-AC05-00OR22725, DE-AC52-07NA27344] FX This work was supported in part by U.S. DOE Grants No. DE-FC02-09ER41582 (UNEDF SciDAC Collaboration) and No. DE-FG02-87ER40371 and by U.S. DOE Contracts No. DE-AC52-07NA27344 and No. DE-AC05-00OR22725. Computational resources were provided by Livermore Computing at LLNL and by the Oak Ridge Leadership Computing Facility at ORNL [21], which is supported by the DOE Office of Science under Contract No. DE-AC05-00OR22725. NR 34 TC 54 Z9 55 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 202502 DI 10.1103/PhysRevLett.106.202502 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200008 PM 21668224 ER PT J AU Velizhanin, KA Piryatinski, A AF Velizhanin, Kirill A. Piryatinski, Andrei TI Numerical Study of Carrier Multiplication Pathways in Photoexcited Nanocrystal and Bulk Forms of PbSe SO PHYSICAL REVIEW LETTERS LA English DT Article ID MULTIPLE EXCITON GENERATION; QUANTUM DOTS; SEMICONDUCTOR NANOCRYSTALS; MULTIEXCITON GENERATION; IMPACT IONIZATION; SOLAR-CELLS; EFFICIENCY AB Employing the interband exciton scattering model, we perform a numerical study of the direct photogeneration and population relaxation processes contributing to carrier multiplication (CM) in nanocrystalline and bulk PbSe. We argue that in both cases the impact ionization is the main mechanism of CM. This explains the weak contribution of the direct photogeneration to the total quantum efficiency (QE). An investigation of the size scaling of QE in nanocrystals and a comparison to the bulk limit provide microscopic insight into the experimentally observed trends. C1 [Velizhanin, Kirill A.; Piryatinski, Andrei] Los Alamos Natl Lab, Div Theoret, Ctr Nonlinear Studies CNLS, Los Alamos, NM 87545 USA. RP Velizhanin, KA (reprint author), Los Alamos Natl Lab, Div Theoret, Ctr Nonlinear Studies CNLS, Los Alamos, NM 87545 USA. EM apiryat@lanl.gov RI Piryatinski, Andrei/B-5543-2009; Velizhanin, Kirill/C-4835-2008 FU BES Office; DOE; Los Alamos LDRD; CNLS FX This work was supported by the BES Office, DOE, Los Alamos LDRD funds, and CNLS. We thank V. Klimov and D. Smith for stimulating discussions and comments on the manuscript. NR 27 TC 26 Z9 26 U1 0 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 207401 DI 10.1103/PhysRevLett.106.207401 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200024 PM 21668261 ER PT J AU Vieyra, HA Oeschler, N Seiro, S Jeevan, HS Geibel, C Parker, D Steglich, F AF Vieyra, H. A. Oeschler, N. Seiro, S. Jeevan, H. S. Geibel, C. Parker, D. Steglich, F. TI Determination of Gap Symmetry from Angle-Dependent Hc2 Measurements on CeCu2Si2 SO PHYSICAL REVIEW LETTERS LA English DT Article ID ANGULAR-DEPENDENCE; CRITICAL FIELDS; SUPERCONDUCTIVITY; MAGNETISM; CRYSTAL; STATE AB The tetragonal heavy-fermion compound CeCu2Si2 exhibits a superconducting ground state (S type, T-c = 0.67 K) close to a magnetic instability. Here, we present angle-resolved resistivity measurements of the upper critical field H-c2. In-plane rotation of S-type CeCu2Si2 single crystals reveals a fourfold oscillation of H-c2. An extended weak-coupling BCS model for a d-wave symmetry including strong Pauli-limiting effects confirms the aforementioned angular dependence and points towards d(xy) symmetry of the order parameter. C1 [Vieyra, H. A.; Oeschler, N.; Seiro, S.; Jeevan, H. S.; Geibel, C.; Steglich, F.] Max Planck Inst Chem Phys Solids, D-01187 Dresden, Germany. [Parker, D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Vieyra, HA (reprint author), Max Planck Inst Chem Phys Solids, Nothnitzer Str 40, D-01187 Dresden, Germany. EM Hugo.Vieyra@cpfs.mpg.de FU IMPRS-Dresden; U.S. Department of Energy, Basic Energy Sciences, Materials Science and Engineering FX We are grateful to Peter Thalmeier for helpful discussions. H. A. V. acknowledges support by the IMPRS-Dresden. Work at ORNL supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Science and Engineering. NR 32 TC 17 Z9 17 U1 2 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 207001 DI 10.1103/PhysRevLett.106.207001 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200021 PM 21668257 ER PT J AU Zhang, Y Ke, XZ Chen, CF Yang, JH Kent, PRC AF Zhang, Yi Ke, Xuezhi Chen, Changfeng Yang, Jihui Kent, Paul R. C. TI Nanodopant-Induced Band Modulation in AgPbmSbTe2+m-Type Thermoelectrics SO PHYSICAL REVIEW LETTERS LA English DT Article ID SOLID-SOLUTIONS; HIGH FIGURE; MERIT; PBTE; GAPS; SB; BI AB The structure-property relation is a key outstanding problem in the study of nanocomposite materials. Here we elucidate the fundamental physics of nanodopants in thermoelectric nanocomposites XPbmYTe2+m (X = Ag, Na; Y = Sb, Bi). First-principles calculations unveil a sizable band-gap widening driven by nanodopant-induced lattice strain and a band split-off mainly caused by the spin-orbit interaction in nanodopant. Boltzmann transport calculations on PbTe with modified band mimicking nanodopant-induced modulations show significant but competing effects on high-temperature electron transport behavior. These results offer insights for understanding experimental findings and optimizing thermoelectric properties of narrow band-gap semiconductor nanocomposites. C1 [Zhang, Yi; Ke, Xuezhi; Chen, Changfeng] Univ Nevada, Dept Phys, Las Vegas, NV 89154 USA. [Zhang, Yi; Ke, Xuezhi; Chen, Changfeng] Univ Nevada, HiPSEC, Las Vegas, NV 89154 USA. [Ke, Xuezhi] E China Normal Univ, Dept Phys, Shanghai 200062, Peoples R China. [Yang, Jihui] GM RD Ctr, Elect Energy Res Lab, Warren, MI 48090 USA. [Kent, Paul R. C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Zhang, Y (reprint author), Univ Nevada, Dept Phys, Las Vegas, NV 89154 USA. RI Zhang, Yi/C-9291-2011; Yang, Jihui/A-3109-2009; Kent, Paul/A-6756-2008 OI Kent, Paul/0000-0001-5539-4017 FU DOE [DE-FC52-06NA26274, DE-FC26-04NT42278]; GM; DOE Offices of Advanced Scientific Computing Research and Basic Energy Sciences; NSFC [11074074] FX This work was supported by DOE Grants No. DE-FC52-06NA26274, No. DE-FC26-04NT42278, and by GM, and used resources of NCCS and CNMS at ORNL, sponsored by DOE Offices of Advanced Scientific Computing Research and Basic Energy Sciences. X. K. is also supported by NSFC Grant No. 11074074. NR 30 TC 14 Z9 14 U1 0 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2011 VL 106 IS 20 AR 206601 DI 10.1103/PhysRevLett.106.206601 PG 4 WC Physics, Multidisciplinary SC Physics GA 767LX UT WOS:000290859200019 PM 21668249 ER PT J AU Banks, JA Nishiyama, T Hasebe, M Bowman, JL Gribskov, M dePamphilis, C Albert, VA Aono, N Aoyama, T Ambrose, BA Ashton, NW Axtell, MJ Barker, E Barker, MS Bennetzen, JL Bonawitz, ND Chapple, C Cheng, CY Correa, LGG Dacre, M DeBarry, J Dreyer, I Elias, M Engstrom, EM Estelle, M Feng, L Finet, C Floyd, SK Frommer, WB Fujita, T Gramzow, L Gutensohn, M Harholt, J Hattori, M Heyl, A Hirai, T Hiwatashi, Y Ishikawa, M Iwata, M Karol, KG Koehler, B Kolukisaoglu, U Kubo, M Kurata, T Lalonde, S Li, KJ Li, Y Litt, A Lyons, E Manning, G Maruyama, T Michael, TP Mikami, K Miyazaki, S Morinaga, S Murata, T Mueller-Roeber, B Nelson, DR Obara, M Oguri, Y Olmstead, RG Onodera, N Petersen, BL Pils, B Prigge, M Rensing, SA Riano-Pachon, DM Roberts, AW Sato, Y Scheller, HV Schulz, B Schulz, C Shakirov, EV Shibagaki, N Shinohara, N Shippen, DE Sorensen, I Sotooka, R Sugimoto, N Sugita, M Sumikawa, N Tanurdzic, M Theissen, G Ulvskov, P Wakazuki, S Weng, JK Willats, WWGT Wipf, D Wolf, PG Yang, LX Zimmer, AD Zhu, QH Mitros, T Hellsten, U Loque, D Otillar, R Salamov, A Schmutz, J Shapiro, H Lindquist, E Lucas, S Rokhsar, D Grigoriev, IV AF Banks, Jo Ann Nishiyama, Tomoaki Hasebe, Mitsuyasu Bowman, John L. Gribskov, Michael dePamphilis, Claude Albert, Victor A. Aono, Naoki Aoyama, Tsuyoshi Ambrose, Barbara A. Ashton, Neil W. Axtell, Michael J. Barker, Elizabeth Barker, Michael S. Bennetzen, Jeffrey L. Bonawitz, Nicholas D. Chapple, Clint Cheng, Chaoyang Correa, Luiz Gustavo Guedes Dacre, Michael DeBarry, Jeremy Dreyer, Ingo Elias, Marek Engstrom, Eric M. Estelle, Mark Feng, Liang Finet, Cedric Floyd, Sandra K. Frommer, Wolf B. Fujita, Tomomichi Gramzow, Lydia Gutensohn, Michael Harholt, Jesper Hattori, Mitsuru Heyl, Alexander Hirai, Tadayoshi Hiwatashi, Yuji Ishikawa, Masaki Iwata, Mineko Karol, Kenneth G. Koehler, Barbara Kolukisaoglu, Uener Kubo, Minoru Kurata, Tetsuya Lalonde, Sylvie Li, Kejie Li, Ying Litt, Amy Lyons, Eric Manning, Gerard Maruyama, Takeshi Michael, Todd P. Mikami, Koji Miyazaki, Saori Morinaga, Shin-ichi Murata, Takashi Mueller-Roeber, Bernd Nelson, David R. Obara, Mari Oguri, Yasuko Olmstead, Richard G. Onodera, Naoko Petersen, Bent Larsen Pils, Birgit Prigge, Michael Rensing, Stefan A. Mauricio Riano-Pachon, Diego Roberts, Alison W. Sato, Yoshikatsu Scheller, Henrik Vibe Schulz, Burkhard Schulz, Christian Shakirov, Eugene V. Shibagaki, Nakako Shinohara, Naoki Shippen, Dorothy E. Sorensen, Iben Sotooka, Ryo Sugimoto, Nagisa Sugita, Mamoru Sumikawa, Naomi Tanurdzic, Milos Theissen, Guenter Ulvskov, Peter Wakazuki, Sachiko Weng, Jing-Ke Willats, William W. G. T. Wipf, Daniel Wolf, Paul G. Yang, Lixing Zimmer, Andreas D. Zhu, Qihui Mitros, Therese Hellsten, Uffe Loque, Dominique Otillar, Robert Salamov, Asaf Schmutz, Jeremy Shapiro, Harris Lindquist, Erika Lucas, Susan Rokhsar, Daniel Grigoriev, Igor V. TI The Selaginella Genome Identifies Genetic Changes Associated with the Evolution of Vascular Plants SO SCIENCE LA English DT Article ID SMALL RNAS; MESSENGER-RNAS; ARABIDOPSIS; MOELLENDORFFII; MECHANISM; LAND; PERSPECTIVE; SIRNAS AB Vascular plants appeared similar to 410 million years ago, then diverged into several lineages of which only two survive: the euphyllophytes (ferns and seed plants) and the lycophytes. We report here the genome sequence of the lycophyte Selaginella moellendorffii (Selaginella), the first nonseed vascular plant genome reported. By comparing gene content in evolutionarily diverse taxa, we found that the transition from a gametophyte- to a sporophyte-dominated life cycle required far fewer new genes than the transition from a nonseed vascular to a flowering plant, whereas secondary metabolic genes expanded extensively and in parallel in the lycophyte and angiosperm lineages. Selaginella differs in posttranscriptional gene regulation, including small RNA regulation of repetitive elements, an absence of the trans-acting small interfering RNA pathway, and extensive RNA editing of organellar genes. C1 [Banks, Jo Ann] Purdue Univ, Dept Bot & Plant Pathol, W Lafayette, IN 47907 USA. [Nishiyama, Tomoaki] Kanazawa Univ, Adv Sci Res Ctr, Kanazawa, Ishikawa 9200934, Japan. [Nishiyama, Tomoaki; Hasebe, Mitsuyasu; Cheng, Chaoyang; Hirai, Tadayoshi; Ishikawa, Masaki; Iwata, Mineko; Kubo, Minoru; Kurata, Tetsuya; Obara, Mari; Oguri, Yasuko; Onodera, Naoko; Sato, Yoshikatsu; Shinohara, Naoki; Sugimoto, Nagisa; Wakazuki, Sachiko] Japan Sci & Technol Agcy, ERATO, Okazaki, Aichi 4448585, Japan. [Hasebe, Mitsuyasu; Aono, Naoki; Aoyama, Tsuyoshi; Hiwatashi, Yuji; Miyazaki, Saori; Morinaga, Shin-ichi; Murata, Takashi; Sumikawa, Naomi] Natl Inst Nat Sci, Natl Inst Basic Biol, Okazaki, Aichi 4448585, Japan. [Hasebe, Mitsuyasu; Aoyama, Tsuyoshi; Hiwatashi, Yuji; Murata, Takashi] Grad Univ Adv Studies, Sch Life Sci, Dept Basic Sci, Okazaki, Aichi 4448585, Japan. [Bowman, John L.; Floyd, Sandra K.] Monash Univ, Sch Biol Sci, Melbourne, Vic 3800, Australia. [Bowman, John L.] Univ Calif Davis, Plant Biol Sect, Davis, CA 95616 USA. [Gribskov, Michael; Li, Kejie; Li, Ying] Purdue Univ, Dept Biol Sci, W Lafayette, IN 47907 USA. [dePamphilis, Claude; Axtell, Michael J.] Penn State Univ, Dept Biol, University Pk, PA 16802 USA. [dePamphilis, Claude; Axtell, Michael J.] Penn State Univ, Huck Inst Life Sci, University Pk, PA 16802 USA. [dePamphilis, Claude] Penn State Univ, Grad Program Plant Biol, University Pk, PA 16802 USA. [dePamphilis, Claude] Penn State Univ, Inst Mol Evolutionary Genet, University Pk, PA 16802 USA. [Albert, Victor A.] SUNY Buffalo, Dept Biol Sci, Buffalo, NY 14260 USA. [Ambrose, Barbara A.; Karol, Kenneth G.; Litt, Amy] New York Bot Garden, Bronx, NY 10458 USA. [Ashton, Neil W.; Barker, Elizabeth] Univ Regina, Dept Biol, Regina, SK S4S 0A2, Canada. [Barker, Michael S.] Univ Arizona, Dept Ecol & Evolutionary Biol, Tucson, AZ 85721 USA. [Bennetzen, Jeffrey L.; DeBarry, Jeremy; Yang, Lixing; Zhu, Qihui] Univ Georgia, Dept Genet, Athens, GA 30602 USA. [Bonawitz, Nicholas D.; Chapple, Clint; Weng, Jing-Ke] Purdue Univ, Dept Biochem, W Lafayette, IN 47907 USA. [Correa, Luiz Gustavo Guedes; Koehler, Barbara] Univ Potsdam, Dept Mol Biol, D-14476 Potsdam, Germany. [Dacre, Michael; Manning, Gerard] Salk Inst Biol Studies, Razavi Newman Ctr Bioinformat, La Jolla, CA 92037 USA. [Dreyer, Ingo] Univ Potsdam, Heisenberg Grp Biophys & Mol Plant Biol, D-14476 Potsdam, Germany. [Elias, Marek] Charles Univ Prague, Dept Bot, Fac Sci, Prague 12801 2, Czech Republic. [Elias, Marek] Univ Prague, Fac Sci, Ostrava 71000, Czech Republic. [Engstrom, Eric M.] Coll William & Mary, Dept Biol, Williamsburg, VA 23187 USA. [Estelle, Mark; Prigge, Michael] Univ Calif San Diego, Sect Cell & Dev Biol, La Jolla, CA 92093 USA. [Feng, Liang] Univ Georgia, Inst Bioinformat, Athens, GA 30602 USA. [Finet, Cedric] Ecole Normale Super Lyon, Lab Reprod & Dev Plantes, F-69364 Lyon, France. [Frommer, Wolf B.; Lalonde, Sylvie] Carnegie Inst Sci, Dept Plant Biol, Stanford, CA 94305 USA. [Fujita, Tomomichi] Hokkaido Univ, Fac Sci, Sapporo, Hokkaido 0600810, Japan. [Gramzow, Lydia; Theissen, Guenter] Univ Jena, Dept Genet, D-07743 Jena, Germany. [Gutensohn, Michael; Schulz, Burkhard] Purdue Univ, Dept Hort & Landscape Architecture, W Lafayette, IN 47907 USA. [Gutensohn, Michael] Univ Halle Wittenberg, Inst Biol, D-06120 Halle, Germany. [Harholt, Jesper; Petersen, Bent Larsen; Sorensen, Iben; Ulvskov, Peter; Willats, William W. G. T.] Univ Copenhagen, Dept Plant Biol & Biotechnol, DK-1871 Frederiksberg C, Denmark. [Hattori, Mitsuru; Sugita, Mamoru] Nagoya Univ, Ctr Gene Res, Nagoya, Aichi 4648602, Japan. [Hattori, Mitsuru] Univ Tokyo, Sch Sci, Dept Chem, Bunkyo Ku, Tokyo 1130033, Japan. [Heyl, Alexander] Free Univ Berlin, Dahlem Ctr Plant Sci, Inst Biol Appl Genet, D-14195 Berlin, Germany. [Hirai, Tadayoshi] Univ Tsukuba, Ctr Gene Res, Grad Sch Life & Environm Sci, Tsukuba, Ibaraki 3058572, Japan. [Kolukisaoglu, Uener] Univ Rostock, Ctr Life Sci Automat, D-18119 Rostock, Germany. [Kolukisaoglu, Uener] Univ Tubingen, Studiengangskoordinat Nanosci, D-72076 Tubingen, Germany. [Kurata, Tetsuya] Nara Inst Sci & Technol, Grad Sch Biol Sci, Plant Global Educ Project, Nara 6300192, Japan. [Li, Ying] Mayo Clin, Div Biomed Stat & Informat, Rochester, MN 55905 USA. [Lyons, Eric; Scheller, Henrik Vibe] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Maruyama, Takeshi] Hokkaido Univ, Grad Sch Life Sci, Sapporo, Hokkaido 0600810, Japan. [Michael, Todd P.] Rutgers State Univ, Dept Plant Biol & Pathol, Piscataway, NJ 08854 USA. [Michael, Todd P.] Waksman Inst Microbiol, Piscataway, NJ 08854 USA. [Michael, Todd P.] Monsanto Co, Genome Anal Ctr, St Louis, MO 63167 USA. [Mikami, Koji] Hokkaido Univ, Fac Fisheries Sci, Hakodate, Hokkaido 0418611, Japan. [Miyazaki, Saori] Natl Inst Genet, Mishima, Shizuoka 4118540, Japan. [Morinaga, Shin-ichi] Univ Tokyo, Grad Sch Arts & Sci, Tokyo 1538902, Japan. [Mueller-Roeber, Bernd] Bernd Max Planck Inst Mol Plant Physiol, D-14476 Potsdam, Germany. [Nelson, David R.] Univ Tennessee, Dept Microbiol Immunol & Biochem, Memphis, TN 38163 USA. [Obara, Mari] Japan Sci & Technol Agcy, Sapporo, Hokkaido 0600819, Japan. [Olmstead, Richard G.] Univ Washington, Dept Biol, Seattle, WA 98195 USA. [Onodera, Naoko] Dalhousie Univ, Dept Biochem & Mol Biol, Halifax, NS B3H 4R2, Canada. [Pils, Birgit] Wellcome Trust Ctr Human Genet, Oxford OX3 7BN, England. [Pils, Birgit] Sias AG, CH-8634 Hombrechtikon, Switzerland. [Rensing, Stefan A.; Zimmer, Andreas D.] Univ Freiburg, Fac Biol, D-79104 Freiburg, Germany. [Rensing, Stefan A.] Univ Freiburg, BIOSS Ctr Biol Signaling Studies, D-79104 Freiburg, Germany. [Rensing, Stefan A.] Univ Freiburg, Freiburg Initiat Syst Biol FRISYS, D-79104 Freiburg, Germany. [Mauricio Riano-Pachon, Diego] Max Planck Inst Mol Plant Physiol, Bioinformat Grp, GabiPD Team, D-14476 Potsdam, Germany. [Mauricio Riano-Pachon, Diego] Univ Los Andes, Dept Ciencias Biol, Bogota, Colombia. [Roberts, Alison W.] Univ Rhode Isl, Dept Biol Sci, Kingston, RI 02881 USA. [Scheller, Henrik Vibe; Loque, Dominique] Joint BioEnergy Inst, Feedstocks Div, Emeryville, CA 94608 USA. [Schulz, Christian] Ruhr Univ Bochum, Dept Evolut & Biodivers Plants, D-44780 Bochum, Germany. [Shakirov, Eugene V.; Shippen, Dorothy E.] Texas A&M Univ, Dept Biochem & Biophys, College Stn, TX 77843 USA. [Shibagaki, Nakako] Osaka Univ, Grad Sch Engn, Suita, Osaka 5650871, Japan. [Shinohara, Naoki; Sotooka, Ryo] Hokkaido Univ, Sch Sci, Sapporo, Hokkaido 0600810, Japan. [Sorensen, Iben] Cornell Univ, Dept Plant Biol, Ithaca, NY 14850 USA. [Tanurdzic, Milos] Cold Spring Harbor Lab, Cold Spring Harbor, NY 11724 USA. [Weng, Jing-Ke] Salk Inst Biol Studies, Jack H Skirball Ctr Chem Biol & Prote, La Jolla, CA 92037 USA. [Wipf, Daniel] Univ Bourgogne, INRA, UMR 1088, CNRS 5184, F-21065 Dijon, France. [Wolf, Paul G.] Utah State Univ, Dept Biol, Logan, UT 84322 USA. [Mitros, Therese; Rokhsar, Daniel] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Hellsten, Uffe; Otillar, Robert; Salamov, Asaf; Schmutz, Jeremy; Shapiro, Harris; Lindquist, Erika; Lucas, Susan; Rokhsar, Daniel; Grigoriev, Igor V.] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. RP Banks, JA (reprint author), Purdue Univ, Dept Bot & Plant Pathol, W Lafayette, IN 47907 USA. EM banksj@purdue.edu RI dePamphilis, Claude/P-6652-2016; Schmutz, Jeremy/N-3173-2013; Elias, Marek/D-6851-2014; Petersen, Bent/H-9437-2014; Ulvskov, Peter/I-1228-2014; Feng, Liang/I-5010-2014; Kolukisaoglu, Uener/J-8831-2014; Harholt, Jesper/F-6865-2014; Weng, Jing-Ke/A-6900-2015; Sato, Yoshikatsu/I-6129-2014; Loque, Dominique/A-8153-2008; Wolf, Paul/F-7664-2010; Dreyer, Ingo/N-4747-2014; Riano-Pachon, Diego/A-1755-2010; Dacre, Michael/C-1131-2008; Harholt, Jesper/F-3760-2011; Shakirov, Eugene/A-1363-2012; Tanurdzic, Milos/A-5712-2012; Mikami, Koji/A-9825-2012; Weng, Jing-Ke/E-7343-2013; Zhu, Qihui/N-2625-2013; Frommer, Wolf B/A-8256-2008; Ye, Mingli/G-4909-2012; Yang, Lixing/A-7073-2013; Li, Kejie/D-3595-2013 OI Nelson, David/0000-0003-0583-5421; Willats, William/0000-0003-2064-4025; Prigge, Michael/0000-0003-0671-2538; Scheller, Henrik/0000-0002-6702-3560; Nishiyama, Tomoaki/0000-0003-1279-7806; Bowman, John/0000-0001-7347-3691; Barker, Michael/0000-0001-7173-1319; Michael, Todd/0000-0001-6272-2875; DeBarry, Jeremy/0000-0001-5718-2675; Tanurdzic, Milos/0000-0002-7564-0868; Manning, Gerard/0000-0002-5087-9151; Gribskov, Michael/0000-0002-1718-0242; HIWATASHI, YUJI/0000-0002-3996-0549; Schmutz, Jeremy/0000-0001-8062-9172; Elias, Marek/0000-0003-0066-6542; Petersen, Bent/0000-0002-2004-9077; Ulvskov, Peter/0000-0003-3776-818X; Kolukisaoglu, Uener/0000-0002-8656-5963; Harholt, Jesper/0000-0002-7984-0066; Weng, Jing-Ke/0000-0003-3059-0075; Wolf, Paul/0000-0002-4317-6976; Riano-Pachon, Diego/0000-0001-9803-3465; Dacre, Michael/0000-0002-5561-1656; Shakirov, Eugene/0000-0003-2689-7410; Weng, Jing-Ke/0000-0003-1079-3668; FU Office of Science of the U.S. DOE [DE-AC02-05CH11231]; NSF [0844413, 0515435, 0519970, 0638595, 0922742, 1020443, 0607123, 0744800, 1020660, 1036466, 0735191, 0228660, 0421604]; Japan Society for the Promotion of Science; Ministry of Education, Culture, Sports, Science, and Technology, Japan; Australian Research Council [FF0561326]; Lewis B and Dorothy Cullman Program; Natural Sciences and Engineering Research Council of Canada (NSERC) [2982]; NIH [GM84051, T32 GM007757, T32-HG00035, GM065383]; Life Sciences Research Foundation; National Human Genome Research Institute (NHGRI) [HG004164]; German Science Foundation (Deutsche Forschungsgemeinschaft, DFG) [DR 430/4-2]; Czech Ministry of Education [21620828]; Jeffress Memorial Trust [J-938]; DOE [DE-FG02-04ER15542]; Danish Council for Independent Research, Technology and Production Sciences [009-066624/274-09-0314]; Villum Kann Rasmussen Foundation; U.S. Department of Agriculture (USDA) [DE-FG02-08ER64630]; Danish Council for Strategic Research [09-063090]; Marie Curie FP6 RTN ZOONET; DFG [RE 837/10-2, BMBF FRISYS 0313921]; Bundesministerium fuer Bildung und Forschung, Germany [0315046]; USDA NRI [2007-35318-18389]; Burgundy Regional Council [20100112095254682-1] FX Selaginella sequences were deposited at GenBank with the accession numbers GL377566 to GL378322.1 and HM173080. Genome sequencing and analysis were performed by the U.S. Department of Energy (DOE), Joint Genome Institute, supported by the Office of Science of the U.S. DOE, Contract DE-AC02-05CH11231 (I.V.G., U.H., D.L., E.L., S.L., T.M., R.O., D.R., A.S., J.S., H.V.S.). Support was provided by NSF 0844413 (J.A.B.); Japan Society for the Promotion of Science (M.H., T.N., T.F., K.M., T.M., M.S.); Ministry of Education, Culture, Sports, Science, and Technology, Japan (M.H., T.N., T.F.); NSF 0515435 and Australian Research Council FF0561326 (J.L.B.); NSF 0519970 (M.G.); NSF 0638595 (C.D.); NSF 0922742 (V.A.A.); The Lewis B and Dorothy Cullman Program (B.A.A., A.L.); NSF 1020443 (B.A.A.); Natural Sciences and Engineering Research Council of Canada (NSERC) 2982 (N.W.A.); NIH GM84051 (M.J.A.); NSERC (E.I.B.); NIH T32 GM007757 and NSERC PGS-D (M.S.B.); NSF 0607123 (J.L.B.); Life Sciences Research Foundation (NDB); National Human Genome Research Institute (NHGRI) HG004164 (M.D.); German Science Foundation (Deutsche Forschungsgemeinschaft, DFG) DR 430/4-2 (I.D.); Czech Ministry of Education 21620828 (M.E.); Jeffress Memorial Trust J-938 (E.M.E.); NSF 0744800 (M.E. and M.P.); DOE DE-FG02-04ER15542 (W.B.F. and S.L.); The Danish Council for Independent Research, Technology and Production Sciences 009-066624/274-09-0314 (J.H.); The Villum Kann Rasmussen Foundation (J.H., I.S., B.P., P.U., W.W.); NIH T32-HG00035, NSF 1020660, and NSF 1036466 (K.G.K.); NSF 0735191 (E.L.); NHGRI HG004164 (G.M); U.S. Department of Agriculture (USDA) DE-FG02-08ER64630 (T.P.M.); NSF 0228660 (R.G.O.); The Danish Council for Strategic Research 09-063090 (B.L.P. and P.U.); Marie Curie FP6 RTN ZOONET (B.P.); DFG RE 837/10-2, BMBF FRISYS 0313921 (S.A.R.); Bundesministerium fuer Bildung und Forschung, Germany, GABI-FUTURE grant 0315046 (D.M.R.); USDA NRI 2007-35318-18389 (A.W.R.); NSF 0421604 (C.S.); NIH GM065383 (D.E.S.); Burgundy Regional Council 20100112095254682-1 (D.W.); and DFG RE 837/10-2 (A.D.Z.). K. Wall, D. Hurley, and S. Hentel provided computational assistance. NR 25 TC 297 Z9 348 U1 18 U2 161 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 J9 SCIENCE JI Science PD MAY 20 PY 2011 VL 332 IS 6032 BP 960 EP 963 DI 10.1126/science.1203810 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 766FO UT WOS:000290766600042 PM 21551031 ER PT J AU Dunkle, JA Wang, LY Feldman, MB Pulk, A Chen, VB Kapral, GJ Noeske, J Richardson, JS Blanchard, SC Cate, JHD AF Dunkle, Jack A. Wang, Leyi Feldman, Michael B. Pulk, Arto Chen, Vincent B. Kapral, Gary J. Noeske, Jonas Richardson, Jane S. Blanchard, Scott C. Cate, Jamie H. Doudna TI Structures of the Bacterial Ribosome in Classical and Hybrid States of tRNA Binding SO SCIENCE LA English DT Article ID AMINOACYL-TRANSFER-RNA; CRYSTAL-STRUCTURE; RECYCLING FACTOR; 70S RIBOSOME; CRYO-EM; INTERMEDIATE STATES; TRANSLATION FACTORS; MESSENGER-RNA; TRANSLOCATION; DYNAMICS AB During protein synthesis, the ribosome controls the movement of tRNA and mRNA by means of large-scale structural rearrangements. We describe structures of the intact bacterial ribosome from Escherichia coli that reveal how the ribosome binds tRNA in two functionally distinct states, determined to a resolution of similar to 3.2 angstroms by means of x-ray crystallography. One state positions tRNA in the peptidyl-tRNA binding site. The second, a fully rotated state, is stabilized by ribosome recycling factor and binds tRNA in a highly bent conformation in a hybrid peptidyl/exit site. The structures help to explain how the ratchet-like motion of the two ribosomal subunits contributes to the mechanisms of translocation, termination, and ribosome recycling. C1 [Dunkle, Jack A.; Pulk, Arto; Noeske, Jonas; Cate, Jamie H. Doudna] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Dunkle, Jack A.; Pulk, Arto; Noeske, Jonas; Cate, Jamie H. Doudna] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Wang, Leyi; Feldman, Michael B.; Blanchard, Scott C.] Cornell Univ, Weill Cornell Med Coll, Dept Physiol & Biophys, New York, NY 10065 USA. [Feldman, Michael B.] Weill Cornell Rockefeller Univ Sloan Kettering Tr, New York, NY 10065 USA. [Chen, Vincent B.; Kapral, Gary J.; Richardson, Jane S.] Duke Univ, Med Ctr, Dept Biochem, Durham, NC 27710 USA. [Cate, Jamie H. Doudna] Univ Calif Berkeley, Lawrence Berkeley Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Cate, JHD (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. EM jcate@lbl.gov RI Blanchard, Scott/A-5804-2009; OI Pulk, Arto/0000-0001-8793-3038 FU National Institutes of Health [GM65050, GM079238, GM074127-04S1, GM088674, P01-GM63210, GM07739]; National Cancer Institute [CA92584]; National Center for Research Resources [RR-15301]; U.S. Department of Energy [DE-AC03 76SF00098, DE-AC02-06CH11357]; Human Frontiers in Science Program FX We thank K. Hamadani for purified RRF; K. Nierhaus for tRNAPhe overexpression plasmids; K. Frankel, S. Classen, and G. Meigs for help with data measurement at the SIBYLS and 8.3.1 beamlines at the Advanced Light Source (ALS); R. Kanagalaghatta, D. Neau, F. Murphy, and I. Kourinov for help with data measurement at ID-24 at the Advanced Photon Source (APS); J. Headd for help with Phenix refinement; and J. Holton for useful crystallographic discussions. We also thank J. Doudna and H. Noller for helpful comments on the manuscript. Atomic coordinates and structure factors are deposited in the Protein Data Bank (accession codes 3R8N and 3R8S for the fully rotated state RF, 3R8O and 3R8T for the unrotated state R0). This work was funded by the National Institutes of Health (GM65050 to J.H.D.C., GM079238 to S.C.B, and GM074127-04S1, GM088674, and P01-GM63210 project IV to J. S. R.), National Cancer Institute grant CA92584 for the SIBYLS and 8.3.1 beam lines at the ALS, and National Center for Research Resources grant RR-15301 for the Northeastern Collaborative Access Team beam lines at 24-ID at APS, and by the U.S. Department of Energy (DE-AC03 76SF00098 for the SIBYLS and 8.3.1 beamlines at the ALS, and DE-AC02-06CH11357 for the APS). M.B.F. is a trainee in the Weill Cornell/Rockefeller University/SloanKettering Tri-Institutional MD-PhD Program supported by NIH Medical Scientist Training Program grant GM07739. J.N. is supported by a Human Frontiers in Science Program Postdoctoral Fellowship. NR 47 TC 177 Z9 179 U1 2 U2 19 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 J9 SCIENCE JI Science PD MAY 20 PY 2011 VL 332 IS 6032 BP 981 EP 984 DI 10.1126/science.1202692 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 766FO UT WOS:000290766600048 PM 21596992 ER PT J AU Barman, TS Macintosh, B Konopacky, QM Marois, C AF Barman, Travis S. Macintosh, Bruce Konopacky, Quinn M. Marois, Christian TI CLOUDS AND CHEMISTRY IN THE ATMOSPHERE OF EXTRASOLAR PLANET HR8799b SO ASTROPHYSICAL JOURNAL LA English DT Article DE brown dwarfs; planetary systems; stars: atmospheres; stars: low-mass ID INTEGRAL FIELD SPECTROGRAPH; BROWN DWARF ATMOSPHERES; STAR ADAPTIVE OPTICS; ORBITING HR 8799; BINARY T DWARF; MODEL ATMOSPHERES; ULTRACOOL DWARFS; CARBON-MONOXIDE; MU-M; INFRARED-SPECTROSCOPY AB Using the integral field spectrograph OSIRIS, on the Keck II telescope, broad near-infrared H- and K-band spectra of the young exoplanet HR8799b have been obtained. In addition, six new narrowband photometric measurements have been taken across the H and K bands. These data are combined with previously published photometry for an analysis of the planet's atmospheric properties. Thick photospheric dust cloud opacity is invoked to explain the planet's red near-IR colors and relatively smooth near-IR spectrum. Strong water absorption is detected, indicating a hydrogen-rich atmosphere. Only weak CH4 absorption is detected at K band, indicating efficient vertical mixing and a disequilibrium CO/CH4 ratio at photospheric depths. The H-band spectrum has a distinct triangular shape consistent with low surface gravity. New giant planet atmosphere models are compared to these data with best-fitting bulk parameters, T-eff = 1100 K +/- 100 and log(g) = 3.5 +/- 0.5 (for solar composition). Given the observed luminosity (log L-obs/L-circle dot similar to -5.1), these values correspond to a radius of 0.75 R-Jup-0.12(+0.17) and a mass of similar to 0.72 M-Jup-0.6(+2.6)-strikingly inconsistent with interior/evolution models. Enhanced metallicity (up to similar to 10x that of the Sun) along with thick clouds and non-equilibrium chemistry are likely required to reproduce the complete ensemble of spectroscopic and photometric data and the low effective temperatures (< 1000 K) required by the evolution models. C1 [Barman, Travis S.] Lowell Observ, Flagstaff, AZ 86001 USA. [Macintosh, Bruce; Konopacky, Quinn M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Marois, Christian] Natl Res Council Canada, Herzberg Inst Astrophys, Victoria, BC V9E 2E7, Canada. RP Barman, TS (reprint author), Lowell Observ, 1400 W Mars Hill Rd, Flagstaff, AZ 86001 USA. EM barman@lowell.edu FU W.M. Keck Foundation; NSF; National Science Foundation (United States); Science and Technology Facilities Council (United Kingdom); National Research Council (Canada); CONICYT (Chile); Australian Research Council (Australia); Ministerio da Ciencia e Tecnologia (Brazil); Ministerio de Ciencia; Tecnologia e Innovacion Productiva (Argentina); NASA; U.S. Department of Energy, Lawrence Livermore National Laboratory [DE-AC52-07NA27344 (LLNL-JRNL-476433)] FX We thank the referee, Jonathan Fortney, for his careful review of our paper. Additional thanks go out to Shelley Wright, Jim Lyke, and James Larkin for their assistance with all things OSIRIS-related. We also thank Brad Hansen, Mark Marley, Didier Saumon, and Tristan Guillot for many useful discussions on the vagaries of planets and brown dwarfs. We are indebted to Jim Lyke, Al Conrad, Hien Tran, Scott Dahm, Randy Campbell, Terry Stickel, and the entire Keck staff for their assistance in maximizing our observing efficiency. T.B. acknowledges the Kavli Institute for Theoretical Physics and the participants of the 2010 workshop on Exoplanets for providing a stimulating environment. This research has benefited from the SpeX Prism Spectral Libraries, maintained by Adam Burgasser. The data presented herein were obtained at the W.M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California and the National Aeronautics and Space Administration. The Observatory was made possible by the generous financial support of the W.M. Keck Foundation. The authors wish to recognize and acknowledge the very significant cultural role and reverence that the summit of Mauna Kea has always had within the indigenous Hawaiian community. We are most fortunate to have the opportunity to conduct observations from this mountain. Observations were also obtained at the Gemini Observatory, which is operated by the Association of Universities for Research in Astronomy, Inc., under a cooperative agreement with the NSF on behalf of the Gemini partnership: the National Science Foundation (United States), the Science and Technology Facilities Council (United Kingdom), the National Research Council (Canada), CONICYT (Chile), the Australian Research Council (Australia), Ministerio da Ciencia e Tecnologia (Brazil) and Ministerio de Ciencia, Tecnologia e Innovacion Productiva (Argentina). Most of the numerical work was carried out at the NASA Advanced Supercomputing facilities. This research was supported by NASA Origins of Solar Systems grants to LLNL and Lowell Observatory. This research was also supported by JPL/NexSci RSA awards. Portions of this work were performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 (LLNL-JRNL-476433). We thank all these institutions for their support. NR 91 TC 141 Z9 141 U1 0 U2 9 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X J9 ASTROPHYS J JI Astrophys. J. PD MAY 20 PY 2011 VL 733 IS 1 AR 65 DI 10.1088/0004-637X/733/1/65 PG 18 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 760HE UT WOS:000290314600065 ER PT J AU Childress, M Aldering, G Aragon, C Antilogus, P Bailey, S Baltay, C Bongard, S Buton, C Canto, A Chotard, N Copin, Y Fakhouri, HK Gangler, E Kerschhaggl, M Kowalski, M Hsiao, EY Loken, S Nugent, P Paech, K Pain, R Pecontal, E Pereira, R Perlmutter, S Rabinowitz, D Runge, K Scalzo, R Thomas, RC Smadja, G Tao, C Weaver, BA Wu, C AF Childress, M. Aldering, G. Aragon, C. Antilogus, P. Bailey, S. Baltay, C. Bongard, S. Buton, C. Canto, A. Chotard, N. Copin, Y. Fakhouri, H. K. Gangler, E. Kerschhaggl, M. Kowalski, M. Hsiao, E. Y. Loken, S. Nugent, P. Paech, K. Pain, R. Pecontal, E. Pereira, R. Perlmutter, S. Rabinowitz, D. Runge, K. Scalzo, R. Thomas, R. C. Smadja, G. Tao, C. Weaver, B. A. Wu, C. TI KECK OBSERVATIONS OF THE YOUNG METAL-POOR HOST GALAXY OF THE SUPER-CHANDRASEKHAR-MASS TYPE Ia SUPERNOVA SN 2007if SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: dwarf; supernovae: general; supernovae: individual (SN 2007if) ID DIGITAL SKY SURVEY; STELLAR POPULATION SYNTHESIS; COMPACT DWARF GALAXIES; STAR-FORMING GALAXIES; TO-LIGHT RATIOS; METALLICITY RELATION; FACTORY OBSERVATIONS; LUMINOSITY FUNCTION; FORMATION RATES; DATA RELEASE AB We present Keck LRIS spectroscopy and g-band photometry of the metal-poor, low-luminosity host galaxy of the super-Chandrasekhar-mass Type Ia supernova SN 2007if. Deep imaging of the host reveals its apparent magnitude to be m(g) = 23.15 +/- 0.06, which at the spectroscopically measured redshift of z(helio) = 0.07450 +/- 0.00015 corresponds to an absolute magnitude of M-g = -14.45 +/- 0.06. Galaxy g - r color constrains the mass-to-light ratio, giving a host stellar mass estimate of log(M-*/M-circle dot) = 7.32 +/- 0.17. Balmer absorption in the stellar continuum, along with the strength of the 4000 angstrom break, constrains the age of the dominant starburst in the galaxy to be t(burst) = 123(-77)(+165) Myr, corresponding to a main-sequence turnoff mass of M/M-circle dot = 4.6(-1.4)(+2.6). Using the R-23 method of calculating metallicity from the fluxes of strong emission lines, we determine the host oxygen abundance to be 12 + log(O/H)(KK04) = 8.01 +/- 0.09, significantly lower than any previously reported spectroscopically measured Type Ia supernova host galaxy metallicity. Our data show that SN 2007if is very likely to have originated from a young, metal-poor progenitor. C1 [Childress, M.; Aldering, G.; Aragon, C.; Bailey, S.; Fakhouri, H. K.; Hsiao, E. Y.; Loken, S.; Perlmutter, S.; Runge, K.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Phys, Berkeley, CA 94720 USA. [Childress, M.; Fakhouri, H. K.; Perlmutter, S.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Antilogus, P.; Bongard, S.; Canto, A.; Pain, R.; Wu, C.] Univ Paris 07, Univ Paris 06, Lab Phys Nucl & Hautes Energies, CNRS IN2P3, F-75252 Paris 05, France. [Baltay, C.; Rabinowitz, D.; Scalzo, R.] Yale Univ, Dept Phys, New Haven, CT 06250 USA. [Buton, C.; Kerschhaggl, M.; Kowalski, M.; Paech, K.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Chotard, N.; Copin, Y.; Gangler, E.; Pereira, R.; Smadja, G.] Univ Lyon, F-69622 Villeurbanne, France. [Chotard, N.; Copin, Y.; Gangler, E.; Pereira, R.; Smadja, G.] Univ Lyon 1, F-69622 Villeurbanne, France. [Chotard, N.; Copin, Y.; Gangler, E.; Pereira, R.; Smadja, G.] CNRS, IN2P3, Inst Phys Nucl Lyon, F-75700 Paris, France. [Nugent, P.; Thomas, R. C.] Lawrence Berkeley Natl Lab, Computat Res Div, Computat Cosmol Ctr, Berkeley, CA 94611 USA. [Pecontal, E.] Univ Lyon 1, Ctr Rech Astron Lyon, F-69561 St Genis Laval, France. [Scalzo, R.] Australian Natl Univ, Mt Stromlo Observ, Res Sch Astron & Astrophys, Weston, ACT 2611, Australia. [Tao, C.] Ctr Phys Particules Marseille, F-13288 Marseille 09, France. [Tao, C.] Tsinghua Univ, Tsinghua Ctr Astrophys, Beijing 100084, Peoples R China. [Weaver, B. A.] NYU, Ctr Cosmol & Particle Phys, New York, NY 10003 USA. RP Childress, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Phys, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM mjchildress@lbl.gov RI Kowalski, Marek/G-5546-2012; Copin, Yannick/B-4928-2015; Perlmutter, Saul/I-3505-2015; OI Copin, Yannick/0000-0002-5317-7518; Perlmutter, Saul/0000-0002-4436-4661; Scalzo, Richard/0000-0003-3740-1214 FU Office of Science, Office of High Energy Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; Gordon & Betty Moore Foundation; CNRS/IN2P3; CNRS/INSU; PNC; National Natural Science Foundation of China [10903010]; National Science Foundation [ANI-0087344]; University of California, San Diego FX This work was supported by the Director, Office of Science, Office of High Energy Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, by a grant from the Gordon & Betty Moore Foundation, and in France by support from CNRS/IN2P3, CNRS/INSU, and PNC. C. W. acknowledges support from the National Natural Science Foundation of China grant 10903010. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Director, Office of Science, Office of Advanced Scientific Computing Research, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We thank them for a generous allocation of storage and computing time. HPWREN is funded by National Science Foundation Grant Number ANI-0087344, and the University of California, San Diego. NR 106 TC 13 Z9 13 U1 0 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X J9 ASTROPHYS J JI Astrophys. J. PD MAY 20 PY 2011 VL 733 IS 1 AR 3 DI 10.1088/0004-637X/733/1/3 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 760HE UT WOS:000290314600003 ER PT J AU Pai, AP Lara, P Pan, C Hillegonds, D AF Pai, A. P. Lara, P. Pan, C. Hillegonds, D. TI Direct measurement of calcium metabolism in patients with castration-resistant prostate cancer using a novel isotope tracing approach in urine. SO JOURNAL OF CLINICAL ONCOLOGY LA English DT Meeting Abstract C1 Univ Calif Davis, Med Ctr, Sacramento, CA 95817 USA. Univ Calif Davis, Sacramento, CA 95817 USA. Lawrence Livermore Natl Lab, Livermore, CA USA. NR 0 TC 0 Z9 0 U1 0 U2 1 PU AMER SOC CLINICAL ONCOLOGY PI ALEXANDRIA PA 2318 MILL ROAD, STE 800, ALEXANDRIA, VA 22314 USA SN 0732-183X EI 1527-7755 J9 J CLIN ONCOL JI J. Clin. Oncol. PD MAY 20 PY 2011 VL 29 IS 15 SU S MA e15083 PG 1 WC Oncology SC Oncology GA V31JQ UT WOS:000208880303786 PM 28020431 ER PT J AU Pan, C Wang, S White, RD Gandara, DR Lara, P Li, T Mack, P Rodriguez-Fahrni, A Lee, JS Malfatti, M Turteltaub, K Henderson, PT AF Pan, C. Wang, S. White, R. deVere Gandara, D. R. Lara, P. Li, T. Mack, P. Rodriguez-Fahrni, A. Lee, J. S. Malfatti, M. Turteltaub, K. Henderson, P. T. TI A phase 0 microdosing trial of an in vivo assay for predicting chemoresistance to platinum. SO JOURNAL OF CLINICAL ONCOLOGY LA English DT Meeting Abstract C1 Univ Calif Davis, Sacramento, CA 95817 USA. Lawrence Livermore Natl Lab, Livermore, CA USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU AMER SOC CLINICAL ONCOLOGY PI ALEXANDRIA PA 2318 MILL ROAD, STE 800, ALEXANDRIA, VA 22314 USA SN 0732-183X EI 1527-7755 J9 J CLIN ONCOL JI J. Clin. Oncol. PD MAY 20 PY 2011 VL 29 IS 15 SU S MA 2578 PG 1 WC Oncology SC Oncology GA V31JQ UT WOS:000208880301393 PM 28022281 ER PT J AU Leitner, T AF Leitner, Thomas TI Guidelines for HIV in court cases SO NATURE LA English DT Letter C1 Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Leitner, T (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM tkl@lanl.gov RI Brown, Jeremy/B-4544-2010 OI Brown, Jeremy/0000-0002-1447-8633 FU NIAID NIH HHS [R01 AI087520] NR 0 TC 3 Z9 3 U1 0 U2 2 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 J9 NATURE JI Nature PD MAY 19 PY 2011 VL 473 IS 7347 BP 284 EP 284 DI 10.1038/473284a PG 1 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 765QA UT WOS:000290722400019 PM 21593845 ER PT J AU Agakishiev, H Aggarwal, MM Ahammed, Z Alakhverdyants, AV Alekseev, I Alford, J Anderson, BD Anson, CD Arkhipkin, D Averichev, GS Balewski, J Beavis, DR Behera, NK Bellwied, R Betancourt, MJ Betts, RR Bhasin, A Bhati, AK Bichsel, H Bielcik, J Bielcikova, J Biritz, B Bland, LC Bordyuzhin, IG Borowski, W Bouchet, J Braidot, E Brandin, AV Bridgeman, A Brovko, SG Bruna, E Bueltmann, S Bunzarov, I Burton, TP Cai, XZ Caines, H Calderon, M Cebra, D Cendejas, R Cervantes, MC Chajecki, Z Chaloupka, P Chattopadhyay, S Chen, HF Chen, JH Chen, JY Chen, L Cheng, J Cherney, M Chikanian, A Choi, KE Christie, W Chung, P Codrington, MJM Corliss, R Cramer, JG Crawford, HJ Leyva, AD De Silva, LC Debbe, RR Dedovich, TG Derevschikov, AA de Souza, RD Didenko, L Djawotho, P Dogra, SM Dong, X Drachenberg, JL Draper, JE Dunlop, C Efimov, LG Elnimr, M Engelage, J Eppley, G Estienne, M Eun, L Evdokimov, O Fatemi, R Fedorisin, J Fersch, RG Filip, P Finch, E Fine, V Fisyak, Y Gagliardi, CA Gangadharan, DR Geurts, F Ghosh, P Gorbunov, YN Gordon, A Grebenyuk, OG Grosnick, D Guertin, SM Gupta, A Gupta, S Guryn, W Haag, B Hajkova, O Hamed, A Han, LX Harris, JW Hays-Wehle, JP Heinz, M Heppelmann, S Hirsch, A Hjort, E Hoffmann, GW Hofman, DJ Huang, B Huang, HZ Humanic, TJ Huo, L Igo, G Jacobs, P Jacobs, W Jena, C Jin, F Joseph, J Judd, EG Kabana, S Kang, K Kapitan, J Kauder, K Ke, HW Keane, D Kechechyan, A Kettler, D Kikola, DP Kiryluk, J Kisiel, A Kizka, V Klein, SR Knospe, AG Koetke, DD Kollegger, T Konzer, J Koralt, I Koroleva, L Korsch, W Kotchenda, L Kouchpil, V Kravtsov, P Krueger, K Krus, M Kumar, L Kurnadi, P Lamont, MAC Landgraf, JM LaPointe, S Lauret, J Lebedev, A Lednicky, R Lee, JH Leight, W LeVine, MJ Li, C Li, L Li, N Li, W Li, X Li, X Li, Y Li, ZM Lisa, MA Liu, F Liu, H Liu, J Ljubicic, T Llope, WJ Longacre, RS Love, WA Lu, Y Lukashov, EV Luo, X Ma, GL Ma, YG Mahapatra, DP Majka, R Mall, OI Manweiler, R Margetis, S Markert, C Masui, H Matis, HS Matulenko, YA McDonald, D McShane, TS Meschanin, A Milner, R Minaev, NG Mioduszewski, S Mitrovski, MK Mohammed, Y Mohanty, B Mondal, MM Morozov, B Morozov, DA Munhoz, MG Mustafa, MK Naglis, M Nandi, BK Nayak, TK Netrakanti, PK Nogach, LV Nurushev, SB Odyniec, G Ogawa, A Oh, K Ohlson, A Okorokov, V Oldag, EW Olson, D Pachr, M Page, BS Pal, SK Pandit, Y Panebratsev, Y Pawlak, T Pei, H Peitzmann, T Perkins, C Peryt, W Pile, P Planinic, M Ploskon, MA Pluta, J Plyku, D Poljak, N Porter, J Poskanzer, AM Potukuchi, BVKS Powell, CB Prindle, D Pruneau, C Pruthi, NK Pujahari, PR Putschke, J Qiu, H Raniwala, R Raniwala, S Ray, RL Redwine, R Reed, R Ritter, HG Roberts, JB Rogachevskiy, OV Romero, JL Ruan, L Rusnak, J Sahoo, NR Sakrejda, I Salur, S Sandweiss, J Sangaline, E Sarkar, A Schambach, J Scharenberg, RP Schmah, AM Schmitz, N Schuster, TR Seele, J Seger, J Selyuzhenkov, I Seyboth, P Shah, N Shahaliev, E Shao, M Sharma, M Shi, SS Shou, QY Sichtermann, EP Simon, F Singaraju, RN Skoby, MJ Smirnov, N Solanki, D Sorensen, P Spinka, HM Srivastava, B Stanislaus, TDS Staszak, D Steadman, SG Stevens, JR Stock, R Strikhanov, M Stringfellow, B Suaide, AAP Suarez, MC Subba, NL Sumbera, M Sun, XM Sun, Y Sun, Z Surrow, B Svirida, DN Symons, TJM de Toledo, AS Takahashi, J Tang, AH Tang, Z Tarini, LH Tarnowsky, T Thein, D Thomas, JH Tian, J Timmins, AR Tlusty, D Tokarev, M Trainor, TA Trentalange, S Tribble, RE Tribedy, P Tsai, OD Ullrich, T Underwood, DG Van Buren, G van Nieuwenhuizen, G Vanfossen, JA Varma, R Vasconcelos, GMS Vasiliev, AN Videbaek, F Viyogi, YP Vokal, S Voloshin, SA Wada, M Walker, M Wang, F Wang, G Wang, H Wang, JS Wang, Q Wang, XL Wang, Y Webb, G Webb, JC Westfall, GD Whitten, C Wieman, H Wissink, SW Witt, R Witzke, W Wu, YF Xiao, Z Xie, W Xu, H Xu, N Xu, QH Xu, W Xu, Y Xu, Z Xue, L Yang, Y Yang, Y Yepes, P Yip, K Yoo, IK Zawisza, M Zbroszczyk, H Zhan, W Zhang, JB Zhang, S Zhang, WM Zhang, XP Zhang, Y Zhang, ZP Zhao, F Zhao, J Zhong, C Zhou, W Zhu, X Zhu, YH Zoulkarneev, R Zoulkarneeva, Y AF Agakishiev, H. Aggarwal, M. M. Ahammed, Z. Alakhverdyants, A. V. Alekseev, I. Alford, J. Anderson, B. D. Anson, C. D. Arkhipkin, D. Averichev, G. S. Balewski, J. Beavis, D. R. Behera, N. K. Bellwied, R. Betancourt, M. J. Betts, R. R. Bhasin, A. Bhati, A. K. Bichsel, H. Bielcik, J. Bielcikova, J. Biritz, B. Bland, L. C. Bordyuzhin, I. G. Borowski, W. Bouchet, J. Braidot, E. Brandin, A. V. Bridgeman, A. Brovko, S. G. Bruna, E. Bueltmann, S. Bunzarov, I. Burton, T. P. Cai, X. Z. Caines, H. Calderon, M. Cebra, D. Cendejas, R. Cervantes, M. C. Chajecki, Z. Chaloupka, P. Chattopadhyay, S. Chen, H. F. Chen, J. H. Chen, J. Y. Chen, L. Cheng, J. Cherney, M. Chikanian, A. Choi, K. E. Christie, W. Chung, P. Codrington, M. J. M. Corliss, R. Cramer, J. G. Crawford, H. J. Leyva, A. Davila De Silva, L. C. Debbe, R. R. Dedovich, T. G. Derevschikov, A. A. Derradi de Souza, R. Didenko, L. Djawotho, P. Dogra, S. M. Dong, X. Drachenberg, J. L. Draper, J. E. Dunlop, C. Efimov, L. G. Elnimr, M. Engelage, J. Eppley, G. Estienne, M. Eun, L. Evdokimov, O. Fatemi, R. Fedorisin, J. Fersch, R. G. Filip, P. Finch, E. Fine, V. Fisyak, Y. Gagliardi, C. A. Gangadharan, D. R. Geurts, F. Ghosh, P. Gorbunov, Y. N. Gordon, A. Grebenyuk, O. G. Grosnick, D. Guertin, S. M. Gupta, A. Gupta, S. Guryn, W. Haag, B. Hajkova, O. Hamed, A. Han, L-X. Harris, J. W. Hays-Wehle, J. P. Heinz, M. Heppelmann, S. Hirsch, A. Hjort, E. Hoffmann, G. W. Hofman, D. J. Huang, B. Huang, H. Z. Humanic, T. J. Huo, L. Igo, G. Jacobs, P. Jacobs, W. Jena, C. Jin, F. Joseph, J. Judd, E. G. Kabana, S. Kang, K. Kapitan, J. Kauder, K. Ke, H. W. Keane, D. Kechechyan, A. Kettler, D. Kikola, D. P. Kiryluk, J. Kisiel, A. Kizka, V. Klein, S. R. Knospe, A. G. Koetke, D. D. Kollegger, T. Konzer, J. Koralt, I. Koroleva, L. Korsch, W. Kotchenda, L. Kouchpil, V. Kravtsov, P. Krueger, K. Krus, M. Kumar, L. Kurnadi, P. Lamont, M. A. C. Landgraf, J. M. LaPointe, S. Lauret, J. Lebedev, A. Lednicky, R. Lee, J. H. Leight, W. LeVine, M. J. Li, C. Li, L. Li, N. Li, W. Li, X. Li, X. Li, Y. Li, Z. M. Lisa, M. A. Liu, F. Liu, H. Liu, J. Ljubicic, T. Llope, W. J. Longacre, R. S. Love, W. A. Lu, Y. Lukashov, E. V. Luo, X. Ma, G. L. Ma, Y. G. Mahapatra, D. P. Majka, R. Mall, O. I. Manweiler, R. Margetis, S. Markert, C. Masui, H. Matis, H. S. Matulenko, Yu A. McDonald, D. McShane, T. S. Meschanin, A. Milner, R. Minaev, N. G. Mioduszewski, S. Mitrovski, M. K. Mohammed, Y. Mohanty, B. Mondal, M. M. Morozov, B. Morozov, D. A. Munhoz, M. G. Mustafa, M. K. Naglis, M. Nandi, B. K. Nayak, T. K. Netrakanti, P. K. Nogach, L. V. Nurushev, S. B. Odyniec, G. Ogawa, A. Oh, K. Ohlson, A. Okorokov, V. Oldag, E. W. Olson, D. Pachr, M. Page, B. S. Pal, S. K. Pandit, Y. Panebratsev, Y. Pawlak, T. Pei, H. Peitzmann, T. Perkins, C. Peryt, W. Pile, P. Planinic, M. Ploskon, M. A. Pluta, J. Plyku, D. Poljak, N. Porter, J. Poskanzer, A. M. Potukuchi, B. V. K. S. Powell, C. B. Prindle, D. Pruneau, C. K. Pruthi, N. Pujahari, P. R. Putschke, J. Qiu, H. Raniwala, R. Raniwala, S. Ray, R. L. Redwine, R. Reed, R. Ritter, H. G. Roberts, J. B. Rogachevskiy, O. V. Romero, J. L. Ruan, L. Rusnak, J. Sahoo, N. R. Sakrejda, I. Salur, S. Sandweiss, J. Sangaline, E. Sarkar, A. Schambach, J. Scharenberg, R. P. Schmah, A. M. Schmitz, N. Schuster, T. R. Seele, J. Seger, J. Selyuzhenkov, I. Seyboth, P. Shah, N. Shahaliev, E. Shao, M. Sharma, M. Shi, S. S. Shou, Q. Y. Sichtermann, E. P. Simon, F. Singaraju, R. N. Skoby, M. J. Smirnov, N. Solanki, D. Sorensen, P. Spinka, H. M. Srivastava, B. Stanislaus, T. D. S. Staszak, D. Steadman, S. G. Stevens, J. R. Stock, R. Strikhanov, M. Stringfellow, B. Suaide, A. A. P. Suarez, M. C. Subba, N. L. Sumbera, M. Sun, X. M. Sun, Y. Sun, Z. Surrow, B. Svirida, D. N. Symons, T. J. M. Szanto de Toledo, A. Takahashi, J. Tang, A. H. Tang, Z. Tarini, L. H. Tarnowsky, T. Thein, D. Thomas, J. H. Tian, J. Timmins, A. R. Tlusty, D. Tokarev, M. Trainor, T. A. Trentalange, S. Tribble, R. E. Tribedy, P. Tsai, O. D. Ullrich, T. Underwood, D. G. Van Buren, G. van Nieuwenhuizen, G. Vanfossen, J. A., Jr. Varma, R. Vasconcelos, G. M. S. Vasiliev, A. N. Videbaek, F. Viyogi, Y. P. Vokal, S. Voloshin, S. A. Wada, M. Walker, M. Wang, F. Wang, G. Wang, H. Wang, J. S. Wang, Q. Wang, X. L. Wang, Y. Webb, G. Webb, J. C. Westfall, G. D. Whitten, C., Jr. Wieman, H. Wissink, S. W. Witt, R. Witzke, W. Wu, Y. F. Xiao, Z. Xie, W. Xu, H. Xu, N. Xu, Q. H. Xu, W. Xu, Y. Xu, Z. Xue, L. Yang, Y. Yang, Y. Yepes, P. Yip, K. Yoo, I-K. Zawisza, M. Zbroszczyk, H. Zhan, W. Zhang, J. B. Zhang, S. Zhang, W. M. Zhang, X. P. Zhang, Y. Zhang, Z. P. Zhao, F. Zhao, J. Zhong, C. Zhou, W. Zhu, X. Zhu, Y. H. Zoulkarneev, R. Zoulkarneeva, Y. CA STAR Collaboration TI Observation of the antimatter helium-4 nucleus SO NATURE LA English DT Article ID QUARK-GLUON PLASMA; ANTIPROTONS; COLLISIONS; ELECTRON AB High-energy nuclear collisions create an energy density similar to that of the Universe microseconds after the Big Bang(1); in both cases, matter and antimatter are formed with comparable abundance. However, the relatively short-lived expansion in nuclear collisions allows antimatter to decouple quickly from matter, and avoid annihilation. Thus, a high-energy accelerator of heavy nuclei provides an efficient means of producing and studying antimatter. The antimatter helium-4 nucleus ((4)(He) over bar), also known as the anti-alpha ((alpha) over bar), consists of two antiprotons and two antineutrons (baryon number B = -4). It has not been observed previously, although the alpha-particle was identified a century ago by Rutherford and is present in cosmic radiation at the ten per cent level(2). Antimatter nuclei with B -1 have been observed only as rare products of interactions at particle accelerators, where the rate of antinucleus production in high-energy collisions decreases by a factor of about 1,000 with each additional antinucleon(3-5). Here we report the observation of (4)<(He) over bar, the heaviest observed antinucleus to date. In total, 18 (4)(He) over bar counts were detected at the STAR experiment at the Relativistic Heavy Ion Collider (RHIC; ref. 6) in 10(9) recorded gold-on-gold (Au+Au) collisions at centre-of-mass energies of 200 GeV and 62 GeV per nucleon-nucleon pair. The yield is consistent with expectations from thermodynamic(7) and coalescent nucleosynthesis(8) models, providing an indication of the production rate of even heavier antimatter nuclei and a benchmark for possible future observations of (4)(He) over bar in cosmic radiation. C1 [Agakishiev, H.; Alakhverdyants, A. V.; Averichev, G. S.; Bunzarov, I.; Dedovich, T. G.; Efimov, L. G.; Fedorisin, J.; Filip, P.; Kechechyan, A.; Kizka, V.; Lednicky, R.; Panebratsev, Y.; Rogachevskiy, O. V.; Shahaliev, E.; Tokarev, M.; Vokal, S.; Zoulkarneev, R.; Zoulkarneeva, Y.] Joint Inst Nucl Res, Dubna 141980, Russia. [Aggarwal, M. M.; Bhati, A. K.; K. Pruthi, N.] Panjab Univ, Chandigarh 160014, India. [Ahammed, Z.; Dong, X.; Grebenyuk, O. G.; Hjort, E.; Jacobs, P.; Kiryluk, J.; Klein, S. R.; Masui, H.; Matis, H. S.; Naglis, M.; Odyniec, G.; Olson, D.; Ploskon, M. A.; Porter, J.; Poskanzer, A. M.; Powell, C. B.; Ritter, H. G.; Sakrejda, I.; Schmah, A. M.; Sichtermann, E. P.; Sun, X. M.; Symons, T. J. M.; Thomas, J. H.; Wieman, H.; Zhang, Y.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Alekseev, I.; Bordyuzhin, I. G.; Koroleva, L.; Morozov, B.; Svirida, D. N.] Alikhanov Inst Theoret & Expt Phys, Moscow 117218, Russia. [Alford, J.; Anderson, B. D.; Bouchet, J.; Joseph, J.; Keane, D.; Kumar, L.; Margetis, S.; Pandit, Y.; Subba, N. L.; Vanfossen, J. A., Jr.; Zhang, W. M.] Kent State Univ, Kent, OH 44242 USA. [Anson, C. D.; Chajecki, Z.; Humanic, T. J.; Lisa, M. A.] Ohio State Univ, Columbus, OH 43210 USA. [Arkhipkin, D.; Beavis, D. R.; Bland, L. C.; Burton, T. P.; Christie, W.; Debbe, R. R.; Didenko, L.; Dunlop, C.; Fine, V.; Fisyak, Y.; Gordon, A.; Guryn, W.; Lamont, M. A. C.; Landgraf, J. M.; Lauret, J.; Lebedev, A.; Lee, J. H.; LeVine, M. J.; Ljubicic, T.; Longacre, R. S.; Love, W. A.; Mitrovski, M. K.; Ogawa, A.; Pile, P.; Ruan, L.; Sorensen, P.; Tang, A. H.; Ullrich, T.; Van Buren, G.; Videbaek, F.; Webb, J. C.; Xu, Z.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Balewski, J.; Betancourt, M. J.; Corliss, R.; Hays-Wehle, J. P.; Leight, W.; Milner, R.; Redwine, R.; Seele, J.; Steadman, S. G.; Surrow, B.; van Nieuwenhuizen, G.; Walker, M.] MIT, Cambridge, MA 02139 USA. [Behera, N. K.; Nandi, B. K.; Pujahari, P. R.; Sarkar, A.; Varma, R.] Indian Inst Technol, Bombay 400076, Maharashtra, India. [Bellwied, R.; De Silva, L. C.; Timmins, A. R.] Univ Houston, Houston, TX 77204 USA. [Betts, R. R.; Evdokimov, O.; Hofman, D. J.; Kauder, K.; Pei, H.; Suarez, M. C.] Univ Illinois, Chicago, IL 60607 USA. [Bhasin, A.; Dogra, S. M.; Gupta, A.; Gupta, S.; Potukuchi, B. V. K. S.] Univ Jammu, Jammu 180001, India. [Bichsel, H.; Cramer, J. G.; Kettler, D.; Prindle, D.; Trainor, T. A.] Univ Washington, Seattle, WA 98195 USA. [Bielcik, J.; Hajkova, O.; Krus, M.; Pachr, M.] Czech Tech Univ, FNSPE, Prague 11519, Czech Republic. [Bielcikova, J.; Chaloupka, P.; Chung, P.; Kapitan, J.; Kouchpil, V.; Rusnak, J.; Sumbera, M.; Tlusty, D.] Nucl Phys Inst AS CR, Rez 25068, Czech Republic. [Biritz, B.; Cendejas, R.; Gangadharan, D. R.; Guertin, S. M.; Huang, H. Z.; Igo, G.; Kurnadi, P.; Shah, N.; Staszak, D.; Trentalange, S.; Tsai, O. D.; Wang, G.; Whitten, C., Jr.; Xu, W.; Zhao, F.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Borowski, W.; Estienne, M.; Kabana, S.] SUBATECH, F-44307 Nantes, France. [Braidot, E.; Peitzmann, T.] NIKHEF, NL-1098 XG Amsterdam, Netherlands. [Braidot, E.; Peitzmann, T.] Univ Utrecht, NL-1098 XG Amsterdam, Netherlands. [Brandin, A. V.; Kotchenda, L.; Kravtsov, P.; Lukashov, E. V.; Okorokov, V.; Strikhanov, M.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Bridgeman, A.; Krueger, K.; Spinka, H. M.; Underwood, D. G.] Argonne Natl Lab, Argonne, IL 60439 USA. [Brovko, S. G.; Calderon, M.; Cebra, D.; Draper, J. E.; Haag, B.; Liu, H.; Mall, O. I.; Reed, R.; Romero, J. L.; Salur, S.; Sangaline, E.] Univ Calif Davis, Davis, CA 95616 USA. [Bruna, E.; Caines, H.; Chikanian, A.; Finch, E.; Harris, J. W.; Heinz, M.; Knospe, A. G.; Majka, R.; Ohlson, A.; Putschke, J.; Sandweiss, J.; Smirnov, N.] Yale Univ, New Haven, CT 06520 USA. [Bueltmann, S.; Koralt, I.; Plyku, D.] Old Dominion Univ, Norfolk, VA 23529 USA. [Cai, X. Z.; Chen, J. H.; Han, L-X.; Jin, F.; Li, W.; Ma, G. L.; Ma, Y. G.; Shou, Q. Y.; Tian, J.; Xue, L.; Zhang, S.; Zhao, J.; Zhong, C.; Zhu, Y. H.] Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Bhasin, A.; Cervantes, M. C.; Codrington, M. J. M.; Djawotho, P.; Drachenberg, J. L.; Gagliardi, C. A.; Hamed, A.; Huo, L.; Mioduszewski, S.; Mohammed, Y.; Pal, S. K.; Tribble, R. E.] Texas A&M Univ, College Stn, TX 77843 USA. [Bhasin, A.; Chattopadhyay, S.; Ghosh, P.; Mohanty, B.; Mondal, M. M.; Nayak, T. K.; Sahoo, N. R.; Singaraju, R. N.; Tribedy, P.; Viyogi, Y. P.] Variable Energy Cyclotron Ctr, Kolkata 700064, India. [Chen, H. F.; Huang, B.; Li, C.; Lu, Y.; Luo, X.; Shao, M.; Sun, Y.; Tang, Z.; Wang, X. L.; Xu, Y.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Chen, J. Y.; Chen, L.; Ke, H. W.; Li, N.; Li, Z. M.; Liu, F.; Shi, S. S.; Wu, Y. F.; Xu, N.; Yang, Y.; Zhang, J. B.] CCNU HZNU, Inst Particle Phys, Wuhan 430079, Peoples R China. [Cheng, J.; Kang, K.; Li, Y.; Wang, Y.; Xiao, Z.; Zhang, X. P.; Zhu, X.] Tsinghua Univ, Beijing 100084, Peoples R China. [Cherney, M.; Gorbunov, Y. N.; McShane, T. S.; Seger, J.] Creighton Univ, Omaha, NE 68178 USA. [Choi, K. E.; Oh, K.; Yoo, I-K.] Pusan Natl Univ, Pusan 609735, South Korea. [Leyva, A. Davila; Hoffmann, G. W.; Li, L.; Markert, C.; Oldag, E. W.; Ray, R. L.; Schambach, J.; Thein, D.; Wada, M.] Univ Texas Austin, Austin, TX 78712 USA. [Derevschikov, A. A.; Matulenko, Yu A.; Meschanin, A.; Minaev, N. G.; Morozov, D. A.; Nogach, L. V.; Nurushev, S. B.; Vasiliev, A. N.] Inst High Energy Phys, Protvino 142281, Russia. [Derradi de Souza, R.; Takahashi, J.; Vasconcelos, G. M. S.] Univ Estadual Campinas, BR-13083859 Sao Paulo, Brazil. [Elnimr, M.; LaPointe, S.; Pruneau, C.; Sharma, M.; Tarini, L. H.; Voloshin, S. A.] Wayne State Univ, Detroit, MI 48201 USA. [Eppley, G.; Geurts, F.; Llope, W. J.; McDonald, D.; Roberts, J. B.; Yepes, P.] Rice Univ, Houston, TX 77251 USA. [Eun, L.; Heppelmann, S.] Penn State Univ, University Pk, PA 16802 USA. [Fatemi, R.; Fersch, R. G.; Korsch, W.; Webb, G.; Witzke, W.] Univ Kentucky, Lexington, KY 40506 USA. [Grosnick, D.; Koetke, D. D.; Manweiler, R.; Stanislaus, T. D. S.] Valparaiso Univ, Valparaiso, IN 46383 USA. [Hirsch, A.; Kikola, D. P.; Konzer, J.; Li, X.; Mustafa, M. K.; Netrakanti, P. K.; Scharenberg, R. P.; Skoby, M. J.; Srivastava, B.; Stringfellow, B.; Wang, F.; Wang, Q.; Xie, W.] Purdue Univ, W Lafayette, IN 47907 USA. [Jacobs, W.; Page, B. S.; Selyuzhenkov, I.; Stevens, J. R.; Wissink, S. W.] Indiana Univ, Bloomington, IN 47408 USA. [Jena, C.; Mahapatra, D. P.] Inst Phys, Bhubaneswar 751005, Orissa, India. [Kisiel, A.; Pawlak, T.; Peryt, W.; Pluta, J.; Zawisza, M.; Zbroszczyk, H.] Warsaw Univ Technol, PL-00661 Warsaw, Poland. [Kollegger, T.; Schuster, T. R.; Stock, R.; Zhou, W.] Goethe Univ Frankfurt, D-60325 Frankfurt, Germany. [Li, X.; Xu, Q. H.] Shandong Univ, Jinan 250100, Shandong, Peoples R China. [Munhoz, M. G.; Suaide, A. A. P.; Szanto de Toledo, A.] Univ Sao Paulo, BR-05508090 Sao Paulo, Brazil. [Planinic, M.; Poljak, N.] Univ Zagreb, HR-10002 Zagreb, Croatia. [Qiu, H.; Sun, Z.; Wang, J. S.; Xu, H.; Yang, Y.; Zhan, W.] Inst Modern Phys, Lanzhou 730000, Peoples R China. [Raniwala, R.; Raniwala, S.; Solanki, D.] Univ Rajasthan, Jaipur 302004, Rajasthan, India. [Schmitz, N.; Seyboth, P.; Simon, F.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Tarnowsky, T.; Wang, H.; Westfall, G. D.] Michigan State Univ, E Lansing, MI 48824 USA. [Witt, R.] USN Acad, Annapolis, MD 21402 USA. RI Takahashi, Jun/B-2946-2012; Alekseev, Igor/J-8070-2014; Yoo, In-Kwon/J-6222-2012; Peitzmann, Thomas/K-2206-2012; Witt, Richard/H-3560-2012; Yip, Kin/D-6860-2013; Xue, Liang/F-8077-2013; Voloshin, Sergei/I-4122-2013; Pandit, Yadav/I-2170-2013; Lednicky, Richard/K-4164-2013; Yang, Yanyun/B-9485-2014; Rusnak, Jan/G-8462-2014; Bielcikova, Jana/G-9342-2014; Sumbera, Michal/O-7497-2014; Strikhanov, Mikhail/P-7393-2014; Xu, Wenqin/H-7553-2014; Bruna, Elena/C-4939-2014; Dogra, Sunil /B-5330-2013; Chaloupka, Petr/E-5965-2012; Huang, Bingchu/H-6343-2015; Derradi de Souza, Rafael/M-4791-2013; Suaide, Alexandre/L-6239-2016; Svirida, Dmitry/R-4909-2016; Inst. of Physics, Gleb Wataghin/A-9780-2017; Okorokov, Vitaly/C-4800-2017; Ma, Yu-Gang/M-8122-2013; OI Takahashi, Jun/0000-0002-4091-1779; Alekseev, Igor/0000-0003-3358-9635; Peitzmann, Thomas/0000-0002-7116-899X; Yip, Kin/0000-0002-8576-4311; Xue, Liang/0000-0002-2321-9019; Pandit, Yadav/0000-0003-2809-7943; Yang, Yanyun/0000-0002-5982-1706; Sumbera, Michal/0000-0002-0639-7323; Strikhanov, Mikhail/0000-0003-2586-0405; Xu, Wenqin/0000-0002-5976-4991; Bruna, Elena/0000-0001-5427-1461; Huang, Bingchu/0000-0002-3253-3210; Derradi de Souza, Rafael/0000-0002-2084-7001; Suaide, Alexandre/0000-0003-2847-6556; Okorokov, Vitaly/0000-0002-7162-5345; Ma, Yu-Gang/0000-0002-0233-9900; Fisyak, Yuri/0000-0002-3151-8377; Bhasin, Anju/0000-0002-3687-8179; Ke, Hongwei/0000-0003-1463-7291; Sorensen, Paul/0000-0001-5056-9391; Thomas, James/0000-0002-6256-4536 FU RHIC Operations Group; RACF at BNL; NERSC Center at LBNL; Open Science Grid consortium; Offices of NP and HEP within the US DOE Office of Science; US NSF; Sloan Foundation; DFG cluster of excellence 'Origin and Structure of the Universe' of Germany; CNRS/IN2P3; FAPESP; CNPq of Brazil; Ministry of Education and Science of the Russian Federation; NNSFC; CAS; MoST; MoE of China; GA and MSMT of the Czech Republic; FOM and NWO of the Netherlands; DAE, DST and CSIR of India; Polish Ministry of Science and Higher Education; Korea Research Foundation; Ministry of Science, Education and Sports of Croatia; RosAtom of Russia FX We thank the RHIC Operations Group and RACF at BNL, the NERSC Center at LBNL and the Open Science Grid consortium for providing resources and support. This work was supported in part by the Offices of NP and HEP within the US DOE Office of Science, the US NSF, the Sloan Foundation, the DFG cluster of excellence 'Origin and Structure of the Universe' of Germany, CNRS/IN2P3, FAPESP, CNPq of Brazil, the Ministry of Education and Science of the Russian Federation, NNSFC, CAS, MoST and MoE of China, GA and MSMT of the Czech Republic, FOM and NWO of the Netherlands, DAE, DST and CSIR of India, the Polish Ministry of Science and Higher Education, the Korea Research Foundation, the Ministry of Science, Education and Sports of Croatia, and RosAtom of Russia. NR 30 TC 56 Z9 57 U1 5 U2 68 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAY 19 PY 2011 VL 473 IS 7347 BP 353 EP 356 DI 10.1038/nature10079 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 765QA UT WOS:000290722400043 ER PT J AU Liu, HH AF Liu, Hui-Hai TI A note on equations for steady-state optimal landscapes SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID RIVER NETWORKS; ENERGY-DISSIPATION; DRAINAGE NETWORKS; MINIMUM ENERGY; MODEL; EVOLUTION; BASIN; HILLSLOPE AB Based on the optimality principle (that the global energy expenditure rate is at its minimum for a given landscape under steady state conditions) and calculus of variations, we have derived new governing equations for describing steady-state optimal landscapes. Other than building on the well-established Manning's equation, this work does not rely on any empirical relationships (such as those relating hydraulic parameters to local slopes). Using additional constraints, we also theoretically demonstrate that discharge is a power function of local slope, which is consistent with field data and previous studies. Citation: Liu, H.-H. (2011), A note on equations for steady-state optimal landscapes, Geophys. Res. Lett., 38, L10402, doi:10.1029/2011GL047619. C1 Univ Calif Berkeley, Lawrence Berkeley Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Liu, HH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Div Earth Sci, MS 90-1116, Berkeley, CA 94720 USA. EM hhliu@lbl.gov FU U.S. Department of Energy (DOE) [DE-AC02-05CH11231] FX We are indebted to Yingqi Zhang and Dan Hawkes at Lawrence Berkeley National Laboratory for their critical and careful review of a preliminary version of this manuscript. We also appreciate the constructive comments from Riccardo Rigon and an anonymous reviewer. This work was supported by the U.S. Department of Energy (DOE), under DOE contract DE-AC02-05CH11231. NR 25 TC 4 Z9 4 U1 2 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAY 19 PY 2011 VL 38 AR L10402 DI 10.1029/2011GL047619 PG 4 WC Geosciences, Multidisciplinary SC Geology GA 767QX UT WOS:000290872200006 ER PT J AU Soderholm, L Skanthakumar, S Wilson, RE AF Soderholm, L. Skanthakumar, S. Wilson, Richard E. TI Structural Correspondence between Uranyl Chloride Complexes in Solution and Their Stability Constants SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID X-RAY-SCATTERING; AQUEOUS-SOLUTION; DIOXOURANIUM(VI) ION; UO22+ ION; AQUA ION; COORDINATION; URANIUM(VI); CATION; EXAFS; SPECIATION AB Pair-distribution functions (PDF)s were obtained from high-energy X-ray scattering (HEXS) data on a series of uranyl solutions as a function of chloride ion concentration. Analyses reveal that chloride forms only inner-sphere complexes with the uranyl, replacing inner-sphere waters such that the total uranyl coordination number decreases from 4.7 waters at [Cl(-)] = 0 m to 4.4 (1.7 water and 2.7 Cl(-)) at [Cl(-)] = 6.8 m. Some of the second-coordination sphere waters reorient upon uranyl inner-sphere chloride complexation in order to hydrogen bond with the bound anion. Similar data obtained on a series of solutions maintained at constant ionic strength are used to confirm structural assignments through determining stability constants for the addition of chloride to uranyl and comparison with published values. The stability constants, beta(1) = 1.5(10) m(-1), beta(2) = 0.8(4) m(-2), and beta(3) = 0.4(1) m(-3), obtained in a series of solutions with constant ionic strength of 5.3 m, are in reasonable agreement with previously published results determined by solvent extraction. The agreement of s ability constants supports our peak assignments for the PDF and thus our structural model for uranyl chloride complexes in solution. Using coordination numbers and speciation determined here as a function of chloride ion concentration, the monochloro species is found to have four coordinating waters in the uranyl equatorial plane, the dichoro species is found to be an equilibrium of three and two coordinating waters, and the trichloro species has only a single water in the equatorial plane. These values correspond to total average coordination numbers of 5, 4.3, and 4 for the mono-, di-, and trichlorouranyl complexes. From the equilibrium value of the dichloro species, it can be further estimated that Delta G = -0.5 kcal/mol for the conversion of five to four coordinate species. Overall, the HEXS data support the assertion that uranyl chloride correlations do exist and the results are not simply the result of solvent-ion effects. C1 [Soderholm, L.; Skanthakumar, S.; Wilson, Richard E.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Soderholm, L (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ls@anl.gov RI Wilson, Richard/H-1763-2011 OI Wilson, Richard/0000-0001-8618-5680 FU U.S. DOE, OBES, Chemical Sciences, Geosciences, and Biosciences Division [DE- AC02-06CH11357]; OBES, Materials Sciences [DE- AC02-06CH11357] FX We acknowledge the Actinide Facility for technical support during synchrotron experiments. This work is supported by the U.S. DOE, OBES, Chemical Sciences, Geosciences, and Biosciences Division under Contract DE- AC02-06CH11357. The APS is supported by OBES, Materials Sciences, under the same contract number. NR 51 TC 22 Z9 22 U1 2 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 19 PY 2011 VL 115 IS 19 BP 4959 EP 4967 DI 10.1021/jp111551t PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 761UU UT WOS:000290427300012 PM 21526745 ER PT J AU Xu, Q Ban, CM Dillon, AC Wei, SH Zhao, YF AF Xu, Qiang Ban, Chunmei Dillon, Anne C. Wei, Su-Huai Zhao, Yufeng TI First-Principles Study of Lithium Borocarbide as a Cathode Material for Rechargeable Li ion Batteries SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID AB-INITIO; LIXBC; SUPERCONDUCTIVITY; ELECTRODES; CHEMISTRY; OXIDES; BC3 AB Computational simulations within density functional theory are performed to investigate the potential application of a lithium borocarbide (LiBC) compound as a unique material for lithium ion batteries. The graphene-like BC sheets are predicted to be Li+ intercalation hosts with the Li ion capacity surprisingly surpassing that of graphite. Here, the layered LixBC structure is preserved with x >= 0.5, indicating that half of the Li ions in the LiBC compound are rechargeable. Furthermore, the intercalation potential (equilibrium lithium-insertion voltage of 2.3-2.4 V relative to lithium metal) is significantly higher than that in graphite, allowing Li0.5BC to function as a cathode material. The reversible electrochemical reaction, LiBC reversible arrow Li0.5BC 0.5Li, enables a specific energy density of 1088 W h/kg and a volumetric energy density of 2463 Wh/L. The volume change is less than 3% during the charging and discharging process. This discovery could lead to the development of a unique high-capacity LiBC Li ion cathode material. C1 [Xu, Qiang; Ban, Chunmei; Dillon, Anne C.; Wei, Su-Huai; Zhao, Yufeng] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Zhao, YF (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM Yufeng.Zhao@nrel.gov FU U.S. Department of Energy through the DOE's Office of Energy Efficiency and Renewable Energy Office of the Vehicle Technologies [DE-AC36-08GO28308]; NREL FX This work was funded by the U.S. Department of Energy under Subcontract Number DE-AC36-08GO28308 through the DOE's Office of Energy Efficiency and Renewable Energy Office of the Vehicle Technologies Program and NREL's Laboratory Directed Research and Development Program. NR 35 TC 13 Z9 13 U1 4 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 19 PY 2011 VL 2 IS 10 BP 1129 EP 1132 DI 10.1021/jz200440m PG 4 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 767GQ UT WOS:000290843700004 PM 26295314 ER PT J AU Beckham, GT Peters, B AF Beckham, Gregg T. Peters, Baron TI Optimizing Nucleus Size Metrics for Liquid-Solid Nucleation from Transition Paths of Near-Nanosecond Duration SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID MONTE-CARLO SIMULATIONS; LENNARD-JONES SYSTEM; CRYSTAL-NUCLEATION; RATE CONSTANTS; MOLECULAR-DYNAMICS; REACTION COORDINATE; CROSS-NUCLEATION; PHASE FORMATION; ISING-MODEL; BARRIERS AB We determine the mechanism for the liquid-solid phase transition in the Lennard-Jones fluid close to coexistence with aimless shooting and likelihood maximization. The reaction coordinate for this process is a product of a structural descriptor and the size of the nascent solid nucleus and is quantitatively verified with the committor probability histogram test. This study identifies the first accurate scalar reaction coordinate for the liquid-solid nucleation process in Lennard-Jonesium, which will likely extend to nucleation processes in other spherically symmetric fluids. On the basis of our results, we propose a structural correction factor for the commonly cited nucleus size reaction coordinate from classical nucleation theory that enables connection of simulation data to stochastic models of nucleation kinetics. In addition, we show that aimless shooting is able to obtain reasonable acceptance rates for transitions with highly diffusive characteristics, which has been problematic for transition path sampling methods for diffusive processes such as nucleation and macromolecular transitions. C1 [Beckham, Gregg T.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. [Beckham, Gregg T.] Colorado Sch Mines, Dept Chem Engn, Golden, CO 80401 USA. [Peters, Baron] Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. [Peters, Baron] Univ Calif Santa Barbara, Dept Chem & Biochem, Santa Barbara, CA 93106 USA. RP Beckham, GT (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. EM gregg.beckham@nrel.gov FU NSF [0955502]; National Renewable Energy Laboratory FX B.P. was supported by NSF CAREER Award 0955502. We acknowledge Peter Bolhuis and Wolfgang Lechner for helpful discussions. Computational time for this research was supported in part by the Golden Energy Computing Organization at the Colorado School of Mines using resources acquired with financial assistance from the National Science Foundation and the National Renewable Energy Laboratory. NR 64 TC 27 Z9 27 U1 0 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 19 PY 2011 VL 2 IS 10 BP 1133 EP 1138 DI 10.1021/jz2002887 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 767GQ UT WOS:000290843700005 PM 26295315 ER PT J AU Wang, XB Xantheas, SS AF Wang, Xue-Bin Xantheas, Sotiris S. TI Photodetachment of Isolated Bicarbonate Anion: Electron Binding Energy of HCO3- SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID CARBON-DIOXIDE; WAVE-FUNCTIONS; CONFIGURATION-INTERACTION; COUPLED-CLUSTER; GAS-PHASE; PHOTOELECTRON-SPECTROSCOPY; AQUEOUS-SOLUTION; BASIS-SETS; CHEMISTRY; SYSTEM AB We report the first direct photodetachment photoelectron spectroscopy of HCO3- in the gas phase under low-temperature conditions. The observed photoelectron spectra are complicated due to excitations of manifolds in both vibrational and electronic states. A long and single vibrational progression with a frequency of 530 +/- 20 cm(-1) is partially resolved in the threshold of the T = 20 K, 266 nm spectrum. The adiabatic electron detachment energy (ADE) of HCO3-, or, in other words, the electron affinity (EA) of neutral HCO3, is experimentally determined from the (0,0) transition to be 3.680 +/- 0.015 eV. The computed values of the Franck-Condon integral and intensity are favorable for observing the (0,0) transition. High-level ab initio calculations at the CCSD-(T) level of theory produce an estimated anharmonic frequency of 546 cm(-1) for HCO3 and a value of 3.79 eV for the (0,0) transition, both in good agreement with the experimentally determined values. C1 [Wang, Xue-Bin; Xantheas, Sotiris S.] Pacific NW Natl Lab, Div Chem & Mat Sci, Richland, WA 99352 USA. [Wang, Xue-Bin] Washington State Univ, Dept Phys, Richland, WA 99354 USA. RP Wang, XB (reprint author), Pacific NW Natl Lab, Div Chem & Mat Sci, 902 Battelle Blvd,POB 999,MS K1-83, Richland, WA 99352 USA. EM xuebin.wang@pnl.gov; sotiris.xantheas@pnl.gov RI Xantheas, Sotiris/L-1239-2015 FU Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy (DOE); DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory; Department of Energy's Office of Biological and Environmental Research FX This work was supported by the Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy (DOE). Part of this work was performed at the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory, which is operated by Battelle for the DOE. This research was performed in part using the Molecular Science Computing Facility (MSCF) in the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research. Additional computer resources were provided by the Office of Basic Energy Sciences, U.S. Department of Energy at the National Energy Research Scientific Computing Center (NERSC), a U.S. Department of Energy Office of Science user facility at Lawrence Berkeley National Laboratory. NR 46 TC 4 Z9 4 U1 3 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 19 PY 2011 VL 2 IS 10 BP 1204 EP 1210 DI 10.1021/jz200327f PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 767GQ UT WOS:000290843700018 PM 26295327 ER PT J AU Jiang, DE Overbury, SH Dai, S AF Jiang, De-en Overbury, Steven H. Dai, Sheng TI Interaction of Gold Clusters with a Hydroxylated Surface SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID TEMPERATURE CO OXIDATION; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; SELECTIVE OXIDATION; AU CATALYSTS; NANOPARTICLES; NANOCLUSTERS; DENSITY; TITANIA; SILICA AB We explore the interaction between gold nanoclusters and a fully hydroxylated surface, Mg(OH)(2)'s basal plane, by using a density functional theory-enabled local basin-hopping technique for global-minimum search. We find strong interaction of gold nanoclusters with the surface hydroxyls via a short bond between edge Au atoms and O atoms of the -OH groups. We expect that this strong interaction is ubiquitous on hydroxylated support surfaces and helps the gold nanoclusters against sintering, thereby contributing to their CO-oxidation activity at low temperatures. C1 [Jiang, De-en; Overbury, Steven H.; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Overbury, Steven H.; Dai, Sheng] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Jiang, DE (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM jiangd@ornl.gov RI Jiang, De-en/D-9529-2011; Overbury, Steven/C-5108-2016; Dai, Sheng/K-8411-2015 OI Jiang, De-en/0000-0001-5167-0731; Overbury, Steven/0000-0002-5137-3961; Dai, Sheng/0000-0002-8046-3931 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 39 TC 19 Z9 20 U1 4 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 19 PY 2011 VL 2 IS 10 BP 1211 EP 1215 DI 10.1021/jz200420t PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 767GQ UT WOS:000290843700019 PM 26295328 ER PT J AU Ressler, JJ Burke, JT Escher, JE Angell, CT Basunia, MS Beausang, CW Bernstein, LA Bleuel, DL Casperson, RJ Goldblum, BL Gostic, J Hatarik, R Henderson, R Hughes, RO Munson, J Phair, LW Ross, TJ Scielzo, ND Swanberg, E Thompson, IJ Wiedeking, M AF Ressler, J. J. Burke, J. T. Escher, J. E. Angell, C. T. Basunia, M. S. Beausang, C. W. Bernstein, L. A. Bleuel, D. L. Casperson, R. J. Goldblum, B. L. Gostic, J. Hatarik, R. Henderson, R. Hughes, R. O. Munson, J. Phair, L. W. Ross, T. J. Scielzo, N. D. Swanberg, E. Thompson, I. J. Wiedeking, M. TI Surrogate measurement of the Pu-238(n, f) cross section SO PHYSICAL REVIEW C LA English DT Article ID NEUTRON FISSION AB The neutron-induced fission cross section of Pu-238 was determined using the surrogate ratio method. The (n, f) cross section over an equivalent neutron energy range 5-20 MeV was deduced from inelastic alpha-induced fission reactions on Pu-239, with U-235(alpha, alpha' f) and U-236(alpha, alpha' f) used as references. These reference reactions reflect U-234(n, f) and U-235(n, f) yields, respectively. The deduced Pu-238(n, f) cross section agrees well with standard data libraries up to similar to 10 MeV, although larger values are seen at higher energies. The difference at higher energies is less than 20%. C1 [Ressler, J. J.; Burke, J. T.; Escher, J. E.; Bernstein, L. A.; Bleuel, D. L.; Casperson, R. J.; Gostic, J.; Hatarik, R.; Henderson, R.; Scielzo, N. D.; Swanberg, E.; Thompson, I. J.; Wiedeking, M.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Angell, C. T.; Goldblum, B. L.; Munson, J.; Swanberg, E.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Basunia, M. S.; Hatarik, R.; Phair, L. W.] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA. [Beausang, C. W.; Hughes, R. O.; Ross, T. J.] Univ Richmond, Dept Phys, Richmond, VA 23173 USA. [Ross, T. J.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. RP Ressler, JJ (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM ressler2@llnl.gov RI Escher, Jutta/E-1965-2013; Burke, Jason/I-4580-2012 FU US Department of Energy [DE-AC52-07NA27344 (LLNL), DE-AC02-05CH11231 (LBNL)]; Department of Energy's NNSA, Office of Nonproliferation Research and Development [NA-22] FX The authors thank the 88-Inch Cyclotron operations and facilities staff for the support of this study. We would also like to thank the Department of Energy's NNSA, Office of Nonproliferation Research and Development (NA-22), for financial support. This work was performed under the auspices of the US Department of Energy under Contracts No. DE-AC52-07NA27344 (LLNL) and No. DE-AC02-05CH11231 (LBNL). NR 29 TC 23 Z9 23 U1 1 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAY 19 PY 2011 VL 83 IS 5 AR 054610 DI 10.1103/PhysRevC.83.054610 PG 7 WC Physics, Nuclear SC Physics GA 766DF UT WOS:000290760500002 ER PT J AU Cao, QH Damanik, A Ma, E Wegman, D AF Cao, Qing-Hong Damanik, Asan Ma, Ernest Wegman, Daniel TI Probing lepton flavor triality with Higgs boson decay SO PHYSICAL REVIEW D LA English DT Article AB If neutrino tribimaximal mixing is explained by a non-Abelian discrete symmetry such as A(4), T-7, Delta(27), etc., the charged-lepton Higgs sector has a Z(3) residual symmetry (lepton flavor triality), which may be observed directly in the decay chain H-0 -> psi(0)(2)(psi) over bar (0)(2), then psi(0)(2)(($) over bar (0)(2)) -> l(i)(+) l(j)(-) (i not equal j), where H-0 is a standard-model-like Higgs boson and psi(0)(2) is a scalar particle needed for realizing the original discrete symmetry. If kinematically allowed, this unusual and easily detectable decay is observable at the LHC with 1 fb(-1) for E-cm = 7 TeV. C1 [Cao, Qing-Hong] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Cao, Qing-Hong] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Damanik, Asan] Sanata Dharma Univ, Dept Phys, Yogyakarta, Indonesia. [Ma, Ernest; Wegman, Daniel] Univ Calif Riverside, Dept Phys & Astron, Riverside, CA 92521 USA. RP Cao, QH (reprint author), Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. RI lebert, thomas/H-4032-2011; OI Wegman, Daniel/0000-0002-8189-1313; Damanik, Asan/0000-0003-3241-0162 FU U.S. Department of Energy [DE-AC02-06CH11357, DE-FG03-94ER40837]; Argonne National Laboratory; University of Chicago Joint Theory Institute [03921-07-137]; Ministry of National Education, Indonesia FX Q. H. C. is supported in part by the U.S. Department of Energy under Grant No. DE-AC02-06CH11357 and the Argonne National Laboratory and University of Chicago Joint Theory Institute Grant No. 03921-07-137. A. D. is supported by the Program of Academic Recharging C (PAR-C), Ministry of National Education, Indonesia. E. M. and D. W. are supported in part by the U.S. Department of Energy under Grant No. DE-FG03-94ER40837. A. D. thanks the Department of Physics and Astronomy, University of California, Riverside for hospitality during his visit. NR 17 TC 17 Z9 17 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAY 19 PY 2011 VL 83 IS 9 AR 093012 DI 10.1103/PhysRevD.83.093012 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 766DI UT WOS:000290760800003 ER PT J AU Velizhanin, KA Chien, CC Dubi, Y Zwolak, M AF Velizhanin, Kirill A. Chien, Chih-Chun Dubi, Yonatan Zwolak, Michael TI Driving denaturation: Nanoscale thermal transport as a probe of DNA melting SO PHYSICAL REVIEW E LA English DT Article ID HEAT-CONDUCTION; NONLINEAR MODEL; DYNAMICS; CHAINS AB DNA denaturation has been a subject of intense study due to its relationship to DNA transcription and its fundamental importance as a nonlinear structural transition. Many aspects of this phenomenon, however, remain poorly understood. Existing models fit quite well with experimental results on the fraction of unbound base pairs versus temperature, but yield incorrect results for other essential quantities such as the base pair fluctuation time scales. Here we demonstrate that nanoscale thermal transport can serve as a sensitive probe of the underlying microscopic physics responsible for the dynamics of DNA denaturation. Specifically, we show that the heat transport properties of DNA are altered significantly as it denatures, and this alteration encodes detailed information on the dynamics of thermal fluctuations and their interaction along the strand. This finding allows for the discrimination between models of DNA denaturation and will help shed new light on the nonlinear vibrational dynamics of this important molecule. C1 [Velizhanin, Kirill A.; Chien, Chih-Chun; Dubi, Yonatan; Zwolak, Michael] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Velizhanin, Kirill A.] Los Alamos Natl Lab, CNLS, Los Alamos, NM 87545 USA. RP Velizhanin, KA (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM kirill@lanl.gov; mpz@lanl.gov RI Zwolak, Michael/G-2932-2013; Dubi, Yonatan/G-5304-2013; Velizhanin, Kirill/C-4835-2008 OI Zwolak, Michael/0000-0001-6443-7816; FU US Department of Energy; CNLS FX The authors would like to thank A. R. Bishop, K. Rasmussen, and B. Alexandrov for valuable discussions. This research is supported by the US Department of Energy through the LANL/LDRD Program. K. A. V. also acknowledges the support provided by CNLS. NR 31 TC 12 Z9 12 U1 0 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 J9 PHYS REV E JI Phys. Rev. E PD MAY 19 PY 2011 VL 83 IS 5 AR 050906 DI 10.1103/PhysRevE.83.050906 PN 1 PG 4 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 766DZ UT WOS:000290762500002 PM 21728482 ER PT J AU Lunin, A Yakovlev, V Grudiev, A AF Lunin, A. Yakovlev, V. Grudiev, A. TI Analytical solutions for transient and steady state beam loading in arbitrary traveling wave accelerating structures SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article AB Analytical solutions are derived for both transient and steady state gradient distributions in the traveling wave (TW) accelerating structures with arbitrary variation of parameters over the structure length. The results of the unloaded and beam loaded cases are presented. Finally, the exact analytical shape of the rf pulse waveform was found in order to apply the transient beam loading compensation scheme during the structure filling time. The obtained theoretical formulas were cross-checked by direct numerical simulations on the CLIC main linac accelerating structure and demonstrated a good agreement. The proposed methods provide a fast and reliable tool for the initial stage of the TW structure analysis. C1 [Lunin, A.; Yakovlev, V.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Grudiev, A.] CERN, CH-1211 Geneva 23, Switzerland. RP Lunin, A (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. NR 21 TC 3 Z9 3 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD MAY 19 PY 2011 VL 14 IS 5 AR 052001 DI 10.1103/PhysRevSTAB.14.052001 PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 766EJ UT WOS:000290763500001 ER PT J AU Vorobiev, A Major, J Dosch, H Mueller-Buschbaum, P Falus, P Felcher, GP Velthuis, SGET AF Vorobiev, A. Major, J. Dosch, H. Mueller-Buschbaum, P. Falus, P. Felcher, G. P. Velthuis, S. G. E. te TI Phase and Microphase Separation of Polymer Thin Films Dewetted from Silicon-A Spin-Echo Resolved Grazing Incidence Neutron Scattering Study SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID DIBLOCK COPOLYMER FILMS; X-RAY; ANGLE; DIFFRACTION; SIMULATION; SURFACES; REFLECTIVITY; TRANSITIONS; ORDER AB An understanding of the structure of ultrathin polymer films on solid substrates has scientific importance in applications as well as in fundamental studies of polymer diffusion or adsorption. We present studies of the organization of dewetted droplets of polymers on a silicon surface using a new neutron scattering technique, spin echo resolved grazing incidence scattering (SERGIS), that has the potential to address at the same time the droplet droplet correlations and the chemical configuration inside each droplet. For the seminal experiments, the polarized neutron reflectometer EVA at the Institut Laue-Langevin, Grenoble, France, was equipped with a spin echo setup, and measurements were taken on surface structures previously characterized by different techniques. The dewetted polymers used in our studies were pure polystyrene, a mixture of polystyrene and polyparamethylstyrene, and a diblock copolymer of the two homopolymers. Even with a provisional setup SERGIS, we were able to determine the correlation between the droplets, providing results in excellent agreement with those obtained by atomic force microscopy and grazing incidence small-angle X-ray and neutron scattering. In addition, it was confirmed that the correlation function for diblock copolymer droplets is more complex than for polymer mixtures, exhibiting partial ordering of the copolymer within each droplet. C1 [Vorobiev, A.; Major, J.; Dosch, H.] Max Planck Inst Metallforsch, D-70569 Stuttgart, Germany. [Mueller-Buschbaum, P.] Tech Univ Munich, Lehrstuhl Funkt Mat, Phys Dept E13, D-85747 Garching, Germany. [Falus, P.; Felcher, G. P.; Velthuis, S. G. E. te] Argonne Natl Lab, Argonne, IL 60439 USA. [Dosch, H.] DESY, D-2000 Hamburg, Germany. RP Vorobiev, A (reprint author), Max Planck Inst Metallforsch, Heisenbergstr 3, D-70569 Stuttgart, Germany. EM alexei.vorobiev@esrf.fr RI te Velthuis, Suzanne/I-6735-2013; Muller-Buschbaum, Peter/C-3397-2017 OI te Velthuis, Suzanne/0000-0002-1023-8384; Muller-Buschbaum, Peter/0000-0002-9566-6088 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-06CH11357]; Max Planck Society, Munich; DFG [SPP 1164, Mu1487/2] FX The support of the management and staff at the Institut Laue-Langevin, Grenoble, France, is gratefully acknowledged. This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under contract No. DE-AC02-06CH11357 (PF, SGEtV, and GPF) and by focused neutron research funding of the Max Planck Society, Munich. P.M.B. acknowledges funding by the DFG Schwerpunktprogramm SPP 1164 "Nano- and Microfluidics" (Mu1487/2). NR 50 TC 3 Z9 3 U1 2 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 19 PY 2011 VL 115 IS 19 BP 5754 EP 5765 DI 10.1021/jp1120756 PG 12 WC Chemistry, Physical SC Chemistry GA 761US UT WOS:000290427100007 PM 21504157 ER PT J AU Khodadadi, S Curtis, JE Sokolov, AP AF Khodadadi, S. Curtis, J. E. Sokolov, A. P. TI Nanosecond Relaxation Dynamics of Hydrated Proteins: Water versus Protein Contributions SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID METHYL-GROUP DYNAMICS; MOLECULAR-DYNAMICS; NEUTRON-SCATTERING; DIELECTRIC-SPECTROSCOPY; GLASS-TRANSITION; SIDE-CHAIN; LYSOZYME; SOLVENT; SIMULATIONS; PLASTOCYANIN AB We have studied picosecond to nanosecond dynamics of hydrated protein powders using dielectric spectroscopy and molecular dynamics (MD) simulations. Our analysis of hydrogen-atom single particle dynamics from MD simulations focused on "main" (tau(main) approximate to tens of picoseconds) and "slow" (tau(slow) approximate to nanosecond) relaxation processes that were observed in dielectric spectra of similar hydrated protein samples. Traditionally, the interpretation of these processes observed in dielectric spectra has been ascribed to the relaxation behavior of hydration water tightly bounded to a protein and not to protein atoms. Detailed analysis of the MD simulations and comparison to dielectric data indicate that the observed relaxation process in the nanosecond time range of hydrated protein spectra is mainly due to protein atoms. The relaxation processes involve the entire structure of protein including atoms in the protein backbone, side chains, and turns. Both surface and buried protein atoms contribute to the slow processes; however, surface atoms demonstrate slightly faster relaxation dynamics. Analysis of the water molecule residence and dipolar relaxation correlation behavior indicates that the hydration water relaxes at much shorter time scales. C1 [Khodadadi, S.; Curtis, J. E.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Sokolov, A. P.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Sokolov, A. P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Khodadadi, S (reprint author), NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. EM sheila.khodadadi@nist.gov FU NSF [DMR-1059562]; National Research Council FX We acknowledge the partial financial support from NSF (DMR-1059562). S.K. acknowledges the National Research Council for support. Certain commercial equipment, instruments, materials, suppliers, or software are identified in this paper to foster understanding. Such identification does not imply recommendation or endorsement by the National Institute of Standards and Technology, nor does it imply that the materials or equipment identified are necessarily the best available for the purpose. NR 44 TC 28 Z9 28 U1 1 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 19 PY 2011 VL 115 IS 19 BP 6222 EP 6226 DI 10.1021/jp1122213 PG 5 WC Chemistry, Physical SC Chemistry GA 761US UT WOS:000290427100056 PM 21513284 ER PT J AU Ishizaki, A Fleming, GR AF Ishizaki, Akihito Fleming, Graham R. TI On the Interpretation of Quantum Coherent Beats Observed in Two-Dimensional Electronic Spectra of Photosynthetic Light Harvesting Complexes SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID WAVE-PACKET INTERFEROMETRY; ENERGY-TRANSFER; PHYSIOLOGICAL TEMPERATURE; DYNAMICS; MODEL; DECOHERENCE; EXCITATION; VIBRATIONS; MOLECULES; SYSTEMS AB The observation of long-lived electronic quantum coherence in a photosynthetic light harvesting system [Engel et al. Nature 2007, 446, 782] has led to much effort being devoted to elucidation of the quantum mechanisms of the photosynthetic excitation energy transfer. In this paper we examine the question of whether the decay of the coherent beating signal is due to quantum mechanical decoherence or ensemble dephasing (also called "fake decoherence"). We compare results based on the quantum master equation description of the time-evolution of the reduced density matrix with a mixed quantum/classical approach where the ensemble average is calculated after the dynamics. The two methods show good agreement with results from the quantum master equation in terms of the decay of quantum coherent oscillations when ensemble average is considered for the mixed quantum/classical approach. However, the results also demonstrate it remains possible that the quantum coherent motion is robust under individual realizations of the environment-induced fluctuations contrary to intuition obtained from the reduced density matrices, indicating that the decay of the observed quantum coherence should be understood as ensemble dephasing. Our calculations imply that coherence is a property of the pigment-protein system, not simply the preparation method of the electronic excitation. C1 [Fleming, Graham R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Fleming, GR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM GRFleming@lbl.gov RI Ishizaki, Akihito/A-7069-2010 OI Ishizaki, Akihito/0000-0002-0246-4461 FU Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC03-76SF000098] FX We acknowledge an allocation of supercomputing time from the National Energy Research Scientific Computing Center. This work was supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract DE-AC02-05CH11231 and the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy through Grant DE-AC03-76SF000098. NR 59 TC 67 Z9 67 U1 3 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAY 19 PY 2011 VL 115 IS 19 BP 6227 EP 6233 DI 10.1021/jp112406h PG 7 WC Chemistry, Physical SC Chemistry GA 761US UT WOS:000290427100057 PM 21488648 ER PT J AU Green, J Tyrrell, Z Radosz, M Hong, K Mays, JW AF Green, Jade Tyrrell, Zachary Radosz, Maciej Hong, Kunlun Mays, Jimmy W. TI Nanostructure of Solid Precipitates Obtained by Expansion of Polystyrene-block-Polybutadiene Solutions in Near Critical Propane: Block Ratio and Micellar Solution Effects SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID COPOLYMER THIN-FILMS; ANIONIC-POLYMERIZATION; MODEL POLYDIENES; POLYISOPRENE; POLYOLEFINS; PRESSURE; SOLVENT; PHASE AB In contrast to incompressible liquid solutions, compressible near-critical solutions of block copolymers allow for controlling rapid structure transformations with pressure alone. For example, when dissolved in near-critical propane, polystyrene-block-polybutadiene can form a random molecular solution at high pressures, a micellar solution at moderate pressures, and a solvent-free precipitate at low pressures. In contrast to the unstructured virgin copolymer, such a propane-treated precipitate rapidly self-assembles toward structures characteristic of equilibrated block copolymers, such as lamellae, spheres, or cylinders, which depend on the block ratio rather than on the decompression rate or temperature, at least within the rate and temperature ranges investigated in this work. At lower temperatures, however, say below 40 degrees C, glass transition of the styrene-butadiene diblocks can inhibit independent structure formation, while crystallization of their hydrogenated-butadiene analogues can preserve the micellar-solution structure. C1 [Green, Jade; Tyrrell, Zachary; Radosz, Maciej] Univ Wyoming, Soft Mat Lab, Dept Chem & Petr Engn, Laramie, WY 82071 USA. [Hong, Kunlun; Mays, Jimmy W.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Green, J (reprint author), Univ Wyoming, Soft Mat Lab, Dept Chem & Petr Engn, Laramie, WY 82071 USA. RI Hong, Kunlun/E-9787-2015 OI Hong, Kunlun/0000-0002-2852-5111 FU National Science Foundation at the University of Wyoming [CTS-0625338]; NIH [P20 RR0-16474]; National Institutes of Health, Institute for Research Resources [P20 RR15640]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy [CNMS2006-114] FX The authors gratefully acknowledge the practical help and valuable advice by Dr. W. Winoto. This work is funded by a National Science Foundation Grant CTS-0625338 at the University of Wyoming. J.G.'s stipend is funded by NIH Grant #P20 RR0-16474 from the INBRE Program of the National Center for Research Resources. The TEM facility is funded by the National Institutes of Health, Institute for Research Resources, and Grant P20 RR15640 to the Neuroscience Center of Biomedical Research Excellence. The polymer samples used in this work were synthesized at Oak Ridge National Laboratory's Center for Nanophase Materials Sciences, sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy, through User Project CNMS2006-114. NR 17 TC 0 Z9 0 U1 0 U2 6 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 19 PY 2011 VL 115 IS 19 BP 9465 EP 9470 DI 10.1021/jp201762e PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 761UV UT WOS:000290427400020 PM 21686070 ER PT J AU Proslier, T Klug, JA Elam, JW Claus, H Becker, NG Pellin, MJ AF Proslier, Thomas Klug, Jeffrey A. Elam, Jeffrey W. Claus, Helmut Becker, Nicholas G. Pellin, Michael J. TI Atomic Layer Deposition and Superconducting Properties of NbSi Films SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID THIN-FILMS; SILICIDE FORMATION; SURFACE-REACTIONS; NIOBIUM; SI2H6; WF6; HYDROGEN; NB3SI; HEAT AB Atomic layer deposition was used to synthesize niobium suicide (NbSi) films with a 1:1 stoichiometry, using NbF5 and Si2H6 as precursors. The growth mechanism at 200 degrees C was examined by in-situ quartz crystal microbalance (QCM) and quadrupole mass spectrometer (QMS). This study revealed a self-limiting reaction with a growth rate of 4.5 angstrom/cycle. NbSi was found to grow only on oxide-free films prepared using halogenated precursors. The electronic properties, growth rate, chemical composition, and structure of the films were studied over the deposition temperature range 150-400 degrees C. For all temperatures, the films are found to be stoichiometric NbSi (1:1) with no detectable fluorine impurities, amorphous with a density of 6.65 g/cm(3), and metallic with a resistivity rho = 150 mu Omega.cm at 300 K for films thicker than 35 nm. The growth rate was nearly constant for deposition temperatures between 150 and 275 degrees C but increases above 300 degrees C, suggesting the onset of non-self-limiting growth. The electronic properties of the films were measured down to 1.2 K and revealed a superconducting transition at T-c = 3.1 K. To our knowledge, a superconducting niobium silicide film with a 1:1 stoichiometry has never been grown before by any technique. C1 [Proslier, Thomas; Klug, Jeffrey A.; Elam, Jeffrey W.; Claus, Helmut; Becker, Nicholas G.; Pellin, Michael J.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Proslier, T (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM prolier@anl.gov RI Pellin, Michael/B-5897-2008; Klug, Jeffrey/A-3653-2013 OI Pellin, Michael/0000-0002-8149-9768; FU U.S. Department of Energy, Office of Science [DE-AC02-06CH11357]; American Recovery and Reinvestment Act (ARRA) through the US Department of Energy, Office of High Energy Physics Department of Science FX The work was supported by the U.S. Department of Energy, Office of Science, under Contract DE-AC02-06CH11357 and by the American Recovery and Reinvestment Act (ARRA) through the US Department of Energy, Office of High Energy Physics Department of Science. The electron microscopy was accomplished at the Electron Microscopy Center for Materials Research at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated under Contract DE-AC02-06CH11357. NR 34 TC 7 Z9 7 U1 1 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 19 PY 2011 VL 115 IS 19 BP 9477 EP 9485 DI 10.1021/jp201873b PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 761UV UT WOS:000290427400022 ER PT J AU Li, ZJ Zhang, ZR Kay, BD Dohnalek, Z AF Li, Zhenjun Zhang, Zhenrong Kay, Bruce D. Dohnalek, Zdenek TI Polymerization of Formaldehyde and Acetaldehyde on Ordered (WO3)(3) Films on Pt(111) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SELECTIVE CATALYTIC-REDUCTION; ENERGY-LOSS SPECTROSCOPY; NITRIC-OXIDE; GAS-PHASE; V2O5-WO3/TIO2 CATALYSTS; METATHESIS ACTIVITY; TUNGSTEN-OXIDE; TITANIUM-OXIDE; WO3 CATALYSTS; ADSORPTION AB Polymerization of formaldehyde, H2CO, and acetaldehyde, CH3CHO, was studied under ultrahigh vacuum conditions on a model catalyst consisting of an ultrathin WO3 film supported on Pt(111). The onset of polymerization is observed at very low temperatures of 70 and 80 K for H2CO and CH3CHO, respectively, as documented by the evolution of the infrared reflection-absorption spectra. The amount of polymer increases with increasing coverage and saturates at 5 and 8 monolayers (ML) for the H2CO and CH3CHO multilayer films, respectively. Upon heating, the polymers decompose around 250 and 190 K for H2CO and CH3CHO, respectively, as evidenced mass spectrometrically by the desorption of their monomers and oligomers into the gas phase. The heats of H2CO and CH3CHO sublimation and polymerization determined on the basis of our experiments are in good agreement with previously published values. C1 [Li, Zhenjun; Zhang, Zhenrong; Kay, Bruce D.; Dohnalek, Zdenek] Pacific NW Natl Lab, Chem & Mat Sci Div, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Dohnalek, Z (reprint author), Pacific NW Natl Lab, Chem & Mat Sci Div, Fundamental & Computat Sci Directorate, POB 999,Mail Stop K8-88, Richland, WA 99352 USA. EM Bruce.Kay@pnl.gov; Dohnalek@pnl.gov RI Li, Zhenjun/F-4714-2010; OI Zhang, Zhenrong/0000-0003-3969-2326 FU U.S. Department of Energy Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences; Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory (PNNL); U.S. DOE by Battelle Memorial Institute [DE-AC06-76RLO 1830] FX This work was supported by the U.S. Department of Energy Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences, and was performed at EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory (PNNL). PNNL is operated for the U.S. DOE by Battelle Memorial Institute under contract no. DE-AC06-76RLO 1830. Computational resources were provided at EMSL and the National Energy Research Scientific Computing Center at Lawrence Berkeley National Laboratory. NR 53 TC 13 Z9 14 U1 2 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 19 PY 2011 VL 115 IS 19 BP 9692 EP 9700 DI 10.1021/jp202169x PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 761UV UT WOS:000290427400048 ER PT J AU Aad, G Abbott, B Abdallah, J Abdelalim, AA Abdesselam, A Abdinov, O Abi, B Abolins, M Abramowicz, H Abreu, H Acerbi, E Acharya, BS Ackers, M Adams, DL Addy, TN Adelman, J Aderholz, M Adomeit, S Adragna, P Adye, T Aefsky, S Aguilar-Saavedra, JA Aharrouche, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akdogan, T Akesson, TPA Akimoto, G Akimov, AV Alam, MS Alam, MA Albrand, S Aleksa, M Aleksandrov, IN Aleppo, M Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Aliyev, M Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, J Alviggi, MG Amako, K Amaral, P Amelung, C Ammosov, VV Amorim, A Amoros, G Amram, N Anastopoulos, C Andeen, T 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Cataneo, F Catinaccio, A Catmore, JR Cattai, A Cattani, G Caughron, S Cavallari, A Cavalleri, P Cavalli, D Cavalli-Sforza, M Cavasinni, V Cazzato, A Ceradini, F Cerna, C Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cetin, SA Cevenini, F Chafaq, A Chakraborty, D Chan, K Chapleau, B Chapman, JD Chapman, JW Chareyre, E Charlton, DG Chavda, V Cheatham, S Chekanov, S Chekulaev, SV Chelkov, GA Chen, H Chen, L Chen, S Chen, T Chen, X Cheng, S Cheplakov, A Chepurnov, VF El Moursli, RC Chernyatin, V Cheu, E Cheung, SL Chevalier, L Chevallier, F Chiefari, G Chikovani, L Childers, JT Chilingarov, A Chiodini, G Chizhov, MV Choudalakis, G Chouridou, S Christidi, IA Christov, A Chromek-Burckhart, D Chu, ML Chudoba, J Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciobotaru, MD Ciocca, C Ciocio, A Cirilli, M Ciubancan, M Clark, A Clark, PJ Cleland, W Clemens, JC Clement, B Clement, C Clifft, RW Coadou, Y Cobal, M Coccaro, A Cochran, J Coe, P Cogan, JG Coggeshall, J Cogneras, E Cojocaru, CD 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Zhang, D. Zhang, H. Zhang, J. Zhang, X. Zhang, Z. Zhao, L. Zhao, T. Zhao, Z. Zhemchugov, A. Zheng, S. Zhong, J. Zhou, B. Zhou, N. Zhou, Y. Zhu, C. G. Zhu, H. Zhu, Y. Zhuang, X. Zhuravlov, V. Zieminska, D. Zilka, B. Zimmermann, R. Zimmermann, S. Zimmermann, S. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zmouchko, V. V. Zobernig, G. Zoccoli, A. Zolnierowski, Y. Zsenei, A. zur Nedden, M. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Charged-particle multiplicities in pp interactions measured with the ATLAS detector at the LHC SO NEW JOURNAL OF PHYSICS LA English DT Article ID TRANSVERSE-MOMENTUM SPECTRA; SQUARE-ROOT-S; CM ENERGIES; DISTRIBUTIONS; COLLISIONS; COLLIDER; TEV AB Measurements are presented from proton-proton collisions at centre-of-mass energies of root s = 0.9, 2.36 and 7 TeV recorded with the ATLAS detector at the LHC. Events were collected using a single-arm minimum-bias trigger. The charged-particle multiplicity, its dependence on transverse momentum and pseudorapidity and the relationship between the mean transverse momentum and charged-particle multiplicity are measured. Measurements in different regions of phase space are shown, providing diffraction-reduced measurements as well as more inclusive ones. The observed distributions are corrected to well-defined phase-space regions, using model-independent corrections. The results are compared to each other and to various Monte Carlo (MC) models, including a new AMBT1 pythia6 tune. In all the kinematic regions considered, the particle multiplicities are higher than predicted by the MC models. The central charged-particle multiplicity per event and unit of pseudorapidity, for tracks with p(T) > 100 MeV, is measured to be 3.483 +/- 0.009 (stat) +/- 0.106 (syst) at root s = 0.9 TeV and 5.630 +/- 0.003 (stat) +/- 0.169 (syst) at root s = 7 TeV. 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[Demirkoz, B.; Helsens, C.; Osuna, C.; Pacheco Pages, A.; Padilla Aranda, C.; Perez Codina, E.] Univ Autonoma Barcelona, Inst Fis Altes Energies, IFAE, ES-08193 Bellaterra, Barcelona, Spain. [Borjanovic, I.; Krstic, J.; Popovic, D. S.; Reljic, D.; Sijacki, Dj; Simic, Lj; Vranjes, N.; Milosavljevic, M. Vranjes] Univ Belgrade, Inst Phys, Belgrade 11001, Serbia. [Bozovic-Jelisavcic, I.; Mamuzic, J.; Mudrinic, M.] Vinca Inst Nucl Sci, Belgrade 11000, Serbia. [Kastanas, A.; Lipniacka, A.; Mohn, B.; Stugu, B.; Tonoyan, A.] Univ Bergen, Dept Phys & Technol, NO-5007 Bergen, Norway. [Alonso, J.; Arguin, J-F; Bach, A. M.; Galtieri, A. Barbaro; Beringer, J.; Biesiada, J.; Ciocio, A.; Einsweiler, K.; Gaponenko, A.; Gilchriese, M.; Haber, C.; Heinemann, B.; Hinchliffe, I.; Joseph, J.; Korn, A.; Leggett, C.; Lys, J.; Quarrie, D. R.; Ruwiedel, C.; Siegrist, J.; Skinnari, L. A.; Stavropoulos, G.; Tompkins, L.; Varouchas, D.] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Phys, Berkeley, CA 94720 USA. [Aliev, M.; Giorgi, F. M.; Grancagnolo, S.; Herrberg, R.; Kind, O.; Kolanoski, H.; Kwee, R.; Lacker, H.; Leyton, M.; Lohse, T.; Mandrysch, R.; Garcia, Y. Rodriguez; Schulz, H.; Sidoti, A.; zur Nedden, M.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Battaglia, A.; Beck, H. P.; Borer, C.; Ereditato, A.; Martin, T. Fonseca; Gallo, V.; Haug, S.; Kabana, S.; Topfel, C.; Venturi, N.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, High Energy Phys Lab, CH-3012 Bern, Switzerland. [Bansil, H. S.; Booth, J. R. A.; Bracinik, J.; Bright-Thomas, P. G.; Charlton, D. G.; Collins, N. J.; Curtis, C. J.; Dowell, J. D.; Garvey, J.; Hadley, D. R.; Harrison, K.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Homer, R. J.; Lilley, J. N.; Mahout, G.; Martin, T. A.; Mclaughlan, T.; McMahon, T. J.; Newman, P. R.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Typaldos, D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham B15 2TT, W Midlands, England. [Akdogan, T.; Arik, E.; Arik, M.; Dogan, O. B.; Istin, S.; Rador, T.] Bogazici Univ, Fac Sci, Dept Phys, TR-80815 Bebek, Turkey. [Cetin, S. A.] Dogus Univ, Fac Arts & Sci, Dept Phys, TR-34722 Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.; Diblen, F.] Gaziantep Univ, Fac Engn, Dept Engn Phys, TR-27310 Sehitkamil, Gaziantep, Turkey. Istanbul Tech Univ, Fac Arts & Sci, Dept Phys, TR-34469 Istanbul, Turkey. [Antonelli, S.; Bellagamba, L.; Bertin, A.; Bindi, M.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Ciocca, C.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Giacobbe, B.; Giusti, P.; Massa, I.; Mengarelli, A.; Monzani, S.; Piccinini, M.; Polini, A.; Rinaldi, L.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Spighi, R.; Valentinetti, S.; Villa, M.; Vitale, A.; Zoccoli, A.] INFN Sez Bologna, IT-40127 Bologna, Italy. Univ Bologna, Dipartimento Fis, IT-40127 Bologna, Italy. [Ackers, M.; Alhroob, M.; Anders, C. F.; Arutinov, D.; Barbero, M.; Bartsch, D.; Brock, I.; Cammin, J.; Cristinziani, M.; Desch, K.; Dingfelder, J.; Fischer, P.; Fleischmann, S.; Gaycken, G.; Geich-Gimbel, Ch; Gonella, L.; Hillert, S.; Huegging, F.; Ince, T.; Janus, M.; Khoriauli, G.; Koevesarki, P.; Kokott, T.; Kostyukhin, V. V.; Kroseberg, J.; Krueger, H.; Kruth, A.; Lapoire, C.; Lehmacher, M.; Loddenkoetter, T.; Mathes, M.; Mazur, M.; Meuser, S.; Moeser, N.; Mueller, K.; Nanava, G.; Nattermann, T.; Nuncio-Quiroz, A-E; Hanninger, G. Nunes; Peric, I.; Poghosyan, T.; Psoroulas, S.; Radics, B.; Rottlaender, I.; Runolfsson, O.; Schmieden, K.; Schmitz, M.; Schumacher, J. W.; Stockmanns, T.; Therhaag, J.; Treis, J.; Tsung, J-W; Uchida, K.; Uhlenbrock, M.; Vlasov, N.; Vogel, A.; von Toerne, E.; Wermes, N.; Wienemann, P.; Zendler, C.; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Ahlen, S. P.; Black, K. M.; Butler, J. M.; Harrington, R. D.; Hazen, E.; Lewandowska, M.; Love, J.; Marin, A.; Nation, N. R.; Posch, C.; Shank, J. T.; Whitaker, S. P.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Aefsky, S.; Amelung, C.; Bensinger, J. R.; Blocker, C.; Kirsch, L. E.; Pomeroy, D.; Skvorodnev, N.; Wellenstein, H.] Brandeis Univ, Dept Phys, Waltham, MA 02454 USA. [Caloba, L. P.; Cerqueira, A. S.; Torres, R. Coura; Gesualdi Mello, A. Da Rocha; Da Silva, P. V. M.; do Vale, M. A. B.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Perantoni, M.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, BR-21945970 Rio De Janeiro, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-05508900 Sao Paulo, Brazil. [Adams, D. L.; Armstrong, S. R.; Assamagan, K.; Begel, M.; Bernius, C.; Chen, H.; Chernyatin, V.; Dhullipudi, R.; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Greenwood, Z. D.; Hackenburg, R.; Klimentov, A.; Lanni, F.; Lynn, D.; Ma, H.; Maeno, T.; Majewski, S.; Nevski, P.; Nikolopoulos, K.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Park, W.; Pleier, M-A; Poblaguev, A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Rajagopalan, S.; Redlinger, G.; Sawyer, L.; Snyder, S.; Sondericker, J.; Steinberg, P.; Stumer, I.; Takai, H.; Tamsett, M. 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P.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Archambault, J. P.; Cojocaru, C. D.; Gillberg, D.; Heelan, L.; Khakzad, M.; Liu, C.; McCarthy, T. G.; Oakham, F. G.; Randrianarivony, K.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Braem, A.; Catinaccio, A.; Cattai, A.; Cerri, A.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dudarev, A.; Foussat, A.; Gonidec, A.; Gorini, B.; Correia, A. M. Henriques; Hoecker, A.; Koblitz, B.; La Rosa, A.; Mapelli, A.; Martin, B.; Messina, A.; Morley, A. K.; Nairz, A. M.; Nicquevert, B.; Petersen, B. A.; Poppleton, A.; Salzburger, A.; Sfyrla, A.; Szeless, B.; Tricoli, A.; Zsenei, A.] CERN, CH-1211 Geneva, Switzerland. [Anderson, K. J.; Boveia, A.; Brubaker, E.; Canelli, F.; Choudalakis, G.; Costin, T.; Feng, E. J.; Fiascaris, M.; Gardner, R. W.; Gupta, A.; Jen-La Plante, I.; Kapliy, A.; Melachrinos, C.; Merritt, F. S.; Onyisi, P. U. E.; Oreglia, M. J.; Pilcher, J. E.; Shochet, M. J.; Tuggle, J. M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Diaz, M. A.; Panes, B.; Quinonez, F.; Romero Maltrana, D.; Urrejola, P.] Pontificia Univ Catolica Chile, Fac Fis, Dept Fis, Santiago 4860, Chile. [Brooks, W. K.; Kuleshov, S.; Oyarzun, A.; Pezoa, R.; Prokoshin, F.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Cheng, S.; Han, H.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Tong, G.; Xie, Y.; Xu, G.; Yang, Y.; Yuan, L.; Zheng, S.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Gong, C.; Han, L.; Jiang, Y.; Jin, G.; Li, S.; Liu, M.; Liu, Y.; Wu, Y.; Xu, C.; Zhang, D.; Zhao, Z.] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, CN Anhui, Peoples R China. [Chen, S.; Chen, T.; Ping, J.; Yu, J.] Nanjing Univ, Dept Phys, Nanjing 210093, CN Jiangsu, Peoples R China. [Feng, C.; Ge, P.; He, M.; Miao, J.; Wang, J.; Zhan, Z.; Zhang, X.; Zhu, C. G.] Shandong Univ, High Energy Phys Grp, Jinan 250100, CN Shandong, Peoples R China. [Busato, E.; Calvet, D.; Calvet, S.; Cinca, D.; Febbraro, R.; Ghodbane, N.; Gris, P. L. Y.; Guicheney, C.; Pallin, D.; Podlyski, F.; Santoni, C.; Says, L. P.; Vazeille, F.; Viret, S.] Univ Clermont Ferrand, Lab Phys Corpusculaire, Clermont Univ, FR-63177 Aubiere, France. [Andeen, T.; Angerami, A.; Brooijmans, G.; Copic, K.; Dodd, J.; Grau, N.; Gray, H. M.; Guo, J.; Hughes, E. W.; Leltchouk, M.; Mateos, D. Lopez; Marshall, Z.; Parsons, J. A.; Penson, A.; Perez, K.; Reale, V. Perez; Spano, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY 10533 USA. [Boelaert, N.; Dam, M.; Driouichi, C.; Facius, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Jez, P.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Lundquist, J.; Mackeprang, R.; Petersen, T. C.; Rensch, B.; Simonyan, M.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen 0, Denmark. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Mastroberardino, A.; Morello, G.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Collegato Cosenza, IT-87036 Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Mastroberardino, A.; Morello, G.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, IT-87036 Arcavacata Di Rende, Italy. [Dabrowski, W.; Dwuznik, M.; Idzik, M.; Jelen, K.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Rulikowska-Zarebska, E.; Toczek, B.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, FPACS, AGH UST, PL-30059 Krakow, Poland. [Banas, E.; Blocki, J.; Bruckman de Renstrom, P. A.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa; Malecki, P.; Olszewski, A.; Olszowska, J.; Richter-Was, E.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Daya, R. K.; Yagci, K. Dindar; Firan, A.; Goldin, D.; Hadavand, H. K.; Hoffman, J.; Ilchenko, Y.; Ishmukhametov, R.; Joffe, D.; Kama, S.; Kasmi, A.; Kehoe, R.; Liang, Z.; Lu, L.; Renkel, P.; Rios, R. R.; Stroynowski, R.; Ye, J.; Zarzhitsky, P.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Galyaev, E.; Izen, J. M.; Lou, X.; Reeves, K.] Univ Texas Dallas, Richardson, TX 75080 USA. [Bechtle, P.; Kuutmann, E. Bergeaas; Boehler, M.; Brandt, G.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Gosdzik, B.; Gregor, I. M.; Hiller, K. H.; Hristova, I.; Husemann, U.; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Mehlhase, S.; Mijovic, L.; Moenig, K.; Naumann, T.; Nozicka, M.; Cavalcanti, T. Perez; Petschull, D.; Placakyte, R.; Rubinskiy, I.; Stelzer, H. J.; Terwort, M.; Vankov, P.; Wildt, M. A.; Zhu, H.] DESY, D-22603 Hamburg, Germany. [Bunse, M.; Dobos, D.; Goessling, C.; Hirsch, F.; Klaiber-Lodewigs, J.; Klingenberg, R.; Krasel, O.; Mass, M.; Muenstermann, D.; Rajek, S.; Reisinger, I.; Walbersloh, J.; Weber, J.; Wunstorf, R.] TU Dortmund, DE-44221 Dortmund, Germany. [Goepfert, T.; Kar, D.; Kobel, M.; Leonhardt, K.; Ludwig, A.; Mader, W. F.; Prudent, X.; Schaarschmidt, J.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01069 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Fowler, A. J.; Ko, B. R.; Oh, S. H.; Wang, C.; Yamaoka, J.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; O'Brien, B. J.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, Edinburgh EH9 3JZ, Midlothian, Scotland. [Griesmayer, E.] Fachhsch Wiener Neustadt, AT-2700 Wiener Neustadt, Austria. [Annovi, A.; Antonelli, M.; Bilokon, H.; Cerutti, F.; Curatolo, M.; Esposito, B.; Ferrer, M. L.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Ventura, S.; Vilucchi, E.; Wen, M.] INFN Lab Nazl Frascati, IT-00044 Frascati, Italy. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Bell, P. J.; Bell, W. H.; Berglund, E.; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Efthymiopoulos, I.; Ferrere, D.; Gadomski, S.; Navarro, J. E. Garcia; Gaumer, O.; Gonzalez-Sevilla, S.; Goulette, M. P.; Hamilton, A.; Leger, A.; Lister, A.; Macina, D.; Latour, B. Martin dit; Mikulec, B.; Moneta, L.; Herrera, C. Mora; Morone, M-C; Nektarijevic, S.; Orellana, F.; Pasztor, G.; Pohl, M.; Robichaud-Veronneau, A.; Rosselet, L.; Urquijo, P.; Wu, X.] Univ Geneva, Sect Phys, CH-1211 Geneva 4, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Coccaro, A.; Cornelissen, T.; Cuneo, S.; Dameri, M.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Morettini, P.; Odino, G. A.; Olcese, M.; Osculati, B.; Parodi, F.; Rossi, L. P.; Schiavi, C.] INFN Sez Genova, IT-16146 Genoa, Italy. Univ Genoa, Dipartimento Fis, IT-16146 Genoa, Italy. [Chikovani, L.; Djobava, T.; Khubua, J.; Magradze, E.; Mchedlidze, G.; Mosidze, M.; Tskhadadze, E. G.] Georgian Acad Sci, Inst Phys, GE-380077 Tbilisi, Rep of Georgia. [Chikovani, L.; Djobava, T.; Khubua, J.; Magradze, E.; Mchedlidze, G.; Mosidze, M.; Tskhadadze, E. G.] Tbilisi State Univ, HEP Inst, GE-380086 Tbilisi, Rep of Georgia. [Astvatsatourov, A.; Dueren, M.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35392 Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Gemmell, A.; Kenyon, M.; McGlone, H.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Pickford, A.; Robson, A.; Saxon, D. H.; Shaw, C.; Smith, K. M.; St Denis, R. D.; Steele, G.; Stewart, G. A.; Thompson, A. S.; Wraight, K.; Wright, C.] Univ Glasgow, Dept Phys & Astron, Glasgow G12 8QQ, Lanark, Scotland. [Ay, C.; Blumenschein, U.; Brandt, O.; Erdmann, J.; Evangelakou, D.; Grosse-Knetter, J.; Guindon, S.; Haller, J.; Henrichs, A.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Mann, A.; Meyer, J.; Morel, J.; Park, S. J.; Prell, S.; Quadt, A.; Roe, A.; Shabalina, E.; Uhrmacher, M.; Weber, P.; Weingarten, J.] Univ Gottingen, Inst Phys 2, D-37077 Gottingen, Germany. [Albrand, S.; Andrieux, M-L; Clement, B.; Collot, J.; Crepe-Renaudin, S.; de Saintignon, P.; Delsart, P. A.; Donini, J.; Dzahini, D.; Hostachy, J-Y; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Martin, Ph; Polci, F.; Stark, J.; Sun, X.; Trocme, B.] CNRS IN2P3, LPSC, FR-38026 Grenoble, France. [Albrand, S.; Andrieux, M-L; Clement, B.; Collot, J.; Crepe-Renaudin, S.; de Saintignon, P.; Delsart, P. A.; Donini, J.; Dzahini, D.; Hostachy, J-Y; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Martin, Ph; Polci, F.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, FR-38026 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Brandenburg, G. W.; Franklin, M.; Hurst, P.; Huth, J.; Jeanty, L.; Kagan, M.; Kashif, L.; Outschoorn, V. Martinez; Mills, C.; Moed, S.; Morii, M.; Prasad, S.; Smith, B. C.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Childers, J. T.; Dietzscha, T. A.; Foehlisch, F.; Geweniger, C.; Hanke, P.; Henke, M.; Khomich, A.; Kluge, E-E; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H-C; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, D-69120 Heidelberg, Germany. [Radescu, V.; Schaetzel, S.; Schoening, A.] Inst Phys, D-69120 Heidelberg, Germany. [Kugel, A.; Maenner, R.; Schroer, N.] ZITI Ruprecht Karls Univ Heidelberg, DE-68131 Mannheim, Germany. [Ohsugi, T.] Hiroshima Univ, Fac Sci, Higashihiroshima, JP Hiroshima 7398526, Japan. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Saeki Ku, Hiroshima, JP Hiroshima 7315193, Japan. [Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Jain, V.; Luehring, F.; Marino, C. P.; Ogren, H.; Penwell, J.; Price, D.; Rust, D. R.; Whittington, D.; Yang, Y.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. 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A.; Mineev, M.; Nikolaev, K.; Olchevski, A. G.; Peshekhonov, V. D.; Romanov, V. M.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.] Joint Inst Nucl Res, RU-141980 JINR Dubna, Moscow Region, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Ishii, K.; Ishino, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Manabe, A.; Mitsui, S.; Morita, Y.; Murakami, K.; Nagano, K.; Nozaki, M.; Odaka, S.; Ohska, T. K.; Sasaki, O.; Sasaki, T.; Suzuki, Y.; Tanaka, S.; Terada, S.; Tojo, J.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Org, KEK, Tsukuba, Ibaraki 3050801, Japan. [Hayakawa, T.; Homma, Y.; Ichimiya, R.; Ishikawa, A.; Kawagoe, K.; King, M.; Kiyamura, H.; Kurashige, H.; Matsushita, T.; Miyazaki, K.; Nishiyama, T.; Ochi, A.; Okada, S.; Omachi, C.; Suita, K.; Takeda, H.; Tani, K.; Tokunaga, K.; Yamazaki, Y.] Kobe Univ, Grad Sch Sci, Nada Ku, JP Kobe 6578501, Japan. [Takashima, R.] Kyoto Univ, Fushimi Ku, Kyoto, JP Kyoto 6128522, Japan. [Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, FCE, Dept Fis, IFLP CONICET UNLP, RA-1900 La Plata, Argentina. [Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Brodbeck, T. J.; Catmore, J. R.; Cheatham, S.; Chilingarov, A.; Davidson, R.; De Mora, L.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Ratoff, P. N.; Sloan, T. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster LA1 4YB, England. [Bianco, M.; Brambilla, E.; Cataldi, G.; Cazzato, A.; Chiodini, G.; Coluccia, R.; Crupi, R.; Gorini, E.; Grancagnolo, F.; Guida, A.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] INFN Sez Lecce, IT-73100 Lecce, Italy. [Allport, P. P.; Austin, N.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Houlden, M. A.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Maxfield, S. J.; Mehta, A.; Migas, S.; Prichard, P. M.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wiglesworth, C.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Bianco, M.; Brambilla, E.; Cazzato, A.; Coluccia, R.; Crupi, R.; Gorini, E.; Guida, A.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Fis, IT-73100 Lecce, Italy. [Cindro, V.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, SI-1000 Ljubljana, Slovenia. [Cindro, V.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Dept Phys, SI-1000 Ljubljana, Slovenia. [Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Cooper, B. D.; Eisenhandler, E.; Ellis, K.; Landon, M. P. J.; Lloyd, S. L.; Morin, J.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Stevenson, K.; Castanheira, M. Teixeira Dias; Traynor, D.] Queen Mary Univ London, Dept Phys, London E1 4NS, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Boorman, G.; Cooper-Smith, N. J.; Cowan, G.; Edwards, C. A.; George, S.; Goncalo, R.; Hayden, D.; Kilvington, G.; McMahon, T. R.; Misiejuk, A.; Rose, M.; Strong, J. A.; Teixeira-Dias, P.] Univ London, Dept Phys, Egham TW20 0EX, Surrey, England. [Baker, S.; Boeser, S.; Butterworth, J. M.; Byatt, T.; Campanelli, M.; Christidi, I. A.; Davison, A. R.; Dean, S.; Drohan, J. G.; Jansen, E.; Jones, T. W.; Konstantinidis, N.; Monk, J.; Nash, M.; Nurse, E.; Ozcan, V. E.; Prabhu, R.; Richards, A.; Robinson, J. E. M.; Sherwood, P.; Simmons, B.; Taylor, C.; Waugh, B. M.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Beau, T.; Bordoni, S.; Calderini, G.; Camard, A.; Cavalleri, P.; Chareyre, E.; De Cecco, S.; Derue, F.; Imbault, D.; Krasny, M. W.; Lacour, D.; Laforge, B.; Le Dortz, O.; Lellouch, J.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph; Theveneaux-Pelzer, T.; Trincaz-Duvoid, S.; Trinh, T. N.; Vannucci, F.] Univ Paris 07, Lab Phys Nucl & Hautes Energies, Univ Paris 06, CNRS IN2P3, F-75252 Paris 05, France. [Akesson, T. P. A.; Alonso, A.; Groth-Jensen, J.; Hedberg, V.; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.] Lund Univ, Fysiska Inst, SE-22100 Lund, Sweden. [Barreiro, F.; Cantero, J.; Del Peso, J.; Glasman, C.; Labarga, L.; Lagouri, T.; March, L.; Nebot, E.; Rodier, S.; Terron, J.] Univ Autonoma Madrid, Fac Ciencias, Dept Fis Teor, ES-28049 Madrid, Spain. [Aharrouche, M.; Arnaez, O.; Bendel, M.; Blum, W.; Buescher, V.; Eckweiler, S.; Edmonds, K.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Ji, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Meyer, C.; Moreno, D.; Neusiedl, A.; Rieke, S.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Siragusa, G.; Tapprogge, S.; Anh, T. Vu] Johannes Gutenberg Univ Mainz, Inst Phys, DE-55099 Mainz, Germany. [Almond, J.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Foster, J. M.; Howarth, J.; Hughes-Jones, R. E.; Ibbotson, M.; Jones, G.; Keates, J. R.; Kelly, M.; Kolya, S. D.; Lane, J. L.; Loebinger, F. K.; Marshall, R.; Martyniuk, A. C.; Marx, M.; Masik, J.; Miyagawa, P. S.; Nasteva, I.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Plano, W. G.; Schwanenberger, C.; Snow, S. W.; Tevlin, C. M.; Watts, S.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester M13 9PL, Lancs, England. [Aoun, S.; Bee, C.; Benchouk, C.; Bernardet, K.; Bousson, N.; Cerna, C.; Clemens, J. C.; Coadou, Y.; Correard, S.; Delpierre, P.; Djama, F.; Etienne, F.; Feligioni, L.; Henry-Couannier, F.; Hoffmann, D.; Hubaut, F.; Kuna, M.; Le Guirriec, E.; Leveque, J.; Li, B.; Monnier, E.; Odier, J.; Petit, E.; Pralavorio, P.; Qian, Z.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, CNRS IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Thompson, E. N.; van Eldik, N.; Willocq, S.; Woudstra, M. J.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Chapleau, B.; Corriveau, F.; Dobbs, M.; Dufour, M-A; Guler, H.; Klemetti, M.; Potter, C. T.; Robertson, S. 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[Aderholz, M.; Barillari, T.; Beimforde, M.; Bethke, S.; Capriotti, D.; Cortiana, G.; Dannheim, D.; Dedes, G.; Dietl, H.; Dubbert, J.; Ehrich, T.; Flowerdew, M. J.; Giovannini, P.; Goettfert, T.; Groh, M.; Haefner, P.; Hauff, D.; Hott, T.; Jantsch, A.; Kaiser, S.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Lutz, G.; Macchiolo, A.; Manz, A.; Menke, S.; Mohrdieck-Moeck, S.; Moser, H. G.; Nisius, R.; Oberlack, H.; Pospelov, G. E.; Potrap, I. N.; Rauter, E.; Richter, R.; Salihagic, D.; Schacht, P.; Seuster, R.; Stonjek, S.; Valderanis, C.; von der Schmitt, H.; von Loeben, J.; Zhuravlov, V.] Werner Heisenberg Inst, Max Planck Inst Phys, D-80805 Munich, Germany. [Shimojima, M.; Tanaka, Y.] Nagasaki Inst Appl Sci, JP Nagasaki 8510193, Japan. [Hasegawa, S.; Itoh, Y.; Ohshima, T.; Okumura, Y.; Sugimoto, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Grad Sch Sci, Chikusa Ku, Nagoya, Aichi 4648602, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Cevenini, F.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Doria, A.; Giordano, R.; Iacobucci, G.; Izzo, V.; Merola, L.; Musto, E.; Patricelli, S.; Rossi, E.; Sekhniaidze, G.] INFN Sez Napoli, IT-80126 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Cevenini, F.; Chiefari, G.; della Volpe, D.; Giordano, R.; Merola, L.; Musto, E.; Patricelli, S.; Rossi, E.] Univ Naples Federico II, Dipartimento Sci Fis, IT-80126 Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Metcalfe, J.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Consonni, M.; De Groot, N.; Filthaut, F.; Klok, P. F.; Konig, A. C.; Koetsveld, F.; Magrath, C. A.; Ordonez, G.; Raas, M.; Timmermans, C. J. W. P.] Radboud Univ Nijmegen, NIKHEF, Dept Expt High Energy Phys, NL-6525 AJ Nijmegen, Netherlands. [Bentvelsen, S.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Buis, E. J.; Colijn, A. P.; Dankers, R.; Daum, C.; de Jong, P.; De Nooij, L.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Koutsman, A.; Lee, H.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Muijs, A.; Mussche, I.; Ottersbach, J. P.; Peters, O.; Reichold, A.; Rijpstra, M.; Ruckstuhl, N.; Salamanna, G.; Sandstroem, R.; Snuverink, J.; Ta, D.; Tsiakiris, M.; Turlay, E.; van der Graaf, H.; van der Kraaij, E.; van der Poel, E.; Van Eijk, B.; van Kesteren, Z.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.] Nikhef Natl Inst Subat Phys, NL-1098 XG Amsterdam, Netherlands. [Bentvelsen, S.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Buis, E. J.; Colijn, A. P.; Dankers, R.; Daum, C.; de Jong, P.; De Nooij, L.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Koutsman, A.; Lee, H.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Muijs, A.; Mussche, I.; Ottersbach, J. P.; Peters, O.; Reichold, A.; Rijpstra, M.; Ruckstuhl, N.; Salamanna, G.; Sandstroem, R.; Snuverink, J.; Ta, D.; Tsiakiris, M.; Turlay, E.; van der Graaf, H.; van der Kraaij, E.; van der Poel, E.; Van Eijk, B.; van Kesteren, Z.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.] Univ Amsterdam, NL-1098 XG Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; de Lima, J. G. Rocha; Suhr, C.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Bobrovnikov, V. B.; Bogdanchikov, A.; Kazanin, V. A.; Kolachev, G. M.; Korol, A.; Malyshev, V.; Maslennikov, A. L.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.; Zaytsev, A.] Budker Inst Nucl Phys BINP, RU Novosibirsk 630090, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; Djilkibaev, R.; Konoplich, R.; Krasznahorkay, A.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Shibata, A.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA. [Arms, K. E.; Fernando, W.; Fisher, M. J.; Gan, K. K.; Kagan, H.; Kass, R. D.; Moss, J.; Rahimi, A. M.; Strang, M.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 7008530, Japan. [Abbott, B.; Gutierrez, P.; Huang, G. S.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Kocnar, A.] Palacky Univ, Olomouc 77207, Czech Republic. [Brau, J. E.; Ptacek, E.; Reinsch, A.; Robinson, M.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abreu, H.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Bernat, P.; Blanchard, J-B; Bourdarios, C.; Breton, D.; Collard, C.; De La Taille, C.; De Regie, J. B. De Vivie; Diglio, S.; Dudziak, F.; Duflot, L.; Escalier, M.; Falou, A. C.; Fayard, L.; Fournier, D.; Grivaz, J-F; Heller, M.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Lounis, A.; Makovec, N.; Matricon, P.; Nakahama, Y.; Niedercorn, F.; Perus, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Veillet, J. J.; Vukotic, I.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, CNRS, IN2P3, Orsay, France. [Hanagaki, K.; Hirose, M.; Meguro, T.; Nomachi, M.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka 5600043, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Czyczula, Z.; Gjelsten, B. K.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Pylypchenko, Y.; Read, A. L.; Rohne, O.; Samset, B. H.; Stapnes, S.; Strandlie, A.; Taga, A.] Univ Oslo, Dept Phys, NO-0316 Oslo 3, Norway. [Abdesselam, A.; Apolle, R.; Barr, A. J.; Beauchemin, P. H.; Boddy, C. R.; Brett, N. D.; Buchanan, J.; Buckingham, R. M.; Buira-Clark, D.; Coe, P.; Coniavitis, E.; Cooper-Sarkar, A. M.; Dennis, C.; Doglioni, C.; Farrington, S. M.; Ferrando, J.; Gallas, E. J.; Gilbert, L. M.; Gwenlan, C.; Hawes, B. M.; Holmes, A.; Horton, K.; Howell, D. F.; Huffman, T. B.; Issever, C.; Karagoz, M.; King, R. S. B.; Kirsch, G. P.; Kundu, N.; Larner, A.; Lau, W.; Lavorato, A.; Liang, Z.; Livermore, S. S. A.; Loken, J.; Mattravers, C.; Mermod, P.; Mitra, A.; Nickerson, R. B.; Pinder, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Wooden, G.] Univ Oxford, Dept Phys, Oxford OX1 3RH, England. [Bellomo, M.; Cambiaghi, M.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesi, V.] INFN Sez Pavia, IT-27100 Pavia, Italy. [Cambiaghi, M.; Conta, C.; Franchino, S.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.] Univ Pavia, Dipartimento Fis Nucl & Teor, IT-27100 Pavia, Italy. [Alison, J.; Degenhardt, J.; Donega, M.; Dressnandt, N.; Fratina, S.; Hance, M.; Hines, E.; Jackson, B.; Kroll, J.; Kunkle, J.; LeGeyt, B. C.; Lipeles, E.; Martin, F. F.; Olivito, D.; Ospanov, R.; Reece, R.; Stahlman, J.; Thomson, E.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, High Energy Phys Grp, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Nesterov, S. Y.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Zalite, Yo K.] Petersburg Nucl Phys Inst, RU-188300 Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Francavilla, P.; Giangiobbe, V.; Lupi, A.; Mazzoni, E.; Roda, C.; Sarri, F.; Zenonos, Z.] INFN Sez Pisa, IT-56127 Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Francavilla, P.; Giangiobbe, V.; Lupi, A.; Mazzoni, E.; Roda, C.; Sarri, F.; Zenonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, IT-56127 Pisa, Italy. [Boudreau, J.; Boulahouache, C.; Cleland, W.; Kittelmann, T.; Mueller, J.; Paolone, V.; Prieur, D.; Savinov, V.; Tsulaia, V.; Wendler, S.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Amorim, A.; Anjos, N.; Carvalho, J.; Conde Muino, P.; Do Valle Wemans, A.; Fernandes, B.; Fiolhais, M. C. N.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Magalhaes Martins, P. J.; Maio, A.; Maneira, J.; Morais, A.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Soares, M.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000149 Lisbon, Portugal. [Aguilar-Saavedra, J. A.; Castro, N. F.] Univ Granada, Dept Fis Teor & Cosmos, E-18071 Granada, Spain. [Aguilar-Saavedra, J. A.; Castro, N. F.] CAFPE, E-18071 Granada, Spain. [Chudoba, J.; Gallus, P.; Gunther, J.; Havranek, M.; Hruska, I.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Kvasnicka, O.; Lipinsky, L.; Lokajicek, M.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Panuskova, M.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, CZ-18221 Prague 8, Czech Republic. [Davidek, T.; Dolejsi, J.; Dolezal, Z.; Drasal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Inst Particle & Nucl Phys, CZ-18000 Prague 8, Czech Republic. [Augsten, K.; Holy, T.; Horazdovsky, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.] Czech Tech Univ, CZ-16635 Prague 6, Czech Republic. [Ammosov, V. V.; Borisov, A.; Bozhko, N. I.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Gapienko, V. A.; Golovnia, S. N.; Gorokhov, S. A.; Goryachev, V. N.; Gushchin, V. N.; Ivashin, A. V.; Kabachenko, V. V.; Karyukhin, A. N.; Kholodenko, A. G.; Kiver, A. M.; Kopikov, S. V.; Koreshev, V.; Korotkov, V. A.; Kozhin, A. S.; Lapin, V. V.; Larionov, A. V.; Levitski, M. S.; Minaenko, A. A.; Mitrofanov, G. Y.; Moisseev, A. M.; Myagkov, A. G.; Nikolaenko, V.; Pleskach, A. V.; Ryadovikov, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Sviridov, Yu M.; Vorobiev, A. P.; Vovenko, A. S.; Zaets, V. G.; Zaitsev, A. M.; Zenin, A. V.; Zenin, O.; Zmouchko, V. V.] State Res Ctr Inst High Energy Phys, Moscow 142281, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Botterill, D.; Burke, S.; Clifft, R. W.; Dallison, S. J.; Dewhurst, A.; Emeliyanov, D.; Fisher, S. M.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Greenfield, D.; Hart, J. C.; Haywood, S. J.; Kirk, J.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Strube, J.; Tyndel, M.; Weber, M.; Wickens, F. J.; Wielers, M.; Zajacova, Z.] Sci & Technol Facil Council, Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Benslama, K.; Ju, X.; Ming, Y.; Ortega, E. O.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Shiga 5258577, Japan. [Anulli, F.; Artoni, G.; Bagnaia, P.; Biglietti, M.; Bini, C.; Borroni, S.; Caloi, R.; Cavallari, A.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvoa, A.; Dionisi, C.; Falciano, S.; Gentile, S.; Giagu, S.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Maiani, C.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Tehrani, F. Safai; Camillocci, E. Solfaroli; Spila, F.; Valente, P.; Vari, R.; Veneziano, S.; Zanello, L.] INFN Sez Roma, IT-00185 Rome, Italy. [Artoni, G.; Bagnaia, P.; Biglietti, M.; Bini, C.; Borroni, S.; Caloi, R.; Cavallari, A.; Ciapetti, G.; D'Orazio, A.; Dionisi, C.; Gentile, S.; Giagu, S.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Maiani, C.; Tehrani, F. Safai; Camillocci, E. Solfaroli; Spila, F.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, IT-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Nardo, R.; Di Simone, A.; Liberti, B.; Marchese, F.; Paoloni, A.; Salamon, A.; Santonico, R.] INFN Sez Roma Tor Vergata, IT-00133 Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Nardo, R.; Di Simone, A.; Marchese, F.; Paoloni, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, IT-00133 Rome, Italy. [Bacci, C.; Baroncelli, A.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Spiriti, E.; Stanescu, C.; Tonazzo, A.] INFN Sez Roma Tre, IT-00146 Rome, Italy. [Bacci, C.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.; Tonazzo, A.] Univ Roma Tre, Dipartimento Fis, IT-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Goujdami, D.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies RUPHE, Fac Sci Ain Chock, MA Casablanca, Morocco. Ctr Natl Energie Sci Tech Nucl CNESTEN, Rabat 10001, Morocco. [Derkaoui, J. E.; Ouchrif, M.] Univ Mohamed Premier, LPTPM, Fac Sci, Oujda 60000, Morocco. [El Moursli, R. Cherkaoui; Ghazlane, H.] Univ Mohammed 5, Fac Sci, Rabat 10000, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Boonekamp, M.; Chevalier, L.; Chevallier, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Le Menedeu, E.; Legendre, M.; Lenzi, B.; Mansoulie, B.; Meyer, J-P; Morange, N.; Nicolaidou, R.; Ouraou, A.; Pomarede, D. M.; Resende, B.; Royon, C. R.; Schune, Ph; Schwindling, J.; Virchaux, M.] CEA, DSM IRFU, Ctr Etudes Saclay, FR-91191 Gif Sur Yvette, France. [Bangert, A.; Chouridou, S.; Damiani, D. S.; Dubbs, T.; Fowler, K.; Grillo, A. A.; Hare, G. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W; Schumm, B. A.; Seiden, A.; Taylor, G.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys SCIPP, Santa Cruz, CA 95064 USA. [Forbush, D. A.; Goussiou, A. G.; Griffiths, J.; Harris, O. M.; Kuykendall, W.; Lubatti, H. J.; Mockett, P.; Policicchio, A.; Rosati, S.; Rothberg, J.; Ventura, D.; Verducci, M.; Wang, J. C.; Watts, G.; Zhao, T.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Booth, C. N.; Booth, P.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Duxfield, R.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Lehto, M.; Mayne, A.; Mcfayden, J. A.; Nicolas, L.; Owen, S.; Paganis, E.; Sutton, M. R.; Tovey, D. R.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield S3 7RH, S Yorkshire, England. [Hasegawa, Y.; Ohshita, H.; Takeshita, T.] Shinshu Univ, Dept Phys, Fac Sci, Matsumoto, JP Nagano 3908621, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Sipica, V.; Stahl, T.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Komaragiri, J. R.; O'Neil, D. C.; Petteni, M.; Schouten, D.; Stelzer, B.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Gao, Y. S.; Grenier, P.; Haas, A.; Hansson, P.; Horn, C.; Jackson, P.; Kenney, C. J.; Kim, P. C.; Kocian, M.; Koi, T.; Lowe, A. J.; Miller, D. W.; Mount, R.; Nelson, S.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Wilson, M. G.; Wittgen, M.; Young, C.] Stanford Linear Accelerator Ctr, Accelerator Lab, Stanford, CA 94309 USA. [Batkova, L.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.; Zilka, B.] Comenius Univ, Fac Math Phys & Informat, SK-84248 Bratislava, Slovakia. [Antos, J.; Brunckob, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, SK-04353 Kosice, Slovakia. Univ Johannesburg, Dept Phys, ZA-2006 Johannesburg, South Africa. [Leney, K. J. C.; Vickey, T.] Univ Witwatersrand, Sch Phys, ZA-2050 Johannesburg, South Africa. [Asman, B.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Hidvegi, A.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Lesser, J.; Lundberg, J.; Milstead, D. A.; Moa, T.; Nordkvist, B.; Ohm, C. C.; Papadelis, A.; Ramstedt, M.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden. [Asman, B.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Lundberg, J.; Milstead, D. A.; Moa, T.; Nordkvist, B.; Ohm, C. C.; Ramstedt, M.; Sellden, B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Grahn, K-J; Lund-Jensen, B.] Royal Inst Technol KTH, Dept Phys, SE-10691 Stockholm, Sweden. [Ahmad, A.; Caputo, R.; Deluca, C.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Grimm, K.; Hobbs, J.; Jia, J.; Khodinov, A.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.; Yurkewicz, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [De Santo, A.; Potter, C. J.; Salvatore, F.] Univ Sussex, Dept Phys & Astron, Brighton BN1 9QH, E Sussex, England. [Lee, J. S. H.; Patel, N.; Saavedra, A. F.; Varvell, K. E.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, AU Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Meng, Z.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhong, J.; Zhou, Y.] Acad Sinica, Inst Phys, TW Taipei 11529, Taiwan. [Harpaz, S. Behar; Ben Ami, S.; Bressler, S.; Hershenhorn, A. D.; Kajomovitz, E.; Landsman, H.; Lifshitz, R.; Rozen, Y.; Tarem, S.; Tennenbaum-Katan, Y. D.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Technion, IL Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Brodet, E.; Etzion, E.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hod, N.; Kreisel, A.; Mahalalel, Y.; Munwes, Y.; Oren, Y.; Reinherz-Aronis, E.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.; Urkovsky, E.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 IL Tel Aviv, Israel. [Iliadis, D.; Kordas, K.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Fac Sci, Dept Phys, Div Nucl & Particle Phys, GR-54124 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Imori, M.; Isobe, T.; Kanaya, N.; Kaneda, M.; Kataoka, Y.; Kawamoto, T.; Kessoku, K.; Kobayashi, T.; Kubota, T.; Mashimo, T.; Masubuchi, T.; Matsumoto, H.; Matsunaga, H.; Nakamura, K.; Ninomiya, Y.; Nomoto, H.; Oda, S.; Okuyama, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamamura, T.; Yamazaki, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Bunkyo Ku, JP Tokyo 1130033, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Imori, M.; Isobe, T.; Kanaya, N.; Kaneda, M.; Kataoka, Y.; Kawamoto, T.; Kessoku, K.; Kobayashi, T.; Kubota, T.; Mashimo, T.; Masubuchi, T.; Matsumoto, H.; Matsunaga, H.; Nakamura, K.; Ninomiya, Y.; Nomoto, H.; Oda, S.; Okuyama, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamamura, T.; Yamazaki, T.] Dept Phys, Bunkyo Ku, JP Tokyo 1130033, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 1920397, Japan. [Jinnouchi, O.; Kanno, T.; Kuze, M.] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan. [Bailey, D. C.; Bain, T.; Beare, B.; Brelier, B.; Montero, S. Carron; Cheung, S. L.; Deviveiros, P. O.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Jankowski, E.; Joo, K. K.; Krieger, P.; Le Maner, C.; Martens, F. K.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Sandhu, P.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada. [Canepa, A.; Caron, B.; Chekulaev, S. V.; Fortin, D.; Losty, M. J.; Nugent, I. M.; Oram, C. J.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Taylor, W.] York Univ, Dept Phys & Astron, N York, ON M3J 1P3, Canada. [Hara, K.; Kim, S. H.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Inst Pure & Appl Sci, Tsukuba, JP Ibaraki 3058571, Japan. [Hamilton, S.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.] Tufts Univ, Ctr Sci & Technol, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Rodriguez, D.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Benedict, B. H.; Bold, T.; Ciobotaru, M. D.; Deng, J.; Dobson, M.; Eschrich, I. Gough; Grabowska-Bold, I.; Hawkins, D.; Lankford, A. J.; Okawa, H.; Porter, R.; Scannicchio, D. A.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Wheeler-Ellis, S. J.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Acharya, B. S.; Cobal, M.; De Lotto, B.; De Sanctis, U.; Del Papa, C.; Pinamonti, M.; Shaw, K.; Suruliz, K.] INFN Grp Collegato Udine, IT-33100 Udine, Italy. [Acharya, B. S.; Cobal, M.; Suruliz, K.] Abdus Salaam Int Ctr Theoret Phys, IT-34014 Trieste, Italy. [De Lotto, B.; De Sanctis, U.; Del Papa, C.; Pinamonti, M.; Shaw, K.] Univ Udine, Dipartimento Fis, IT-33100 Udine, Italy. [Benekos, N.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Khandanyan, H.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Belanger-Champagne, C.; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Hansen, C. J.] Uppsala Univ, Dept Phys & Astron, SE-75120 Uppsala, Sweden. [Amoros, G.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Ctr Mixto UVEG CSIC, Inst Fis Corpuscular IFIC, ES-46071 Valencia, Spain. [Amoros, G.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, Dept Fis Mol & Nucl, Dept Ing Elect, Bellaterra 08193, Spain. [Amoros, G.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Escobar, C.; Ferrer, A.; Fuster, J.; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Ros, E.; Salt, J.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Inst Microelect Barcelona IMB CNM CSIC, Bellaterra 08193, Spain. [Axen, D.; Gay, C.; Loh, C. W.; Mills, W. J.; Muir, A.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC V6T 1Z1, Canada. [Astbury, A.; Banerjee, Sw; Bansal, V.; Berghaus, F.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R; McPherson, R. A.; Plamondon, M.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC V8W 3P6, Canada. [Kimura, N.; Yorita, K.] Waseda Univ, WISE, Shinjuku Ku, Tokyo 1698555, Japan. [Alon, R.; Barak, L.; Duchovni, E.; Frank, T.; Gabizon, O.; Gross, E.; Klier, A.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Asfandiyarov, R.; Montoya, G. D. Carrillo; Hernandez, A. M. Castaneda; Castaneda-Miranda, E.; Chen, X.; Dos Anjos, A.; Fang, Y.; Fasching, D.; Ferguson, D.; Castillo, L. R. Flores; Gonzalez, S.; Gutzwiller, O.; Ji, H.; Cheong, A. Leung Fook; Li, H.; Ma, L. L.; Garcia, B. R. Mellado; Pan, Y. B.; Pataraia, S.; Morales, M. I. Pedraza; Peng, H.; Poveda, J.; Quayle, W. B.; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Zhu, Y.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Meyer, J.; Redelbach, A.; Stroehmer, R.; Trefzger, T.] Univ Wurzburg, Inst Phys, D-97074 Wurzburg, Germany. [Barisonzi, M.; Becks, K. H.; Boek, J.; Braun, H. M.; Dopke, J.; Drees, J.; Flick, T.; Gerlach, P.; Glitza, K. W.; Gorfine, G.; Grah, C.; Hamacher, K.; Harenberg, T.; Henss, T.; Hirschbuehl, D.; Imhaeuser, M.; Kalinin, S.; Kersten, S.; Kootz, A.; Kuhl, T.; Lenz, T.; Lenzen, G.; Maettig, P.; Mechtel, M.; Sandhoff, M.; Sandvoss, S.; Sartisohn, G.; Schultes, J.; Siebel, A.; Sturm, P.; Thadome, J.; Voss, T. T.; Wagner, W.; Wahlen, H.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C, D-42097 Wuppertal, Germany. [Adelman, J.; Atoian, G.; Auerbach, B.; Baker, O. K.; Almenar, C. Cuenca; Demers, S.; Garberson, F.; Golling, T.; Hsu, P. J.; Kaplan, B.; Lee, L.; Lockwitz, S.; Loginov, A.; Martin, A. J.; Schmidt, M. P.; Sherman, D.; Thioye, M.; Tipton, P.; Wall, R.; Zeller, M.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Grabski, V.; Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Biscarat, C.; Cogneras, E.; Rahal, G.] CNRS IN2P3, Ctr Calcul, F-69622 Villeurbanne, France. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hermann Herder Str 3, D-79104 Freiburg Ibr, Germany. 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